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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 127 records · Page 7
All sourcesNASA NTRSDOE OSTI
DOE OSTI2018

Relationship between laser energy input, microstructures and magnetic properties of selective laser melted Fe-6.9%wt Si soft magnets

Highlights: • Effect of laser energy input on magnetic properties of SLM Fe-6.9%wt.Si is described; • Magnetic properties can be described as function of as-built microstructure after stress-relief post-treatment; • Samples with density >99% and strong crystallographic texture along BD have the best magnetic properties; • At very high laser energy, a strong cube texture forms that deteriorates the magnetic properties. - Abstract: Selective Laser Melting (SLM), a powder-bed Additive Manufacturing technology, can be used in combination with high temperature post-annealing to produce high-silicon steel parts characterised by quasi-static magnetic properties comparable to those of commercial electrical steel. However, the role of the as-built microstructure on the magnetic properties is still unexplored. Therefore, in this study the effect of the energy input of the processing laser on the magnetic properties of the material is investigated. The magnetic properties are determined for 4 mm-high rings obtained using three laser energy input values that provide a good compromise in terms of porosity and crack formation. The best magnetic properties are obtained for the rings built using a value of energy input that produces a strong fibrous crystallographic texture, in which one of the crystallographic <001> axes is preferentially aligned along the build direction. Whether the magnetic properties change with sample direction as a result of the crystallographic texture will be the subject of future research.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Magnetic Texture in Insulating Single Crystal High Entropy Oxide Spinel Films

Magnetic insulators are important materials for a range of next-generation memory and spintronic applications. Structural constraints in this class of devices generally require a clean heterointerface that allows effective magnetic coupling between the insulating layer and the conducting layer. However, there are relatively few examples of magnetic insulators that can be synthesized with surface qualities that would allow these smooth interfaces and precisely tuned interfacial magnetic exchange coupling, which might be applicable at room temperature. In this work, we demonstrate an example of how the configurational complexity in the magnetic insulator layer can be used to realize these properties. The entropy-assisted synthesis is used to create single-crystal (Mg 0.2 Ni 0.2 Fe 0.2 Co 0.2 Cu 0.2 )Fe 2 O 4 films on substrates spanning a range of strain states. These films show smooth surfaces, high resistivity, and strong magnetic responses at room temperature. Furthermore, local and global magnetic measurements further demonstrate how strain can be used to manipulate the magnetic texture and anisotropy. These findings provide insight into how precise magnetic responses can be designed using compositionally complex materials that may find application in next-generation magnetic devices.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2020

High precision magnetic field measurement and mapping of the LEReC 180 degree bending magnet using very low field NMR with hall combined probe (140 - 350 gauss)

The Relativistic Heavy Ion Collider (RHIC) at BNL are using the Low Energy RHIC Electron Cooling (LEReC) to conduct experiments that search for the quantum chromodynamic (QCD) critical point. The first ever electron cooling based on the RF acceleration of electron beams was experimentally demonstrated on April 5, 2019 at LEReC at BNL. The first critical step in obtaining successful 3D non-magnetized cooling of the Au ion bunches in the RHIC cooling section was matching the electron beam energy with a relative error less than 5*10 -4 to the ion beam energy. Part of the LEReC beamline is a dipole magnet that bends the electron beam 180 degree. One of the most outstanding measurement challenges is that the dipole field is so low (≈200 G). Most of the existing NMR probes can only measure fields >400 G. Lower signal-to-noise ratio at low fields is requires the use of larger sample volumes. Working with CAYLAR, a NMR probe has been redesigned and optimized for these low field measurements with high resolution. We report the methods, challenges, and results for extensive magnetic field mappings of the 180 dipole magnet. A combination of NMR and Hall sensors has been successfully implemented to measure uniform field regimes inside the magnet center area and non-uniform field regimes at the magnet ends. Detailed measurement and mapping have been performed at five radii and five heights along the beam trajectory. Meanwhile a finite element magnetic modeling simulation of the magnet using Opera software has been performed. The calculated and measured data are compared, and the calculated data is good reference for measured data over long length mapping from magnet edge to center. The measured magnetic measurement data is directly useful for beam instrumentation, diagnostics and operation.

Magnetic Field Measurement↗
DOE OSTI2025

Dilute magnetic impurity-induced effective phonon magnetic moment in Fe-doped monolayer MoS 2

Realization of large effective phonon magnetic moment in monolayer MoS 2 has established an important route for exploring intriguing magnetic phenomena in a nonmagnetic material. The sizable coupling between the orbital transition and the circularly polarized phonon results in the large effective phonon magnetic moment. In this work, using magneto-Raman spectroscopy, we investigate substitutional doping of magnetic atoms as a tuning knob of the electronic and phononic properties of MoS 2 . We show that Fe-doping polarizes the spin of the conduction bands and introduces a localized Fe band underneath the conduction band. As a result, an additional orbital transition between the Mo 4d and Fe 3d states emerges, producing an orbital-phonon hybridized mode at 283 cm −1 . Our magnetic field dependent measurements demonstrate that this new mode carries 2.8 $\mu_{\mathrm{B}}$ effective phonon magnetic moment, which is comparable to that of the undoped MoS 2 . Moreover, even though a long-range magnetic order is absent in Fe-doped MoS 2 , the local magnetic moment of Fe modifies the nature of the spin fluctuation, producing monotonically increasing quasielastic scattering spectral weight as temperature decreases. Our results highlight two-dimensional dilute magnetic semiconductors synthesized by substitutional doping as a promising material platform to manipulate the phonon magnetic moment through orbital-phonon coupling.

36 MATERIALS SCIENCE↗
DOE OSTI2018

Effect of Mechanical Stresses and Annealing on the Magnetic Structure and the Magnetic Impedance of Amorphous CoFeSiBCr Microwires

The structural and magnetic properties of amorphous ferromagnetic microwires can undergo significant measurements under the action of external mechanical stresses and heat treatment. The study of transformations occurring in this case is important for designing various sensors of mechanical stresses, loading, and temperature and also for inducing in the wires a certain type of magnetic anisotropy that plays a significant role in the realization of various effects in them. In this work, the influence of external stresses and annealing on the processes of the magnetization and the magnetic impedance of Co{sub 71}Fe{sub 5}B{sub 11}Si{sub 10}Cr{sub 3} microwires having a low positive magnetostriction (~10{sup -8}) in amorphous state has been studied. The influence of external stresses leads to a sharp change in the character of the magnetization reversal curve, which was due to the change in the sign of the magnetostriction and the type of magnetic anisotropy. The amplitude of higher harmonics and the value of the magnetic impedance, respectively, are sensitive to mechanical stresses. Elastic stresses in the wires with a partial crystallization do not lead to a marked change in the magnetic properties; however, annealing can lead to a substantial increase in the axial magnetic anisotropy of the wires existing in the stressed state. The experimental results are analyzed in the framework of a magnetostriction model of induced magnetic anisotropy.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Effect of atom substitutions on the magnetic properties in Ce 2 Fe 17 : Toward permanent magnet applications

Due to the rapidly developing technologies and huge market demand, there has been increasing interest internationally in exploring permanent magnet formulations in addition to the well-known Nd 2 Fe 14 B and SmCo 5 /Sm 2 Co 17 . Given Fe's low materials cost and generally high magnetization, Fe-rich rare earth binaries such as Ce 2 Fe 17 comprise a rich “hunting ground” for such new materials. While this compound suffers from a low ordering point and is a heli magnet, these difficulties are easily remedied by the substitution of appropriate amounts of cobalt for Fe, with room-temperature saturation magnetization as high as 1.5 T. In this work, we try to switch the all-important magnetic anisotropy from planar to uniaxial behavior in Ce 2 Fe 17 via 18 h - and 6 c -type atom substitutions with Si, Ir, and numerous other atoms. The uniaxial magnetocrystalline anisotropy is successfully achieved in the 6 c -site-substituted Ce 2 Fe 15 Ir 2 systems, along with large magnetization. We find that iridium substitution, in particular, induces a substantial uniaxial anisotropy of 11.25 MJ/m 3 , which is comparable to most of the current rare earth permanent magnets. Although the iridium substitution is costly, the finding of Ir-triggered uniaxial magnetic anisotropy indicates the potential of Ce–Fe-based alloys for permanent magnets.

36 MATERIALS SCIENCE↗
DOE OSTI2017

Conceptual magnet design study for fusion nuclear science facility [Magnet design study for fusion nuclear science facility]

The Fusion Nuclear Science Facility (FNSF) is a nuclear confinement device to provide the integrated fusion environment with fusion reactor components. The FNSF is the stepping stone to bridge the technical gaps of burning plasma and nuclear science between the International Thermal Nuclear Experimental Reactor (ITER), currently under construction in the south of France, and the demonstration power plant (DEMO). For the next-step fusion reactors, resistive copper magnet cannot be a sustainable solution due to large power consumption in coils of large size needed. Both Low temperature superconductor (LTS) and high temperature superconductor (HTS) are considered for the FNSF magnet design based on the state-of-the-art fusion superconducting magnet technology. Input parameters to FNSF magnet design include magnetic field of 7.5 T at plasma center with a major radius of 4.8 m and minor radius of 1.2 m, and a peak field of over 16 T on the TF coils. The high magnetic field can be achieved by using the high performance ternary Restack Rod Process (RRP) Nb3Sn strands for toroidal field (TF) magnets and a high aspect ratio rectangular cable-in-conduit conductor (CICC) design. The conductor design concept and TF coil winding pack composition and dimension are discussed based on the horizontal maintenance scheme. Neutron radiation limits for the LTS and HTS conductors and electrical insulation materials are reviewed based on the available materials previously tested. The material radiation limits for FNSF magnets are defined as part of the conceptual design studies. In conclusion, the global structural analysis of FNSF magnets based on the radial build was performed to validate feasibility for the plant layout toward horizontal maintenance and global structural integrity of its magnet system.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2016

Towards developing a compact model for magnetization switching in straintronics magnetic random access memory devices

Strain-mediated magnetization switching in a magnetic tunneling junction (MTJ) by exploiting a combination of piezoelectricity and magnetostriction has been proposed as an energy efficient alternative to spin transfer torque (STT) and field induced magnetization switching methods in MTJ-based magnetic random access memories (MRAM). Theoretical studies have shown the inherent advantages of strain-assisted switching, and the dynamic response of the magnetization has been modeled using the Landau-Lifshitz-Gilbert (LLG) equation. However, an attempt to use LLG for simulating dynamics of individual elements in large-scale simulations of multi-megabyte straintronics MRAM leads to extremely time-consuming calculations. Hence, a compact analytical solution, predicting the flipping delay of the magnetization vector in the nanomagnet under stress, combined with a liberal approximation of the LLG dynamics in the straintronics MTJ, can lead to a simplified model of the device suited for fast large-scale simulations of multi-megabyte straintronics MRAMs. In this work, a tensor-based approach is developed to study the dynamic behavior of the stressed nanomagnet. First, using the developed method, the effect of stress on the switching behavior of the magnetization is investigated to realize the margins between the underdamped and overdamped regimes. The latter helps the designer realize the oscillatory behavior of the magnetization when settling along the minor axis, and the dependency of oscillations on the stress level and the damping factor. Next, a theoretical model to predict the flipping delay of the magnetization vector is developed and tested against LLG-based numerical simulations to confirm the accuracy of findings. Lastly, the obtained delay is incorporated into the approximate solutions of the LLG dynamics, in order to create a compact model to liberally and quickly simulate the magnetization dynamics of the MTJ under stress. Using the developed delay equation, the efficiency of the straintronics switching over the STT method is highlighted by analytically investigating the energy-delay trade-off of both methodologies.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2023

Multi-$\mathcal{k}$ magnetic structure and large anomalous Hall effect in candidate magnetic Weyl semimetal NdAlGe

Here, the magnetic structure, magnetoresistance (MR), and Hall effect of the noncentrosymmetric magnetic semimetal NdAlGe are investigated, revealing an unusual magnetic state and anomalous transport properties that are associated with the electronic structure of this compound. The magnetization and MR measurements are both highly anisotropic and indicate an Ising-like magnetic system. The magnetic structure is complex in that it involves two magnetic ordering vectors, including an incommensurate spin density wave and commensurate ferrimagnetic state in zero field. We have discovered a large anomalous Hall conductivity that reaches ≈430 Ω –1 cm –1 , implying that it originates from an intrinsic Berry curvature effect stemming from Weyl nodes found in the electronic structure. These electronic structure calculations indicate the presence of nested Fermi surface pockets with nesting wave vectors like the measured magnetic ordering wave vector and the presence of Weyl nodes in proximity to the Fermi surface. We associate the incommensurate magnetic structure with the large anomalous Hall response to be the result of the combination of Fermi surface nesting and the Berry curvature associated with Weyl nodes.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

Application of a new model of residual magnetization of iron for calculating the deflecting magnet of an accelerator

Allowing for residual magnetization of iron is necessary when calculating the magnetic field of elements of electron-optical channels in charged-particle accelerators because the contribution of residual magnetization to the field in the gap can be on the order of mT. Moreover, the magnitude and sign of this contribution depend on the magnetization process. Earlier, we proposed a model of residual magnetization of iron with the use of a small number of magnetic domain types. Here, an algorithm for magnetic-field calculation with the use of this model is described. The ability of the algorithm was demonstrated for the case of a simplest electromagnet with an O-shaped magnetic circuit. Comparison with the measurement results demonstrated a satisfactory accuracy of allowing for residual magnetization.

43 PARTICLE ACCELERATORS↗
DOE OSTI2022

Milli-magnetic monopole dark matter and the survival of galactic magnetic fields

A bstract Dark sectors with Abelian gauge symmetries can interact with ordinary matter via kinetic mixing. In such scenarios, magnetic monopoles of a broken dark U(1) will appear in our sector as confined milli-magnetically charged objects under ordinary electromagnetism. Halo ellipticity constraints are shown to significantly bound the strength of dark magnetic Coulomb monopole interactions. The bound magnetic monopole ground state, which in vacuum is stable and has no magnetic charge or moment, is shown to become quantum mechanically unstable in the presence of an external, ordinary magnetic field. If these states contribute sizably to the local dark matter density, they extract significant energy from the galactic magnetic field. We revise and extend this “Parker Bound” on galactic magnetic energy loss to milli-magnetic monopoles which leads to the strongest existing constraints on these states, satisfying our halo ellipticity bounds, over a wide range of magnetic monopole masses.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
DOE OSTI2019

Magnetic and magnetic inverse spin Hall effects in a non-collinear antiferromagnet

The spin Hall effect (SHE)1,2,3,4,5 achieves coupling between charge currents and collective spin dynamics in magnetically ordered systems and is a key element of modern spintronics6,7,8,9. However, previous research has focused mainly on non-magnetic materials, so the magnetic contribution to the SHE is not well understood. Here we show that antiferromagnets have richer spin Hall properties than do non-magnetic materials. We find that in the non-collinear antiferromagnet10 Mn3Sn, the SHE has an anomalous sign change when its triangularly ordered moments switch orientation. We observe contributions to the SHE (which we call the magnetic SHE) and the inverse SHE (the magnetic inverse SHE) that are absent in non-magnetic materials and that can be dominant in some magnetic materials, including antiferromagnets. We attribute the dominance of this magnetic mechanism in Mn3Sn to the momentum-dependent spin splitting that is produced by non-collinear magnetic order. This discovery expands the horizons of antiferromagnet spintronics and spin–charge coupling mechanisms.

phonons, thermal conductivity, thermoelectric, spi↗
DOE OSTI2022

The 3D magnetic topology and plasma dynamics in open stochastic magnetic field lines

We report the thermal quench triggered by locked modes is known to be mainly due to open stochastic magnetic field lines connected to the wall boundary. It is essential to understand the 3D structure of open stochastic field lines since it determines the overall plasma dynamics in the system. In this study, we analyze the 3D magnetic topology for two key concepts, the connection length L c and the effective magnetic mirror ratio M eff , and present a comprehensive picture of electron and ion dynamics related to the magnetic topology. The connection length determines the 3D structure of the ambipolar potential, and a sharp potential drop across distinct L c regions induces the E × B transport and mixing across the field line. The confinement of electrons and ions along the field line is determined by the ambipolar potential and [Formula: see text] configuration. Electron and ion temperatures in magnetic hills (M eff < 1) are lower than in magnetic wells (M eff > 1) because particles in magnetic hills are more likely to escape toward the wall boundary along the field line. The mixing between the magnetic wells and hills by E × B and magnetic drift motions results in collisionless detrapping of electrons and ions, which reduces their temperature efficiently. Numerical simulations of two different magnetic configurations demonstrate the importance of the collisionless detrapping mechanism, which could be the main cause of plasma temperature drop during the thermal quench.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Two distinctive regimes in the charge transport of a magnetic topological ultra thin film

Abstract The effect of the magnetic impurities on the charge transport in a magnetic topological ultra-thin film (MTF) is analytically investigated by applying the semi-classical Boltzmann framework through a modified relaxation-time approximation. Our results for the relaxation time of electrons as well as the charge conductivity of the system exhibit two distinct regimes of transport. We show that the generated charge current in a MTF is always dissipative and anisotropic when both conduction bands are involved in the charge transport. The magnetic impurities induce a chirality selection rule for the transitions of electrons which can be altered by changing the orientation of the magnetic impurities. On the other hand, when a single conduction band participates in the charge transport, the resistivity is isotropic and can be entirely suppressed due to the corresponding chirality selection rule. Our findings propose a method to determine an onset thickness at which a crossover from a three-dimensional magnetic topological insulator to a (two-dimensional) MTF occurs.

Sabzalipour, Amir (ORCID:0000000195830880)↗
DOE OSTI2017

Magnetic structure and dispersion relation of the S = 1 2 quasi-one-dimensional Ising-like antiferromagnet BaCo 2 V 2 O 8 in a transverse magnetic field

Here, BaCo 2 V 2 O 8 consists of Co chains in which a Co 2+ ion carries a fictitious spin 1/2 with Ising anisotropy. We performed elastic and inelastic neutron scattering experiments in BaCo 2 V 2 O 8 in a magnetic field perpendicular to the c axis which is the chain direction. With applying magnetic field along the a axis at 3.5 K, the antiferromagnetic order with the easy axis along the c axis, observed in zero magnetic field, is completely suppressed at 8 T, while the magnetic field gradually induces an antiferromagnetic order with the spin component along the b axis. We also studied magnetic excitations as a function of transverse magnetic field. The lower boundary of the spinon excitations splits gradually with increasing magnetic field. The overall feature of the magnetic excitation spectra in the magnetic field is reproduced by the theoretical calculation based on the spin 1/2 XXZ antiferromagnetic chain model, which predicts that the dynamic magnetic structure factor of the spin component along the chain direction is enhanced and that along the field direction has clear incommensurate correlations.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Upper limit for the effect of elastic bending stress on the saturation magnetization of L a 0.8 S r 0.2 Mn O 3

In this study, using polarized neutron reflectometry, we measured the influence of elastic bending stress on the magnetization depth profile of a La 0.8 Sr 0.2 MnO 3 (LSMO) epitaxial film grown on a SrTiO 3 substrate. The elastic bending strain of ±0.03% has no obvious effect on the magnetization depth profile at saturation. This result is in stark contrast to that of (La 1-x Pr x )1-yCayMnO 3 (LPCMO) films for which strain of ±0.01% produced dramatic changes in the magnetization profile and Curie temperature. We attribute the difference between the influence of strain on the saturation magnetization in LSMO (weak or none) and LPCMO (strong) to a difference in the ability of LSMO (weak or none) and LPCMO (strong) to phase separate. Our observation provides an upper limit of tuning LSMO saturation magnetization via elastic strain effect.

36 MATERIALS SCIENCE↗