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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,243 records · Page 69
All sourcesNASA NTRSDOE OSTI
DOE OSTI2022

Interfacial Exchange Phenomena Driven by Ferromagnetic Domains

Abstract Interfacial proximity effects in antiferromagnetic/ferromagnetic (AFM/FM) bilayers control the exchange‐bias (EB) phenomena exploited in most spintronic devices, although still is lack of full understanding. Discordant results, including different exchange‐bias field ( H E ), coercivity ( H C ), or blocking temperature ( T B ) found even in similar systems, are usually ascribed to uncontrolled parameters, namely dissimilar interfacial defects, structure, and thicknesses. Here, it is shown in the very same sample that the magnetic domain structure during the magnetization reversal of the FM layer controls those mentioned effects. Simultaneous transport and vectorial‐resolved magnetic measurements performed in a V 2 O 3 /Co system during warming after different field cooling (FC) procedures exhibit a strong dependence on the FC angle and the domain structure of the FM layer. Remarkably, magnetization reversal analysis reveals 35 K of variation in T B and up to a factor of two in H E . These observations can be explained within the random‐field model for the interfacial exchange coupling with a fixed AFM domain structure in contact with a variable (angle‐dependent) FM domain structure. The results highlight the importance of the domain structure and magnetization reversal of the FM layer (not previously considered) in the EB phenomena, with potential to tailor interfacial effects in future spintronic devices.

36 MATERIALS SCIENCE↗
DOE OSTI2020

Thermodynamics of energy magnetization

We construct the thermodynamics of energy magnetization in the presence of gravitomagnetic field. We show that the free energy must be modified to account for the modification of the energy current operator in the presence of a confining potential. The explicit expression of the energy magnetization is derived for a periodic system, and the Streda formula for the thermal Hall conductivity is rigorously established. Furthermore, we demonstrate our theory of the energy magnetization and the Streda formula in a Chern insulator.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Direct evidence of ferromagnetism in MnSb 2 Te 4

We report the magnetic imaging of ferromagnetic domains in the van der Waals single crystal MnSb 2 Te 4 from two different sources using cryogenic magnetic force microscopy. The magnetic field dependence of the domains reveals very weak pinning of domain walls in MnSb 2 Te 4 , resulting in a negligibly small magnetic hysteresis loop. Furthermore, the temperature dependence of the domain contrast reveals a mean field like behavior, in good agreement with that of bulk magnetization measurements.

36 MATERIALS SCIENCE↗
DOE OSTI2022

Magnetization reversal driven by electron localization-delocalization crossover in the inverse spinel Co 2 VO 4

Neutron diffraction, magnetization, and muon spin relaxation measurements, supplemented by density functional theory (DFT) calculations are employed to unravel temperature-driven magnetization reversal in inverse spinel Co 2 VO 4 . All measurements show a second-order magnetic phase transition at T C = 168 K to a collinear ferrimagnetic phase. Neutron diffraction measurements reveal two antiparallel ferromagnetic (FM) sublattices, belonging to magnetic ions on two distinct crystal lattice sites, where the relative balance between the two sublattices determine the net FM moment in the unit cell. As the evolution of the ordered moment with temperature differs between the two sublattices, the net magnetic moment reaches a maximum at T NC = 138 K and reverses its sign at T MR = 65 K. The DFT results suggest that the underlying microscopic mechanism for the reversal is a delocalization of the unfilled 3d -shell electrons on one sublattice just below T C , followed by a gradual localization as the temperature is lowered. Furthermore, this delocalized-localized crossover is supported by muon spectroscopy results, as strong T 1 relaxation observed below T C indicates fluctuating internal fields.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Single pair of Weyl fermions in the half-metallic semimetal EuC d 2 A s 2 [A Single Pair of Weyl Fermions in Half-metallic EuCd 2 As 2 Semimetal]

Materials with the ideal case of a single pair of Weyl points (WPs) are highly desirable for elucidating the unique properties of Weyl fermions. EuCd 2 As 2 is an antiferromagnetic topological insulator or Dirac semimetal depending on the different magnetic configurations. Using first-principles band-structure calculations, we show that inducing ferromagnetism in EuCd 2 As 2 can generate a single pair of WPs from splitting the single pair of antiferromagnetic Dirac points due to its half-metallic nature. Analysis with a low-energy effective Hamiltonian shows that a single pair of WPs is obtained in EuCd 2 As 2 because the Dirac points are very close to the zone center and the ferromagnetic exchange splitting is large enough to push one pair of WPs to merge and annihilate at Γ while the other pair survives. As a result, we predict that alloying with Ba at the Eu site can stabilize the ferromagnetic configuration and generate a single pair of Weyl points without application of a magnetic field.

36 MATERIALS SCIENCE↗
NASA NTRS1974

Electromagnetic flow rate meter

A liquid metal, whose flow rate is to be determined, is directed through a chamber made of electrically-insulating material on which there is impressed a magnetic field perpendicular to the direction of flow of the liquid metal. The magnetic field is made to increase in strength in a downstream direction of the flow of liquid metal. At least a pair of electrodes are disposed in the chamber traversely and perpendicular to the direction of flow and an ammeter is connected between the electrodes. Electrodes may be disposed in the top or the bottom of the chamber and each may be segmented. Oppositely disposed electrodes may be used with at least one dividing wall extending from each electrode to cause reversal of the direction of flow of the liquid metal. The magnetic field may be provided by electromagnets or permanent magnets such as shaded pole permanent magnets.

Banks, B. A.↗
NASA NTRS2000

Environmental Exposure Conditions for Teflon FEP on the Hubble Space Telescope Investigated

The Hubble Space Telescope (HST) was launched into low Earth orbit on April 24,1990. During the first servicing mission in December 1993 (3.6 years after launch), multilayer insulation (MLI) blankets were retrieved from the two magnetic sensing systems located on the light shield. Retrieval of one of the solar arrays during this mission also provided MLI blanket material from the solar array drive arm. These MLI materials were analyzed in ground-based facilities, and results indicate that the space-facing outer layer of the MLI, aluminized Teflon FEP (DuPont; fluorinated ethylene propylene), was beginning to degrade. Close inspection of the FEP revealed through-the-thickness cracks in areas with the highest solar exposure and stress concentration. During the second servicing mission in February 1997 (6.8 years after launch), astronauts observed and documented severe cracking in the outer layer of the MLI blankets on both the solar-facing and anti-solar-facing surfaces. During this second mission, some material from the outer layer of the light shield MLI was retrieved and subsequently analyzed in ground-based facilities. After the second servicing mission, a Failure Review Board was convened by NASA Goddard Space Flight Center to address the MLI degradation problem on HST. Members of the Electro-Physics Branch of the NASA Glenn Research Center at Lewis Field participated on this board. To determine possible degradation mechanisms, board researchers needed to consider all environmental constituents to which the FEP MLI surfaces were exposed. On the basis of measurements, models, and predictions, environmental exposure conditions for FEP surfaces on HST were estimated for various time periods from launch in 1990 through 2010, the planned end-of-life for HST. The table summarizes these data including the number and temperature ranges of thermal cycles; equivalent Sun hours; fluence and absorbed radiation dose from solar event x rays; fluence and absorbed dose from solar wind protons and electrons trapped in Earth s magnetic field; fluence of plasma electrons and protons; and atomic oxygen fluence.

Dever, Joyce A.↗
NASA NTRS2014

Material Challenges and Opportunities for Commercial Electric Aircraft

Significant reduction in carbon dioxide emission for future air transportation system will require adoption of electric propulsion system and more electric architectures. Various options for aircraft electric propulsion include hybrid electric, turboelectric, and full electric system. Realization of electric propulsion system for commercial aircraft applications will require significant increases in power density of electric motors and energy density of energy storage system, such as the batteries and fuel cells. In addition, transmission of MW of power in the aircraft will require high voltage power transmission system to reduce the weight of the power transmission system. Finally, there will be significant thermal management challenges. Significant advances in material technologies will be required to meet these challenges. Technologies of interest include materials with higher electrical conductivity than Cu, high thermal conductivity materials, and lightweight electrically insulating materials with high breakdown voltage, high temperature magnets, advanced battery and fuel cell materials, and multifunctional materials. The presentation will include various challenges for commercial electric aircraft and provide an overview of material improvements that will be required to meet these challenges.

materials↗
DOE OSTI2012

High-Field Combined-Function Magnets for a 1.5 x 1.5 TeV Muon Collider Storage Ring

A new storage ring lattice based on combined function high-field magnets and conceptual designs of superconducting magnets with dipole and quadrupole coils for a muon collider with a c.o.m. energy of 3 TeV and an average luminosity of 4x10^{34 } cm^{-2} s^{-1} are presented. Magnets are designed to provide the required focusing field gradient and bending field in the aperture with the appropriate operation margin. Magnets have large apertures to provide an adequate space for internal absorbers, vacuum insulation, beam pipe, and helium channel. Coil cross-sections were optimized to achieve the best possible field quality in the magnet aperture occupied with beams. Magnet parameters are reported and compared with the requirements. Energy depositi on calculations with the MARS code have allowed to optimize parameters of inner absorbers and collimators in interconnect regions, thus reducing peak power density and dynamic loads to the tolerable levels.

43 PARTICLE ACCELERATORS↗
DOE OSTI2017

Role of polar compensation in interfacial ferromagnetism of LaNiO 3 /CaMnO 3 superlattices

Polar compensation can play an important role in the determination of interfacial electronic and magnetic properties in oxide heterostructures. Using x-ray absorption spectroscopy, x-ray magnetic circular dichroism, bulk magnetometry, and transport measurements, we find that interfacial charge redistribution via polar compensation is essential for explaining the evolution of interfacial ferromagnetism in LaNiO 3 /CaMnO 3 superlattices as a function of LaNiO 3 layer thickness. In insulating superlattices (four unit cells or less of LaNiO 3 ), magnetism is dominated by Ni-Mn superexchange, while itinerant electron-based Mn-Mn double exchange plays a role in thicker metallic superlattices. X-ray magnetic circular dichroism and resonant x-ray scattering show that Ni-Mn superexchange contributes to the magnetization even in metallic superlattices. This Ni-Mn superexchange interaction can be explained in terms of polar compensation at the LaNiO 3 -CaMnO 3 interface. Finally, these results highlight the different mechanisms responsible for interfacial ferromagnetism and the importance of understanding compensation due to polar mismatch at oxide-based interfaces when engineering magnetic properties.

36 MATERIALS SCIENCE↗
DOE OSTI2018

Signatures of long-range-correlated disorder in the magnetotransport of ultrathin topological insulators

In an ultrathin topological insulator (TI) film, a hybridization gap opens in the TI surface states, and the system is expected to become either a trivial insulator or a quantum spin Hall insulator when the chemical potential is within the hybridization gap. Here we show, however, that these insulating states are destroyed by the presence of a large and long-range-correlated disorder potential, which converts the expected insulator into a metal. We perform transport measurements in ultrathin dual-gated topological insulator films as a function of temperature, gate voltage, and magnetic field, and we observe a metalliclike nonquantized conductivity, which exhibits a weak antilocalizationlike cusp at low magnetic fields and gives way to a nonsaturating linear magnetoresistance at large fields. We explain these results by considering the disordered network of electron- and hole-type puddles induced by charged impurities. We argue theoretically that such disorder can produce an insulator-to-metal transition as a function of increasing disorder strength, and we derive a condition on the band gap and the impurity concentration necessary to observe the insulating state. Finally, we explain the linear magnetoresistance in terms of strong spatial fluctuations of the local conductivity using both numerical simulations and a theoretical scaling argument.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Magnetic properties of the quasi-XY Shastry-Sutherland magnet ER 2 Be 2 SiO 7

Polycrystalline and single-crystal samples of the insulating Shastry-Sutherland compound Er 2 ⁢Be 2 ⁢SiO 7 were synthesized via a solid-state reaction and the floating zone method, respectively. The crystal structure, Er single-ion anisotropy, zero-field magnetic ground state, and magnetic phase diagrams along high-symmetry crystallographic directions were investigated with bulk measurement techniques, x-ray and neutron diffraction, and neutron spectroscopy. Here, we establish that Er 2 ⁢Be 2 ⁢SiO 7 crystallizes in a tetragonal space group with planes of orthogonal Er dimers and a strong preference for the Er moments to lie in the local plane perpendicular to each dimer bond. We also find that this system has a noncollinear ordered ground state in zero field with a transition temperature of 0.841 K consisting of antiferromagnetic dimers and in-plane moments. Finally, we mapped out the H-T phase diagrams for Er 2 ⁢Be 2 ⁢SiO 7 along the directions H ∥ [001], [100], and [110]. While an increasing in-plane field simply induces a phase transition to a field-polarized phase, we identify three metamagnetic transitions in the H ∥ [001] case. Single-crystal neutron diffraction results reveal that the H ∥ [001] phase diagram can be explained predominantly by the expected field-induced behavior of classical, anisotropic moments, although the microscopic origin of one phase requires further investigation.

36 MATERIALS SCIENCE↗
DOE OSTI2013

Solid solution studies of layered honeycomb-ordered phases O₃–Na₃M₂SbO₆ (M=Cu, Mg, Ni, Zn)

Complete solid solutions with the composition Na₃M 2–x M´ x SbO₆ where M, M´=Cu, Mg, Ni, Zn have been synthesized by conventional solid state techniques and were investigated using X-ray diffraction, magnetic susceptibility and optical measurements. All compositions crystallize in a monoclinic unit cell and exhibit a layered structure with a honeycomb cationic ordering within the slabs. These compounds also exhibit Curie–Weiss behavior at high temperature and the magnetic moment values verify the presence of Cu²⁺ and/or Ni²⁺. The antiferromagnetic order of Na₃Ni₂SbO₆ is suppressed upon substitution of Ni²⁺ with Mg²⁺ or Zn²⁺. The spin gap observed in Na₃Cu₂SbO₆ is also suppressed by substitution of Cu²⁺ with Mg²⁺ or Zn²⁺. The Na₃Ni 2–x Cu x SbO₆ compositions follow an expected transition from an antiferromagnetic ordering to the spin gap of the copper end member. The estimated band gaps for these compounds have been determined from diffuse reflectance measurements. - Graphical abstract: Complete solid solutions with the composition Na₃M 2–x M´ x SbO₆ where M, M´=Cu, Mg, Ni, Zn have been synthesized using conventional solid state techniques and were investigated using X-ray diffraction, magnetism and optical measurements. Based on an ionic radii point of view the lattice parameter shifting in the composition containing copper are opposite of what would be expected. The Cu²⁺ is Jahn–Teller active which distorts the C2/m cell, increasing the β angle between the a and c parameters and explains this shifting pattern. Highlights: • The solid solutions O₃–Na₃M 2–x M´ x SbO₆(M, M´=Cu, Mg, Ni, Zn) were synthesized. • These compounds crystallize in the C2/m space group. • The Jahn–Teller active Cu²⁺ causes distortion of the monoclinic cell. • The Cu²⁺ spin gap magnetic properties are diluted upon 25% substitution. • All compositions are insulating and have large band gaps.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Tetragonal Kondo Insulator EuCd 2 Sb 2 Discovered via High Pressure High Temperature Synthesis

Abstract Magnetic and electronic properties of quantum materials heavily rely on the crystal structure even in the same chemical compositions. In this study, it is demonstrated that a layered tetragonal EuCd 2 Sb 2 structure can be obtained by treating bulk trigonal EuCd 2 Sb 2 under high pressure (6 GPa) and high temperature (600 °C). Magnetization measurements of the newly formed layered tetragonal EuCd 2 Sb 2 confirm an antiferromagnetic ordering with Neel temperature ( T N ) around 16 K, which is significantly higher than that ( T N ≈ 7 K) of trigonal EuCd 2 Sb 2 , consistent with heat capacity measurements. Moreover, bad metal behavior is observed in the temperature dependence of the electrical resistivity and the resistivity shows a dramatic increase around the Neel temperature. Electronic structure calculations with local density approximation dynamic mean–field theory (LDA+DMFT) show that this material is strongly correlated with well‐formed large magnetic moments, due to Hund's coupling, which is known to dramatically suppress the Kondo scale.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Accelerated vortex dynamics across the magnetic 3D-to-2D crossover in disordered superconductors

Disorder can have remarkably disparate consequences in superconductors, driving superconductor–insulator transitions in ultrathin films by localizing electron pairs and boosting the supercurrent carrying capacity of thick films by localizing vortices (magnetic flux lines). Though the electronic 3D-to-2D crossover at material thicknesses d ~ ξ (coherence length) is well studied, a similarly consequential magnetic crossover at d ~ L c (pinning length) that should drastically alter material properties remains largely underexamined. According to collective pinning theory, vortex segments of length L c bend to adjust to energy wells provided by point defects. Consequently, if d truncates L c , a change from elastic to rigid vortex dynamics should increase the rate of thermally activated vortex motion S. Here, we characterize the dependence of S on sample thickness in Nb and cuprate films. The results for Nb are consistent with collective pinning theory, whereas creep in the cuprate is strongly influenced by sparse large precipitates. In conclusion, we leverage the sensitivity of S to d to determine the generally unknown scale L c , establishing a new route for extracting pinning lengths in heterogeneously disordered materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

On the initiation and evolution of dielectric breakdown in auto-magnetizing liner experiments

Auto-magnetizing (AutoMag) liners are cylindrical tubes composed of discrete metallic helices encapsulated in insulating material; when driven with a ~2 MA, ~100-ns prepulse on the 20 MA, 100-ns rise time Z accelerator, AutoMag targets produced >150 T internal axial magnetic fields. Once the current rise rate of the pulsed power driver reaches sufficient magnitude, the induced electric fields in the liner cause dielectric breakdown of the insulator material and, with sufficient current, the cylindrical target radially implodes. The dielectric breakdown process of the insulating material in AutoMag liners has been studied in experiments on the 500–900 kA, ~100-ns rise time Mykonos accelerator. Multi-frame gated imaging enabled the first time-resolved observations of photoemission from dynamically evolving plasma distributions during the breakdown process in AutoMag targets. Using magnetohydrodynamic simulations, we calculate the induced electric field distribution and provide a detailed comparison to the experimental data. We find that breakdown in AutoMag targets does not primarily depend on the induced electric field in the gaps between conductive helices as previously thought. Finally, to better control the dielectric breakdown time, a 12–32 mJ, 170 ps ultraviolet (λ = 266 nm) laser was implemented to irradiate the outer surface of AutoMag targets to promote breakdown in a controlled manner at a lower internal axial field. Here, the laser had an observable effect on the time of breakdown and subsequent plasma evolution, indicating that pulsed UV lasers can be used to control breakdown timing in AutoMag.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗