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NASA NTRS2014

Current and Future Perspectives of Aerosol Research at NASA Goddard Space Flight Center

Aerosols are tiny atmospheric particles that are emitted from various natural and anthropogenic sources. They affect climate through direct and indirect interactions with solar and thermal radiation, clouds, and atmospheric circulation (Solomon et al. 2007). The launch of a variety of sophisticated satellite-based observing systems aboard the Terra, Aqua, Aura, SeaWiFS (see appendix for all acronym expansions), CALIPSO, and other satellites in the late 1990s to mid-2000s through the NASA EOS and other U.S. and non-U.S. programs ushered in a golden era in aerosol research. NASA has been a leader in providing global aerosol characterizations through observations from satellites, ground networks, and field campaigns, as well as from global and regional modeling. AeroCenter (http://aerocenter.gsfc.nasa.gov/), which was formed in 2002 to address the many facets of aerosol research in a collaborative manner, is an interdisciplinary union of researchers (~200 members) at NASA GSFC and other nearby institutions, including NOAA, several universities, and research laboratories. AeroCenter hosts a web-accessible regular seminar series and an annual meeting to present up-to-date aerosol research, including measurement techniques; remote sensing algorithms; modeling development; field campaigns; and aerosol interactions with radiation, clouds, precipitation, climate, biosphere, atmospheric chemistry, air quality, and human health. The 2013 annual meeting was held at the NASA GSFC Visitor Center on 31 May 2013, which coincided with the seventh anniversary of the passing of Yoram Kaufman, a modern pioneer in satellite-based aerosol science and the founder of AeroCenter. The central theme of this year's meeting was "current and future perspectives" of NASA's aerosol science and satellite missions.

aerocenter↗
NASA NTRS2000

Remote Sensing of Aerosol and Aerosol Radiative Forcing of Climate from EOS Terra MODIS Instrument

The recent launch of EOS-Terra into polar orbit has begun to revolutionize remote sensing of aerosol and their effect on climate. Terra has five instruments, two of them,Moderate Resolution Imaging Spectroradiometer (MODIS) and Multiangle Imaging Spectro-Radiometer (MISR) are designed to monitor global aerosol in two different complementary ways. Here we shall discuss the use of the multispectral measurements of MODIS to derive: (1) the global distribution of aerosol load (and optical thickness) over ocean and land; (2) to measure the impact of aerosol on reflection of sunlight to space; and (3) to measure the ability of aerosol to absorb solar radiation. These measurements have direct applications on the understanding of the effect of aerosol on climate, the ability to predict climate change, and on the monitoring of dust episodes and man-made pollution. Principles of remote sensing of aerosol from MODIS will be discussed and first examples of measurements from MODIS will be provided.

Kaufman, Yoram↗
NASA NTRSDate not supplied

Identifying Chemical and Optical Smoke Signatures in Suborbital Observations to Improve Model Projections

Biomass Burning (BB) fires are expected to occur more frequently in the future due to climate change, the build‐up of fuels due to fire suppression, and the expansion of the wildland‐urban interface [Schoennagel et al., 2017; Shivdenko & Schepaschenko, 2013; Stevens et al., 2014; Turner et al., 2019; Yue et al., 2015; Tilman et al., 2001]. Accurate knowledge of the abundance, distribution, and optical properties of absorbing aerosols such as BB smoke is essential to understanding regional and global aerosol radiative effects [Boucher et al., 2013]. It is recognized that differing fuel types (e.g., rice straw, ponderosa pine), combustion modes (i.e., flaming, smoldering or both) and temperature/ moisture content produce smoke with differing optical characteristics (e.g., aerosol light scattering and absorption) and component mixing ratios [e.g., BC, OC and inorganic species such as sulfate, potassium, chloride; Streets et al. 2003; Reid et al., 2005a, b; Janhäll et al., 2010; Sayer et al., 2014]. However, climate models often ascribe a fixed set of emission factors [i.e., amount of particulate for a given species released in the atmosphere per unit dry fuel burned; Darmenov and Dasilva, 2013] and optical properties [Hess et al., 1998] to all BB aerosol plumes, inherently limiting accurate representation of the global and regional heterogeneity of BB. The overarching goal of the proposed work is to improve the microphysical and optical representation of different types of Biomass Burning in Chemistry Transport Models. Our strategy is to capitalize on multiple airborne campaigns (e.g., ARCTAS, SEAC4RS, ORACLES, FIREX-AQ), which sampled different types of BB plumes at different aging stages. Models, when improved and combined with satellite, airborne, and ground observations will help address many aerosol science objectives from the NASA Decadal survey [National Academies of Sciences, Engineering, and Medicine. 2018].

Meloe Shenandoah F Kacenelenbogen↗
NASA NTRS2019

AERONET Remotely Sensed Measurements and Retrievals of Biomass Burning Aerosol Optical Properties During the 2015 Indonesian Burning Season

An extreme biomass-burning event occurred in Indonesia from September through October 2015 due to severe drought conditions, partially caused by a major El Nino event, thereby allowing for significant burning of peatland that had been previously drained. This event had the highest sustained aerosol optical depths (AOD) ever monitored by the global Aerosol Robotic Network (AERONET). The newly developed AERONET Version 3 algorithms retain high AOD at the longer wavelengths when associated with high Angstrom Exponents (AEs), which thereby allowed for measurements of AOD at 675 nanometers as high as approximately 7, the upper limit of Sun photometry. Measured AEs at the highest monitored AOD levels were subsequently utilized to estimate instantaneous values of AOD at 550 nanometers in the range of 11 to 13, well beyond the upper measurement limit. Additionally, retrievals of complex refractive indices, size distributions, and single scattering albedos (SSA) were obtained at much higher AOD levels than possible from almucantar scans due to the ability to perform retrievals at smaller solar zenith angles with new hybrid sky radiance scans. For retrievals made at the highest AOD levels the fine mode volume median radii were approximately 0.25 to 0.30 microns, which are very large particles for biomass burning. Very high SSA values (approximately 0.975 from 440 to 1020 nanometers) are consistent with the domination by smoldering combustion of peat burning. Estimates of the percentage peat contribution to total biomass burning aerosol based on retrieved SSA and laboratory measured peat SSA were approximately 80-85 percent, in excellent agreement with independent estimates.

Eck, T. F.↗
NASA NTRSDate not supplied

Uncertainty in Observational Estimates of the Aerosol Direct Radiative Effect and Forcing

Aerosols continue to be responsible for the largest uncertainty in determining the anthropogenic radiative forcing of the climate. To both reconcile the large range in satellite-based estimates of the aerosol direct radiative effect (DRE, the direct interaction with solar radiation by all aerosols) and to optimize the design of future observing systems, we build a framework for assessing uncertainty in aerosol DRE and the aerosol direct radiative forcing (DRF, the radiative effect of just anthropogenic aerosols, RF_ari). Shortwave aerosol radiative kernels (Jacobians) were derived using the MERRA-2 reanalysis data. These radiative kernels are used to compute a lower-bound on the systematic uncertainty in observational estimates of the aerosol DRE/DRF by making the optimistic assumption that global aerosol observations can be made with the accuracy found in the Aerosol Robotic Network (AERONET) sun photometer retrievals. The total uncertainty is shown to be dominated by contributions from the aerosol single scattering albedo uncertainty. These uncertainty estimates were compared to a literature survey of mostly satellite-based aerosol DRE/DRF values. Comparisons to previous studies reveal that most have significantly underestimated the aerosol DRE uncertainty. Past estimates of the aerosol DRF uncertainty are smaller (on average) than our optimistic observational estimates, including the aerosol DRF uncertainty given in the Intergovernmental Panel on Climate Change (IPCC) fifth assessment report (AR5).

Tyler James Thorsen↗
NASA NTRSDate not supplied

Uncertainty in Observational Estimates of the Aerosol Direct Radiative Effect and Forcing

Aerosols continue to be responsible for the largest uncertainty in determining the anthropogenic radiative forcing of the climate. To both reconcile the large range in satellite-based estimates of the aerosol direct radiative effect (DRE, the direct interaction with solar radiation by all aerosols) and to optimize the design of future observing systems, we build a framework for assessing uncertainty in aerosol DRE and the aerosol direct radiative forcing (DRF, the radiative effect of just anthropogenic aerosols, RF_ari). Shortwave aerosol radiative kernels (Jacobians) were derived using the MERRA-2 reanalysis data. These radiative kernels are used to compute a lower-bound on the systematic uncertainty in observational estimates of the aerosol DRE/DRF by making the optimistic assumption that global aerosol observations can be made with the accuracy found in the Aerosol Robotic Network (AERONET) sun photometer retrievals. The total uncertainty is shown to be dominated by contributions from the aerosol single scattering albedo uncertainty. These uncertainty estimates were compared to a literature survey of mostly satellite-based aerosol DRE/DRF values. Comparisons to previous studies reveal that most have significantly underestimated the aerosol DRE uncertainty. Past estimates of the aerosol DRF uncertainty are smaller (on average) than our optimistic observational estimates, including the aerosol DRF uncertainty given in the Intergovernmental Panel on Climate Change (IPCC) fifth assessment report (AR5).

Tyler James Thorsen↗
NASA NTRS1993

Earth observing scanning polarimeter

Climate forcing by tropospheric aerosols is receiving increased attention because of the realization that the climate effects may be large, while our knowledge of global aerosol characteristics and temporal changes is very poor. Tropospheric aerosols cause a direct radiative forcing due simply to their scattering and absorption of solar radiation, as well as an indirect effect as cloud condensation nuclei which can modify the shortwave reflectivity of clouds. Sulfate aerosols tend to increase planetary albedo through both the direct and indirect effects; a cooling due to anthropogenic sulfate aerosols has been estimated of order 1 W/sq m, noting that this is similar in magnitude to the present anthropogenic greenhouse gas warming. Other aerosols, including those from biomass burning and wind-blown desert dust are also of potential climatic importance. At present, the only global monitoring of tropospheric aerosols is a NOAA operational product, aerosol optical thickness, obtained using channel-1 (0.58-0.68 mu m) radiances from the AVHRR. With this single channel radiance data, one must use an approach which is based on the inferred excess of reflected radiance owing to scattering by the aerosols over that expected from theoretical calculations. This approach is suited only for situations where the surface has a low albedo that is well known a priori. Thus, the NOAA operational product is restricted to coverage over the ocean at AVHRR scan angles well away from sun glint, and aerosol changes are subject to confusion with changes caused by either optically thin or subpixel clouds. Because optically thin aerosols have only a small effect on the radiance, accurate measurements for optical thickness less than 0.1 (which is a typical background level) are precluded. Moreover, some of the largest and most important aerosol changes are expected over land. The Earth Observing Scanning Polarimeter (EOSP) instrument, based upon design heritage and analysis techniques developed for planetary missions, will retrieve tropospheric aerosol characteristics from measurements of multispectral radiance and polarization. Moreover, the same radiance and polarization measurements will also provide very precise information on cloud properties and maps of surface characteristics for cloud-free regions. These capabilities also give EOSP the unique ability to discriminate aerosol from clouds and surface.

Travis, Larry↗
NASA NTRSDate not supplied

Relating Changing Aerosols to Changing Clouds: Two Decades of Terra and Aqua Observations

The global aerosol system of today is not the same as it was two decades ago when Terra and Aqua were launched. As a result of a changing climate (natural and anthropogenic) convolved with changes in human activity (deliberate and accidental), some regions have experienced significant changes to their total aerosol burden (increases or decreases of total loading) or their aerosol composition (as defined by relative size or source type). Other regions have had less or no significant changes. At the same time, changes in aerosol amount and composition affect clouds through direct and indirect microphysical and radiative processes. We can theoretically predict what might happen to clouds when you add aerosol to an otherwise pristine environment. Conversely, there is the situation of removing aerosol from a polluted environment. Over the past two decades, sensors on both Earth Observing Satellites (Terra and Aqua) have observed the radiative signatures of aerosols and clouds, as well as their changes. Via massive efforts by their respective characterization teams, the resulting data records appear to have a minimum of artificial drifts. Therefore, we are trying to assess, region by region, our 20-year records of aerosols and clouds, along with meteorological variables. Where have been the most significant changes of aerosols and/or clouds? Where do the changes in clouds conform with expectations based on changes of aerosols and meteorology and where do they not? In addition to separate ‘aerosol’ and ‘cloud’ retrievals from the Moderate Resolution Imaging Spectrometer (MODIS), there is a ‘twilight zone’ that is not accounted for in either product. What are these regions, and have they changed over the past two decades? We will present our early efforts at characterizing the MODIS view of aerosol and cloud changes, while also relating to changes in radiative fluxes at the top-of-atmosphere (TOA) from corresponding observations by the Clouds and the Earth's Radiant Energy System (CERES).

aerosols↗
NASA NTRS2007

Anomalies in the South American Monsoon Induced by Aerosols

We have investigated the direct effects of aerosols on the water cycle of the South American monsoon using the NASA finite-volume general circulation model (fvGCM). Global aerosol forcings are computed from radiative transfer functions derived from global distributions of five species of aerosols, i.e., dust, black carbon, organic carbon, sulphate and sea salt from the Goddard Chemistry Aerosol Radiation Transport (GOCART) model. Comparing fvGCM experiments without aerosol forcing, and with different combinations of aerosol forcing, we evaluate the impacts of aerosol direct heating on the onset, maintenance and evolution of the South American summer monsoon. We find that during the pre-monsoon season (September-October-November) Saharan dust contribute to heating of the atmosphere over the central and eastern equatorial Atlantic/Africa region through the elevated heat pump mechanism. The heating generates an anomalous Walker circulation with sinking motion, and low level northeasterlies over the Caribbean and northwestern South America. The low level flow is blocked by the Andes, and turn south and southeastward, increasing the low level jet (LLJ) along the eastern slope of the Andes. The increased LLJ transports more moisture from the Atlantic and the Amazon, enhancing the moisture convergence over subtropical land regions of South America. The moisture convergence was further accelerated by atmospheric heating by biomass burning over the Amazon. The net results of the dust and biomass heating are: a) an advance of the monsoon rainy season, b) an enhanced LLJ and c) a shifting the South America monsoon land precipitation equatorward, with increased rain over southern Brazil and reduced rain over the La Plata basin. ramifications of this elevated heating heat pump mechanism in aerosol monsoon water cycle on climate variability and change will be discussed. The ramifications of this "elevated heating heat pump" mechanism in aerosol monsoom water cycle on climate variability and change will be discussed.

Lau, K. M. William↗
NASA NTRS1981

Stratospheric aerosols

The current state of information on stratospheric aerosols is reviewed. Aerosol properties such as size, size distribution, composition, refractive index, number density, extinction, optical depth, and single scattering albedo are considered and generalized as much as possible to be representative of the global aerosol in times of volcanic and nonvolcanic (background) periods. Data are presented that show the global distribution of stratospheric aerosols as measured by the stratospheric aerosol and gas experiment (SAGE) satellite system for background and volcanic (post-Mount St. Helens) conditions. In addition, lidar and dustsonde data are presented that show the changes in stratospheric aerosol over an 8-year period.

Mccormick, M. P.↗
NASA NTRS1986

Distribution and geochemistry of aerosols in the tropical North Atlantic troposphere - Relationship to Saharan dust

Estimates of global aerosol production suggest that mobilization of natural eolian material greatly exceeds anthropogenic-related emissions, and it appears that soil material transported from arid regions by wind might be mainly responsible for the distribution of certain clay materials in oceanic sediments. In connection with studies related to an investigation of these possibilities, the present paper provides a discussion of the aerosol spatial distribution and its water-soluble chemical composition in the tropical North Atlantic troposphere during the ABLE-Barbados mission. Particular attention is given to the composition of the water-soluble fraction, since its chemical reactivity is important with respect to various atmospheric and biogeochemical processes. On the basis of the obtained results, it is suggested that Saharan dust has also a significant impact on the aerosol chemistry over the tropical North Atlantic.

Talbot, R. W.↗
NASA NTRS2000

Preliminary Results from an Assimilation of TOMS Aerosol Observations Into the GOCART Model

At NASA Goddard we are developing a global aerosol data assimilation system that combines advances in remote sensing and modeling of atmospheric aerosols. The goal is to provide high resolution, 3-D aerosol distributions to the research community. Our first step is to develop a simple assimilation system for Saharan mineral aerosol. The Goddard Chemistry and Aerosol Radiation model (GOCART) provides accurate 3-D mineral aerosol size distributions that compare well with TOMS satellite observations. Surface, mobilization, wet and dry deposition, convective and long-range transport are all driven by assimilated fields from the Goddard Earth Observing System Data Assimilation System, GEOS-DAS. Our version of GOCART transports sizes from.08-10 microns and only simulates Saharan dust. TOMS radiance observations in the ultra violet provide information on the mineral and carbonaceous aerosol fields. We use two main observables in this study: the TOMS aerosol index (AI) which is directly related to the ratio of the 340 and 380 radiances and the 380 radiance. These are sensitive to the aerosol optical thickness, the single scattering albedo and the height of the aerosol layer. The Goddard Aerosol Assimilation System (GAAS) uses the Data Assimilation Office's Physical-space Statistical Analysis System (PSAS) to combine TOMS observations and GOCART model first guess fields. At this initial phase we only assimilate observations into the the GOCART model over regions of Africa and the Atlantic where mineral aerosols dominant and carbonaceous aerosols are minimal, Our preliminary results during summer show that the assimilation with TOMS data modifies both the aerosol mass loading and the single scattering albedo. Assimilated aerosol fields will be compared with assimilated aerosol fields from GOCART and AERONET observations over Cape Verde.

daSilva, Arlindo↗
NASA NTRS2004

A New, More Physically Based Algorithm, for Retrieving Aerosol Properties over Land from MODIS

The MOD Imaging Spectrometer (MODIS) has been successfully retrieving aerosol properties, beginning in early 2000 from Terra and from mid 2002 from Aqua. Over land, the retrieval algorithm makes use of three MODIS channels, in the blue, red and infrared wavelengths. As part of the validation exercises, retrieved spectral aerosol optical thickness (AOT) has been compared via scatterplots against spectral AOT measured by the global Aerosol Robotic NETwork (AERONET). On one hand, global and long term validation looks promising, with two-thirds (average plus and minus one standard deviation) of all points falling between published expected error bars. On the other hand, regression of these points shows a positive y-offset and a slope less than 1.0. For individual regions, such as along the U.S. East Coast, the offset and slope are even worse. Here, we introduce an overhaul of the algorithm for retrieving aerosol properties over land. Some well-known weaknesses in the current aerosol retrieval from MODIS include: a) rigid assumptions about the underlying surface reflectance, b) limited aerosol models to choose from, c) simplified (scalar) radiative transfer (RT) calculations used to simulate satellite observations, and d) assumption that aerosol is transparent in the infrared channel. The new algorithm attempts to address all four problems: a) The new algorithm will include surface type information, instead of fixed ratios of the reflectance in the visible channels to the mid-IR reflectance. b) It will include updated aerosol optical properties to reflect the growing aerosol retrieved from eight-plus years of AERONE". operation. c) The effects of polarization will be including using vector RT calculations. d) Most importantly, the new algorithm does not assume that aerosol is transparent in the infrared channel. It will be an inversion of reflectance observed in the three channels (blue, red, and infrared), rather than iterative single channel retrievals. Thus, this new formulation of the MODIS aerosol retrieval over land includes more physically based surface, aerosol and radiative transfer with fewer potentially erroneous assumptions.

Levy, Robert C.↗
NASA NTRS1999

GOCART Model Simulated Tropospheric Aerosols and Comparison with Satellite, Sun Photometer, and Field Measurement Data

We present the results of tropospheric sulfate, dust, carbonaceous, and sea salt aerosols simulated in the Goddard Ozone Chemistry Aerosol Radiation and Transport (GOCART) model. Because it is a global model and uses assimilated meteorological data produced by the Goddard Data Assimilation Office, the GOCART model is an ideal tool for global aerosol analysis combining the satellite and in-situ field measurement data. The aerosol optical depth for total aerosols are compared with that retrieved from TOMS and AVHRR remote sensing instruments and from ground-based sun photometer measurements. Individual aerosol concentrations are compared with field measurements at different geographical locations. The distributions of different aerosol types to total aerosol optical depth will be discussed.

Chin, Mian↗
NASA NTRS2000

Toward Creating A Global Retrospective Climatology of Aerosol Properties

Tropospheric aerosols are thought to cause a significant direct and indirect climate forcing, but the magnitude of this forcing remains highly uncertain because of poor knowledge of global aerosol characteristics and their temporal changes. The standard long-term global product, the one-channel Advanced Very-High-Resolution Radiometer (AVHRR) aerosol optical thickness over the ocean, relies on a single predefined aerosol model and can be inaccurate in many cases. Furthermore, it provides no information on aerosol column number density, thus making it impossible to estimate the indirect aerosol effect on climate. Total Ozone Mapping Spectrometer (TOMS) data can be used to detect absorbing aerosols over land, but are insensitive to aerosols located below one kilometer. It is thus clear that innovative approaches must be employed in order to extract a more quantitative and accurate aerosol climatology from available satellite and other measurements, thus enabling more reliable estimates of the direct and indirect aerosol forcings. The Global Aerosol Climatology Project (GACP) was established in 1998 as part of the Global Energy and Water Cycle Experiment (GEWEX). Its main objective is to analyze satellite radiance measurements and field observations to infer the global distribution of aerosols, their properties, and their seasonal and interannual variations. The overall goal is to develop advanced global aerosol climatologies for the period of satellite data and to make the aerosol climatologies broadly available through the GACP web site.

Curran, Robert J.↗
NASA NTRS2003

The MODIS Aerosol Algorithm, Products, Validation and Applications

The MODerate resolution Imaging Spectroradiometer (MODIS) currently aboard both the Terra and Aqua satellites produces a suite of products designed to characterize global aerosol distribution, optical thickness and particle size. Never before has a space-borne instrument been able to provide such detailed information, complementing field and modeling efforts to produce a comprehensive picture of aerosol characteristics. The three years of Terra-MODIS data have been validated by comparing with co-located AERONET observations of aerosol optical thickness and derivations of aerosol size parameters. Some 8000 comparison points located at 133 AERONET sites around the globe show that the MODIS aerosol optical thickness retrievals are accurate to within the pre-launch expectations. MODIS-derived size parameters are also compared with AERONET retrievals and found to agree well for fine-mode dominated aerosol regimes. Aerosol regimes dominated by dust aerosol are less accurate, attributed to what is thought to be nonsphericity. Errors due to nonsphericity will be reduced by introducing a new set of empirical phase functions, derived without any assumptions of particle shape. The major innovation that MODIS bring to the field of remote sensing of aerosol is the measure of particle size and the separation of finemode and coarsemode dominated aerosol regimes. Particle size can separate finemode man-made aerosols created during combustion, from larger natural aerosols originating from salt spray or wind erosion. This separation allows for the calculation of aerosol radiative effect and the estimation of the man-made aerosol radiative forcing. MODIS can also be used in regional studies of aerosol-cloud interaction that affect the global radiative and hydrological cycles.

Remer, L. A.↗
DOE OSTI2020

Source attribution of Arctic black carbon and sulfate aerosols and associated Arctic surface warming during 1980–2018

Observations show that the concentrations of Arctic sulfate and black carbon (BC) aerosols have declined since the early 1980s. Previous studies have reported that reducing sulfate aerosols potentially contributed to the recent rapid Arctic warming. In this study, a global aerosol–climate model (Community Atmosphere Model, version 5) equipped with Explicit Aerosol Source Tagging (CAM5-EAST) is applied to quantify the source apportionment of aerosols in the Arctic from 16 source regions and the role of aerosol variations in affecting changes in the Arctic surface temperature from 1980 to 2018. The CAM5-EAST simulated surface concentrations of sulfate and BC in the Arctic had a decrease of 43% and 23%, respectively, in 2014–2018 relative to 1980–1984 mainly due to the reduction of emissions from Europe, Russia and local Arctic sources. Increases in emissions from South and East Asia led to positive trends in Arctic sulfate and BC in the upper troposphere. All aerosol radiative impacts are considered including aerosol–radiation and aerosol–cloud interactions, as well as black carbon deposition on snow- and ice-covered surfaces. Within the Arctic, sulfate reductions caused a top-of-atmosphere (TOA) warming of 0.11 and 0.25 W m -2 through aerosol–radiation and aerosol–cloud interactions, respectively. While the changes in Arctic atmospheric BC has little impact on local radiative forcing, the decrease in BC in snow and ice led to a net cooling of 0.05 W m -2 . By applying climate sensitivity factors for different latitudinal bands, global changes in sulfate and BC during 2014–2018 (with respect to 1980–1984) exerted a +0.088 and 0.057 K Arctic surface warming, respectively, through aerosol–radiation interactions. Through aerosol–cloud interactions, the sulfate reduction caused an Arctic warming of +0.193 K between the two time periods. The weakened BC effect on snow–ice albedo led to an Arctic surface cooling of -0.041 K. The changes in atmospheric sulfate and BC outside the Arctic produced a total Arctic warming of +0.25 K, the majority of which is due to the midlatitude changes in radiative forcing. Our results suggest that changes in aerosols over the midlatitudes of the Northern Hemisphere have a larger impact on Arctic temperature than other regions through enhanced poleward heat transport. The combined total effects of sulfate and BC produced an Arctic surface warming of +0.297 K, explaining approximately 20% of the observed Arctic warming since the early 1980s.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS2005

The Goddard Chemistry Aerosol Radiation and Transport Model

The Goddard Chemistry Aerosol Radiation and Transport (GOCART) model is one of the fourteen global models participating in the International AEROCOM activity. The Oslo workshop is the 4th AEROCOM workshop. In this workshop, we are going to show updated model results of global aerosol extinction and absorption, vertical profiles, and direct and indirect effects. We will also discuss with other participants on model similarities and discrepancies, issues related to comparisons with in-situ and remote sensing data, and future directions.

Chin, Mian↗