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At least 1,261 records · Page 70

Unified Mechanism behind the Appearance of T-Odd TRI and ROT Asymmetries in Actinide Fission Induced by Cold Polarized Neutrons

Some shortcomings of the approaches that are used to describe T-odd ROT and TRI asymmetries in true ternary fission via reactions involving the emission of prescission alpha particles and which are based on employing the classical method of trajectory calculations are analyzed. These shortcomings are caused by the disregard of the interference between the fission widths of different sJ{sub s} neutron resonance states formed in the first well of the deformation potential of fissile compound nuclei. It is shown that the method used in some studies to determine T-odd TRI-asymmetries for prescission alpha particles is at odds with basic concepts of the generalizedmodel of the nucleus and approaches to constructing collective (for example, bending) vibrations of a fissile compound nucleus. Quantum-mechanical fission theory is generalized via employing a unified mechanism of formation of T-odd TRI and ROT asymmetries for prescission alpha particles and evaporated photons (neutrons). The proposed mechanism takes correctly into account the effect of quantum rotation of a fissile compound nucleus on the angular distributions of fission fragments and alpha particles for true ternary fission, as well as on the angular distribution of prompt photons (neutrons) emitted by fragments originating from the delayed fission of the aforementioned nuclei.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The Differential Cross Section and Λ Recoil Polarization from γδ -> Κ0(ρ)

Presented is the analysis of the differential cross section and Λ recoil polarization from the reaction γδ -> Κ0(ρ). This work measured these observables over beam energies from 0.90 GeV to 3.0 GeV. These measurements are the first in this channel to cover such a wide range of energies. The data were taken using the CEBAF Large Acceptance Spectrometer (CLAS) at Jefferson Laboratory (JLAB) along with a tagged photon beam. This analysis was completed by identifying events of interest that decayed into the final state topology of π-π+,π-&rho'(ρ). Through conservation of energy and momentum, the Κ0, Λ and missing mass of the spectator proton were reconstructed. Utilizing the same analysis techniques, the observables were measured on two different experiments with good agreement. Photoproduction of strange mesons from the neutron are difficult to measure, consequently there are only a few measurements of this kind. Despite that, these reactions supply essential complementary data to those on the proton. The differential cross sections and the recoil polarization extracted, span the region where new nucleon resonances have been found from studies of the reaction γρ -> Κ+Λ. Comparisons between the Κ+Λ and Κ0Λ cross section demonstrate that possible interference terms near 1900 MeV are less pronounced in the latter. This unexpected result inspired a partial wave analyses (PWA) to be fitted to the data. The fit solution shows that this measurement fostered an improvement on the knowledge of observed resonance parameters, necessary to understanding these excited states. The study of nucleon resonances is a key motivating factor since the resonance masses can be calculated from the theory of the strong nuclear force, called quantum chromodynamics, or QCD.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Exploring Interatomic Coulombic Decay by Free Electron Lasers

To exploit the high intensity of laser radiation, we propose to select frequencies at which single-photon absorption is of too low energy and two or more photons are needed to produce states of an atom that can undergo interatomic Coulombic decay (ICD) with its neighbors. For Ne{sub 2} it is explicitly demonstrated that the proposed multiphoton absorption scheme is much more efficient than schemes used until now, which rely on single-photon absorption. Extensive calculations on Ne{sub 2} show how the low-energy ICD electrons and Ne{sup +} pairs are produced for different laser intensities and pulse durations. At higher intensities the production of Ne{sup +} pairs by successive ionization of the two atoms becomes competitive and the respective emitted electrons interfere with the ICD electrons. It is also shown that a measurement after a time delay can be used to determine the contribution of ICD even at high laser intensity.

38 RADIATION CHEMISTRY, RADIOCHEMISTRY, AND NUCLEA↗

Examples of Current and Future Uses of Neural-Net Image Processing for Aerospace Applications

Feed forward artificial neural networks are very convenient for performing correlated interpolation of pairs of complex noisy data sets as well as detecting small changes in image data. Image-to-image, image-to-variable and image-to-index applications have been tested at Glenn. Early demonstration applications are summarized including image-directed alignment of optics, tomography, flow-visualization control of wind-tunnel operations and structural-model-trained neural networks. A practical application is reviewed that employs neural-net detection of structural damage from interference fringe patterns. Both sensor-based and optics-only calibration procedures are available for this technique. These accomplishments have generated the knowledge necessary to suggest some other applications for NASA and Government programs. A tomography application is discussed to support Glenn's Icing Research tomography effort. The self-regularizing capability of a neural net is shown to predict the expected performance of the tomography geometry and to augment fast data processing. Other potential applications involve the quantum technologies. It may be possible to use a neural net as an image-to-image controller of an optical tweezers being used for diagnostics of isolated nano structures. The image-to-image transformation properties also offer the potential for simulating quantum computing. Computer resources are detailed for implementing the black box calibration features of the neural nets.

Decker, Arthur J.↗

Single-crystalline germanium nanomembrane photodetectors on foreign nanocavities

Miniaturization of optoelectronic devices offers tremendous performance gain. As the volume of photoactive material decreases, optoelectronic performance improves, including the operation speed, the signal-to-noise ratio, and the internal quantum efficiency. Over the past decades, researchers have managed to reduce the volume of photoactive materials in solar cells and photodetectors by orders of magnitude. However, two issues arise when one continues to thin down the photoactive layers to the nanometer scale (for example, <50 nm). First, light-matter interaction becomes weak, resulting in incomplete photon absorption and low quantum efficiency. Second, it is difficult to obtain ultrathin materials with single-crystalline quality. We introduce a method to overcome these two challenges simultaneously. It uses conventional bulk semiconductor wafers, such as Si, Ge, and GaAs, to realize single-crystalline films on foreign substrates that are designed for enhanced light-matter interaction. We use a high-yield and high-throughput method to demonstrate nanometer-thin photodetectors with significantly enhanced light absorption based on nanocavity interference mechanism. As a result, these single-crystalline nanomembrane photodetectors also exhibit unique optoelectronic properties, such as the strong field effect and spectral selectivity.

77 NANOSCIENCE AND NANOTECHNOLOGY↗

Electro-optical measurement of intense electric field on a high energy pulsed power accelerator

We describe a direct electro-optical approach to measuring a strong 118 MV/m narrow pulse width (~ 33 ns) electric field in the magnetically insulated transmission line (MITL) of a pulsed power accelerator. To date, this is the highest direct external electric field measured electro-optically in a pulsed power accelerator, and it is between two to three orders of magnitude higher than values reported in comparable high energy scientific experiments. The MITL electric field is one of the most important operating parameters in an accelerator and is critical to understanding the properties of the radiation output. However, accurately measuring these high fields using conventional pulsed power diagnostics is difficult due to the strength of interfering particles and fields. Our approach uses a free-space laser beam with a dielectric crystal sensor that is highly immune to electromagnetic interference and does not require an external calibration. Here we focus on device theory, operating parameters, laboratory and pulsed power accelerator experiments as well as challenges that were overcome in the measurement environment.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

High harmonic generation spectroscopy via orbital angular momentum

We present an experimental technique using orbital angular momentum (OAM) in a fundamental laser field to drive high harmonic generation (HHG). The mixing of beams with different OAM allows us to generate two laser foci tightly spaced which generate harmonics that interfere in the far field. Thus, this technique is an OAM based in situ HHG interferometric spectroscopic method. With this tool, we measure the phase and amplitude of the angle dependent multiorbital HHG emission in molecular nitrogen

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Interference in nonlinear Compton scattering using a Schrödinger-equation approach

The interference between Compton scattering and nonlinear Compton scattering from a two-color field in the X-ray regime is theoretically examined for bound electrons. Here, the underlying phase shifts are analyzed using a perturbative approach in the incoming classical field. The perturbative approach is bench marked with a non-perturbative approach in the classical field. The interference for different combinations of linear polarization of the two fields is examined when the Compton and the nonlinear Compton scattered waves have the same wave vector and polarization. Only two cases exhibit interference. When there is interference, the calculations reveal an intrinsic phase difference between the Compton scattered wave function and the nonlinear Compton scattered wave function of either 0 or pi depending on the scattering angle.

74 ATOMIC AND MOLECULAR PHYSICS↗

Nonadiabatic tunneling via conical intersections and the role of the geometric phase

As a ubiquitous quantum effect, tunneling has attracted attention ever since the dawn of quantum mechanics. However, recent evidence suggests that nonadiabatic atomic tunneling near a conical intersection (CI) behaves differently from its adiabatic counterpart, producing lifetime differences of up to two orders of magnitude. Using two-dimensional models, we demonstrate here that the failure of the adiabatic model in describing tunneling near a CI can be attributed largely to the neglect of the geometric phase, which is associated with the adiabatic electronic wave function transported around a CI. Furthermore, the geometric phase–induced destructive interference among wave functions following different paths around the CI, manifested as a node in the adiabatic wave function, retards tunneling.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Waveguiding and Dispersion Properties of Interband Cascade Laser Frequency Combs

Mid-infrared semiconductor lasers have emerged as indispensable compact coherent sources for military and commercial applications. While much of the historical emphasis has been on maximizing the output power and/or spectral purity, a recent new focus has been on engineering these lasers to operate as optical frequency combs (OFCs) for broadband real-time spectroscopy. In particular, the combination of low-drive-power and broad gain bandwidth has made interband cascade laser (ICL) OFCs an attractive complement to quantum cascade laser OFCs operating at longer wavelengths. Moreover, ICL combs can potentially be incorporated into fully-integrated dual-comb spectrometers that employ fast, room-temperature IC photodetectors processed on the same chip.However, the high refractive index of the ICL’s GaSb substrate poses some challenges to the optical waveguiding. Because the modal index is considerably lower than that of the substrate, the optical field can penetrate the bottom cladding layer and leak into the GaSb, inducing wavelength-dependent interference that modifies the gain and group velocity dispersion (GVD) profiles. Even when the effect on lasing threshold is small, the comb properties can be adversely affected. Using the sub-threshold Fourier transform technique, we studied ICL combs with various ridge widths, substrate thicknesses, and center wavelengths. This allowed us to evaluate the effects of modal leakage on the GVD. We find that the resonant nature of the substrate modes induces oscillations, which affect both the spectral bandwidth and the phase-locking properties above threshold. Strategies to mitigate the GVD’s undesired and unpredictable spectral variation will be presented.

Meyer, J. R↗

Bell Inequality Experiment for a High Brightness Time-Energy Entangled Source

A periodically poled MgO - doped LiNbO3 (MgO:LN) non-degenerate photon pair source is utilized for spontaneous parametric down-conversion of 532-nanometer photons into time-energy entangled pairs of 800- and 1600-nanometer photons. The entangled photons are separated using previously detailed sorting optics, such that each wavelength is independently directed through one of two modified Mach-Zehnder interferometers - also known as a Franson interferometer - after which they are fiber-optically guided to high-efficiency photon detectors. Output from the detectors is sent to a high resolution time tagger, where coincidences between the entangled photons are recorded. By varying the length of the long path in one Mach-Zehnder interferometer, it is possible to observe high visibility sinusoidal fringes in the measured coincidence rates (while no variation is seen in single photon detection rates). These fringes - due to interference between the photon probability amplitudes - are indicative of a violation of the Bell inequality, and confirm inconsistencies with local hidden variable theory for the correlations of the time-energy entangled photon pairs.

Time-Energy Entanglement↗

Applications of Emerging Parallel Optical Link Technology to High Energy Physics Experiments

Modern particle detectors depend upon optical fiber links to deliver event data to upstream trigger and data processing systems. Future detector systems can benefit from the development of dense arrangements of high speed optical links emerging from the telecommunications and storage area network market segments. These links support data transfers in each direction at rates up to 120 Gbps in packages that minimize or even eliminate edge connector requirements. Emerging products include a class of devices known as optical engines which permit assembly of the optical transceivers in close proximity to the electrical interfaces of ASICs and FPGAs which handle the data in parallel electrical format. Such assemblies will reduce required printed circuit board area and minimize electromagnetic interference and susceptibility. We will present test results of some of these parallel components and report on the development of pluggable FPGA Mezzanine Cards equipped with optical engines to provide to collaborators on the Versatile Link Common Project for the HI-LHC at CERN.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Reshaped Weyl fermionic dispersions driven by Coulomb interactions in MoTe 2

In this work, we report the direct evidence of impacts of the Coulomb interaction in a prototypical Weyl semimetal, MoTe 2 , that alter its bare bands in a wide range of energy and momentum. Our quasiparticle interference patterns measured using scanning tunneling microscopy are shown to match the joint density of states of quasiparticle energy bands including momentum-dependent self-energy corrections, while electronic energy bands based on the other simpler local approximations of the Coulomb interaction fail to explain neither the correct number of quasiparticle pockets nor the shape of their dispersions observed in our spectrum. With this, we predict a transition between type-I and type-II Weyl fermions with doping and resolve its disparate quantum oscillation experiments, thus highlighting the critical roles of Coulomb interactions in layered Weyl semimetals.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

A microscopic perspective on moiré materials

Quantum materials research has experienced a veritable renaissance in the past 6 years, with a surge of experimental reports of nearly every known electronic phase of matter and of several unique and unexpected phases, all found in an emerging class of highly tunable 2D materials, known as moiré materials1,2,3. Here, moiré materials are designed through either the rotational misalignment of identical 2D atomic crystals or the lattice mismatch of dissimilar 2D atomic crystals (Fig. 1). Both these incommensurability conditions cause long-wavelength (~10 nm) interference patterns between the two constituent atomic lattices, forming an enlarged moiré superlattice that generically hosts flat electronic bands, which are highly conducive to correlated, collective phases of matter.

36 MATERIALS SCIENCE↗

Nonadiabatic dissociation of molecular Bose-Einstein condensates: Competition between chemical reactions

Here, we provide a framework to solve generic models describing the dissociation of multiple molecular Bose Einstein condensates in a nonadiabatic regime. The competition between individual chemical reactions can lead to non-trivial dependence on critical components such as path interference and symmetries, thus, affecting the final distribution of atomic population. We find an analytical solution for an illustrative example model involving four atomic modes. When the system parameters satisfy CPT symmetry, where C is charge conjugation, P is parity, and T is time-reversal symmetry, our solution predicts a population imbalance between atomic modes that is exponentially sensitive to system parameters. However, a weakly broken symmetry alters the population in each atomic mode and can reverse the population imbalance. Our solution also demonstrates a strong quantum correlation between atomic modes that leads to the spontaneous production of atoms in a multi-mode squeezed state. Moreover, in our framework, a time-dependent non-Hermitian quantum mechanics naturally manifests which can alternatively be realized experimentally in photonic systems.

74 ATOMIC AND MOLECULAR PHYSICS↗

Chromatic interferometry with small frequency differences

By developing a ‘two-crystal’ method for color erasure, we can broaden the scope of chromatic interferometry to include optical photons whose frequency difference falls outside of the 400 nm to 4500 nm wavelength range, which is the passband of a PPLN crystal. We demonstrate this possibility experimentally, by observing interference patterns between sources at 1064.4 nm and 1063.6 nm, corresponding to a frequency difference of about 200 GHz.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Modeling Electronic Quantum Transport with Machine Learning

We present a machine learning approach to solve electronic quantum transport equations of one-dimensional nanostructures. The transmission coefficients of disordered systems were computed to provide training and test data sets to the machine. The system’s representation encodes energetic as well as geometrical information to characterize similarities between disordered configurations, while the Euclidean norm is used as a measure of similarity. Errors for out-of-sample predictions systematically decrease with training set size, enabling the accurate and fast prediction of new transmission coefficients. The remarkable performance of our model to capture the complexity of interference phenomena lends further support to its viability in dealing with transport problems of undulatory nature.

97 MATHEMATICS AND COMPUTING↗

Pressure Distortion of the H{sub 2}–He Collision-induced Absorption at the Photosphere of Cool White Dwarf Stars

Collision-induced absorption (CIA) from molecular hydrogen is a dominant opacity source in the atmosphere of cool white dwarfs. It results in a significant flux depletion in the near-IR and IR parts of their spectra. Because of the extreme conditions of helium-rich atmospheres (where the density can be as high as a few g cm{sup −3}), this opacity source is expected to undergo strong pressure distortion and the currently used opacities have not been validated at such extreme conditions. To check the distortion of the CIA opacity, we applied state-of-the-art ab initio methods of computational quantum chemistry to simulate the CIA opacity at high densities. The results show that the CIA profiles are significantly distorted above densities of 0.1 g cm{sup −3} in a way that is not captured by the existing models. The roto-translational band is enhanced and shifted to higher frequencies as an effect of the decrease of the interatomic separation of the H{sub 2} molecule. The vibrational band is blueward shifted and split into Q {sub R} and Q {sub P} branches, separated by a pronounced interference dip. Its intensity is also substantially reduced. The distortions result in a shift of the maximum of the absorption from 2.3 μm to 3–7 μm, which could potentially explain the spectra of some very cool, helium-rich white dwarfs.

79 ASTRONOMY AND ASTROPHYSICS↗