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NASA NTRS1998

Radiative Flux Changes by Aerosols from North America, Europe, and Africa over the Atlantic Ocean: Measurements and Calculations from TARFOX and ACE-2

Aerosol effects on atmospheric radiative fluxes provide a forcing function that is a major source of uncertainty in understanding the past climate and predicting climate change. To help reduce this uncertainty, the 1996 Tropospheric Aerosol Radiative Forcing Experiment (TARFOX) and the 1997 second Aerosol Characterization Experiment (ACE-2) measured the properties and radiative effects of American, European, and African aerosols over the Atlantic. In TARFOX, radiative fluxes and microphysics of the American aerosol were measured from the UK C-130 while optical depth spectra, aerosol composition, and other properties were measured by the University of Washington C-131A and the CIRPAS Pelican. Closure studies show that the measured flux changes agree with those derived from the aerosol measurements using several modelling approaches. The best-fit midvisible single-scatter albedos (approx. 0.89 to 0.93) obtained from the TARFOX flux comparisons are in accord with values derived by independent techniques. In ACE-2 we measured optical depth and extinction spectra for both European urban-marine aerosols and free-tropospheric African dust aerosols, using sunphotometers on the R/V Vodyanitskiy and the Pelican. Preliminary values for the radiative flux sensitivities (Delta Flux / Delta Optical depth) computed for ACE-2 aerosols (boundary layer and African dust) over ocean are similar to those found in TARFOX. Combining a satellite-derived optical depth climatology with the aerosol optical model validated for flux sensitivities in TARFOX provides first-cut estimates of aerosol-induced flux changes over the Atlantic Ocean.

Russell, P. B.↗
NASA NTRS2002

The Micro-Pulse Lidar Network (MPL-Net)

In the early 1990s, the first small, eye-safe, and autonomous lidar system was developed, the Micro-pulse Lidar (MPL). The MPL has proven to be useful in the field because it can be automated, runs continuously (day and night), is eye-safe, can easily be transported and set up, and has a small field-of-view which limits multiple scattering concerns. The MPL acquires signal profiles of backscattered laser light from aerosols and clouds. The signals are analyzed to yield multiple layer heights, optical depths of each layer, average extinction-to-backscatter ratio of each layer, and profiles of extinction in each layer. The MPL has been used in a wide variety of field studies over the past 10 years, leading to nearly 20 papers and many conference presentations. In 2000, a new project using MPL systems was started at NASA Goddard Space Flight Center. The MPL-Net project is currently working to establish a worldwide network of MPL systems, all co-located with NASA's AERONET sunphotometers for joint measurements of optical depth and sky radiance. Automated processing algorithms have been developed to produce data products on a next day basis for all sites and some field experiments. Initial results from the first several sites are shown, along with aerosol data collected during several major field campaigns. Measurements of the aerosol extinction-to-backscatter ratio at several different geographic regions, and for various aerosol types are shown. This information is used to improve the construction of look up tables of the ratio, needed to process aerosol profiles acquired with satellite based lidars.

Welton, Ellsworth J.↗
NASA NTRS2002

MPL-Net Measurements of Aerosol and Cloud Vertical Distributions at Co-Located AERONET Sites

In the early 1990s, the first small, eye-safe, and autonomous lidar system was developed, the Micropulse Lidar (MPL). The MPL acquires signal profiles of backscattered laser light from aerosols and clouds. The signals are analyzed to yield multiple layer heights, optical depths of each layer, average extinction-to-backscatter ratios for each layer, and profiles of extinction in each layer. In 2000, several MPL sites were organized into a coordinated network, called MPL-Net, by the Cloud and Aerosol Lidar Group at NASA Goddard Space Flight Center (GSFC) using funding provided by the NASA Earth Observing System. tn addition to the funding provided by NASA EOS, the NASA CERES Ground Validation Group supplied four MPL systems to the project, and the NASA TOMS group contributed their MPL for work at GSFC. The Atmospheric Radiation Measurement Program (ARM) also agreed to make their data available to the MPL-Net project for processing. In addition to the initial NASA and ARM operated sites, several other independent research groups have also expressed interest in joining the network using their own instruments. Finally, a limited amount of EOS funding was set aside to participate in various field experiments each year. The NASA Sensor Intercomparison and Merger for Biological and Interdisciplinary Oceanic Studies (SIMBIOS) project also provides funds to deploy their MPL during ocean research cruises. All together, the MPL-Net project has participated in four major field experiments since 2000. Most MPL-Net sites and field experiment locations are also co-located with sunphotometers in the NASA Aerosol Robotic Network. (AERONET). Therefore, at these locations data is collected on both aerosol and cloud vertical structure as well as column optical depth and sky radiance. Real-time data products are now available from most MPL-Net sites. Our real-time products are generated at times of AERONET aerosol optical depth (AOD) measurements. The AERONET AOD is used as input to our processing routines, which calculate the aerosol layer top height and extinction profile, and our MPL calibration value. A variety of other data products are available or under development. We present an overview of the MPL-Net project and discuss data products useful to the AERONET community. Results from several sites and field experiments will be presented.

Welton, Ellsworth J.↗
NASA NTRS2003

Calculations of Aerosol Radiative Forcing in the SAFARI Region from MODIS Data

SAFARI 2000 provided the opportunity to validate MODIS aerosol retrievals and to correct any assumptions in the retrieval process. By comparing MODIS retrievals with ground-based sunphotometer data, we quantified the degree to which the MODIS algorithm underestimated the aerosol optical thickness. This discrepancy was attributed to underestimating the degree of light absorption by the southern African smoke aerosol. Correcting for this underestimation of absorption, produces more realistic aerosol retrievals that allow various applications of the MODIS aerosol products. One such application is the calculation of the aerosol radiative forcing at the top and bottom of the atmosphere. The combination of MODIS accuracy, coverage, resolution and the ability to separate fine and coarse mode make this calculation substantially advanced over previous attempts with other satellites. We focus on the oceans adjacent to southern Africa and use a solar radiative transfer model to perform the flux calculations. The forcing at the top of atmosphere is calculated to be 10 W/sq m, while the forcing at the surface is -26 W/sq m. These results resemble those calculated from INDOEX data, and are most sensitive to assumptions of aerosol absorption, the same parameter that initially interfered with our retrievals.

Remer, L. A.↗
NASA NTRS2003

University of Washington Airborne Studies in Support of the CLAMS-2001 Field Study

The main activity under this grant was participation in the Chesapeake Lighthouse and Aircraft Measurements for Satellites (CLAMS) field study from 10 July through 2 August 2001. The Cloud and Aerosol Research Group (CARG) from the University of Washington (UW) flew its Convair-580 research aircraft on thirteen occasions, for a total of 45 research flight hours, in support of CLAMS. Some of the main accomplishments of these flights were: 1) Aerosol and trace gas measurements and sunphotometer measurements of aerosol optical depth and column water vapor and ozone from close to Ocean surface to approx. 10,000 ft off Delmarva Peninsula on various occasions; 2) Measurements of aerosol properties on seven occasions beneath the Terra satellite, once beneath AVHRR, and five times beneath the ER-2 aircraft; 3) Measurements of aerosol properties in the vicinity of the (CERES instrumented) Chesapeake Bay lighthouse (COVE) on nine occasions; 4) Use of the NASA Goddard Cloud Absorption Radiometer (CAR) to obtain measurements of BRDF of the ocean surface on fifteen occasions and over Great Dismal Swamp on two occasions; 5) Measurements of aerosol properties over instrumented buoys 44014, 44004, and 41001. 6) On July 17 (a CLAMS 'Golden Day') six aircraft, including the Convair-580 and ER-2, were stacked above the Chesapeake Bay lighthouse under clear skies at the time of the Terra overpass.

Hobbs, Peter V.↗
NASA NTRS2003

The "RED Versa NIR" Plane to Retrieve Broken-Cloud Optical Depth from Ground-Based Measurements"

A new method for retrieving cloud optical depth from ground-based measurements of zenith radiance in the RED and near infrared (MR) spectral regions is introduced. Because zenith radiance does not have a one-to-one relationship with optical depth, it is absolutely impossible to use a monochromatic retrieval. On the other side, algebraic combinations of spectral radiances such as NDCI while largely removing nouniquiness and the radiative effects of cloud inhomogeneity, can result in poor retrievals due to its insensitivity to cloud fraction. Instead, both RED and NIR radiances as points on the 'RED vs. NIR' plane are proposed to be used for retrieval. The proposed retrieval method is applied to Cimel measurements at the Atmospheric Radiation Measurements (ARM) site in Oklahoma. Cimel, a multi-channel sunphotometer, is a part of AERONET - a ground-based network for monitoring aerosol optical properties. The results of retrieval are compared with the ones from Microwave Radiometer (MWR) and Multi-Filter Rotating Shadowband Radiometers (MFRSR) located next to Cimel at the ARM site. In addition, the performance of the retrieval method is assessed using a fractal model of cloud inhomogeneity and broken cloudiness. The preliminary results look very promising both theoretically and from measurements.

Marshak, A.↗
NASA NTRS2003

Retrieval of Ozone Column Content from Airborne Sun Photometer Measurements During SOLVE II: Comparison with SAGE III, POAM III,THOMAS and GOME Measurements

During the Second SAGE 111 Ozone Loss and Validation Experiment (SOLVE II), the 14- channel NASA Ames Airborne Trackmg Sunphotometer (AATS-14) was mounted on the NASA DC-8 and successfully measured spectra of total and aerosol optical depth (TOD and AOD) during the sunlit portions of eight science flights. Values of ozone column content above the aircraft have been derived from the AATS-14 data by using a linear least squares method. For each AATS-14 measured TOD spectrum, this method iteratively finds the ozone column content that yields the best match between measured and calculated TOD. The calculations assume the known Chappuis ozone band shape and a three-parameter AOD shape (quadratic in log-log space). Seven of the AATS-14 channels (each employing an interference filter with a nominal full-width at half maximum bandpass of -5 nm) are within the Chappuis band, with center wavelengths between 452.9 nm and 864.5 nm. One channel (604.4 nm) is near the peak, and three channels (499.4, 519.4 and 675.1 nm) have ozone absorption within 30-40% of that at the peak. For the typical DC-8 SOLVE II cruising altitudes of approx. 8-12 km and the background stratospheric aerosol conditions that prevailed during SOLVE 11, absorption of incoming solar radiation by ozone comprised a significant fraction of the aerosol-plus-ozone optical depth measured in the four AATS-14 channels centered between 499.4 and 675.1 nm. Typical AODs above the DC-8 ranged from 0.003-0.008 in these channels. For comparison, an ozone overburden of 0.3 atm-cm (300 DU) translates to ozone optical depths of 0.009,0.014, 0.041, and 0.012, respectively, at these same wavelengths. In this paper, we compare AATS-14 values of ozone column content with temporally and spatially near-coincident values derived from measurements acquired by the Stratospheric Aerosol and Gas Experiment III (SAGE III) and the Polar Ozone and Aerosol Measurement 111 (POAM III) satellite sensors. We also compare AATS-14 ozone retrievals during selected DC-8 latitudinal and longitudinal transects with total column ozone data acquired by the Total Ozone Mapping Spectrometer (TOMS) and the Global Ozone Monitoring Experiment (GOME) satellite sensors. To enable this comparison, the amount of ozone in the column below the aircraft is estimated by combining SAGE and/or POAM data with high resolution, fast response in-situ ozone measurements acquired during the DC-8 ascent at the start of each science flight.

Livingston, J.↗
NASA NTRS2003

Airborne Sun Photometer Measurements of Aerosol Optical Depth during SOLVE II: Comparison with SAGE III and POAM III Measurements

The 14-channel NASA Ames Airborne Tracking Sunphotometer (AATS-14) was operated aboard the NASA DC-8 during the Second SAGE III Ozone Loss and Validation Experiment (SOLVE II) and obtained successful measurements during the sunlit segments of eight science flights. These included six flights out of Kiruna, Sweden, one flight out of NASA Dryden Flight Research Center (DFRC), and the Kiruna-DFRC return transit flight. Values of spectral aerosol optical depth (AOD), columnar ozone and columnar water vapor have been derived from the AATS-14 measurements. In this paper, we focus on AATS-14 AOD data. In particular, we compare AATS-14 AOD spectra with temporally and spatially near-coincident measurements by the Stratospheric Aerosol and Gas Experiment III (SAGE III) and the Polar Ozone and Aerosol Measurement III (POAM III) satellite sensors. We examine the effect on retrieved AOD of uncertainties in relative optical airmass (the ratio of AOD along the instrument-to-sun slant path to that along the vertical path) at large solar zenith angles. Airmass uncertainties result fiom uncertainties in requisite assumed vertical profiles of aerosol extinction due to inhomogeneity along the viewing path or simply to lack of available data. We also compare AATS-14 slant path solar transmission measurements with coincident measurements acquired from the DC-8 by the NASA Langley Research Center Gas and Aerosol Measurement Sensor (GAMS).

Russell, P.↗
NASA NTRS2003

Vertically Resolved Aerosol Optical Properties over the ARM SGP Site

In order to meet one of its goals - to relate observations of radiative fluxes and radiances to the atmospheric composition - the Department of Energy's Atmospheric Radiation Measurement (ARM) program has pursued measurements and modeling activities that attempt to determine how aerosols impact atmospheric radiative transfer, both directly and indirectly. However, significant discrepancies between aerosol properties measured in situ or remotely remain. To this end, the ARM program will conduct an Aerosol Intensive Operational Period (IOP) in May 2003 at the ARM Southern Great Plains (SGP) site in north central Oklahoma. The IOP involves airborne measurements from two airplanes over the heavily instrumented SGP site. We will give an overview of early airborne results obtained aboard Center for Interdisciplinary Remotely-Piloted Aircraft Studies (CIRPAS) Twin Otter aircraft. The aircraft will carry instrumentation to perform in-situ measurements of aerosol absorption, scattering, extinction and particle size including such novel techniques as the photoacoustic and cavity ring-down methods. Aerosol optical depth and extinction will be measured with the NASA Ames Airborne Tracking 14-channel sunphotometer. Furthermore up- and downwelling solar (broadband and spectral) and infrared radiation will be measured using three different instruments. The up-looking radiation instruments will be mounted on a newly developed stabilized platform, which will keep the instruments level up to aircraft pitch and roll angles of 10 degrees. Additional effort will be directed toward measurement of cloud condensation nucleus concentration as a function of supersaturation and relating CCN concentration to aerosol composition and size distribution. This relation is central to description of the aerosol indirect effect.

Schmid, B.↗
NASA NTRS2003

Synergism of MODIS Aerosol Remote Sensing from Terra and Aqua

The MODerate-resolution Imaging Spectro-radiometer (MODIS) sensors, aboard the Earth Observing System (EOS) Terra and Aqua satellites, are showing excellent competence at measuring the global distribution and properties of aerosols. Terra and Aqua were launched on December 18, 1999 and May 4, 2002 respectively, with daytime equator crossing times of approximately 10:30 am and 1:30 pm respectively. Several aerosol parameters are retrieved at 10-km spatial resolution from MODIS daytime data over land and ocean surfaces. The parameters retrieved include: aerosol optical thickness (AOT) at 0.47, 0.55 and 0.66 micron wavelengths over land, and at 0.47, 0.55, 0.66, 0.87, 1.2, 1.6, and 2.1 microns over ocean; Angstrom exponent over land and ocean; and effective radii, and the proportion of AOT contributed by the small mode aerosols over ocean. Since the beginning of its operation, the quality of Terra-MODIS aerosol products (especially AOT) have been evaluated periodically by cross-correlation with equivalent data sets acquired by ground-based (and occasionally also airborne) sunphotometers, particularly those coordinated within the framework of the AErosol Robotic NETwork (AERONET). Terra-MODIS AOT data have been found to meet or exceed pre-launch accuracy expectations, and have been applied to various studies dealing with local, regional, and global aerosol monitoring. The results of these Terra-MODIS aerosol data validation efforts and studies have been reported in several scientific papers and conferences. Although Aqua-MODIS is still young, it is already yielding formidable aerosol data products, which are also subjected to careful periodic evaluation similar to that implemented for the Terra-MODIS products. This paper presents results of validation of Aqua-MODIS aerosol products with AERONET, as well as comparative evaluation against corresponding Terra-MODIS data. In addition, we show interesting independent and synergistic applications of MODIS aerosol data from both Terra and Aqua. In certain situations, this combined analysis of Terra- and Aqua-MODIS data offers an insight into the diurnal cycle of aerosol loading.

Ichoku, Charles↗
NASA NTRS2003

Measurement and Modeling of Vertically Resolved Aerosol Optical Properties and Radiative Fluxes Over the ARM SGP Site

In order to meet one of its goals - to relate observations of radiative fluxes and radiances to the atmospheric composition - the Department of Energy's Atmospheric Radiation Measurement (ARM) program has pursued measurements and modeling activities that attempt to determine how aerosols impact atmospheric radiative transfer, both directly and indirectly. However, significant discrepancies between aerosol properties measured in situ or remotely remain. One of the objectives of the Aerosol Intensive Operational Period (TOP) conducted by ARM in May 2003 at the ARM Southern Great Plains (SGP) site in north central Oklahoma was to examine and hopefully reduce these differences. The IOP involved airborne measurements from two airplanes over the heavily instrumented SGP site. We give an overview of airborne results obtained aboard the Center for Interdisciplinary Remotely-Piloted Aircraft Studies (CIRPAS) Twin Otter aircraft. The Twin Otter performed 16 research flights over the SGP site. The aircraft carried instrumentation to perform in-situ measurements of aerosol absorption, scattering, extinction and particle size. This included such novel techniques as the photoacoustic and cavity ring-down methods for in-situ absorption (675 nm) and extinction (675 and 1550 nm) and a new multiwavelength, filter-based absorption photometer (467, 530, 660 nm). A newly developed instrument measured cloud condensation nucleus concentration (CCN) concentrations at two supersaturation levels. Aerosol optical depth and extinction (354-2139 nm) were measured with the NASA Ames Airborne Tracking 14-channel sunphotometer. Furthermore, up-and downwelling solar (broadband and spectral) and infrared radiation were measured using seven individual radiometers. Three up-looking radiometers werer mounted on a newly developed stabilized platform, keeping the instruments level up to aircraft pitch and roll angles of approximately 10(exp 0). This resulted in unprecedented continuous vertical profiles of radiative fluxes, which we will compare to modeled fluxes using the aforementioned data as input.

Schmid, B.↗
NASA NTRS2003

Investigation of Overlap Correction Techniques for Application in the Micro-Pulse Lidar Network (MPLNET)

The Micro-Pulse Lidar NETwork (MPLNET) is comprised of micro-pulse lidars (MPL) stationed around the globe to provide measurements of aerosol and cloud vertical distribution on a continuous basis. MPLNET sites are co-located with sunphotometers in the AErosol Robotic NETwork (AERONET) to provide joint measurements of aerosol optical depth, size, and other inherent optical properties. The IPCC 2001 report discusses . the importance of obtaining routine measurements of aerosol vertical structure, especially for absorbing aerosols. MPLNET provides exactly this sort of measurement, including calculation of aerosol extinction profiles, in a near real-time basis for all sites in the network. In order to obtain aerosol profiles, near range signal returns (0-6 km) must be accurately measured by the MPL. This measurement is complicated by the instrument s overlap range: Le., the minimum distance at which returning signals are completely in the instrument s field-of-view (FOV). Typical MPL overlap distances are large, between 5 - 6 km, due to the narrow FOV of the MPL receiver. A function describing the MPL overlap must be determined and used to correct signals in this range. Currently, overlap functions for MPLNET are determined using horizontal MPL measurements along a path with 10-1 5 km clear line-of-sight and a homogenous atmosphere. These conditions limit the location and ease in which successful overlaps can be obtained. Furthermore, the current MPLNET process of correcting for overlap increases the uncertainty and bias error for the near range signals and the resulting aerosol extinction profiles. To address these issues, an alternative overlap correction method using a small-diameter, wide FOV receiver is being considered for potential use in MPLNET. The wide FOV receiver has a much shorter overlap distance and will be used to calculate the overlap function of the MPL receiver. This approach has a significant benefit in that overlap corrections could be obtained without the need for horizontal measurements. A review of both overlap methods is presented, including a discussion of the impact on reducing the uncertainty and bias error in MPLNET aerosol profiles.

Berkoff, Timothy A.↗
NASA NTRS2003

Inferring Cloud Properties from Passive Solar Sensors

The most common approach for retrieving cloud optical depth from ground-based observations uses downwelling fluxes measured by pyranometers and Multi-Filter Rotating Shadowband Radiometers (MFRSR). The key element in both retrieval techniques is the one-to-one mapping of the "observed" fluxes into cloud optical depth through plane-parallel radiative transfer. Both methods are expected to work well only for completely overcast clouds giving an effective optical depth for the whole sky. To infer cloud optical depth locally one can assume to use a narrow-field-of view radiometer that measures radiances instead of fluxes. However, lack of one-to-one relationships between radiance and cloud optical depth, prevents the direct use of radiances either. Here we discuss a new method for retrieving cloud optical depth from ground-based measurements of zenith radiance in the RED and near infrared (NIR) spectral regions. In addition to an algebraic combinations of spectral radiances such as Normalized Difference Cloud Index (NDCI) that largely removes nonuniqueness and the radiative effects of cloud inhomogeneity but can result in poor retrievals due to its insensitivity to cloud fraction, both RED and NIR radiances as points on the "RED vs. NIR" plane are proposed to be used for retrieval. The proposed retrieval method is applied to a multi- channel sunphotometer (as a part of AERONET) measurements at the ARM site in Oklahoma. The results of retrieval are compared with the ones from Microwave Radiometer (MWR) and MFRSR. In addition to cloud optical depth, the new retrieval method also infers a "radiatively effective" cloud fraction.

Marshak, A.↗
NASA NTRS2004

How Can AERONET Help with Monitoring Clouds?

When conditions are inappropriate to make AErosol RObotic NETwork (AERONET) measurements for aerosol studies, new measurements related to cloud physics can be made instead. As such, several AERONET CIMEL sunphotometers have been equipped with a new "cloud mode." This mode allows the CIMELs to make measurements of zenith radiance when the Sun in blocked by clouds. When in cloud mode, a CIMEL points straight up every 10-15 minutes and takes 10 measurements over a 9 second time interval at four wavelengths: 440,670,870, and 1020 nm. For cloudy conditions above green vegetation, the spectral contrast in surface albedo dominates over Rayleigh and aerosol effects. We have developed a new method for retrieving cloud optical depth, even for broken clouds, that uses data from the 670 (and/or 440) and 870 nm channels. In addition to cloud optical depth, the method also infers a "radiatively effective" cloud fraction. The results of the retrievals at the ARM Central Facility in Oklahoma are compared with the ones from Microwave Radiometer (MWR) and Multi-Filter Rotating Shadowband Radiometers (MFRSR).

Marshak, A.↗
NASA NTRS2004

Aerosol Optical Depth Measurements by Airborne Sun Photometer in SOLVE II: Comparisons to SAGE III, POAM III and Airborne Spectrometer Measurements

The 14-channel NASA Ames Airborne Tracking Sunphotometer (AATS-14) measured solar-beam transmission on the NASA DC-8 during the Second SAGE III Ozone Loss and Validation Experiment (SOLVE II). This paper presents AATS-14 results for multiwavelength aerosol optical depth (AOD), including its spatial structure and comparisons to results from two satellite sensors and another DC-8 instrument. These are the Stratospheric Aerosol and Gas Experiment III (SAGE III), the Polar Ozone and Aerosol Measurement III (POAM III) and the Direct beam Irradiance Airborne Spectrometer (DIAS).

Russell, P.↗
NASA NTRS2004

A Comparison of Aerosol Optical Property Measurements Made During the DOE Aerosol Intensive Operating Period and Their Effects on Regional Climate

The amount of radiant energy an aerosol absorbs has profound effects on climate and air quality. It is ironic that aerosol absorption coefficient is one of the most difficult to measure aerosol properties. One of the main purposes of the DOE Aerosol Intensive Operating Period (IOP) flown in May, 2003 was to assess our ability to measure absorption coefficient in situ. This paper compares measurements of aerosol optical properties made during the IOP. Measurements of aerosol absorption coefficient were made by Particle Soot Absorption Photometer (PSAP) aboard the CIRPAS Twin-Otter (U. Washington) and on the DOE Cessna 172 (NOAA-C,MDL). Aerosol absorption coefficient was also measured by a photoacoustic instrument (DRI) that was operated on an aircraft for the first time during the IOP. A new cavity ring-down (CRD) instrument, called Cadenza (NASA-AkC), measures the aerosol extinction coefficient for 675 nm and 1550 nm light, and simultaneously measures the scattering coefficient at 675 nm. Absorption coefficient is obtained from the difference of measured extinction and scattering within the instrument. Measurements of absorption coefficient from all of these instruments during appropriate periods are compared. During the IOP, several significant aerosol layers were sampled aloft. These layers are identified in the remote (AATS-14) as well as in situ measurements. Extinction profiles measured by Cadenza are compared to those derived from the Ames Airborne Tracking Sunphotometer (AATS-14, NASA-ARC). The regional radiative impact of these layers is assessed by using the measured aerosol optical properties in a radiative transfer model.

Strawa, Anthony W.↗
NASA NTRS2004

In-Situ Measurements of Aerosol Optical Properties using New Cavity Ring-Down and Photoacoustics Instruments and Comparison with more Traditional Techniques

Carbonaceous species (BC and OC) are responsible for most of the absorption associated with aerosol particles. The amount of radiant energy an aerosol absorbs has profound effects on climate and air quality. It is ironic that aerosol absorption coefficient is one of the most difficult aerosol properties to measure. A new cavity ring-down (CRD) instrument, called Cadenza (NASA-ARC), measures the aerosol extinction coefficient for 675 nm and 1550 nm light, and simultaneously measures the scattering coefficient at 675 nm. Absorption coefficient is obtained from the difference of measured extinction and scattering within the instrument. Aerosol absorption coefficient is also measured by a photoacoustic (PA) instrument (DRI) that was operated on an aircraft for the first time during the DOE Aerosol Intensive Operating Period (IOP). This paper will report on measurements made with this new instrument and other in-situ instruments during two field recent field studies. The first field study was an airborne cam;oaign, the DOE Aerosol Intensive Operating Period flown in May, 2003 over northern Oklahoma. One of the main purposes of the IOP was to assess our ability to measure extinction and absorption coefficient in situ. This paper compares measurements of these aerosol optical properties made by the CRD, PA, nephelometer, and Particle Soot Absorption Photometer (PSAP) aboard the CIRPAS Twin-Otter. During the IOP, several significant aerosol layers were sampled aloft. These layers are identified in the remote (AATS-14) as well as in situ measurements. Extinction profiles measured by Cadenza are compared to those derived from the Ames Airborne Tracking Sunphotometer (AATS-14, NASA-ARC). The regional radiative impact of these layers is assessed by using the measured aerosol optical properties in a radiative transfer model. The second study was conducted in the Caldecott Tunnel, a heavily-used tunnel located north of San Francisco, Ca. The aerosol sampled in this study was characterized by fresh automobile and diesel exhaust. Measurements from Cadenza and from an aethalometer are presented. The aethalometer is a filter-based photometer and the infrared channel is calibrated to produce a measure of BC mass loading.

Strawa, A. W.↗
NASA NTRS2004

Cloud-Vegetation Radiative Interaction: What Can We Learn from it about Cloud Optical Properties?

Because of their radiative interactions, the vegetation canopy and the atmosphere are coupled together; each serves as a boundary condition to the radative transfer equations in the adjacent medium. To better understand radiative processes in these media we need an accurate description of their interactions. This presentation outlines a technique needed to describe interactions between vegetation and clouds and exploits it to retrieve cloud optical depth from ground-based radiance measurements. measurements of zenith radiance in the RED and NIR spectral regions. In addition to an algebraic combinations of spectral radiances such as Normalized Difference Cloud Index (NDCI) that can result in poor retrievals due to its insensitivity to cloud fraction, both RED and NIR radiances as points on the "RED vs. NIR" plane are proposed to be used for retrieval. The proposed method is applied to a multi-channel sunphotometer (as a part of AERONET) measurements at the ARM site in Oklahoma. In addition to cloud optical depth, the new method also infers a "radiatively effective" cloud fraction.

Marshak, Alexander↗