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At least 1,207 records · Page 67

Laser-Induced Incandescence in Microgravity

Knowledge of soot concentration is important due to its presence and impact upon a wide range of combustion processes ranging from diffusion to premixed flames, laminar to turbulent processes and homogeneous to heterogeneous combustion. Measurement of soot volume fraction (f(sub v)) is essential to discerning its formation and growth. The presence of soot also affects other physical and chemical properties of combustion thereby affecting studies not directly concerned with either its formation or growth, such as radiative heat transfer, CO oxidation and fuel vaporization or pyrolysis rates. Microgravity offers unique opportunities for studying both soot growth and the effect of soot radiation upon flame structure and spread. Spatial scales and residence time scales are greatly extended in 0-g facilitating soot growth studies. With the varied geometries, short duration microgravity test times and time-varying processes there is a demand for measurement of f(sub v) with high spatial and temporal resolution. Laser-induced incandescence (LII) has advanced f(sub v) measurements in many 1-g combustion processes. To create laser-induced incandescence, a pulsed high intensity laser heats soot to incandescence temperatures. Using appropriate spectral and temporal detection conditions, the resulting incandescence can be selectively detected apart from the non-laser-heated soot and flame gases. Theoretical modelling and experiments have shown that the resulting incandescence is representative of f(sub v). Using an intensified array camera and a laser sheet for excitation, one- and two-dimensionally resolved LII images of f(sub v) have been obtained in 1-g. LII has been characterized and developed at NASA-Lewis for soot volume fraction determination in a wide range of 1-g combustion applications. Broadly grouped, the characterization work has included studies of excitation intensity, excitation wavelength and the optimum temporal and spectral detection conditions to enable an accurate representation of soot volume fraction by LII. Tests for special requirements imposed by different combustion processes have been performed in laminar and turbulent diffusion flames, rich sooting premixed flames, single droplet combustion, and other heterogeneous combustion. These studies demonstrated LII's high sensitivity, temporal and spatial capabilities and its geometric versatility. In contrast to the advantages offered to combustion studies by a microgravity environment, advanced diagnostics, specifically those requiring pulsed laser diagnostics have been limited due to the size, weight and power limitations in a low-gravity environment. Reported here are the first demonstrations of LII performed in a microgravity environment. Examples are shown for laminar and turbulent gas-jet diffusion flames in 0-g.

VanderWal, Randy L.↗

High-Performance Simulation of Dynamic Hydrologic Exchange and Implications for Surrogate Flow and Reactive Transport Modeling in a Large River Corridor

Hydrologic exchange flows (HEFs) have environmental significance in riverine ecosystems. Key river channel factors that influence the spatial and temporal variations of HEFs include river stage, riverbed morphology, and riverbed hydraulic conductivity. However, their impacts on HEFs were often evaluated independently or on small scales. In this study, we numerically evaluated the combined interactions of these factors on HEFs using a high-performance simulator, PFLOTRAN, for subsurface flow and transport. The model covers 51 square kilometers of a selected river corridor with large sinuosity along the Hanford Reach of the Columbia River in Washington, US. Three years of spatially distributed hourly river stages were applied to the riverbed. Compared to the simulation when riverbed heterogeneity is not ignored, the simulation using homogeneous riverbed conductivity underestimated HEFs, especially upwelling from lateral features, and overestimated the mean residence times derived from particle tracking. To derive a surrogate model for the river corridor, we amended the widely used transient storage model (TSM) for riverine solute study at reach scale with reactions. By treating the whole river corridor as a batch reactor, the temporal changes in the exchange rate coefficient for the TSM were derived from the dynamic residence time estimated from the hourly PFLOTRAN results. The TSM results were evaluated against the effective concentrations in the hyporheic zone calculated from the PFLOTRAN simulations. Our results show that there is potential to parameterize surrogate models such as TSM amended with biogeochemical reactions while incorporating small-scale process understandings and the signature of time-varying streamflow to advance the mechanistic understanding of river corridor processes at reach to watershed scales. However, the assumption of a well-mixed storage zone for TSM should be revisited when redox-sensitive reactions in the storage zones play important roles in river corridor functioning.

Fang, Yilin↗

Observation of Absorbing Aerosols Above Clouds over the South-East Atlantic Ocean from the Geostationary Satellite SEVIRI – Part 1: Method Description and Sensitivity

High temporal resolution observations from satellites have a great potential for studying the impact of biomass burning aerosols and clouds over the South East Atlantic Ocean (SEAO). This paper presents a method developed to retrieve simultaneously aerosol and cloud properties in aerosol above cloud conditions from the geostationary instrument Meteosat Second Generation/Spinning Enhanced Visible and Infrared Imager (MSG/SEVIRI). The above-cloud Aerosol Optical Thickness (AOT), the Cloud Optical Thickness (COT) and the Cloud droplet Effective Radius (CER) are derived from the spectral contrast and the magnitude of the signal measured in three channels in the visible to shortwave infrared region. The impact of the absorption from atmospheric gases on the satellite signal is corrected by applying transmittances calculated using the water vapour profiles from a Met Office forecast model. The sensitivity analysis shows that a 10% error on the humidity profile leads to an 18.5% bias on the above-cloud AOT, which highlights the importance of an accurate atmospheric correction scheme. In situ measurements from the CLARIFY-2017 airborne field campaign are used to constrain the aerosol size distribution and refractive index that is assumed for the aforementioned retrieval algorithm. The sensitivities in the retrieved AOT, COT and CER to the aerosol model assumptions are assessed. Between 09:00-15:00 UTC, an uncertainty of 40% is estimated on the above-cloud AOT, which is dominated by the sensitivity of the retrieval to the single scattering albedo. The absorption AOT is less sensitive to the aerosol assumptions with an uncertainty generally lower than 17% between 09:00-15:00 UTC. Outside of that time range, as the scattering angle decreases, the sensitivity of the AOT and the absorption AOT to the aerosol model increases. The retrieved cloud properties are only weakly sensitive to the aerosol model assumptions throughout the day, with biases lower than 6% on the COT and 3% on the CER. The stability of the retrieval over time is analysed. For observations outside of the backscattering glory region, the time-series of the aerosol and cloud properties are physically consistent, which confirms the ability of the retrieval to monitor the temporal evolution of aerosol above cloud events over the SEAO.

Peers, Fanny↗

Observation of absorbing aerosols above clouds over the south-east Atlantic Ocean from the geostationary satellite SEVIRI – Part 1: Method description and sensitivity

High-temporal-resolution observations from satellites have a great potential for studying the impact of biomass burning aerosols and clouds over the south-east Atlantic Ocean (SEAO). This paper presents a method developed to simultaneously retrieve aerosol and cloud properties in aerosol above-cloud conditions from the geostationary instrument Meteosat Second Generation/Spinning Enhanced Visible and Infrared Imager (MSG/SEVIRI). The above-cloud aerosol optical thickness (AOT), the cloud optical thickness (COT) and the cloud droplet effective radius (CER) are derived from the spectral contrast and the magnitude of the signal measured in three channels in the visible to shortwave infrared region. The impact of the absorption from atmospheric gases on the satellite signal is corrected by applying transmittances calculated using the water vapour profiles from a Met Office forecast model. The sensitivity analysis shows that a 10 % error on the humidity profile leads to an 18.5 % bias on the above-cloud AOT, which highlights the importance of an accurate atmospheric correction scheme. In situ measurements from the CLARIFY-2017 airborne field campaign are used to constrain the aerosol size distribution and refractive index that is assumed for the aforementioned retrieval algorithm. The sensitivities in the retrieved AOT, COT and CER to the aerosol model assumptions are assessed. Between 09:00 and 15:00 UTC, an uncertainty of 40 % is estimated on the above-cloud AOT, which is dominated by the sensitivity of the retrieval to the single-scattering albedo. The absorption AOT is less sensitive to the aerosol assumptions with an uncertainty generally lower than 17 % between 09:00 and 15:00 UTC. Outside of that time range, as the scattering angle decreases, the sensitivity of the AOT and the absorption AOT to the aerosol model increases. The retrieved cloud properties are only weakly sensitive to the aerosol model assumptions throughout the day, with biases lower than 6 % on the COT and 3 % on the CER. The stability of the retrieval over time is analysed. For observations outside of the backscattering glory region, the time series of the aerosol and cloud properties are physically consistent, which confirms the ability of the retrieval to monitor the temporal evolution of aerosol above-cloud events over the SEAO.

cloud properties↗

Factors influencing the temporal growth rate of the high order TM{sub 0n} modes in the Ka-band overmoded Cherenkov oscillator

When the wavelength of overmoded Cherenkov oscillator goes into Ka-band, power handling capacity becomes an essential issue. Using the TM{sub 02} mode or higher order TM{sub 0n} modes as the operating mode is a potential solution. This paper is aimed to find some proper parameters to make the temporal growth rate of the TM{sub 02} mode higher in our previously studied Gigawatt (GW)-class Ka band oscillator. An accurate and fast calculation method of the “hot” dispersion equation is derived for rectangular corrugated SWSs, which are widely used in the high frequency Cherenkov devices. Then, factors that affect the temporal growth rate of the high order TM{sub 0n} modes are analyzed, including the depth of corrugation, the radius of drift tube, and the diode voltage. Results show that, when parameters are chosen properly, the temporal growth rate of the TM{sub 02} mode can be as high as 0.3 ns{sup −1}.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

Compression of femtosecond ytterbium fibre laser pulses using nonlinear processes in silica fibre

The temporal compression of 100-fs nanojoule laser pulses using nonlinear processes in silica fibre has been studied by numerical simulation and experimentally. The simulation results demonstrate that, in the case of spectral broadening in a normal dispersion fibre, followed by the temporal compression of the pulse in a compressor with a negative second-order dispersion, up to 90 % of the compressed pulse energy can be concentrated in the main peak, whose duration is a factor of 8 shorter than the initial laser pulse duration. In our experiments, 100-fs ytterbium fibre laser pulses have been compressed to pulses with an ∼13-fs main peak accounting for 87 % of the compressed pulse energy. At an average ytterbium laser output power of 4.2 W, the average power at the compressor output has been 3.1 W. (paper)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Learning Temporal and Spatial Correlations Jointly: A Unified Framework for Wind Speed Prediction

Leveraging both temporal and spatial correlations to predict wind speed remains one of the most challenging and less studied areas of wind speed prediction. In this paper, the problem of predicting wind speeds for multiple sites is investigated by using the spatio-temporal correlation. We proposed a deep architecture termed predictive spatio-temporal network (PSTN), which is a unified framework integrating a convolutional neural network (CNN) and a long short-term memory (LSTM). Initially, the spatial features are extracted from the spatial wind speed matrices (SWSMs) by the CNN at the bottom of the model. Then, the LSTM captures the temporal dependencies among the spatial features extracted from contiguous time points. Lastly, the predicted wind speeds are given by the last state of the top layer of the LSTM, which are generated by using the spatial features and temporal dependencies. Though composed of two kinds of architectures, PSTN is trained with one loss function in an end-to-end (E2E) manner, which can learn temporal and spatial correlations jointly. Experiments for short-term predictions are conducted on real-world data, whose results demonstrate that PSTN outperforms prior methods.

42 ENGINEERING↗

On the Feasibility of Studying Shortwave Aerosol Radiative Forcing of Climate Using Dual-Wavelength Aerosol Backscatter Lidar

The current low confidence in the estimates of aerosol-induced perturbations of Earth's radiation balance is caused by the highly non-uniform compositional, spatial and temporal distributions of tropospheric aerosols on a global scale owing to their heterogeneous sources and short lifetimes. Nevertheless, recent studies have shown that the inclusion of aerosol effects in climate model calculations can improve agreement with observed spatial and temporal temperature distributions. In light of the short lifetimes of aerosols, determination of their global distribution with space-borne sensors seems to be a necessary approach. Until recently, satellite measurements of tropospheric aerosols have been approximate and did not provide the full set of information required to determine their radiative effects. With the advent of active aerosol remote sensing from space (e.g., PICASSO-CENA), the applicability fo lidar-derived aerosol 180 deg -backscatter data to radiative flux calculations and hence studies of aerosol effects on climate needs to be investigated.

Redemann, Jens↗

Bayesian inference and predictive performance of soil respiration models in the presence of model discrepancy

Bayesian inference of microbial soil respiration models is often based on the assumptions that the residuals are independent (i.e., no temporal or spatial correlation), identically distributed (i.e., Gaussian noise), and have constant variance (i.e., homoscedastic). In the presence of model discrepancy, as no model is perfect, this study shows that these assumptions are generally invalid in soil respiration modeling such that residuals have high temporal correlation, an increasing variance with increasing magnitude of CO 2 efflux, and non-Gaussian distribution. Relaxing these three assumptions stepwise results in eight data models. Data models are the basis of formulating likelihood functions of Bayesian inference. This study presents a systematic and comprehensive investigation of the impacts of data model selection on Bayesian inference and predictive performance. We use three mechanistic soil respiration models with different levels of model fidelity (i.e., model discrepancy) with respect to the number of carbon pools and the explicit representations of soil moisture controls on carbon degradation; therefore, we have different levels of model complexity with respect to the number of model parameters. The study shows that data models have substantial impacts on Bayesian inference and predictive performance of the soil respiration models such that the following points are true: (i) the level of complexity of the best model is generally justified by the cross-validation results for different data models; (ii) not accounting for heteroscedasticity and autocorrelation might not necessarily result in biased parameter estimates or predictions, but will definitely underestimate uncertainty; (iii) using a non-Gaussian data model improves the parameter estimates and the predictive performance; and (iv) accounting for autocorrelation only or joint inversion of correlation and heteroscedasticity can be problematic and requires special treatment. Although the conclusions of this study are empirical, the analysis may provide insights for selecting appropriate data models for soil respiration modeling.

58 GEOSCIENCES↗

EPR Investigation of Temporal and Thermal Stability of Irradiated Sweeteners

Abstract Electron paramagnetic resonance was used to study the dosimetric properties of commercial sweeteners (sucrose, saccharin, and stevia). The results concluded that sugar has dosimetric properties of interest, which makes it suitable for dose reconstruction, emergency response, and nuclear forensics applications. The radiation dose response was investigated by irradiating samples up to 10 Gy and found to be linear. The post-irradiation stability of samples was observed to be useful for the intended applications. The results showed that the post-irradiation intensities vary from one sample to another, with the general trend demonstrating a small increase in intensities shortly after irradiation followed by an approximately constant leveling out. Finally, the effect of isochronal annealing was studied by heating samples to various temperatures. The results showed an overall stable behavior of the signal below melting temperature.

Environmental Sciences & Ecology↗

Active Raman sounding of the earth's water vapor field

The typically weak cross-sections characteristic of Raman processes has historically limited their use in atmospheric remote sensing to nighttime application. However, with advances in instrumentation and techniques, it is now possible to apply Raman lidar to the monitoring of atmospheric water vapor, aerosols and clouds throughout the diurnal cycle. Upper tropospheric and lower stratospheric measurements of water vapor using Raman lidar are also possible but are limited to nighttime and require long integration times. However, boundary layer studies of water vapor variability can now be performed with high temporal and spatial resolution. This paper will review the current state-of-the-art of Raman lidar for high-resolution measurements of the atmospheric water vapor, aerosol and cloud fields. In particular, we describe the use of Raman lidar for mapping the vertical distribution and variability of atmospheric water vapor, aerosols and clouds throughout the evolution of dynamic meteorological events. The ability of Raman lidar to detect and characterize water in the region of the tropopause and the importance of high-altitude water vapor for climate-related studies and meteorological satellite performance are discussed.

Earth (Planet)↗

Influence of liquid conductance on the temporal evolution of self-organization patterns in atmospheric pressure DC glow discharges

Abstract Self-Organized Patterns (SOPs) at plasma-liquid interface in atmospheric pressure plasma discharges refer to the formation of intricate and puzzling structures due to the interplay of electrodynamic and hydrodynamic processes. Studies conducted to date have shown that this phenomenon results in the formation of distinctive patterns such as circular ring, star, gear, dots, spikes, etc., and primarily depends on working gas, electrolyte type, gap distance, current, conductivity, etc. However, an adequate understanding of how these patterns change from one type to another is still not available. This study aims to elucidate the influence of initial liquid conductance ( σ i ) on the temporal evolution of SOPs in liquid-anode discharges. The discharge was generated in a pin-to-liquid anode configuration at a constant helium (He) flow rate of 500 sccm and DC applied voltage of 6 kV at a gap distance of 12 mm. Through the gradual increment of σ i from 1.8 μ S to 4820 μ S, we observe that the trend in the evolution of SOPS takes place as solid discs, spikes, dots, rings, double rings, and stars. The continuous formation of reactive species onto the liquid anode in all conductive solutions results in a decrease in pH, an increase in bulk liquid temperature, and an increase in total dissolved solutes, and these have been confirmed through experimental measurements. Observations using optical emission spectroscopy show that the electrons at the plasma-liquid interface participate in the reduction of cations followed by their excitation & ionization due to which electron density as well as emissions from excited species (mainly hydroxyl radicals & excited nitrogen) decrease with time. Our investigation provides experimental evidence on the presence of cations at the plasma-liquid interface required for SOP formation.

Physics↗

WMLES for the Fifth High-Lift PredictionWorkshop Cases Using FUN3D

This paper presents solution assessments and grid convergence studies for the test cases outlined in the Fifth High-Lift Prediction Workshop (HLPW-5), focusing on the high-lift Common Research Models (CRM-HL). The study utilizes a wall-modeled large-eddy simulation (WMLES) methodology developed in the unstructured-grid, node-centered flow solver FUN3D. The second-order accurate simulations conducted in this study utilize a finite-volume spatial discretization and an implicit temporal scheme. Large-scale turbulent features are resolved away from the wall, with small-scale effects captured by the Vreman subgrid-scale model. An equilibrium wall function uses the first grid point off the wall serving as the critical interface between the wall model and the large-eddy simulation region, thus requiring careful placement in grid design. WMLES solutions are assessed for HLPW-5 cases, including a clean wing-body configuration and geometry-buildup configurations corresponding to the 5.1\% ONERA CRM-HL model. Grid-convergence studies are systematically conducted using uniformly refined grids. Moreover, simulation results and grid sensitivity are presented for the NASA 5.2\% CRM-HL configuration at both moderate and flight-scale Reynolds numbers. Overall, WMLES results are satisfactory and agree well with available experimental data, especially on sufficiently fine grids.

high-lift aerodynamics↗

Detecting Change in Urban Areas at Continental Scales with MODIS Data

Urbanization is one of the most important components of global environmental change, yet most of what we know about urban areas is at the local scale. Remote sensing of urban expansion across large areas provides information on the spatial and temporal patterns of growth that are essential for understanding differences in socioeconomic and political factors that spur different forms of development, as well the social, environmental, and climatic impacts that result. However, mapping urban expansion globally is challenging: urban areas have a small footprint compared to other land cover types, their features are small, they are heterogeneous in both material composition and configuration, and the form and rates of new development are often highly variable across locations. Here we demonstrate a methodology for monitoring urban land expansion at continental to global scales using Moderate Resolution Imaging Spectroradiometer (MODIS) data. The new method focuses on resolving the spectral and temporal ambiguities between urban/non-urban land and stable/changed areas by: (1) spatially constraining the study extent to known locations of urban land; (2) integrating multitemporal data from multiple satellite data sources to classify c. 2010 urban extent; and (3) mapping newly built areas (2000-2010) within the 2010 urban land extent using a multi-temporal composite change detection approach based on MODIS 250 m annual maximum enhanced vegetation index (EVI). We test the method in 15 countries in East-Southeast Asia experiencing different rates and manifestations of urban expansion. A two-tiered accuracy assessment shows that the approach characterizes urban change across a variety of socioeconomic/political and ecological/climatic conditions with good accuracy (70-91% overall accuracy by country, 69-89% by biome). The 250 m EVI data not only improve the classification results, but are capable of distinguishing between change and no-change areas in urban areas. Over 80% of the error in the change detection can be related to definitional issues or error propagation, rather than algorithm error. As such, these methods hold great potential for routine monitoring of urban change, as well as for providing a consistent and up-to-date dataset on urban extent and expansion for a rapidly evolving region.

Urban areas↗

Photocarrier Transfer across Monolayer MoS 2 –MoSe 2 Lateral Heterojunctions

In-plane heterojuctions formed from two monolayer semiconductors represent the finest control of electrons in condensed matter and have attracted significant interest. Various device studies have shown the effectiveness of such structures to control electronic processes, illustrating their potentials for electronic and optoelectronic applications. However, information about the physical mechanisms of charge carrier transfer across the junctions is still rare, mainly due to the lack of adequate experimental techniques. Here we show that transient absorption measurements with high spatial and temporal resolution can be used to directly monitor such transfer processes. We studied MoS 2 –MoSe 2 in-plane heterostructures fabricated by chemical vapor deposition and lithographic patterning followed by laser-generated vapor sulfurization. Transient absorption measurements in reflection geometry revealed evidence of exciton transfer from MoS 2 to MoSe 2 . By comparing the experimental data with a simulation, we extracted an exciton transfer velocity of 10 4 m s–1 . These results provide valuable information for understanding and controlling in-plane carrier transfer in two-dimensional lateral heterostructures for their electronic and optoelectronic applications.

two-dimensional material↗

Role of tau versus TDP-43 pathology on medial temporal lobe atrophy in aging and Alzheimer's disease

Hippocampal atrophy on magnetic resonance imaging is an important biomarker in Alzheimer's disease (AD). While hippocampal atrophy was thought to result from tau tangles in AD, different neuropathologies can lead to hippocampal atrophy, especially TAR DNA-binding protein 43 (TDP-43) pathology. In this narrative review, we evaluate existing studies on the relative contribution of tau and TDP-43 pathology to medial temporal lobe (MTL) atrophy. We report a clear association of both tau and TDP-43 neuropathology with MTL atrophy, even after correcting for other neuropathologies. Next, we discuss a potential synergism between tau and TDP-43 and the relative timing of the effects of both neuropathologies. Finally, avenues for future research will be discussed. A better understanding of the interplay between tau and TDP-43 neuropathologies and their effect on atrophy will help with the development of more specific biomarkers for limbic-predominant age-related TDP-43 encephalopathy and pinpointing of the optimal timing for testing anti-tau and anti-TDP-43 treatments in trials.

60 APPLIED LIFE SCIENCES↗