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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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DOE OSTI2021

Physical Sciences Vistas Issue 3 2021

In this issue, highlights of our contributions to mission operations include descriptions of the following. • How exact and scrupulous planning in concert with sophisticated science enabled a first-ever direct measurement of a radionuclide with a half-life as short as six days. The work, which included operations at the Los Alamos Neutron Science Centers (LANSCE) Weapons Neutron Research Facility and the Isotope Production Facility’s hot cell facility, is a boon for both astrophysics and weapons science. • An introduction to Christie Davis and her role in ensuring the Lab’s execution of simultaneous excellence. • A look at progress by AOT’s Target and Experimental Support Team in reclaiming long-dormant space in a radiological controlled area for new work improving target systems for the Lujan Center. • A story showcasing a cross-organizational effort to minimize the directorate’s legacy and environmental footprint. Staff from across the Lab joined together to ensure the safe and efficient disposal of Rocky Flats legacy waste stored in a transportainer at the Target Fabrication Facility. • How the Lab’s Utilities and Infrastructure experts collaborated with stakeholders in our directorate to safety execute preventive maintenance on the LANSCE mesa’s large electrical substation. The Safe Conduct of Research principles provided a common framework for the planning and process. • A description of the resources called upon and the procedures undertaken by MPA to inventory the division’s time-sensitive chemicals, including the careful and conscientious response of an alert team member when something seemed amiss.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗
DOE OSTI2021

A holistic approach to the optimization of neutron beam transport at the LANSCE facility

An advanced neutron beam collimation system has been developed as part of an effort to optimize neutron beam transport at the Weapons Neutron Research (WNR) Facility, located within the Los Alamos Neutron Science Center (LANSCE). The goal of this work was to develop and demonstrate techniques to tailor neutron delivery in order to provide maximum available flux on sample with a specific beam profile, while simultaneously reducing unwanted background. A holistic approach was taken, upgrading the facility spallation target, facility metrology infrastructure, and flight path shutter insert to support the implementation of this advanced collimation system. Here, modern instruments and software were employed to conduct facility surveys, characterization of as-built geometry of critical components, 3D ray tracing and neutron transport calculations. Beam images and flux measurements were acquired after installation to evaluate the performance of the collimation system and to demonstrate consistent agreement with MCNP simulations which showed an 87% increase of flux on sample while providing suppression of background neutron impingement on the sample frame by 10 3 .

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2024

Commissioning a time-gated camera for fast neutron beamline spatial-energy characterization at LANSCE-WNR spallation source

An energy-resolved fast neutron beam imaging diagnostic has been successfully commissioned at the Weapons Neutron Research (WNR) spallation source within the Los Alamos Neutron Science Center (LANSCE) facility. This diagnostic replaces the existing analog phosphor image plates, which integrate across all neutron energies, as well as other particles, with a near-real-time energy-sensitive imaging capability. The system uses a fast plastic scintillator coupled with an intensified CCD camera. Specifically, the Teledyne Pi-MAX4 camera is coupled with either a 4 mm thick Eljen (EJ) 204 or 228 plastic scintillator. These scintillators are most sensitive to the fast neutrons (0.8-800 MeV) directly from the spallation source rather than low energy background radiation. Experimentally, these plastic scintillators were shown to have sufficiently fast decay to differentiate the bright gamma flash from the spallation neutrons. The spatial resolution is dominated by neutron beam divergence, with minimal additional contributions from scatter and light divergence. The system successfully resolved changes in neutron beam characteristics caused by intentional proton steering variations. Additionally, simulations of scintillator light yield as a function of thickness conducted using PHITS (with Scinful-QMD package) found that increasing scintillator thickness from 4 mm to 6 or 8 mm could potentially increase brightness ~ 3x. This may be explored if there is a need to reduce image acquisition time from several minutes to under one minute.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2022

Physical Sciences Vistas Perspectives on LANSCE Issue 2, 2022

What’s LANSCE? The Los Alamos Neutron Science Center is a facility at the Lab with one of the nation’s most powerful linear accelerators, which is a half-mile in length. What’s an accelerator? An accelerator is a machine that uses electric or time-varying magnetic fields to accelerate nuclear particles to high velocities.

43 PARTICLE ACCELERATORS↗
DOE OSTI2018

Physics design of the next-generation spallation neutron target-moderator-reflector-shield assembly at LANSCE

Here, we discuss the physics design of the next-generation spallation neutron target-moderator-reflector-shield (TMRS) assembly for the Manuel Lujan Jr. Neutron Scattering Center (Lujan Center) at the Los Alamos Neutron Science Center (LANSCE). We developed this TMRS to improve the neutronic performance of the Lujan Center in the intermediate energy range (keV–MeV) enabling a variety of new nuclear physics experiments, as well as increasing the quality of the ongoing experiments. The results of our Monte Carlo optimization study indicate that the new TMRS will generate keV–MeV neutrons with higher intensity and improved time resolution. At the same time, the new design largely maintains its current performance in the cold and thermal ranges supporting materials research. In this article we show that the new TMRS has the potential to enhance the Lujan Center’s experimental capability in a wider interval of energies – cold to intermediate – after its scheduled installation in 2020.

43 PARTICLE ACCELERATORS↗
DOE OSTI2017

The Prompt Fission Neutron Spectrum of 235U for Einc 0.7-5.0 MeV

The Chi-Nu experiment aims to accurately measure the prompt fission neutron spectrum (PFNS) for the major actinides. At the Los Alamos Neutron Science Center (LANSCE), fission can be induced using the white neutron source. Using a two arm time of flight (T.O.F) technique; Chi-Nu presents a preliminary result of the low energy component of the 235U PFNS measured using an array of 22-Lithium glass scintillators.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗
DOE OSTI2023

Laboratory Directed Research and Development Program: FY 2021 Completed Projects

Oak Ridge National Laboratory (ORNL) is the US Department of Energy’s (DOE’s) largest multiprogram science, technology, and energy laboratory. It possesses distinctive capabilities in neutron science, computing, advanced materials, nuclear science and technology, and other fields. Using these capabilities, ORNL conducts basic and applied R&D to support DOE’s overarching mission “to ensure America’s security and prosperity by addressing its energy, environmental and nuclear challenges through transformative science and technology solutions.”1 As a national resource, ORNL also applies its capabilities and skills to specific needs of other federal agencies and customers through the DOE Strategic Partnership Projects (SPP) Program. Information about the laboratory and its programs is available on the ORNL website.2 The Laboratory Directed Research and Development (LDRD) Program at ORNL operates under the authority of the DOE Order 413.2C, “Laboratory Directed Research and Development,”3 which establishes DOE’s requirements for the program while providing the laboratory director broad flexibility for program implementation. The LDRD Program funds are obtained through a charge to all laboratory programs. Although it represents a relatively small portion of the overall research budget, the LDRD Program plays an essential role in maintaining the laboratory’s ability to respond to national needs. The program allows ORNL to improve its distinctive capabilities and to enhance its ability to conduct cutting-edge R&D. In accordance with the DOE order, R&D projects funded through the LDRD Program at ORNL support the following goals: (1) maintain the scientific and technical vitality of the laboratory; (2) enhance the laboratory’s ability to address future DOE missions; (3) foster creativity and stimulate exploration of forefront areas of science and technology; (4) serve as a proving ground for new concepts in R&D; and (5) support high-risk, potentially high-value R&D. This report provides an overview of the LDRD Program at ORNL in FY 2021 and contains summaries of all LDRD research projects that concluded between October 1, 2020, and September 30, 2021.

99 GENERAL AND MISCELLANEOUS↗
DOE OSTI2022

Hadron-Induced Radiation Damage in Fast Heavy Inorganic Scintillators

Fast and heavy inorganic scintillators with suitable radiation tolerance are required to face the challenges presented at future hadron colliders of high energy and intensity. Up to 5 GGy and 5 × 1018 neq/cm2 of one-MeV-equivalent neutron fluence is expected by the forward calorimeter at the Future Hadron Circular Collider. This paper reports the results of an investigation of proton- and neutron-induced radiation damage in various fast and heavy inorganic scintillators, such as LYSO:Ce crystals, LuAG:Ce ceramics, and BaF2 crystals. The experiments were carried out at the Blue Room with 800 MeV proton fluence up to 3.0 × 1015 p/cm2 and at the East Port with one MeV equivalent neutron fluence up to 9.2 × 1015 neq/cm2, respectively, at the Los Alamos Neutron Science Center. Experiments were also carried out at the CERN PS-IRRAD proton facility with 24 GeV proton fluence up to 8.2 × 1015 p/cm2. Research and development will continue to develop LuAG:Ce ceramics and BaF2:Y crystals with improved optical quality, F/T ratio, and radiation hardness.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

Structure in the event-by-event energy-dependent neutron-$γ$ multiplicity correlations in 252 Cf(sf)

The emission of neutrons and γ rays by fission fragments reveal important information about the properties of fragments immediately following scission. The initial fragment properties, correlations between fragments, and emission competition give rise to correlations in neutron-γ emission. Recent theoretical and experimental advances have been proposed to explain the mechanism of angular momentum generation in fission, which would result in observable signature in neutron-γ emission correlations. In this paper, we present a novel analysis method of neutrons and γ rays emitted by fission fragments that allows us to discern structure in the observed correlations. We have analyzed data collected on 252 Cf (sf) at the Chi-Nu array at the Los Alamos Neutron Science Center. Through our analysis of the energy-differential neutron-γ multiplicity covariance, we have observed enhanced neutron-γ correlations, corresponding to rotational band γ-ray transitions, at γ-ray energies of 0.7 and 1.2 MeV. To shed light on the origin of this structure, we compare the experimental data with the predictions of three model calculations. The origin of the observed correlation structure is understood in terms of a positive spin-energy correlation in the generation of angular momentum in fission.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2018

Progress Towards an Indirect Neutron Capture Capability at LANSCE: October 2017 – March 2018

We describe progress developing the Device for Indirect Capture Experiments on Radionuclides (DICER) on flight path 13 at the Lujan Center at the Los Alamos Neutron Science Center (LANSCE). This capability is being developed to tightly constrain neutron-capture cross section on short-lived radioactive nuclides of high importance to weapons-program sponsors via neutron total cross section measurements on the same nuclides. In this report, we describe progress in this endeavor during October 2017 through March 2018.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2018

Progress Towards an Indirect Neutron Capture Capability at LANSCE: October 2017 – September 2018

We describe progress developing the Device for Indirect Capture Experiments on Radionuclides (DICER) on flight path 13 at the Lujan Center at the Los Alamos Neutron Science Center (LANSCE). This capability is being developed to tightly constrain neutron-capture cross section on short-lived radioactive nuclides of high importance to weapons-program sponsors via neutron total cross section measurements on the same nuclides. In this report, we describe progress in this endeavor during October 2017 through September 2018.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2021

New capability for neutron transmission measurements at LANSCE: The DICER instrument

A new capability for neutron transmission measurements has been developed at the Los Alamos Neutron Science Center (LANSCE). The DICER (Device for Indirect Capture Experiments on Radionuclides) instrument is designed to tightly constrain neutron-capture cross sections for short-lived radionuclides that are beyond the reach of direct techniques, via measurement and analysis of neutron transmission resonances on these same radionuclides. The innovative DICER apparatus enables simultaneous sample-in and sample-out measurements, thus minimizing the amount of sample material needed and reducing the measurements time by half. A description of the current status of the new transmission station, along with a performance overview and results from known reactions, will be presented here.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2026

Analysis of Second Target Station Target Removal Dose Rates

The Second Target Station (STS) project at Oak Ridge National Laboratory’s spallation neutron source is a crucial initiative for maintaining U.S. leadership in neutron sciences. The STS aims to create the world’s brightest pulsed cold neutron source, enabling cutting-edge research across various scientific disciplines. To ensure safe and efficient maintenance operations, understanding the effects of shutdown dose rates from activated components within the STS target systems is essential. This study establishes a computational framework for calculating decay gamma sources and subsequent shutdown dose rates utilizing advanced methods to account for all activation channels, including high-energy interactions down to thermal neutron capture. This study describes a novel integration of multiple tools and provides an effective means of analyzing activation and shutdown dose rates at spallation neutron facilities. A custom-developed script automates the decay gamma source generation process, ensuring proper sampling during the variance reduction phase, which is critical for accurate predictions of shutdown dose rates.

Transmutation↗
DOE OSTI2019

Progress Toward an Indirect Neutron Capture Capability at LANSCE: October 2018 – September 2019

We describe progress developing the Device for Indirect Capture Experiments on Radionuclides (DICER) on flight path 13 at the Lujan Center at the Los Alamos Neutron Science Center (LANSCE). This capability is being developed to tightly constrain neutron-capture cross section on short-lived radioactive nuclides of high importance to weapons-program sponsors via neutron total cross section measurements on the same nuclides. In this report, we describe progress in this endeavor during October 2018 through September 2019.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2024

Innovative approaches to neutron beam optimization: A case study of FP14 at LANSCE

This paper describes an experimental method to acquire high resolution energy- and spatially- resolved neutron beam spots using the time-gated neutron imaging system with Teledyne Pi-MAX4 camera. These experimental data offer a unique opportunity for benchmarking beam spot simulations. High-quality simulations depend significantly on a high-fidelity geometry model, which can be challenging for legacy facilities. We informed our MCNPX geometry model by latest metrology survey employing Leica laser tracker ATS600. It gave us a high fidelity description of our facility geometry. Such a robust integration of novel tools and methods yields a previously unattainable level of accuracy in both predicting and capturing neutron beam spots, marking a notable advancement over traditional methods reliant on static image plates. Here, to demonstrate the practical application of these tools, we are showing a non-uniform beam spot challenge at our Flight Path 14 (FP14) at the Los Alamos Neutron Science Center (LANSCE). Our precise MCNPX prediction of beam spot shifting as function of neutron energy was confirmed by experimental beam spot measured with extremely high level of detail. Results of this research demonstrate a significant leap in neutron beam optimization at LANSCE and set a new benchmark in beam spot characterization. The advanced methods presented here have potential for adoption at similar research facilities worldwide, aiming at substantial improvement in neutron beam delivery for experiments.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2018

Gallium nitride (GaN) devices as a platform technology for radiation hard inertial confinement fusion diagnostics

Inertial Confinement Fusion (ICF) is undergoing more detailed research to increase neutron yield and will require high resolution imaging near the target. Neutron damage to diagnostics remains a serious issue in understanding and achieving ICF. We have demonstrated that Gallium Nitride (GaN) optoelectronic devices have exceptional neutron radiation hardness, by systematic testing of neutron radiation effects in GaN devices and materials with elevated neutron fluence levels and a broad neutron energy spectrum. During the 2013-2017 run cycles at Los Alamos Neutron Science Center (LANSCE), we irradiated various GaN materials and devices with fast and thermal plus resonance neutrons at several beamlines. This work presents a radiation hardness study for Aluminum Gallium Nitride and Gallium Nitride (AlGaN/GaN) deep UV LEDs irradiated at the LANSCE 4FP60R beamline. The fluence level was up to 2.4 × 10 13 neutrons/cm 2 for neutrons with energies greater than 0.1 MeV. The device performance was monitored in real time. After three years of irradiation studies, we found that the GaN devices maintained operation in the forward active region. The current and voltage relation (I-V curves) varied insignificantly in the linear region. Finally, our results demonstrate the radiation hardness needed for laser fusion diagnostics at least up to 10 17 neutron yield per shot, if the diagnostics is placed 1 m away from the target, where the neutron fluence per shot is approximately 8 × 10 11 n/cm 2 . The GaN devices can operate for multiple shots.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗