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NASA's High-Resolution GEOS Forecasting and Reanalysis Products: Support for TOLNet

Stratospheric intrusions (SIs) the introduction of ozone-rich stratospheric air into the troposphere – have been the interest of decades of research for their link with surface ozone air quality exceedances, especially at the high elevations in the western USA in springtime; however, the impact of SIs in the remaining seasons and over the rest of the USA is less clear. We can expect MERRA-2 to realistically represent both atmospheric dynamics and composition. The operational GEOS weather forecasting system, GEOS-FP, has a similar ozone observing system to MERRA-2, while NASA's new global high-resolution air quality forecast system, GEOS-CF, combines the operational GEOS weather forecasting model with the state-of-the-science GEOS-Chem chemistry module (version 12), simulating a wide range of additional air pollutants and tracers which strengthens this detailed analysis of the intrusions and the sources for the high ozone concentrations. Using a multitude of observational datasets, including lidar, air craft, ozonesondes and air quality monitoring surface sites, in combination with the GEOS forecast and reanalysis products, we aim to provide the public with tools which are available in near-real time to enhance their capability to identify the impact of stratospheric air on surface ozone concentrations separate from anthropogenic sources. In particular, improved understanding of the connections between large-scale climate variability and local-scale dynamically-driven air quality events may support improved seasonal prediction of SI events.

Knowland, K. Emma↗

Comparing Satellite Measurements of Volcanic SO2 Mass from OMI, OMPS and TROPOMI

Sulfur dioxide (SO2) is a major air pollutant that contributes to acid rain and aerosol formation (e.g., sulfates), adversely affects the environment and human health, and explosive volcanic SO2 emissions can impact climate. The majority of SO2 emissions are related to anthropogenic processes (e.g., fossil fuel burning, metal ore smelting operations), although natural processes such as volcanic eruptions and degassing also play an important role as anthropogenic SO2 emissions continue to decline. Generally, the most interest in volcanoes occurs during major eruptions. We will focus on comparing volcanic SO2 outgassing that occurs on an almost daily basis from lesser known volcanoes using satellite data. At NASA’s Global Sulfur Dioxide Monitoring Home page (https://so2.gsfc.nasa.gov/), we have been posting daily SO2 maps from 40 volcanic and industrial regions around the world using measurements from three satellite instruments; the Ozone Monitoring Instrument (OMI) onboard NASA’s Earth Observing System Aura satellite, the Ozone Monitoring and Profiler Suite (OMPS) onboard the NASA-NOAA Suomi National Polar-orbiting Partnership (NPP) satellite, and the TROPOspheric Monitoring Instrument (TROPOMI) onboard the ESA/Copernicus Sentinel-5 Precursor satellite. These instruments in low Earth sun-synchronous polar orbits with 1:30-2:00 pm equator crossing local time provide daily SO2 maps at different spatial resolutions: 13 x 24 km2, 50 x 50 km2 and 5.5 x 3.5 km2 for OMI, OMPS and TROPOMI respectively. Data from OMI are available since October 2004 (partial coverage since 2008), from OMPS since 2012 and from TROPOMI since 2018. We will present comparative SO2 mass time-series (see Hunga-Tonga plot) and statistical analyses of recent eruptions that have data from all the instruments.

SO2↗

Volatile chemical product emissions enhance ozone and modulate urban chemistry

Decades of air quality improvements have substantially reduced the motor vehicle emissions of volatile organic compounds (VOCs). Today, volatile chemical products (VCPs) are responsible for half of the petrochemical VOCs emitted in major urban areas. We show that VCP emissions are ubiquitous in US and European cities and scale with population density. We report significant VCP emissions for New York City (NYC), including a monoterpene flux of 14.7 to 24.4 kg ⋅ d−1 ⋅ km−2 from fragranced VCPs and other anthropogenic sources, which is comparable to that of a summertime forest. Photochemical modeling of an extreme heat event, with ozone well in excess of US standards, illustrates the significant impact of VCPs on air quality. In the most populated regions of NYC, ozone was sensitive to anthropogenic VOCs (AVOCs), even in the presence of biogenic sources. Within this VOC-sensitive regime, AVOCs contributed upwards of ∼20 ppb to maximum 8-h average ozone. VCPs accounted for more than 50% of this total AVOC contribution. Emissions from fragranced VCPs, including personal care and cleaning products, account for at least 50% of the ozone attributed to VCPs. We show that model simulations of ozone depend foremost on the magnitude of VCP emissions and that the addition of oxygenated VCP chemistry impacts simulations of key atmospheric oxidation products. NYC is a case study for developed megacities, and the impacts of VCPs on local ozone are likely similar for other major urban regions across North America or Europe.

Matthew M. Coggon↗

Contamination Impact of Station Brush Fire on Cleanroom Facilities

Brush and forest fires, both naturally occurring and anthropogenic in origin, in proximity to space flight hardware processing facilities raise concerns about the threat of contamination resulting from airborne particulate and molecular components of smoke. Perceptions of the severity of the threat are possibly heightened by the high sensitivity of the human sense of smell to some components present in the smoke of burning vegetation.On August 26th, 2009, a brushfire broke out north of Pasadena, California, two miles from the Jet Propulsion Laboratory. The Station Fire destroyed over 160,000 acres, coming within a few hundred yards of JPL. Smoke concentrations on Lab were very heavy over several days. All Lab operations were halted, and measures were taken to protect personnel, critical hardware, and facilities. Evaluation of real-time cleanroom monitoring data, visualinspection of facilities, filter systems, and analysis of surface cleanliness samples revealed facility environments andhardware were minimally effected.Outside air quality easily exceeded Class Ten Million. Prefilters captured most large ash and soot; multi-stage filtration greatly minimized the impact on the HEPA/ULPA filters. Air quality in HEPA filtered spacecraft assembly cleanrooms remained within Class 10,000 specification throughout. Surface cleanliness was inimally affected, as large particles were effectively removed from the airstream, and sub-micron particles have extremely long settling rates. Approximate particulate fallout within facilities was 0.00011% area coverage/day compared to 0.00038% area coverage/day during normal operations. Deposition of condensable airborne components, as measured in real time, peaked at approximately1.0 ng/cm2/day compared to 0.05 ng/cm2/day nominal.

airborne particulate contamination↗

NASA's GEOS Composition Model Assessment of PM2.5 During Wildfires: Inferring the Impact of PM2.5 Exposure on Adverse Respiratory & Cardiovascular Conditions

Particulate matter pollution is a mixture of solid and liquid droplets floating in the air that can lead to reduced air quality and increased adverse health impact. Fine particulate matter (PM2.5) can be emitted into the air from anthropogenic sources such as the burning of fossil fuels, motor vehicles, and powerplant emissions. Exposure to PM2.5 can aggravate pre-existing respiratory and cardiovascular conditions. When PM2.5 is inhaled it can cause damage to the lungs such as reduced lung function and shortness of breath. After being inhaled PM2.5 can enter the bloodstream and cause harm to the heart. One major natural source of PM2.5 exposure is from wildfire smoke. The particulates within the smoke from the wildfires can spread from the initial source region, potentially impacting communities both near and far. During and after wildfire events, PM2.5 levels can exceed the WHO air quality guidelines (10 m.g/m^3 annual mean; 25 m.g/m^3 daily mean), becoming hazardous to an individual's health. Global models can be used to simulate the emission and transport of these particulates and subsequently they can be valuable to air quality forecasting in highly polluted areas. The NASA Goddard Earth Observing System (GEOS) Composition Forecast (GEOS-CF) system has been used to produce near-real time air quality forecasts of atmospheric composition at a high global resolution of 25x25 km2. The GEOS-CF system utilizes the GEOS weather forecast model coupled with GEOS-Chem (version 11) chemistry module to provide analyses and forecasts of various toxic air pollutants, including PM2.5. The GEOS-CF simulated high levels of PM2.5 (40 m.g/m^3 to 250 m.g/m^3 ), exceeding the WHO guidelines, during multiple recent regional and global wildfire seasons, including the 2017 Washington State and Northern and Southern California wildfire seasons. Furthermore, the GEOS-CF simulated PM2.5 applied to a human health assessment model, BenMAP (The Environmental Benefits Mapping and Analysis Program, version 1.3), estimates the impact on adverse respiratory health conditions due to PM2.5 exposure from wildfires. The GEOS-CF predicted PM2.5 during the wildfire season with the corresponding BenMAP results provides an assessment of the human health impact of PM2.5 exposure.

Saunders, Emily↗

Climate Impacts on Tropospheric Ozone and Hydroxyl

Climate change may influence tropospheric ozone and OH via several main pathways: (1) altering chemistry via temperature and humidity changes, (2) changing ozone and precursor sources via surface emissions, stratosphere-troposphere exchange, and light- ning, and (3) affecting trace gas sinks via the hydrological cycle and dry deposition. We report results from a set of coupled chemistry-climate model simulations designed to systematically study these effects. We compare the various effects with one another and with past and projected future changes in anthropogenic and natural emissions of ozone precursors. We find that white the overall impact of climate on ozone is probably small compared to emission changes, some significant seasonal and regional effects are apparent. The global effect on hydroxyl is quite large, however, similar in size to the effect of emission changes. Additionally, we show that many of the chemistry-climate links that are not yet adequately modeled are potentially important.

Shindell, Drew T.↗

Constraining Black Carbon Aerosol over Asia using OMI Aerosol Absorption Optical Depth and the Adjoint of GEOS-Chem

Accurate estimates of the emissions and distribution of black carbon (BC) in the region referred to here as Southeastern Asia (70degE-l50degE, 11degS-55degN) are critical to studies of the atmospheric environment and climate change. Analysis of modeled BC concentrations compared to in situ observations indicates levels are underestimated over most of Southeast Asia when using any of four different emission inventories. We thus attempt to reduce uncertainties in BC emissions and improve BC model simulations by developing top-down, spatially resolved, estimates of BC emissions through assimilation of OMI observations of aerosol absorption optical depth (AAOD) with the GEOS-Chem model and its adjoint for April and October of 2006. Overwhelming enhancements, up to 500%, in anthropogenic BC emissions are shown after optimization over broad areas of Southeast Asia in April. In October, the optimization of anthropogenic emissions yields a slight reduction (1-5%) over India and parts of southern China, while emissions increase by 10-50% over eastern China. Observational data from in situ measurements and AERONET observations are used to evaluate the BC inversions and assess the bias between OMI and AERONET AAOD. Low biases in BC concentrations are improved or corrected in most eastern and central sites over China after optimization, while the constrained model still underestimates concentrations in Indian sites in both April and October, possibly as a. consequence of low prior emissions. Model resolution errors may contribute up to a factor of 2.5 to the underestimate of surface BC concentrations over northern India. We also compare the optimized results using different anthropogenic emission inventories and discuss the sensitivity of top-down constraints on anthropogenic emissions with respect to biomass burning emissions. In addition, the impacts of brown carbon, the formulation of the observation operator, and different a priori constraints on the optimization are investigated. Overall, despite these limitations and uncertainties, using OMI AAOD to constrain BC sources improves model representation of BC distributions, particularly over China.

Aerosols↗

Great Lakes Water Resources II: A Google Earth Engine Tool to Automate Wetland Mapping Using Optical and Radar Satellite Sensors in the Great Lakes Basin for Wetland Management and Monitoring

The Great Lakes Basin is one of the world’s largest freshwater ecosystems. The Basin harbors over 200,000 acres of wetlands. These wetlands provide a variety of environmental, ecological, and recreational functions to over 30 million people in the region. Some of these functions include improving water quality, mitigating flood impacts, providing wildlife habitat, and housing recreational activities. However, due to anthropogenic activities, habitat conversion and degradation threaten to disrupt or destroy remaining wetland ecosystems. Maps of wetland distribution based on ground surveys are costly and labor-intensive, prohibiting timely evaluations of wetland loss and gain. The Great Lakes Water Resources II team at the NASA Jet Propulsion Laboratory developed the Wetlands Extent Tool 2.0 (WET 2.0) in Google Earth Engine to automate mapping of wetland distribution in the Great Lakes Basin. The team partnered with the US Fish and Wildlife Service (USFWS), Environmental Protection Agency (EPA), Minnesota Department of Natural Resources (MDNR), the National Oceanic and Atmospheric Administration (NOAA), and Ducks Unlimited (DU). WET 2.0 incorporates Landsat 8 Operational Land Imager (OLI), Sentinel-1 C-band Synthetic Aperture Radar (C-SAR), and Sentinel-2 Multispectral Instrument (MSI) satellite data. WET 2.0 is trained to classify anywhere in the Great Lakes Basin. Utilizing a Random Forest classifier, WET 2.0 is capable of automatically mapping wetland extent in the entire Great Lakes Basin, achieving a mean overall accuracy of 80.12% when tested in Michigan. Findings and maps produced in WET 2.0 will enable our partners to identify areas of ecosystem degradation and wetland destruction in order to enact environmental practices and policy initiatives to maintain environmental and economic health in the area.

Water Resources↗

Great Lakes Water Resources II: A Google Earth Engine Tool to Automate Wetland Extent Mapping Using Optical and Radar Satellite Sensors in the Great Lakes Basin for Wetland Management and Monitoring

The Great Lakes Basin is one of the world’s largest freshwater ecosystems. The Basin harbors over 200,000 acres of wetlands that provide a variety of environmental, ecological, and recreational functions to over 30 million people in the region. Some of these functions include improving water quality, mitigating flood impacts, providing wildlife habitat, and housing recreational activities. However, due to anthropogenic activities, habitat conversion and degradation threaten to disrupt or destroy remaining wetland ecosystems. Maps of wetland distribution based on ground surveys are costly and labor-intensive, prohibiting timely evaluations of wetland loss and gain. The Great Lakes Water Resources II team at the NASA Jet Propulsion Laboratory developed the Wetlands Extent Tool 2.0 (WET 2.0) in Google Earth Engine to automate mapping of wetland distribution in the Great Lakes Basin. The team partnered with the US Fish and Wildlife Service, Environmental Protection Agency, Minnesota Department of Natural Resources, the National Oceanic and Atmospheric Administration, and Ducks Unlimited. WET 2.0 incorporates Landsat 8 Operational Land Imager (OLI), Sentinel-1 C-band Synthetic Aperture Radar (C-SAR), and Sentinel-2 Multispectral Instrument (MSI) data. Utilizing a Random Forest classifier, WET 2.0 is capable of automatically mapping wetland extent in the entire Great Lakes Basin, achieving a mean overall accuracy of 80.12% when tested in Michigan.Findings and maps produced by WET 2.0 will enable our partners to identify areas of ecosystem degradation and wetland destruction in order to enact environmental practices and policy initiatives to maintain environmental and economic health in the area.

Water Resources↗

Biogeochemical Impact of Long-Range Transported Dust over Northern South China Sea

Transpacific transport and impact of Asian dust aerosols have been well documented (e.g., results from ACE-Asia and regional follow-on campaigns), but little is known about dust invasion to the South China Sea (SCS). On 19-21 March 2010, a fierce Asian dust storm affected large areas from the Gobi deserts to the West Pacific, including Taiwan and Hong Kong. As a pilot study of the 7-SEAS (Seven South East Asian Studies) in the northern SCS, detailed characteristics of long-range transported dust aerosols were first observed by a comprehensive set of ground-based instruments deployed at the Dongsha islands (20deg42'52" N, 116deg43'51" E). Aerosol measurements such as particle mass concentrations, size distribution, optical properties, hygroscopicity, and vertical profiles help illustrate the evolution of this dust outbreak. Our results indicate that these dust particles were mixed with anthropogenic and marine aerosols, and transported near the surface. Satellite assessment of biogeochemical impact of dust deposition into open oceans is hindered by our current inability in retrieving areal dust properties and ocean colors over an extensive period of time, particularly under the influence of cloudy conditions. In this paper, we analyze the changes of retrieved Chlorophyll-a (Chl-a) concentration over the northern SCS, considered as oligotophic waters in the spring, from long-term SeaWiFS measurements since 1997. Over the past decade, six long-range transported dust events are identified based on spatiotemporal evolutions of PM10 measurements from regional monitoring stations, with the aid of trajectory analysis. Multi-year composites of Chl-a imagery for dust event and non-dust background during March-April are applied to overcome insufficient retrievals of Chl-a due to cloudy environment. Due to anthropogenic modification within a shallow boundary layer off the densely populated and industrial southeast coast of China, the iron ion activation of deliquescent dust particles enhances the efficiency of fertilization for biological productivity. Compared to the West Pacific, the marine ecosystem in the northern SCS is much more susceptible to the biogeochemical impact of long-range transported Asian dust.

Tsay, Si-Chee↗

Half of global methane emissions come from highly variable aquatic ecosystem sources

Atmospheric methane is a potent greenhouse gas that plays a major role in controlling the Earth’s climate. The causes of the renewed increase of methane concentration since 2007 are uncertain given the multiple sources and complex biogeochemistry. Here, we present a metadata analysis of methane fluxes from all major natural, impacted and human-made aquatic ecosystems. Our revised bottom-up global aquatic methane emissions combine diffusive, ebullitive and/or plant-mediated fluxes from 15 aquatic ecosystems. We emphasize the high variability of methane fluxes within and between aquatic ecosystems and a positively skewed distribution of empirical data, making global estimates sensitive to statistical assumptions and sampling design. We find aquatic ecosystems contribute (median) 41% or (mean) 53% of total global methane emissions from anthropogenic and natural sources. We show that methane emissions increase from natural to impacted aquatic ecosystems and from coastal to freshwater ecosystems. We argue that aquatic emissions will probably increase due to urbanization, eutrophication and positive climate feedbacks and suggest changes in land-use management as potential mitigation strategies to reduce aquatic methane emissions.

aquatic ecosystem↗

Comprehensive Severe Weather Impact Assessment and Monitoring using Synthetic Aperture Radar and Auxiliary Data

Remote sensing datasets, particularly acquired by Synthetic Aperture Radar (SAR) sensors, have become increasingly important in severe weather disaster impact studies given their ability to observe the Earth largely irrespective of weather and sunlight conditions. The reliability of existing SAR change detection products applied on a pair of SAR images is constrained by the limitation of current methods to differentiate and classify disaster specific changes from anthropogenic surface alterations. Moreover, the inherent properties of the sensors, variations in SAR backscatter due to changes in surface conditions, and other factors exacerbate these limitations. We proposed a novel procedure expanding on earlier SAR-based change detection methods to exclude anthropogenic alterations and other sources of ambiguity that might lead to inaccurate mapping of the impacts of severe weather disasters. We applied the proposed procedure that is based on long term interferometric and amplitude-based change detection analyses of Sentinel- 1 SAR imagery to two study sites recently impacted by severe weather disasters (Flooding post severe weather events in urban centers; Hailstorm damage on crops). For the first case study, Sentinel-1 SLC scenes from two flood events in the Houston area (April 2016 flooding event and Hurricane Harvey of August-September 2017) were used to construct a flood map depicting areas repeatedly affected by the flood. Pixels with consistent coherence values in the pre-disaster coherence stack were retained for comparison with the pre- and post-disaster coherence stack and pixels with significant decline (greater than 60%) in coherence values were retained in the final flood map. The findings of the applied technique were calibrated and validated through datasets from NOAA/NWS Service storm reports, aerial imaging (NOAA and Civil Air Patrol), Federal Emergency Management Agency (FEMA) reporting, and targeted collections of NASA’s L-band UAVSAR data. Findings and products derived from the adopted methodology can be useful in disaster response and mitigation activities.

Gebremichael, Esayas↗

Anthropogenic Influences Alter the Response and Seasonality of Evapotranspiration: A Case Study Over Two High Mountain Asia Basins

Earth's vegetation has been increasing over the past decades, altering water and energy cycles by changing evapotranspiration (ET). Greening, caused by climatic and anthropogenic factors, has high rates in High Mountain Asia (HMA). Here we focus on two HMA basins (the Yangtze and the Ganges-Brahmaputra) to contrast the impacts of climate- and human-induced greening on ET. Though the rate of greening is similar in both basins, anthropogenic influences lead to dissimilar responses in ET. In the Yangtze, climate-induced greening increases ET, with the increase in moisture being high enough to meet the ET demand. In the Ganges-Brahmaputra, irrigation-induced greening does not alter annual ET, only pre-monsoon ET increases. The dry season declines in water storage due to pumping decrease ET, while laboriously meeting the demand. This study provides a representative example of the contrasting influences of climate induced and anthropogenic driven processes on the seasonality of ET.

Fadji Z Maina↗

Formation of Cirrus Clouds near the Tropical Tropopause and Their Implications for Stratospheric Humidity, Radiation Budgets, and Climate

Optically-thin cirrus clouds are a nearly ubiquitous feature of the transition layer between the tropical troposphere and stratosphere (known as the Tropical Tropopause Layer). Given their high occurrence frequency, these clouds have significant impacts on the Earth's radiation budget, with a particularly strong influence on the outgoing longwave radiation. Further, ice crystal growth and sedimentation in these clouds dehydrates air in the cold TTL to very low water vapor mixing ratios. Since transport from the troposphere into the stratosphere occurs primarily through the tropical tropopause and the Brewer-Dobson circulation transports air from the TTL throughout the stratosphere, cloud processes in the TTL cold trap essentially regulate the humidity of the entire stratosphere. It has been shown that even small changes in stratospheric humidity can have significant impacts on the Earth's radiation budget and climate, with magnitudes comparable to anthropogenic changes in greenhouse gases. The humidity of air crossing the TTL cold trap depends to first order on tropical tropopause temperatures, but also on deep convection reaching the TTL, large-scale transport (in balance with TTL radiative heating), atmospheric waves, and cloud microphysical processes. Gaps in our understanding of TTL transport and cloud processes motivated the NASA Airborne Tropical TRopopause EXperiment (ATTREX). ATTREX used the long-range (16,000 km), high-altitude (20 km) Global Hawk unmanned aircraft system equipped with twelve instruments measuring clouds, water vapor, meteorological conditions, chemical tracers, chemical radicals, and radiation. I will discuss the physics of TTL cirrus formation and the impact of these clouds on water vapor and radiation budgets, including new results emerging from the ATTREX measurements.

Jensen, Eric↗

East Asian Studies of Tropospheric Aerosols and their Impact on Regional Climate (EAST -AIRC): An overview

As the most populated region of the world, Asia is a major source of aerosols with potential large impact over vast downstream areas, Papers published in this special section describe the variety of aerosols observed in China and their effects and interactions with the regional climate as part of the East Asian Study of Tropospheric Aerosols and their Impact on Regional Climate (EAST-AIRC), The majority of the papers are based on analyses of observations made under three field projects, namely, the Atmospheric Radiation Measurements (ARM) Mobile Facility mission in China (AMF-China), the East Asian Study of Tropospheric Aerosols: An International Regional Experiment (EAST-AIRE), and the Atmospheric Aerosols of China and their Climate Effects (AACCE), The former two are U,S,-China collaborative projects, and the latter is a part of the China's National Basic Research program (or often referred to as "973 project"), Routine meteorological data of China are also employed in some studies, The wealth of general and speCIalized measurements lead to extensive and close-up investigations of the optical, physical, and chemical properties of anthropogenic, natural, and mixed aerosols; their sources, formation, and transport mechanisms; horizontal, vertical, and temporal variations; direct and indirect effects; and interactions with the East Asian monsoon system, Particular efforts are made to advance our understanding of the mixing and interaction between dust and anthropogenic pollutants during transport. Several modeling studies were carried out to simulate aerosol impact on radiation budget, temperature, precipitation, wind and atmospheric circulation, fog, etc, In addition, impacts of the Asian monsoon system on aerosol loading are also simulated.

Zhangqing, Li↗

Space-based Ornithology-Studying Bird Migration and Environmental Change in North America

Natural fluctuations in the availability of critical stopover sites coupled with anthropogenic destruction of wetlands, land-use change, and anticipated losses due to climate change present migratory birds with a formidable challenge. We have developed an individual-based, spatially explicit bird migration model that simulates the migration routes, timing and energy budgets of individual birds under dynamic weather and land surface conditions. Our model incorporates biophysical constraints, individual bird energy status, bird behavior, and flight aerodynamics. We model the speed, direction, and timing of individual birds moving through a user specified Lagrangian grid. The model incorporates environmental properties including wind speed and direction, topography, dynamic hydrologic properties of the landscape, and environmental suitability. The model is driven by important variables estimated from satellite observations of the land surface, by data assimilation products from weather and climate models, and biological field data. We illustrate the use of the model to study the impact of both short- and long-term environmental variatios, e.g. climate, drought, anthropogenic, on migration timing (phenology), spatial pattern, and fitness (survival and reproductive success). We present several theoretical simulations of the spring migration of Pectoral Sandpiper (Calidris melanotos) in North America with emphasis on the Central flyway from the Gulf of Mexico to Alaska.

Smith, James↗

Rapid Expansion of Northern Peatlands and Doubled Estimate of Carbon Storage

Northern peatlands are an integral part of the global carbon cycle—a strong sink of atmospheric carbon dioxide and source of methane. Increasing anthropogenic carbon dioxide and methane in the atmosphere are thought to strongly impact these environments, and yet, peatlands are not routinely included in Earth system models. Here we present a quantification of the sink and stock of northern peat carbon from the last glacial period through the pre-industrial period. Additional data and new algorithms for reconstructing the history of peat carbon accumulation and the timing of peatland initiation increased the estimate of total northern peat carbon stocks from 545 Gt to 1,055 Gt of carbon. Further, the post-glacial increases in peatland initiation rate and carbon accumulation rate are more abrupt than previously reported. Peatlands have been a strong carbon sink throughout the Holocene, but the atmospheric partial pressure of carbon dioxide has been relatively stable over this period. While processes such as permafrost thaw and coral reef development probably contributed some additional carbon to the atmosphere, we suggest that deep ocean upwelling was the most important mechanism for balancing the peatland sink and maintaining the observed stability.

Nichols, Jonathan E.↗

Comparison of Aerosol Classification Results from Airborne High Spectral Resolution Lidar (HSRL) Measurements and the Calipso Vertical Feature Mask

Knowledge of the vertical profile, composition, concentration, and size of aerosols is required for assessing the direct impact of aerosols on radiation, the indirect effects of aerosols on clouds and precipitation, and attributing these effects to natural and anthropogenic aerosols. Because anthropogenic aerosols are predominantly submicrometer, fine mode fraction (FMF) retrievals from satellite have been used as a tool for deriving anthropogenic aerosols. Although column and profile satellite retrievals of FMF have been performed over the ocean, such retrievals have not yet been been done over land. Consequently, uncertainty in satellite estimates of the anthropogenic component of the aerosol direct radiative forcing is greatest over land, due in large part to uncertainties in the FMF. Satellite measurements have been used to detect and evaluate aerosol impacts on clouds; however, such efforts have been hampered by the difficulty in retrieving vertically-resolved cloud condensation nuclei (CCN) concentration, which is the most direct parameter linking aerosol and clouds. Recent studies have shown correlations between average satellite derived column aerosol optical thickness (AOT) and in situ measured CCN. However, these same studies, as well as others that use detailed airborne in situ measurements have noted that vertical variability of the aerosol distribution, impacts of relative humidity, and the presence of coarse mode aerosols such as dust introduce large uncertainties in such relations.

Burton, S. P.↗