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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 127 records · Page 7
All sourcesNASA NTRSDOE OSTI
DOE OSTI2023

Reducing ion diffusion at atmospheric pressure through intermingled positive and negative ions

Increasing ion molecule reaction times for ambient ionization techniques can increase sensitivity of detection. Longer reaction times result in an increase in analyte signal relative to the reactant ion signal, however with a subsequent decrease in the total ion intensity. This loss in the total number of ions reaching the detector limits the extent to which increased reaction time can improve detection in practical applications. In this study ion loss was measured using either electric fields or gas flow to control ion transit time. Ion transit times ranged from 40 ms to 8s, which resulted in ion densities ranging from 5 x 10 6 to 2 x 10 4 ions/cm 3 , respectively. These results provide insights into practical reaction time limitations or experimental boundaries when exploring sensitivity enhancements in ambient ionization. When exploring longer reaction times with an atmospheric flow tube coupled to a mass spectrometer (AFT-MS), an additional corona discharge ionization source of the same polarity was added in an attempt to increase total ion signal, but no improvement in signal was observed. This observation suggested that there was a maximum ion density being reached by the corona discharge that could not be increased by adding more of the same polarity ions. A hypothesis was that intermingling both polarities of ions would reduce ion loss and increase the measured ion signal. When two corona discharge sources—one each of positive and negative polarity—were used simultaneously in an AFT-MS, the total ion signal of either polarity measured by the MS was approximately double the current from a single corona discharge source. An increase in the negative ion signal was also observed when ~10 parts-per-trillion vapor levels of an explosive (RDX) were introduced. In this case both the nitrate reactant ions and the RDX signal more than doubled with the addition of a corona discharge source producing positive ions. When intermingling positive and negative ions, an increase in ion current was also observed when the AFT was coupled directly to a Faraday detector or to an ion mobility spectrometer. This was the first demonstration of interfacing the AFT to an IMS. The observations and developments from this work will help in creating more portable instruments with improved sensitivity for detection of chemicals.

47 OTHER INSTRUMENTATION↗
NASA NTRS1998

Spatial Distribution of Ionospheric Plasma and Field Structures in the High-Latitude F Region

Ion density and velocity measurements from the Dynamics Explorer 2 (DE 2) spacecraft are used to obtain the average magnetic local time versus invariant latitude distribution of irregularities in the high-latitude F region ionosphere. To study the small-scale structure and its relationship to background conditions in the ionosphere, we have formed a reduced database using 2-s (approx. = 16 km) segments of the ion density and velocity data. The background gradients associated with each 2-s segment and the spectral characteristics, such as power at 6 Hz (approx. = 1.3 km) and spectral index, are among the reduced parameters used in this study. The relationship between the observed plasma structure and its motion is complex and dependent on the externally applied fields as well as locally generated plasma structure. The evolution of plasma structures also depends critically on the conductivity of the underlying ionosphere. Observations indicate an enhancement of irregularity amplitudes in two spatially isolated regions in both the ion density and the velocity. Convective properties seem to play a more important role in winter hemisphere where smaller-scale structures are maintained outside the source regions. (Delta)V irregularity amplitudes are enhanced in the cusp and the polar cap during northward interplanetary magnetic field regardless of season. The power in (Delta)V is usually higher than that associated with local polarization electric fields, suggesting that the observed structure in (Delta)N/N is strongly influenced by (Delta)V structure applied to large density gradients.

Kivanc, O.↗
NASA NTRS1963

A model of the quiet ionosphere.

Analysis of electron and ion density measurements obtained with rockets suggests simple model of the quiet ionosphere

IONOSPHERIC ELECTRON DENSITY↗
NASA NTRS1977

A hollow cathode hydrogen ion source

High current density ion sources have been used to heat plasmas in controlled thermonuclear reaction experiments. High beam currents imply relatively high emission currents from cathodes which have generally taken the form of tungsten filaments. A hydrogen ion source is described which was primarily developed to assess the emission current capability and design requirements for hollow cathodes for application in neutral injection devices. The hydrogen source produced ions by electron bombardment via a single hollow cathode. Source design followed mercury ion thruster technology, using a weak magnetic field to enhance ionization efficiency.

Sovey, J. S.↗
NASA NTRS1986

Evidence of high densities and ion outflows in the polar cap during the recovery phase

The composition and characteristics of the polar cap plasma for an Oct. 14, 1981 outflow of polar wind ions are examined using data from the DE 1 satellite. The on-board instruments included a plasma wave instrument, a retarding ion mass spectrometer (RIMS) and a high altitude plasma instrument (HAPI). The outflow took place at an altitude of about 19,000 km at a magnetic local time of about midnight. The total plasma density measured was about 50/cu cm, which was an order of magnitude higher than normally recorded at that location and altitude. The background hydrogen plasma was disturbed by highly collimated flows of hydrogen and oxygen ions. The H(+) ions had a mean energy of 0.15 eV and a density of 6-10/cu cm. The O(+) ions had an average density of 20/cu cm and a temperature of 0.26 eV. The total flux of outflowing H(+) and O(+) was about 10 million/sq cm per sec. The HAPI data indicated that the O(+) ions appeared in the dayside ionosphere and the H(+) ions detected by the RIMS originated in the nightside polar cap.

Gallagher, D. L.↗
NASA NTRS2001

Polar Observations of Topside Field-Aligned O+ Flows and Auroral Forms

Measurements of thermal O+ ion densities, field-aligned velocities, and fluxes from the Thermal Ion Dynamics Experiment (TIDE) on Polar obtained near 5000 km altitude over the Southern Hemisphere are compared with auroral images from the Ultraviolet Imager (UVI). Three passes were selected for analysis in this paper based on data availability from the TIDE and UVI instruments. Results indicate upward O+ flows in the cleft region but downward O+ flows in the polar cap region. Also, the O+ ion density follows a decreasing trend from the poleward side of the cusp region into the nightside aurora region. The magnitude of the downward O+ parallel velocities increases from dayside to nightside across the polar cap boundary. The upflows tend to occur over or near auroral forms, while the downflows are seen in relatively dark regions, such as the polar cap. These results are consistent with a cleft ion fountain source for the polar cap O+ ions. In the nightside polar cap, the results indicate a transition from downward to upflowing field-aligned O+ ions near boundaries of bright auroral arcs.

Stevenson, B. A.↗
NASA NTRS2000

POLAR Observations of Topside Field-Aligned O+ Flows and Auroral Forms

Measurements of thermal O (sup +) ion densities, field-aligned velocities, and fluxes from the Thermal Ion Dynamics Experiment (TIDE) on POLAR obtained near 5000 km altitude over the Southern hemisphere are compared with auroral images from the Ultra Violet Imager (UVI). We find upward O (sup +) flows in the cleft region, but subsonic O (sup +) downflows in the polar cap region. Also, the O (sup +) ion density follows a decreasing trend from the poleward side of the cusp region into the nightside aurora region. The magnitude of the downward O (sup +) parallel velocities increases from dayside to nightside across the polar cap boundary. The upflows tend to occur over or near auroral forms, while the downflows are seen in relatively dark regions, such as the polar cap. These results are consistent with a cleft ion fountain source for the polar cap O (sup +) ions. In the nightside polar cap, the results indicate a transition from downward to upflowing field-aligned O (sup +) ions near boundaries of bright auroral arcs.

Stevenson, B. A.↗
NASA NTRS1993

Plasma transport in the equatorial ionosphere during the great magnetic storm of March 1989

We have modeled plasma transport in the low-latitude and equatorial ionosphere during the great magnetic storm of March 1989. Our goal was to provide a consistent explanation for the DMSP (Defense Meteorological Satellite Program) observations of dramatic decreases in ion density and rapid ion drifts in the low latitude ionosphere over South America during the storm. The modeling effort supports the hypothesis that abnormally large upward drifts lifted F region plasma above the satellite's altitude and created the density depletions observed by DMSP. Modeled O(+) densities at the satellite's altitude have a strong qualitative resemblance to DMSP observations. Both the model and the observations indicate a deep density trough with extremely sharp boundaries surrounding the equator. The widths of both the modeled and the observed equatorial troughs increase with time. Vertical ion drifts predicted by the model also have been compared with DMSP measurements. Like the observed vertical drifts, the modeled drifts reversed sign near the trough boundaries. The modeled vertical drifts are of the same order and direction as the vertical component of E x B convection near the equator, but of opposite direction (downward) near the trough boundaries and outside of the trough.

Rasmussen, C. E.↗
NASA NTRS1960

Ionospheric Measurements Using Environmental Sampling Techniques

Two rockets were flown to peak altitudes of 220 km in September 1959 to test various methods planned for future measurements of ionization parameters in the ionosphere, exosphere, and interplanetary plasma. The experiments used techniques which sample the ambient environment in the immediate vicinity of the research vehicle. Direct methods were chosen since indirect propagation techniques do not provide the temperatures of charged particles, are insensitive to ion densities, and cannot measure local electron densities under all conditions. Very encouraging results have been obtained from a preliminary analysis of data provided by one of the two flights. A new rf probe technique was successfully used to determine the electron density profile. This was indicated by its agreement with the results of a companion cw propagation experiment, particularly when the probe data were corrected for the effects of the ion sheath which surrounds the vehicle. The characteristics of this sheath were determined directly in flight by an electric field meter which provided the sheath field, and by a Langmuir probe which measured the total potential across the sheath. The electron temperatures deduced from the Langmuir probe data are greater than the neutral gas temperatures previously measured for the same location and season, but these measurements possibly were taken under different atmospheric conditions. Ion densities were calculated from the ion trap data for several altitudes ranging from 130 to 210 km and were found to be within 20 percent of the measured electron densities.

Bourdeau, R. E.↗
NASA NTRS1982

Ion thruster charge-exchange plasma flow

The electron bombardment ion thruster has been under development for a number of years and during this time, studies of the plasmas produced by the thrusters and their interactions with spacecraft have been evaluated, based on available data. Due to diagnostic techniques used and facility effects, there is uncertainty as to the reliability of data from these early studies. This paper presents data on the flow of the charge-exchange plasma produced just downstream of the thruster's ion optics. The 'end-effect' of a cylindrical Langmuir probe is used to determine ion density and directed ion velocity. Results are compared with data obtained from a retarding potential analyzer-Faraday cup.

Carruth, M. R., Jr.↗
NASA NTRS1986

Global large scale structures in the F region

Measurements of neutral densities, temperatures and ion density and temperature by the Atmosphere Explorer C and E satellites exhibit fluctuations made up of coherent waves of scale size from hundreds to thousands of kilometers. The fluctuations in the AE-C data are found at times of low magnetic activity to extend from the auroral region in one hemisphere across the equator to the corresponding region in the other hemisphere with little change in apparent wavelength. The fluctuations in the AE-E data similarly exhibit at times of low magnetic activity nearly uniform wave structure encircling the equatorial belt. Typical examples of waves of more than 1000 km apparent wavelength in both the AE-C and AE-E data are presented. These observations during quiet times may be explained by a system of quasi-stationary waves excited by the auroral belts that are distributed about the Earth possibly with tidal or sub-tidal periods and scale lengths determined by the structure of the belts. According to this interpretation, Traveling Ionospheric Disturbance (TID's) are manifestations of transient wave systems moving past a ground observatory that result from changes in magnetic activity with periods and scale sizes associated with the regions of enhanced auroral activity. Some evidence suggesting tidal-like stationary waves from the Millstone Hill incoherent scatter radar is presented.

Gross, S. H.↗
NASA NTRS1995

The High Latitudes in the International Reference Ionosphere; Meeting C4 of Commission C, COSPAR Scientific Assembly, 30th, Hamburg, Germany, July 11-21, 1994

An international conference on high-latitude ionospheric modeling produced 27 papers in the areas of ionospheric mapping, electron density and distribution, ion density and distribution, ionospheric storems, ionospheric composition, and ionospheric sounding techniques. Upgrades to the International Reference Ionosphere (IRI) model were proposed in several papers.

Rawer, K.↗
DOE OSTI2024

Molecular Dynamics Study of the Effect of Grafting Density on Ion Diffusivity in a MARTINI Coarse-Grained Strong Polyelectrolyte Brush

Because surface-grafted polyelectrolyte brushes (PEBs) are responsive to external stimuli, such as electric fields and ionic strength, PEBs are attractive for applications ranging from drug delivery to separation technologies. Essential to PEB utilization is understanding how critical parameters like grafting density (σ) impact the PEB structure and the dynamics of the PEB and counterions. To study the effect of σ on PEB and the counterion structure and dynamics, we fine-tune a coarse-grained model that retains the chemical specificity of a strong polyelectrolyte, poly[(2-(methacryloyloxy)ethyl) trimethylammonium chloride] (PMETAC), using the MARTINI force field. Using “salt-free” conditions where the counterion concentration balances the charge on the brush, we build coarse-grained (CG) molecular dynamics simulations for MARTINI PMETAC brushes (N = 150 monomers; M W = 31.2 kg/mol) at experimentally relevant values of σ = 0.05, 0.10, 0.20, and 0.40 chains/nm 2 . Using 5 μs simulations, we investigate the effects of grafting density on the PEB structure, ion dissociation dynamics, polymer mobility, and counterion diffusivity. Results show that competition between electrostatic interactions, steric hindrance, and polymer mobility controls counterion diffusivity. Finally, the interplay of these factors leads to diffusivity that depends non-monotonically on σ, with counterion diffusivity peaking at an intermediate σ = 0.10 chains/nm 2 .

36 MATERIALS SCIENCE↗
NASA NTRS2004

Cross-Scale Coupling in the Inner Magnetosphere

Magnetosphere-ionosphere (MI) coupling has interested scientists for decades and, in spite of experimental and theoretical research efforts, is still one of the least well-known dynamic processes in space plasma. The reason for this is that the numerous physical processes associated with MI coupling occur over multiple spatial lengths and temporal scales. One typical example of MI coupling is small- and large-scale ring current (RC) electrodynamic coupling. In this talk, we will address the two primary issues of RC electrodynamic coupling: (1) RC self-consistent coupling with electromagnetic ion cyclotron (EMIC) waves (small-scale electrodynamic coupling) and (2) RC self-consistent MI coupling that includes calculation of the magnetospheric electric field (large-scale electrodynamic coupling). We also will emphasize the role of the heavy ions in the number of wave-particle interaction magnetospheric processes. In particular, we will discuss some of the experimental and theoretical studies that have investigated the role of the heavy ions (mainly He(+) and O(+)) in generation and propagation of electromagnetic ion cyclotron waves and their contribution to the heating of magnetospheric electrons and ions. The more recent studies have also shown that the heavy ions can greatly contribute to a generation of lower hybrid waves, ring current precipitation phenomena, and the overall energy redistribution in the inner magnetosphere. Using newly developed 2.5-dimensional particle-in-cell simulations, we study the energization and nonlinear coupling of different plasma waves in the presence of the heavy ions. We have shown that the high frequency wave modes critically depend on the heavy ion density and irrespective of the driven wave modes, both the light and heavy ions undergo significant transverse acceleration. But for the large heavy-ion densities, even the electrons are significantly accelerated in the parallel direction by the waves below the LH frequency.

Khazanov, G. V.↗
NASA NTRS2004

The Role of the Heavy Ions in the Wave Magnetospheric Phenomena

This talk will emphasize the role of the heavy ions in the number of wave-particle interaction magnetospheric processes. In particular, we will discuss some of the experimental and theoretical studies that have investigated the role of the heavy ions (mainly He(+) and O(+)) in generation and propagation of electromagnetic ion cyclotron waves and their contribution to the heating of magnetospheric electrons and ions. The more recent studies have also shown that the heavy ions can greatly contribute to a generation of lower hybrid waves, ring current precipitation phenomena, and the overall energy redistribution in the inner magnetosphere. Using newly developed 2.5-dimensional particle-in-cell simulations, we study the energization and nonlinear coupling of different plasma waves in the presence of the heavy ions. We have shown that the high frequency wave modes critically depend on the heavy ion density and irrespective of the driven wave modes, both the light and heavy ions undergo significant transverse acceleration. But for the large heavy-ion densities, even the electrons are significantly accelerated in the parallel direction by the waves below the LH frequency.

Khazanov, G. V.↗
DOE OSTI2024

Bayesian inference of electron density and ion temperature profiles from neutral beam and halo Balmer- α emission at Wendelstein 7-X

By employing Bayesian inference techniques, the full electron density profile from the plasma core to the edge of Wendelstein 7-X (W7-X) is inferred solely from neutral hydrogen beam and halo Balmer- α (H α ) emission data. The halo is a cloud of neutrals forming in the vicinity of the injected neutral beam due to multiple charge exchange reactions. W7-X is equipped with several neutral hydrogen beam heating sources and an H α spectroscopy system that views these sources from different angles and penetration depths in the plasma. As the beam and halo emission form complex spectra for each spatial point that are non-linearly dependent on the plasma density profile and other parameters, a complete model from the neutral beam injection and halo formation through to the spectroscopic measurements is required. The model is used here to infer electron density profiles for a range of common W7-X plasma scenarios. The inferred profiles show good agreement with profiles determined by the Thomson scattering and interferometry diagnostics across a broad range of absolute densities without any changes to the input or fitting parameters. The time evolution of the density profile in a discharge with continuous core density peaking is successfully reconstructed, demonstrating sufficient spatial resolution to infer strongly shaped profiles. Furthermore, it is shown as a proof of concept that the model is also able to infer the main ion temperature profile using the same data set.

forward modeling↗