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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,135 records · Page 63
All sourcesNASA NTRSDOE OSTI
NASA NTRS1986

Real-time measurement of ice growth during simulated and natural icing conditions using ultrasonic pulse-echo techniques

Results of tests to measure ice accretion in real-time using ultrasonic pulse-echo techniques are presented. Tests conducted on a 10.2 cm diameter cylinder exposed to simulated icing conditions in the NASA Lewis Icing Research Tunnel and on an 11.4 cm diameter cylinder exposed to natural icing conditions in flight are described. An accuracy of + or - 0.5 mm is achieved for real-time ice thickness measurements. Ice accretion rate is determined by differentiating ice thickness with respect to time. Icing rates measured during simulated and natural icing conditions are compared and related to icing cloud parameters. The ultrasonic signal characteristics are used to detect the presence of surface water on the accreting ice shape and thus to distinguish between dry ice growth and wet growth. The surface roughness of the accreted ice is shown to be related to the width of the echo signal received from the ice surface.

Hansman, R. J., Jr.↗
NASA NTRS2000

Optical Measurements of Axial and Tangential Steady-State Blade Deflections Obtained Simultaneously

Case-mounted fiber-optic sensors have been used by aircraft engine manufacturers mainly to monitor blade vibration in fans and compressors. The simplest probe arrangement is a spot probe where, typically, a center fiber transmits laser light, and the outer fibers collect the reflected light from the blade tips and transmit it to a photodetector. Because the spot of incident light is fixed in space, whereas the blade deflects dynamically, the reflected light will originate from slightly different portions of the blade tip under different operating conditions. Unless corrections are developed to compensate for this effect, some error in vibratory tangential amplitude will occur. For monitoring vibrations, this error is usually not critical. However, when steady-state blade deflections are being measured, it is very important to fix the spot on the blade tip at a particular location because the operating speed blade deflections are evaluated against a low-speed reference run. The change in speed usually implies a significant change in the blade orientation and possibly its shape brought about by the aerodynamic and centrifugal loading. It is most convenient to select the blade s leading and trailing edges as the fixed points for which deflections will be evaluated. To capture the blade edges at various speeds, the light probe must be movable. This was achieved by mounting the probe in an eccentric hole in a bushing that fit the fan case in the region that overlapped the path of the blade edge. The probe was actuated to search for a blade edge while all the blades were viewed on an oscilloscope. The blade edge was considered to be captured when a pulse associated with a particular blade was significantly reduced in magnitude but was clearly distinguishable from the background noise level. By tracing the axial position of either blade edge, one could extend the deflection measurement to two dimensions: axial and tangential. These blade deflection measurements were obtained during a wind tunnel test of a fan prototype.

Kurkov, Anatole P.↗
DOE OSTI2024

Ultrafast laser triggered electron emission from ultrananocrystalline diamond pyramid tip cathode

Nitrogen-incorporated ultrananocrystalline diamond [(N)UNCD] pyramid tip cathode has been considered as a next-generation high peak current electron source for dielectric laser accelerators as well as other high peak current particle accelerator applications. In this work, we study non-linear photoemission from an (N)UNCD pyramid tip cathode using an ultrafast laser with the pulse length of 150 fs with the central wavelength of 800 nm in the peak intensity range of 10 9 –10 10 W/cm 2 . We demonstrated that as the incident laser intensity increases, the current emitted from the nano-tip first increases as a power function with an exponent of about 5 and then starts to roll over to an exponent of 3. This roll over is attributed to the Coulomb interaction between electrons emitted from the tip also known as the space charge. We also measured the photoemission electron energy spectra that show electrons with energies as high as ~10 eV. Based on the shape of the electron energy spectra, we conclude that the high-energy electrons are thermally emitted electrons due to ultrafast laser heating at the tip of the (N)UNCD pyramid tip cathode.

43 PARTICLE ACCELERATORS↗
NASA NTRS2001

Dynamic Finite Element Predictions for Mars Sample Return Cellular Impact Test #4

The nonlinear, transient dynamic finite element code, MSC.Dytran, was used to simulate an impact test of an energy absorbing Earth Entry Vehicle (EEV) that will impact without a parachute. EEVOs are designed to return materials from asteroids, comets, or planets for laboratory analysis on Earth. The EEV concept uses an energy absorbing cellular structure designed to contain and limit the acceleration of space exploration samples during Earth impact. The spherical shaped cellular structure is composed of solid hexagonal and pentagonal foam-filled cells with hybrid graphite-epoxy/Kevlar cell walls. Space samples fit inside a smaller sphere at the center of the EEVOs cellular structure. Pre-test analytical predictions were compared with the test results from a bungee accelerator. The model used to represent the foam and the proper failure criteria for the cell walls were critical in predicting the impact loads of the cellular structure. It was determined that a FOAM1 model for the foam and a 20% failure strain criteria for the cell walls gave an accurate prediction of the acceleration pulse for cellular impact.

Fasanella, Edwin L.↗
DOE OSTI2021

2D monochromatic x-ray imaging for beam monitoring of an x-ray free electron laser and a high-power femtosecond laser

Single-shot simultaneous beam monitoring of an x-ray free electron laser (XFEL) and a high-power femtosecond laser is demonstrated using 2D monochromatic Kα imaging. In a pump-probe experiment carried out at the Matter in Extreme Conditions end-station of the Linac Coherent Light Source, a thin solid titanium foil irradiated by a 25-TW relativistic intensity laser for fast electron isochoric heating was probed by a 7.0 keV XFEL beam for x-ray Thomson scattering measurements. Using a spherical crystal imager (SCI), the spatial overlap of the beams was examined by measuring 4.5 keV titanium Kα x rays produced by laseraccelerated fast electrons and the x-ray beam. Changes in XFEL-induced Kα emission patterns were observed down to a ~20×40 μm2 rectangular shape as the beam was focused. Laser-only and two-beam shots reveal that large spatial offsets of laser-induced Kα spots in a horizontal direction is attributed to imprecise target positioning rather than shot-to-shot laser pointing variations. As a consequence, successful beam overlapping was observed on ~58% of all two-beam shots for 10 μm thick samples. The Kα measurements also show a linear relationship between total Kα yields and integrated x-ray scattering signals. Monochromatic xray imaging with SCI could be used as an on-shot beam pointing diagnostic in XFEL-laser or multiple short-pulse laser experiments.

47 OTHER INSTRUMENTATION↗
DOE OSTI2024

Harnessing complexity: Nonlinear optical phenomena in L-shapes, nanocrescents, and split-ring resonators

Here, we conduct systematic studies of the optical characteristics of plasmonic nanoparticles that exhibit C 2v symmetry. In particular, we analyze three distinct geometric configurations: an L-type shape, a crescent, and a split-ring resonator shaped like the Greek letter π. Optical properties are examined using the finite-difference time-domain method. It is demonstrated that all three shapes exhibit two prominent plasmon modes associated with the two axes of symmetry. This is in addition to a wide range of resonances observed at high frequencies corresponding to quadrupole modes and peaks due to sharp corners. Next, to facilitate nonlinear analysis, we employ a semiclassical hydrodynamic model, where the electron pressure term is explicitly accounted for. This model goes beyond the standard Drude description and enables capturing nonlocal and nonlinear effects. Employing this model enables us to rigorously examine the second-order angular resolved nonlinear optical response of these nanoparticles in each of the three configurations. Two pumping regimes are considered, namely, continuous wave (CW) and pulsed excitations. For CW pumping, we explore the properties of the second harmonic generation (SHG). Polarization and angle-resolved SHG spectra are obtained, revealing strong dependence on the nanoparticle geometry and incident wave polarization. The C 2v symmetry is shown to play a key role in determining the polarization states and selection rules of the SHG signal. For pulsed excitations, we discuss the phenomenon of broadband terahertz (THz) generation induced by the difference-frequency generation . It is shown that the THz emission spectra exhibit unique features attributed to the plasmonic resonances and symmetry of the nanoparticles. The polarization of the generated THz waves is also examined, revealing interesting patterns tied to the nanoparticle geometry. To gain deeper insight, we propose an analytical theory that agrees very well with the numerical experiments. The theory shows that the physical origin of the THz radiation is the mixing of various frequency components of the fundamental pulse by the second-order nonlinear susceptibility. An expression for the far-field THz intensity is derived in terms of the incident pulse parameters and the nonlinear response tensor of the nanoparticle. The results presented in this work offer new insights into the linear and nonlinear optical properties of nanoparticles with C 2v symmetry. The demonstrated strong SHG response and efficient broadband THz generation hold great promise for applications in nonlinear spectroscopy, nanophotonics, and optoelectronics. The proposed theoretical framework also provides a valuable tool for understanding and predicting the nonlinear behavior of other related nanostructures.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

NO PLIF flow visualization and time-resolved temperature distributions in laser induced breakdown plumes

NO planar laser induced fluorescence (PLIF) is used to obtain images of laser-induced breakdown plasma plumes in NO-seeded nitrogen and dry air at near atmospheric pressure. Single-shot PLIF-images show that the plume development 5–50 μs after the breakdown pulse is fairly reproducible shot-to-shot, although the plume becomes increasingly stochastic on longer timescales, 100–500 μs. The stochastic behavior of the plume is quantified using probability distributions of the loci of the plume boundary. Analysis of the single-shot images indicates that the mixing of the plume with ambient gas on sub-ms time scale is insignificant. The induced flow velocity in the plume is fairly low, up to 30 m s –1 , suggesting that laser breakdowns are ineffective for mixing enhancement in high speed flows. The ensemble-averaged PLIF images indicate the evolution of the plume from an initially elongated shape to near-spherical to toroidal shape, with a subsequent radial expansion and formation of an axial jet in the center. Temperature distributions in the plume in air are obtained from the NO PLIF images, using two rotational transitions in the NO(X, v' = 0 → A, v'' = 0) band, J'' = 6.5 and 12.5 of the Q R 12 + Q 2 branch. The results indicate that the temperature in the plume remains high, above 1000 K, for approximately 100 μs, after which it decays gradually, to below 500 K at 500 μs. The residual NO fraction in the plume is ~0.1%, indicating that repetitive laser-assisted ignition may result in significant NO-generation. Furthermore, these measured temperature and velocity distributions can be used for detailed validation of kinetic models of laser-induced breakdown and assessment of their predictive capability.

42 ENGINEERING↗
DOE OSTI2022

Suppression of toroidal Alfvén eigenmodes by the electron cyclotron current drive in KSTAR plasmas

Advanced operation scenarios such as high poloidal beta ( β P ) or high q min are promising concepts to achieve the steady-state high-performance fusion plasmas. However, those scenarios are prone to substantial Alfvénic activity, causing fast-ion transport and losses. Recent experiments with the advanced operation scenario on KSTAR tokamak have shown that the electron cyclotron current drive (ECCD) is able to mitigate and suppress the beam-ion driven toroidal Alfvén eigenmodes (TAEs) for over several tens of global energy confinement time. Co-current directional intermediate off-axis ECCD lowers the central safety factor slightly and tilts the central q -profile shape so that the continuum damping in the core region increases. Besides, the rise of central plasma pressure and increased thermal-ion Landau damping contribute to TAE stabilization. While the TAEs are suppressed, neutron emission rate and total stored energy increase by approximately 45% and 25%, respectively. Fast-ion transport estimated by TRANSP calculations approaches the classical level during the TAE suppression period. Substantial reduction in fast-ion loss and neutron deficit is also observed. Subsequently, enhancement of fast-ion confinement by suppressing the TAEs leads to an increase of non-inductive current fraction and will benefit the sustainment of the long-pulse high-performance discharges.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1975

Asteroid observations and planetary atmospheres analysis

Photoelectric observations of Eros and 30 other asteroids providing information on their surface characteristics, shape, and rotation axes are reported. Photographs of 18 asteroids and 4 comets yielding accurate position information on various dates were obtained. Photometric observations were made of the Saturn satellite lapetus, and electronographic images of the Uranus and Neptune satellites were obtained experimentally with a Spectracon tube to assess photometry by that method. Planetary patrol photographs of Venus and deconvolved area scans of Uranus were taken. UBV photometry of the Galilean satellites for the period 1973-1974 was completely analyzed and accepted for publication. An improved magnitude and color index for Minas were derived from 1974 area scans. A special photomultiplier tube with a suppressor grid was incorporated into a pulse-counting photometer with special added circuitry for carrying out the observations concerning the constancy of solar system dimensions over cosmic time.

Baum, W. A.↗
DOE OSTI2025

Analysis methodology of coherent oscillations in time- and angle-resolved photoemission spectroscopy

Oscillatory signals from coherently excited phonons are regularly observed in ultrafast pump–probe experiments on condensed matter samples. Electron–phonon coupling implies that coherent phonons also modulate the electronic band structure. These oscillations can be probed with energy and momentum resolution using time- and angle-resolved photoemission spectroscopy (trARPES), which reveals the orbital dependence of the electron–phonon coupling for a specific phonon mode. However, a comprehensive analysis remains challenging when multiple coherent phonon modes couple to multiple electronic bands. Complex spectral line shapes due to strong correlations in quantum materials add to this challenge. In this work, we examine how the frequency domain representation of trARPES data facilitates a quantitative analysis of coherent oscillations of the electronic bands. Here, we investigate the frequency domain representation of the photoemission intensity and the first moment of the energy distribution curves. Both quantities provide complementary information and are able to distinguish oscillations of binding energy, linewidth, and intensity. We analyze a representative trARPES dataset of the transition metal dichalcogenide WTe 2 and construct composite spectra, which intuitively illustrate how much each electronic band is affected by a specific phonon mode. We also show how a linearly chirped probe pulse can generate extrinsic artifacts that are distinct from the intrinsic coherent phonon signal.

47 OTHER INSTRUMENTATION↗
DOE OSTI2023

Field-induced spin level crossings within a quasi-$XY$ antiferromagnetic state in $Ba$ 2 $FeSi$ 2 $O$ 7

Here, we present a high-field study of the strongly anisotropic easy-plane square lattice $S$ = 2 quantum magnet $Ba$ 2 $FeSi$ 2 $O$ 7 . This compound is a rare high-spin antiferromagnetic system with very strong easy-plane anisotropy, such that the interplay between spin level crossings and antiferromagnetic order can be studied. We observe a magnetic field-induced spin level crossing occurring within an ordered state. This spin level crossing appears to preserve the magnetic symmetry while producing a nonmonotonic dependence of the order parameter magnitude. The resulting temperature–magnetic field phase diagram exhibits two dome-shaped regions of magnetic order overlapping around 30 T. The ground state of the lower-field dome is predominantly a linear combination of |$S^z$ = 0$\rangle$ and |$S^z$ = 1$\rangle$ states, while the ground state of the higher-field dome can be approximated by a linear combination of |$S^z$ = 1$\rangle$ and |$S^z$ = 2$\rangle$ states. At 30 T, where the spin levels cross, the magnetization exhibits a slanted plateau, the magnetocaloric effect shows a broad hump, and the electric polarization shows a weak slope change. We determined the detailed magnetic phase boundaries and the spin level crossings using measurements of magnetization, electric polarization, and the magnetocaloric effect in pulsed magnetic fields to 60 T. Furthermore, we calculate these properties using a mean-field theory based on direct products of SU(5) coherent states and find good agreement. Finally, we measure and calculate the magnetically induced electric polarization that reflects magnetic ordering and spin level crossings. This multiferroic behavior provides another avenue for detecting phase boundaries and symmetry changes.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS2001

Measuring Rocket Engine Temperatures with Hydrogen Raman Spectroscopy

Optically accessible, high pressure, hot fire test articles are available at NASA Marshall for use in development of advanced rocket engine propellant injectors. Single laser-pulse ultraviolet (UV) Raman spectroscopy has been used in the past in these devices for analysis of high pressure H2- and CH4-fueled combustion, but relies on an independent pressure measurement in order to provide temperature information. A variation of UV Raman (High Resolution Hydrogen Raman Spectroscopy) is under development and will allow temperature measurement without the need for an independent pressure measurement, useful for flows where local pressure may not be accurately known. The technique involves the use of a spectrometer with good spectral resolution, requiring a small entrance slit for the spectrometer. The H2 Raman spectrum, when created by a narrow linewidth laser source and obtained from a good spectral resolution spectrograph, has a spectral shape related to temperature. By best-fit matching an experimental spectrum to theoretical spectra at various temperatures, a temperature measurement is obtained. The spectral model accounts for collisional narrowing, collisional broadening, Doppler broadening, and collisional line shifting of each Raman line making up the H2 Stokes vibrational Q-branch spectrum. At pressures from atmospheric up to those associated with advanced preburner components (5500 psia), collisional broadening though present does not cause significant overlap of the Raman lines, allowing high resolution H2 Raman to be used for temperature measurements in plumes and in high pressure test articles. Experimental demonstrations of the technique are performed for rich H2-air flames at atmospheric pressure and for high pressure, 300 K H2-He mixtures. Spectrometer imaging quality is identified as being critical for successful implementation of technique.

Wehrmeyer, Joseph A.↗
DOE OSTI2026

Demonstration of tokamak vertical stability control based on non-inductive Faraday-effect polarimetry measurements

Long-pulse or steady-state fusion reactors are envisioned to control vertical stability based on non-inductive measurements, i.e. that do not rely on temporal change of magnetic field. For the first time, vertical stability control using non-inductive Faraday-effect polarimetry measurements has been demonstrated. The Radial Interferometer-Polarimeter system on DIII-D is capable of microsecond resolution and was used to absolutely determine the vertical position of the plasma magnetic axis Z 0 . A vertical stability controller was developed to robustly stabilize diverted plasmas using Faraday-based measurements. The system was able to stabilize against vertical displacement events with growth rates up to 350 s -1 in elongated and elliptical plasma shapes, and instabilities with even higher growth rates are likely to be controllable with further improvements to controller tuning. Tests show that the Faraday-based controller remains effective and is capable of recovering from loss of control even when the plasma vertical position is far from the region where the linear model used to calculate Z 0 is most valid. Faraday control has also been activated during plasma ramp-up, demonstrating the robustness of the technique to larger systematic diagnostic uncertainty at low electron density.

Faraday-effect polarimetry↗
NASA NTRS2006

Lunar Geodetic Opportunities with the Laser Altimeter on LRO

The Lunar Reconnaissance Orbiter (LRO) is to be launched at the end of 2008 and will carry 7 instruments, one of which is a laser altimeter (LOLA), and obtain observations of the Moon for a period of 1 year. The orbit will be near polar and approximately circular at 50 km altitude with monthly orbital adjustments to maintain the mean altitude. The LOLA instrument has a -10 cm single-shot accuracy, with 5 beams, and operates at 28 Hz. It provides 5 adjacent profiles, each approximately 12 to 15 meters apart with a swath of approximately 65 meters. The 5 beams are arranged in a cross-shaped pattern that provides simultaneous along and cross track altimetry and providing slopes in 2 orthogonal directions every 50 meters along track. In combination with the LRO tracking data LOLA will be used to improve the model of the lunar gravity by using the altimeter on both the lunar near-side and far-side as an additional tracking system to enable precise positioning of the LRO spacecraft at about the 50 meter level rms. The instrument is expected to provide full polar coverage at very high northern and southern latitudes with spatial resolutions of 25 meters or better. In addition to the range to the surface LOLA measures the surface roughness from the spreading of the laser pulse and also the reflectance of the surface at 1064 nm. These measurements in conjunction with the altimetry will assist in the selection of future landing sites for future robotic and human missions to the Moon.

Zuber, Maria T.↗
DOE OSTI2022

Discharge intermittency considerably changes ZnO spatial distribution in porous Zn anodes

Porous Zn anodes are ubiquitous in primary batteries and are under development for low-cost rechargeable batteries. Spatial distribution of ZnO discharge product is a critical factor in these, because it can passivate the active material. In rechargeable cells this is related to a major failure mechanism called shape change, in which ZnO is relocated to inactive locations. In this work we demonstrate rest steps during discharge of primary Zn anodes dramatically alter the placement of ZnO in the anode. In alkaline electrolyte, ZnO discharge product is typically modeled as precipitating close to Zn particles, forming a porous ZnO shell around the Zn core. Further, anodes discharged continuously at low-rate are compared to anodes similarly discharged intermittently, using in situ computed tomography from a synchrotron source. Zn–ZnO core-shell structures are produced during continuous discharge but are not found in cells discharged intermittently. Continuously discharged cells showed that ZnO was formed most strongly near the separator, in agreement with Zn anode battery models. In pulse-discharged cells, ZnO was more radially distributed and was in large formations not physically connected to Zn particles. Thus, discharge intermittency changes spatial distribution of ZnO in ways that are unpredicted by Zn anode models.

25 ENERGY STORAGE↗
NASA NTRS2005

Aerosol properties computed from aircraft-based observations during the ACE- Asia campaign: A case study of lidar ratio closure and aerosol radiative effects - 2

For a vertical profile with three distinct layers (marine boundary, pollution and dust), observed during the ACE-Asia campaign, we carried out a comparison between the modeled lidar ratio vertical profile and that obtained from collocated airborne NASA AATS-14 sunphotometer and shipborne Micro-Pulse Lidar (MPL) measurements. Vertically resolved lidar ratio was calculated from two size distribution vertical profiles - one obtained by inversion of sunphotometer-derived extinction spectra, and one measured in-situ - combined with the same refractive index model based on aerosol chemical composition. The aerosol model implies single scattering albedos of 0.78 - 0.81 and 0.93 - 0.96 at 0.523 microns (the wavelength of the lidar measurements), in the pollution and dust layers, respectively. The lidar ratios calculated from the two size distribution profiles have close values in the dust layer; they are however, significantly lower than the lidar ratios derived from combined lidar and sunphotometer measurements, most probably due to the use of a simple nonspherical model with a single particle shape in our calculations. In the pollution layer, the two size distribution profiles yield generally different lidar ratios. The retrieved size distributions yield a lidar ratio which is in better agreement with that derived from lidar/sunphotometer measurements in this layer, with still large differences at certain altitudes (the largest relative difference was 46%). We explain these differences by non-uniqueness of the result of the size distribution retrieval and lack of information on vertical variability of particle refractive index. Radiative transfer calculations for this profile showed significant atmospheric radiative forcing, which occurred mainly in the pollution layer. We demonstrate that if the extinction profile is known then information on the vertical structure of absorption and asymmetry parameter is not significant for estimating forcing at TOA and the surface, while it is of importance for estimating vertical profiles of radiative forcing and heating rates.

Kuzmanoski, Maja↗
NASA NTRS2016

Space Launch System Vibration Analysis Support

The ultimate goal for my efforts during this internship was to help prepare for the Space Launch System (SLS) integrated modal test (IMT) with Rodney Rocha. In 2018, the Structural Engineering Loads and Dynamics Team will have 10 days to perform the IMT on the SLS Integrated Launch Vehicle. After that 10 day period, we will have about two months to analyze the test data and determine whether the integrated vehicle modes/frequencies are adequate for launching the vehicle. Because of the time constraints, NASA must have newly developed post-test analysis methods proven well and with technical confidence before testing. NASA civil servants along with help from rotational interns are working with novel techniques developed and applied external to Johnson Space Center (JSC) to uncover issues in applying this technique to much larger scales than ever before. We intend to use modal decoupling methods to separate the entangled vibrations coming from the SLS and its support structure during the IMT. This new approach is still under development. The primary goal of my internship was to learn the basics of structural dynamics and physical vibrations. I was able to accomplish this by working on two experimental test set ups, the Simple Beam and TAURUS-T, and by doing some light analytical and post-processing work. Within the Simple Beam project, my role involves changing the data acquisition system, reconfiguration of the test set up, transducer calibration, data collection, data file recovery, and post-processing analysis. Within the TAURUS-T project, my duties included cataloging and removing the 30+ triaxial accelerometers, coordinating the removal of the structure from the current rolling cart to a sturdy billet for further testing, preparing the accelerometers for remounting, accurately calibrating, mounting, and mapping of all accelerometer channels, and some testing. Hammer and shaker tests will be performed to easily visualize mode shapes at low frequencies. Short analytical projects using MATLAB were also assigned to aid in research efforts. These included integration of acceleration data for comparison to measured displacement data. Laplace and Fourier transforms were also investigated to determine viability as a method of modal decoupling. In addition to these projects, I was also able contribute work that would benefit future interns and the division as a whole. I gave a short presentation and answered questions to aid in the recruitment of subsequent interns and co-ops for the division. I also assisted in revisions and additions to Intern/Co-Op Handbook to provide incoming employees with background information on the organization they are about to work for. I further developed tutorial on Pulse software, which was used for data acquisition for both experiments and will be helpful to interns and engineers that may be unfamiliar to the software. I gained a diverse range of experience throughout my internship. I was introduced to advanced dynamics and analytical techniques. This was through new experience with both hands on experimentation and analytical post processing methods. I was exposed to the benefits of interdepartmental collaboration and developed stronger skills in time management by coordinating two different tests at once. This internship provided an excellent opportunity to see how engineering theories applied to real life scenarios, and an introduction to how NASA/JSC solves technical problems.

Johnson, Katie↗
DOE OSTI2021

Electron thermalization and relaxation in laser-heated nickel by few-femtosecond core-level transient absorption spectroscopy

Direct measurements of photoexcited carrier dynamics in nickel are made using few-femtosecond extreme ultraviolet (XUV) transient absorption spectroscopy at the nickel M 2,3 edge. It is observed that the core-level absorption line shape of photoexcited nickel can be described by a Gaussian broadening (σ) and a red shift (ω s ) of the ground-state absorption spectrum. Theory predicts and the experimental results verify that after initial rapid carrier thermalization, the electron temperature increase (ΔT ) is linearly proportional to the Gaussian broadening factor σ, providing quantitative real-time tracking of the relaxation of the electron temperature. Measurements reveal an electron cooling time for 50 nm thick polycrystalline nickel films of 640 ± 80 fs. With hot thermalized carriers, the spectral red shift exhibits a power-law relationship with the change in electron temperature of ω s ∝ ΔT 1.5 . Rapid electron thermalization via carrier-carrier scattering accompanies and follows the nominal 4-fs photoexcitation pulse until the carriers reach a quasithermal equilibrium. Entwined with a <6 fs instrument response function, carrier thermalization times ranging from 34 fs to 13 fs are estimated from experimental data acquired at different pump fluences and it is observed that the electron thermalization time decreases with increasing pump fluence. Here, the study provides an initial example of measuring electron temperature and thermalization in metals in real time with XUV light, and it lays a foundation for further investigation of photoinduced phase transitions and carrier transport in metals with core-level absorption spectroscopy.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗