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DOE OSTI2022

On a Unified Core Characterization Methodology to Support the Systematic Assessment of Rare Earth Elements and Critical Minerals Bearing Unconventional Carbon Ores and Sedimentary Strata

A significant gap exists in our understanding and ability to predict the spatial occurrence and extent of rare earth elements (REE) and certain critical minerals (CM) in sedimentary strata. This is largely due to a lack of existing, systematic, and well-distributed REE and CM samples and analyses in United States sedimentary basins. In addition, the type of sampling and characterization performed to date has generally lacked the resolution and approach required to constrain geologic and geographic heterogeneities typical of subsurface, mineral resources. Here, we describe a robust and systematic method for collecting core scale characterization data that can be applied to studies on the contextual and spatial attributes, the geologic history, and lithostratigraphy of sedimentary basins. The methods were developed using drilled cores from coal bearing sedimentary strata in the Powder River Basin, Wyoming (PRB). The goal of this effort is to create a unified core characterization methodology to guide systematic collection of key data to achieve a foundation of spatially and geologically constrained REEs and CMs. This guidance covers a range of measurement types and methods that are each useful either individually or in combination to support characterization and delineation of REE and CM occurrences. The methods herein, whether used in part or in full, establish a framework to guide consistent acquisition of geological, geochemical, and geospatial datasets that are key to assessing and validating REE and CM occurrences from geologic sources to support future exploration, assessment, and techno-economic related models and analyses.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1983

LOX/hydrocarbon fuel carbon formation and mixing data analysis

By applying the Priem-Heidmann Generalized-Length vaporization correlation, the computer model developed by the present study predicts the spatial variation of propellant vaporization rate using the injector cold flow results to define the streamtubes. The calculations show that the overall and local propellant vaporization rate and mixture ratio change drastically as the injection element type or the injector operating condition is changed. These results are compared with the regions of carbon formation observed in the photographic combustion testing. The correlation shows that the fuel vaporization rate and the local mixture ratio produced by the injector element have first order effects on the degree of carbon formation.

Fang, J.↗

NASA NTRS1987

A mathematical model for predicting cyclic voltammograms of electronically conductive polypyrrole

Polypyrrole is an attractive polymer for use as a high-energy-density secondary battery because of its potential as an inexpensive, lightweight, and noncorrosive electrode material. A mathematical model to simulate cyclic voltammograms for polypyrrole is presented. The model is for a conductive porous electrode film on a rotating disk electrode (RDE) and is used to predict the spatial and time dependence of concentration, overpotential, and stored charge profiles within a polypyrrole film. The model includes both faradic and capacitance charge components in the total current density expression.

Yeu, Taewhan↗

NASA NTRS1988

Current-driven resistive ballooning modes in axially bounded solar flare plasmas

The most unstable current-driven resistive modes of an axially bounded coronal loop are found in computer simulations to exhibit the spatial structure of ballooning modes. The observed modes are not confined to mode rational surfaces, but instead have broad radial extent. A theory assuming ballooning mode spatial structure predicts that a minimum current should be required for linear instability, and that, when the mode is unstable, the linear growth rate scales linearly with the resistivity eta below a critical resistivity, and scales as cu root of eta for larger resistivities. Both predictions are borne out by simulation results. Both theory and simulation analyses of the mode suggest that the strong radial structure of the mode near the ends of the system is the primary contributing factor to the instability of the mode. A helical current sheet is formed in the nonlinear evolution of the mode near the edge of the current channel and is accompanied by a strong radial gradient in the current and partial current reversal.

Otani, Niels F.↗

NASA NTRS1988

A mathematical model for predicting cyclic voltammograms of electronically conductive polypyrrole

Yeu, Taewhan↗

NASA NTRS1993

Luminosity segregation in galaxy clusters as an indication of dynamical evolution

Theoretical models describing the dynamical evolution of self-gravitating systems predict a spatial mass segregation for more evolved systems, with the more massive objects concentrated toward the center of the configuration. From the observational point of view, however, the existence of mass segregation in galaxy clusters seems to be a matter of controversy. A special problem in this connection is the formation of cD galaxies in the centers of galaxy clusters. The most promising scenarios of their formation are galaxy cannibalism (merger scenario) and growing by cooling flows. It seems to be plausible to consider the swallowing of smaller systems by a dominant galaxy as an important process in the evolution of a cD galaxy. The stage of the evolution of the dominant galaxy should be reflected by the surrounding galaxy population, especially by possible mass segregation effects. Assuming that mass segregation is tantamount to luminosity segregation we analyzed luminosity segregation in roughly 40 cD galaxy clusters. Obviously there are three different groups of clusters: (1) clusters with luminosity segregation, (2) clusters without luminosity segregation, and (3) such objects exhibiting a phenomenon which we call antisegregation in luminosity, i.e. a deficiency of bright galaxies in the central regions of clusters. This result is interpreted in the sense of different degrees of mass segregation and as an indication for different evolution stages of these clusters. The clusters are arranged in the three segregation classes 2, 1, and 0 (S2 = strong mass segregation, S1 = moderate mass segregation, S0 = weak or absent mass segregation). We assume that a galaxy cluster starts its dynamical evolution after virialization without any radial mass segregation. Energy exchange during encounters of cluster members as well as merger processes between cluster galaxies lead to an increasing radial mass segregation in the cluster (S1). If a certain degree of segregation (S2) has been established, an essential number of slow-moving and relative massive cluster members in the center will be cannibalized by the initial brightest cluster galaxy. This process should lead to the growing of the predominate galaxy, which is accompanied by a diminution of the mass segregation (transition to S1 and S0, respectively) in the neighborhood of the central very massive galaxy. An increase of the areal density of brighter galaxies towards the outer cluster regions (antisegregation of luminosity), i.e. an extreme low degree of mass segregation was estimated for a substantial percentage of cD clusters. This result favors the cannibalism scenario for the formation of cD galaxies.

Baier, F. W.↗

NASA NTRS1989

Lunar landing and launch facilities (Complex 39L): Guidance systems and propellant systems

After a general, overall definition of Complex 39L during the previous two years, the 1988-89 projects were chosen to focus on more specific aspects, specifically, guidance systems and propellant systems. Six teams or subtasks were formulated: cascade refrigeration for boil-off recovery of cryogenic storage vessels; lunar ground-based radar system to track space vehicles; microwave altimeter for spacecraft; development of a computational model for the determination of lunar surface and sub-surface temperatures; lunar cryogenic facility for the storage of fuels; and lunar lander fuel inventory tent for the storage of cryogenic vessels. At the present time, a cascade refrigeration system for a cryogenic boil-off recovery system has been designed. This is to serve as a baseline system. The ground-based tracking system uses existing technology to implement a reliable tracking radar for use on the lunar surface. A prototype has been constructed. The microwave altimeter is for use on lunar landers. It makes use of the Doppler effect to measure both altitude and the vertical velocity component of the spacecraft. A prototype has been constructed. A computational model that predicts the spatial and temporal temperature profiles of the lunar subsurface was formulated. Propellant storage vessels have been designed. A support for these vessels which minimizes heat leaks was also designed. Further work on the details of the Fuel Inventory Tent (FIT) was performed. While much design work on the overall Complex 39L remains to be done, significant new work has been performed in the subject areas.

Source record↗

NASA NTRS1995

The global frequency-wave number spectrum of oceanic variability estimated from TOPEX/POSEIDON altimetric measurements: The Journal of Geophysical Research - Volume 100, No. C12

Two years of altimetric data from the TOPEX/POSEIDON spacecraft have been used to produce preliminary estimates of the space and time spectra of global variability for both sea surface height and slope. The results are expressed in terms of both degree variances from spherical harmonic expansions and in along-track wavenumbers. Simple analytic approximations both in terms of piece-wise power laws and Pade fractions are provided for comparison with independent measurements and for easy use of the results. A number of uses of such spectra exist, including the possibility of combining the altimetric data with other observations, predictions of spatial coherences, and the estimation of the accuracy of apparent secular trends in sea level.

Wunsch, Carl↗

NASA NTRS2001

A New "Cloud Mode" for the AERONET

A key to predicting climate change is to observe an understand the global distribution of clouds and their physical properties such as optical thickness and droplet size. Since clouds change rapidly over short time and space intervals, they are difficult to simulate in computer models. But it is essential that global climate models predict realistic spatial and temporal distribution of cloud optical depth. The best way to verify these distributions is to infer optical depth from global coverage satellite data. However, satellite methods have many sources of uncertainty; thus, independent and reliable ground-based estimates are essential for validation. For aerosol, there is the AERONET - a ground based monitoring network that consists of identical multi-channel radiometers for assessing aerosol optical properties and validating their satellite retrievals. In addition to AEROSOL, we want the network monitoring CLOUD optical properties. It will use AERONET "time" (inappropriate for aerosol studies) to make basic new measurements related to cloud physics. In the presentation we will report on a new technique that retrieves cloud optical thickness for even broken clouds above green vegetation from surface measurements of zenith radiance in the visible (VIS) and near-IR (NIR) spectral regions. The idea of the method is simple: since green vegetation reflects 40-50% of incoming radiation in the NIR and only 5-10% in the VIS region, ground measurements under thin clouds have little spectral contrast between VIS and NIR, while thick clouds reflect much more of the surface-reflected radiation in the NIR than in VIS. Based on this idea, we use a combination of measurements (spectral indices) in VIS and NIR to estimate cloud optical thickness. By analogy with NDVI, the simplest index that can be defined is the Normalized Difference Cloud Index (NDCI) which is a ratio between the difference and the sum of two radiances measured for two narrow spectral bands in VIS and NIR.

Marshak, Alexander↗

NASA NTRS2011

The Hyperspectral Thermal Emission Spectrometer (HyTES): Preliminary Results

The Hyperspectral Thermal Emission Spectrometer (HyTES) is being developed as part of the risk reduction activities associated with the Hyperspectral Infrared Imager (HyspIRI). HyspIRI is one of the Tier 2 Decadal Survey Missions. HyTES will provide information on how to place the filters on the HyspIRI Thermal Infrared Instrument (TIR) as well as provide antecedent science data. The pushbroom design has 512 spatial pixels over a 50-degree field of view and 256 spectral channels between 7.5 micrometers to 12 micrometers. HyTES includes many key enabling state-of-the-art technologies including a high performance convex diffraction grating, a quantum well infrared photodetector (QWIP) focal plane array, and a compact Dyson-inspired optical design. The Dyson optical design allows for a very compact and optically fast system (F/1.6). It also minimizes cooling requirements due to the fact it has a single monolithic prism-like grating design which allows baffling for stray light suppression. The monolithic configuration eases mechanical tolerancing requirements which are a concern since the complete optical assembly is operated at cryogenic temperatures ((is) approximately 100K). The QWIP allows for optimum spatial and spectral uniformity and provides adequate responsivity or D-star to allow 200mK noise equivalent temperature difference (NEDT) operation across the LWIR passband. Assembly of the system is nearly complete. After completion, alignment results will be presented which show low keystone and smile distortion. This is required to minimize spatial-spectral mixing between adjacent spectral channels and spatial positions. Predictions show the system will have adequate signal to noise for laboratory calibration targets.

Moon Mineralogical Mapper (M3).↗

NASA NTRS2015

On Theoretical Broadband Shock-Associated Noise Near-Field Cross-Spectra

The cross-spectral acoustic analogy is used to predict auto-spectra and cross-spectra of broadband shock-associated noise in the near-field and far-field from a range of heated and unheated supersonic off-design jets. A single equivalent source model is proposed for the near-field, mid-field, and far-field terms, that contains flow-field statistics of the shock wave shear layer interactions. Flow-field statistics are modeled based upon experimental observation and computational fluid dynamics solutions. An axisymmetric assumption is used to reduce the model to a closed-form equation involving a double summation over the equivalent source at each shock wave shear layer interaction. Predictions are compared with a wide variety of measurements at numerous jet Mach numbers and temperature ratios from multiple facilities. Auto-spectral predictions of broadband shock-associated noise in the near-field and far-field capture trends observed in measurement and other prediction theories. Predictions of spatial coherence of broadband shock-associated noise accurately capture the peak coherent intensity, frequency, and spectral width.

Miller, Steven A. E.↗

NASA NTRS2019

Effects of Volcanic Emissions on Clouds During Kilauea Degassing Events

Aerosols influence Earth’s radiative balance directly by scattering and absorbing solar radiation, and indirectly by modifying cloud properties. Current scientific consensus indicates that these effects may offset as much as 50% of the warming due to greenhouse gas emissions. Over the last two decades dramatic volcanic events in Hawaii have produced localized aerosol emissions in otherwise clean environments. These are “natural experiments" where the aerosol effects on clouds and climate can be partitioned from other effects like meteorology and industrial emissions. Therefore, these events provide a unique opportunity to learn about possible effects of aerosol pollution on climate through cloud modification. In this work we use the version 5 of the NASA Goddard Earth Observing System (GEOS-5) and satellite retrievals to analyze and evaluate the strength of the aerosol indirect effect on liquid and ice clouds during the 2008 and 2018 Kilauea degassing events using different emissions scenarios (0, 1, and 5 actual emissions). Our results suggested that the 2018 event was stronger and more regionally significant with respect to cloud formation process for both liquid and ice clouds, while the 2008 affected local liquid clouds only. GEOS-5 predictions reproduced spatial patterns for all parameters, however better precision could be gained by using more accurate plume parameters for height and ash concentration.

Breen, K. H.↗

NASA NTRS2019

Using Computational Flow Imaging to Optimize Filtered Rayleigh Scattering Measurements of an Isolator Shock Train

Filtered Rayleigh scattering (FRS) is a laser diagnostic where the intensity of elastically scattered light is measured after it passes through a molecular absorption filter. The filter removes background interference that overwhelms the relatively weak scattering from the gas molecules. However, with a filter, the measured light intensity depends on many of the scattering gas properties, including pressure, density, temperature, and velocity. In this work, CFD simulations of an isolator shock train flow field are input into a physics-based model to predict the values of FRS intensity measurements in a proposed experiment. The goal is to evaluate if a simplistic FRS setup (that utilizes one camera, laser, and absorption filter) can be used to accurately quantify number density despite the fact that the scattered light intensity also depends on other gas properties. It is found that the experimental setup can be optimized such that a linear relationship describes the number density with an average prediction error of 2%. The vast majority of the flow exhibits prediction errors of less than 3%, but small regions of the flow reach up to 11% error. A sensitivity analysis shows that the prediction error increases with the central wavelength of the incident laser light and decreases with the angle between the camera and laser propagation directions. The optimal experimental parameters are chosen based on a compromise between the prediction error, spatial resolution, and the amount of unfiltered light. In the future, the proposed FRS setup will be implemented to acquire new and valuable information on an isolator shock train, a flow field that has been traditionally studied using wall static pressure measurements and path-integrated visualization techniques, such as schlieren and shadowgraphy.

Hunt, Robin L.↗

DOE OSTI2022

Transient convective delayed neutron precursor of {sup 235}U for the molten salt reactor experiment

This work investigates the delayed neutron precursors from the fission of {sup 235}U in molten salt reactors. The six delayed neutron groups predict the spatial distribution of the advective transport for radioactive mass transfer in the molten-salt reactor experiment (MSRE). The Mole code, using the framework of the Multiphysics Object-Oriented Simulation Environment (MOOSE), was used to compute the delayed neutron concentration of the whole system. This approach can be used for analysis of reactivity in circulating conditions. The effect of delayed neutron concentrations on the static or dynamic behavior of the system in MSRE was analyzed. Using this approach, the pattern and validation of delayed neutron for a range of parameters of interest are reported and discussed herein. (authors)

21 SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLANTS↗

DOE OSTI2022

Stream Temperature Predictions for River Basin Management in the Pacific Northwest and Mid-Atlantic Regions Using Machine Learning

Stream temperature (Ts) is an important water quality parameter that affects ecosystem health and human water use for beneficial purposes. Accurate Ts predictions at different spatial and temporal scales can inform water management decisions that account for the effects of changing climate and extreme events. In particular, widespread predictions of Ts in unmonitored stream reaches can enable decision makers to be responsive to changes caused by unforeseen disturbances. In this study, we demonstrate the use of classical machine learning (ML) models, support vector regression and gradient boosted trees (XGBoost), for monthly Ts predictions in 78 pristine and human-impacted catchments of the Mid-Atlantic and Pacific Northwest hydrologic regions spanning different geologies, climate, and land use. The ML models were trained using long-term monitoring data from 1980–2020 for three scenarios: (1) temporal predictions at a single site, (2) temporal predictions for multiple sites within a region, and (3) spatiotemporal predictions in unmonitored basins (PUB). In the first two scenarios, the ML models predicted Ts with median root mean squared errors (RMSE) of 0.69–0.84 °C and 0.92–1.02 °C across different model types for the temporal predictions at single and multiple sites respectively. For the PUB scenario, we used a bootstrap aggregation approach using models trained with different subsets of data, for which an ensemble XGBoost implementation outperformed all other modeling configurations (median RMSE 0.62 °C).The ML models improved median monthly Ts estimates compared to baseline statistical multi-linear regression models by 15–48% depending on the site and scenario. Air temperature was found to be the primary driver of monthly Ts for all sites, with secondary influence of month of the year (seasonality) and solar radiation, while discharge was a significant predictor at only 10 sites. The predictive performance of the ML models was robust to configuration changes in model setup and inputs, but was influenced by the distance to the nearest dam with RMSE <1 °C at sites situated greater than 16 and 44 km from a dam for the temporal single site and regional scenarios, and over 1.4 km from a dam for the PUB scenario. Our results show that classical ML models with solely meteorological inputs can be used for spatial and temporal predictions of monthly Ts in pristine and managed basins with reasonable (<1 °C) accuracy for most locations.

54 ENVIRONMENTAL SCIENCES↗

NASA NTRS1994

Is Linear Displacement Information Or Angular Displacement Information Used During The Adaptation of Pointing Responses To An Optically Shifted Image?

Twenty-four observers looked through a pair of 20 diopter wedge prisms and pointed to an image of a target which was displaced vertically from eye level by 6 cm at a distance of 30 cm. Observers pointed 40 times, using only their right hand, and received error-corrective feedback upon termination of each pointing response (terminal visual feedback). At three testing distances, 20, 30, and 40 cm, ten pre-exposure and ten post-exposure pointing responses were recorded for each hand as observers reached to a mirror-viewed target located at eye level. The difference between pre- and post-exposure pointing response (adaptive shift) was compared for both Exposed and Unexposed hands across all three testing distances. The data were assessed according to the results predicted by two alternative models for processing spatial-information: one using angular displacement information and another using linear displacement information. The angular model of spatial mapping best predicted the observer's pointing response for the Exposed hand. Although the angular adaptive shift did not change significantly as a function of distance (F(2,44) = 1.12, n.s.), the linear adaptive shift increased significantly over the three testing distances 02 44) = 4.90 p less than 0.01).

Bautista, Abigail B.↗

NASA NTRS1995

Intelligent automated surface grid generation

The goal of our research is to produce a flexible, general grid generator for automated use by other programs, such as numerical optimizers. The current trend in the gridding field is toward interactive gridding. Interactive gridding more readily taps into the spatial reasoning abilities of the human user through the use of a graphical interface with a mouse. However, a sometimes fruitful approach to generating new designs is to apply an optimizer with shape modification operators to improve an initial design. In order for this approach to be useful, the optimizer must be able to automatically grid and evaluate the candidate designs. This paper describes and intelligent gridder that is capable of analyzing the topology of the spatial domain and predicting approximate physical behaviors based on the geometry of the spatial domain to automatically generate grids for computational fluid dynamics simulators. Typically gridding programs are given a partitioning of the spatial domain to assist the gridder. Our gridder is capable of performing this partitioning. This enables the gridder to automatically grid spatial domains of wide range of configurations.

Yao, Ke-Thia↗

NASA NTRS2006

NASA Radiation Track Image GUI for Assessing Space Radiation Biological Effects

The high-charge high-energy (HZE) ion components of the galactic cosmic rays when compared to terrestrial forms of radiations present unique challenges to biological systems. In this paper we present a deoxyribonucleic acid (DNA) breakage model to visualize and analyze the impact of chromatin domains and DNA loops on clustering of DNA damage from X rays, protons, and HZE ions. Our model of DNA breakage is based on a stochastic process of DNA double-strand break (DSB) formulation that includes the amorphous model of the radiation track and a polymer model of DNA packed in the cell nucleus. Our model is a Monte-Carlo simulation based on a randomly located DSB cluster formulation that accomodates both high- and low-linear energy transfer radiations. We demonstrate that HZE ions have a strong impact on DSB clustering, both along the chromosome length and in the nucleus volume. The effects of chromosomal domains and DNA loops on the DSB fragment-size distribution and the spatial distribution of DSB in the nucleus were studied. We compare our model predictions with the spatial distribution of DSB obtained from experiments. The implications of our model predictions for radiation protection are discussed.

Ponomarev, Artem L.↗