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At least 127 records · Page 7

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NASA NTRS1989

Implications of AAOE observations for proposed chemical explanations of the seasonal and interannual behavior of Antarctic ozone

Model simulations were used to investigate the seasonal and interannual behavior of ozone for different choices of initial odd nitrogen concentration in July and different assumptions on the heterogeneous reactions, with particular consideration given to the possible contribution of chlorine chemistry to the ozone hole phenomenon. The numerical experiments were selected based on the simulations of the observed trace gas concentrations during the Airborne Antarctic Ozone Experiment in 1987. In all cases considered, the catalytic cycle associated with the formation and photolysis of Cl2O2 could account for more than half of the photochemical removal of O3 within the Antarctic vortex through mid-September. The reaction of BrO with ClO, which accounts for 15-20 percent of O3 removal in the same period, tends to play a more important role toward the end of September, when the concentration of ClO is expected to decrease. No simple relationship was found between the increase in chlorine lavel and the interannual decrease in Antarctic O3.

Ko, M. K. W.↗

NASA NTRS1989

Lagrangian photochemical modeling studies of the 1987 Antarctic spring vortex. II - Seasonal trends in ozone

A photochemical model consisting of 40 species and 107 reactions is integrated along 80-day air parcel trajectories calculated in the lower stratosphere for the springtime Antarctic. For the trajectory starting at 58 deg S, which may be regarded as outside the circumpolar vortex, only a small change in O3 occurs in the model. In contrast, for the air parcel starting in the vortex at 74 deg S, the O3 concentration is reduced by 93 percent during the 80 days from the beginning of August to late October. The model results for several species are compared with measurements from the Airborne Antarctic Ozone Experiment and, in general, good agreement is obtained. In the model, the dentrification of the air parcels in polar stratospheric clouds increases the amount of chlorine present in active form. Heterogeneous reactions maintain high active chlorine which destroys O3 via the formation of the ClO dimer. Results of calculations with reduced concentrations of inorganic chlorine show considerably reduced O3 destruction rates and compare favorably with the behavior of total O3 since the late 1970s. The remaining major uncertainties in the photochemical aspects of the Antarctic ozone hole are highlighted.

Austin, J.↗

NASA NTRS1990

A comparison of ER-2 measurements of stratospheric water vapor between the 1987 Antarctic and 1989 Arctic Airborne missions

Vertical profiles of water vapor inside the Antarctic vortex have been compared with those taken outside it over Punta Arenas (53 deg S, 71 deg W). A similar exercise was performed with Arctic vortex profiles and those taken over Stavanger (59 deg N, 6 deg E). Residual water, defined as the stratospheric water vapor mixing ratio with the contribution from methane oxidation subtracted, is also shown as profiles inside and outside the vortex for both missions. The Arctic and Antarctic profiles of water vapor and residual water are compared. Locally dehydrated air was evident both inside and outside the Antarctic vortex, but such dehydration was not evident in and around the Arctic vortex. Arctic profiles of residual water are consistent with nontropical entry for some air.

Kelly, K. K.↗

NASA NTRS1990

Meteorite infall as a function of mass - Implications for the accumulation of meteorites on Antarctic ice

Antarctic meteorites are considerably smaller, on average, than those recovered elsewhere in the world, and seem to represent a different portion of the mass distribution of infalling meteorites. When an infall rate appropriate to the size of Antarctic meteorites is used (1000 meteorites 10 grams or larger/sq km/1 million years), it is found that direct infall can produce the meteorite accumulations found on eight ice fields in the Allan Hills region in times ranging from a few thousand to nearly 200,000 years, with all but the Allan Hills Main and Near Western ice fields requiring less than 30,000 years. Meteorites incorporated into the ice over time are concentrated on the surface when the ice flows into a local area of rapid ablation. The calculated accumulation times, which can be considered the average age of the exposed ice, agree well with terrestrial ages for the meteorites and measured ages of exposed ice. Since vertical concentration of meteorites through removal of ice by ablation is sufficient to explain the observed meteorite accumulations, there is no need to invoke mechanisms to bring meteorites from large areas to the relatively small blue-ice patches where they are found. Once a meteorite is on a bare ice surface, freeze-thaw cycling and wind break down the meteorite and remove it from the ice. The weathering lifetime of a 100-gram meteorite on Antarctic ice is on the order of 10,000 + or - 5,000 years.

Huss, Gary R.↗

NASA NTRS1990

Global impact of the Antarctic ozone hole - Dynamical dilution with a three-dimensional chemical transport model

The hypothesis that, once the Antarctic ozone hole is photochemically generated in the spring, the ozone deficit remains in the stratosphere throughout the year was investigated using a three-dimensional chemical transport model (CTM) for the stratosphere with linearized ozone chemistry. An Antarctic ozone hole was imposed on the basis of observations, and the dynamical dilution of the ozone-depleted air was followed for the next 12 months. The CTM calculations show that the transport of ozone-poor air from the Antarctic vortex results in measurable decreases to column ozone, extending to 30 deg S during the austral summer. By the end of the year, about 70 percent of the initially prescribed ozone deficit is replenished through stratospheric chemistry.

Prather, Michael↗

NASA NTRS1990

Global impact of the Antarctic ozone hole - Chemical propagation

A model is presented for the chemical mixing of stratospheric air, that combines photochemistry, molecular diffusion, and strain (i.e., the stretching of air parcels due to wind shear). The model is applied to the case in which chemically perturbed air parcels from the Antarctic stratosphere are transported to mid-latidudes and strained into thin ribbon-like filaments until they are diffusively mixed with the ambient stratosphere. Results show that, following the breakup of the polar vortex, Antarctic air with substantially depleted ozone will not contribute any additional ozone loss at mid-latitudes as it is mixed with ambient air, supporting the results of simulations of the Antarctic ozone hole by Prather et al. (1990). Nevertheless, air processed by polar stratospheric clouds but transported to mid-latitudes before substantive ozone depletion, can lead to additional loss after mixing with ambient air.

Prather, Michael↗

NASA NTRS1991

Generation of abnormal trace element abundances in Antarctic eucrites by weathering processes

Data were obtained on the trace- and major-element compositions of 16 Antarctic abnormal eucrites, many of which exhibiting positive (but sometimes negative) Ce anomalies, positive Eu anomalies, and low abundances of the remainder of the REEs. The results of data analysis suggest that the unusual REE patterns of abnormal Antarctic eucrites arise from weathering effects generated in or on the Antarctic ice. The suggested scenario involves the formation of melt water and its equilibration with the atmosphere, promoting the dissolution of REE-rich phosphates and the oxidation of Ce. As a result, tetravalent Ce is fractionated from the trivalent REE in solution.

Mittlefehldt, David W.↗

NASA NTRS1991

Thermoluminescence survey of 12 meteorites collected by the European 1988 Antarctic meteorite expedition to Allan Hills and the importance of acid washing for thermoluminescence sensitivity measurements

Natural and induced thermoluminescence (TL) data are reported for 12 meteorites recovered from the Allan Hills region of Antarctica by the European field party during the 1988/1989 field season. The samples include one with extremely high natural TL, ALH88035, suggestive of exposure to unusually high radiation doses (i.e., low degrees of shielding), and one, ALH88034, whose low natural TL suggests reheating within the last 100,000 years. The remainder have natural TL values suggestive of terrestrial ages similar to those of other meteorites from Allan Hills. ALH88015 (L6) has induced TL data suggestive of intense shock. TL sensitivities of these meteorites are generally lower than observed falls of their petrologic types, as is also observed for Antarctic meteorites in general. Acid-washing experiments indicate that this is solely the result of terrestrial weathering rather than a nonterrestrial Antarctic-non-Antarctic difference. However, other TL parameters, such as natural TL and induced peak temperature-width, are unchanged by acid washing and are sensitive indicators of a meteorite's metamorphic and recent radiation history.

Benoit, P. H.↗

NASA NTRS1992

Antarctic lakes (above and beneath the ice sheet): Analogues for Mars

The perennial ice covered lakes of the Antarctic are considered to be excellent analogues to lakes that once existed on Mars. Field studies of ice covered lakes, paleolakes, and polar beaches were conducted in the Bunger Hills Oasis, Eastern Antarctica. These studies are extended to the Dry Valleys, Western Antarctica, and the Arctic. Important distinctions were made between ice covered and non-ice covered bodies of water in terms of the geomorphic signatures produced. The most notable landforms produced by ice covered lakes are ice shoved ridges. These features form discrete segmented ramparts of boulders and sediments pushed up along the shores of lakes and/or seas. Sub-ice lakes have been discovered under the Antarctic ice sheet using radio echo sounding. These lakes occur in regions of low surface slope, low surface accumulations, and low ice velocity, and occupy bedrock hollows. The presence of sub-ice lakes below the Martian polar caps is possible. The discovery of the Antarctic sub-ice lakes raises possibilities concerning Martian lakes and exobiology.

Rice, J. W., Jr.↗

NASA NTRS1993

The diatom record from beneath the West Antarctic Ice Sheet and the global proxy perspective

Recent glaciological evaluation and modeling of the marine-based West Antarctic Ice Sheet (WAIS) support the possibility that the WAIS disintegrated during one or more Pleistocene interglacial period(s). The magnitude of sea level and oxygen isotope variation during certain late-Pleistocene interglacial periods is also consistent with the possibility of major retreat of the WAIS. Although oxygen isotopes from deep-sea sediments provide the best available proxy record for global ice volume (despite the ambiguities in the record), the source of ice volume changes must be hypothesized. Based on the intensity of interglacial isotopic shifts recorded in Southern Ocean marine sedimentary records, stage 11 (400,000 years ago) is the strongest candidate for WAIS collapse, but the records for stages 9, 7, and 5.5 are all consistent with the possibility of multiple late-Pleistocene collapses. Seismic reflection studies through the WAIS have revealed thick successions of strata with seismic characteristics comparable to upper Tertiary marine sediments. Small samples of glacial diamictons from beneath the ice sheet have been collected via hot-water drilled access holes. These sediments include mixed diatom assemblages of varying ages. Late-Miocene diatoms dominate many samples, probably reflecting marine deposition in West Antarctic basins prior to development of a dominantly glacial phase in West Antarctica. In addition to late-Miocene diatoms, samples from Upstream B (1988/89) contain rare post-Miocene diatoms, many of which imply deposition in the West Antarctic interior during one or more Pleistocene deglaciation periods. Age-diagnostic fossils in glacial sediments beneath ice sheets provide relatively coarse chronostratigraphic control, but they do contain direct evidence of regional deglaciation. Thus, sub-glacial till samples provide the evidence regarding the source of ice sheet variability seen in well-dated proxy records. Combined, these independent data sets can provide a more comprehensive and less speculative interpretation of the history of past glacial minima in currently glaciated polar regions.

Scherer, Reed P.↗

NASA NTRS1992

Analysis of Antarctic stratospheric aerosol properties using SAGE II extinction measurements

Multispectra aerosol extinction data for the fall and spring of 1987 measured by the SAGE II sensor are employed to determine the physical characteristics of aerosols within the springtime Antarctic polar vortex. Attention is given to the physical processes that give rise to the apparent springtime 'cleansing' of the Antarctic stratosphere. The inferred vertical and radial structure compare favorably with in situ measurements but yield a previously unavailable 2D structure to the distribution of aerosols within the polar vortex. The springtime 'cleansing' of the Antarctic stratosphere is found to be a result of both large-scale subsidence and the preferential removal of large particles by the nucleation and subsequent sedimentation of polar stratospheric clouds.

Thomason, Larry W.↗

NASA NTRS1992

Dynamic constraints on CO2 uptake by an iron-fertilized Antarctic

The topics covered include the following: tracer distribution and dynamics in the Antarctic Ocean; a model of Antarctic and Non-Antarctic Oceans; effects on an anthropogenically affected atmosphere; effects of seasonal iron fertilization; and implications of the South Atlantic Ventilation Experiment C-14 results.

Peng, Tsung-Hung↗

NASA NTRS1993

The mid-infrared transmission spectra of Antarctic ureilites

The mid-IR (4000-450/cm; 2.5-22.2 microns) transmission spectra of seven Antarctic ureilites and 10 Antarctic H-5 ordinary chondrites are presented. The ureilite spectra show a number of absorption bands, the strongest of which is a wide, complex feature centered near 1000/cm (10 microns) due to Si-O stretching vibrations in silicates. The profiles and positions of the substructure in this feature indicate that Mg-rich olivines and pyroxenes are the main silicates responsible. The relative abundances of these two minerals, as inferred from the spectra, show substantial variation from meteorite to meteorite, but generally indicate olivine is the most abundant (olivine:pyroxene = 60:40 to 95:5). Both the predominance of olivine and the variable olivine-to-pyroxene ratio are consistent with the known composition and heterogeneity of ureilites. The H-5 ordinary chondrites spanned a range of weathering classes and were used to provide a means of addressing the extent to which the ureilite spectra may have been altered by weathering processes. It was found that, while weathering of these meteorites produces some weak bands due to the formation of small amounts of carbonates and hydrates, the profile of the main silicate feature has been little affected by Antarctic exposure in the meteorites studied here. The mid-IR ureilite spectra provide an additional means of testing potential asteroidal parent bodies for the ureilites.

Sandford, Scott A.↗

NASA NTRS1994

Spread of denitrification from 1987 Antarctic and 1988-1989 Arctic stratospheric vortices

Vertical profiles of N2O and NO(y) taken by the ER-2 outside the vortex are used to construct average vertical profiles of F(NO(y)) = NO(y)/(A-N2O), where A is the tropospheric content of N2O three years prior to the measurements. The southern hemisphere had less nitrous oxide in the range 400 less than Theta less than 470 K, by up to 25% relative to the northern hemisphere. F(NO(y)) is the ratio of NOy produced to N2O lost in a stratospheric air mass since entry from the troposphere. The profiles of F(NO(y)) have the following characteristics: (1) Relative to 1991-1992, a year without denitrification inside or outside the vortex, the northern hemisphere in 1988-1989 showed denitrification outside the vortex ranging up to 25% and averaging 17% above Theta = 425 K. (2) Relative to the northern hemisphere in 1991-1992, the southern hemisphere in 1987 showed denitrification outside the vortex ranging up to 32% and averaging 20% above Theta = 400 K. (3) Below Theta = 400 K the southern hemisphere showed enhancements of F(NO(y)) relative to the northern hemisphere in 1991-1992 ranging up to 200% at Theta = 375 K, outside the vortex. Corresponding profiles of residual water, R(H2O) = H2O - 2(1.6 - CH4), are considered and shown to be consistent with those of F(NO(y)) in the sense that they show deficits outside the Antarctic vortex, which was both dehydrated and denitrified, but not outside the 1988-1989 Arctic vortex, which was denitrified but not dehydrated. R(H2O) is the water content of stratospheric air with the contribution from methane oxidation subtracted. Comparison of F(NO(y)) and R(H2O) below 400 K outside the Antarctic vortex leads to the suggetion that dehydration in the Antarctic vortex occurs by the sedimentation of ice crystals large enough to fall out of the stratosphere, whereas denitrification occurs mainly on mixed nitric acid-water crystals which evaporate below the base of the vortex at Theta = 400 K but above the tropopause.

Tuck, A. F.↗

NASA NTRS1993

Use of stratospheric aerosol properties as diagnostics of Antarctic vortex processes

Physical properties of the stratospheric aerosol population are inferred from cloud-free SAGE II multiwavelength extinction measurements in the Antarctic during late summer (February/March) and spring (September/October, November). Seasonal changes in these properties are used to infer physical processes occurring in the Antarctic stratosphere over the course of the winter. The analysis suggests that the apparent springtime cleansing of the Antarctic stratosphere is the result of aerosol redistribution through subsidence of the polar vortex air mass and sedimentation of large polar stratospheric cloud particles. The analysis also suggests that vortex processes are responsible for a significant downward transport of aerosol through the tropopause.

Thomason, Larry W.↗

NASA NTRS1995

Present-day Antarctic ice mass changes and crustal motion

The peak vertical velocities predicted by three realistic, but contrasting, present-day scenarios of Antarctic ice sheet mass balance are found to be of the order of several mm/a. One scenario predicts local uplift rates in excess of 5 mm/a. These rates are small compared to the peak Antarctic vertical velocities of the ICE-3G glacial rebound model, which are in excess of 20 mm/a. If the Holocene Antarctic deglaciation history protrayed in ICE-3G is realistic, and if regional upper mantle viscosity is not an order of magnitude below 10(exp 21) Pa(dot)s, then a vast geographical region in West Antarctica is uplifting at a rate that could be detected by a future Global Positioning System (GPS) campaign. While present-day scenarios predict small vertical crustal velocities, their overall continent-ocean mass exchange is large enough to account for a substantial portion of the observed secular polar motion (omega m(arrow dot)) and time-varying zonal gravity field.

James, Thomas S.↗

NASA NTRS1993

The Mid-Infrared Transmission Spectra of Antarctic Ureilites

The mid-infrared (4000-450 1/cm; 2.5-22.2 micron) transmission spectra of seven Antarctic ureilites and 10 Antarctic H-5 ordinary chondrites are presented. The ureilite spectra show a number of absorption bands, the strongest of which is a wide, complex feature centered near 1000 1/cm (10 micron) due to Si-O stretching vibrations in silicates. The profiles and positions of the substructure in this feature indicate that Mg-rich olivines and pyroxenes are the main silicates responsible. The relative abundances of these two minerals, as inferred from the spectra, show substantial variation from meteorite to meteorite, but generally indicate olivine is the most abundant (olivine:pyroxene = 60:40 to 95:5). Both the predominance of olivine and the variable olivine-to-pyroxene ratio are consistent with the known composition and heterogeneity of ureilites. The H-5 ordinary chondrites spanned a range of weathering classes and were used to provide a means of addressing the extent to which the ureilite spectra may have been altered by weathering processes. It was found that, while weathering of these meteorites produces some weak bands due to the formation of small amounts of carbonates and hydrates, the profile of the main silicate feature has been little affected by Antarctic exposure in the meteorites studied here. The mid-infrared ureilite spectra provide an additional means of testing potential asteroidal parent bodies for the ureilites. At present, the best candidates include the subset of S-type asteroids having low albedos and weak absorption features in the near infrared.

Sandford, Scott A.↗

NASA NTRS1996

ATMOS/ATLAS-3 Observations of Long-Lived Tracers and Descent in the Antarctic Vortex in November 1994

Observations of the long-lived tracers N2O, CH4 and HF obtained by the Atmospheric Trace Molecule Spectroscopy (ATMOS) instrument in early November 1994 are used to estimate average descent rates during winter in the Antarctic polar vortex of 0.5 to 1.5 km/month in the lower stratosphere, and 2.5 to 3.5 km/month in the middle and upper stratosphere. Descent rates inferred from ATMOS tracer observations agree well with theoretical estimates obtained using radiative heating calculations. Air of mesospheric origin (N2O less than 5 ppbV) was observed at altitudes above about 25 km within the vortex. Strong horizontal gradients of tracer mixing ratios, the presence of mesospheric air in the vortex in early spring, and the variation with altitude of inferred descent rates indicate that the Antarctic vortex is highly isolated from midlatitudes throughout the winter from approximately 20 km to the stratopause. The 1994 Antarctic vortex remained well isolated between 20 and 30 km through at least mid-November.

Abrams, M. C.↗