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DOE OSTI2023

Phonon mixing in the charge density wave state of ScV6Sn6

Abstract Kagomé metals are widely recognized, versatile platforms for exploring topological properties, unconventional electronic correlations, magnetic frustration, and superconductivity. In the R V 6 Sn 6 family of materials ( R = Sc, Y, Lu), ScV 6 Sn 6 hosts an unusual charge density wave ground state as well as structural similarities with the A V 3 Sb 5 system ( A = K, Cs, Rb). In this work, we combine Raman scattering spectroscopy with first-principles lattice dynamics calculations to reveal phonon mixing processes in the charge density wave state of ScV 6 Sn 6 . In the low temperature phase, we find at least four new peaks in the vicinity of the V-containing totally symmetric mode near 240 cm −1 suggesting that the density wave acts to mix modes of P 6/ m m m and $$R\bar{3}m$$ R 3 ¯ m symmetry - a result that we quantify by projecting phonons of the high symmetry state onto those of the lower symmetry structure. We also test the stability of the short-range ordered density wave state under compression and propose that both physical and chemical pressure quench the effect. We discuss these findings in terms of symmetry and the structure-property trends that can be unraveled in this system.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

DOE OSTI2020

Lattice phase shifts and mixing angles for an arbitrary number of coupled channels

We present a lattice method for determining scattering phase shifts and mixing angles for the case of an arbitrary number of coupled channels. The proposed method combines a spherical wall boundary condition and a channel-mixing auxiliary potential to extract the full-rank S-matrix from the radial wave functions. We consider the scattering problem of two spin-1 bosons interacting with a test potential involving up to four coupled channels. For this benchmark system, the phase shifts and mixing angles are shown to agree on the lattice and in the continuum. Our method should allow to extend previous two-channel nuclear lattice EFT simulations to mixing of more than two partial waves.

Bovermann, Lukas↗

DOE OSTI2022

Lower‐Hybrid Wave Structures and Interactions With Electrons Observed in Magnetotail Reconnection Diffusion Regions

Abstract We investigate waves close to the lower‐hybrid frequency in 12 magnetotail reconnection electron diffusion region (EDR) events with guide field levels of near‐zero to 30%. In about half of the events, the wave vector has a small component along the current sheet normal, consistent with known lower‐hybrid drift wave properties, but the perpendicular magnetic field fluctuations can be comparable or greater than the parallel component, a feature unique to the waves inside and adjacent to EDRs. Another new wave property is that the wave vector has a significant component along the current sheet normal in some events and completely along the normal for one event. In 1/4 of the events, the term has a significant contribution to the wave electric field, possibly a feature of lower‐hybrid waves more likely to exist in the diffusion region than further away from the X‐line. Electron temperature variations are correlated with the wave potential, due to wave electric field acceleration and crossings at the corrugated separatrix region with different amounts of mixing between reconnection inflowing and outflowing populations. The latter also leads to the anti‐correlation between parallel and perpendicular temperature components. Using four‐spacecraft measurements, the magnetic field line twisting is demonstrated by the correlated fluctuations in and . The lower‐hybrid wave in the EDR of weak guide field reconnection may be generated near separatrices and penetrate to the mid‐plane or locally generated, and the latter possibility is beyond the prediction of previous reconnection simulations.

79 ASTRONOMY AND ASTROPHYSICS↗

DOE OSTI2020

Precise β branching-ratio measurement for the 0 + → 0 + superallowed decay of 34 Ar

We have measured the branching ratio for the superallowed 0 + → 0 + β transition from 34 Ar to be 0.9448(8), and determined its ft value to be 3058.1(28) s, a result with ±0.09% precision, which is a factor of three improvement over the previous result based on current world data. The ft-value ratio for the mirror pair of superallowed transitions 34 Ar → 34 Cl and 34 Cl → 34 S, becomes the most precise yet measured and, in a sensitive test of the method used to calculate the isospin-symmetry-breaking correction, δ C , it agrees well with the ratio as calculated with Woods-Saxon radial wave functions. This confirms the method used in the most recent survey of superallowed decays to extract V ud , the up-down quark-mixing element of the Cabibbo-Kobayashi-Maskawa matrix. Additionally, our branching-ratio results for the four observed Gamow-Teller branches to 1 + states in 34 Cl are shown to agree well with shell-model calculations based on the same effective interactions that were used in the determination of δ C .

39 ≤ A ≤ 58↗

DOE OSTI2025

51 V NMR evidence for interlayer-modulated charge order and a first-order low-temperature transition in CsV 3 ⁢Sb 5

Charge order in the kagome superconductor CsV 3 ⁢Sb 5 exhibits a complex three-dimensional organization and intermediate-temperature anomalies whose bulk character has remained unsettled. We use orientation-dependent 51 V NMR as a site-selective probe to determine the stacking of the charge density wave (CDW) state and its thermal evolution. Below 𝑇 CDW ≈ 94K, the field-linear splitting of the 51 V central transition together with the anisotropy of the Knight shift tensor identify an interlayer-modulated 3⁢𝑞 CDW whose local environments are consistent with a four-layer 2 × 2 × 4 stacking with mixed trihexagonal/Star-of-David distortions, in agreement with synchrotron x-ray determinations. For comparison, RbV 3 ⁢Sb 5 serves as a reference exhibiting a uniform trihexagonal 2 × 2 × 2 stacking, allowing us to isolate features unique to the 2 × 2 × 4 state in CsV 3 ⁢Sb 5 . With 𝐻 0 ∥ 𝑐, the 51 V quadrupolar satellites through the intermediate temperature scale near 𝑇 CO ≈ 65K reorganize into two well-resolved electric-field-gradient manifolds that coexist over a finite interval; their relative spectral weights interchange on cooling while the total integrated satellite intensity remains conserved and 𝜈 𝑄 within each manifold is nearly temperature independent. The coexistence without critical broadening, together with conserved intensity, provides bulk evidence consistent with a first-order charge-order transition near 𝑇 CO . Our measurements do not resolve whether this lower-temperature transition corresponds to a distinct in-plane order or a reorganization of the 3⁢𝑞 state; rather, they delimit this window and provide bulk, site-resolved constraints that connect prior reported anomalies to a thermodynamic first-order transition.

Wang, Xiaoling [California State Univ., East Bay, ↗

DOE OSTI2024

Non-resonant picosecond three-wave mixing in the gas phase

We report on the experimental observation of non-resonant, second-order optical sum-frequency generation (SFG) in five different atomic and molecular gases. The measured signal is attributed to a SFG process by characterizing its intensity scaling and its polarization behavior. We show that the electric quadrupole mechanism cannot explain the observed trends and suggest a mechanism based on symmetry breaking along the incident beam path arising from laser-induced species ground state number density gradients. Our results demonstrate that the SFG is about four orders of magnitude stronger than the third-harmonic generation (THG) and independent from any externally applied electric fields. In conclusion, these features make this method suitable for gas number density measurements at the picosecond time scale in reactive flows and plasmas.

LaCombe, Grayson↗

DOE OSTI2024

Extreme terahertz magnon multiplication induced by resonant magnetic pulse pairs

Nonlinear interactions of spin-waves and their quanta, magnons, have emerged as prominent candidates for interference-based technology, ranging from quantum transduction to antiferromagnetic spintronics. Yet magnon multiplication in the terahertz (THz) spectral region represents a major challenge. Intense, resonant magnetic fields from THz pulse-pairs with controllable phases and amplitudes enable high order THz magnon multiplication, distinct from non-resonant nonlinearities such as the high harmonic generation by below-band gap electric fields. Here, we demonstrate exceptionally high-order THz nonlinear magnonics. It manifests as 7th-order spin-wave-mixing and 6th harmonic magnon generation in an antiferromagnetic orthoferrite. We use THz two-dimensional coherent spectroscopy to achieve high-sensitivity detection of nonlinear magnon interactions up to six-magnon quanta in strongly-driven many-magnon correlated states. The high-order magnon multiplication, supported by classical and quantum spin simulations, elucidates the significance of four-fold magnetic anisotropy and Dzyaloshinskii-Moriya symmetry breaking. Moreover, our results shed light on the potential quantum fluctuation properties inherent in nonlinear magnons.

36 MATERIALS SCIENCE↗

DOE OSTI2023

Four-dimensional dynamics of multirotational transition stimulated rotational Raman scattering in air

Stimulated rotational Raman scattering in air is a powerful parasitic process that degrades high intensity laser beams and pulses propagated over significant distances. Conversely, it is used beneficially in the context of Raman lasers. Through this inelastic scattering process, laser photons are converted to higher (anti-Stokes) or lower (Stokes) energies, according to rotational mode transitions in nitrogen and oxygen diatomic molecules. The full wave-mixing problem involves numerous frequencies, and it is consistently assumed that only one rotational mode contributes to the conversion process. We instead present a dynamic 4D multirotational model that is implemented in a parallelized manner within the Virtual Beamline++ optical modeling package allowing high-resolution 4D studies. We highlight the effect that spontaneous emission plays in large and small beam-width setups, even in the highly saturating regime. The weaker transition modes play a large role in the persistent dynamics and can lead to complex spatiotemporal coupling through nonlinear competition of the modes. We highlight how and why these weaker modes persist, how the size and shape of speckle patterns depends highly on the initial beam profile, and how weaker modes can transiently become stronger as a result of such competition.

47 OTHER INSTRUMENTATION↗

DOE OSTI2025

Effects of Atmosphere and Ocean Horizontal Model Resolution on Tropical Cyclone and Upper-Ocean Response Forecasts in Four Major Hurricanes

A coupled atmosphere–ocean model is necessary for tropical cyclone (TC) prediction to accurately characterize ocean feedback on atmospheric processes within the TC environment. Here, the ECMWF coupled global model is run at horizontal resolutions from 9 to 1.4 km in the atmosphere, as well as 25 and 8 km in the ocean, to identify how resolution impacts forecast accuracy of four observed major TCs in the Atlantic: Irma, Florence, Teddy, and Ida. Most of the resolutions used here are unprecedented for global models. GOES-16 and synthetic aperture radar (SAR) satellite images and best track data are used for atmospheric validation. Salinity and temperature observations from Air-Launched Autonomous Micro-Observer (ALAMO) floats are used to validate modeled upper-ocean response, including mixed layer deepening, sea surface cooling, and near-inertial waves in the wakes of TCs. Increasing atmospheric resolution leads to more realistic TC structure and stronger winds, significantly improving TC intensity forecasts and modestly improving track errors. Ocean resolution impacts the upper-ocean response but does not influence atmospheric forecasts for the fast-moving TCs considered here. Stronger mixing, sea surface cooling, and near-inertial oscillations are found for both higher atmosphere and ocean resolutions, provided the initial upper-ocean state is the same for the two ocean resolutions. Whether this agrees better with the ALAMO observations also depends on the realism of the initial upper-ocean state in the model, emphasizing the importance of ocean initialization for the accurate upper-ocean response. Overall, the model at all resolutions correctly predicts stronger mixing, surface cooling, and near-inertial oscillation amplitudes to the right of a TC center, as observed by ALAMO floats.

Atmosphere-ocean interaction↗

DOE OSTI2021

Integrating CVMix into GOTM (v6.0): a consistent framework for testing, comparing, and applying ocean mixing schemes

Abstract. The General Ocean Turbulence Model (GOTM) is a one-dimensional water column model, including a set of state-of-the-art turbulence closure models, and has widely been used in various applications in the ocean modeling community. Here, we extend GOTM to include a set of newly developed ocean surface vertical mixing parameterizations of Langmuir turbulence via coupling with the Community Vertical Mixing Project (CVMix). A Stokes drift module is also implemented in GOTM to provide the necessary ocean surface waves information to the Langmuir turbulence parameterizations, as well as to facilitate future development and evaluation of new Langmuir turbulence parameterizations. In addition, a streamlined workflow with Python and Jupyter notebooks is also described, enabled by the newly developed and more flexible configuration capability of GOTM. The newly implemented Langmuir turbulence parameterizations are evaluated against theoretical scalings and available observations in four test cases, including an idealized wind-driven entrainment case and three realistic cases at Ocean Station Papa, the northern North Sea, and the central Baltic Sea, and compared with the existing general length scale scheme in GOTM. The results are consistent with previous studies. This development extends the capability of GOTM towards including the effects of ocean surface waves and provides useful toolsets for the ocean modeling community to further study the effects of Langmuir turbulence in a broader scope.

58 GEOSCIENCES↗

DOE OSTI2023

Goldstone bosons and fluctuating hydrodynamics with dipole and momentum conservation

We develop a Schwinger-Keldysh effective field theory describing the hydrodynamics of a fluid with conserved charge and dipole moments, together with conserved momentum. The resulting hydrodynamic modes are highly unusual, including sound waves with quadratic (magnon-like) dispersion relation and subdiffusive decay rate. Hydrodynamics itself is unstable below four spatial dimensions. We show that the momentum density is, at leading order, the Goldstone boson for a dipole symmetry which appears spontaneously broken at finite charge density. Unlike an ordinary fluid, the presence or absence of energy conservation qualitatively changes the decay rates of the hydrodynamic modes. This effective field theory naturally couples to curved spacetime and background gauge fields; in the flat spacetime limit, we reproduce the “mixed rank tensor fields” previously coupled to fracton matter.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2024

Self-similar Reynolds-averaged mechanical–scalar turbulence models for reshocked Richtmyer–Meshkov instability-induced mixing in the small Atwood number limit

Analytical self-similar solutions to two-, three-, and four-equation Reynolds-averaged mechanical–scalar turbulence models describing incompressible turbulent Richtmyer–Meshkov instability-induced mixing in planar geometry derived in the small Atwood number limit are extended to construct models for reshocked Richtmyer–Meshkov mixing. In this study, the models are based on the turbulent kinetic energy K and its dissipation rate ε, together with the scalar variance S and its dissipation rate χ modeled either differentially or algebraically. The three- and four-equation models allow for a simultaneous description of mechanical and scalar mixing, i.e., mixing layer growth and molecular mixing. Mixing layer growth parameters and other physical observables were obtained explicitly as functions of the model coefficients and were used to calibrate the model coefficients. Here, the solutions for the singly shocked Richtmyer–Meshkov case for the mixing layer width and the turbulent fields are used to construct piecewise-continuous generalizations of these quantities for times after reshock. For generality, the post-reshock mixing layer width is not assumed to grow with the same power-law as the pre-reshock width, and an impulsive approximation applied to Rayleigh–Taylor instability growth is used to establish the expression for the post-reshock width. A four-equation model is then used to illustrate the spatiotemporal behavior of the mean and turbulent fields and late-time turbulent equation budgets across the mixing layer. The reference solutions derived here can provide systematic calibrations and better understanding of mechanical–scalar turbulence models and their predictions for reshocked Richtmyer–Meshkov instability-induced turbulent mixing in the very large Reynolds number limit.

42 ENGINEERING↗

DOE OSTI2024

Shallow Bound States and Hints for Broad Resonances with Quark Content b ¯ c ¯ u d in B − D ¯ and B * − D ¯ Scattering from Lattice QCD

We present the first determination of the energy dependence of the B − D ¯ and B * − D ¯ isospin-0, S -wave scattering amplitudes both below and above the thresholds using lattice QCD, which allows us to investigate rigorously whether mixed bottom-charm b ¯ c ¯ u d tetraquarks exist as bound states or resonances. The scattering phase shifts are obtained using Lüscher’s method from the energy spectra in two different volumes. To ensure that no relevant energy level is missed, we use large, symmetric 7 × 7 and 8 × 8 correlation matrices that include, at both source and sink, B ( * ) − D ¯ scattering operators with the lowest three or four possible back-to-back momenta in addition to local b ¯ c ¯ u d operators. We fit the energy dependence of the extracted scattering phase shifts using effective-range expansions. We observe sharp peaks in the B ( * ) − D ¯ scattering rates close to the thresholds, which are associated with shallow bound states, either genuine or virtual, a few MeV or less below the B ( * ) − D ¯ thresholds. In addition, we find hints for resonances with masses of order 100 MeV above the thresholds and decay widths of order 200 MeV. Published by the American Physical Society 2024

Alexandrou, Constantia↗

DOE OSTI2023

Modeling and optimization of steady flow of natural gas and hydrogen mixtures in pipeline networks

Here, we extend the canonical problems of simulation and optimization of steady-state gas flows in pipeline networks with compressors to the transport of mixtures of highly heterogeneous gases injected throughout a network. Our study is motivated by proposed projects to blend hydrogen generated using clean energy into existing natural gas pipeline systems as part of efforts to reduce the reliance of energy systems on fossil fuels. Flow in a pipe is related to endpoint pressures by a basic Weymouth equation model, with an ideal gas equation of state, where the wave speed depends on the hydrogen concentration. At vertices, in addition to mass balance, we also consider mixing of incoming flows of varying hydrogen concentrations. The problems of interest are the heterogeneous gas flow simulation (HGFS), which determines system pressures and flows given fixed boundary conditions and compressor settings, as well as the heterogeneous gas flow optimization (HGFO), which extremizes an objective by determining optimal boundary conditions and compressor settings. We examine conditions for uniqueness of solutions to the HGFS, as well as compare and contrast mixed-integer and continuous nonlinear programming formulations for the HGFO. We develop computational methods to solve both problems, and examine their performance using four test networks of increasing complexity.

08 HYDROGEN↗

DOE OSTI2025

Amplitude analysis of ψ3686→γKS0KS0

Using (2712 ± 14) × 106ψ(3686) events collected with the BESIII detector, we perform the first amplitude analysis of the radiative decay ψ3686→γKS0KS0$$ \psi (3686)\to \gamma {K}_S^0{K}_S^0 $$ within the mass region MKS0KS0<2.8$$ {M}_{K_S^0{K}_S^0}<2.8 $$ GeV/c2. Employing a one-channel K-matrix approach for the description of the dynamics of the KS0KS0$$ {K}_S^0{K}_S^0 $$ system, the data sample is well described with four poles for the f0-wave and three poles for the f2-wave. The determined pole positions are consistent with those of well-established resonance states. The observed f0 and f2 states are found to be in agreement with those produced in radiative J/ψ decays. The production behaviors of f0 and f2 poles in ψ3686→γKS0KS0$$ \psi (3686)\to \gamma {K}_S^0{K}_S^0 $$ are qualified with their residues and the converted branching fractions. By comparing with J/ψ→γKS0KS0$$ J/\psi \to \gamma {K}_S^0{K}_S^0 $$ decay, the ratios Bψ3686→γf0,2BJ/ψ→γf0,2$$ \frac{\mathcal{B}\left(\psi (3686)\to \gamma {f}_{0,2}\right)}{\mathcal{B}\left(J/\psi \to \gamma {f}_{0,2}\right)} $$ are determined, which provides crucial experimental inputs on the internal structure of the f0,2 states, especially their potential mixing with glueball components.

Ablikim, M↗

DOE OSTI2021

Roadmap for Advanced Power System Measurements

Conditions in the electric power grid are changing rapidly. Changes are driven, in particular, by the increased penetration of renewable resources in the generation mix. Part of the solution to dealing with the changing conditions is the better use of measurement systems, taking advantage of the better understanding of measurements that was heralded by digital technology. Another part of the solution is the communication of samples of the directly observable voltages and currents by means of continuous point-on-wave values. The increased bandwidth capability of such a system allows more complicated measurement models to be built at the point of use. Additional measurements and analyses can then be performed. This Roadmap hinges on these two aspects of measuring: improved measurements supported by high-bandwidth (raw data) communications. Following an introduction to the overall subject, the report explores the impact of what can be thought of as the digital revolution in measurement. In essence, that revolution has served to clarify ideas about measurement and is continuing to lead to improved processes. An extensive survey of the relevant literature was performed . Webinars were held to learn from the wider community of practitioners. Based on this information, a number of gaps were identified whose continued existence would hamper the solution of the challenges now facing measurement and communication in the power grid. The underlying value propositions are interoperability (presently not very satisfactory in many measurements); greater (and less challenging) adoption of distributed energy resources; and improved international competitiveness. Underlying all that, of course, is progress toward a more reliable and resilient power system. The identified gaps were addressed in four major thrusts: technology deployment and demonstration, education, instrumentation testing and standards, and analytical methods. For each of the thrusts, multiple goals are defined to guide the implementation. The thrusts were designed to close gaps and unlock high-value use cases. After discussing the literature review, gap analysis, high-value use cases, and research thrusts in chapters 2-5, the report culminates in chapter 6 with a roadmap that links each aspect together to form a unified plan. Developing a research portfolio aligned with this plan will ensure that advanced measurement systems are in place to support reliable operation of the power system as it modernizes.

24 POWER TRANSMISSION AND DISTRIBUTION↗

DOE OSTI2020

An Intelligent Adaptable Monitoring Package. Final Report

The “Intelligent Adaptable Monitoring Package” project was a four-year effort that demonstrated the feasibility of integrated sensing packages at tidal and wave energy sites. Such integration is generally required by the breadth of sensors required to understand environmental effects at marine energy sites and the operational difficulty of deploying, maintaining, and recovering such sensors. Over the course of the project, the Adaptable Monitoring Package (AMP) was deployed in multiple settings, each corresponding to a project budget period: - Budget Period 1: Demonstration of cabled deployment at Pacific Northwest National Laboratory’s Marine Science Laboratory. The deployment highlighted AMP hardware endurance over a 4-month deployment in a tidally-dominated environment and laid the groundwork for machine learning algorithms to detect and classify targets present in active sonar data. - Budget Period 2: Demonstration of an autonomous deployment at PacWave South off the coast of Newport, Oregon. The deployment highlighted the stability of AMP hardware and software, with the autonomous package collecting data on a duty cycle over a 1.5-month deployment. - Budget Period 3: Demonstration of an autonomous deployment powered by a wave energy converter at the U.S. Navy’s Wave Energy Test Site. The deployment highlighted the potential of wave energy to power ocean observatories and led to the development of machine learning algorithms to detect and classify targets in optical camera data. In aggregate, this project’s greatest success was demonstrating the AMP’s flexibility in a range of deployment scenarios. Each budget period represented a “first of a kind” demonstration of integrated instrumentation – cabled AMP, autonomous AMP, wave-energy powered AMP – and each deployment helped to identify and set goals for the next. Further, despite the exploratory nature of these deployments, each one achieved high system up-time and proved that flexible integration of multiple sensors in a single package represents a viable strategy for marine energy environmental monitoring. The key lessons learned from the project are: - Without continuous power, either from a shore cable or in situ source, many of the benefits of integration are lost (If continuous power is not available, the ability to detect rare events is lost, as is the ability to minimize the risk of behavioral changes through adaptive sensing. However, even on a duty cycle, there is still value in being able to acquire synchronous data from multiple sensors.); and - Observations from a moving platform present substantially greater data processing challenges than those from stationary platforms. Finally, these deployments also demonstrate an important truth: successful integration alone does not guarantee that relevant data are collected. To grow the knowledge base about environmental interactions with marine energy converters, integrated systems, like the AMP, need to include the right sensor mix and connect the data pipelines to effective processing algorithms. These deployments establish a strong foundation for future collaborations with the environmental research community: not only to understand the environmental effects of marine energy, but also to improve our general ability to study life in the sea.

16 TIDAL AND WAVE POWER↗

DOE OSTI2020

Utilizing Commercial Submersible Mixer Pumps for Sludge Removal in Savannah River Site's Tank 26 - 20289

The Savannah River Site (SRS) Liquid Waste System (LWS) safely manages, stores, treats, and dispositions liquid radioactive waste. The LWS consists of 51 underground waste storage tanks (eight of which are operationally closed and filled with grout), waste evaporators, treatment facilities, and solidification facilities, known as the Defense Waste Processing Facility (DWPF) and Saltstone Production Facility (SPF). One of the waste storage tanks, Tank 26, was placed into service in 1980 as an F Tank Farm (FTF) Evaporator Feed Tank. From 1980 to 2013, Tank 26 received F Canyon receipts and dilute supernate that was then transferred to the 242-16F FTF Evaporator for volume reduction. In 2013, the steam tube bundle failed in the FTF Evaporator, and the decision was made not to repair/resume evaporator operation. During operation of Tank 26, solids built up to a level of 2.03 m in the tank with a volume of 1062.9 kL. Due to the evaporator failure and subsequent shutdown, the solids in Tank 26 were selected to feed Sludge Batch 10, which is collected and prepped prior to being sent to DWPF for final disposition. To accomplish solids removal, Commercial Submersible Mixer Pumps (CSMPs) were selected to slurry the solids in preparation to be sent to Tank 51. Four CSMPs were installed in Tank 26 with each one installed in a separate quadrant of Tank 26. This work would mark the first deployment of CSMPs in an SRS waste tank. The CSMPs were developed in response to operational issues from previous mixing pumps and budgetary constraints. The CSMPs use the concept of modifying commercially available equipment for nuclear waste applications. The CSMPs consist of a 230-horsepower submersible mixing pump (manufactured by GPM, Inc.) joined to a mast fabricated at SRS. For this application, Savannah River Remediation (SRR) design services was challenged to provide a mast design that required no steel superstructure support system on top of Tank 26. Also, SRR design services provided a simplified Tank 26 riser interface that did not require extensive machine parts to adjust height of the suction screen of the CSMP within the tank. Other design improvements include no requirements for tank top radiation monitors and no requirements for flushing of the CSMPs during startup/shutdown operations. The CSMPs were operated at an initial height of 2.29 m above the Tank 26 bottom for 10 days. After sludge sounding, the CSMPs were lowered to a height of 1.52 m with no issues due to proper work planning and the simplified riser interface. With the CSMPs lowered to a level of 1.52 meters above the tank bottom, the CSMPs were operated for 12 days and another sounding was performed. The sounding level came back matching the disturbance depth results of the first pump run. Chemistry samples were analyzed while the tank was left to settle. The analysis revealed enough weight percent solids to provide good feed to Sludge Batch 10. Also, the results revealed the supernate within the mixture would provide good salt solution feed to Salt Waste Processing Facility (SWPF) Salt Batch 3. So, the plan was modified to let the disturbed solids settle and decant the salt solution for addition to SWPF Salt Batch 3. Then water will be added back to Tank 26, and the CSMPs run in order to wash the solids to decrease settling time prior to being sent to Tank 51 for Sludge Batch 10. Utilizing CSMPs for waste removal in an SRS Tank has provided a cost-effective means for further waste removal efforts. In addition, the CSMPs are easier to operate by utilizing a robust and simplified design. The CSMPs performed quite well with no process shutdown or delays during operation. As a result, CSMPs are integral to the future of removing radioactive waste from storage tanks at SRS. (authors)

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗