Search NASA⌕ Search

SEARCH · Search NASA

Results for “BRILLOUIN EFFECT”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.

At least 127 records · Page 7
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Laser-plasma instabilities in long scale-length plasmas relevant to shock-ignition

We present 2D particle-in-cell simulations of laser-plasma instabilities (LPI) performed using conditions relevant to experiments on the OMEGA and NIF laser facilities. The laser intensity used is 2×10 15 W cm -2 , which allows comparison with previous experiments and simulations investigating shock ignition, though this is a relatively low intensity for the scheme. We find that the large convective gain of the instabilities leads to dynamics that are largely controlled by pump depletion and to scattering or absorption by LPIs predominantly occurring away from the quarter-critical density. The two-plasmon decay (TPD) instability is dominant for OMEGA-type conditions and remains important at the NIF-scale. In both cases, most absorption from TPD occurs near its Landau cutoff density, and we examine its nonlinear dynamics in this region, focusing on the ion-acoustic waves responsible for saturation. For NIF-type conditions, stimulated Raman scattering (SRS) and stimulated Brillouin scattering divert significant fractions of laser energy, and we find that SRS backscatter can occur with high gain at low densities due to kinetic effects. An in-depth analysis of hot-electron production is performed to identify the main sources and their characteristic electron temperature. For both simulations presented, the overall hot-electron temperature lies between 30 and 35 keV. This is relatively low and will likely increase shock pressure; however, the distributions also contain a significant number of high-energy (E k >100 keV) electrons that would likely cause unacceptable preheat. We, therefore, suggest some strategies that may be utilized to minimize this high-energy component. I. INTROD

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

Deep Neural Network Assisted Distributed Strain and Temperature Fiber Sensor System for Natural Gas Pipeline Monitoring

Natural gas pipeline integrity monitoring is crucial to detect potential leaks, find structural issues, and prevent environmental damage. This article presents a system of natural gas pipeline monitoring that uses a specialized double Brillouin peak sensing fiber along with the Brillouin optical time domain analysis (BOTDAs) technique. The calibrated sensing fiber coefficients for strain and temperature are 41.8 kHz/ με and 0.9 MHz/°C for peak 1; and 47.2 kHz/ με , and 1.11 MHz/°C for peak 2, respectively. Initially, lab tests were performed by installing a short section of double Brillouin peak fiber (DBPF) on a 1-in steel pipe under pressure up to 1000 per square inch (psi) at elevated temperatures. Simultaneous distributed measurements of temperature and pressure-induced hoop strain were successfully measured. Considering the long processing speed to extract Brillouin frequency shift (BFS), we employ a novel probabilistic deep neural network (PDNN) framework for rapid BFS prediction. Additionally, using the Finite Element Method, the effects of the pipeline pressure on hoop strain were modeled and compared to the experimental hoop strain under the same set of pipeline conditions. Finally, an actual 4-in outer diameter steel natural gas pipeline was used for pilot-scale tests, where hoop strain was measured at various pressure levels. Leaks were simulated to demonstrate accurate pipeline integrity monitoring. At an internal pipe pressure of 1000 psi, hoop strain of approximately 300 με was observed, and the sensitivity was calculated as 0.28 με /psi. The results of this pilot-scale study demonstrated that the system is capable of performing distributed monitoring sufficient to detect pipeline pressure and the presence of leaks to ensure the safe operation of gas pipelines in the field.

03 NATURAL GAS↗
DOE OSTI2018

Electronic Structure of FeSe Monolayer Superconductors: Shallow Bands and Correlations

Electronic spectra of typical single FeSe layer superconductor—FeSe monolayer film on SrTiO{sub 3} substrate (FeSe/STO) obtained from ARPES data reveal several puzzles: what is the origin of shallow and the so called “replica” bands near the M-point and why the hole-like Fermi surfaces near the Γ-point are absent. Our extensive LDA+DMFT calculations show that correlation effects on Fe-3d states can almost quantitatively reproduce rather complicated band structure, which is observed in ARPES, in close vicinity of the Fermi level for FeSe/STO. Rather unusual shallow electron-like bands around the M-point in the Brillouin zone are well reproduced. Detailed analysis of the theoretical and experimental quasiparticle bands with respect to their origin and orbital composition is performed. It is shown that for FeSe/STO system the LDA calculated Fe-3d{sub xy} band, renormalized by electronic correlations within DMFT gives the quasiparticle band almost exactly in the energy region of the experimentally observed “replica” quasiparticle band at the Mpoint. However, correlation effects alone are apparently insufficient to eliminate the hole-like Fermi surfaces around the Γ-point, which are not observed in most ARPES experiments. The Fermi surfaces remain here even if Coulomb and/or Hund interaction strengths are increased while overall agreement with ARPES worsens. Increase of number of electrons also does not lead to vanishing of this Fermi surface and makes agreement of LDA+DMFT results with ARPES data much worse. We also present some simple estimates of “forward scattering” electron-optical phonon interaction at FeSe/STO interface, showing that it is apparently irrelevant for the formation of “replica” band in this system and significant increase of superconducting T{sub c}.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

Effects of moiré lattice structure on electronic properties of graphene

Here, we study structural and electronic properties of graphene grown on silicone carbide (SiC) substrate using a scanning tunneling microscope, spot-profile-analysis low-energy electron diffraction, and angle-resolved photoemission spectroscopy. We find several new replicas of Dirac cones in the Brillouin zone. Their locations can be understood in terms of a combination of basis vectors linked to SiC 6 × 6 and graphene 6√3×6√3 reconstruction. Therefore, these new features originate from the moiré caused by the lattice mismatch between SiC and graphene. More specifically, Dirac cone replicas are caused by underlying weak modulation of the ionic potential by the substrate that is then experienced by the electrons in the graphene. We also demonstrate that this effect is equally strong in single- and trilayer graphene; therefore, the additional Dirac cones are intrinsic features rather than the result of photoelectron diffraction. These new features in the electronic structure are very important for the interpretation of recent transport measurements and can assist in tuning the properties of graphene for practical applications.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Intrinsic origin and enhancement of topological responses in ferrimagnetic antiperovskite Mn 4 N

Using first-principles calculations here we investigate the intrinsic origins of the anomalous Hall effect (AHE) and the anomalous Nernst effect (ANE) in antiperovskite ferrimagnet Mn 4 N. We predict that the AHE is significantly enhanced under both compressive and tensile strain; however, the ANE generally decreases under epitaxial strain, except for 1% compressive strain. We connect this behavior to the evolution of the Berry curvature with strain, suggesting similar strategies for achieving large AHE and ANE changes with modest amounts of strain. Finally, we find that the nonmonotonic characteristics of the AHE and ANE stem from the formation and movement of new Weyl points at the periphery of the Brillouin zone under compressive and tensile strains.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2023

Raman Wavelength Conversion in Ionic Liquids

Here, we explore the use of room-temperature ionic liquids (ILs) as Raman wavelength converters. ILs provide an engineerable framework to design suitable liquids for wavelength conversion over a broad spectral range, through careful selection of the molecular structures of the IL anions and cations so that specific characteristics can be obtained, such as a desirable Raman shift, low Brillouin scattering, and good optical transmission in the pump and Stokes wavelengths. Applying such criteria, we demonstrate that 1-ethyl-3-methylimidazolium dicyanamide (EMIM DCA) is an effective medium for conversion of 532-nm pulses from a Q-switched Nd :YAG laser to 603 nm. This corresponds to an approximate 2200 cm –1 shift, which can be used to generate mid-infrared radiation through subsequent difference frequency generation for optical pumping of CO 2 lasers. Threefold-higher Raman conversion efficiency is obtained in EMIM DCA compared with water under identical conditions in a proof-of-principle single-pass conversion setup, resulting in an efficient generation of multimillijoule, <6 ns duration, high-quality orange laser pulses in a wavelength region that is difficult to access at high energies. Consequently, we examine ILs representing two other classes of Raman-active functional groups and obtain conversion up to the fifth-order Stokes shift and first anti-Stokes shift. Through the tunable selection of their components and their useful dynamical properties, ILs provide a platform for efficient, simple, and alignment-tolerant high-energy Raman shifting with numerous industrial and technological applications.

74 ATOMIC AND MOLECULAR PHYSICS↗
DOE OSTI2019

Gravitational perturbations of nonsingular black holes in conformal gravity

It is believed that in the near future, gravitational wave detections will become a promising tool not only to test gravity theories, but also to probe extremely curved spacetime regions in our universe, such as the surroundings of black holes. In this paper, we investigate the quasinormal modes (QNMs) of the axial gravitational perturbations of a class of nonsingular black holes conformally related to the Schwarzschild black hole. Here, these nonsingular black holes can be regarded as the vacuum solution of a family of conformal gravity theories which are invariant under conformal transformations. After conformal symmetry is broken, these black holes produce observational signatures different from those of the Schwarzschild black hole, such as their QNM frequencies. We assume that the spacetime is described by the Einstein equation with the effective energy momentum tensor of an anisotropic fluid. The master equation describing the QNMs is derived, and the QNM frequencies are evaluated with the Wentzel-Kramers-Brillouin (WKB) method up to the 6th order. As expected, the QNM spectra of these nonsingular black holes deviate from those of the Schwarzschild black hole, indicating the possibility of testing these black hole solutions with the help of future gravitational wave detections.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1988

Investigation of stimulated Brillouin scattering switching in mid infrared fibers

Backward stimulated Brillouin scattering (SBS) has been experimentally studied in midinfrared transparent AgCl and KRS-5 fibers. In the present scheme, pump transmission through the fibers and acoustooptic radiative effects are simultaneously observed. The SBS shifted scattered light spectrum is investigated by laser heterodyne spectroscopy using HgCdTe and very fast metal-oxide-metal diode broadband mixers. The results suggest that reflection under high incident laser power departs from simple Fresnel surface reflection.

Yu, Chung↗
NASA NTRS1995

Radial energy transport by magnetospheric ULF waves: Effects of magnetic curvature and plasma pressure

The 'radial' transport of energy by internal ULF waves, stimulated by dayside magnetospheric boundary oscillations, is analyzed in the framework of one-fluid magnetohydrodynamics. (the term radial is used here to denote the direction orthogonal to geomagnetic flux surfaces.) The model for the inhomogeneous magnetospheric plasma and background magnetic field is axisymmetric and includes radial and parallel variations in the magnetic field, magnetic curvature, plasma density, and low but finite plasma pressure. The radial mode structure of the coupled fast and intermediate MHD waves is determined by numerical solution of the inhomogeneous wave equation; the parallel mode structure is characterized by a Wentzel-Kramer-Brillouin (WKB) approximation. Ionospheric dissipation is modeled by allowing the parallel wave number to be complex. For boudnary oscillations with frequencies in the range from 10 to 48 mHz, and using a dipole model for the background magnetic field, the combined effects of magnetic curvature and finite plasma pressure are shown to (1) enhance the amplitude of field line resonances by as much as a factor of 2 relative to values obtained in a cold plasma or box-model approximation for the dayside magnetosphere; (2) increase the energy flux delivered to a given resonance by a factor of 2-4; and (3) broaden the spectral width of the resonance by a factor of 2-3. The effects are attributed to the existence of an 'Alfven buoyancy oscillation,' which approaches the usual shear mode Alfven wave at resonance, but unlike the shear Alfven mode, it is dispersive at short perpendicular wavelengths. The form of dispersion is analogous to that of an internal atmospheric gravity wave, with the magnetic tension of the curved background field providing the restoring force and allowing radial propagation of the mode. For nominal dayside parameters, the propagation band of the Alfven buoyancy wave occurs between the location of its (field line) resonance and that of the fast mode cutoff that exists at larger radial distances.

Kouznetsov, Igor↗
DOE OSTI2018

Interfacial Dzyaloshinskii-Moriya Interaction: Effect of $5d$ Band Filling and Correlation with Spin Mixing Conductance

The Dzyaloshinskii-Moriya interaction (DMI) at the heavy metal (HM) and ferromagnetic metal (FM) interface has been recognized as a key ingredient in spintronic applications. Here we investigate the chemical trend of DMI on the $5d$ band filling ($5d^3-5d^{10}$) of the HM element in HM/FM ($\mathrm{FM = CoFeB, Co)/MgO}$ multilayer thin films. DMI is quantitatively evaluated by measuring asymmetric spin wave dispersion using Brillouin light scattering. Sign reversal and 20 times modification of the DMI coefficient $D$ have been measured as the $5d$ HM element is varied. The chemical trend can be qualitatively understood by considering the $5d$ and $3d$ bands alignment at the HM/FM interface and the subsequent orbital hybridization around the Fermi level. Furthermore, a correlation is observed between DMI and effective spin mixing conductance at the HM/FM interfaces. Finally, our results provide new insights into the interfacial DMI for designing future spintronic devices.

42 ENGINEERING↗
DOE OSTI2019

Emergent Magnetic State in (111)-Oriented Quasi-Two-Dimensional Spinel Oxides

We report on the emergent magnetic state of (111)-oriented CoCr 2 O 4 ultrathin films sandwiched between Al 2 O 3 spacer layers in a quantum confined geometry. At the two-dimensional crossover, polarized neutron reflectometry reveals an anomalous enhancement of the total magnetization compared to the bulk value. Synchrotron X-ray magnetic circular dichroism measurements demonstrate the appearance of a long-range ferromagnetic ordering of spins on both Co and Cr sublattices. Furthermore, brillouin function analyses and ab-initio density functional theory calculations further corroborate that the observed phenomena are due to the strongly altered magnetic frustration invoked by quantum confinement effects, manifested by the onset of a Yafet–Kittel-type ordering as the magnetic ground state in the ultrathin limit, which is unattainable in the bulk.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

Bulk Fermi surfaces of the Dirac type-II semimetallic candidate NiTe 2

Here, we present a study on the Fermi surface of the Dirac type-II semimetallic candidate NiTe 2 via the temperature and angular dependence of the de Haas–van Alphen (dHvA) effect measured in single crystals grown through Te flux. In contrast to its isostructural compounds like PtSe 2 , band-structure calculations predict NiTe 2 to display a tilted Dirac node very close to its Fermi level that is located along the Γ to A high-symmetry direction within its first Brillouin zone. The angular dependence of the dHvA frequencies is found to be in agreement with the first-principles calculations when the electronic bands are slightly shifted with respect to the Fermi level (ε F ), and therefore provide support for the existence of a Dirac type-II node in NiTe 2 . Nevertheless, we observed mild disagreements between experimental observations and density functional theory (DFT) calculations as, for example, nearly isotropic and light experimental effective masses. This indicates that the dispersion of the bands is not well captured by DFT. Despite the coexistence of Dirac-like fermions with topologically trivial carriers, samples of the highest quality display an anomalous and large either linear or sublinear magnetoresistivity. Finally, this suggests that Lorentz invariance breaking Dirac-like quasiparticles dominate the carrier transport in this compound.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

The Importance of Avoided Crossings in Understanding High Valley Degeneracy in Half‐Heusler Thermoelectric Semiconductors

Abstract Half‐Heusler (hH) compounds are promising candidates for inexpensive, low‐toxicity thermoelectric materials. It is well known that engineering electronic bands with high valley degeneracy is an effective approach for enhancing the performance of thermoelectric materials, and there are several routes for achieving high valley degeneracy in hH systems. For instance, there are multiple locations in the first Brillouin zone where the valence band maximum can be found (at the Γ‐, L‐, or W‐point), and there are two competing low‐lying conduction bands at the X‐point, where the conduction band minimum is located. By converging the multiple valence band and conduction band extrema, the valley degeneracy, and hence, performance of these materials can be improved. Here, group theoretical and tight‐binding approaches, in addition to first‐principles density functional theory calculations, are used to study the chemical origins of various band extrema in both the n‐type and p‐type compounds, with particular focus on ZrNiSn and NbFeSb. Specifically, the importance of avoided crossings is explained. The results of this work can be used to better understand and develop design strategies for engineering better performing hH thermoelectrics.

Brod, Madison K.↗
DOE OSTI2018

Two Topologically Distinct Dirac-Line Semimetal Phases and Topological Phase Transitions in Rhombohedrally Stacked Honeycomb Lattices

Three-dimensional topological semimetals can support band crossings along one-dimensional curves in the momentum space (nodal lines or Dirac lines) protected by structural symmetries and topology. We consider rhombohedrally (ABC) stacked honeycomb lattices supporting Dirac lines protected by time-reversal, inversion and spin rotation symmetries. For typical band structure parameters there exists a pair of nodal lines in the momentum space extending through the whole Brillouin zone in the stacking direction. We show that these Dirac lines are topologically distinct from the usual Dirac lines which form closed loops inside the Brillouin zone. In particular, an energy gap can be opened only by first merging the Dirac lines going through the Brillouin zone in a pairwise manner so that they turn into closed loops inside the Brillouin zone, and then by shrinking these loops into points. We show that this kind of topological phase transition can occur in rhombohedrally stacked honeycomb lattices by tuning the ratio of the tunneling amplitudes in the directions perpendicular and parallel to the layers. We also discuss the properties of the surface states in the different phases of the model.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2024

Phonon Thermal Transport in UO 2 via Self-Consistent Perturbation Theory

Computing thermal transport from first-principles in UO 2 is complicated due to the challenges associated with Mott physics. Here, we use irreducible derivative approaches to compute the cubic and quartic phonon interactions in UO 2 from first principles, and we perform enhanced thermal transport computations by evaluating the phonon Green’s function via self-consistent diagrammatic perturbation theory. Our predicted phonon lifetimes at T = 600 K agree well with our inelastic neutron scattering measurements across the entire Brillouin zone, and our thermal conductivity predictions agree well with previous measurements. Finally, both the changes due to thermal expansion and self-consistent contributions are nontrivial at high temperatures, though the effects tend to cancel, and interband transitions yield a substantial contribution.

36 MATERIALS SCIENCE↗
NASA NTRS1976

Bragg interactions in periodic media

The interaction of electromagnetic waves of wavelength lambda with periodic structures of spatial period lambda are studied. The emphasis of the work is on Bragg interactions where lambda approximately equal to 2 lambda/N and the Bragg order N takes on the values 1, 2,.... An extended coupled waves (ECW) theory is developed for the case N greater or equal to 2 and the results of the theory are found to compare favorably with the exact results of Floquet theory. Numerous numerical results are displayed as Brillouin diagrams for the first few Bragg orders. Moreover, explicit expressions for coupling coefficients, bandgap shifts and bandgap widths are derived for singly periodic media. Particular note is taken of phase speeding effects.

Jaggard, D. L.↗
DOE OSTI2018

Reduced electronic correlation effects in half substituted Ba(Fe 1-x Co x ) 2 As 2

In this work, we report a comprehensive study of the tridimensional nature and orbital character of the low-energy electronic structure in 50% Cobalt doped Ba(Fe 1-x Co x ) 2 As 2 ( d 6.5 ), by using polarization- and photon energy-dependent angle-resolved photoemission spectroscopy. An extra electron-like Fermi surface is observed around the Brillouin zone boundary compared with isoelectronic K y Fe 2-x Se 2 ( d 6.5 ). The bands near the Fermi level (E F ) are mainly derived from Fe/Co 3 d t 2g orbitals, revealing visible dispersions along the k z direction. In combination with the local density approximation and the dynamical mean-field theory calculations, we find that the As 4 p bands are non-renormalized and the whole 3d band needs to be renormalized by a “single” factor of ~1.6, indicating moderate electronic correlation effects. The “single” factor description of the correlation strength among the different 3 d orbitals is also in sharp contrast to orbital-dependent correlation effects in BaFe 2 As 2 . Our findings indicate a remarkable reduction of correlation effects with little difference among 3 d orbitals in BaFeCoAs 2 , due to the increased filling of the electronic 3 d shell in the presence of significant Hund's coupling. Finally, the results support that the electronic correlation effects and multiple orbital physics play an important role in the superconductivity of the 122 system and in other ferropnictides.

36 MATERIALS SCIENCE↗
DOE OSTI2018

Two-dimensional ferroelectric topological insulators in functionalized atomically thin bismuth layers

We introduce a class of two-dimensional (2D) materials that possess coexisting ferroelectric and topologically insulating orders. Such ferroelectric topological insulators (FETIs) occur in noncentrosymmetric atomic layer structures with strong spin-orbit coupling (SOC). Here, we showcase a prototype 2D FETI in an atomically thin bismuth layer functionalized by CH 2 OH, which exhibits a large ferroelectric polarization that is switchable by a ligand molecule rotation mechanism and a strong SOC that drives a band inversion leading to the topologically insulating state. An external electric field that switches the ferroelectric polarization also tunes the spin texture in the underlying atomic lattice. Moreover, the functionalized bismuth layer exhibits an additional quantum order driven by the valley splitting at the K and K' points in the Brillouin zone stemming from the symmetry breaking and strong SOC in the system, resulting in a remarkable state of matter with the simultaneous presence of the quantum spin Hall and quantum valley Hall effect. These phenomena are predicted to exist in other similarly constructed 2D FETIs, thereby offering a unique quantum material platform for discovering novel physics and exploring innovative applications.

2-dimensional systems↗