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Emerging Functionality in Transition-Metal Compounds Driven by Spatial Confinement and Broken Symmetry

This research project investigates the emerging functionality in transition-metal-compounds (TMCs) driven by spatial confinement and broken symmetry. It combines advanced growth capabilities with cutting-edge characterization and first principles theory to probe and control the properties of TMC interfaces, including the utilization and development of state-of-the-art atomically resolved electron microscopy and spectroscopy to determine the structure, composition, and bonding at TMC interfaces. The proposed research will focus on four challenging areas: 1) manipulate interfaces to design new material phases such as magnetic metals with unique polar structure (net dipole) to achieve multiple functionality; 2) explore electronic mismatch or screening at interfaces of insulating/poor metal TMCs to produce novel electronic and magnetic properties; 3) elucidate and exploit the role of defects, both point and extended, on the functionality of interfaces; 4) develop advanced electron microscopy/spectroscopy techniques to explore temperature dependent phase transitions and couple these structural tools with new nonlinear optical probes of the electronic structure. The research team aims to close the materials-by-design loop of make, measure, model, and modify. The program promises to enhance our ability to engineer the desired physical properties at interfaces, superlattices (periodic arrays of films of different compounds), and heterostructures of TMCs.

36 MATERIALS SCIENCE↗

On the termination of the closed field line region of the magnetotail

Experimental models and global computer simulations are used to study the field structure and location of the site where the closed plasma sheet terminates. The site - also called the 'distant neutral line' - is described with references to several solar-wind parameters that can change its characteristic properties. A laboratory experiment is then conducted in which a flowing magnetized plasma beam interacts with a dipole field. High-latitude nightside reconnection is supported by the simulation results comparing the effects of northward and southward interplanetary fields. The results support the models by Dungey (1961, 1963) that predict high-latitude nightside reconnection and an open magnetosphere. A significant finding is that a magnetic neutral line at the closed-field line region is not a necessary component of the region.

Birn, J.↗

A NICER View of PSR J0030+0451: Evidence for a Global-Scale Multipolar Magnetic Field

Recent modeling of Neutron Star Interior Composition Explorer observations of thermal X-ray pulsations from the surface of the isolated millisecond pulsar PSRJ0030+0451 suggests that the hot emitting regions on the pulsar’s surface are far from antipodal, which is at odds with the classical assumption that the magnetic field in the pulsar magnetosphere is predominantly that of a centered dipole. Here, we review these results and examine previous attempts to constrain the magnetospheric configuration of PSRJ0030+0451. To the best of our knowledge, there is in fact no direct observational evidence that PSRJ0030+0451’s magnetic field is a centered dipole. Developing models of physically motivated, non-canonical magnetic field configurations and the currents that they can support poses a challenging task. However, such models may have profound implications for many aspects of pulsar research, including pulsar braking, estimates of birth velocities, and interpretations of multi-wavelength magnetospheric emission.

A V Bilous↗

Statistical Theory of the Ideal MHD Geodynamo

A statistical theory of geodynamo action is developed, using a mathematical model of the geodynamo as a rotating outer core containing an ideal (i.e., no dissipation), incompressible, turbulent, convecting magnetofluid. On the concentric inner and outer spherical bounding surfaces the normal components of the velocity, magnetic field, vorticity and electric current are zero, as is the temperature fluctuation. This allows the use of a set of Galerkin expansion functions that are common to both velocity and magnetic field, as well as vorticity, current and the temperature fluctuation. The resulting dynamical system, based on the Boussinesq form of the magnetohydrodynamic (MHD) equations, represents MHD turbulence in a spherical domain. These basic equations (minus the temperature equation) and boundary conditions have been used previously in numerical simulations of forced, decaying MHD turbulence inside a sphere [1,2]. Here, the ideal case is studied through statistical analysis and leads to a prediction that an ideal coherent structure will be found in the form of a large-scale quasistationary magnetic field that results from broken ergodicity, an effect that has been previously studied both analytically and numerically for homogeneous MHD turbulence [3,4]. The axial dipole component becomes prominent when there is a relatively large magnetic helicity (proportional to the global correlation of magnetic vector potential and magnetic field) and a stationary, nonzero cross helicity (proportional to the global correlation of velocity and magnetic field). The expected angle of the dipole moment vector with respect to the rotation axis is found to decrease to a minimum as the average cross helicity increases for a fixed value of magnetic helicity and then to increase again when average cross helicity approaches its maximum possible value. Only a relatively small value of cross helicity is needed to produce a dipole moment vector that is aligned at approx.10deg with the rotation axis.

Shebalin, J. V.↗

Experimental study of the persistent current in RHIC superconducting dipole

The first goal [1] of this study is to reduce the high order magnetic component (mostly sextupole component) generated by persistent current in RHIC superconducting dipoles [2]. For Beam Energy Scan Phase II (BES-II) [3,4], reduction of lattice non-linearity is desirable for better beam control and beam lifetime. The sextupole component from RHIC dipole persistent current was too strong to be compensated at low operating current. The store length demonstrated in 2010 low energy operation at 3.85 GeV [5] was 10 minutes partially due to the lattice non -linearity. The measurement and compensation of lattice non-linearity were very difficult with such a short lifetime.

43 PARTICLE ACCELERATORS↗

Optical-Frequency Magnetic Polarizability in a Layered Semiconductor

The optical response of crystals is most commonly attributed to electric dipole interactions between light and matter. Although metamaterials support “artificial” magnetic resonances supported by mesoscale structuring, there are no naturally occurring materials known to exhibit a nonzero optical-frequency magnetic polarizability. Here, we experimentally demonstrate and quantify a naturally occurring nonzero magnetic polarizability in a layered semiconductor system: two-dimensional (Ruddlesden-Popper phase) hybrid organic-inorganic perovskites. These results demonstrate the only known material with an optical-frequency permeability that differs appreciably from vacuum, informing future efforts to find, synthesize, or exploit atomic-scale optical magnetism for novel optical phenomena such as negative index of refraction and electromagnetic cloaking.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Static electric and magnetic multipole susceptibilities for Dirac one-electron atoms in the ground state

We present tabulated data for several families of static electric and magnetic multipole susceptibilities for hydrogenic atoms with nuclear charge numbers from the range 1⩽Z⩽137. Atomic nuclei are assumed to be point-like and spinless. The susceptibilities considered include the multipole electric polarizabilities α{sub EL→EL} and magnetizabilities (magnetic susceptibilities) χ{sub ML→ML} with 1⩽L⩽4 (i.e., the dipole, quadrupole, octupole and hexadecapole ones), the electric-to-magnetic cross-susceptibilities α{sub EL→M(L−1)} with 2⩽L⩽5 and α{sub EL→M(L+1)} with 1⩽L⩽4, the magnetic-to-electric cross-susceptibilities χ{sub ML→E(L−1)} with 2⩽L⩽5 and χ{sub ML→E(L+1)} with 1⩽L⩽4 (it holds that χ{sub ML→E(L∓1)}=α{sub E(L∓1)→ML}), and the electric-to-toroidal-magnetic cross-susceptibilities α{sub EL→TL} with 1⩽L⩽4. Numerical values are computed from general exact analytical formulas, derived by us elsewhere within the framework of the Dirac relativistic quantum mechanics, and involving generalized hypergeometric functions {sub 3}F{sub 2} of the unit argument.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Controlling beam trajectory and transport in a tapered helical undulator

In this paper we present a detailed discussion of the helical undulator system developed for high extraction efficiency experiments in the tapered-enhanced stimulated superradiant amplification regime. The design is based on permanent magnet technology and comprises two Halbach arrays orthogonally oriented and shifted by 90° with respect to each other. When used in low energy beamlines for THz generation, the electron beam trajectory and transport are particularly sensitive to the undulator off-axis fields so that it becomes important to complement on-axis field measurements with analysis and tuning of the higher-order field components. Here we describe how the pulsed wire measurement technique can be effectively used to retrieve on- and off-axis magnetic field characteristics of the undulator. A simple two-dipole model is developed to guide the final adjustments to the permanent magnet positions along the array to tune the quadrupole and sextupole components of the field.

free-electron lasers↗

Electron Cloud Measurements in Fermilab Booster

Fermilab Booster synchrotron requires an intensity upgrade from 4.5x1012 to 6.5x1012 protons per pulse as a part of Fermilabs Proton Improvement Plan-II (PIP-II). One of the factors which may limit the high-intensity performance is the fast transverse instabilities caused by electron cloud effects. According to the experience in the Recycler, the electron cloud gradually builds up over multiple turns in the combined function magnets and can reach final intensities orders of magnitude greater than in a pure dipole. Since the Booster synchrotron also incorporates combined function magnets, it is essential to discover any existence of an electron cloud. And if it does, its effects on the PIP-II era Booster and its mitigating techniques. As the first step, the presence or absence of the electron cloud was investigated using the clearing bunch technique. This paper presents experimental details and observations of the bunch-by-bunch tune shifts of beams with various bunch train structures at low and high intensities and simulation results conducted using PyECLOUD.

43 PARTICLE ACCELERATORS↗

Electron Cloud Measurements in Fermilab Booster

Fermilab Booster synchrotron requires an intensity upgrade from 4.5x1012 to 6.5x1012 protons per pulse as a part of Fermilab's Proton Improvement Plan-II (PIP-II). One of the factors which may limit the high-intensity performance is the fast transverse instabilities caused by electron cloud effects. According to the experience in the Recycler, the electron cloud gradually builds up over multiple turns inside the combined function magnets and can reach final intensities orders of magnitude greater than in a pure dipole. Since the Booster synchrotron also incorporates combined function magnets, it is important to measure the presence of electron cloud. The presence or apparent absence of the electron cloud was investigated using two different methods: measuring bunch-by-bunch tune shift by changing the bunch train structure at different intensities and propagating a microwave carrier signal through the beampipe and analyzing the phase modulation of the signal. This paper presents the results of the two methods and corresponding simulation results conducted using PyECLOUD software.

43 PARTICLE ACCELERATORS↗

Improved stellarator permanent magnet designs through combined discrete and continuous optimizations

A common optimization problem in the areas of magnetized plasmas and fusion energy is the design of magnets to produce a given three-dimensional magnetic field distribution to high precision. When designing arrays of permanent magnets for stellarator plasma confinement, such problems have tens of thousands of degrees of freedom whose solutions, for practical reasons, should be constrained to discrete spaces. We perform a direct comparison between two algorithms that have been developed previously for this purpose, and demonstrate that composite procedures that apply both algorithms in sequence can produce substantially improved results. One approach uses a continuous, quasi-Newton procedure to optimize the dipole moments of a set of magnets and then projects the solution onto a discrete space. The second uses an inherently discrete greedy optimization procedure that has been enhanced and generalized for this work. Further, the approaches are both applied to design arrays cubic rare-Earth permanent magnets to confine a quasi-axisymmetric plasma with a magnetic field on axis of 0.5 T. The first approach tends to find solutions with higher field accuracy, whereas the second can find solutions with substantially (up to 30%) fewer magnets. When the approaches are combined, they can obtain solutions with magnet quantities comparable to the second approach while matching the field accuracy of the first.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

The magnetic field of Neptune

The Voyager 2 observations obtained during the Neptune encounter are used to develop a spherical harmonic model of the planetary magnetic field of Neptune. The model yields a dipole of magnitude 0.14 G R(N) exp 3, tilted by 47 deg toward 72 deg west longitude. Neptune's quadrupole is equal to or exceeding in magnitude the surface dipole field; the octupole is also very large, although less well constrained. The characteristics of the Neptune's magnetic field are illustrated using contour maps of the field on the planet's surface.

Connerney, J. E. P.↗

Thomson scattering in magnetic fields

The equation of transfer in Thomson scattering atmospheres with magnetic fields is solved using Monte Carlo methods. Two cases, a plane parallel atmosphere with a magnetic field perpendicular to the atmosphere, and a dipole star, are investigated. The wavelength dependence of polarization from plane-parallel atmosphere is qualitatively similar to that observed in the magnetic white dwarf Grw+70 deg 8247, and the field strength determined by the calculation, 320 MG, is quantitatively similar to that determined from the line spectrum. The dipole model does not resemble the data as well as the single plane-parallel atmosphere.

Whitney, Barbara↗

Saturn's ring current and inner magnetosphere

The Voyager 1 magnetic field observations at Saturn are shown in a graph. The departure of the oberved magnetic field from the field of a dipole is considered. The observed field magnitude is appreciable less than that of the model dipole at small radial distances and greater than the model dipole in the more distant magnetosphere. These characteristics can be understood by introducing a model current system similar to a system originally applied to observations of the Jovian magnetic disk. Saturn's ring current has important implications for charged-particle motion in Saturn's magnetosphere, particularly the absorption of trapped radiation by its many satellites and rings. The absorption signature observed by the Voyager 1 cosmic ray experiment near the orbital position of Rhea illustrates well the effects of Saturn's ring current on charged particle trajectories.

Connerney, J. E. P.↗

The magnetic field of planets

The strength of the dipole fields H sub Oi of the various inspected planets are connected by simple scaling law, involving observable angular velocity omega, planetary radia R sub p velocity omega and amplitude alpha of planetary precession, and radia R sub c, densities RHO sub c, conductivities sigma sub c of their liquid cores according to the contemporary models of planetary inner structure. The Lunar paleofield of 1G, its decay to zero is also explained in the frame of precession-dynamo model, evolution of the Earth-Moon system and primeval satellites in its suggested by Runcorn.

Dolginov, S. S.↗

Elementary Theoretical Forms for the Spatial Power Spectrum of Earth's Crustal Magnetic Field

The magnetic field produced by magnetization in Earth's crust and lithosphere can be distinguished from the field produced by electric currents in Earth's core because the spatial magnetic power spectrum of the crustal field differs from that of the core field. Theoretical forms for the spectrum of the crustal field are derived by treating each magnetic domain in the crust as the point source of a dipole field. The geologic null-hypothesis that such moments are uncorrelated is used to obtain the magnetic spectrum expected from a randomly magnetized, or unstructured, spherical crust of negligible thickness. This simplest spectral form is modified to allow for uniform crustal thickness, ellipsoidality, and the polarization of domains by an periodically reversing, geocentric axial dipole field from Earth's core. Such spectra are intended to describe the background crustal field. Magnetic anomalies due to correlated magnetization within coherent geologic structures may well be superimposed upon this background; yet representing each such anomaly with a single point dipole may lead to similar spectral forms. Results from attempts to fit these forms to observational spectra, determined via spherical harmonic analysis of MAGSAT data, are summarized in terms of amplitude, source depth, and misfit. Each theoretical spectrum reduces to a source factor multiplied by the usual exponential function of spherical harmonic degree n due to geometric attenuation with attitude above the source layer. The source factors always vary with n and are approximately proportional to n(exp 3) for degrees 12 through 120. The theoretical spectra are therefore not directly proportional to an exponential function of spherical harmonic degree n. There is no radius at which these spectra are flat, level, or otherwise independent of n.

Voorhies, C.↗

Dynamics of the Magnetic Moment of an Anisotropic Nanoparticle and a Plane Lattice in an Alternating Field

Dynamic regimes of the magnetic moment of a nanoparticle with an uniaxial or cubic anisotropy are studied. Regular oscillations with different attractor shapes and periods and regimes of chaotic and quasi-periodical dynamics are revealed. The dynamic bistability states are discovered; the transitions between the oscillation regimes belonging to bistability are obtained by means of the pulsed change in the alternating field amplitude. It has been shown that the 90°-remagnatization of the nanoparticle is caused by the alternating field action. The nanoparticle lattice parameters at which the dipole interaction effect on the oscillation regimes of magnetic momenta can be neglected are revealed.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Chandra X-Ray Observatory's Radiation Environment and the AP-8/AE-8 Model

The Chandra X-ray Observatory (CXO) was launched on July 23, 1999 and reached its final orbit on August 7, 1999. The CXO is in a highly elliptical orbit, approximately 140,000 km x 10,000 km, and has a period of roughly 63.5 hours (approx. 2.6 days). It transits the Earth's Van Allen belts once per orbit during which no science observations can be performed due to the high radiation environment. The Chandra X-ray Observatory Center (CXC) currently uses the National Space Science Data Center's "near Earth" AP-8/AE-8 radiation belt model to predict the start and end times of passage through the radiation belts. However, our scheduling software only uses a simple dipole model of the Earth's magnetic field. The resulting B, L magnet coordinates, do not always give sufficiently accurate predictions of the start and end times of transit of the Van Allen belts. We show this by comparing to the data from Chandra's on-board radiation monitor, the EPHIN (Electron, Proton, Helium Instrument particle detector) instrument. We present evidence that demonstrates this mis- of the radiation belts as well as data that also demonstrate the significant variability of one radiation belt transit to the next as experienced by the CXO. We present an explanation for why the dipole implementation of the AP-8/AE-8 gives inaccurate results. We are also investigating use of the Magnetospheric Specification and Forecast Model (MSM) - a model that also accounts for radiation belt variability and geometry.

Virani, S. N.↗