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At least 1,153 records · Page 64

Identifying Two-Dimensional Z{sub 2} Antiferromagnetic Topological Insulators

We revisit the question of whether a two-dimensional topological insulator may arise in a commensurate Néel antiferromagnet, where staggered magnetization breaks the symmetry with respect to both elementary translation and time reversal, but retains their product as a symmetry. In contrast to the so-called Z{sub 2} topological insulators, an exhaustive characterization of antiferromagnetic topological phases with the help of topological invariants has been missing. We analyze a simple model of an antiferromagnetic topological insulator and chart its phase diagram, using a recently proposed criterion for centrosymmetric systems [13]. We then adapt two methods, originally designed for paramagnetic systems, and make antiferromagnetic topological phases manifest. The proposed methods apply far beyond the particular examples treated in this work, and admit straightforward generalization. We illustrate this by two examples of non-centrosymmetric systems, where no simple criteria have been known to identify topological phases. We also present, for some cases, an explicit construction of edge states in an antiferromagnetic topological insulator.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Correlation between antiferromagnetic and Mott states in spin orbit coupled Sr 2 Ir O 4 : A study of Sr 2 Ir 1 – x M x O 4 ( M = Fe or Co)

Sr 2 IrO 4 is an archetypal spin-orbit-coupled Mott insulator with an antiferromagnetic state below 240 K. Here we report results of our study on single crystals of Sr 2 Ir 1–x Fe x O 4 (0 ≤ x < 0.32) and Sr 2 Ir 1–x Co x O 4 (0 ≤ x < 0.22). Fe doping retains the antiferromagnetic state but simultaneously precipitates an emergent metallic state whereas Co doping causes a rapid collapse of both the antiferromagnetic and Mott states, giving rise to a confined metallic state featuring a pronounced linearity of the basal-plane resistivity up to 700 K. The results indicate tetravalent Fe 4+ (3d 4 ) ions in the intermediate spin state with S = 1 and Co 4+ (3d 5 ) ions in the high spin state with S = 5/2 substituting for Ir 4+ (5d 5 ) ions in Sr 2 IrO 4 , respectively. The effective magnetic moment closely tracks the Néel temperature as doping increases, suggesting that the spin state of the dopant predominately determines the magnetic properties in doped Sr 2 IrO 4 . Furthermore, all relevant properties including charge-carrier density (e.g., 10 28 /m 3 ), Sommerfeld coefficient (e.g., 19 mJ / mole K 2 ), and Wilson ratio (e.g., 2.6) consistently demonstrate an emergent metallic state that is both robust and highly correlated in the two systems, arising from the percolation of bound states and the weakening of structural distortions. Furthermore, this study strongly indicates that the antiferromagnetic and Mott states are correlated in an unconventional manner in Sr 2 IrO 4 .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Enhancement in the transport critical current density J{sub c} in YBa{sub 2}Cu{sub 3}O{sub 7−δ} added with an insulating nano crystalline YBa{sub 2}HfO{sub 5.5} perovskite

When a magnetic field is applied to type II superconductors, such as YBa{sub 2}Cu{sub 3}0{sub 7−δ} (YBCO), the flux quanta penetrate the material as a regular array of vortices. However when transport currents are applied, they act to move these vortices, thus lowers the critical current density (J{sub c}) as well as destroying superconductivity. The development of microstructures made of YBCO materials has enabled engineers to increase the critical current density, within Type II materials by introducing flux pinning centres into the material. The microstructure and flux pinning properties of YBa{sub 2}Cu{sub 3}O{sub 7−δ} system with varying levels (0-5 wt. %) of a nano perovskite ceramic insulator; YBa{sub 2}HfO{sub 5.5} addition was studied in detail. Orthorhombic YBa{sub 2}Cu{sub 3}O{sub 7−δ} powder was prepared through conventional solid state route and a modified combustion method was used for synthesizing nanocrystalline YBa{sub 2}HfO{sub 5.5}. The structure and microstructure of the samples examined by X-ray diffraction and scanning electron microscopy showed that YBa{sub 2}HfO{sub 5.5} and YBCO remained unreacted even at higher processing temperature without deteriorating the superconducting properties. The scanning electron microscope image shows that YBa{sub 2}HfO{sub 5.5} forms an electrical-network between grains. These observations suggest that the YBa{sub 2}HfO{sub 5.5} addition to the Y-123-compounds improve the electrical connection between superconducting grains and substantial improvements in the relative electrical transport properties of the composites. The variation of sintering temperature, density, critical transition temperature (T{sub c}) and magnetic field dependence of critical current density (J{sub c}) of YBa{sub 2}Cu{sub 3}O{sub 7−δ} having different proportions of YBa{sub 2}HfO{sub 5.5} in the matrix were also studied in detail. It is found that the addition of these elements considerably enhances the flux pinning strength of the system, and there is also an increase of critical temperature (T{sub c}) and critical current density (J{sub c}) up to an optimum value of 8.76 × 10{sup 4} A/cm{sup 2} for a concentration of 2 wt % addition of nano YBa{sub 2}HfO{sub 5.5}. The enhancement of the critical current density in the YBa{sub 2}Cu{sub 3}O{sub 7−δ} - YBa{sub 2}HfO{sub 5.5} samples is attributed to the sustained formation of the insulating and non-reacting YBa{sub 2}HfO{sub 5.5} phase acting as pinning center. The addition of YBa{sub 2}HfO{sub 5.5} in YBa{sub 2}Cu{sub 3}O{sub 7−δ} bulk superconductor also enhances the pinning force density from 3 ×10{sup 6} N/m{sup 3} to 69.6 × 10{sup 6}N/m{sup 3} at 77 K.

36 MATERIALS SCIENCE↗

Competing Zero-Field Chern Insulators in Superconducting Twisted Bilayer Graphene

The discovery of magic angle twisted bilayer graphene has unveiled a rich variety of superconducting, magnetic, and topologically nontrivial phases. Here, we show that the zero-field states at odd integer filling factors in h-BN nonaligned devices are consistent with symmetry broken Chern insulators, as is evidenced by the observation of the anomalous Hall effect near moiré cell filling factor ν = +1. The corresponding Chern insulator has a Chern number C = ±1 and a relatively high Curie temperature of T c ≈ 4.5 K. In a perpendicular magnetic field above B > 0.5 T we observe a transition of the ν = +1 Chern insulator from Chern number C = ±1 to C = 3, characterized by a quantized Hall plateau with R yx = h/3e 2 . These observations demonstrate that interaction-induced symmetry breaking leads to zero-field ground states that include almost degenerate and closely competing Chern insulators, and that states with larger Chern numbers couple most strongly to the B field. In addition, the device reveals strong superconducting phases with critical temperatures of up to T c ≈ 3.5 K. By providing the first demonstration of a system that allows gate-induced transitions between magnetic and superconducting phases, our observations mark a major milestone in the creation of a new generation of quantum electronics.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Enhancement of charge-neutral fermionic excitations near the spin-flop transition in the magnetic Kondo material YbIr 3 Si 7

The new Kondo material YbIr 3 Si 7 , similar to other Kondo insulators, has been reported to exhibit charge-neutral fermionic excitations through measurements of specific heat and thermal conductivity at low temperatures. We performed 29 Si-NMR on YbIr 3 Si 7 to investigate the magnetic response of charge-neutral fermions from a microscopic perspective. In low magnetic fields parallel to the c axis, a single NMR peak in the paramagnetic state splits into three peaks below TN. In contrast, only a slight shift of the single NMR peak was observed in high magnetic fields. This spectral change as a function of the c-axis magnetic field is interpreted as a spin-flop transition, at which the magnetic moments oriented along the c axis antiferromagnetic (AFM-I) phase are rotated to the ab plane with a ferromagnetic component along the c-axis (AFM-II phase). In the vicinity of the spin-flop magnetic field H M , the nuclear spin-lattice relaxation rate 1/T 1 was found to be proportional to temperature at low temperatures, indicating the existence of charge-neutral fermions. Furthermore, a peak of 1/T 1 versus the c-axis magnetic field suggests that the charge-neutral fermions in YbIr 3 Si 7 are closely related to its magnetic properties. Our findings shed light on the origin of charge-neutral fermions in insulators.

36 MATERIALS SCIENCE↗

Epitaxial strain modulated electronic properties of interface controlled nickelate superlattices

For this study, perovskite nickelate heterostructures consisting of single unit cells of EuNiO 3 and LaNiO 3 have been grown on a set of single crystalline substrates by pulsed laser interval deposition to investigate the effect of epitaxial strain on electronic and magnetic properties at the extreme interface limit. Despite the variation of substrate in-plane lattice constants and lattice symmetry, the structural response to heterostructuring is primarily controlled by the presence of the EuNiO 3 layer. In sharp contrast to bulk LaNiO 3 or EuNiO 3 , the superlattices grown under tensile strains exhibit metal-to-insulator transitions (MIT) below room temperature. The onset of magnetic and electronic transitions associated with the MIT can be further separated by application of large tensile strain. Furthermore, these transitions can be entirely suppressed by very small compressive strain. X-ray resonant absorption spectroscopy measurements reveal that such strain-controlled MIT is directly linked to a strain-induced self-doping effect without any chemical doping.

36 MATERIALS SCIENCE↗

Effects of Annealing Temperature and Compaction Pressure on Magnetic Properties of Fe–Si Powder Cores Fabricated by an Improved Bluing Method

Fe-6.5wt%Si soft magnetic powder cores were prepared by using an improved bluing insulation method. A high-quality oxide insulation layer with good temperature stability was found to distribute continuously in the intervals between the Fe–Si particles. The effects of the annealing temperature and the compaction pressure on the core’s magnetic properties were investigated in detail. It was found that high temperature and low compaction pressure are beneficial to decrease the core’s inner stress and high compaction pressure is helpful to reduce the air gap. All the variations of the magnetic performance for the powder cores discussed in this paper were explained reasonably by considering these two factors. From the point of view of low loss, 760 °C and 2090 MPa were confirmed to be the relatively best annealing temperature and compaction pressure, respectively. The μ{sub e}, the % μ{sub e} at 100 Oe, and the loss at 50 kHz/1000 Gs for the core prepared under these two conditions are 63.57, 72.82%, and 547.66 mW/cm{sup 3}, respectively.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Magnon Landau Levels and Spin Responses in Antiferromagnets

We study gauge fields produced by gradients of the Dzyaloshinskii-Moriya interaction and propose a model of an AFM topological insulator of magnons. In the long wavelength limit, the Landau levels induced by the inhomogeneous Dzyaloshinskii-Moriya interaction exhibit relativistic physics described by the Klein-Gordon equation. The spin Nernst response due to the formation of magnonic Landau levels is compared to similar topological responses in skyrmion and vortex-antivortex crystal phases of AFM insulators. Here, our studies show that AFM insulators exhibit rich physics associated with topological magnon excitations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Investigations of surface structural, dynamical, and magnetic properties of systems exhibiting multiferroicity, and topological phases by helium scattering spectroscopies (Final Report)

We propose to investigate the surface structural, dynamics and magnetic properties of the novel class of topological insulator crystals, as well as crystals that exhibit multiferroicity, magnetoelectricity and thermoelectricity. Topological insulators (TIs) are a new class of insulators in which a bulk gap for electronic excitations is generated because of the strong spin-orbit coupling inherent to these systems. These materials are distinguished from ordinary insulators by the presence of gapless metallic surface states, resembling chiral edge modes in quantum Hall systems, but with unconventional spin textures. These exotic metallic states are formed by topological conditions that also render the electrons travelling on such surfaces insensitive to scattering by impurities. The electronic quasi-particles populating the topological surface state are Dirac fermions; they have a linear dispersion and thus are massless just like photons. We propose to investigate the interaction of these massless Dirac fermions with the massive lattice in the newly discovered crystals, Bi 2 Se 3 , Bi 2 Te 3 and Sb 2 Te 3 . We shall use inelastic helium beam scattering from surfaces to search for related signatures in surface phonon dispersions mappings that cover the entire surface Brillouin zone of these materials. Our recent investigations of the (001) surface of the multiferroic crystals (Li/Na)Cu 2 O 2 revealed an anomalous surface structural behavior where surface Cu$^{2+}$ row rise above the surface plane as the crystal was cooled. Subsequent worming revealed the onset of a thermally activated incommensurate surface phase, driven by the elevated rows. We are currently investigating the structure of the magnetic phases in these quasi-one-dimensional magnetic rows. Multiferroics are excellent candidates for large magnetoelectric response. We propose to extend this investigation to the class of delafossites which are also multiferroics and have been investigated as good candidates for thermoelectric power devices. They are also typical triangular lattice antiferromagnets with geometric magnetic frustration that leads to helimagnetic structures.

36 MATERIALS SCIENCE↗

Atomic-scale tailoring of spin susceptibility via non-magnetic spin-orbit impurities

Abstract Following the discovery of topological insulators, there has been a renewed interest in superconducting systems that have strong spin-orbit (SO) coupling. Here we address the fundamental question of how the spin properties of a otherwise spin-singlet superconducting ground state evolve with increasing SO impurity density. We have mapped out the Zeeman critical field phase diagram of superconducting Al films that were deposited over random Pb cluster arrays of varying density. These phase diagrams give a direct measure of the Fermi liquid spin renormalization, as well as the spin orbit scattering rate. We find that the spin renormalization is a linear function of the average Pb cluster -to- cluster separation and that this dependency can be used to tune the spin susceptibility of the Al over a surprisingly wide range from 0.8χ 0 to 4.0χ 0 , where χ 0 is the non-interacting Pauli susceptibility.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Vortices, skyrmions, and chirality waves in frustrated Mott insulators with a quenched periodic array of impurities

Finite-Q magnetic instabilities are rather common in frustrated magnets. When the magnetic susceptibility is maximized at multiple-Q vectors related through lattice symmetry operations, exotic magnetic orderings such as vortex and skyrmion crystals may follow. Here, we show that a periodic array of nonmagnetic impurities, which can be realized through charge density wave ordering, leads to a rich phase diagram featuring a plethora of chiral magnetic phases, especially when there is a simple relation between the reciprocal vectors of the impurity superlattice and the magnetic Q vectors. We also investigate the effect of changing the impurity concentration or disturbing the impurity array with small quenched randomness. Lastly, alternative realizations of impurity superlattices are briefly discussed.

36 MATERIALS SCIENCE↗

Three-dimensional quantum Hall effect and metal–insulator transition in ZrTe 5

The discovery of the quantum Hall effect (QHE) in two-dimensional electronic systems has given topology a central role in condensed matter physics. Although the possibility of generalizing the QHE to three-dimensional (3D) electronic systems was proposed decades ago, it has not been demonstrated experimentally. Here we report the experimental realization of the 3D QHE in bulk zirconium pentatelluride (ZrTe 5 ) crystals. We perform low-temperature electric-transport measurements on bulk ZrTe 5 crystals under a magnetic field and achieve the extreme quantum limit, where only the lowest Landau level is occupied, at relatively low magnetic fields. In this regime, we observe a dissipationless longitudinal resistivity close to zero, accompanied by a well-developed Hall resistivity plateau proportional to half of the Fermi wavelength along the field direction. This response is the signature of the 3D QHE and strongly suggests a Fermi surface instability driven by enhanced interaction effects in the extreme quantum limit. By further increasing the magnetic field, both the longitudinal and Hall resistivity increase considerably and display a metal–insulator transition, which represents another magnetic-field-driven quantum phase transition. Lastly, our findings provide experimental evidence of the 3D QHE and a promising platform for further exploration of exotic quantum phases and transitions in 3D systems.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Electromechanical Properties of 1-mm-Wide Superconducting Cables Comprised of Exfoliated YBCO Filaments

Development of multifilament YBCO cables is an important step toward the manufacture of practical superconducting magnets based on second generation high-temperature superconductor technology. Currently, magnets manufactured from wide 2G tapes suffer from high magnetization loss and poor reliability. The presence of an insulation substrate is to insulate YBCO layers from each other, which allows only lateral (along the tape face) current sharing. Here we present an exfoliated multilayer cable with electrically coupled (1 mm wide) filaments that permit normal (across the tape) current sharing within the cable. Finally, this development can potentially enable fast ramping and stable high-field magnets for applications in fusion, energy storage, and transportation.

2G conductor↗

Magnetic Structure and Spin Fluctuation in Colossal Magnetoresistance Ferrimagnet Mn 3 Si 2 Te 6

The ferrimagnetic insulator Mn 3 Si 2 Te 6 , which features a Curie temperature T c at 78 K and a delicate yet consequential magnetic frustration, exhibits colossal magnetoresistance (CMR) when the magnetic field is applied along the magnetic hard axis, surprisingly inconsistent with existing precedents [Y. Ni, H. Zhao, Y. Zhang, B. Hu, I. Kimchi, and G. Cao, Phys. Rev. B 103, L161105 (2021)]. This discovery motivates a thorough single-crystal neutron diffraction study in order to gain insights into the magnetic structure and its hidden correlation with the new type of CMR. Here we report a noncollinear magnetic structure below the T c where the moments lie predominantly within the basal plane but tilt toward the c axis by ≈10° at ambient conditions. A substantial magnetic diffuse scattering decays slowly and persists well above the T c . The evolution of the spin correlation lengths agrees well with the electrical resistivity, underscoring the role of spin fluctuation contributing to the magnetoresistivity near the transition. Further, application of magnetic field along the c axis renders a swift occurrence of CMR but only a slow tilting of the magnetic moments toward the c axis. The unparalleled changes indicate a nonconsequential role of magnetic polarization.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Orthogonal magnetization and symmetry breaking in pyrochlore iridate Eu 2 Ir 2 O 7

We present that electrons in the pyrochlore iridates experience a large interaction energy in addition to a strong spin–orbit interaction. Both features make the iridates promising for realizing novel states such as the topological Mott insulator. The pyrochlore iridate Eu 2 Ir 2 O 7 shows a metal–insulator transition at T N ~ 120 K below which a magnetically ordered state develops. Using torque magnetometry, we uncover an unusual magnetic response. A magnetic field H applied in its a–b plane produces a nonlinear magnetization M ⊥ orthogonal to the plane. M ⊥ displays a d-wave field-angle pattern consistent with octupolar order, with a handedness dictated by field cooling, leading to symmetry breaking of the chirality ω. Lastlyl, a surprise is that the lobe orientation of the d-wave pattern is sensitive to the direction of the field when the sample is field-cooled below T N , suggestive of an additional order parameter η already present at 300 K.

36 MATERIALS SCIENCE↗

Charge Conservation beyond Uniformity: Spatially Inhomogeneous Electromagnetic Response in Periodic Solids

Nonlinear electromagnetic response functions have reemerged as a crucial tool for studying quantum materials, due to recently appreciated connections between optical response functions, quantum geometry, and band topology. Most attention has been paid to responses to spatially uniform electric fields, relevant to low-energy optical experiments in conventional solid state materials. However, magnetic and magnetoelectric phenomena are naturally connected by responses to spatially varying electric fields due to Maxwell’s equations. Furthermore, in the emerging field of moiré materials, characteristic lattice scales are much longer, allowing spatial variation of optical electric fields to potentially have a measurable effect in experiments. In order to address these issues, we develop a formalism for computing linear and nonlinear responses to spatially inhomogeneous electromagnetic fields. Starting with the continuity equation, we derive an expression for the second-quantized current operator that is manifestly conserved and model independent. Crucially, our formalism makes no assumptions on the form of the microscopic Hamiltonian and so is applicable to model Hamiltonians derived from tight-binding or calculations. We then develop a diagrammatic Kubo formalism for computing the wave vector dependence of linear and nonlinear conductivities, using Ward identities to fix the value of the diamagnetic current order by order in the vector potential. We apply our formula to compute the magnitude of the Kerr effect at oblique incidence for a model of a moiré-Chern insulator and demonstrate the experimental relevance of spatially inhomogeneous fields in these systems. We further show how our formalism allows us to compute the (orbital) magnetic multipole moments and magnetic susceptibilities in insulators. Turning to nonlinear response, we use our formalism to compute the second-order transverse response to spatially varying transverse electric fields in our moiré-Chern insulator model, with an eye toward the next generation of experiments in these systems. Published by the American Physical Society 2024

Physics↗

Interface magnetism of Co{sub 2}FeGe Heusler alloy layers and magnetoresistance of Co{sub 2}FeGe/MgO/Fe magnetic tunnel junctions

The interface magnetism between Co{sub 2}FeGe Heusler alloy layers and MgO layers was investigated using {sup 57}Fe Mössbauer spectroscopy. Interface-sensitive samples, where the {sup 57}Fe isotope was used only for the interfacial atomic layer of the Co{sub 2}FeGe layer on the MgO layer, were prepared using atomically controlled alternate deposition. The {sup 57}Fe Mössbauer spectra of the interface-sensitive samples at room temperature were found similar to those of the bulk-sensitive Co{sub 2}FeGe films in which the {sup 57}Fe isotope was distributed throughout the films. On the other hand, the tunnel magnetoresistance effect of magnetic tunnel junctions with Co{sub 2}FeGe layers as the ferromagnetic electrodes showed strong reduction at room temperature. These results indicate that the strong temperature dependence of the tunneling magnetoresistance of magnetic tunnel junctions using Heusler alloy electrodes cannot be attributed simply to the reduction of the magnetization at the interfaces between the Heusler alloy and insulator layers.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Critical behavior at a dynamic vortex insulator-to-metal transition

An array of superconducting islands placed on a normal metal film offers a tunable realization of nanopatterned superconductivity. This system enables elucidating open questions concerning the nature of competing vortex states and phase transitions between them. A square array creates the egg crate potential in which magnetic field-induced vortices are frozen into a vortex insulator. We observe a vortex insulator-to-vortex metal transition driven by the applied electric current and determine critical exponents strikingly coinciding with those for thermodynamic liquid-gas transition. Lastly, our findings offer a comprehensive description of dynamic critical behavior and establish a deep connection between equilibrium and nonequilibrium phase transitions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗