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At least 1,153 records · Page 64

Radiochemistry Results from IER-163 Comet Irradiation

A critical experiment was performed on the Comet assembly to provide nuclear data in a non-thermal neutron spectrum and to re-establish experimental capability relevant to the Stockpile Stewardship and Technical Nuclear Forensic programs. Irradiation foils were placed at specific locations in the Zeus all oralloy critical experiment to obtain fission ratios and activation products. After the irradiation was completed and a cooling down period of time had elapsed, passive gamma ray measurements were performed on all the foils and several of the foils were packaged and shipped to Los Alamos National Laboratory (LANL) for further radiochemical analysis. The results from the Los Alamos National Laboratory’s non-destructive and radiochemical analyses are presented. Monte Carlo simulations of the experiment are described and compared to the experimental results.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

LAFD: TA-16 HE Facility Familiarization Tour, OJT 55258

Los Alamos National Laboratory (LANL) will conduct familiarization tours for personnel of the Los Alamos County Fire Department (LAFD) at TA-16 high explosives (HE) facilities. These familiarization tours are official LANL business; the purpose of these tours is to orient LAFD firefighters to the facility so that they can respond efficiently and quickly to a variety of emergency situations. This orientation includes, among other topics, ingress and egress of the area and buildings, layout and organization of the facility, evacuation procedures and assembly points, and areas of concern within the various buildings at the facility. LAFD firefighters have the skills and abilities to perform firefighting operations and other emergency response tasks that cannot be provided by LANL personnel who have the required clearance. This handout provides details of the information, along with maps and diagrams, to be presented during the familiarization tours. The handout will be distributed to the trainees at the time of the tour. A corresponding checklist will also be used as guidance during the familiarization tours to ensure that all required information is presented to LAFD personnel.

99 GENERAL AND MISCELLANEOUS↗

LAFD: TA-55 General Facility Familiarization Tour, Course #55261

Los Alamos National Laboratory (LANL) will conduct familiarization tours for personnel of the Los Alamos County Fire Department (LAFD) at the TA-55 General Facility. These familiarization tours are official LANL business; the purpose of these tours is to orient LAFD firefighters to the facility so that they can respond efficiently and quickly to a variety of emergency situations. This orientation includes, among other topics, ingress and egress of the area and buildings, layout and organization of the facility, evacuation procedures and assembly points, and areas of concern within the various buildings at the facility. LAFD firefighters have the skills and abilities to perform firefighting operations and other emergency response tasks that cannot be provided by LANL personnel who have the required clearance level. This handout provides details of the information, along with maps and diagrams, to be presented during the familiarization tours. The handout will be distributed to the trainees at the time of the tour. A corresponding checklist will also be used as guidance during the familiarization tours to ensure that all required information is presented to LAFD personnel.

99 GENERAL AND MISCELLANEOUS↗

The ARGUS Solution Reactor and Molybdenum Production: A Summary Report Based on Open Literature

The (Aqueous Homogeneous Reactor) AHR was conceptualized at Los Alamos for work in advancing weapon design with initial experiments completed at Los Alamos National Laboratory (LANL) and Oak Ridge National Laboratory (ORNL) in the early 1940s and 1950s. The reactor design was discovered to be an efficient mean of production for medical radio isotopes (e.g. molybdenum-99 and other fission products) due to its streamlined process of extracting target radioactive sources from the fissile solution via a separation system. As the demand for medical radioisotopes has increased so has the need for a safe and low cost isotope source, the most commonly used of which is technetium-99m (99m Tc), daughter product from molybdenum decay. Studies indicate solution reactors pose a significantly lower hazard to the workers, public and environment, compared to other modern reactors (International Atomic Energy Agency 2008). The inherent safety and ability to selectively extract radionuclides from its fuel solution make AHRs particularly well suited for medical isotope production. This discussion narrows its focus to one of the longest running aqueous homogeneous reactor systems, ARGUS. A study of the conversion of ARGUS to a low-enriched uranyl (LEU) sulfate fuel solution was part of the Global Threat Reduction Initiative (GTRI) program. The goal of this paper is to provide a summary of the ARGUS reactor system based on open literature available.

07 ISOTOPE AND RADIATION SOURCES↗

Panel Session 2: Hot Topics in US DOE Environmental Management

The well-attended Panel Session was chaired by Martin Schneider. The four panelists did not provide presentations. Rather the session was a discussion focusing on pressing issues facing US DOE Environmental Management (EM) sites and how the program is moving forward. The session began by momentarily reflecting on a success: the three Tank Waste Treatment Facilities will soon be coming online. These three facilities will treat as much waste in two years as was treated in the past 30 years. That is a significant milestone in progress. Also, safety enhancements at WIPP are a big success. The panelists noted that there will be challenges with the victories of the startup of the Waste Treatment Facilities. Treating tank waste is the last EM mission and will help with the relationships with the stakeholders, regulators and Congress. One of the biggest challenges will be moving back to full operation mode. Although the operation will increase productivity of reducing/managing the tank waste, it will decrease life cycle cost and lessen years of cleanup. The challenge will be having people understand that EM will be operating 24/7 and that maintenance will be key in keeping the operations. EM will be working together with the regulators to show tangible progress that will be effective and efficient. By working together, they can find opportunities/technologies for streamlining and accelerating cleanup. Recent changes to the regulatory framework between DOE-EM Los Alamos Field Office and New Mexico Environmental Department have helped cleanup in Los Alamos. Every year EM and the agencies review progress and come to agreements on the next work priorities. At Savannah River Site, the Federal Facility Agreement among EM, South Carolina Department of Health and Environmental Control, and Environmental Protection Agency (EPA) has developed a small core team that work are shared by together in resolving issues that come up. The discussion moved on to how progress can be made by sharing lessons learned among the contractors. An example of how these learned lessons can be shared is that key representatives from projects across the EM sites participate in various forums to review/contribute to the work planned. Other opportunities can be by temporary assignments of DOE staff to gain experience and by monthly EM Headquarters report that provide the lessons learned across the EM sites. The panelists discussed how skyline changes are the best examples of tangible progress. Decontamination and Demolition (D and D) of structures are the easiest tangible progress that can be seen. Whereas tank waste cleanup is the hardest to see. Disposal of waste onsite versus offsite is another challenge, and timely discussions are necessary to get to the best value to the government.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Fission Product Yield Modeling and Evaluation

Although independent and cumulative fission product yields have been a part of evaluated libraries for decades, there have been few updates over the years. The fission product yield sub-library in the ENDF/B-VIII.0 library is still largely based on the evaluation of England and Rider from the mid-90’s, with only more recent updates to the energy dependence of 239 Pu below 2 MeV and fixes to isomeric states and missing fission products. Over the past several years, there have been a wealth of new measurements of independent and cumulative fission product yields, particularly those with short half-lives, and there have been significant improvements in the modeling of prompt and delayed fission observables. Here, we describe recent progress in the improvement of fission product yield calculations, using the BeoH code and the underlying Hauser Fesh-bach Fission Fragment Decay (HF 3 D) model, developed at Los Alamos National Laboratory. We will describe our recent calculations for consistent prompt and delayed fission observables for major and minor actinides, including new work investigating isomeric ratios. We will detail the ongoing evaluation process for energy-dependent fission product yields from thermal up to 20 MeV incident neutron energy and some validation work that has been performed for these new fission product yield calculations. Additionally, we will discuss future perspectives of this work, highlighting the need for additional data.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

First Event-by-Event Identification of Cherenkov Radiation from Sub-Mev Particles in Liquid Argon

This Letter reports the event-by-event observation of Cherenkov light from sub-MeV electrons in a high scintillation light-yield liquid argon detector by the coherent CAPTAIN-Mills (CCM) experiment. The CCM200 detector, located at Los Alamos National Laboratory, instruments seven tons (fiducial volume) of liquid argon with 200 eight-inch photomultiplier tubes, 80% of which are coated in a wavelength-shifting material and the remaining 20% are uncoated. In the prompt time region of an event, defined as - 6 ≤ t < 0 ns relative to the event start time t = 0 , the uncoated photomultiplier tubes are primarily sensitive to visible Cherenkov photons. Using gamma rays from a Na 22 source for production of sub-MeV electrons, we isolated prompt Cherenkov light with > 5 σ confidence and developed a selection to obtain a low-background electromagnetic sample. This is the first event-by-event observation of Cherenkov photons from sub-MeV electrons in a high-yield scintillator detector and represents a milestone in low-energy particle detector development.

Aguilar-Arevalo, A. A. [UNAM, Mexico]↗

Godiva IV Thermal Neutron Dosimetry Modeling and Variance Reduction

The transfer of the Godiva IV experiment from the Los Alamos Critical Experiments Facility (LACEF) to the National Critical Experiments Research Center (NCERC) introduced a vastly different experiment room return to the neutron flux. The contribution of the background to the burst neutron energy spectrum is significant in the thermal and epithermal neutron energies. Target materials may be placed in various locations in the Godiva room, or outside of the room, for thermal neutron activation. Modeling of this dosimetry problem in Monte Carlo N-Particle (MCNP) presented a novel challenge compared to previous Godiva IV glory hole irradiation simulations. An advanced dosimetry modeling framework for high efficiency calculations in locations far from the Godiva IV fission source was desired. The mesh-based weight windows and point detector advanced variance reduction techniques in MCNP were implemented and tested using adaptations of the critical experiment benchmark model of the Godiva IV problem. The models were validated against measured activations of Nickel, Indium, Scandium, and Cobalt foils at locations 2 meters from the Godiva IV core. Dosimetry measurements were performed in collaboration with Sandia National Laboratory. The weight windows and point detector variance reduction coupled method resulted in the highest problem efficiency.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Self-Consistent Relativistic Electron Scattering using the Sherlock Scattering Model for X-ray Diagnostics

We present on a new, self-consistent, arbitrary-temperature Romberg integration scheme for modeling electron scattering in materials in a LANL Lagrangian Shock Hydro (LSH) code. Electron beam-target interactions are fundamental to a wide range of scientific and technological applications. When high-energy electron beams hit their target, they may scatter, deposit energy, or ionize the source. These processes govern the behavior and outcomes in nanotechnology manufacturing, electron microscopy, and modern X-ray diagnostics. Simulating these interactions is essential for interpreting experimental results, predicting material responses, and designing efficient tools and experiments. At Los Alamos, this is done using a LSH code, which is a multi-dimension, multi-material, massively parallel, multi-physics code used to simulate applications from asteroid impacts to electron beam interactions. By effectively and efficiently modeling the way that electrons scatter from the beam we can bolster these simulations and more accurately predict experimental outcomes. The model currently implemented in the LSH of interest is based on work by Papp and does not self-consistently preserve momentum in the slightly relativistic regime; here we adopt a model proposed by Braams and Karney and implement a Romberg integration scheme to compute the diffusion tensor. In this paper we will provide background on the Braams-Karney diffusion tensor as well as the Romberg integration scheme we employed to numerically solve for it. We will show that our integration scheme is accurate in solving for the set of scalar potentials used to re-express the diffusion tensor in differential form, and in solving for the diffusion coefficients in the larger LSH code. By using this diffusion tensor rather than the existing Papp one, and numerically integrating it with a Romberg method, we produce much more accurate, self-consistent results.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Optimizing Simulation Fidelity in Direct-Drive Inertial Confinement Fusion with Cassio

Recently, the National Ignition Facility (NIF) demonstrated that inertial confinement fusion (ICF) is capable to achieve thermonuclear (TN) ignition in the laboratory, making it a crucial method on the path to replicate the Sun’s power production mechanism on Earth. However, the physics governing the high-energy density environments is very complex and remains a challenge to fully understand and model. For example, dopants in the TN fuel are important diagnostic tools to extract the thermodynamic conditions of the plasma. However, if their concentration is chosen too high, they can significantly degrade the performance of an ICF capsule. In this study, we use the Los Alamos National Laboratory radiation-hydrodynamics code Cassio to model ICF implosions of capsules which contain deuterium fuel with high-Z dopants like Krypton and Argon from the high-Z campaign conducted 15 years ago. We focus on how chosen computational and physics parameters influence the implosion outcomes. By systematically changing the resolution of the computational mesh and the photon energies as well as modifying settings for the laser drive and TN fuel pre-heat effects, we assess the impact on experimentally measured performance metrics like neutron production from TN burn and x-ray emission during the implosion. Our results will help to improve the fidelity of simulations and guide future numerical studies and experimental designs.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

FY24 Status of Engineered Barrier Systems Research

This report describes research and development (R&D) activities conducted during Fiscal Year 2024 (FY24) specifically related to the Engineered Barrier System (EBS) R&D Work Package in the Spent Fuel and High-Level Waste Disposition Campaign supported by the United States (U.S.) Department of Energy (DOE). The R&D activities focus on understanding EBS component evolution and interactions within the EBS, as well as interactions between the host media and the EBS. The R&D team represented in this report consists of individuals from Sandia National Laboratories, Lawrence Berkeley National Laboratory (LBNL), Los Alamos National Laboratory (LANL), and Vanderbilt University. EBS R&D work also leverages international collaborations to ensure that the DOE program is active and abreast of the latest advances in nuclear waste disposal.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

White Rock Canyon Riparian Monitoring

Lands at Los Alamos National Laboratory (LANL) are owned and managed by the Department of Energy, National Nuclear Security Administration (DOE/NNSA). The Laboratory’s eastern boundary is in White Rock Canyon (WRC) along the Rio Grande within Technical Areas (TAs) 70 and 33, with approximately 4 miles of property along the river (Figure 1). Feral cattle have been documented along the Rio Grande in WRC since the 1980s. Cattle activity is known to be especially harmful to riparian ecosystems, which are hubs for biodiversity and crucial habitat used by multiple endangered species in this region, including the Southwestern Willow Flycatcher and Yellow-billed Cuckoo on LANL property (Poessel 2020, Sanchez 2021). To gain a comprehensive understanding of the status of riparian ecosystems within WRC and the damage feral cattle populations are imposing, ecologists at LANL conducted a month-long vegetation monitoring project in September 2025. Riparian vegetation monitoring protocols and rapid assessments of cattle impacts were used to quantify the intensity and extent of cattle damage. The data collected will be used as a baseline for comparison following the removal of feral cattle from the canyon. Abundant cattle sign indicates current and heavy utilization of the riparian areas that were surveyed. There are multiple wallowing areas where soils are completely denuded of vegetation and highly compacted. Based on the severity and extent of impact observed in these areas, cattle use appears consistent and on-going over an extended period of years, supporting the need for removal and restoration management.

54 ENVIRONMENTAL SCIENCES↗

Cataloging Legacy Data from the Tritium Systems Test Assembly Program

The Tritium Systems Test Assembly (TSTA) at Los Alamos National Laboratory, operational from 1984 to 2001, was critical in advancing fusion fuel cycle technologies, including tritium storage, gas separation, and pumping. TSTA’s contributions, particularly in safe tritium operations, have influenced subsequent fusion projects. This paper discusses the ongoing effort to digitize and catalog TSTA’s historical data to create a searchable resource for the fusion research community. While the long-term objective is to develop a relational database for structured data management, the project remains in the early phase, with current efforts focused on scanning and indexing physical documents. Initial plans for database implementations are also presented, outlining key considerations for structure, query indexing, and standardization. As digitization progresses, future discussions will refine these implantation details to ensure an efficient and comprehensive system. This initiative aims to preserve critical legacy data, enhance the design of tritium system facilities, and support the next generation of fusion energy research.

42 ENGINEERING↗

Possible Energy Storage Legislation for New Mexico [Slides]

Energy security is a core component of the national mission of Los Alamos National Laboratory and an emerging initiative, with about $10M in play now. Los Alamos National Laboratory is a leading laboratory for fuel cells, smart grid, wind resource allocation, and biofuels. The New Mexico Legislature demonstrates interest and leadership in maximizing all our state’s natural energy resources. We are here today in response to requests originated by Representative Hall and Chairman Keller for potential legislation for a New Mexico energy storage strategy. In preparation for today’s testimony, we have accommodated input from a broad spectrum of stakeholders.

25 ENERGY STORAGE↗

LAFD: TA-15 DARHT Firefighter Facility Familiarization Tour, OJT 53044, Revision 0.2

The Los Alamos National Laboratory (LANL or the Lab) will conduct familiarization tours for the Los Alamos County Fire Department (LAFD) at the Dual-Axis Radiographic Hydrodynamic Test (DARHT) Facility, TA-15-0312. The purpose of these tours is to orient LAFD firefighters to the DARHT facility layout and hazards. This document provides information and figures to supplement the familiarization tours. The document will be distributed to the trainees at the time of the familiarization tour. A checklist (Attachment A) has also been developed to ensure that all required information is consistently presented to LAFD personnel during the familiarization tours.

99 GENERAL AND MISCELLANEOUS↗

LAFD: TA-3 NISC & SCC Facility Familiarization Tour, OJT #53356

Los Alamos National Laboratory (LANL, the Laboratory, or the Lab) conducts familiarization tours for Los Alamos County Fire Department (LAFD) personnel at the Strategic Computing Complex (SCC), TA-03-2327, and the Nonproliferation & International Security Complex (NISC), TA-03-2322. These tours are official LANL business; their purpose is to orient the firefighters to the SCC and the NISC so that they can respond efficiently and quickly to a variety of emergency situations. The tour includes ingress and egress of the buildings, layout and organization of the buildings, evacuation procedures, and areas of concern to emergency responders within these buildings. LAFD firefighters have the training, skills, and abilities to perform these emergency responder tasks; other LANL personnel who have the required clearance level cannot perform these tasks. This handout provides details of the information, along with maps and diagrams, to be presented during the familiarization tours. The report will be distributed to the trainees at the time of the tour. A corresponding checklist will also be used as guidance during the familiarization tours to ensure that all required information is presented to the LAFD personnel.

99 GENERAL AND MISCELLANEOUS↗

ISO 14001:2015 Environmental Management System Management Assessment Internal Review Assessing Organization: EPC-ES LANL-ASMT-2022-0289 (Spring 2023)

The Environmental Protection and Compliance Division-Environmental Stewardship Group of Los Alamos National Laboratory conducted a management assessment that supports the implementation of the Los Alamos National Laboratory Environmental Management System according to International Organization for Standardization (ISO) 14001:2015, Environmental Management System. The assessment resulted in zero findings of nonconformity, five opportunities for improvement, four noteworthy practices, and three observations.

54 ENVIRONMENTAL SCIENCES↗

A non-intrusive framework using acoustic signals and deep learning for boiling diagnostics in visual-limited environments

Accurate monitoring of boiling heat transfer is critical for safeguarding high-power systems operating in environments where conventional optical diagnostics are hindered by radiation fields or restricted visual accessibility. This study presents a non-intrusive framework that integrates hydroacoustic sensing with deep learning to infer near-wall boiling characteristics and enable predictive thermal assessment without visual access. In a prototypical subcooled flow-boiling facility representative of the Isotope Production Facility (IPF) at Los Alamos, hydrophones capture boiling-induced acoustic emissions that are transformed into background-removed Short-Time Fourier Transform (STFT) spectrograms. A convolutional neural network (CNN) then regresses heat flux, wall superheat, and key bubble parameters directly from these spectrograms. The CNN achieved predictive accuracy under nominal conditions and demonstrated robustness and generalization under acoustic noise for Signal-to-Noise Ratios (SNRs) down to approximately 0 dB. When integrated into an ANSYS CFX wall-boiling model, the acoustically inferred parameters reproduced boiling curve and critical heat flux (CHF) values consistent with image-based benchmarks. Furthermore, the model retained reliable performance under moderate variations in bulk temperature, flow rate, and hydrophone placement, confirming its generalizability across practical boundary conditions. These results demonstrate the feasibility of hydroacoustic-based deep learning as a viable path toward real-time, radiation-tolerant boiling diagnostics and predictive thermal safety assessment in inaccessible systems such as the IPF.

42 ENGINEERING↗