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At least 127 records · Page 7

Pulse height response of an optical particle counter to monodisperse aerosols

The pulse height response of a right angle scattering optical particle counter has been investigated using monodisperse aerosols of polystyrene latex spheres, di-octyl phthalate and methylene blue. The results confirm previous measurements for the variation of mean pulse height as a function of particle diameter and show good agreement with the relative response predicted by Mie scattering theory. Measured cumulative pulse height distributions were found to fit reasonably well to a log normal distribution with a minimum geometric standard deviation of about 1.4 for particle diameters greater than about 2 micrometers. The geometric standard deviation was found to increase significantly with decreasing particle diameter.

Wilmoth, R. G.↗

Direct Demonstration of the Concept of Unrestricted Effective-Medium Approximation

The modified unrestricted effective-medium refractive index is defined as one that yields accurate values of a representative set of far-field scattering characteristics (including the scattering matrix) for an object made of randomly heterogeneous materials. We validate the concept of the modified unrestricted effective-medium refractive index by comparing numerically exact superposition T-matrix results for a spherical host randomly filled with a large number of identical small inclusions and Lorenz-Mie results for a homogeneous spherical counterpart. A remarkable quantitative agreement between the superposition T-matrix and Lorenz-Mie scattering matrices over the entire range of scattering angles demonstrates unequivocally that the modified unrestricted effective-medium refractive index is a sound (albeit still phenomenological) concept provided that the size parameter of the inclusions is sufficiently small and their number is sufficiently large. Furthermore, it appears that in cases when the concept of the modified unrestricted effective-medium refractive index works, its actual value is close to that predicted by the Maxwell-Garnett mixing rule.

Scattering↗

Fabry-Perot interferometer measurement of static temperature and velocity for ASTOVL model tests

A spectrally resolved Rayleigh/Mie scattering diagnostic was developed to measure temperature and wing-spanwise velocity in the vicinity of an ASTOVL aircraft model in the Lewis 9 x 15 Low Speed Wind Tunnel. The spectrum of argon-ion laser light scattered by the air molecules and particles in the flow was resolved with a Fabry-Perot interferometer. Temperature was extracted from the spectral width of the Rayleigh scattering component, and spanwise gas velocity from the gross spectral shift. Nozzle temperature approached 800 K, and the velocity component approached 30 m/s. The measurement uncertainty was about 5 percent for the gas temperature, and about 10 m/s for the velocity. The large difference in the spectral width of the Mie scattering from particles and the Rayleigh scattering from gas molecules allowed the gas temperature to be measured in flow containing both naturally occurring dust and LDV seed (both were present).

Kourous, Helen E.↗

Absorption profile of a planetary atmosphere - A proposal for a scattering independent determination.

The use of scattering theory to infer atmospheric optical parameters requires the separation of absorption and scattering. It is demonstrated that a gradient flux relation exists that would provide the absorption (altitude) profile independently of scattering and irrespective of the state of polarization of the light field. The relation is derived for an atmosphere of plane-parallel or spherical geometry and for broad (continuum) and narrow (spectral line) frequency bands. The results are shown to hold, in particular, for the polarizations induced by both Rayleigh and Mie scattering in the field. Experimental setups are proposed for each of the cases considered of atmospheric geometry and frequency bandwidth.

Fymat, A. L.↗

On the Inversion of Light Scattering Data into Information on Aerosol Properties

The Backus-Gilbert inversion technique was applied to scattering data and calculated examples were given to ascertain its ability to recover the aerosol properties with no a-priori assumptions. In order to cheque this inversion procedure as well as other techniques (such as Daves' and Herman's et al.), a controlled experiment was performed. The experiment dealt with spherical particles the Mie scattering curves of which was measured by use of a dye-laser. These curves were used to accurately determine the refractive index of the particles. Mixtures of three different known sizes were then prepared and the scattering intensity vs. wavelength was measured at 90 deg scattering angle. The mixtures contained also various known relative concentrations of the three sizes. The analysis of the measured results will be shown and discussed.

Cohen, A.↗

Geophysics of Mars

A physical model of Mars is presented on the basis of light-scattering observations of the Martian atmosphere and surface and interior data obtained from observations of the geopotential field. A general description of the atmosphere is presented, with attention given to the circulation and the various cloud types, and data and questions on the blue haze-clearing effect and the seasonal darkening wave are summarized and the Mie scattering model developed to explain these observations is presented. The appearance of the planet from earth and spacecraft through Mariner 9 is considered, and attention is given to the preparation of topographical contour maps, the canal problem and large-scale lineaments observed from Mariner 9, the gravity field and shape of the planet and the application of Runcorn's geoid/convection theory to Mars. Finally, a summary of Viking results is presented and their application to the understanding of Martian geophysics is discussed.

Wells, R. A.↗

Assessment of Radiation Scattering by Dust in Mars Entry

The impact of gas phase radiation scattering by dust particle presence in Mars entry scenarios is assessed using a suite of numerical tools. A hypersonic gas and dilute particle multiphase flow is simulated using a mixed continuum model and an efficient size distribution quadrature scheme. Radiative transport is simulated with a hybrid ray-tracing and P1 spherical harmonics model. The NASA HARA radiation code and a Lorentz-Mie scattering model are used to predict the gas-particle mixture radiative properties. Application of the numerical suite to a representative case based on the Mars 2020 entry shows that, even at conditions in excess of the strongest recorded dust storm, the augmentation in surface radiative heat flux due to scattering alone is lower than 1%, and therefore negligible. Predictions with even higher dust loading conditions confirm that even highly uncertain dust mass profiles are unlikely to be a concern for the scattering augmentation mechanism.

Andrew Hinkle↗

Laser velocimetry technique applied to the Langley 0.3 meter transonic cryogenic tunnel

A low power laser velocimeter operating in the forward scatter mode was used to measure free stream mean velocities in the Langley 0.3 Meter Transonic Cryogenic Tunnel. Velocity ranging from 51 to 235 m/s was measured. Measurements were obtained for a variety of nominal tunnel conditions: Mach numbers from 0.20 to 0.77, total temperatures from 100 to 250 K, and pressures from 101 to 152 kPa. Particles were not injected to augment the existing Mie scattering materials. Liquid nitrogen droplets were the existing liqht scattering material. Tunnel vibrations and thermal effects had no detrimental effects on the optical system.

Gartrell, L. R.↗

Laser Radar Study Using Resonance Absorption for Remote Detection Of Air Pollutants

A laser radar using resonance absorption has an advantage of increased detection range and sensitivity compared with that achieved by Raman or resonance back scattering. In this paper, new laser radar system using resonance absorption is proposed and results obtained from this laser radar system are discussed. NO2, SO2 gas has an absorption spectrum at 4500 A and 3000 A respectively as shown in Fig. 1. A laser light including at least a set of an absorption peak (lambda)1 and a valley (lambda)2 is emitted into a pollutant atmosphere. The light reflected with a topographical reflector or an atmospheric Mie scattering as distributed reflectors is received and divided into two wavelength components (lambda)1 and (lambda)2. The laser radar system used in the investigation is shown in Fig', 2 and consists of a dye laser transmitter, an optical receiver with a special monochrometer and a digital processer. Table 1 shows the molecular constants of NO2, and SO2 and the dye laser used in this experiment. In this system, the absolute concentration of the pollutant gas can be measured in comparison with a standard gas cell. The concentration of NO2, SO2 as low as 0.1 ppm have been measured at 100 m depth resolution. For a 1 mJ laser output, the observable range of this system achieved up to 300 m using the distributed Mie reflector. The capability and technical limitation of the system will be discussed in detail.

Igarashi, Takashi↗

Feasibility of Rayleigh Scattering Flow Diagnostics in the National Transonic Facility

Laser-based Rayleigh light scattering (RLS) was performed in the National Transonic Facility (NTF) at NASA Langley Research Center. The goal was to determine if the free-stream flow undergoes clustering (early stage of condensation from gas to liquid) or remains in a pure diatomic molecular phase. Data indicate that clusters are not observable down to levels of 10% of the total light scatter for a variety of total pressures at one N2 cryogenic-mode total temperature (Tt = -50 F = 227 K) and one air-mode temperature (Tt = +130 F = 327 K). Thus RLS appears viable as a qualitative or quantitative diagnostic for flow density in NTF in the future. Particles are distinguished from optically unresolvable clusters because they are much larger and individually resolvable in the laser beam image with Mie scattering. The same RLS apparatus was also used, without modification, to visualize naturally occurring particles entrained in the flow for both cryogenic and air-modes. Estimates of the free-stream particle flux are presented, which may be important for interpretation of laminar-to-turbulent boundary-layer transition studies. 1

Herring, Gregory C.↗

Graupel and Snow Determination in Convection Using Dual-Wavelength Radar

Convective storms contain significant amounts of snow and graupel that each have different scattering properties for radar and radiometer remote sensing. TRMM TMI algorithms have relied heavily on radiative transfer calculations based on cloud model predicted microphysics information. In general, without in situ aircraft measurements, it is very difficult to separate snow and graupel using remote measurements. At the 94 GHZ frequency, snow is weakly attenuating while graupel is strongly attenuating. With a non-attenuating frequency such as X-band, one can distinguish Mie scattering from larger hydrometeors as well as attenuation from graupel. The presence of supercooled water will also cause attenuation of the 94 GHz radar signal, but this is mainly in convective updrafts. We will present preliminary results aimed at distinguishing snow from graupel using dual-wavelength (9.6 GHz, 94 GHz) measurements from aircraft overflights of convective storms in Florida. Measurements were made with the 9.6 GHz ER-2 Doppler Radar (EDOP) and the 94 GHz Cloud Radar System (CRS) over a number of different precipitation systems. Analysis of the vertical profiles at the two wavelengths provides information on snow and graupel regions, as well as supercooled water. The presentation will include examples from different cases and discussion of the results.

Heymsfield, Gerald↗

The spectral bidirectional reflectance of snow

A radiative transfer model for the bidirectional reflectance-distribution function (BRDF) shows that snow is moderately anisotropic in the near-infrared wavelengths. Although the directional-hemispherical albedo of snow decreases as the grains become larger, the forward scattering also increases, with the result that the illumination and viewing geometry must be considered when interpreting physical properties of the surface layer of the snow pack from remote sensing data. Measurements of the BRDF for a variety of snow conditions were made throughout the winter and spring seasons with a spectroradiometer, for wavelengths from 0.38 to 1.11 microns. Coincident with these the surface grain properties were analyzed by stereological methods. The data show that Mie scattering calculations using an equivalent spherical radius match the directional-hemispherical reflectance, but the BRDF usually shows a small peak in the backscattered direction that would not occur from spherical grains. The sphere with the same surface-to-volume ratio as the ice grains is used as the equivalent sphere.

Dozier, J.↗

Martian atmosphere modeling between 0.4 and 3.5 microns - Comparison of theory and experiment

A model of the lower atmosphere of Mars has been constructed that combines aerosol absorption and scattering with a line-by-line analysis of CO2 and H2O in a multilayer radiative transfer program. Aerosol composition previously inferred from the NASA Lear Jet Observatory data was used to measure the optical complex indices of refraction of appropriate Martian analogs from 0.4 to 2.5 microns. The aerosol vertical particle density scale was deduced using the Viking camera observations of the soil and sky intensities between 0.4 and 1.0 microns in comparison with those modeled using a multilayer Mie scattering program. A comparison of observed Mars atmospheric absorptions was made with those obtained using Lorentz, Voigt, and Doppler line profiles in a multilayer model of the CO2 and H2O. The Voigt line profile of CO2 absorption at approximately 4976 kaysers was then combined in a multilayer aerosol model of the Martian atmosphere. An evaluation of the effect on the line shape was made using several aerosol loadings.

Egan, W. G.↗

Particle sizing by weighted measurements of scattered light

A description is given of a measurement method, applicable to a poly-dispersion of particles, in which the intensity of scattered light at any angle is weighted by a factor proportional to that angle. Determination is then made of four angles at which the weighted intensity is four fractions of the maximum intensity. These yield four characteristic diameters, i.e., the diameters of the volume/area mean (D sub 32 the Sauter mean) and the volume/diameter mean (D sub 31); the diameters at cumulative volume fractions of 0.5 (D sub v0.5 the volume median) and 0.75 (D sub v0.75). They also yield the volume dispersion of diameters. Mie scattering computations show that an average diameter less than three micrometers cannot be accurately measured. The results are relatively insensitive to extraneous background light and to the nature of the diameter distribution. Also described is an experimental method of verifying the conclusions by using two microscopic slides coated with polystyrene microspheres to simulate the particles and the background.

Buchele, Donald R.↗

Administrative Report on Training Awards

During the tenure of this award, the recipient (David Harker) conducted areas of research which resulted in the award of a doctorate degree (August 1999) from the University of Wyoming. The primary science activity was investigation of silicate dust mineralogy in comets, particularly comet C/1995 O1 (Hale-Bopp). Determination of the dust mineralogy permits us to address an important astrophysical question of relevance to the origins and evolution of solar systems, "Do comets contain relic interstellar dust grains? Since, comets represent the frozen reservoirs of primitive proto-solar dust and ice, we can gain insight into the problem of understanding the formation of protoplanetesimals in the. early solar nebula. Mid-infrared spectrophotometry (7 - 14 micron, R approx. = 180 - 360) of Hale-Bopp was obtained with the NASA/Ames HIFOGS at four distinct epochs pre- and post- perihelion ion from 1996 October through 1997 June. These observations were conducted at the Wyoming Infrared Observatory and the NASA Infrared Telescope Facility, and were supported by funds from this training grant. The emission at mid-IR wavelengths in cometary comae arises from carbon grains, and small silicate grains which produce resonance features. Hale-Bopp had the strongest silicate feature observed from any comet to date. Theoretical calculations utilizing Mie Scattering Theory were employed to construct Synthetic cometary spectra to fit with the observed HIFOGS 10 microns spectral feature of Hale-Bopp. Our analysis suggests that the observed spectra can be modeled with the Hanner grain size distribution peaked at alpha((sub p) = 0.2 microns of fractal porous grains with porosity parameter D = 2.5. This model spectrum also fits photometry points in the 3 - 5 microns region. Comparison with the ISO SWS spectrum of Hale-Bopp obtained 1996 October reveals that the crystalline olivine grains must be at it temperature hotter than computed from Mie theory.

Woodward, Charles E.↗

Subcentimeter-size particle distribution functions in planetary rings from Voyager radio and photopolarimeter occultation data

Analysis of measurements of the scattered and direct components of Voyager 1 radio occultation signals at 3.5 and 13 cm wavelengths yield estimates of the distribution functions of supracentimeter-size particles and thickness of relatively broad regions in Saturn's rings. If mearurements of signal amplitude at a shorter wavelength are combined with the previously analyzed data, the shape of the distribution functions characterizing the smaller particles can be constrained. If size distributions of arbitrary form were considered, many solutions are found that are consistent with the three available observations of signal amplitude. The best-fit power law was calculated to the three observations at three wavelengths for several of the embedded Saturn ringlets. Mie scattering theory predicts that the measured phase of the radio occultation signal is highly sensitive to particles ranging from 0.1 to 1.0 wavelengths in size, thus additional constraints on the subcentimeter-size distribution functions for both the Saturn and Uranus rings can in principle be derived from radio phase measurements.

Zebker, Howard A.↗

The clouds of Venus - An anisotropic scattering model

The phase function for anisotropic scattering is applied to a homogeneous atmospheric model to ascertain the effects of anisotropy on the near-infrared spectrum of Venus. Young's (1971) equivalent widths for the 7820-A CO2 band are analyzed to derive allowed combinations of CO2 specific abundance, continuum albedo, pressure, and degree of anisotropy. From these combinations, values are derived for the photon mean free path and total optical thickness of the clouds. The Venera 10 measurement of the transmitted flux at 7200 A is then used in conjunction with spherical-albedo requirements to reduce the range of possible solutions to the equivalent-width analysis. Through the application of approximate similarity relations, the 'true' (i.e., anisotropic) atmospheric parameters are derived from the isotropic values. For an assumed Mie scatterer with an average anisotropy factor of 0.7, the results indicate a total optical thickness of about 55 with a single-scattering albedo of 0.9992 to 0.9995.

Lestrade, J. P.↗

Optical and Probe Diagnostics Applied to Reacting Flows

We plan to explore three major threads during the fellowship period. The first interrogates the flame synthesis of carbon nanotubes using aerosol catalysts. Laser light scattering will reveal changes in particle size at various heights above the burner. Analysis of the flame gas by mass spectroscopy will reveal the chemical composition of the mixture. Finally, absorption measurements will map the nanotube concentration within the flow. The second thread explores soot oxidation kinetics. Cavity ring-down absorption measurements of the carbonaceous aerosol can provide a measure of the mass concentration with time and, hence, an oxidation rate. Spectroscopic and direct probe measurements will provide the temperature of the system needed for subsequent modeling. The third thread will explore the details of turbulent flame dynamics. Laser induced incandescence will be applied to measurements of soot volume fraction in a 2-d configuration. Analysis of seed tracer particles by planar laser light MIE scattering will reveal the elemental fuel mixture fraction in the flames. Cavity ring-down spectroscopy, a pulsed transient absorption method, will determine the instantaneous mass loading and its fluctuation. Finally, fluorescence measurements will investigate the formation of PAH's in these flames.

Ticich, Thomas M.↗