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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 127 records · Page 7
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Quantum Versus Classical Switching Dynamics of Driven Dissipative Kerr Resonators

Here, we report a first-principles study of the driven dissipative dynamics for Kerr oscillators in the mesoscopic regime. This regime is characterized by large Kerr nonlinearity, realized here using the nonlinear kinetic inductance of a large array of Josephson junctions. The experimentally measured nonlinear resonance lineshapes of the junction array modes show significant deviations from steady-state numerical predictions, and necessitate time-dependent numerical simulations indicative of strong measurement-induced dephasing in the system arising from the large cross-Kerr effect between array modes. Analytical and numerical calculations of switching rate corroborate this by showing the emergence of a slow time scale, which is much longer than the linear decay rate and is set by fluctuation-induced switching times in the bistable regime. Furthermore, our analysis shows that the usual quantum-activated escape treatment is inadequate for prediction of the switching rates at large frequency shifts caused by strong nonlinearities, necessitating a quantum treatment that utilizes the full system Liouvillian. Based on our analysis, we identify a universal crossover parameter that delineates the regimes of validity of semiclassical and quantum descriptions, respectively. Our work shows how dynamical switching effects in strongly nonlinear systems provide a platform to study quantum-to-classical transitions.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

No evidence for a strong decrease of planetesimal accretion in old white dwarfs

ABSTRACT A large fraction of white dwarfs are accreting or have recently accreted rocky material from their planetary systems, thereby ‘polluting’ their atmospheres with elements heavier than helium. In recent years, the quest for mechanisms that can deliver planetesimals to the immediate vicinity of their central white dwarfs has stimulated a flurry of modelling efforts. The observed time evolution of the accretion rates of white dwarfs through their multi-Gyr lifetime is a crucial test for dynamical models of evolved planetary systems. Recent studies of cool white dwarf samples have identified a significant decrease of the mass accretion rates of cool, old white dwarfs over Gyr time-scales. Here, we revisit those results using updated white dwarf models and larger samples of old polluted H- and He-atmosphere white dwarfs. We find no compelling evidence for a strong decrease of their time-averaged mass accretion rates for cooling times between 1 and 8 Gyr. Over this period, the mass accretion rates decrease by no more than a factor of the order of 10, which is one order of magnitude smaller than the decay rate found in recent works. Our results require mechanisms that can efficiently and consistently deliver planetesimals inside the Roche radius of white dwarfs over at least 8 Gyr.

Blouin, Simon (ORCID:0000000296321436)↗
DOE OSTI2024

Fast permeability measurement for tight reservoir cores using only initial data of the one chamber pressure pulse decay test

Here, in this study, a mathematical model for fast determination of the permeabilities of tight rocks using measurements taken from the initial period of the One Chamber Pressure Pulse Decay (OC-PPD) test is presented. The model applies to measurements taken both before and after the pressure pulse front has reached the downstream end of the specimen. The analytical solutions for the pressure decay in the upstream chamber are derived based on a parabolic arc approximation of pore pressure distribution along the test specimen. This approximation allows converting the initial–boundary value problem of fluid diffusion in the specimen, governed by partial differential equations, to a system of ordinary differential equations that can be easily solved by explicit formulae. Thus, an explicit formula for the pressure decay rate is obtained, which enables inverse analysis of the initial experimental data to estimate the rock permeability. The proposed method expedites the pulse decay test as it does not require the system to reach equilibrium. The method is validated with three sets of experimental data of the OC-PPD test using helium as the diffusing fluid, for which the relative error of the permeability is found to be less than 6%. This method is particularly useful if the equilibrium time of the pulse decay test for rock specimens with permeabilities in the range of nano-Darcy takes hours or days.

early-time solution↗
DOE OSTI2020

The dark matter interpretation of the 3.5-keV line is inconsistent with blank-sky observations

Observations of nearby galaxies and galaxy clusters have reported an unexpected x-ray emission line around 3.5 kilo–electron volts (keV). Proposals to explain this line include decaying dark matter—in particular, that the decay of sterile neutrinos with a mass around 7 keV could match the available data. If this interpretation is correct, the 3.5-keV line should also be emitted by dark matter in the halo of the Milky Way. We used more than 30 megaseconds of XMM-Newton (X-ray Multi-Mirror Mission) blank-sky observations to test this hypothesis, finding no evidence of the 3.5-keV line emission from the Milky Way halo. We set an upper limit on the decay rate of dark matter in this mass range, which is inconsistent with the possibility that the 3.5-keV line originates from dark matter decay.

Dessert, Christopher↗
DOE OSTI2022

Energy-resolved and time-dependent unimolecular dissociation of hydroperoxyalkyl radicals (˙QOOH)

Hydroperoxyalkyl radicals (˙QOOH) are transient intermediates in the atmospheric oxidation of volatile organic compounds and combustion of hydrocarbon fuels in low temperature (<1000 K) environments. The carbon-centered ˙QOOH radicals are a critical juncture in the oxidation mechanism, but have generally eluded direct experimental observation of their structure, stability, and dissociation dynamics. Recently, this laboratory demonstrated that a prototypical ˙QOOH radical [˙CH 2 (CH 3 ) 2 COOH] can be synthesized by an alternative route, stabilized in a pulsed supersonic expansion, and characterized by its infrared (IR) spectroscopic signature and unimolecular dissociation rate to OH radical and cyclic ether products. The present study focuses on a partially deuterated ˙QOOD analog ˙CH 2 (CH 3 ) 2 COOD, generated in the laboratory by H-atom abstraction from partially deuterated tert-butyl hydroperoxide, (CH 3 ) 3 COOD. IR spectral features associated with jet-cooled and isolated ˙QOOD radicals are observed in the vicinity of the transition state (TS) barrier leading to OD radical and cyclic ether products. Furthermore, the overtone OD stretch (2ν OD ) of ˙QOOD is identified by IR action spectroscopy with UV laser-induced fluorescence detection of OD products. Direct time-domain measurement of the unimolecular dissociation rate for ˙QOOD (2ν OD ) extends prior rate measurements for ˙QOOH. Partial deuteration results in a small increase in the TS barrier predicted by high level electronic structure calculations due to changes in zero-point energies; the imaginary frequency is unchanged. Comparison of the unimolecular decay rates obtained experimentally with those predicted theoretically for both ˙QOOH and ˙QOOD confirm that unimolecular decay is enhanced by heavy-atom tunneling involving simultaneous O–O bond elongation and C–C–O angle contraction along the reaction pathway.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2026

Durable Thin‐Film Porous Transport Electrodes for High Current Density PEM Water Electrolysis

Proton exchange membrane water electrolyzers rely on relatively expensive Ir-based catalysts for efficient and durable hydrogen production. To reduce system costs, Ir loadings can be reduced if performance and durability are maintained. Sputter deposition is a readily scalable method to synthesize uniform, low-loading catalyst layers with controlled composition. A catalyst applied directly to the porous transport layer can have advantages for performance, manufacturing simplicity, and catalyst recovery. Suitable porous transport layer porosity can minimize activity losses when reducing loadings. Here, methods are presented to deposit metallic Ir as well as amorphous and rutile Ir oxides. The activity and durability of these materials in the porous transport electrode architecture is evaluated. The metallic and amorphous forms have better initial activity, however, operation at 3 A cm −2 with 0.1 mg Ir cm −2 shows that only rutile IrO 2 maintains performance beyond 100 h with a 50 mV improvement after 700 h. A >10x reduced dissolution rate is shown for rutile IrO 2 . With a low-porosity transport layer and 0.4 mg Ir cm −2 , a steady-state voltage decay rate of 6 µV h −1 is achieved. The results demonstrate that sputter-deposited rutile IrO 2 porous transport electrodes with low Ir loading can be operated at high current density to reduce hydrogen production costs.

08 HYDROGEN↗
DOE OSTI2020

Comparison of fluence-rate determination techniques for the Advanced Test Reactor-Critical Facility

A technique using small, enriched uranium-aluminum alloy monitors to measure fission rates in fuel plate assembly reactors was developed at the Idaho National Laboratory Radiation Measurements Laboratory in support of Advanced Test Reactor Critical (ATR-C) Facility irradiations. Previous measurements were performed to determine the correlation between the beta-particle activity and the fission rate in the U-Al monitors following irradiation. The American Society for Testing and Materials (ASTM) has established a standard practice E704 for determining neutron fluence rate by radioactivation of depleted uranium by measuring the concentration of fission-products in irradiated uranium monitors. Rather than measuring the beta-particle decay from fission-products, the decay rate of fission-products is determined by gamma-ray spectroscopy. The feasibility of using a method adapted from the ASTM standard practice E704 was investigated for ATR-C irradiations and compared to the present method by analyzing a subset of 21 monitor wires using both methods. The resulting calculated fission rates agreed with an average standard deviation of 7.45%, within the average combined measurement error of 9.05%. Practical considerations such as expected fluence-rates, sample activity, and counting-time were compared between the two methods and the sources of error for each method were investigated. Quality assurance measurements utilizing the modified ASTM standard method are recommended for future test irradiation, but gross-beta-particle counting remains the most practical solution for ATR-C fluence-rate determination.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2023

${\Lambda}_c^{+}$ polarimetry using the dominant hadronic mode

The polarimeter vector field for multibody decays of a spin-half baryon is intro duced as a generalisation of the baryon asymmetry parameters. Using a recent amplitude analysis of the ${\Lambda}_c^{+}$ → $pK^-π^+$ decay performed at the LHCb experiment, we compute the distribution of the kinematic-dependent polarimeter vector for this process in the space of Mandelstam variables to express the polarised decay rate in a model-agnostic form. The obtained representation can facilitate polarisation measurements of the ${\Lambda}_c^{+}$ baryon and eases inclusion of the ${\Lambda}_c^{+}$ → $pK^-π^+$ decay mode in hadronic amplitude analyses.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

The Standard Model Theory of Neutron Beta Decay

We review the status of the Standard Model theory of neutron beta decay. Particular emphasis is put on the recent developments in the electroweak radiative corrections. Given that some existing approaches give slightly different results, we thoroughly review the origin of discrepancies, and provide our recommended value for the radiative correction to the neutron and nuclear decay rates. The use of dispersion relation, lattice Quantum Chromodynamics, and an effective field theory framework allows for high-precision theory calculations at the level of 10 –4 , turning neutron beta decay into a powerful tool to search for new physics, complementary to high-energy collider experiments. We offer an outlook to the future improvements.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2020

Global description of $β$ – decay with the axially deformed Skyrme finite-amplitude method: Extension to odd-mass and odd-odd nuclei

Here we use the finite-amplitude method (FAM), an efficient implementation of the quasiparticle random phase approximation, to compute $β$-decay rates with Skyrme energy-density functionals for 3983 nuclei, essentially all the medium-mass and heavy isotopes on the neutron-rich side of stability. We employ an extension of the FAM that treats odd-mass and odd-odd nuclear ground states in the equal filling approximation. Our rates are in reasonable agreement both with experimental data where available and with rates from other global calculations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Kaluza-Klein graviton freeze-in and big bang nucleosynthesis

In models featuring extra spatial dimensions, particle collisions in the early Universe can produce Kaluza-Klein gravitons. Such particles will later decay, potentially impacting the process of big bang nucleosynthesis. In this paper, we consider scenarios in which gravity is free to propagate throughout n flat, compactified extra dimensions, while the fields of the Standard Model are confined to a ( 3 + 1 )-dimensional brane. We calculate the production and decay rates of the states that make up the Kaluza-Klein graviton tower and determine the evolution of their abundances in the early Universe. We then go on to evaluate the impact of these decays on the resulting light element abundances. We identify significant regions of previously unexplored parameter space that are inconsistent with measurements of the primordial helium and deuterium abundances. In particular, we find that for the case of one extra dimension (two extra dimensions), the fundamental scale of gravity must be M ⋆ ≳ 2 × 10 13 GeV ( M ⋆ ≳ 1 0 10 GeV ) unless the temperature of the early Universe was never greater than T ∼ 2 TeV ( T ∼ 1 GeV ). For larger values of n , these constraints are less stringent. For the case of n = 6 , for example, our analysis excludes all values of M ⋆ less than ∼ 10 6 GeV , unless the temperature of the Universe was never greater than T ∼ 3 TeV . The results presented here severely limit the possibility that black holes were efficiently produced through particle collisions in the early Universe’s thermal bath. Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2023

How Long Does the Hydrogen Atom Live?

It is possible that the proton is stable while atomic hydrogen is not. This is the case in models with new particles carrying baryon number which are light enough to be stable themselves, but heavy enough so that proton decay is kinematically blocked. Models of new physics that explain the neutron lifetime anomaly generically have this feature, allowing for atomic hydrogen to decay through electron capture on a proton. We calculate the radiative hydrogen decay rate involving the emission of a few hundred keV photon, which makes this process experimentally detectable. In particular, we show that the low energy part of the Borexino spectrum is sensitive to radiative hydrogen decay, and turn this into a limit on the hydrogen lifetime of order 10 30 s or stronger. For models where the neutron mixes with a dark baryon, X, this limits the mixing angle to roughly 10 –11 , restricting the n → XY branching to 10 –4 , over a wide range of parameter space.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2022

Black hole induced false vacuum decay: the role of greybody factors

We study false vacuum decay catalyzed by black holes. We consider a toy two-dimensional model of a scalar field with an unstable potential in the background of a dilaton black hole. A realistic black hole in four dimensions possesses the potential barrier for linear field perturbations. We model this barrier — the greybody factor — for spherically-symmetric perturbations in the toy model by adding a coupling between the scalar field and dilaton. We compute analytically the decay rate for the black hole in thermal equilibrium (Hartle-Hawking state) and for the radiating black hole in empty space (Unruh state). Our results show that, contrary to the Hartle-Hawking vacuum, the decay probability of the Unruh vacuum remains exponentially suppressed at all black hole temperatures. We argue that this result holds also in four dimensions.

2D Gravity↗
DOE OSTI2025

Search for resonance-enhanced C P and angular asymmetries in the Λ c + → p μ + μ − decay at LHCb

The first measurement of the C P asymmetry of the decay rate ( A C P ) and the C P average ( Σ A FB ) and C P asymmetry ( Δ A FB ) of the forward-backward asymmetry in the muon system of Λ c + → p μ + μ − decays is reported. The measurement is performed using a data sample of proton-proton collisions, recorded by the LHCb experiment from 2016 to 2018 at a center-of-mass energy of 13 TeV, which corresponds to an integrated luminosity of 5.4 fb − 1 . The asymmetries are measured in two regions of dimuon mass near the ϕ -meson mass peak. The dimuon-mass integrated results are A C P = ( − 1.1 ± 4.0 ± 0.5 ) % , Σ A FB = ( 3.9 ± 4.0 ± 0.6 ) % , Δ A FB = ( 3.1 ± 4.0 ± 0.4 ) % , where the first uncertainty is statistical and the second systematic. The results are consistent with the conservation of C P symmetry and the Standard Model expectations. © 2025 CERN, for the LHCb Collaboration 2025 CERN

Aaij, R. (ORCID:0000000305331952)↗
DOE OSTI2024

Pure-Water-Fed Forward-Bias Bipolar Membrane CO 2 Electrolyzer

Coupling renewable electricity to reduce carbon dioxide (CO 2 ) electrochemically into carbon feedstocks offers a promising pathway to produce chemical fuels sustainably. While there has been success in developing materials and theory for CO 2 reduction, the widespread deployment of CO 2 electrolyzers has been hindered by challenges in the reactor design and operational stability due to CO 2 crossover and (bi)carbonate salt precipitation. Herein, we design asymmetrical bipolar membranes assembled into a zero-gap CO 2 electrolyzer fed with pure water, solving both challenges. By investigating and optimizing the anion-exchangelayer thickness, cathode differential pressure, and cell temperature, the forward-bias bipolar membrane CO 2 electrolyzer achieves a CO faradic efficiency over 80% with a partial current density over 200 mA cm –2 at less than 3.0 V with negligible CO 2 crossover. In addition, this electrolyzer achieves 0.61 and 2.1 mV h –1 decay rates at 150 and 300 mA cm –2 for 200 and 100 h, respectively. Postmortem analysis indicates that the deterioration of catalyst/polymer– electrolyte interfaces resulted from catalyst structural change, and ionomer degradation at reductive potential shows the decay mechanism. Furthermore, all these results point to the future research direction and show a promising pathway to deploy CO 2 electrolyzers at scale for industrial applications.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Unimolecular dissociation dynamics of electronically excited HCO(Ã 2 A"): rotational control of nonadiabatic decay

The photoinduced unimolecular decay of the electronically excited HCO(Ã 2 A") is investigated in a combined experimental–theoretical study. The molecule is excited to the (1, n 2 , 0) combination bands, which decay via Renner–Teller coupling to the ground electronic state. The rovibrational state distribution of the CO fragment was measured via the high-n Rydberg H-atom time-of-flight method and calculated using a wave packet method on an accurate set of potential energy surfaces. It is shown that the non-adiabatic decay rate is strongly modulated by the HCO rotational angular momentum, which leaves unique signatures in the product state distribution. Finally, the experimentally observed bimodal rotational distribution of the dominant CO(v = 0) fragment is likely due to decay of different vibronic states populated by the excitation and modulated by the excited state lifetime, which is in turn controlled by the parent rotational quantum number.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

First implementation of gyrokinetic exact linearized Landau collision operator and comparison with models

Gyrokinetic simulations are fundamental to understanding and predicting turbulent transport in magnetically confined fusion plasmas. Previous simulations have used model collision operators with approximate field-particle terms of unknown accuracy and/or have neglected collisional finite Larmor radius (FLR) effects. We have implemented the linearized Fokker–Planck collision operator with exact field-particle terms and full FLR effects in a gyrokinetic code (GENE). The new operator, referred to as “exact” in this paper, allows the accuracy of model collision operators to be assessed. The conservative Landau form is implemented because its symmetry underlies the conservation laws and the H-theorem, and enables numerical methods to preserve this conservation, independent of resolution. The implementation utilizes the finite-volume method recently employed to discretize the Sugama collision model in GENE, allowing direct comparison between the two operators. Results show that the Sugama model appears accurate for the growth rates of trapped electron modes (TEMs) driven only by density gradients, but appreciably underestimates the growth rates as the collisionality and electron temperature gradient increase. The TEM turbulent fluxes near the nonlinear threshold using the exact operator are similar to the Sugama model for the n e = d ln T e /d ln n e = 0 case, but substantially larger than the Sugama model for the n e = 1 case. The FLR effects reduce the growth rates increasingly with wavenumber deepening a “valley” at the intermediate binormal wavenumber as the unstable mode extends from the TEM regime to the electron temperature gradient instability regime. Application to the Hinton–Rosenbluth problem shows that zonal flows decay faster as the radial wavenumber increases and the exact operator yields weaker decay rates.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗