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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 127 records · Page 7
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Ferrimagnetic 120 ° magnetic structure in Cu 2 OSO 4

We report magnetic properties of a 3d 9 (Cu 2+ ) magnetic insulator Cu 2 OSO 4 measured on both powder and single crystal. The magnetic atoms of this compound form layers whose geometry can be described either as a system of chains coupled through dimers or as a kagome lattice where every third spin is replaced by a dimer. Specific heat and DC susceptibility show a magnetic transition at 20 K, which is also confirmed by neutron scattering. Magnetic entropy extracted from the specific heat data is consistent with an S=1/2 degree of freedom per Cu 2+ , and so is the effective moment extracted from DC susceptibility. The ground state has been identified by means of neutron diffraction on both powder and single crystal and corresponds to an ~120° spin structure in which ferromagnetic intradimer alignment results in a net ferrimagnetic moment. No evidence is found for a change in lattice symmetry down to 2 K. Finally, our results suggest that Cu 2 OSO 4 represents a type of model lattice with frustrated interactions where interplay between magnetic order, thermal and quantum fluctuations can be explored.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2021

Magnetic structure and multiferroicity of Sc-substituted hexagonal YbFeO 3

The hexagonal rare-earth ferrite RFeO 3 family represents a unique class of multiferroics exhibiting weak ferromagnetism, and a strong coupling between magnetism and structural trimerization is predicted. However, the hexagonal structure for RFeO 3 remains metastable in conventional conditions. We have succeeded in stabilizing the hexagonal structure of polycrystalline YbFeO 3 by partial Sc substitution of Yb. Using bulk magnetometry and neutron diffraction, we find that Yb 0.42 Sc 0.58 FeO 3 orders into a canted antiferromagnetic state with the Néel temperature T N ~ 165K, below which the Fe 3+ moments form the triangular configuration in the ab plane and their in-plane projections are parallel to the [100] axis, consistent with magnetic space group P6 3 c'm'. It is determined that the spin canting is aligned along the c axis, giving rise to the weak ferromagnetism. Furthermore, the Fe 3+ moments reorient toward a new direction below reorientation temperature T R ~ 40K, satisfying magnetic subgroup P6 3 , while the Yb 3+ moments order independently and ferrimagnetically along the c axis at the characteristic temperature T Yb ~ 15K. Interestingly, reproducible modulation of electric polarization induced by magnetic field at low temperature is achieved, suggesting that the delicate structural distortion associated with two-up/one-down buckling of the Yb/Sc planes and tilting of the FeO 5 bipyramids may mediate the coupling between ferroelectric and magnetic orders under magnetic field. Furthermore, the present work represents substantial progress to search for high-temperature multiferroics in hexagonal ferrites and related materials.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2022

Interplay of electronic structure, magnetism, strain, and defects in carbide $\mathrm{MX}$enes

We report the two-dimensional (2D) magnetic and semiconducting materials, including carbide MXenes, are in high demand for magneto-electronic devices and applications. Here, we report a first-principles study of electronic structure and magnetism of a Ti 2 C MXene, its derivatives Ti 2 CT 2 (T = -F, -O, -OH, -H), and the effect of single vacancy defects (25% C, 12.5% O, and 12.5% and 5.5% Ti) and transition metal (V, Cr, Mn, and Co) dopings. The MAX phase Ti 2 AlC is a non-magnetic (NM) metal which upon removal of Al layer forms a pristine Ti 2 C MXene with A-type antiferromagnetic (AFM) semiconductor having reliable transition temperature (T N = 41K) predicted by the Heisenberg model. All the functionalized MXenes are stable as NM metal except for Ti 2 CO 2 which remains semiconducting with NM ground state. The significant effect of spin–orbit coupling (SOC) is evident in the band structure forming Dirac-like cones and band inversions near the Fermi level. Depending upon the type of vacancy defects Ti 2 CO 2 is NM metal and ferromagnetic (FM) metal. The transition metal (TM) doped MXenes fulfill FM Stoner criterion. The V- and Co-doped MXenes are metals, whereas Cr- and Mn-doped are half-metal and semiconductor.

2D magnetism↗
NASA NTRS1974

The motion and magnetic structure of the plasma sheet near 30 earth radii

Data taken by the NASA-GSFC magnetometer aboard the Explorer 34 satellite are analyzed in an effort to ascertain the average motion and magnetic field structure of the plasma sheet near 30 earth radii. It is found that the flapping motion of the plasma sheet in the solar ecliptic Z-coordinate is characterized by a typical speed of 90 km/sec and an amplitude of plus or minus 2 earth radii. Results suggest that there exists a layer of nearly uniform cross-tail current density in the central region of the plasma sheet approximately 2.3-2.6 earth radii thick within which the solar-magnetospheric X-component of the magnetic field changes from 10 gamma to -10 gamma.

Bowling, S. B.↗
DOE OSTI2020

Electronic structure, magnetic properties, and exchange splitting of gadolinium intermetallics

Here, we report here the electronic structure calculations of the magnetic moment, magneto-crystalline anisotropy energy (MAE), and density of states (DOS) of Gd-metal, GdAl 2 , GdAl 3 , GdCo 2 , GdCo 3 , and GdCo 5 . From the DOS, the exchange splitting energy is derived to map ferrimagnetic to paramagnetic phase transition (Curie temperature, T C ). The employed theoretical method here is based on advanced density functional theory, specifically the linearized augmented plane wave method (LAPW) within the local spin density approximation (LSDA), including spin–orbit coupling (SOC) and Hubbard model parameter (U). DOS analysis of both Gd-Al and Gd-Co systems reveals a strong correlation between exchange splitting energy and T C . The Gd-Co system exhibits an enormous exchange splitting energy among Co-3d electrons, vastly overwhelming the vanishing Gd 5d exchange splitting. Finally, these findings suggest that exchange splitting of Co-3d electrons plays a key role in the ground state magnetism and magnetic transition temperatures in these materials.

36 MATERIALS SCIENCE↗
NASA NTRS2014

Hi-C Observations of an Active Region Corona, and Investigation of the Underlying Magnetic Structure

The solar corona is much hotter (>=10(exp 6) K) than its surface (approx 6000 K), puzzling astrophysicists for several decades. Active region (AR) corona is again hotter than the quiet Sun (QS) corona by a factor of 4-10. The most widely accepted mechanism that could heat the active region corona is the energy release by current dissipation via reconnection of braided magnetic field structure, first proposed by E. N. Parker three decades ago. The first observational evidence for this mechanism has only recently been presented by Cirtain et al. by using High-resolution Coronal Imager (Hi-C) observations of an AR corona at a spatial resolution of 0.2 arcsec, which is required to resolve the coronal loops, and was not available before the rocket flight of Hi-C in July 2012. The Hi-C project is led by NASA/MSFC. In the case of the QS, work done by convection/granulation on the inter-granular feet of the coronal field lines translates into the heat observed in the corona. In the case of the AR, as here, there could be flux emergence, cancellation/submergence, or shear flows generating large stress and tension in coronal field loops which is released as heat in the corona. We are currently investigating the changes taking place in photospheric feet of the magnetic field involved with brightenings in the Hi-C AR corona. For this purpose, we are also using SDO/AIA data of +/- 2 hours around the 5 minutes Hi-C flight. In the present talk, I will first summarize some of the results of the Hi-C observations and then present some results from our recent analysis on what photospheric processes feed the magnetic energy that dissipates into heat in coronal loops.

Tiwari, S. K.↗
NASA NTRS2004

The Effects of Differential Rotation on the Magnetic Structure of the Solar Corona: MHD Simulations

Coronal holes are magnetically open regions from which the solar wind streams. Magnetic reconnection has been invoked to reconcile the apparently rigid rotation of coronal holes with the differential rotation of magnetic flux in the photosphere. This mechanism might also be relevant to the formation of the slow solar wind, the properties of which seem to indicate an origin from the opening of closed magnetic field lines. We have developed a global MHD model to study the effect of differential rotation on the coronal magnetic field. Starting from a magnetic flux distribution similar to that of Wang et al., which consists of a bipolar magnetic region added to a background dipole field, we applied differential rotation over a period of 5 solar rotations. The evolution of the magnetic field and of the boundaries of coronal holes are in substantial agreement with the findings of Wang et al.. We identified examples of interchange reconnection and other changes of topology of the magnetic field. Possible consequences for the origin of the slow solar wind are also discussed.

Lionello, Roberto↗
DOE OSTI2021

Magnetic structure of triangular lattice compound Tb2Ni0.90Si2.94

AlB 2 -type ternary intermetallic compound Tb 2 Ni 0.90 Si 2.94 (space group P 6=mmm, hP 3, No. 191) was reported to exhibit spin freezing behaviour of the ferromagnetic clusters present in the system below T f = 9:9 K, along with the presence of spatially limited antiferromagnetic phase. In this work, on the basis of variable temperature zero-field neutron diffraction measurements, we have shown that the antiferromagnetic phase transition occurs for the compound below T N ~13 K. Neutron diffraction study indicates ab-plane non-collinear sine-modulated antiferromagnetic ordering of the system with wave vectors of k 1 = [±1/6, ±1/6, 0] and k 2 = [±1/3, ±1/3, 0] down to 1.7 K. The weak and diffuse nature of the magnetic Bragg peaks along with limited coherence length further confirm the short-range nature of the antiferromagnetic phase in this compound.

36 MATERIALS SCIENCE↗
NASA NTRS1982

On the three-dimensional magnetic structure of the plasmoid created in the magnetotail at substorm onset

The magnetic field in the plasmoid which is created by the reconnection of magnetic field lines at a neutral line formed in the near-earth region of the plasma sheet at substorm onset, and which flows out of the magnetotail into the magnetosphere's wake, displays a strong positive or negative Y(SM) component that has been difficult to reconcile with the standard, two-dimensional reconnection geometry. It is shown that this deviation of the magnetic field is a manifestation of the newly-reconnected field line loop's draping toward the tail's central or midnight meridian, and that the draping is a consequence of the three-dimensional plasma flow associated with the reconnection process.

Hones, E. W., Jr.↗
DOE OSTI2022

A combined first principles study of the structural, magnetic, and phonon properties of monolayer CrI3

The first magnetic 2D material discovered, monolayer (ML) CrI3, is particularly fascinating due to its ground state ferromagnetism. However, because ML materials are difficult to probe experimentally, much remains unresolved about ML CrI3’s structural, electronic, and magnetic properties. Here, we leverage Density Functional Theory (DFT) and high-accuracy Diffusion Monte Carlo (DMC) simulations to predict lattice parameters, magnetic moments, and spin–phonon and spin–lattice coupling of ML CrI3. We exploit a recently developed surrogate Hessian DMC line search technique to determine CrI3’s ML geometry with DMC accuracy, yielding lattice parameters in good agreement with recently published STM measurements—an accomplishment given the ~10% variability in previous DFT-derived estimates depending upon the functional. Strikingly, we find that previous DFT predictions of ML CrI3’s magnetic spin moments are correct on average across a unit cell but miss critical local spatial fluctuations in the spin density revealed by more accurate DMC. DMC predicts that magnetic moments in ML CrI3 are 3.62 μB per chromium and -0.145 μB per iodine, both larger than previous DFT predictions. The large disparate moments together with the large spin–orbit coupling of CrI3’s I-p orbital suggest a ligand superexchange-dominated magnetic anisotropy in ML CrI3, corroborating recent observations of magnons in its 2D limit. We also find that ML CrI3 exhibits a substantial spin–phonon coupling of ~3.32 cm-1. Our work, thus, establishes many of ML CrI3’s key properties, while also continuing to demonstrate the pivotal role that DMC can assume in the study of magnetic and other 2D materials.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1986

On the magnetic structure of the quiet transition region

Existing models of the quiet chromosphere-corona transition region predict a distribution of emission measure over temperature that agrees with observation for a T greater than about 100,000 K. These 'network' models assume that all magnetic field lines that emerge from the photosphere extend into and are in thermal contact with the corona. It is shown that the observed fine-scale structure of the photospheric magnetic network instead suggests a two-component picture in which magnetic funnels that open into the corona emerge from only a fraction of the network. The gas that makes up the hotter transition region is mostly contained within these funnels, as in standard models, but, because the funnels are more constricted in our picture, the heat flowing into the cooler transition region from the corona is reduced by up to an order of magnitude. The remainder of the network is occupied by a population of low-lying loops with lengths less than about 10,000 km. It is proposed that the cooler transition region is mainly located within such loops, which are magnetically insulated from the corona and must, therefore, be heated internally. The fine-scale structure of ultraviolet spectroheliograms is consistent with this proposal, and theoretical models of internally heated loops can explain the behavior of the emission measure below a T of aobut 100,000 K.

Rabin, D.↗
NASA NTRS2014

Magnetic Structure of Sites of Braiding in Hi-C Active Region

High‐resolution Coronal Imager (Hi‐C) observations of an active region (AR) corona, at a spatial resolution of 0.2 arcsec, have offered the first direct evidence of field lines braiding, which could deliver sufficient energy to heat the AR corona by current dissipation via magnetic reconnection, a proposal given by Parker three decades ago. The energy required to heat the corona must be transported from the photosphere along the field lines. The mechanism that drives the energy transport to the corona is not yet fully understood. To investigate simultaneous magnetic and intensity structure in and around the AR in detail, we use SDO/HMI+AIA data of + / ‐ 2 hours around the 5 minute Hi‐C flight. In the case of the QS, work done by convection/granulation on the inter‐granular feet of the coronal field lines probably translates into the heat observed in the corona. In the case of the AR, as here, there could be flux emergence, cancellation/submergence, or shear flows generating large stress and tension in coronal field loops which is released as heat in the corona. However, to the best of our knowledge, there is no observational evidence available to these processes. We investigate the changes taking place in the photospheric feet of the magnetic field involved with brightenings in the Hi‐C AR corona. Using HMI 45s magnetograms of four hours we find that, out of the two Hi‐C sub‐regions where the braiding of field lines were recently detected, flux emergence takes place in one region and flux cancellation in the other. The field in these sub‐regions are highly sheared and have apparent high speed plasma flows at their feet. Therefore, shearing flows plausibly power much of the coronal and transition region heating in these areas of the AR. In addition, the presence of large flux emergence/cancellation strongly suggests that the work done by these processes on the pre‐existing field also drives much of the observed heating.

Tiwari, S. K.↗
NASA NTRS1979

The effects of magnetic structure on the conduction cooling of flare loops

A model of the sheared magnetic field in a coronal loop is used to evaluate the average cross-field suppression of axial thermal conduction. If the energy source is uniform in radius, this can lead to heat-flux reduction by a factor greater than three. When the source is annular, in a region of radius where the current density and shear are peaked, the effect can be significantly larger. In one extreme case, however, in which magnetic tearing provides the heating in a very narrow layer, the spatial resonance of the source excitation in a long loop leads to approximately axial conduction.

Van Hoven, G.↗
NASA NTRS1974

Relation of coronal magnetic structure to the interplanetary proton events of August 2-9, 1972

In order to interpret the time history of protons of energy greater than about 13.5 MeV observed on Pioneers 9 and 10 and IMP 5 from the flares of Aug. 2, 4 and 7, the coronal connection longitudes of the interplanetary field lines were estimated using the solar wind velocities measured on the spacecraft. There is reasonable agreement between the observed magnetic field polarity at Pioneer 9 and the equatorial chromospheric polarity at the inferred connection longitudes. The protons appear to be released preferentially in a large magnetic neutral-line complex that surrounds the flare region (McMath 11976) from Carrington longitudes 0 to 60. Although impulsive proton events were observed from all three flares by Pioneer 9, only the second two were seen at earth, and Pioneer 10 never showed comparable impulsive response. These apparent discrepancies are resolved by comparison with magnetic neutral line structure.

Roelof, E. C.↗
NASA NTRS1984

Magnetic structure of the distant geotail from -60 to -220 earth radii - ISEE-3

ISEE-3 magnetic-field measurements in the region of the geomagnetic tail from -80 to -220 earth radii are reported and discussed. A well-ordered field structure is found, comprising two 7-8-nT lobes separated by a plasma sheet, an embedded neutral sheet with significant By fields, and an intermittent plasma-sheet boundary layer with 5-nT-amplitude (peak-to-peak) electromagnetic waves. The plasma-sheet Bz distribution changes from principally northern orientation near the earth to an approximately equal north-south distribution at 200-220 earth radii. These findings are considered to be in general agreement with magnetic-reconnection models of the magnetosphere, with reconnection either throughout the region observed (in tearing-mode or plasmoid-formation models) or at a constant (about 220-earth-radii) or variable (40-80 to 220-earth-radii) X line (in X-line models).

Tsurutani, B. T.↗
DOE OSTI2024

Nanometric modulations of the magnetic structure of the element Nd

The rare earth neodymium arguably exhibits the most complex magnetic ordering and series of magnetic phase transitions of the elements. Here we report the results of small-angle neutron scattering (SANS) measurements as a function of temperature and applied magnetic field to study magnetic correlations on nanometer length scales in Nd. We support these results with additional neutron diffraction, thermodynamic and synchrotron x-ray measurements. The SANS measurements reveal the presence of modulation vectors characterizing the ordered spin configuration which exhibit changes in magnitude and direction that are phase dependent. Between 5.9 and 7.6 K an additional modulation vector is observed with magnitude Q = 0.12 Å -1 . This scattering appears to originate from order of the Nd layers which contain a center of inversion. Tracking this modulation vector as a function of magnetic field indicates a phase boundary at ≈1 T. The modulation vectors observed in this study establish the presence of nanometer length scale spin textures which are likely stabilized by frustrated Ruderman–Kittel–Kasuya–Yosida (RKKY) interactions.

36 MATERIALS SCIENCE↗