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At least 127 records · Page 7

Image masks of global ship tracks for NASA MODIS data products

Ship tracks, long thin artificial cloud features formed from the pollutants in ship exhaust, are satellite-observable examples of aerosol-cloud interactions (ACI) that can lead to increased cloud albedo and thus increased solar reflectivity, phenomena of interest in solar radiation management. In addition to ship tracks being of interest to meteorologists and policy makers, their observed cloud perturbations provide benchmark evidence of ACI that remain poorly captured by climate models. To broadly analyze the effects of ship tracks, high-resolution satellite imagery data highlighting their presence are required. To support this, we provide a hand labelled dataset to serve as a benchmark for a variety of subsequent analyses. Established from a previous dataset that identified ship track presence using NASA’s MODIS Aqua satellite imager, our first-of-its-kind dataset is comprised of image masks: capturing full ship track regions, including their contours, emission points and dispersive patterns. In total, 300 images, or around 2,500 masked ship tracks, observed under varying conditions are provided, and may facilitate training of machine learning algorithms to automate extraction.

Atmospheric dynamics↗

Constraining the Aerosol Effects on Deep Convective Clouds by Considering the Coupling Between Clouds and the Planetary Boundary Layer

Several mechanisms have been proposed for the aerosol invigoration effect. Although their principles are well established, their actual magnitudes and roles in cloud development remain uncertain and debatable. This uncertainty partly stems from observational-based studies, in which it has been challenging to separate the co-variability between aerosols and meteorology. Addressing this problem requires large data samples. To this end, this study employs the Atmospheric Radiation Measurement data set expanding to 16 years (some up to 17 years, compared to 10 years in previous work) in the U.S. Southern Great Plains. It also conducts a more careful and rigorous analysis to isolate the influences of convective available potential energy (CAPE) and synoptic patterns to address a previously raised concern. We incorporated a new key process affecting aerosol-cloud interaction: cloud-surface coupling. The state/degree of the coupling relationship turns out to play an important role in the invigoration effect. Our analysis reinforces earlier findings of a robust positive relationship between cloud thickness and aerosol loading across CAPE percentiles—but only under cloud-surface coupled conditions. The increase in cloud thickness with aerosol loading is most pronounced in coupled clouds with high CAPE and bases below 1 km. Coupled clouds with bases below 1 km thicken between 1 and 4 km, depending on the CAPE percentile. Decoupled clouds show no such systematic changes. Synoptic patterns also lead to different strengths of the invigoration effect. Clean and polluted air masses are predominantly associated with northerly and southerly winds, respectively, with a stronger invigoration effect in cleaner air masses.

Geosciences↗

Overview of the Nephele Perturbed Parameter Ensemble for Aerosol‐Cloud Interactions in E3SMv3

Aerosol-cloud interactions (aci) are the leading source of uncertainty in inferring climate sensitivity from the historical record. Earth system models (ESMs) struggle to represent aci because the processes responsible for these phenomena occur at much finer time and space scales than can be resolved by any ESM. Observational constraints provide key benchmarks to test ESMs, but cannot be used alone to fully understand aci processes except in very specific cases where causality is controlled; some degree of modeling is required to infer aci and estimate radiative forcing. Here, we generate and characterize a perturbed parameter ensemble (PPE) in version 3 of the Energy Exascale ESM (E3SMv3). We perturb 25 parameters that govern aci processes over 250 members and integrate the model over present-day and preindustrial aerosol emissions. We find that the process representation in E3SMv3 is flexible and can generate global-mean effective radiative forcings due to aci (ERFaci) ranging from −3.0 to +0.9 W m −2 . The positive ERFaci values simulated by a portion of the PPE are implausible and result from parameter combinations that produce unrealistic top-of-atmosphere energy fluxes. While global-mean cloud droplet number concentration always increases in response to anthropogenic aerosol, cloud liquid water path can both increase and decrease, suggesting that precipitation suppression is not the only aerosol-cloud adjustment represented by E3SMv3. Analysis of which processes control liquid cloud adjustment in the PPE points toward stratiform precipitation processes and aerosol activation, which is consistent with many previous ESMs, as well as the new two-moment convective cloud microphysics in E3SMv3.

Nugent, Jacqueline M. [Univ. of Wyoming, Laramie, ↗

Enhancing fire emissions inventories for acute health effects studies: integrating high spatial and temporal resolution data

Daily fire progression information is crucial for public health studies that examine the relationship between population-level smoke exposures and subsequent health events. Issues with remote sensing used in fire emissions inventories (FEI) lead to the possibility of missed exposures that impact the results of acute health effects studies. This paper provides a method for improving an FEI dataset with readily available information to create a more robust dataset with daily fire progression. High temporal and spatial resolution burned area information from two FEI products are combined into a single dataset, and a linear regression model fills gaps in daily fire progression. The combined dataset provides up to 71% more PM 2.5 emissions, 69% more burned area, and 367% more fire days per year than using a single source of burned area information. The FEI combination method results in improved FEI information with no gaps in daily fire emissions estimates. The combined dataset provides a functional improvement to FEI data that can be achieved with currently available data.

63 RADIATION, THERMAL, AND OTHER ENVIRON. POLLUTAN↗

Targeted Mobile Measurements to Isolate the Impacts of Aerosols and Meteorology on Deep Convection

One of the main goals of the Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) Tracking Aerosol Convection Interactions Experiment (TRACER) field campaign near Houston, TX was to improve understanding of meteorology and aerosol effects on deep convective storms. To help TRACER achieve its goals of disentangling aerosol-cloud interactions from meteorology, the Texas A&M University (TAMU) team deployed the new fully mobile Rapid Onsite Atmospheric Measurement Van (ROAM-V) carrying instruments to measure aerosol and atmospheric properties that was moved to multiple locations on a deployment day of isolated convection initiated by the sea breeze.

54 ENVIRONMENTAL SCIENCES↗

Surface and Atmospheric Heating Responses to Spectrally Resolved Albedo of Frozen and Liquid Water Surfaces

Abstract Multiple Earth system models (ESMs) discretize surface albedo into two semi‐broadbands comprising the UV/visible and near‐infrared (NIR) wavelengths. Here, we use an offline single‐column radiative transfer model to investigate the radiative effects of spectrally resolving the surface albedo. We use the Snow, Ice, and Aerosol Radiative model, extended to simulate liquid water, to calculate snow, ice, and liquid water albedo. We flux‐weight the hyperspectral albedo into the coarser spectral bands used by the atmospheric shortwave radiative transfer model. We establish representative atmospheric profiles for the three surface types and compare their shortwave fluxes and atmospheric warming rates with the spectrally resolved albedo to those calculated with the semi‐broadband approximation. Spectrally resolved surface albedo over snow and ice reduces atmospheric warming by darkening the albedo of NIR bands, correcting the too‐strong surface absorption in visible bands, and too‐weak surface absorption in shortwave infrared bands caused by the semi‐broadband approximation. We explore the effects on surface and atmospheric warming rates of varying solar zenith angle, cloud cover, relative humidity, and snow grain/air bubble radii. The semi‐broadband albedo biases can exceed 10% and 2% for the surface and atmospheric net flux respectively, being particularly strong under conditions which alter the distributions of surface insolation (i.e., cloud cover or increased atmospheric water vapor). These results show that transmitting a higher resolution spectral radiation field between the atmosphere and surface reduces biases in surface absorption and atmospheric heating present in ESMs that currently use the semi‐broadband approximation.

54 ENVIRONMENTAL SCIENCES↗

Marine and continental stratocumulus cloud microphysical properties obtained from routine ARM Cimel sunphotometer observations

This study investigates marine and continental stratocumulus (Sc) cloud properties obtained from an automated implementation of a multispectral photometer retrieval. Photometer methods simultaneously retrieve cloud optical depth (τ) and cloud droplet effective radius (r e ), with estimates for liquid water path (LWP) calculated on the availability of those quantities. These applied methods evaluate retrieved cloud properties for Sc identified during a recent 6 year period over the U.S. Department of Energy Atmospheric Radiation Measurement (ARM) program sites in Oklahoma, USA (SGP) and in the Azores, Portugal (ENA). Modest agreement in key quantity retrievals is found between the routine photometer products and multisensor collocated profiling references. Cumulative breakdowns contingent on cloud thickness indicate increases in all retrieved quantities in thicker clouds, with larger discrepancies in the relative performance between the retrievals collected in the presence of drizzle. Under continental cloud conditions, the clouds of a similar thickness and r e to those sampled under marine conditions report a factor of 1.5 larger τ and LWP. An r 2 ≅0.65 is found between photometer τ retrievals and shadowband radiometer measurements, with photometer retrievals reporting a high (relative) bias. The τ intercomparisons indicate that variability between retrievals is a factor of three larger than errors reported from individual retrieval input perturbation tests. Photometer r e retrievals suggest a low r 2 (< 0.1) having a standard deviation ≅ 3 µm when compared to ARM baseline multi-sensor radar/radiometer references (accounting for offsets in the cloud droplet number concentration assumptions of the latter). However, photometer LWP calculations remain relatively unbiased in non-drizzling conditions, with errors O (50 g m −2 ) and r 2 ≅0.5 to collocated radiometer and interferometer references. Additional sensitivity tests for island influences on marine Sc properties suggest that while island-influenced winds may promote larger cloud LWP or thickness, the influence could be within retrieval method uncertainty and/or collocated instrument variability.

54 ENVIRONMENTAL SCIENCES↗

ARM FY2025 Radar Plan

The U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility is dedicated to delivering high-quality radar data that significantly advance our understanding of cloud and precipitation processes, improving climate models. With radars operating across diverse frequencies, scanning modes, and global climate conditions, extensive staffing is essential for effective management. Due to current staffing constraints, achieving the expected level of operational excellence requires a more strategic approach. To address this challenge, ARM has developed an operational radar plan for the upcoming Fiscal Year 2025 (FY25) based on budget and staffing considerations.

54 ENVIRONMENTAL SCIENCES↗

ARM FY2025 Radar Plan

The U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) user facility is dedicated to delivering high-quality radar data that significantly advance our understanding of cloud and precipitation processes, improving climate models. With radars operating across diverse frequencies, scanning modes, and global climate conditions, extensive staffing is essential for effective management. Due to current staffing constraints, achieving the expected level of operational excellence requires a more strategic approach. To address this challenge, ARM has developed an operational radar plan for the upcoming Fiscal Year 2025 (FY25) based on budget and staffing considerations. This report summarizes the Fiscal Year 2024 (FY24) ARM radar-related activities and outlines the strategic plan for FY25. It presents a comprehensive radar plan that includes detailed activities, priorities, and a projected timeline aligned with the ARM radar roadmap. Key tasks, detailed in Table 1, cover various radar operational stages and coordinated efforts among ARM teams.

54 ENVIRONMENTAL SCIENCES↗

Direct Radiative Effects of Aerosols at the ARM SGP and TWP Sites (DOE ASR Final Report)

This effort has examined and quantified aerosol direct radiative effects (DREs) and associated uncertainties at the Department of Energy Atmospheric Radiation Measurement (ARM) Southern Great Plain (SGP) and Tropical Western Pacific (TWP) sites under both clear and all sky conditions by taking advantage of the advanced ARM long-term comprehensive measurements of aerosol, cloud, radiation, and atmospheric state. This effort has filled the knowledge gap in aerosol DREs at the SGP and TWP under all sky conditions based on the ARM observations.

54 ENVIRONMENTAL SCIENCES↗

Can general circulation models (GCMs) represent cloud liquid water path adjustments to aerosol–cloud interactions?

Abstract. General circulation models (GCMs), unlike other lines of evidence, indicate that anthropogenic aerosols cause a global-mean increase in cloud liquid water path (ℒ) and thus a negative adjustment to radiative forcing of the climate by aerosol–cloud interactions. In part 1 of this series of papers, we showed that this is true even in models that reproduce the negative correlation observed in present-day internal variability in ℒ and cloud droplet number concentration (Nd). We studied several possible confounding mechanisms that could explain the noncausal cloud–aerosol correlations in GCMs and that possibly contaminate observational estimates of radiative adjustments. Here, we perform single-column and full-atmosphere GCM experiments to investigate the causal model-physics mechanisms underlying the model radiative adjustment estimate. We find that both aerosol–cloud interaction mechanisms thought to be operating in real clouds – precipitation suppression and entrainment evaporation enhancement – are active in GCMs and behave qualitatively in agreement with physical process understanding. However, the modeled entrainment enhancement has a negligible global-mean effect. This raises the question of whether the GCM estimate is incorrect due to parametric or base-state representation errors or whether the process understanding gleaned from a limited set of canonical cloud cases is insufficiently representative of the diversity of clouds in the real climate. Regardless, even at limited resolution, the GCM physics appears able to parameterize the small-scale microphysics–turbulence interplay responsible for the entrainment enhancement mechanism. We suggest ways to resolve tension between current and future (storm-resolving) global modeling systems and other lines of evidence in synthesis climate projections.

54 ENVIRONMENTAL SCIENCES↗

EPCAPE-Dalhousie Field Campaign Report

This project supported the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE), which aimed to characterize the extent, radiative properties, aerosol interactions, and precipitation of stratocumulus clouds in the Eastern Pacific coastal region of La Jolla, California. Given the frequent anthropogenic aerosols emitted into this region, characterization of this important coastal cloud region and the aerosol impact on the cloud characteristics will improve the understanding of aerosol indirect effects and its representation in global climate models.

54 ENVIRONMENTAL SCIENCES↗

EPCAPE-Dalhousie Field Campaign Report

This project supported the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE), which aimed to characterize the extent, radiative properties, aerosol interactions, and precipitation of stratocumulus clouds in the Eastern Pacific coastal region of La Jolla, California. Given the frequent anthropogenic aerosols emitted into this region, characterization of this important coastal cloud region and the aerosol impact on the cloud characteristics will improve the understanding of aerosol indirect effects and its representation in global climate models. This specific project deployed the fog droplet monitor (FM-120, Droplet Measurement Technologies) at the Scripps Institution of Oceanography’s Mt. Soledad site from 16 February 2023 to 15 February 2024. This instrument measured droplet number size spectra between 2 and 50 microns, from which droplet number concentration, liquid water content, and effective diameter were calculated. These measurements will be used to characterize the seasonal variability of clouds at Mt. Soledad and investigate differences in cloud properties under regional polluted and clean marine conditions. The collected data will soon be posted as part of the digital collection for EPCAPE data hosted by the University of California, San Diego (Russell et al. 2023).

54 ENVIRONMENTAL SCIENCES↗

Optimizing DOE Opportunities to Research Land–Atmosphere Interactions in the U.S. Southeast (Workshop Report)

The southeastern United States (Southeast), with its complex and varied environments, is an area of tremendous economic, ecological, and societal importance to the country. The region is characterized by heterogeneous landscapes (i.e., geology and soil type) and a long history of human land use coupled with a warm temperature regime and high precipitation. As a result, soil erosion and deposition are pronounced, vegetation recovery is rapid, and human modification is extensive across the region. To better understand land–atmosphere interactions in this important and complex region, research communities supported by the U.S. Department of Energy’s Biological and Environmental Research (BER) program identified the Southeast as a priority region of interest. In fall 2024, the third Atmospheric Radiation Measurement Mobile Facility (AMF3), one of three mobile monitoring facilities designed to collect atmospheric and climate data from undersampled regions around the world, will begin operations in northwestern Alabama’s Bankhead National Forest (BNF). The AMF3-BNF 5-year deployment, from 2024–2029, will monitor the effects of feedbacks among aerosols, clouds, and precipitation on plant physiology and canopy-scale fluxes. It will also focus on scale aggregation to resolve the role of local forcing on larger-scale processes. To enable broader AMF3 involvement by the science community, the BER Environmental System Science (ESS) program organized the Southeast Land– Atmosphere Research Opportunities (SELARO) workshop in August 2023. The purpose was to identify gaps in scientific understanding of terrestrial processes in the Southeast (defined as states bounded by the Gulf of Mexico to the south, the Atlantic Ocean to east, the Mississippi River to the west, and extending through Tennessee and North Carolina to the north) and explore opportunities to use the AMF3-BNF deployment to coordinate and leverage research efforts across the region. Many parts of the Southeast have experienced repeated anthropogenic forcings. Farming, hunting, burning, and settlement of the region by Indigenous Peoples first shaped the distribution of plant communities, which in turn influenced European colonization patterns. Timber harvesting was common during the expansion of European settlements, and production forestry continues today. Agricultural production was extensive and then waned through the 20th century, creating a period of afforestation following agricultural abandonment. Today, many formerly agricultural landscapes are undergoing rapid urbanization and suburbanization. Overlying these patterns of anthropogenic land use are frequent disturbances from hurricanes, tornadoes, wildfires, drought, flooding, ice storms, and the occasional blizzard. An additional characteristic of the Southeast is its overall landscape complexity. Unlike the western United States, where broad expanses may share similar characteristics, Southeast topography, drainage patterns, vegetation, and development patterns vary widely across relatively small spatial scales (<1 km). This is due to the region’s underlying geology and soil development, species biodiversity patterns, and land ownership and use coupled with strong forces of erosion, weathering, and rapid plant growth in the warm, wet climate.

54 ENVIRONMENTAL SCIENCES↗

Contact Freezing of Water Droplets by Crystalline Organic Acids

The ability of water to freeze into ice crystals in mixed-phase clouds affects physical properties, including particle size, precipitation rates, and radiative properties. The presence of an insoluble particle at the surface of water droplets can promote ice nucleation at temperatures higher than that of pure water, even in the absence of a collision. However, contact freezing remains an underexplored mode of ice nucleation. Here, we present a study of atmospherically relevant organic acids and their role as effective ice-nucleating particles (INP) in contact mode using a Raman-microscope-equipped environmental chamber. We determined contact freezing temperatures induced by solid crystals of docosanol, adipic acid, cis-pinonic acid, fumaric acid, 4-hydroxybenzoic acid, palmitic acid, phthalic acid, sebacic acid, stearic acid, terephthalic acid, and vanillic acid. All solids except fumaric acid promoted contact freezing of water droplets at significantly higher temperatures than pure water in the chamber (−15.0 to −18.5 °C vs −21.3 °C). Physical and chemical properties were identified which correlate with greater effectiveness of INPs in the contact mode, including crystal lattice mismatch with ice, carbon number, and insolubility in water. In conclusion, we suggest that the presence of these organic solids in atmospheric aerosols may promote atmospheric ice nucleation at warm temperatures.

Clouds↗

Impact on cloud properties of reduced-sulphur shipping fuel in the Eastern North Atlantic

The global reduction in shipping fuel sulphur that culminated in 2020 with an ∼ 80 % reduction has created a large-scale natural experiment on the role of aerosol-cloud interaction (ACI) in the climate system. We compare observations from the Atmospheric Radiation Measurement program's Eastern North Atlantic site (ARM-ENA; 39.1° N, 28.0° W) during two June to September periods: 2016–2018 (pre-2020) and 2021–2023 (post-2020). We find a significant (∼ 15 %) decrease in cloud condensation nuclei concentrations post-2020, which resulted in a decrease in cloud droplet number (N d ) and an increase in effective radius (r e ) of marine boundary layer clouds. However, cloud liquid water path (LWP) increased post-2020. The increase in LWP offset the increase in r e , resulting in insignificant changes to optical depth. MODIS and CERES data in the vicinity of ENA during these periods produce similar results also with negligible change in albedo and optical depth. Regional cloud occurrence declined in line with changes in the large-scale meteorology. Our results highlight the complex interplay of factors that modulate cloud feedbacks in the Eastern North Atlantic.

Mace, Gerald G. [Univ. of Utah, Salt Lake City, UT↗

RCEMIP‐ACI: Aerosol‐Cloud Interactions in a Multimodel Ensemble of Radiative‐Convective Equilibrium Simulations

Aerosol‐cloud interactions are a persistent source of uncertainty in climate research. This study presents findings from a model intercomparison project examining the impact of aerosols on clouds and climate in convection‐permitting radiative‐convective equilibrium (RCE) simulations. Specifically, 11 different modeling teams conducted RCE simulations under varying aerosol concentrations, domain configurations, and sea surface temperatures (SSTs). We analyze the response of domain‐mean cloud and radiative properties to imposed aerosol concentrations across different SSTs. Additionally, we explore the potential impact of aerosols on convective aggregation and large‐scale circulation in large‐domain simulations. The results reveal that the cloud and radiative responses to aerosols vary substantially across models. However, a common trend across models, SSTs, and domain configurations is that increased aerosol loading tends to suppress warm rain formation, enhance cloud water content in the mid‐troposphere, and consequently increase mid‐tropospheric humidity and upper‐tropospheric temperature, thereby impacting static stability. The warming of the upper troposphere can be attributed to reduced lateral entrainment effects due to the higher environmental humidity in the mid‐troposphere. However, models do not agree on aerosol impacts on convective updraft velocity based on the preliminary examination of high‐percentiles of vertical velocity at a single mid‐troposheric layer (500 hPa). In large‐domain simulations, where convection tends to self‐organize, aerosol loading does not consistently influence self‐organization but tends to reduce the intensity of large‐scale circulation forming between convective clusters and dry regions. This reduction in circulation intensity can be explained by the increase in static stability due to the upper tropospheric warming.

54 ENVIRONMENTAL SCIENCES↗

Abrupt reduction in shipping emission as an inadvertent geoengineering termination shock produces substantial radiative warming

Abstract Human activities affect the Earth’s climate through modifying the composition of the atmosphere, which then creates radiative forcing that drives climate change. The warming effect of anthropogenic greenhouse gases has been partially balanced by the cooling effect of anthropogenic aerosols. In 2020, fuel regulations abruptly reduced the emission of sulfur dioxide from international shipping by about 80% and created an inadvertent geoengineering termination shock with global impact. Here we estimate the regulation leads to a radiative forcing of $$+0.2\pm 0.11$$ + 0.2 ± 0.11 Wm −2 averaged over the global ocean. The amount of radiative forcing could lead to a doubling (or more) of the warming rate in the 2020 s compared with the rate since 1980 with strong spatiotemporal heterogeneity. The warming effect is consistent with the recent observed strong warming in 2023 and expected to make the 2020 s anomalously warm. The forcing is equivalent in magnitude to 80% of the measured increase in planetary heat uptake since 2020. The radiative forcing also has strong hemispheric contrast, which has important implications for precipitation pattern changes. Our result suggests marine cloud brightening may be a viable geoengineering method in temporarily cooling the climate that has its unique challenges due to inherent spatiotemporal heterogeneity.

54 ENVIRONMENTAL SCIENCES↗