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At least 1,189 records · Page 66

Characterization and Application of a Hybrid Optical Microscopy/Laser Ablation Liquid Vortex Capture/Electrospray Ionization System for Mass Spectrometry Imaging with Sub-micrometer Spatial Resolution

Herein, a commercial optical microscope, laser microdissection instrument was coupled with an electrospray ionization mass spectrometer via a low profile liquid vortex capture probe to yield a hybrid optical microscopy/mass spectrometry imaging system. The instrument has bright-field and fluorescence microscopy capabilities in addition to a highly focused UV laser beam that is utilized for laser ablation of samples. With this system, material laser ablated from a sample using the microscope was caught by a liquid vortex capture probe and transported in solution for analysis by electrospray ionization mass spectrometry. Both lane scanning and spot sampling mass spectral imaging modes were used. The smallest area the system was able to ablate was ~0.544 μm × ~0.544 μm, achieved by oversampling of the smallest laser ablation spot size that could be obtained (~1.9 μm). With use of a model photoresist surface, known features as small as ~1.5 μm were resolved. The capabilities of the system with real world samples were demonstrated first with a blended polymer thin film containing poly(2-vinylpyridine) and poly(N-vinylcarbazole). Using spot sampling imaging, sub-micrometer sized features (0.62, 0.86, and 0.98 μm) visible by optical microscopy were clearly distinguished in the mass spectral images. A second real world example showed the imaging of trace amounts of cocaine in mouse brain thin tissue sections. Lastly, with use of a lane scanning mode with ~6 μm × ~6 μm data pixels, features in the tissue as small as 15 μm in size could be distinguished in both the mass spectral and optical images.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Higher‐Order Gravity Waves and Traveling Ionospheric Disturbances From the Polar Vortex Jet on 11–15 January 2016: Modeling With HIAMCM‐SAMI3 and Comparison With Observations in the Thermosphere and Ionosphere

Abstract In Vadas et al. (2024, https://doi.org/10.1029/2024ja032521 ), we modeled the atmospheric gravity waves (GWs) during 11–14 January 2016 using the HIAMCM, and found that the polar vortex jet generates medium to large‐scale, higher‐order GWs in the thermosphere. In this paper, we model the traveling ionospheric disturbances (TIDs) generated by these GWs using the HIAMCM‐SAMI3 and compare with ionospheric observations from ground‐based Global Navigation Satellite System (GNSS) receivers, Incoherent Scatter Radars (ISR) and the Super Dual Auroral Radar Network (SuperDARN). We find that medium to large‐scale TIDs are generated worldwide by the higher‐order GWs from this event. Many of the TIDs over Europe and Asia have concentric ring/arc‐like structure, and most of those over North/South America have planar wave structure and occur during the daytime. Those over North/South America propagate southward and are generated by higher‐order GWs from Europe/Asia which propagate over the Arctic. These latter TIDs can be misidentified as arising from geomagnetic forcing. We find that the higher‐order GWs that propagate to Africa and Brazil from Europe may aid in the formation of equatorial plasma bubbles (EPBs) there. We find that the simulated GWs, TIDs and EPBs agree with EISCAT, PFISR, GNSS, and SuperDARN measurements. We find that the higher‐order GWs are concentrated at N at 200 km, in agreement with GOCE and CHAMP data. Thus the polar vortex jet is important for generating TIDs in the northern winter ionosphere via multi‐step vertical coupling through GWs.

Vadas, Sharon L. [Northwest Research Associates Bo↗

Rayleigh instability of confined vortex droplets in critical superconductors

Depending on the Ginzburg-Landau material parameter , superconductors can either be fully diamagnetic if k < 1√2 (type I superconductors) or accommodate magnetic field in the form of Abrikosov vortices if k > 1√2 (type II superconductors).1,2 At Bogomolny critical point, k = kc = 1 √2, a state, infinitely degenerated with respect to vortex spatial configurations, arises.3,4 While conventional type I and type II superconductors are investigated in depth, a thorough understanding of magnetic behaviour in the near-Bogomolny critical regime at k ~ kc is still lacking. Here we report that in restricted systems the critical regime expands over a finite interval of k forming critical superconducting state. We show that in this state, in a sample with dimensions comparable with the vortex core size, vortices merge into a multi-quanta droplet, which undergoes Rayleigh instability5 upon increasing k and decays by emitting single vortices. Superconducting vortices materialize Nielsen-Olesen singular solutions of the Abelian Higgs model pervasive in phenomena ranging from quantum electrodynamics to cosmology.6,7,8,9 Our work, revealing transient dynamics of Abrikosov-Nielsen-Olesen vortices in systems with boundaries, promises access to novel effects in quantum field theory via bench-top laboratory experiments.

Lukyanchuk, I.↗

Spatially and spectrally resolved orbital angular momentum interactions in plasmonic vortex generators

Abstract Understanding the near-field electromagnetic interactions that produce optical orbital angular momentum (OAM) is crucial for integrating twisted light into nanotechnology. Here, we examine the cathodoluminescence (CL) of plasmonic vortices carrying OAM generated in spiral nanostructures. The nanospiral geometry defines a photonic local density of states that is sampled by the electron probe in a scanning transmission electron microscope (STEM), thus accessing the optical response of the plasmonic vortex with high spatial and spectral resolution. We map the full spectral dispersion of the plasmonic vortex in spiral structures designed to yield increasing topological charge. Additionally, we fabricate nested nanospirals and demonstrate that OAM from one nanospiral can be coupled to the nested nanospiral, resulting in enhanced luminescence in concentric spirals of like handedness with respect to concentric spirals of opposite handedness. The results illustrate the potential for generating and coupling plasmonic vortices in chiral nanostructures for sensitive detection and manipulation of optical OAM.

36 MATERIALS SCIENCE↗

Ultrastrong magnon-magnon coupling and chiral spin-texture control in a dipolar 3D multilayered artificial spin-vortex ice

Strongly-interacting nanomagnetic arrays are ideal systems for exploring reconfigurable magnonics. They provide huge microstate spaces and integrated solutions for storage and neuromorphic computing alongside GHz functionality. These systems may be broadly assessed by their range of reliably accessible states and the strength of magnon coupling phenomena and nonlinearities. Increasingly, nanomagnetic systems are expanding into three-dimensional architectures. This has enhanced the range of available magnetic microstates and functional behaviours, but engineering control over 3D states and dynamics remains challenging. Here, we introduce a 3D magnonic metamaterial composed from multilayered artificial spin ice nanoarrays. Comprising two magnetic layers separated by a non-magnetic spacer, each nanoisland may assume four macrospin or vortex states per magnetic layer. This creates a system with a rich 16 N microstate space and intense static and dynamic dipolar magnetic coupling. The system exhibits a broad range of emergent phenomena driven by the strong inter-layer dipolar interaction, including ultrastrong magnon-magnon coupling with normalised coupling rates of $\frac{Δf}{v}$ = 0.57, GHz mode shifts in zero applied field and chirality-control of magnetic vortex microstates with corresponding magnonic spectra.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Vortex entropy and superconducting fluctuations in ultrathin underdoped Bi 2 Sr 2 CaCu 2 O 8+x superconductor

Vortices in superconductors can help identify emergent phenomena but certain fundamental aspects of vortices, such as their entropy, remain poorly understood. Here, we study the vortex entropy in underdoped Bi 2 Sr 2 CaCu 2 O 8+x by measuring both magneto-resistivity and Nernst effect on ultrathin flakes (≤2 unit-cell). We extract the London penetration depth from the magneto-transport measurements on samples with different doping levels. It reveals that the superfluid phase stiffness p s scales linearly with the superconducting transition temperature T c , down to the extremely underdoped case. On the same batch of ultrathin flakes, we measure the Nernst effect via on-chip thermometry. Together, we obtain the vortex entropy and find that it decays exponentially with T c or p s . We further analyze the Nernst signal above T c in the framework of Gaussian superconducting fluctuations. The combination of electrical and thermoelectric measurements in the two-dimensional limit provides fresh insight into high temperature superconductivity.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Geometrically stabilized skyrmionic vortex in FeGe tetrahedral nanoparticles

The concept of topology has dramatically expanded the research landscape of magnetism, leading to the discovery of numerous magnetic textures with intriguing topological properties. A magnetic skyrmion is an emergent topological magnetic texture with a string-like structure in three dimensions and a disk-like structure in one and two dimensions. Skyrmions in zero dimensions have remained elusive due to challenges from many competing orders. Here, by combining electron holography and micromagnetic simulations, we uncover the real-space magnetic configurations of a skyrmionic vortex structure confined in a B20-type FeGe tetrahedral nanoparticle. An isolated skyrmionic vortex forms at the ground state and this texture shows excellent robustness against temperature without applying a magnetic field. Furthermore, our findings shed light on zero-dimensional geometrical confinement as a route to engineer and manipulate individual skyrmionic metastructures.

36 MATERIALS SCIENCE↗

Half-integer level shift of vortex bound states in an iron-based superconductor

Vortices in topological superconductors host Majorana zero modes (MZMs), which are proposed to be building blocks of fault-tolerant topological quantum computers. Recently, a new single-material platform for realizing MZM has been discovered in iron-based superconductors, without involving hybrid semiconductor-superconductor structures. Here we report on a detailed scanning tunneling spectroscopy study of a FeTe 0.55 Se 0.45 single crystal, revealing two distinct classes of vortices present in this system which differ by a half-integer level shift in the energy spectra of the vortex bound states. This level shift is directly tied with the presence or absence of zero-bias peak and also alters the ratios of higher energy levels from integer to half-odd-integer. Our model calculations fully reproduce the spectra of these two types of vortex bound states, suggesting the presence of topological and conventional superconducting regions that coexist within the same crystal. Our findings provide strong evidence for the topological nature of superconductivity in FeTe 0.55 Se 0.45 and establish it as an excellent platform for further studies on MZMs.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Current-driven production of vortex-antivortex pairs in planar Josephson junction arrays and phase cracks in long-range order

Proliferation of topological defects like vortices and dislocations plays a key role in the physics of systems with long-range order, particularly, superconductivity and superfluidity in thin films, plasticity of solids, and melting of atomic monolayers. Topological defects are characterized by their topological charge reflecting fundamental symmetries and conservation laws of the system. Conservation of topological charge manifests itself in extreme stability of static topological defects because destruction of a single defect requires overcoming a huge energy barrier proportional to the system size. However, the stability of driven topological defects remains largely unexplored. Here we address this issue and investigate numerically a dynamic instability of moving vortices in planar arrays of Josephson junctions. We show that a single vortex driven by sufficiently strong current becomes unstable and destroys superconductivity by triggering a chain reaction of self-replicating vortex-antivortex pairs forming linear of branching expanding patterns. Furthermore this process can be described in terms of propagating phase cracks in long-range order with far-reaching implications for dynamic systems of interacting spins and atoms hosting magnetic vortices and dislocations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Jamming, fragility and pinning phenomena in superconducting vortex systems

Abstract We examine driven superconducting vortices interacting with quenched disorder under a sequence of perpendicular drive pulses. As a function of disorder strength, we find four types of behavior distinguished by the presence or absence of memory effects. The fragile and jammed states exhibit memory, while the elastic and pinning dominated regimes do not. In the fragile regime, the system organizes into a pinned state during the first pulse, flows during the second perpendicular pulse, and then returns to a pinned state during the third pulse which is parallel to the first pulse. This behavior is the hallmark of the fragility proposed for jamming in particulate matter. For stronger disorder, we observe a robust jamming state with memory where the system reaches a pinned or reduced flow state during the perpendicular drive pulse, similar to the shear jamming of granular systems. We show signatures of the different states in the spatial vortex configurations, and find that memory effects arise from coexisting elastic and pinned components of the vortex assembly. The sequential perpendicular driving protocol we propose for distinguishing fragile, jammed, and pinned phases should be general to the broader class of driven interacting particles in the presence of quenched disorder.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

A new reversal mode in exchange coupled antiferromagnetic/ferromagnetic disks: distorted viscous vortex

Magnetic vortices have generated intense interest in recent years due to their unique reversal mechanisms, fascinating topological properties, and exciting potential applications. In addition, the exchange coupling of magnetic vortices to antiferromagnets has also been shown to lead to a range of novel phenomena and functionalities. Here we report a new magnetization reversal mode of magnetic vortices in exchange coupled Ir 20 Mn 80 /Fe 20 Ni 80 microdots: distorted viscous vortex reversal. In contrast to the previously known or proposed reversal modes, the vortex is distorted close to the interface and viscously dragged due to the uncompensated spins of a thin antiferromagnet, which leads to unexpected asymmetries in the annihilation and nucleation fields. Lastly, these results provide a deeper understanding of the physics of exchange coupled vortices and may also have important implications for applications involving exchange coupled nanostructures.

36 MATERIALS SCIENCE↗

Center vortex model and the G(2) gauge group

The thick center vortex model is applied to G(2) gauge group to obtain the potentials between static sources of the fundamental and adjoint representations. The group G(2) has only one trivial center element and therefore it does not have any vortices which are defined based on non trivial center elements. To obtain the potential from the thick center vortex model, the idea of the vacuum domain structure is used. The intermediate string tensions from this model are in rough agreement with the G(2) lattice results and the Casimir ratio. We argue that the SU(3) subgroup of G(2) may be responsible for the linear potential at the intermediate distances.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Evaluation of vortex pinning across low angle grain boundary in YBa{sub 2}Cu{sub 3}O{sub 7} film

Vortex pinning potential across a 5 Degree-Sign tilt low angle grain boundary (GB) was evaluated by measuring angular dependences of critical current density in a bicrystal YBa{sub 2}Cu{sub 3}O{sub 7} film under the variable Lorentz force configuration. Trapping angles of the GB depend on directions in the GB plane (70 Degree-Sign -80 Degree-Sign and 15 Degree-Sign -45 Degree-Sign for the c-axis direction and the ab plane one, respectively), due to anisotropic pinning of GB dislocations. Pinning potential across a GB is as large as that of heavy ion irradiated columnar defects, indicating that density and distribution of GBs should be controlled to improve vortex pinning in coated conductors.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Femtosecond laser fabrication of micro and nano-disks in single layer graphene using vortex Bessel beams

We report the fabrication of micro and nano-disks in single layer chemical vapor deposition graphene on glass substrate using femtosecond laser ablation with vortex Bessel beams. The fabricated graphene disks with diameters ranging from 650 nm to 4 μm were characterized by spatially resolved micro-Raman spectroscopy. The variation of ablation threshold was investigated as a function of the number of pulses showing an incubation effect. A very high degree of size control of the fabricated graphene disks is enabled using a sequence of femtosecond pulses with different vortex orders.

36 MATERIALS SCIENCE↗

Spin-wave spectra and stability of the in-plane vortex state in two-dimensional magnetic nanorings

We study theoretically two-dimensional nanorings assumed to have the in-plane vortex magnetic configuration. Using a discrete dipole model we examine the spectrum of normal spin-wave modes vs. the dipolar-to-exchange interaction ratio. We systematize the spin-wave excitations by their azimuthal and radial wave numbers. The lowest-frequency mode, the fundamental (quasiuniform) mode, and the mode hybridization are analyzed; the discussion of the influence of effective pinning at the ring boundaries is provided as well. We study the stability of the in-plane vortex state and discuss the role of the size of the ring and the type of lattice arrangement of the magnetic moments within it. To facilitate comparison with our results we provide the relationships between microscopic parameters, used in our model, and those used in the case of continuous medium.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Comment on “Motion of a helical vortex filament in superfluid {sup 4}He under the extrinsic form of the local induction approximation” [Phys. Fluids 25, 085101 (2013)]

We comment on the paper by Van Gorder [“Motion of a helical vortex filament in superfluid {sup 4}He under the extrinsic form of the local induction approximation,” Phys. Fluids 25, 085101 (2013)]. We point out that the flow of the normal fluid component parallel to the vortex will often lead into the Donnelly–Glaberson instability, which will cause the amplification of the Kelvin wave. We explain why the comparison to local nonlinear equation is unreasonable, and remark that neglecting the motion in the x-direction is not reasonable for a Kelvin wave with an arbitrary wavelength and amplitude. The correct equations in the general case are also derived.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Experimental investigation of magnetic anisotropy in spin vortex discs

We present experimental 2D vector vibrating sample magnetometer measurements to demonstrate the shape anisotropy effects occurring in micrometer-diameter supermalloy spin vortex discs. Measurements made for different disc sizes and orientations confirm the out-of-plane susceptibility is several orders of magnitude smaller than the in-plane susceptibility. These results validate with a high certitude that spin vortices with high diameter to thickness ratio retain in-plane-only magnetization, even when subjected to fields in the out-of-plane direction. These results contribute to further computational simulations of the dynamics of spin vortex structures in colloidal suspensions where external fields may be applied in any arbitrary direction.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Local modification of the magnetic vortex-core velocity by gallium implantation

The dynamics of magnetic vortices in microsquares with local modifications of magnetic parameters and thickness are investigated. By implanting gallium ions with focussed ion beam into permalloy thin-film elements, we have locally tailored their magnetic properties and the layer thickness. The vortex of the Landau domain pattern of a square is resonantly excited to a gyrotropic motion and crosses regions with and without implantation. With time-resolved scanning transmission x-ray microscopy, we observe an abrupt change in the vortex velocity close to the borders between the two regions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗