Results for “finite size” — Page 7

NASA NTRS1993

Electromagnetic fluctuations for anisotropic media and the generalized Kirchhoff's law

In this paper the polarimetric emission parameters for anisotropic media are derived using the generalized Kirchhoff's law for media with a uniform temperature and the fluctuation-dissipation theory for media with a temperature profile. Both finite-size objects and half-space media are considered. When the object has a uniform temperature across its body, the Kirchhoff's law, based on the condition of energy conservation in thermal equilibrium is generalized to obtain the emission parameters of an anisotropic medium, which can be interpreted as the absorptivity or the absorption cross section of the complementary object with a permittivity that is the transpose of the original object. When the medium has a nonuniform temperature distribution, the fluctuation-dissipation theory is applied for deriving the covariances between vector components of the thermal currents and, consequently, the covariances of the polarizations of electric fields radiated by the thermal currents. To verify the formulas derived from the fluctuation-dissipation theory, we let the temperature of the object be a constant and show that the results reduce to those obtained from the generalized Kirchhoff's law.

Yueh, Simon H.↗

NASA NTRS1993

Effects of gas on the global stability of galactic disks - Radial flows

We study numerically the effect of gas on the global stability of a two-component self-gravitating galactic disk embedded in a live halo. The stars are evolved by using a 3D collisionless N-body code, and the gas is represented by an ensemble of finite size inelastic particles. The gravitational interaction of stars and gas is calculated using a TREE method. We find that the evolution of the gaseous distribution in the globally unstable disks can be described by two different regimes. When the gas mass fraction is less than about 10 percent, the gas is channeled toward the galactic center by a growing stellar bar. For higher gas fractions, the gas becomes highly inhomogeneous, and the bar instability in the disk is heavily damped. The gas falls toward the inner kpc due to dynamical friction. Domains of both regimes depend on the efficiency of dissipation in the gas. We also discuss the relevance of the Jeans instability and give an empirical criterion for the global bar instability in a two-component self-gravitating disk.

Shlosman, Isaac↗

NASA NTRS1994

Resolution requirements for velocity gradients in turbulence

Since high resolution numerical simulations of turbulent flows, or experiments at high Reynolds numbers, represent a substantial investment in resources, the estimation of the minimum resolution required for the study of a given property has been the subject of continued interest. Different properties require, in general, different resolutions, and the present paper is dedicated to the requirements for the measurement of the probability distribution functions of the velocity gradients and, in particular, of their low order moments. The deviation of these quantities from the values corresponding to a Gaussian distribution was one of the first indications of the presence of Reynolds number-dependent intermittency and has been the object of recent interest as numerical simulations have become able to explore the distribution of gradients in the low Reynolds number range, while new experiments have extended the range to increasingly high Reynolds numbers. We will use progressive filtering of the results of numerical simulations of isotropic turbulence as a model for the effect of a sensor of finite size. The numerical issues will be addressed first to ensure that the simulations are fully resolved from the point of view of the velocity gradients. This will also give us an estimate for the numerical resolution required for the different quantities.

Jimenez, Javier↗

NASA NTRS1994

Stellar occultation of polarized light from circumstellar electrons. 4: Detached binary systems

The finite sizes of stars in detached binary systems are incorporated in the single scattering approximation of Brown, McLean, & Emslie (1978). In the absence of scatterer occultation, the predicted polarimetric variability is found to be represented by a terminating two harmonic time series, as previously found by Brown et al. (1978). When the occultation of scatterers by the light sources is included, additional Fourier harmonics are introduced. Model results are illustrated for a spherically symmetric scattering envelope centered on the primary star, in which it is found that for occultation effects to be identified in polarimetric data requires the separation of the system to be less than 10 times the radius of the primary, and for the primary to be the dominant light source.

Fox, G. K.↗

NASA NTRS1994

Hybrid simulations of whistler waves generation and current closure by a pulsed tether in the ionosphere

The dynamic response of a magnetized collisionless plasma to an externally driven, finite size, sudden switch-on current source across the magnetic field has been studied using a two dimensional hybrid code. It was found that the predominant plasma response was the excitation of whistler waves and the formation of current closure by induced currents in the plasma. The results show that the current closure path consists of: (a) two antiparallel field-aligned current channels at the end of the imposed current sheet; and (b) a cross-field current region connecting these channels. The formation of the current closure path occured in the whistler timescale much shorter than that of MHD and the closure region expanded continuously in time. The current closure process was accompanied by significant energy loss due to whistler radiation.

Chang, C. L.↗

NASA NTRS1995

Metal colloids and semiconductor quantum dots: Linear and nonlinear optical properties

One aspect of this project involves a collaborative effort with the Solid State Division of ORNL. The thrust behind this research is to develop ion implantion for synthesizing novel materials (quantum dots wires and wells, and metal colloids) for applications in all optical switching devices, up conversion, and the synthesis of novel refractory materials. In general the host material is typically a glass such as optical grade silica. The ions of interest are Au, Ag, Cd, Se, In, P, Sb, Ga and As. An emphasis is placed on host guest interactions between the matrix and the implanted ion and how the matrix effects and implantation parameters can be used to obtain designer level optical devices tailored for specific applications. The specific materials of interest are: CdSe, CdTe, InAs, GaAs, InP, GaP, InSb, GaSb and InGaAs. A second aspect of this research program involves using porous glass (25-200 A) for fabricating materials of finite size. In this part of the program, we are particularly interested in characterizing the thermodynamic and optical properties of these non-composite materials. We also address how phase diagram of the confined material is altered by the interfacial properties between the confined material and the pore wall.

Henderson, D. O.↗

NASA NTRS1993

Analytic Theory and Control of the Motion of Spinning Rigid Bodies

Numerical simulations are often resorted to, in order to understand the attitude response and control characteristics of a rigid body. However, this approach in performing sensitivity and/or error analyses may be prohibitively expensive and time consuming, especially when a large number of problem parameters are involved. Thus, there is an important role for analytical models in obtaining an understanding of the complex dynamical behavior. In this dissertation, new analytic solutions are derived for the complete attitude motion of spinning rigid bodies, under minimal assumptions. Hence, we obtain the most general solutions reported in the literature so far. Specifically, large external torques and large asymmetries are included in the problem statement. Moreover, problems involving large angular excursions are treated in detail. A new tractable formulation of the kinematics is introduced which proves to be extremely helpful in the search for analytic solutions of the attitude history of such kinds of problems. The main utility of the new formulation becomes apparent however, when searching for feedback control laws for stabilization and/or reorientation of spinning spacecraft. This is an inherently nonlinear problem, where standard linear control techniques fail. We derive a class of control laws for spin axis stabilization of symmetric spacecraft using only two pairs of gas jet actuators. Practically, this could correspond to a spacecraft operating in failure mode, for example. Theoretically, it is also an important control problem which, because of its difficulty, has received little, if any, attention in the literature. The proposed control laws are especially simple and elegant. A feedback control law that achieves arbitrary reorientation of the spacecraft is also derived, using ideas from invariant manifold theory. The significance of this research is twofold. First, it provides a deeper understanding of the fundamental behavior of rigid bodies subject to body-fixed torques. Assessment of the analytic solutions reveals that they are very accurate; for symmetric bodies the solutions of Euler's equations of motion are, in fact, exact. Second, the results of this research have a fundamental impact on practical scientific and mechanical applications in terms of the analysis and control of all finite-sized rigid bodies ranging from nanomachines to very large bodies, both man made and natural. After all, Euler's equations of motion apply to all physical bodies, barring only the extreme limits of quantum mechanics and relativity.

Tsiotras, Panagiotis↗

NASA NTRS1996

Study of the velocity gradient tensor in turbulent flow

The behavior of the velocity gradient tensor, A(ij)=delta u(i)/delta x(j), was studied using three turbulent flows obtained from direct numerical simulation The flows studies were: an inviscid calculation of the interaction between two vortex tubes, a homogeneous isotropic flow, and a temporally evolving planar wake. Self-similar behavior for each flow was obtained when A(ij) was normalized with the mean strain rate. The case of the interaction between two vortex tubes revealed a finite sized coherent structure with topological characteristics predictable by a restricted Euler model. This structure was found to evolve with the peak vorticity as the flow approached singularity. Invariants of A(ij) within this structure followed a straight line relationship of the form: gamma(sup 3)+gammaQ+R=0, where Q and R are the second and third invariants of A(ij), and the eigenvalue gamma is nearly constant over the volume of this structure. Data within this structure have local strain topology of unstable-node/saddle/saddle. The characteristics of the velocity gradient tensor and the anisotropic part of a related acceleration gradient tensor H(ij) were also studied for a homogeneous isotropic flow and a temporally evolving planar wake. It was found that the intermediate principal eigenvalue of the rate-of-strain tensor of H(ij) tended to be negative, with local strain topology of the type stable-node/saddle/saddle. There was also a preferential eigenvalue direction. The magnitude of H(ij) in the wake flow was found to be very small when data were conditioned at high local dissipation regions. This result was not observed in the relatively low Reynolds number simulation of homogeneous isotropic flow. A restricted Euler model of the evolution of A(ij) was found to reproduce many of the topological features identified in the simulations.

Cheng, Wei-Ping↗

NASA NTRS1996

Momentum Transfer Studies and Studies of Linear and Nonlinear Optical Properties of Metal Colloids and Semiconductor Quantum Dots

Phase 1 of this work involved design work on a momentum transfer device. The progress on design and testing will be presented. Phase 2 involved the systematic study of the MPD thruster for dual uses. Though it was designed as a thruster for space vehicles, the characteristics of the plasma make it an excellent candidate for industrial applications. This project sought to characterize the system for use in materials processing and characterization. The surface modification on ZnCdTe, CdTe, and ZnTe will be presented. Phase 3 involved metal colloids and semiconductor quantum dots. One aspect of this project involves a collaborative effort with the Solid State Division of ORNL. The thrust behind this research is to develop ion implantation for synthesizing novel materials (quantum dots wires and wells, and metal colloids) for applications in all optical switching devices, up conversion, and the synthesis of novel refractory materials. The ions of interest are Au, Ag, Cd, Se, In, P, Sb, Ga, and As. The specific materials of interest are: CdSe, CdTe, InAs, GaAs, InP, GaP, InSb, GaSb, and InGaAs. A second aspect of this research program involves using porous glass (25-200 A) for fabricating materials of finite size. The results of some of this work will also be reported.

Collins, W. E.↗

NASA NTRS1995

Protostellar Collapse with a Shock

We reexamine both numerically and analytically the collapse of the singular isothermal sphere in the context of low-mass star formation. We consider the case where the onset of collapse is initiated by some arbitrary process which is accompanied by a central output of either heat or kinetic energy. We find two classes of numerical solutions describing this manner of collapse. The first approaches in time the expansion wave solution of Shu, while the second class is characterized by an ever-decreasing central accretion rate and the presence of an outwardly propagating weak shock. The collapse solution which represents the dividing case between these two classes is determined analytically by a similarity analysis. This solution shares with the expansion wave solution the properties that the gas remains stationary with an r(exp -2) density profile at large radius and that, at small radius, the gas free-falls onto a nascent core at a constant rate which depends only on the isothermal sound speed. This accretion rate is a factor of approx. 0.1 that predicted by the expansion wave solution. This reduction is due in part to the presence of a weak shock which propagates outward at 1.26 times the sound speed. Gas in the postshock region first moves out subsonically but is then decelerated and begins to collapse. The existence of two classes of numerical collapse solutions is explained in terms of the instability to radial perturbations of the analytic solution. Collapse occurring in the manner described by some of our solutions would eventually unbind a finite-sized core. However, this does not constitute a violation of the instability properties of the singular isothermal sphere which is unstable both to collapse and to expansion. To emphasize this, we consider a purely expanding solution for isothermal spheres. This solution is found to be self-similar and results in a uniform density core in the central regions of the gas. Our solutions may be relevant to the 'luminosity' problem of protostellar cores since the predicted central accretion rates are significantly reduced relative to that of the expansion wave solution. Furthermore, our calculations indicate that star-forming cloud cores are not very tightly bound and that modest disturbances can easily result in both termination of infall and dispersal of unaccreted material.

Tsai, John C.↗

NASA NTRS1997

Impact Cratering Calculations

Understanding the physical processes of impact cratering on planetary surfaces and atmospheres as well as collisions of finite-size self-gravitating objects is vitally important to planetary science. The observation has often been made that craters are the most ubiquitous landform on the solid planets and the satellites. The density of craters is used to date surfaces on planets and satellites. For large ringed basin craters (e.g. Chicxulub), the issue of identification of exactly what 'diameter' transient crater is associated with this structure is exemplified by the arguments of Sharpton et al. (1993) versus those of Hildebrand et al. (1995). The size of a transient crater, such as the K/T extinction crater at Yucatan, Mexico, which is thought to be the source of SO,-induced sulfuric acid aerosol that globally acidified surface waters as the result of massive vaporization of CASO, in the target rock, is addressed by our present project. The impact process excavates samples of planetary interiors. The degree to which this occurs (e.g. how deeply does excavation occur for a given crater diameter) has been of interest, both with regard to exposing mantle rocks in crater floors, as well as launching samples into space which become part of the terrestrial meteorite collection (e.g. lunar meteorites, SNC's from Mars). Only in the case of the Earth can we test calculations in the laboratory and field. Previous calculations predict, independent of diameter, that the depth of excavation, normalized by crater diameter, is d(sub ex)/D = 0.085 (O'Keefe and Ahrens, 1993). For Comet Shoemaker-Levy 9 (SL9) fragments impacting Jupiter, predicted excavation depths of different gas-rich layers in the atmosphere, were much larger. The trajectory and fate of highly shocked material from a large impact on the Earth, such as the K/T bolide is of interest. Melosh et al. (1990) proposed that the condensed material from the impact upon reentering the Earth's atmosphere induced. radiative heating, and producing global firestorms. The observed reentry splash of the SL-9 impact-induced plumes that reimpact Jupiter (Boslough et al., 1994) supported Melosh's K/T model. The fate of early primitive planetary atmospheres during the latter stages of planetary accretion, resulting from impactors in the 100 to 103 km diameter require modeling, e.g. Newman et al. (1997). Ahrens (1990; 1993) and Chen and Ahrens (1997) found that upon delivery of most of the impact energy to the solid planet, very large ground motions arise, which couple sufficient kinetic energy to the atmosphere to cause substantial atmospheric escape. The trade-off of this model with that of Cameron (1997) who suggests that atmospheric blow-off occurs as a result of the massive impact-induced heating of the atmosphere and Pepin (1997) who uses this heating event to model differential hydrodynamic loss of lighter atmospheric gases, requires further research.

Ahrens, Thomas J.↗

NASA NTRS1996

Kinetics of Diffusional Droplet Growth in a Liquid/Liquid Two-Phase System

We address the problem of diffusional interactions in a finite sized cluster of spherical particles for volume fractions, V(sub v) in the range 0-0.01. We determined the quasi-static monopole diffusion solution for n particles distributed at random in a continuous matrix. A global mass conservation condition is employed, obviating the need for any external boundary condition. The numerical results provide the instantaneous (snapshot) growth or shrinkage rate of each particle, precluding the need for extensive time-dependent computations. The close connection between these snapshot results and the coarsegrained kinetic constants are discussed. A square-root dependence of the deviations of the rate constants from their zero volume fraction value is found for the higher V(sub v) investigated. This behavior is consistent with predictions from diffusion Debye-Huckel screening theory. By contrast, a cube-root dependence, reported in earlier numerical studies, is found for the lower V(sub v) investigated. The roll-over region of the volume fraction where the two asymptotics merge depends on the number of particles, n, alone. A theoretical estimate for the roll-over point predicts that the corresponding V(sub v) varies as n(sup -2), in good agreement with the numerical results.

Glicksman, M. E.↗

NASA NTRS1995

Protostellar Collapse with a Shock

We reexamine both numerically and analytically the collapse of the singular isothermal sphere in the context of low-mass star formation. We consider the case where the onset of collapse is initiated by some arbitrary process which is accompanied by a central output of either heat or kinetic energy. We find two classes of numerical solutions describing this manner of collapse. The first approaches in time the expansion wave solution of Shu, while the second class is characterized by an ever-decreasing central accretion rate and the presence of an outwardly propagating weak shock. The collapse solution which represents the dividing case between these two classes is determined analytically by a similarity analysis. This solution shares with the expansion wave solution the properties that the gas remains stationary with an r(sup -2) density profile at large radius and that, at small radius, the gas free-falls onto a nascent core at a constant rate which depends only on the isothermal sound speed. This accretion rate is a factor of approx. 0.1 that predicted by the expansion wave solution. This reduction is due in part to the presence of a weak shock which propagates outward at 1.26 times the sound speed. Gas in the postshock region first moves out subsonically but is then decelerated and begins to collapse. The existence of two classes of numerical collapse solutions is explained in terms of the instability to radial perturbations of the analytic solution. Collapse occurring in the manner described by some of our solutions would eventually unbind a finite-sized core. However, this does not constitute a violation of the instability properties of the singular isothermal sphere which is unstable both to collapse and to expansion. To emphasize this, we consider a purely expanding solution for isothermal spheres. This solution is found to be self-similar and results in a uniform density core in the central regions of the gas. Our solutions may be relevant to the 'luminosity' problem of protostellar cores since the predicted central accretion rates are significantly reduced relative to that of the expansion wave solution. Furthermore, our calculations indicate that star-forming cloud cores are not very tightly bound and that modest disturbances can easily result in both termination of infall and dispersal of unaccreted material.

Tsai, John C.↗

NASA NTRS1959

Two-Dimensional Diffusion Theory Analysis of Reactivity Effects of a Fuel-Plate-Removal Experiment

Two-dimensional two-group diffusion calculations were performed on the NASA reactor simulator in order to evaluate the reactivity effects of fuel plates removed successively from the center experimental fuel element of a seven- by three-element core loading at the Oak Ridge Bulk Shielding Facility. The reactivity calculations were performed by two methods: In the first, the slowing-down properties of the experimental fuel element were represented by its infinite media parameters; and, in the second, the finite size of the experimental fuel element was recognized, and the slowing-down properties of the surrounding core were attributed to this small region. The latter calculation method agreed very well with the experimented reactivity effects; the former method underestimated the experimental reactivity effects.

Gotsky, Edward R.↗

NASA NTRS1999

Experiments on Nucleation in Different Flow Regimes

The vast majority of metallic engineering materials are solidified from the liquid phase. Understanding the solidification process is essential to control microstructure, which in turn, determines the properties of materials. The genesis of solidification is nucleation, where the first stable solid forms from the liquid phase. Nucleation kinetics determine the degree of undercooling and phase selection. As such, it is important to understand nucleation phenomena in order to control solidification or glass formation in metals and alloys. Early experiments in nucleation kinetics were accomplished by droplet dispersion methods. Dilatometry was used by Turnbull and others, and more recently differential thermal analysis and differential scanning calorimetry have been used for kinetic studies. These techniques have enjoyed success; however, there are difficulties with these experiments. Since materials are dispersed in a medium, the character of the emulsion/metal interface affects the nucleation behavior. Statistics are derived from the large number of particles observed in a single experiment, but dispersions have a finite size distribution which adds to the uncertainty of the kinetic determinations. Even though temperature can be controlled quite well before the onset of nucleation, the release of the latent heat of fusion during nucleation of particles complicates the assumption of isothermality during these experiments. Containerless processing has enabled another approach to the study of nucleation kinetics. With levitation techniques it is possible to undercool one sample to nucleation repeatedly in a controlled manner, such that the statistics of the nucleation process can be derived from multiple experiments on a single sample. The authors have fully developed the analysis of nucleation experiments on single samples following the suggestions of Skripov. The advantage of these experiments is that the samples are directly observable. The nucleation temperature can be measured by noncontact optical pyrometry, the mass of the sample is known, and post processing analysis can be conducted on the sample. The disadvantages are that temperature measurement must have exceptionally high precision, and it is not possible to isolate specific heterogeneous sites as in droplet dispersions.

Bayuzick, R. J.↗

NASA NTRS1999

Experiments on Nucleation in Different Flow Regimes

The vast majority of metallic engineering materials are solidified from the liquid phase. Understanding the solidification process is essential to control microstructure, which in turn, determines the properties of materials. The genesis of solidification is nucleation, where the first stable solid forms from the liquid phase. Nucleation kinetics determine the degree of undercooling and phase selection. As such, it is important to understand nucleation phenomena in order to control solidification or glass formation in metals and alloys. Early experiments in nucleation kinetics were accomplished by droplet dispersion methods [1-6]. Dilitometry was used by Turnbull and others, and more recently differential thermal analysis and differential scanning calorimetry have been used for kinetic studies. These techniques have enjoyed success; however, there are difficulties with these experiments. Since materials are dispersed in a medium, the character of the emulsion/metal interface affects the nucleation behavior. Statistics are derived from the large number of particles observed in a single experiment, but dispersions have a finite size distribution which adds to the uncertainty of the kinetic determinations. Even though temperature can be controlled quite well before the onset of nucleation, the release of the latent heat of fusion during nucleation of particles complicates the assumption of isothermality during these experiments. Containerless processing has enabled another approach to the study of nucleation kinetics [7]. With levitation techniques it is possible to undercool one sample to nucleation repeatedly in a controlled manner, such that the statistics of the nucleation process can be derived from multiple experiments on a single sample. The authors have fully developed the analysis of nucleation experiments on single samples following the suggestions of Skripov [8]. The advantage of these experiments is that the samples are directly observable. The nucleation temperature can be measured by noncontact optical pyrometry, the mass of the sample is known, and post processing analysis can be conducted on the sample. The disadvantages are that temperature measurement must have exceptionally high precision, and it is not possible to isolate specific heterogeneous sites as in droplet dispersions.

Bayuzick, Robert J.↗

NASA NTRS1999

Preliminary Results from the Confined Helium Experiment

We describe the preliminary results from an experiment to measure the heat capacity of helium confined within a stack of evenly spaced silicon plates at temperatures very close to the superfluid transition. The resolution of the heat capacity measurements was generally about 5x10 (exp -9)K, allowing the finite size peak to be mapped in detail. In addition, wide range data containing information on the behavior of the surface specific heat was collected. The preliminary analysis shows fair agreement with theory, but some discrepancies. The results can also be combined with related ground measurements on smaller length scales to perform additional tests of scaling predictions for cross-over to lower dimensional behavior. Some results in this area are also presented.

Lipa, J. A.↗

NASA NTRS1998

Experiments on Nucleation in Different Flow Regimes

The vast majority of metallic engineering materials are solidified from the liquid phase. Understanding the solidification process is essential to control microstructure, which in turn, determines the properties of materials. The genesis of solidification is nucleation, where the first stable solid forms from the liquid phase. Nucleation kinetics determine the degree of undercooling and phase selection. As such, it is important to understand nucleation phenomena in order to control solidification or glass formation in metals and alloys. Early experiments in nucleation kinetics were accomplished by droplet dispersion methods. Dilitometry was used by Turnbull and others, and more recently differential thermal analysis and differential scanning calorimetry have been used for kinetic studies. These techniques have enjoyed success; however, there are difficulties with these experiments. Since materials are dispersed in a medium, the character of the emulsion/metal interface affects the nucleation behavior. Statistics are derived from the large number of particles observed in a single experiment, but dispersions have a finite size distribution which adds to the uncertainty of the kinetic determinations. Even though temperature can be controlled quite well before the onset of nucleation, the release of the latent heat of fusion during nucleation of particles complicates the assumption of isothermality during these experiments. Containerless processing has enabled another approach to the study of nucleation kinetics. With levitation techniques it is possible to undercool one sample to nucleation repeatedly in a controlled manner, such that the statistics of the nucleation process can be derived from multiple experiments on a single sample. The authors have fully developed the analysis of nucleation experiments on single samples following the suggestions of Skripov. The advantage of these experiments is that the samples are directly observable. The nucleation temperature can be measured by noncontact optical pyrometry, the mass of the sample is known, and post-processing analysis can be conducted on the sample. The disadvantages are that temperature measurement must have exceptionally high precision, and it is not possible to isolate specific heterogeneous sites as in droplet dispersions. Levitation processing of refractory materials in ultra high vacuum provides an avenue to conduct these kinetic studies on single samples. Two experimental methods have been identified where ultra high vacuum experiments are possible; electrostatic levitation in ground-based experiments and electromagnetic processing in low earth orbit on TEMPUS. Such experiments, reported here, were conducted on zirconium. Liquid zirconium is an excellent solvent and has a high solubility for contaminants contained in the bulk material as well as those contaminants found in the vacuum environment. Oxides, nitrides, and carbides do not exist in the melt, and do not form on the surface of molten zirconium, for the materials and vacuum levels used in this study. Ground-based experiments with electrostatic levitation have shown that the statistical nucleation kinetic experiments are viable and yield results which are consistent with classical nucleation theory. The advantage of low earth orbit experiments is the ability to vary the flow conditions in the liquid prior to nucleation. The put-pose of nucleation experiments in TEMPUS was to examine.

Bayuzick, R. J.↗