SEARCH · Search NASA
Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.
Quote a phrase for an exact phrase match. Source license links do not imply unrestricted reuse.
A mass shift method using ICP-MS/MS with O 2 reaction gas is used for ultra-trace determinations of U and Th in samples containing W, Ir, Pt, and Au derived polyatomic interferants without the need for extensive chemical sample preprocessing.
Fluorophores covalently bound to azacrown ether ionophores can be assembled into sensitive turn-on chemosensors. The size specificity and electron-rich nature of the ionophore's binding domain contribute to both selectivity and strong turn-on fluorescence sensing by various mechanisms when properly constructed. Aza-18-crown-6 ethers are quite selective for binding to K + and Ba 2+ , yet the more electron-withdrawing dicationic nature of barium imposes a larger electronic effect on turn-on fluorescent sensors. Barium chemosensors can be important for measuring soluble Ba 2+ in drinking water and have gained recent attention for their potential to enhance the detection of rare events in xenon decay. Here we quantify the capability of three chemosensors, marketed for biologically useful K + sensing, as effective probes for Ba 2+ ions. Here, we present measurements from bulk spectrofluorometry to characterize the system in aqueous solutions and demonstrate the usefulness of these species for low-background single-ion fluorescence microscopy, revealing new candidates for Ba 2+ sensing.
Here, we present a study of the relation between X-rays and ultraviolet emission in quasars for a sample of broad-line, radio-quiet objects obtained from the cross-match of the Sloan Digital Sky Survey DR14 with the latest Chandra Source Catalog 2.0 (2332 quasars) and the Chandra COSMOS Legacy survey (273 quasars). The non-linear relation between the ultraviolet (at 2500 Å, L UV ) and the X-ray (at 2 keV, L X ) emission in quasars has been proved to be characterised by a smaller intrinsic dispersion than the observed one, as long as a homogeneous selection, aimed at preventing the inclusion of contaminants in the sample, is fulfilled. By leveraging on the low background of Chandra, we performed a complete spectral analysis of all the data available for the SDSS-CSC2.0 quasar sample (i.e. 3430 X-ray observations), with the main goal of reducing the uncertainties on the source properties (e.g. flux, spectral slope). We analysed whether any evolution of the L X – L UV relation exists by dividing the sample in narrow redshift intervals across the redshift range spanned by our sample, z ≃ 0.5–4. We find that the slope of the relation does not evolve with redshift and it is consistent with the literature value of 0.6 over the explored redshift range, implying that the mechanism underlying the coupling of the accretion disc and hot corona is the same at the different cosmic epochs. We also find that the dispersion decreases when examining the highest redshifts, where only pointed observations are available. These results further confirm that quasars are ‘standardisable candles’, that is we can reliably measure cosmological distances at high redshifts where very few cosmological probes are available.
PIONEER is a high Q-resolution, single-crystal, polarized neutron diffractometer at the Second Target Station (STS), Oak Ridge National Laboratory. It will provide the unprecedented capability of measuring tiny crystals (0.001 mm 3 , i.e., x-ray diffraction size), ultra-thin films (10 nm thickness), and weak structural and magnetic transitions. PIONEER benefits from the increased peak brightness of STS cold-neutron sources and uses advanced Montel mirrors that are able to deliver a focused beam with a high brilliance transfer, a homogeneous profile, and a low background. Monte Carlo simulations suggest that the optimized instrument has a high theoretical peak brilliance of 2.9 × 10 12 n cm -2 sr -1 Å -1 s -1 at 2.5 Å at the sample position, within a 5 × 5 mm 2 region and a ±0.3° divergence range. The moderator-to-sample distance is 60 m, providing a nominal wavelength band of 4.3 Å with a wavelength resolution better than 0.2% in the wavelength range of 1.0–6.0 Å. PIONEER is capable of characterizing large-scale periodic structures up to 200 Å. With a sample-to-detector distance of 0.8 m, PIONEER accommodates various sample environments, including low/high temperature, high pressure, and high magnetic/electric field. Additionally, a large cylindrical detector array (4.0 sr) with a radial collimator is planned to suppress the background scattering from sample environments. Bottom detector banks provide an additional 0.4 sr coverage or can be removed if needed to accommodate special sample environments. We present virtual experimental results to demonstrate the scientific performance of PIONEER in measuring tiny samples.
Here we provide an overview of a pressure cell designed to apply uniaxial pressure to single crystals for the study, by neutron scattering techniques, of strongly correlated magnetic systems and, in particular, quantum magnets. A detailed overview of the pressure cell components, their requirements, and links to the scientific and technical specifications are presented. The pressure cell is able to accommodate a 200 mm 3 single crystal that can be pressurized up to 2 GPa at cryogenic temperatures. The pressure cell is consistent with the requirements of inelastic neutron scattering and, importantly, neutron polarization analysis. A particular strength of the uniaxial pressure cell is the highly uniform and low background for a wide scattering angle of 360° horizontally and ±20° vertically. We show the performance of the uniaxial pressure cell using a relevant neutron scattering instrument, the polarized diffuse scattering instrument, D7. The experiments confirm that the cell complies with the scientific and technical requirements. This uniaxial pressure cell will provide a useful additional tool in the sample environment suite available for the study of quantum magnetism.
Photoconductive semiconductor switches (PCSSs) are fabricated on type IIa diamond substrates with varying boron and nitrogen impurity levels (<10 14 –10 16 cm –3 ). The photoresponse of lateral PCSS is reported over the incident laser wavelength range (212–240 nm), energy per pulse (5–65 μJ), and DC bias (–1.2 to +1.2 kV). The PCSS device with the lowest boron and nitrogen impurity concentration achieves the highest normalized responsivity of 9.1 × 10 –8 A-cm/W-V, peak photocurrent of 8.0 A, and on/off ratio of 2.3 × 10 11 at a DC bias of +1.2 kV with the potential for even higher currents at increased DC bias. All PCSS display fast rise times (<3 ns), limited by the laser's rise time. However, photoresponse measurements reveal that higher impurity levels reduce the photocurrent and decrease the on/off ratio. Furthermore, these results highlight the performance advantages of using low background concentration type IIa diamond substrates for PCSS fabrication and present a promising route toward advanced high-power, high-speed diamond-based switches.
High energy collisions at the High-Luminosity Large Hadron Collider (LHC) produce a large number of particles along the beam collision axis, outside of the acceptance of existing LHC experiments. The proposed Forward Physics Facility (FPF), to be located several hundred meters from the ATLAS interaction point and shielded by concrete and rock, will host a suite of experiments to probe standard model (SM) processes and search for physics beyond the standard model (BSM). In this report, we review the status of the civil engineering plans and the experiments to explore the diverse physics signals that can be uniquely probed in the forward region. FPF experiments will be sensitive to a broad range of BSM physics through searches for new particle scattering or decay signatures and deviations from SM expectations in high statistics analyses with TeV neutrinos in this low-background environment. High statistics neutrino detection will also provide valuable data for fundamental topics in perturbative and non-perturbative QCD and in weak interactions. Experiments at the FPF will enable synergies between forward particle production at the LHC and astroparticle physics to be exploited. We report here on these physics topics, on infrastructure, detector, and simulation studies, and on future directions to realize the FPF’s physics potential.
Cyclotron radiation emission spectroscopy (CRES) is a modern technique for high-precision energy spectroscopy, in which the energy of a charged particle in a magnetic field is measured via the frequency of the emitted cyclotron radiation. The He6-CRES collaboration aims to use CRES to probe beyond the standard model physics at the TeV scale by performing high-resolution and low-background beta-decay spectroscopy of 6 He and 19 Ne. Having demonstrated the first observation of individual, high-energy (0.1–2.5 MeV) positrons and electrons via their cyclotron radiation, the experiment provides a novel window into the radiation of relativistic charged particles in a waveguide via the time-derivative (slope) of the cyclotron radiation frequency, df c /dt. We show that analytic predictions for the total cyclotron radiation power emitted by a charged particle in circular and rectangular waveguides are approximately consistent with the Larmor formula, each scaling with the Lorentz factor of the underlying e ± as γ 4 . This hypothesis is corroborated with experimental CRES slope data.
CUPID is the next generation experiment which will use scintillating cryogenic calorimeters to search for the neutrinoless double β decay. This unobserved process would shed light on the nature of the neutrino, which up to our knowledge could be a Majorana or a Dirac particle, and would give us an important hint to explain the lack of antimatter in the universe. This ambitious search needs a detector with unique characteristics such as an extremely low background level and an excellent energy resolution. CUPID is now in advanced R&D state to optimize the detector design in order to completely exploit the potentialities of scintillating cryogenic calorimeters. In the following I will describe the test performed at the LNGS (Laboratori Nazionali del Gran Sasso) of a single module of the future CUPID detector. In this contribution we present the performance obtained with a novel assembly concept, proving that it matches the requirements for CUPID.
Silicon photomultipliers are regarded as a very promising technology for next-generation, cutting-edge detectors for low-background experiments in particle physics. This work presents systematic reflectivity studies of Silicon Photomultipliers (SiPM) and other samples in liquid xenon at vacuum ultraviolet (VUV) wavelengths. A dedicated setup at the University of Münster has been used that allows to acquire angle-resolved reflection measurements of various samples immersed in liquid xenon with 0.45° angular resolution. Four samples are investigated in this work: one Hamamatsu VUV4 SiPM, one FBK VUV-HD SiPM, one FBK wafer sample and one Large-Area Avalanche Photodiode (LA-APD) from EXO-200. Here, the reflectivity is determined to be 25–36 % at an angle of incidence of 20° for the four samples and increases to up to 65 % at 70° for the LA-APD and the FBK samples. The Hamamatsu VUV4 SiPM shows a decline with increasing angle of incidence. The reflectivity results will be incorporated in upcoming light response simulations of the nEXO detector.
The EXO-200 experiment searched for neutrinoless double-beta decay of 136 Xe with a single-phase liquid xenon detector. It used an active mass of 110 kg of 80.6%-enriched liquid xenon in an ultra-low background time projection chamber with ionization and scintillation detection and readout. Here, this paper describes the design and performance of the various support systems necessary for detector operation, including cryogenics, xenon handling, and controls. Novel features of the system were driven by the need to protect the thin-walled detector chamber containing the liquid xenon, to achieve high chemical purity of the Xe, and to maintain thermal uniformity across the detector.
The LUX-ZEPLIN (LZ) detector is a dual-phase liquid xenon time projection chamber (TPC) installed at the Sanford Underground Research Facility (Lead, South Dakota) at a depth of 1478 meters. Although the main objective of LZ is the direct detection of dark matter, its low background environment allows for the search of other rare processes, such as the neutrinoless double beta decay of xenon isotopes 134 Xe and 136 Xe with the respective Q-values of 826 keV and 2458 keV. The sensitivity of the detector to these decays is directly determined by the energy resolution, which, in turn, is degraded by non-uniformities in detector response. In this work, we present a novel method to correct, in the data, the non-uniformity of the light collected by an array of photosensors in a scintillation detector. This method is based on the knowledge of the light response functions of individual photosensors. With these techniques, we report, at a very early phase of the detector operations, a state-of-the-art energy resolution (σ/μ) of (0.67 ± 0.01)% at 2614 keV for the fiducial volume of 5.6 tonnes of liquid xenon.
The Majorana Demonstrator was a search for neutrinoless double-beta decay (0νββ) in the 76 Ge isotope. It was staged at the 4850-foot level of the Sanford Underground Research Facility (SURF) in Lead, SD. The experiment consisted of 58 germanium detectors housed in a low background shield and was calibrated once per week by deploying a 228 Th line source for 1 to 2 hours. The energy scale calibration determination for the detector array was automated using custom analysis tools. We describe the offline procedure for calibration of the Demonstrator germanium detectors, including the simultaneous fitting of multiple spectral peaks, estimation of energy scale uncertainties, and the automation of the calibration procedure.
The BUTTON-30 detector is a 30-tonne technology demonstrator designed to evaluate the potential of hybrid event detection, simultaneously exploiting both Cherenkov and scintillation light to detect particles produced in neutrino interactions. The detector is installed at a depth of 1.1 km in the Boulby Underground Laboratory allowing to test the performance of this new technology underground in a low background environment. This paper describes the design and construction of the experiment.
The Scintillating Bubble Chamber (SBC) Collaboration is designing a new generation of low background, noble liquid bubble chamber experiments with sub-keV nuclear recoil threshold. These experiments combine the electronic recoil blindness of a bubble chamber with the energy resolution of noble liquid scintillation, and maintain electron recoil discrimination at higher degrees of superheat (lower nuclear recoil thresholds) than Freon-based bubble chambers. A 10-kg liquid argon bubble chamber has the potential to set world leading limits on the dark matter nucleon cross-section for 𝒪(GeV/c 2 ) masses, and to perform a high statistics coherent elastic neutrino nuclear scattering measurement with reactor neutrinos. This work presents a detailed calibration plan to measure the detector response of these experiments, combining photoneutron scattering with two new techniques to induce sub-keV nuclear recoils: nuclear Thomson scattering and thermal neutron capture.
The axion, a hypothetical pseudo-scalar particle proposed by Peccei and Quinn to resolve the strong CP problem in quantum chromodynamics, remains one of the most compelling dark matter candidates. Axions and Axion-Like Particles (ALPs) are characterized by a broad and largely unconstrained parameter space in mass and coupling strength, motivating extensive experimental searches. The International Axion Observatory (IAXO) is a next-generation axion helioscope designed to achieve over an order of magnitude improvement in sensitivity to the axion-photon coupling constant gaγ relative to previous experiments such as the CERN Axion Solar Telescope (CAST). IAXO will employ large-scale superconducting magnets, precision x-ray optics, and ultra-low-background detectors to search for solar axions produced primarily via the Primakoff effect. This work presents the design and performance of the IAXO pathfinder x-ray optic, a technological demonstrator that validated the optical concepts for IAXO through axion searches at CAST. Comprehensive ray-tracing simulations and experimental measurements were conducted to assess the optic's effective area, detection efficiency, and background suppression capabilities. Deployed at CAST in conjunction with Micromegas and GridPix detectors, the Pathfinder demonstrated record-setting sensitivity to both gaγ and the axion-electron coupling gae, establishing the most stringent laboratory constraints on solar axions to date. These results confirm the viability of the IAXO optical design and detector concept, providing a critical technological benchmark that informs the ongoing development of the BabyIAXO and full-scale IAXO telescopes.
Here, we present a summary of the in-orbit performance of the soft X-ray imaging telescope Xtend onboard the X-Ray Imaging and Spectroscopy Mission (XRISM), based on in-flight observation data, including first-light celestial objects, calibration sources, and results from the cross-calibration campaign with other currently operating X-ray observatories. XRISM/Xtend has a large field of view of ${38{^{\prime }_{.}}5}$ $\times$ ${38{^{\prime }_{.}}5}$, covering an energy range of 0.4–13 keV, as demonstrated by the first-light observation of the galaxy cluster Abell 2319. It also features an energy resolution of 170–180 eV at 6 keV, which meets the mission requirement and enables us to resolve He-like and H-like Fe K$\alpha$ lines. Throughout the observation during the performance verification phase, we confirm that two issues identified in the Soft X-ray Imager (SXI) onboard the previous Hitomi mission—light leakage and crosstalk events—are addressed and suppressed in the case of Xtend. A joint cross-calibration observation of the bright quasar 3C 273 results in an effective area measured to be $\sim$420 cm$^{2}$ at1.5 keV and $\sim$310 cm$^{2}$ at 6.0 keV, which matches values obtained in ground tests. We also continuously monitor the health of Xtend by analyzing overclocking data, calibration source spectra, and day-Earth observations; the readout noise is stable and low, and contamination is negligible even one year after launch. A low background level compared with other major X-ray instruments onboard satellites, combined with the largest grasp ($\Omega _{\rm eff}\sim 60$ cm$^2$ deg$^2$) of Xtend, will not only support Resolve analysis, but also enable significant scientific results on its own. This includes near-future follow-up observations and transient searches in the context of time-domain and multi-messenger astrophysics.
The LEGEND Collaboration is searching for neutrinoless double-beta (0𝜈𝛽𝛽) decay by operating high-purity germanium detectors enriched in 76 Ge in a low-background liquid argon environment. Building on key technological innovations from the GERmanium Detector Array (GERDA) experiment and the MAJORANA DEMONSTRATOR experiment, LEGEND-200 has performed a first 0𝜈𝛽𝛽 decay search based on 61.0 kg yr of data. Over half of this exposure comes from our highest performing detectors, including newly developed inverted-coaxial detectors, and is characterized by an estimated background level of 0.5$^{+0.3}_{−0.2}$ cts/(keV ton yr) in the 0𝜈𝛽𝛽 decay signal region. A combined analysis of data from GERDA, the MAJORANA DEMONSTRATOR, and LEGEND-200, characterized by a 90% confidence level exclusion sensitivity of 2.8 ×10 26 yr on the half-life of 0𝜈𝛽𝛽 decay, reveals no evidence for a signal and sets a new observed lower limit at 𝑇$^{0𝜈}_{1/2}$ > 1.9 × 10 26 yr (90% confidence level). Assuming the decay is mediated by Majorana neutrinos, this corresponds to an upper limit on the effective Majorana mass in the range 𝑚 𝛽𝛽 < 75–200 meV, depending on the adopted nuclear matrix element.