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At least 127 records · Page 7

Multi-Probe FY25 Omega EP Shot Request [Slides]

The goal of the Multi-Probe experimental campaign is to assess the feasibility of using multiple probe types (x ray, proton, neutron, and electron) in future LANL radiographic facilities. X-ray and proton platforms have been demonstrated. The first attempts at simultaneous radiography were hampered by cross talk, which was the subject of FY23 & FY24 experiments. The major goal for FY25 is to demonstrate simultaneous radiography of both static and dynamic objects.

36 MATERIALS SCIENCE↗

Probing and Understanding the Spatial and Energy Distributions of Plasmonic Hot Carriers via Single-Molecule Quantum Transport

The generation of hot carriers in plasmonic nanostructures offers new transformative opportunities for a range of applications, including solar energy harvesting, photochemistry, and photodetection. To better understand such phenomena, this project aims to develop an experimental approach to study and understand hot carrier distributions in photoexcited plasmonic nanostructures. The developed experimental approach, combining scanning probe-based single-molecule quantum transport measurements with plasmonic excitation methods, leverages nanoscopic single molecules as quantum energy filters to selectively access hot carriers in a variety of plasmonic nanostructures. This report summarizes the key outcomes, impacts, and lessons learned in the first two years of the project. Over the past two years, important progress was made in achieving the project's goals, including the development of the scanning probe-based experimental platform, fabrication of plasmonic nanostructures, and design and synthesis of the desired molecular candidates. Insights from this research will pave the path toward the development of technologies that will improve the way we harvest solar energy and drive chemical reactions and ultimately help transition the U.S. to a clean and sustainable society.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Multi-Probe Radiography: For 2035 and Beyond

The Multi-Probe Radiography Project is investigating the use of multiple species of probe beams to provide more information from a radiography. Contextual radiographic, source, and measurements information is being provided through a series of four workshops at Los Alamos National Laboratory. The third workshop on Accelerator and Pulsed Power Technology is summarized in this report. The state of the large NNSA facilities such as Scorpius, DARHT, pRad, and Cygnus are presented. Future enhancements and innovative upgrades are also discussed.

43 PARTICLE ACCELERATORS↗

Addressing Experimental Challenges in Probing Dark Energy with Accuracy and Precision with the Rubin Observatory Legacy Survey of Space & Time (LSST)

With support from this award, the Stanford group under the leadership of PI Patricia Burchat focused on pixel-level algorithms that are key to the investigation of dark energy with the Vera C. Rubin Observatory Legacy Survey of Space and Time (LSST). The work was carried out through strong engagement in the DOE-supported LSST Dark Energy Science Collaboration (DESC), for which the PI served as Deputy Spokesperson (07/2019 - 07/2021) and Technical Coordinator (07/2021 - 07/2023). Members of the Burchat group are Full DESC members and are among scientists who have been accepted to join the Rubin Observatory System Integration, Test, and Commissioning (SIT-Com) effort. The specific intellectual focus of the group was the optimization of gravitational lensing as a probe of the evolution of the distribution of dark matter in space and time to learn about the nature of dark energy. The Stanford group pursued an integrated research program to understand in detail, and then remediate or calibrate, systematic effects that could limit the sensitivity of the LSST to cosmic shear as a dark energy probe -- particularly those related to our understanding of the atmospheric point spread function (PSF), challenges associated with blended galaxy images, and impacts of residual camera artifacts. Key to this work was developing, enhancing, and validating the fidelity of simulations that play a key role in the development of our understanding of subtle systematic biases and then using these simulations to develop techniques to characterize and mitigate biases, and associated algorithms for implementation in the LSST or DESC science pipelines. The group’s work included contributions to the open-source GalSim simulation package, which is widely used in the community; simulations and studies of spatial correlations of atmospheric PSFs; studies of temporal correlations of the atmospheric PSF; impacts of chromatic PSFs on cosmic shear calibration; continued studies of anisotropic Gaussian process interpolation of PSF models across the focal plane; and measuring and mitigating impacts of residual camera artifacts on cosmic shear. A primary impact of this work is that it increases the scientific discovery potential of the DOE and NSF investments in the Rubin Observatory Legacy Survey of Space \& Time, by addressing challenges in interpreting astronomical images through more accurate descriptions of the blurring of images due to the atmosphere. Specifically, this work impacts our ability to understand the fundamental nature of dark energy.

Burchat, Patricia Rose↗

Development of Operando Atom Probe to study field-assisted surface chemistry

Recent efforts at PNNL have led to the development of in-situ Atom Probe Tomography (ISAPT) and Operando Atom Probe (OAP), establishing PNNL as a key player in this technology, both in the U.S. and globally. OAP has already pushed the initial limits of APT, which was traditionally used at cryo temperatures (<60 K) and ultra-high vacuum (<10⁻¹² bar), to operate in the presence of reactive gases (up to 10⁻¹⁰ bar) at a maximum temperature of 300 K. Using OAP, we successfully observed Co and Fe oxidation in real-time at the nanoscale, revealing the importance of surface structures in these interactions. Additionally, OAP opens the possibility to explore the influence of local electric fields (EFs) on surface chemistry and hydrogen interactions at the nanoscale.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Calibrator for Airborne Aerosol Probes (CAAP) Field Campaign Report

In this campaign, Calibrator for Airborne Aerosol Probes (CAAP), Mesa Photonics provided its U.S. Department of Energy (DOE) Small Business Innovation Research (SBIR) Phase II prototype of a portable, battery-powered monodisperse aerosol/droplet generator to field-calibrate two aerosol/cloud characterization instruments deployed on the DOE Atmospheric Radiation Measurement (ARM) Aerial Facility (AAF) ArcticShark uncrewed aerial system (UAS) during the flight campaign conducted at ARM’s Southern Great Plains (SGP) atmospheric observatory and the Blackwell-Tonkawa airfield (Oklahoma) in May 2024. The CAAP campaign (May 20-24, 2024) partially overlapped with the main ARM AAF campaign, Turbulent Layers Promoting New Particle Formation (NPFTURBULENCE, May 7-27, 2024, Gannet Hallar, principal investigator). The main goal of the CAAP campaign was field validation of calibration of aerosol and cloud probes deployed on the ArcticShark UAS. The campaign also provided an opportunity to test and evaluate the Mesa Photonics’ monodisperse aerosol/droplet generator prototype in the field, under real-life operational conditions.

54 ENVIRONMENTAL SCIENCES↗

Project FELICIA - A probe to survey the RHIC magnet beampipe diameter for EIC beam screen insertion

The Electron Ion Collider (EIC) Hadron Storage Ring (HSR) will reuse many of the existing superconducting (SC) magnets of the RHIC storage rings. To comply with the beamline vacuum requirements in more demanding operational scenarios, the beampipe of the RHIC SC magnets will be equipped with low surface impedance, low secondary electron yield (SEY) beam screens. The installation of these beam screens will be done with the SC magnets as installed today, thus making it a critical operation for a timely EIC installation. The beam screen inner dimensions must be maximized to retain enough aperture to the beam. On the other hand, keeping enough clearance between the screen and the beampipe is critical to ensure a smooth beam screen installation. A survey probe was designed and built to measure the inner diameter of several RHIC SC magnets in-situ and provide critical data for the beam screen design optimization. This paper reports on the design of the probe and the results from the survey campaign.

43 PARTICLE ACCELERATORS↗

Probing BSM Oscillatory Signals with the DUNE Detectors and the LBNF Neutrino Beam: NSI and Sterile Neutrino Sensitivities

The Deep Underground Neutrino Experiment (DUNE) is a flagship long-baseline accelerator neutrino experiment under construction in the U.S. With a 1,300 km distance between its Near Detector (ND) and Far Detector (FD), the world’s most intense LBNF (Long-Baseline Neutrino Facility) neutrino beam, and high-resolution LArTPC (Liquid Argon Time Projection Chamber) detectors, DUNE will measure the neutrino oscillation parameters with unprecedented precision. In addition to the determination of the neutrino mass ordering and the potential discovery of Charge-Parity violation in the leptonic sector, DUNE's capabilities present a unique opportunity for probing Beyond the Standard Model (BSM) physics signals with neutrinos. Examples of BSM physics manifestations include the presence of Non-Standard Interactions (NSI) of neutrinos with matter, or the existence of sterile neutrinos that mix with 3-Flavor neutrinos. In this study, we present a joint ND+FD fit to simulated data assessing DUNE's sensitivity to probing neutrino NSI, as well as scenarios including sterile neutrino mixing.

Prais, Luiz [Cincinnati U.] (ORCID:000000018224947↗

Tau-Jet Matching and Tag-and-Probe Tau Tagging Efficiencies for HH→bbτ+τ− Searches Using Run 3 CMS Scouting Data

We are studying tau-jet matching efficiency and tau tagging efficiency for the search for Higgs boson pair production in the HH→bbτ+τ− decay channel using Run 3 CMS scouting data. Collision events in the CMS detector produce many particle candidates, so jets are clustered using the anti-kT algorithm to identify possible tau signatures. In Monte Carlo simulation, tau-jet matching efficiency can be measured by comparing generated taus to reconstructed jets. In actual collision data, however, generated taus are not available, so we use a tag-and-probe method with Z→τ+τ− candidate events. In this method, one tau candidate is used as the tag and the other as the probe. The invariant mass of the tau-pair candidates is plotted and fitted with signal and background functions to estimate the number of real tau events and determine the tagging efficiency. By comparing efficiencies in data and Monte Carlo simulation, this work helps evaluate the performance of scouting-based tau reconstruction and tau tagging for future HH→bbτ+τ− searches.

Bellot, Annella [North Central Coll.; Fermilab]↗

Tau-Jet Matching and Tag-and-Probe Tau Tagging Efficiencies for HH→bbτ+τ− Searches Using Run 3 CMS Scouting Data

We are studying tau-jet matching efficiency and tau tagging efficiency for the search for Higgs boson pair production in the HH→bbτ+τ− decay channel using Run 3 CMS scouting data. Collision events in the CMS detector produce many particle candidates, so jets are clustered using the anti-kT algorithm to identify possible tau signatures. In Monte Carlo simulation, tau-jet matching efficiency can be measured by comparing generated taus to reconstructed jets. In actual collision data, however, generated taus are not available, so we use a tag-and-probe method with Z→τ+τ− candidate events. In this method, one tau candidate is used as the tag and the other as the probe. The invariant mass of the tau-pair candidates is plotted and fitted with signal and background functions to estimate the number of real tau events and determine the tagging efficiency. By comparing efficiencies in data and Monte Carlo simulation, this work helps evaluate the performance of scouting-based tau reconstruction and tau tagging for future HH→bbτ+τ− searches.

Bellot, Annella [North Central Coll.; Fermilab]↗

Spinning Hall Probe magnetic compass

In a large range of physics and space experiments, the direction of the magnetic field needs to be determined with an accuracy on the level of one milli radian or better. We have proposed a new type of magnetic compass - a rotation-based one, which provides an alternating signal from the Hall probe proportional to the value of the magnetic field transverse to the axis of rotation. The spinning Hall probe device has been realized. Alignment of the spinning axis for a minimum (zero) value of the signal allows us to find the direction of the magnetic field. The device does not require calibration and is free of any drift problems. The measurement of the rotation axis direction was accomplished by means of a laser and a flat mirror attached to the rotor. The constructed prototype achieved an accuracy for the magnetic field direction in the experiment with the polarized He-3 target on the level of one milli radian.

Wojtsekhowski, Bogdan↗

Probing gluon saturation and nuclear structure in photon-nucleus collisions

We calculate exclusive vector meson photoproduction within the Color Glass Condensate framework in high-energy photon-nucleus scattering probed experimentally in ultra peripheral heavy ion collisions at RHIC and at the LHC. When the free parameters are constrained by the γ + p data from HERA, we predict significant nuclear suppression for both the coherent and incoherent photoproduction cross section in the TeV range. Our results indicate that the LHC data prefers even stronger saturation effects at the highest collision energies. Furthermore, we demonstrate how the linear polarization of photons in ulra peripheral collisions generates azimuthal modulations in the decay products of the exclusively produced vector meson. We show how these measurements can probe details of the nuclear geometry, specifically the deformed structure of the uranium nuclei.

Mäntysaari, Heikki [University of Jyväskylä (Finla↗

Probing Physics beyond the Standard Model through Combined Analyses of Next-generation Type Ia Supernova, Cosmic Microwave Background, and Baryon Acoustic Oscillation Surveys

Observations of Type Ia supernovae (SNe Ia), which probe the late Universe, together with baryon acoustic oscillations (BAO) and the cosmic microwave background (CMB), which probe the intermediate and early epochs, provide complementary constraints on the expansion history of the Universe. In this work, we forecast constraints on dark energy and other extensions to the standard cosmological model by combining the SN Ia sample expected from the Vera C. Rubin Observatory’s Legacy Survey of Space and Time (LSST), data from current and forthcoming CMB surveys, and BAO measurements from the Dark Energy Spectroscopic Instrument (DESI). For the CMB, we use temperature, polarization, and lensing power spectra (TT/EE/TE/ϕϕ) from the South Pole Telescope, the planned Advanced Simons Observatory, and a CMB-S4–like experiment. We derive constraints on ΛCDM and its extensions involving the dark energy equation-of-state parameters (w 0 , w a ) and the sum of neutrino masses ∑m ν using a Markov Chain Monte Carlo (MCMC) sampling framework. We find that the LSST Year 3 SN Ia sample can improve upon the DES Year 5 dark energy constraints by a factor of 2−2.5×, with the gains driven primarily by the significantly higher SN Ia density in the LSST sample. Similarly, DESI-DR3 shows up to a 1.8× improvement on dark energy parameters over DR2, driven largely by the substantial increase in the low-redshift sample. Combining CMB with LSST-Y3-SN Ia and DESI-DR3-BAO yields σ(w 0 ) = 0.028 and σ(w a ) = 0.11 for w 0 w a CDM cosmology with the results being largely independent of the CMB dataset. The constraints weaken by 10%–30% when freeing ∑m ν and spatial curvature. Moreover, the joint analysis of the three datasets can enable a 2σ–3σ detection of ∑m ν .

Raghunathan, Srinivasan [University of California;↗

Computational Fluid Dynamics Modeling to Facilitate Qualification of Stack Sampling Probe Location

Computational fluid dynamics (CFD) modeling was used to help evaluate modifications to a radiological effluent stack and assist with establishing a stack sampling location that met the mixing criteria for qualification. Requirements for stack sampling location are listed in the American National Standards Institute/Health Physics Society (ANSI/HPS) N13.1-2021 standard. Modeling was performed to help develop a suitable design for increasing building ventilation for the radiological effluent stack. The ANSI/HPS N13.1-2021 criteria for the air monitoring probe location are that the coefficient of variation of velocity uniformity, gaseous tracer uniformity, and particulate tracer uniformity must be less than or equal to 20%. Furthermore, no point in the sampling location may have a gaseous tracer concentration that varies from the mean concentration by more than 30%. Additionally, the flow angle at the sampling location must not be more than 20 degrees. The ANSI/HPS N13.1-2021 standard allows for models (physical or computational) to be employed to perform the full suite of qualification tests, followed by a more limited set of verification tests on the actual stack to qualify the stack sampling location. Here, a series of computational model simulations were employed to evaluate the stack qualification criteria. Significant time and re-source savings are achieved using CFD modeling. CFD modeling demonstrated that the stack meets the criteria at the sample probe location. Verification tests were performed on the modified stack to measure the velocity uniformity and flow angle at the stack sampling location, and results demonstrated that the CFD model results may be used to support the qualification of the stack sampling location.

Air Monitoring↗

A new probe of μ Hz gravitational waves with FRB timing

We propose Fast Radio Burst (FRB) timing, which uses the precision measurements of the arrival time differences of repeated FRB signals along multiple sightlines, as a new probe of gravitational waves (GWs) around nHz to μ Hz frequencies, with the highest frequency limited by FRB repeating period. The anticipated experiment requires a sightline separation of tens of AU, achieved by sending radio telescopes to space. We find the signal of arrival time difference induced by GWs depends only on the local GWs in the solar system and we can correlate the measurements from different FRB sources or the same source with different repeaters, which leads to a better sensitivity with a larger number of FRB events detected. The projected sensitivity shows this method is a competitive probe in the nHz to μ Hz frequency range. It can fill the ‘ μ Hz gap’ between pulsar timing arrays and Laser Interferometer Space Antenna (LISA) and is complementary to other proposals of GW detection in this frequency band.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

Atom probe datasets from neutron irradiated Fe-Cr alloys

A series of model Fe–Cr alloys containing 3–18 at.% Cr was neutron irradiated at a nominal temperature of 563 K to 1.82 dpa. Solute distributions were analyzed by atom probe tomography, which revealed α′ precipitation for alloys containing more than 9 at.% Cr. Both the Cr concentration dependence of α′ precipitation and the measured matrix compositions are in agreement with the recently published Fe–Cr phase diagrams. An irradiation-accelerated precipitation process is strongly suggested. Irradiation was carried out in the Advance Test Reactor (ATR) at Idaho National Laboratory. A series of six Fe–Cr alloys of nominal compositions 3, 6, 9, 12, 15 and 18 at.% Cr was irradiated at a neutron fluence (E > 1 MeV) of 1.1 × 1021 n cm−2 at 563 ± 15 K and to a damage level of 1.82 displacements per atom (dpa). Nominal neutron flux and dpa rate are 2.3 × 1014 n cm−2 s−1 and 3.4 × 10−7 dpa s−1, respectively. The microstructures of the Fe–Cr alloys were studied by atom probe tomography (APT) using a Cameca 4000X HR instrument. APT specimens were prepared by a standard lift-out process using a Quanta 3D 200i dual beam scanning electron microscope ensuring that the analyses were performed away from grain boundaries.

Bachhav, Mukesh↗

Probing Signal-Based Inertia and Frequency Response Estimation for Power Systems with High Penetration of Inverter-Based Resources: Preprint

Power system inertia is the inherent capability of a power system to resist changes in its frequency during disturbances. Real-time inertia estimation technology has become more important due to the low-inertia issues caused by the increasing integration levels of inverter-based resources (IBRs) from renewable energy; however, existing inertia estimation methods hardly consider multiple frequency response controls that act within the same time frame as conventional inertial response, thus making measured inertia values vary under different testing conditions. To resolve this issue, this paper proposes a novel real-time estimation method to simultaneously estimate a power system's inertia constant and frequency response droop constant using a well-designed probing signal. First, we formulate the inertia and frequency response model of a power system with IBRs. Second, through the integration and manipulation of the developed model, we propose a multivariate linear regression- based estimation method that is resilient to measurement noise. Third, we design a probing signal that can be injected by IBRs to incite the required transients for estimation. Finally, we validate the proposed estimation method through comprehensive power- hardware-in-the-loop experiments using inverter hardware and a realistic island power system model. The results demonstrate that the proposed method can accurately estimate the inertia and droop value of the power system with grid-following IBRs and grid-forming IBRs with virtual synchronous machine control.

frequency response↗

Probing intergalactic intergalactic magnetic fields with LOFAR LoTSS DR2 data

We use Faraday rotation measurements from the latest catalog LoTSS DR2 from LOFAR to probe intergalactic magnetic fields. To identify the extragalactic component of the observed rotation measure (RM) we use two different techniques: residual rotation measure (RRM) and close radio pairs. For the RRM approach, we conclude that, despite smaller measurement errors in the LOFAR data, robust and conservative treatment of the systematic uncertainties in the Galactic contribution to RM results in the constraint on a homogeneous volume-filling magnetic field at the level 2.4 nG, slightly weaker than previous constraints from NVSS data, and does not allow to probe the presence of over-magnetized bubbles predicted by the AGN feedback model of the IllustrisTNG. Analyzing close radio pairs we found that in only 0.5% of our mock realizations of observed data, the expected contribution from the over-magnetized bubbles does not exceed LoTSS DR2 data.

79 ASTRONOMY AND ASTROPHYSICS↗