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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 127 records · Page 7

The polar ionosphere as a source of the storm time ring current

The transport of ions from the polar ionosphere to the inner magnetosphere during storm time conditions has been computed using a Monte Carlo diffusion code. The effect of the electrostatic turbulence assumed to be present during the substorm expansion phase was simulated by a process that accelerated the ions stochastically perpendicular to the magnetic field with a diffusion coefficient proportional to the rate of energization of the ions by the induced electric field. This diffusion process was continued as the ions were convected from the plasma sheet boundary layer to the double-spiral injection boundary. Inward of the injection boundary the ions were convected adiabatically. By using as input an O(+) flux of 2.8 x 10 to the 8th per sq cm per s (w greater than 10 eV) and an H(+) flux of 5.5 x 10 to the 8th per sq cm per s (w greater than .63 eV) the computed distribution functions of the ions in the ring current were found to be in good agreement, over a wide range in L (4-8), with measurements made with the ISEE 1 satellite during a storm. This O(+) flux and a large part of the H(+) flux appear to be consistent with the DE-1 and DE-2 satellite measurements of the polar ionospheric outflow during disturbed times.

Cladis, J. B.↗

Structural origin of recovered ferroelectricity in BaTi O 3 nanoparticles

Nanoscale BaTiO 3 particles (≈10 nm) prepared by ball-milling a mixture of oleic acid and heptane have been reported to have an electric polarization several times larger than that for bulk BaTiO 3 . In this work, detailed local, intermediate, and long-range structural studies are combined with spectroscopic measurements to develop a model structure of these materials. The X-ray spectroscopic measurements reveal large Ti off-centering as the key factor producing the large spontaneous polarization in the nanoparticles. Temperature-dependent lattice parameter changes reveal the sharpening of the structural phase transitions in these BaTiO 3 nanoparticles compared to the pure nanoparticle systems. In conclusion, sharp crystalline-type peaks in the barium oleate Raman spectra suggest that this component in the composite core-shell matrix, a product of mechanochemical synthesis, stabilizes an enhanced polar structural phase of the BaTiO 3 core nanoparticles.

36 MATERIALS SCIENCE↗

Creating Near Real-time Hourly VIIRS Radiance Mosaic over Polar Regions from SatCORPS Global Cloud Composite (GCC)

While polar orbiting satellites are essential in providing the needed observations over polar regions for data assimilation, weather diagnoses/forecasting, and flight guidance and situation awareness in airborne field campaigns, there is limited temporal coverage. Often, polar mosaics are created by overlaying multiple satellite imagers on top of each other which can lead to transition lines and discontinuities in the data products. To help ease some of these shortcomings, we utilize the NASA Langley Satellite ClOud and Radiation Property retrieval System (SatCORPS) Mosaic algorithm for optimally fusing and merging selected imager radiances from the Visible Infrared Imaging Radiometer Suite (VIIRS) instrument onboard the Suomi National polar-orbiting Partnership (SNPP), Joint Polar Satellite System (JPSS-1), and JPSS-2 satellites, and the MODerate resolution Imaging Spectroradiometer (MODIS) instruments onboard AQUA and TERRA satellites. Since multiple satellites overpasses and instruments are used in creating hourly 3-km composites over the polar regions, selection of the best satellite data for each 3-km composite pixel is based on aggregated ranking of satellite resolution, time, viewing zenith angle, and distance from terminator. This ranking system provides a smoother transition and improves data discontinuity in the merged output resulting in a more seamless polar region dataset. We will discuss the use of this near real-time dataset to support polar airborne field campaigns and SatCORPS satellite-derived Global Cloud Composite (GCC) generation.

Satellite composites↗

Sub-Daily Polar Motion During Epoch '92 with GPS

Data from a worldwide Global Positioning System (GPS) tracking network spanning six days during the EPOCH '92 campaign are used to estimate variations of the Earth's pole position every 30 minutes. The resulting polar motion time series is compared with estimates derived from very long baseline interferometry (VLBI) observations.

Global Positioning System (GPS) VLBI polar motion↗

X-ray polarimetry

The method by which the Bragg-crystal X-ray polarimeters aboard Ariel 5 and OSO 8 operate is briefly described, and some results obtained with these instruments for six Galactic X-ray sources are summarized. A precision measurement of the linear polarization in the Crab Nebula at energies of 2.6 and 5.2 keV is presented. Evidence is given for polarization in Sco X-1, Cyg X-2, Cen X-3, and the X-ray transient A0620-00. The determined or estimated polarizations are approximately 19.2% at 2.6 keV and 19.5% at 5.2 keV for the Crab Nebula, 1.1% at 2.6 keV and 2.4% at 5.2 keV for Sco X-1, 2.5% at 2.6 keV and 9.8% at 5.2 keV for Cyg X-1, an upper limit of 13.5% for A0620-00, an upper limit of 13.5% to the time-averaged polarization of Cen X-3, and an apparent value of about 5% for Cyg X-2.

Long, K. S.↗

Prediction of Complex Observed Shear Wave Splitting Patterns at Ryukyu Subduction Zone Using a Strong Intra-Slab Anisotropy Model

Complex shear wave splitting (SWS) patterns in subduction zones are often interpreted geodynamically as resulting from complex mantle flow; however, this may not always be necessary. We analyzed 7,093 high-quality SWS measurements from teleseismic S waves recorded by Hi-net stations across the Ryukyu arc in Japan. Our findings show a systematic rotation of the fast S polarization from trench-parallel to trench-perpendicular depending on the earthquake backazimuth. For the same earthquake, the measured splitting patterns also vary spatially across the southwest Japan. Using full-wave seismic modeling, we showed that a dipping slab with ~30% shear anisotropy of the tilted transverse isotropy (TTI) type, with a symmetry axis perpendicular to the slab interface, can predict the observed delay times and polarization rotation. Our results highlight the importance of considering dipping anisotropic slabs in interpreting SWS at subduction zones.

58 GEOSCIENCES↗

Initial Response and Complex Polar Cap Structures of the Aurora in Response to the January 10, 1997 Magnetic Cloud

On January 10, 1997, a magnetic cloud originating at the Sun was incident on the Earth. The initial disturbance to the magnetosphere, as reflected in the activities of the aurora, was measured by the Ultraviolet Imager on the Polar Spacecraft. During this event we have observed the development of several unusual unique auroral forms that to our knowledge are unexplained in current models and theories. The observations were made on a global scale with unprecedented spatial and temporal resolution. The first activation of the aurora at local noon occurred within minutes of the arrival of the shock at 0107 UT. The substorm onset was observed at 0334 UT. During the intervening time significant polar cap precipitation occurred.

Spann, J. F.↗

Measurement of the J / ψ Polarization with Respect to the Event Plane in Pb-Pb Collisions at the LHC

We study the polarization of inclusive J/ψ produced in Pb-Pb collisions at $\sqrt{^sNN}$ = 5.02 TeV at the LHC in the dimuon channel, via the measurement of the angular distribution of its decay products. We perform the study in the rapidity region 2.5 < y < 4, for three transverse momentum intervals (2 < p T < 4, 4 < p T < 6, 6 < p T < 10 GeV/c) and as a function of the centrality of the collision for 2 < p T < 6 GeV/c. For the first time, the polarization is measured with respect to the event plane of the collision, by considering the angle between the positive-charge decay muon in the J/ψ rest frame and the axis perpendicular to the event-plane vector in the laboratory system. A small transverse polarization is measured, with a significance reaching 3.9σ at low p T and for intermediate centrality values. The polarization could be connected with the behavior of the quark-gluon plasma, formed in Pb-Pb collisions, as a rotating fluid with large vorticity, as well as with the existence of a strong magnetic field in the early stage of its formation.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Initial Response of the Aurora to the January 10, 1997 Magnetic Cloud

On January 10th, 1997, a magnetic cloud originating at the Sun was incident on the Earth. The initial disturbance to the magnetosphere, as reflected in the intensification of the aurora, was measured by the Ultraviolet Imager on the Polar Spacecraft. The first activation of the aurora at local noon occurred within minutes of the arrival of the shock. The subsequent evolution of the aurora over the next 18 minutes shows that the magnetic disturbance proceeds from local noon, symmetrically around the dawn and dusk flanks to local midnight. The substorm onset was observed to occur 174 minutes after the initial brightening of the aurora and 78 minutes after the southward turning of the IMF (Interplanetary Magnetic Field). During the intervening time, significant polar cap precipitation is observed. The polar cap precipitation begins at the poleward edge of the oval in the post midnight region and develops to form several complex transpolar structures. The polar cap precipitation subsides and quiet conditions are observed for 40 minutes prior to the onset of the substorm. During this event we have observed several unusual unique auroral forms develop that are different from the standard substorm models. We will present interpretation of the development of the pre-substorm events in light of the interplanetary conditions.

Spann, James F., Jr.↗

Interplanetary magnetic field polarity and the size of low-pressure troughs near 180 deg W longitude

The relationship between interplanetary magnetic field polarity and the area of low pressure (300 mbar) troughs near 180 deg W longitude is examined. For most of the winters from 1951 to 1973, the trough size, as indicated by the vorticity area index, is found to be significantly greater when the interplanetary magnetic field is directed away from the sun than when the field is directed towards the sun. This relationship is shown to hold for various combinations of winters and for most months within a winter, and be most pronounced at the time when polarity was determined. It is suggested that the phenomenon is caused by merging of interplanetary magnetic field lines, when polarity is directed away from the sun, with geomagnetic field lines in the Northern Hemisphere (where these measurements were made), allowing energetic particle fluxes to have access to the north polar region

Wilcox, J. M.↗

Polar motion and length of day determination from satellite laser ranging

The kinematic and dynamic models used in obtaining the GSFC MERIT solution (using data from satellite laser ranging) for the x and y coordinates of the earth's rotation pole and the excess length-of-day (LOD) are discussed together with the analysis technique. Comparisons of the GSFC polar motion time series with the time series from the Bureau International de l'Heure shows small but consistent systematic differences (4.6 milliarcsec rms about a mean offset of 1 milliarcsec in the x component, and 2.9 milliarcsec rms about a 21 milliarcsec offset in the y component). A comparison with the data of the National Geodetic Survey's IRIS network shows departures of 2.5 milliarcsec rms about the mean for the x component and 2.0 milliarcsec rms for the y component. The precision of the GSFC earth orientation is estimated to be better than 1 milliarcsec for polar motion and 0.1 msec for excess LOD.

Smith, David E.↗

Multimodality in the Search for New Physics in Pulsar Timing Data and the Case of Kination-amplified Gravitational-wave Background from Inflation

We investigate the kination-amplified inflationary gravitational-wave background (GWB) interpretation of the signal recently reported by various pulsar timing array (PTA) experiments. Kination is a post-inflationary phase in the expansion history dominated by the kinetic energy of some scalar field, characterized by a stiff equation of state w = 1. Within the inflationary GWB model, we identify two modes that can fit the current data sets (NANOGrav and EPTA) with equal likelihood: the kination-amplification (KA) mode and the ordinary, no-kination-amplification (no-KA) mode. The multimodality of the likelihood motivates a Bayesian analysis with nested sampling. We analyze the free spectra of current PTA data and mock free spectra constructed with higher signal-to-noise ratios using nested sampling. The analysis of the mock spectrum designed to be consistent with the best fit to the NANOGrav 15 yr (NG15) data successfully reveals the expected bimodal posterior for the first time while excluding the reheating mode that appears in the fit to the current NG15 data, making a case for our correct and comprehensive treatment of potential multimodal posteriors arising from future PTA data sets. The resultant Bayes factor is $\mathcal{B}$ $\equiv$ Z no–KA /Z KA = 2.9 ± 1.9, indicating comparable statistical significance between the two modes. Given the theoretical model-building challenges of producing highly blue-tilted primordial tensor spectra, the KA mode has the advantage of requiring less blue primordial spectra, compared with the no-KA mode. The synergy between future cosmic microwave background polarization, pulsar timing, and laser interferometer measurements of gravitational waves will help resolve the ambiguity implied by the multimodal posterior in PTA-only searches.

Cosmology↗

On Geomagnetism and Paleomagnetism

A statistical description of Earth's broad scale, core-source magnetic field has been developed and tested. The description features an expected, or mean, spatial magnetic power spectrum that is neither "flat" nor "while" at any depth, but is akin to spectra advanced by Stevenson and McLeod. This multipole spectrum describes the magnetic energy range; it is not steep enough for Gubbins' magnetic dissipation range. Natural variations of core multipole powers about their mean values are to be expected over geologic time and are described via trial probability distribution functions that neither require nor prohibit magnetic isotropy. The description is thus applicable to core-source dipole and low degree non-dipole fields despite axial dipole anisotropy. The description is combined with main field models of modem satellite and surface geomagnetic measurements to make testable predictions of: (1) the radius of Earth's core, (2) mean paleomagnetic field intensity, and (3) the mean rates and durations of both dipole power excursions and durable axial dipole reversals. The predicted core radius is 0.7% above the 3480 km seismologic value. The predicted root mean square paleointensity (35.6 mu T) and mean Virtual Axial Dipole Moment (about 6.2 lx 1022 Am(exp 2)) are within the range of various mean paleointensity estimates. The predicted mean rate of dipole power excursions, as defined by an absolute dipole moment <20% of the 1980 value, is 9.04/Myr and 14% less than obtained by analysis of a 4 Myr paleointensity record. The predicted mean rate of durable axial dipole reversals (2.26/Myr) is 2.3% more than established by the polarity time-scale for the past 84 Myr. The predicted mean duration of axial dipole reversals (5533 yr) is indistinguishable from an observational value. The accuracy of these predictions demonstrates the power and utility of the description, which is thought to merit further development and testing. It is suggested that strong stable stratification of Earth's uppermost outer core leads to a geologically long interval of no dipole reversals and a very nearly axisymmetric field outside the core. Statistical descriptions of other planetary magnetic fields are outlined.

Voorhies, Coerte V.↗

Ultrafast X-ray Absorption Spectroscopy Reveals Excited-State Dynamics of B 12 Coenzymes Controlled by the Axial Base

Polarized time-resolved X-ray absorption spectroscopy at the Co K-edge is used to probe the excited-state dynamics and photolysis of base-off methylcobalamin and the excited-state structure of base-off adenosylcobalamin. For both molecules, the final excited-state minimum shows evidence for an expansion of the cavity around the Co ion by ca. 0.04 to 0.05 Å. The 5-coordinate base-off cob(II)alamin that is formed following photodissociation has a structure similar to that of the 5-coordinate base-on cob(II)alamin, with a ring expansion of 0.03 to 0.04 Å and a contraction of the lower axial bond length relative to that in the 6-coordinate ground state. Here these data provide insights into the role of the lower axial ligand in modulating the reactivity of B 12 coenzymes.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Ultrafast photoinduced band splitting and carrier dynamics in chiral tellurium nanosheets

Trigonal tellurium (Te) is a chiral semiconductor that lacks both mirror and inversion symmetries, resulting in complex band structures with Weyl crossings and unique spin textures. Detailed time-resolved polarized reflectance spectroscopy is used to investigate its band structure and carrier dynamics. The polarized transient spectra reveal optical transitions between the uppermost spin-split H4 and H5 and the degenerate H6 valence bands (VB) and the lowest degenerate H6 conduction band (CB) as well as a higher energy transition at the Lpoint. Surprisingly, the degeneracy of the H6 CB (a proposed Weyl node) is lifted and the spin-split VB gap is reduced upon photoexcitation before relaxing to equilibrium as the carriers decay. Using ab initio density functional theory (DFT) calculations, we conclude that the dynamic band structure is caused by a photoinduced shear strain in the Te film that breaks the screw symmetry of the crystal. The band-edge anisotropy is also reflected in the hot carrier decay rate, which is a factor of two slower along the c-axis than perpendicular to it. The majority of photoexcited carriers near the band-edge are seen to recombine within 30 ps while higher lying transitions observed near 1.2 eV appear to have substantially longer lifetimes, potentially due to contributions of intervalley processes in the recombination rate. These new findings shed light on the strong correlation between photoinduced carriers and electronic structure in anisotropic crystals, which opens a potential pathway for designing novel Te-based devices that take advantage of the topological structures as well as strong spin-related properties.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Improving protonic ceramic electrochemical cell performance via a dual-phase reaction-sintered bilayer electrolyte

Protonic ceramic electrochemical cells (PCCs) are promising energy conversion devices, but their fabrication remains challenging. In particular, the typical electrolytes for PCCs such as BaCe 0.7 Zr 0.1 Y 0.1 Yb 0.1 O 3−δ (7111) and BaCe 0.4 Zr 0.4 Y 0.1 Yb 0.1 O 3−δ (4411) suffer from intrinsic barium evaporation issues during high-temperature sintering. This tendency towards barium loss, combined with their highly refractory nature, leads to a tradeoff between sinterability and chemical stability. To address this tradeoff, we propose a bilayer electrolyte combining layers of 4411 and 7111 materials that is designed to enhance sinterability and conductivity through dual-phase reactive sintering. Our findings demonstrate that the bilayer structure exhibits shrinkage behavior closely matched to that of the fuel electrode substrate, with a higher shrinkage compared to a single-layer 4411 electrolyte. Utilizing this bilayer electrolyte structure, our PCCs achieve a peak power density of 637 mW∙cm −2 in fuel-cell mode and a current density of 1060 mA∙cm −2 at 1.3 V in electrolysis mode at 600 °C. Our PCCs demonstrate high Faradaic efficiency of 83% at 1.3 V and 500 °C. Hybrid distribution of relaxation times (DRT) polarization mapping further reveals that the bilayer structure reduces Ohmic and polarization resistance in both fuel-cell and electrolysis modes.

ceramic processing↗

Direct visualization of electromagnetic wave dynamics by laser-free ultrafast electron microscopy

Integrating femtosecond lasers with electron microscopies has enabled direct imaging of transient structures and morphologies of materials in real time and space. Here, we report the development of a laser-free ultrafast electron microscopy (UEM) offering the same capability but without requiring femtosecond lasers and intricate instrumental modifications. We create picosecond electron pulses for probing dynamic events by chopping a continuous beam with a radio frequency (RF)–driven pulser with the pulse repetition rate tunable from 100 MHz to 12 GHz. As a first application, we studied gigahertz electromagnetic wave propagation dynamics in an interdigitated comb structure. We reveal, on nanometer space and picosecond time scales, the transient oscillating electromagnetic field around the tines of the combs with time-resolved polarization, amplitude, and local field enhancement. This study demonstrates the feasibility of laser-free UEM in real-space visualization of dynamics for many research fields, especially the electrodynamics in devices associated with information processing technology.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Ultrafast Inverse Chirality-Induced Spin Selectivity Observed by THz Emission

Chirality-induced spin selectivity (CISS) phenomena arise from an interplay among structural chirality, electron spin orientation, and charge current. Steady-state observations such as magnetoresistance offer little insight into the timescales that govern the spin-charge interconversion and often conflate interfacial and bulk phenomena. By contrast, inverse CISS involves the conversion of spin to a charge current. Using terahertz (THz) emission spectroscopy, we directly measured an ultrafast charge current due to inverse CISS with picosecond time resolution. Polarity and polarization analysis of the THz emission map the induced charge current direction upon spin injection. We found that a charge current is generated along the spin orientation that changes direction with stereochemical configuration. These observations directly demonstrate the inherent coupling between spin and charge currents in chiral systems, offering key insights into their fundamental dynamics.

74 ATOMIC AND MOLECULAR PHYSICS↗