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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,189 records · Page 66

Influence of post deposition annealing on the microstructural evolution and tensile behavior of austenitic stainless-steel alloy 709 made by laser powder bed fusion

Structural materials used in the next generation nuclear reactors or other advanced energy systems are often required to withstand higher operating temperatures for a longer service life. Alloy 709 (A709), a Nb-containing and N-stabilized Fe-25Ni-20Cr austenitic stainless steel, has been recommended for high-temperature reactor constructions due to the better performance over the baseline Type 316H stainless steel. Here, in the current manuscript, for the first time, the microstructure evolution and tensile behavior of an A709 made by laser powder bed fusion (LPBF) is discussed. The as deposited and heat treated LPBF alloys are compared with a reference wrought alloy. Owing to the chemical segregation and a higher number of dislocations, the LPBF materials show a significantly higher density of precipitates formed during high temperature treatments when compared to the wrought samples. This is reflected when looking at the tensile properties, both at room and elevated temperatures, where LPBF samples show higher strengths compared to wrought materials.

36 MATERIALS SCIENCE↗

Space Station tethered elevator system

The optimized conceptual engineering design of a space station tethered elevator is presented. The tethered elevator is an unmanned, mobile structure which operates on a ten-kilometer tether spanning the distance between Space Station Freedom and a platform. Its capabilities include providing access to residual gravity levels, remote servicing, and transportation to any point along a tether. The report discusses the potential uses, parameters, and evolution of the spacecraft design. Emphasis is placed on the elevator's structural configuration and three major subsystem designs. First, the design of elevator robotics used to aid in elevator operations and tethered experimentation is presented. Second, the design of drive mechanisms used to propel the vehicle is discussed. Third, the design of an onboard self-sufficient power generation and transmission system is addressed.

Haddock, Michael H.↗

Microstructure evolution in ion-irradiated of UO{sub 2}

Uranium dioxide (UO{sub 2}) is today's most widely used nuclear fuel in commercial light water reactors. The cumulative radiation damage during the fission process causes severe degradation in the thermophysical properties of UO{sub 2} fuels, which limits their lifetime and increases their operational cost. There are four main sources for decreasing the thermal conductivity during reactor-irradiation: i) irradiation induced defects, ii) solid fission products, iii) fission gas and volatile fission products, and iv) fission gas precipitation and porosity evolution. Therefore, investigating the defect production and evolution, and fission product transport under irradiation, and revealing their physical mechanisms is of great importance in understanding the degradation of thermophysical properties of UO{sub 2} fuels. (authors)

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Neutronics analyses for the conceptual design of the SNS Second Target Station

The Spallation Neutron Source, in operation at the Oak Ridge National Laboratory since 2006, was designed to allow the addition of a second target station and an upgrade of the accelerator proton power. Both upgrades are now underway. Here we describe the evolution of the design of the target of the second target station with the emphasis on the effects of the proton beam footprint on the energy deposition in the target, stresses induced by the pulsed operation, and the importance of the residual heat. The moderator configurations and their optimization are discussed. With the utilization of pure parahydrogen moderators, small neutron beam cross-sections, and the specific optimization, neutron beams of the second target station will achieve exceptionally high peak brightness and time-averaged brightness.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

New Insights into Structural Evolution of LiNiO 2 Revealed by Operando Neutron Diffraction

LiNiO 2 (LNO) represents the end member in the compositional space of the LiNi 1-x-y Mn x Co y O 2 (as x and y approach zero) cathode system. Despite its high theoretical specific capacity (275 mAh/g), LNO suffers from phase transitions with large volume change and unfavorable reactions upon electrochemical cycling, which restricts its practical use in the application of lithium-ion batteries. While the contributing factor to the structural instability is commonly linked to the undesired volume collapse associated with the H2-H3 phase transition, detailed analysis of structural evolution following the entire route of phase transitions (H1-M-H2-H3) in real time under battery operating conditions remains a challenging task. In this work, we employ operando neutron diffraction to study the structural changes (crystal lattice, Li/Ni–O bond length, O–Ni–O bond angles, and LiO 2 /NiO 2 layer thickness) of LNO cathode in a home-built Li x NiO 2 || graphite full cell during Li + de-/intercalation. In particular, the anomalous increase(decrease) of Ni–O(Li–O) bond length at high SOC (>~85 %) in the H3 phase is discussed in the context of O 2- (2p)→Ni 4+ (3d) negative charge transfer.

25 ENERGY STORAGE↗

MX precipitate behavior in an irradiated advanced Fe-9Cr steel: Self-ion irradiation effects on phase stability

In an effort to optimize Fe-9Cr reduced activation ferritic/martensitic (RAFM) steels and to inform the design and operation of fusion reactors, this work represents the first in a series of cohesive studies dedicated to the evolution of MX-TiC precipitates under accelerated single and dual ion irradiations. This study investigates CNA9, a simplified Fe-9Cr RAFM steel featuring initial MX-TiC precipitate densities of (2.3±0.3)×10²¹ m⁻³. This material was subjected to single self-ion irradiation at damage levels ranging from 1 to 100 displacements per atom (dpa) over a temperature range of 300 to 600°C, with a nominal dose rate of 7×10⁻⁴ dpa/s. Irradiation-induced coarsening was observed, as evidenced by statistically significant increases in mean diameter sizes, at 15 dpa at both 500°C and 600°C, whereas no coarsening was noted at 300°C or 400°C. Further, complete dissolution of precipitates occurred at damage levels of 50 and 100 dpa across the two temperatures tested (300°C and 500°C) while no significant changes were observed at any doses below 15 dpa at 500°C. Experimentally parameterized recoil resolution modeling suggests that the observed radiation stability of MX-TiC precipitates is intricately linked to diffusional changes of solutes resulting from the co-evolution of microstructural features within the experiments. The findings align with current theoretical perspectives on radiation-induced precipitate stability in complex alloys.

36 MATERIALS SCIENCE↗

QCD analysis of Δ S = 0 hadronic parity violation

We present a QCD analysis of the effective weak Hamiltonian at hadronic energy scales for strangeness-nonchanging (ΔS = 0) hadronic processes. Performing a leading-order renormalization group analysis in QCD from the W to the O(2 GeV) energy scale, we derive the pertinent effective Hamiltonian for hadronic parity violation, including the effects of both neutral and charged weak currents. We compute the complete renormalization group evolution of all isosectors and the evolution through heavy-flavor thresholds for the first time. We show that the additional four-quark operators that enter below the W mass scale from QCD operator mixing effects form a closed set, and they result in a 12 x 12 anomalous dimension matrix. Computing the resulting effective Hamiltonian and comparing to earlier results, we affirm the importance of operator mixing effects and find, as an example, that the parity-violating pion-nucleon coupling constant, using the factorization Ansatz and an assessment of the pertinent quark charge of the nucleon in lattice QCD at the 2 GeV scale, is in better agreement with recent experiments.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Effect of electron-to-ion mass ratio on radial electric field generation in tokamak

Generation of coherent radial electric fields in plasma by drift-wave turbulence driven by plasma inhomogeneities is ab initio studied using gyro-kinetic particle simulation for conditions of operational tokamaks. In particular, the effect of the electron-to-ion mass ratio epsilon on the entire evolution of the plasma is considered. In conclusion, it is found that the electric field can be increased, and the turbulence-induced particle transport reduced, by making epsilon smaller, in agreement with many existing experimental observations.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

ExaWind: A multifidelity modeling and simulation environment for wind energy

We introduce the open-source ExaWind modeling and simulation environment for wind energy. The primary physics codes of ExaWind are Nalu-Wind and OpenFAST. Nalu-Wind is a wind-focused computational fluid dynamics (CFD) code that is coupled to the whole-turbine simulation code OpenFAST. The ExaWind environment was created under U.S. Department of Energy funding to achieve the highest-fidelity simulations of wind turbines and wind farms to date, with the goal of enabling disruptive changes to turbine and plant design and operation. Innovation will be gleaned through better understanding of the complex flow dynamics in wind farms, including wake evolution and the impact of wakes on downstream turbines and turbulent flow from complex terrain. High-fidelity predictive simulations employ hybrid turbulence models, geometry/boundary-layer-resolving CFD meshes, atmospheric turbulence, nonlinear structural dynamics, and fluid-structure interaction. While there is an emphasis on very high-fidelity simulations (e.g., blade resolved with full fluid-structure coupling), the ExaWind environment supports lower-fidelity modeling capabilities including actuator-line and -disk methods. Important in the development of ExaWind codes is that the codes scale well on today's largest petascale supercomputers and on the next-generation platforms that will enable exascale computing.

17 WIND ENERGY↗

Quantum Hamiltonian algorithms for maximum independent sets

ABSTRACT We compare two quantum Hamiltonian algorithms that address the maximum independent set problem: one based on the emergent non-Abelian gauge matrix in adiabatic evolution of an energetically isolated manifold of states; the other based on designed application of single-qubit operations. We demonstrate that they are mathematically equivalent in the sense that one is the other’s interaction picture. Despite their mathematical equivalence, our numerical simulations show significant differences between them in performance, which is explained analytically. Intriguingly, this equivalence unveils that the PXP model, recently prominent in quantum dynamics research, can be viewed as quantum diffusion over the median graph of all independent sets governed by the non-Abelian gauge matrix.

Science & Technology - Other Topics↗

Robust Measurements of n -Point Correlation Functions of Driven-Dissipative Quantum Systems on a Digital Quantum Computer

We propose and demonstrate a unified hierarchical method to measure n -point correlation functions that can be applied to driven, dissipative, or otherwise open or nonequilibrium quantum systems. In this method, the time evolution of the system is repeatedly interrupted by interacting an ancilla qubit with the system through a controlled operation, and measuring the ancilla immediately afterward. We discuss the robustness of this method as compared to other ancilla-based interferometric techniques (such as the Hadamard test), and highlight its advantages for near-term quantum simulations of open quantum systems. We implement the method on a quantum computer in order to measure single-particle Green’s functions of a driven-dissipative fermionic system. This Letter shows that dynamical correlation functions for driven-dissipative systems can be robustly measured with near-term quantum computers. Published by the American Physical Society 2024

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Long-Term Monitoring the Damage Performance of Multilayer Dielectric Grating Samples Residing Inside the Compressor Chamber of the OMEGA EP Laser

Understanding of the laser-induced damage threshold and impact of air–vacuum cycling of the optical components in short-pulse laser systems is of fundamental importance. We report the results of a damage-testing campaign that monitored representative pulse compression grating samples that were positioned inside the OMEGA EP grating compressor vacuum chamber during normal operation and routinely damage tested on every quarterly vent for a period of about 10 years. Here, the evolution of their damage resistance under 10-ps and 100-ps pulse lengths are associated with a significant degradation of the laser-induced damage thresholds, which is comparatively larger at 100 ps, is described.

42 ENGINEERING↗

Special features of the inverse-beta-decay reaction proceeding on a proton in a reactor-antineutrino flux

The evolution of the reactor-antineutrino spectrum and the evolution of the spectrum of positrons from the inverse-beta-decay reaction in the course of reactor operation and after reactor shutdown are considered. The present-day status in determining the initial reactor-antineutrino spectrum on the basis of spectra of beta particles from mixtures of products originating from uranium and plutonium fission is described. A local rise of the experimental spectrum of reactor antineutrinos with respect to the expected spectrum is studied.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

A Concept of a Convection–Cloud Chamber to Study Aerosol–Cloud–Drizzle Interactions

Understanding and quantifying the full chain of processes from aerosol activation to drizzle formation, and the associated feedbacks to the aerosol chemical and physical properties, all within a turbulent cloud are some of the toughest challenges in atmospheric chemistry and physics and are keys to the cloud–precipitation puzzle. This paper describes a concept for a new type of research facility consisting of a cloud chamber plus associated instrumentation and computational models, to explore aerosol–cloud interactions and processing, cloud optical properties, entrainment–cloud interactions, and quantitative assessment of drizzle onset. The envisioned design is for a 3 m × 3 m × 9 m chamber, such that the height is sufficient to achieve long lifetimes for aerosol processing and for significant drizzle growth by collision and coalescence. A suite of computational tools for simulating microphysical properties in the chamber provides a digital twin for designing the chamber and a range of example experiments. Theory and test results from novel remote sensing systems for exploring chemical and physical interactions and evolution of aerosols, cloud droplets, and drizzle within turbulent clouds are described. Testing of technology needed for the operation of a large-volume chamber, including aerosol generation methods and novel materials for water vapor boundary conditions, is described. Simulations suggest that spatially uniform turbulence and microphysical properties can be sustained in a steady state, with reasonable aerosol and water vapor fluxes, and that substantial drizzle can be produced through collision and coalescence of cloud droplets. Remaining challenges for more detailed engineering design and a discussion of possible first-light experiments are described.

54 ENVIRONMENTAL SCIENCES↗

Nanostructure and burning mode of light-duty diesel particulate with conventional diesel, biodiesel, and intermediate blends

The nanostructure of diesel particulates has been shown to impact its oxidation rate and burnout trajectory. Additionally, this nanostructure can evolve during the oxidation process, furthering its influence on the burnout process. For this study, exhaust particulates were generated on a light-duty diesel engine with conventional diesel fuel, biodiesel, and intermediate blends of the two at a single load-speed point. Despite the singular engine platform and operating point, the different fuels created particulates with varied nanostructure, thereby greatly expanding the window for observing nanostructure evolution and oxidation. The physical and chemical properties of the particulates in the nascent state and at partial oxidation states were measured in a laboratory reactor and by high-resolution transmission electron microscopy as a function of the degree of oxidation in O 2 . X-ray photoacoustic spectroscopy analysis, thermal desorption, and solvent extraction of the nascent particulate samples reveal a significant organic content in the biodiesel-derived particulates, likely accounting for differences in the nanostructure. This study reports the nanoscale structural changes in the particulate with biofuel blend level and during O 2 oxidation as observed by high-resolution transmission electron microscopy and quantitated by fringe analysis and Brunnauer–Emmet–Teller total surface area measurements. It was observed that initial fuel-related differences in the lamella lengths, spacing, and curvature disappear when the particulate reaches approximately 50% burnout. Specifically, the initial ordered, fullerenic, and amorphous nanostructures converge during the oxidation process and the surface areas of these particulates appear to grow through these complex changes in internal particle structure. The specific surface area, measured at several points along the burnout trajectory, did not match the shrinking core projection and in contrast suggested that internal porosity was increasing. Thus, the appropriate burnout model for these particulates is significantly different from the standard shrinking core assumption, which does not account for any internal structure. An alternative burnout model is supported by high-resolution transmission electron microscopy image analysis.

33 ADVANCED PROPULSION SYSTEMS↗

Development and Commercialization of a Nanosegrated Oxygen Evolution Reaction Electrocatalyst

The research under this CRADA adds to the understanding of how catalyst activity and durability should be balanced and tailored for oxygen evolution reaction. The research also provides technical insights in how catalyst degradation might occur under long-term operation under highly oxidative and acidic conditions. In longer term, the project could benefit the pubic by enabling more efficient, affordable and reliable electrolysis technologies.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Earth-to-orbit transportation for solar power satellites

The cargo transport capability and the cost of space transportation operations for transportation of solar power satellites (SPS) to space are addressed. The history of SPS launch vehicle evolution is shown. Alternative vehicle designs developed include: (1) a parallel burn, crossfeed configuration; (2) single stage to orbit airbreathing/rocket runway takeoff vehicle concept; and (3) a smaller HLLV concept. The smaller HLLV was analyzed to compare the nonrecurring cost benefits of a less challenging development with the recurring cost increases expected due to losses in efficiency associated with smaller vehicle size. The vehicle payload bay size was selected to be adequate to accommodate the SPS transmitter subarrays fully assembled. The resulting vehicle design is compared with the shuttle, the Saturn V, and the reference SPS HLLV. A nonrecurring savings of at least five billion dollars was obtained with a recurring cost penalty of 3% per SPS. The environmental benefits of the small vehicle were deemed more important than the slight increase in upper atmosphere propellant deposition. It is recommended that the small HLLV be adopted as the SPS reference launch system.

Woodcock, G. R.↗

Space platforms

The expanded scientific capabilities available by interfacing an orbital, free-flying experiments platform with Shuttle tending are outlined. The platform would be lifted to orbit by the Shuttle, and modularly increased in size on subsequent flights. Science packages could be left on the 26,000 lb space platform for up to six months. Component sections would include electrical and thermal control systems, berthing ports for payloads and an Orbiter, and an attitude control, communications, and data handling subsection. A 12 kW solar array would furnish power, and interconnect with Spacelab would further enhance the operations range. All berthed science packages would have individual pointing ability and grapples for the Orbiter RMS. Eventual evolution to include facilities for a human crew and a 25 kW solar array is projected.

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