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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,153 records · Page 64
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Historical Land Management Alters New Soil Carbon Inputs by Annual and Perennial Bioenergy Crops

Bioenergy and bioproduct markets are expanding to meet demand for climate-friendly goods and services. Perennial biomass crops are particularly well suited for this goal because of their high yields, low input requirements, and potential to increase soil carbon (C). However, it is unclear how much C is allocated into belowground pools by perennial bioenergy crops and whether the belowground benefits vary with nitrogen (N) fertilizer inputs. Using in situ 13 C pulse-chase labeling, we tested whether the sterile perennial grass Miscanthus × giganteus (miscanthus) or annual maize transfers more photosynthetic C to belowground pools. The experiment took place at two sites in Central and Northwest (NW) Iowa with different management histories and two nitrogen (N) fertilizer rates (0 and 224 kg N ha −1 year −1 ) to determine if the fate of plant-derived soil C depends on soil fertility and crop type (perennial or annual). Maize allocated a greater percentage of total new 13 C to roots than miscanthus, but miscanthus had greater new 13 C in total and belowground plant biomass. We found strong interactions between site and most soil measurements—including new 13 C in mineral and particulate soil organic matter (SOM) pools—which appears to be driven by differences in historical fertilizer management. The NW Iowa site, with a history of manure inputs, had greater plant-available nutrients (phosphorus, potassium, and ammonium) in soils, and resulted in less 13 C from miscanthus in SOM pools compared to maize (approximately 64% less in POM and 70% less in MAOM). In more nutrient-limited soils (Central site), miscanthus transferred 4.5 times more 13 C than maize to the more stable mineral-associated SOM pool. Our results suggest that past management, including historical manure inputs that affect a site's soil fertility, can influence the net C benefits of bioenergy crops.

13C↗
DOE OSTI2017

Ag + reduction and silver nanoparticle synthesis at the plasma–liquid interface by an RF driven atmospheric pressure plasma jet: Mechanisms and the effect of surfactant

Here, the involvement of plasma produced species in the reduction of silver ions at the plasma–liquid interface is investigated using a well-characterized radio-frequency driven atmospheric pressure plasma jet. The absolute gas phase H density was measured using two photon absorption laser induced fluorescence in the free jet. Broadband absorption and transmission electron microscopy were used to study the synthesis of silver nanoparticles (AgNPs). It is shown that fructose, an often used surfactant/stabilizer for AgNP synthesis, also acts as a reducing agent after plasma exposure. Nonetheless, surfactant free AgNP synthesis is observed. Several experimental findings indicate that H plays an important role in the reduction of silver ions for the plasma conditions in this study. Vacuum ultraviolet photons generated by the plasma are able to reduce silver ions in the presence of fructose. Adding H2 to the argon feed gas leads to the production of a large amount of AgNPs having a particle size distribution with a maximum at a diameter of 2–3 nm, which is not observed for argon plasmas. This finding is consistent with a smaller concentration of reducing species at the plasma–liquid interface for Ar with the H2 admixture plasma. The smaller flux of reactive species to the liquid is in this case due to a less strong interaction of the plasma with the liquid. The formation of the nanoparticles was observed even at a distance of 6–7 mm below the tip of the plasma plume, conditions not favoring the injection of electrons.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Electronic surface reconstruction of TiO 2 nanocrystals revealed by resonant inelastic x-ray scattering

The identification of lattice multiphases in TiO 2 nanocrystals is studied by high resolution transmission electron microscope and electron diffraction patterns. Based on the spectroscopic analysis using soft x-ray absorption and resonant inelastic soft x-ray scattering, it is believed that the oxygen vacancies at the interface exhibit structural distortion of the TiO$^{8-}_6$ cluster around the defect site as for the multiphase lattice. We elucidate that the extra 3d electrons nearby induce the inelastic scattering features with the excitation energy dependence owing to different energy relaxation processes, a characteristic of the electron-phonon coupling or the nature of the electron-hole pair at the intermediate state. The manifold dd excitations driven by the strong interaction between Ti-3d and O-2p electrons are noticeably rich, coexisting on both Ti and O sites. Finally, this sophisticated experiment can advance the perspective of nanocomposite TiO 2 for various interactions of surface Ti 3+ in applications of future devices.

36 MATERIALS SCIENCE↗
DOE OSTI2017

Versatile, ultra-low sample volume gas analyzer using a rapid, broad-tuning ECQCL and a hollow fiber gas cell

We describe a versatile mid-infrared (Mid-IR) spectroscopy system developed to measure the concentration of a wide range of gases with an ultra-low sample size. The system combines a rapidly-swept external cavity quantum cascade laser (ECQCL) with a hollow fiber gas cell. The ECQCL has sufficient spectral resolution and reproducibility to measure gases with narrow features (e.g., water, methane, ammonia, etc.), and also the spectral tuning range needed to measure volatile organic compounds (VOCs), (e.g., aldehydes, ketones, hydrocarbons), sulfur compounds, chlorine compounds, etc. The hollow fiber is a capillary tube having an internal reflective coating optimized for transmitting the Mid-IR laser beam to a detector. Sample gas introduced into the fiber (e.g., internal volume = 0.6 ml) interacts strongly with the laser beam, and despite relatively modest path lengths (e.g., L ~ 3 m), the requisite quantity of sample needed for sensitive measurements can be significantly less than what is required using conventional IR laser spectroscopy systems. Example measurements are presented including quantification of VOCs relevant for human breath analysis with a sensitivity of ~2 picomoles at a 1 Hz data rate.

broad-tuning↗
DOE OSTI2019

Fast nonadiabatic dynamics of many-body quantum systems

Modeling many-body quantum systems with strong interactions is one of the core challenges of modern physics. A range of methods has been developed to approach this task, each with its own idiosyncrasies, approximations, and realm of applicability. However, there remain many problems that are intractable for existing methods. In particular, many approaches face a huge computational barrier when modeling large numbers of coupled electrons and ions at finite temperature. Here, we address this shortfall with a new approach to modeling many-body quantum systems. On the basis of the Bohmian trajectory formalism, our new method treats the full particle dynamics with a considerable increase in computational speed. As a result, we are able to perform large-scale simulations of coupled electron-ion systems without using the adiabatic Born-Oppenheimer approximation.

Science & Technology - Other Topics↗
DOE OSTI2025

Disentangling the intertwined orders in a magnetic kagome metal

Intertwined orders appear when multiple orders are strongly interacting, and kagome metals have emerged as new platforms to explore exotic phases. FeGe has been found to develop a charge density wave (CDW) order within magnetic phase, suggesting an intricate interplay of the lattice, charge, and spin degrees of freedom. Recently, postgrowth annealing has been proposed to tune the CDW order from long-range to complete suppression, offering a tuning knob for the CDW order. Here, by comparing the electronic structures of FeGe subjected to different annealing conditions and distinct CDW properties, we report spectral evolution associated with the lattice and spin degrees of freedom. We find band evolution linked to a spin density wave (SDW) order present in both samples with and without CDW order, and another evolution connected to the lattice distortions that onset with the long-range CDW order and revert with the SDW order. Our results reveal a rare competitive cooperation of the lattice, spin, and charge in FeGe.

Oh, Ji Seop↗
DOE OSTI2019

Discovery of topological Weyl fermion lines and drumhead surface states in a room temperature magnet

Topological matter is known to exhibit unconventional surface states and anomalous transport owing to unusual bulk electronic topology. In this study, we use photoemission spectroscopy and quantum transport to elucidate the topology of the room temperature magnet Co 2 MnGa. We observe sharp bulk Weyl fermion line dispersions indicative of nontrivial topological invariants present in the magnetic phase. On the surface of the magnet, we observe electronic wave functions that take the form of drumheads, enabling us to directly visualize the crucial components of the bulk-boundary topological correspondence. By considering the Berry curvature field associated with the observed topological Weyl fermion lines, we quantitatively account for the giant anomalous Hall response observed in this magnet. Our experimental results suggest a rich interplay of strongly interacting electrons and topology in quantum matter.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2021

Microscopic evolution of doped Mott insulators from polaronic metal to Fermi liquid

From polarons to a Fermi liquid Superconductivity in the cuprates emerges by doping an antiferromagnetic “parent” state with holes or electrons. With increased doping, antiferromagnetism gives way to unconventional superconductivity, and the system eventually becomes a Fermi liquid. Koepsell et al . simulated this progression using cold, strongly interacting lithium-6 atoms trapped in an optical lattice. Although the equivalent ordered phases are not yet reachable at the experimentally available temperatures, the researchers were able to measure multipoint spin and hole correlations over a wide range of hole doping. The evolution of these correlators with doping revealed a crossover from a polaronic regime to a Fermi liquid. —JS

Science & Technology - Other Topics↗
DOE OSTI2021

Observation of a prethermal discrete time crystal

Extending the framework of statistical physics to the nonequilibrium setting has led to the discovery of previously unidentified phases of matter, often catalyzed by periodic driving. However, preventing the runaway heating that is associated with driving a strongly interacting quantum system remains a challenge in the investigation of these newly discovered phases. In this work, we utilize a trapped-ion quantum simulator to observe the signatures of a nonequilibrium driven phase without disorder—the prethermal discrete time crystal. Here, the heating problem is circumvented not by disorder-induced many-body localization, but rather by high-frequency driving, which leads to an expansive time window where nonequilibrium phases can emerge. Floquet prethermalization is thus presented as a general strategy for creating, stabilizing, and studying intrinsically out-of-equilibrium phases of matter.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2023

Lead-chelating hole-transport layers for efficient and stable perovskite minimodules

The defective bottom interfaces of perovskites and hole-transport layers (HTLs) limit the performance of p-i-n structure perovskite solar cells. We report that the addition of lead chelation molecules into HTLs can strongly interact with lead(II) ion (Pb 2+ ), resulting in a reduced amorphous region in perovskites near HTLs and a passivated perovskite bottom surface. Here, the minimodule with an aperture area of 26.9 square centimeters has a power conversion efficiency (PCE) of 21.8% (stabilized at 21.1%) that is certified by the National Renewable Energy Laboratory (NREL), which corresponds to a minimal small-cell efficiency of 24.6% (stabilized 24.1%) throughout the module area. Small-area cells and large-area minimodules with lead chelation molecules in HTLs had a light soaking stability of 3010 and 2130 hours, respectively, at an efficiency loss of 10% from the initial value under 1-sun illumination and open-circuit voltage conditions.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

Feasibility of a feedback control of atomic self-organization in an optical cavity

Many interesting nonlinear effects are based on the strong interaction of motional degrees of freedom of atoms with an optical cavity field. Among them is the spatial self-organization of atoms in a pattern where the atoms group in either odd or even sites of the cavity-induced optical potential. An experimental observation of this effect can be simplified by using, along with the original cavity-induced feedback, an additional electronic feedback based on the detection of light leaking the cavity and the control of the optical potential for the atoms. Following our previous study, we show that this approach is more efficient from the laser power perspective than the original scheme without the electronic feedback.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2015

Cluster correlations in dense matter and equation of state

Correlations in strongly interacting matter at subsaturation densities lead to the formation of clusters and the appearance of phases transitions with a change of thermodynamic properties and chemical composition. These features can be described in a generalized relativistic density functional approach using clusters as explicit degrees of freedom with medium-dependent properties. The model is constructed in order to provide equations of state for astrophysical applications. It can be adapted also to nuclear structure calculations with cluster correlations on the surface of heavy nuclei. The appearance of α-particles modifies the neutron skin thickness of neutron-rich nuclei and affects the correlation with the density dependence of the symmetry energy.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2017

Study of compressed baryonic matter at FAIR: JINR participation

The scientific goal of the CBM (Compressed Baryonic Matter) experiment at FAIR (Darmstadt) is to explore the phase diagram of strongly interacting matter at highest baryon densities. The physics program of the CBM experiment is complimentary to the programs to be realized at MPD and BMN facilities at NICA and will start with beam derived by the SIS100 synchrotron. The results of JINR participation in the development of different sub-projects of the CBM experiment are presented.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2018

Light Meson Production in Heavy Ion Collisions in the PHENIX Experiment

Production of a strongly interacting quark−gluon plasma (QGP) has been established in central heavy ion collisions during the studies carried out at the RHIC collider. The experiments on interactions of asymmetric nuclei (Cu + Au, U + U) provide the means to study systematically a jet quenching effect, which is a signature of QGP formation. In this paper, the factors of nuclear modification of π{sup 0} and η mesons in Cu + Au and U + U collisions at 200 GeV measured in the PHENIX experiment at RHIC are presented.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2015

The structure of the nucleon: Elastic electromagnetic form factors

Precise proton and neutron form factor measurements at Jefferson Lab, using spin observables, have recently made a significant contribution to the unraveling of the internal structure of the nucleon. Accurate experimental measurements of the nucleon form factors are a test-bed for understanding how the nucleon's static properties and dynamical behavior emerge from QCD, the theory of the strong interactions between quarks. There has been enormous theoretical progress, since the publication of the Jefferson Lab proton form factor ratio data, aiming at reevaluating the picture of the nucleon. We will review the experimental and theoretical developments in this field and discuss the outlook for the future.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2019

Confronting gravitational-wave observations with modern nuclear physics constraints

Multi-messenger observations of neutron star (NS) mergers have the potential to revolutionize nuclear astrophysics. They will improve our understanding of nucleosynthesis, provide insights about the equation of state (EOS) of strongly interacting matter at high densities, and enable tests of the theory of gravity and of dark matter. We focus on the EOS, where both gravitational waves (GWs) from neutron-star mergers and X-ray observations from space-based detectors such as NICER will provide more stringent constraints on the structure of neutron stars. Furthermore, recent advances in nuclear theory have enabled reliable calculations of the EOS at low densities using effective field theory based Hamiltonians and advanced techniques to solve the quantum many-body problem. In this paper, we address how the first observation of GWs from GW170817 can be combined with modern calculations of the EOS to extract useful insights about the EOS of matter encountered inside neutron stars. We analyze the impact of various uncertainties, the role of phase transitions in the NS core, and discuss how future observations will improve our understanding of dense matter.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2026

Few is different: deciphering many-body dynamics in mesoscopic quantum gases

Emergent macroscopic descriptions of matter, such as hydrodynamics, are central to our description of complex physical systems across a wide spectrum of energy scales. The conventional understanding of these many-body phenomena has recently been shaken by a number of experimental findings. Collective behavior of matter has been observed in mesoscopic systems, such as high-energy hadron–hadron collisions, or ultracold gases with only a few strongly interacting fermions. In such systems, the separation of scales between macroscopic and microscopic dynamics (at the heart of any effective theory) is inapplicable. To address the conceptual challenges that arise from these observations and explore the universality of emergent descriptions of matter, the EMMI Rapid Reaction Task Force was assembled. This document summarizes the RRTF discussions on recent theoretical and experimental advances in this rapidly developing field. Leveraging technological breakthroughs in the control of quantum systems, we can now quantitatively explore what it means for a system to exhibit behavior beyond the sum of its individual parts. In particular, the report highlights how the (in)applicability of hydrodynamics and other effective theories can be probed across three principal frontiers: the size frontier, the equilibrium frontier, and the interaction frontier.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2015

The pMSSM10 after LHC run 1

We present a frequentist analysis of the parameter space of the pMSSM10, in which the following ten soft SUSY-breaking parameters are specified independently at the mean scalar top mass scale M SUSY ≡ √m $\tilde{t}$ 1 m $\tilde{t}$ 2 : the gaugino masses M 1,2,3 , the first-and second-generation squark masses m $\tilde{q}$ 1 = m $\tilde{q}$ 2 , the third-generation squark mass m $\tilde{q}$ 3 , a common slepton mass m $\tilde{ℓ}$ and a common trilinear mixing parameter A , as well as the Higgs mixing parameter μ , the pseudoscalar Higgs mass M A and tanβ , the ratio of the two Higgs vacuum expectation values. We use the MultiNest sampling algorithm with ~ 1.2 ×10 9 points to sample the pMSSM10 parameter space. A dedicated study shows that the sensitivities to strongly interacting sparticle masses of ATLAS and CMS searches for jets, leptons + E-slash T signals depend only weakly on many of the other pMSSM10 parameters. With the aid of the Atom and Scorpion codes, we also implement the LHC searches for electroweakly interacting sparticles and light stops, so as to confront the pMSSM10 parameter space with all relevant SUSY searches. In addition, our analysis includes Higgs mass and rate measurements using the HiggsSignals code, SUSY Higgs exclusion bounds, the measurements of BR(B s →μ + μ - ) by LHCb and CMS, other B -physics observables, electroweak precision observables, the cold dark matter density and the XENON100 and LUX searches for spin-independent dark matter scattering, assuming that the cold dark matter is mainly provided by the lightest neutralino χ-tilde 1 0 . We show that the pMSSM10 is able to provide a supersymmetric interpretation of (g-2) μ , unlike the CMSSM, NUHM1 and NUHM2. As a result, we find (omitting Higgs rates) that the minimum χ2=20.5 with 18 degrees of freedom (d.o.f.) in the pMSSM10, corresponding to a χ2 probability of 30.8 %, to be compared with χ2/d.o.f.=32.8/24(31.1/23)(30.3/22) in the CMSSM (NUHM1) (NUHM2). We display the one-dimensional likelihood functions for sparticle masses, and we show that they may be significantly lighter in the pMSSM10 than in the other models, e.g., the gluino may be as light as ~ 1250 GeV at the 68 % CL, and squarks, stops, electroweak gauginos and sleptons may be much lighter than in the CMSSM, NUHM1 and NUHM2. We discuss the discovery potential of future LHC runs, e + e - colliders and direct detection experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗