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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,279 records · Page 71
All sourcesNASA NTRSDOE OSTI
DOE OSTI2016

MAGIC Cloud Properties from Zenith Radiance Data Final Campaign Summary

Cloud droplet size and optical depth are the most fundamental properties for understanding cloud formation, dissipation and interactions with aerosol and drizzle. They are also a crucial determinant of Earth’s radiative and water-energy balances. However, these properties are poorly predicted in climate models. As a result, the response of clouds to climate change is one of the major sources of uncertainty in climate prediction.

47 OTHER INSTRUMENTATION↗
NASA NTRS1991

The 27-28 October 1986 FIRE Cirrus case study - Retrieval of cloud particle sizes and optical depths from comparative analyses of aircraft and satellite-based infrared measurements

Infrared radiance measurements were acquired from a narrow-field nadir-viewing radiometer based on the NASA ER-2 aircraft during a coincident Landsat 5 overpass on October 28, 1986 as part of the FIRE Cirrus IFO in the vicinity of Lake Michigan. The spectral bandpasses are 9.90-10.87 microns for the ER-2-based radiometer and 10.40-12.50 microns for the Landsat thematic mapper band. After adjusting for spatial and temporal differences, a comparative study using data from these two instruments is undertaken in order to retrieve cirrus cloud ice-crystal sizes and optical depths. Retrieval is achieved by analysis of measurement correlations between the two spectral bands and comparison to multistream radiative transfer model calculations. The results indicate that the equivalent sphere radii of the cirrus ice crystals were typically less than 30 microns. Such particles were too small to be measured by the available in situ instrumentation. Cloud optical depths at a reference wavelength of 11.4 microns ranged from 0.3 to 2.0 for this case study. Supplemental results in support of this study are described using radiation measurements from the King Air aircraft, which was also in near coincidence with the Landsat overpass.

Hammer, Philip D.↗
NASA NTRS1983

Nuclear winter - Global consequences of multiple nuclear explosions

The results of a computerized simulation of the potential global environmental effects of dust and smoke clouds that would be generated by a nuclear war are presented. Short term effects of blast, fire, and radiation are neglected in the series of physical models that include a nuclear war scenario, a particle microphysics model, and a radiative convective model. Account is taken of the altitude-dependent dust, smoke, radioactivity, and NO(x) injections, the temporal evolution of dust and smoke clouds, land and ocean environments, and temperature contrasts. A nuclear exchange would produce thousands of individual smoke and dust clouds rising up to 30 km altitude in the midlatitudes. The smoke, dust, and radioactive debris would cover the entire midlatitudes within 1-2 weeks. The smoke would arise from conflagrations of forests, suburbs, and urban areas. Obscuration of sunlight would induce subfreezing temperatures for several months, disruption of the global circulation patterns, and the arrival of a nuclear winter, followed and accompanied by radioactive fallout, pyrogenic air pollution, and UV-B flux enhancements. It is estimated that a total of only 100 Mtons would be sufficient to plunge the Northern Hemisphere summer to subfreezing temperatures lasting months. Since the probable exchange in a nuclear war would exceed 5000 Mtons, it is expected that many species, including humans, may not survive the war.

Turco, R. P.↗
NASA NTRS1991

Diurnal variability of the hydrologic cycle in a general circulation model

In the present Colorado State University GCM simulation-based analysis of the diurnal and semidiurnal variability of precipitation, precipitable water, evaporation, cloudiness, horizontal moisture flux convergence, and cloud radiative forcing, a realistic afternoon precipitation maximum is obtained over land in warm rainy regions, as well as an early morning maximum over the oceans. The model has been further used to investigate the bases for the oceanic diurnal-precipitation cycle; the results thus obtained indicate that such an oceanic cycle occurs even in the absence of neighboring continents, and tends to have a morning maximum, although the observed phenomenon is generally stronger than the results indicate.

Randall, David A.↗
NASA NTRS1991

A new look at dust and clouds in the Mars atmosphere - Analysis of emission-phase-function sequences from global Viking IRTM observations

The present analysis of emission-phase function (EPF) observations from the IR thermal mapper aboard the Viking Orbiter encompasses polar latitudes, and Viking Lander sites, and spans a wide range of solar longitudes. A multiple scattering radiative transfer model which incorporates a bidirectional phase function for the surface and atmospheric scattering by dust and clouds yields surface albedos and dust and ice optical properties and optical depths for the variety of Mars conditions. It is possible to fit all analyzed EPF sequences corresponding to dust scattering with an albedo of 0.92, rather than the 0.86 given by Pollack et al. on the bases of Viking Lander observations.

Clancy, R. T.↗
NASA NTRS1999

Improving Pixel Level Cloud Optical Property Retrieval using Monte Carlo Simulations

The accurate pixel-by-pixel retrieval of cloud optical properties from space is influenced by radiative smoothing due to high order photon scattering and radiative roughening due to low order scattering events. Both are caused by cloud heterogeneity and the three-dimensional nature of radiative transfer and can be studied with the aid of computer simulations. We use Monte Carlo simulations on variable 1-D and 2-D model cloud fields to seek for dependencies of smoothing and roughening phenomena on single scattering albedo, solar zenith angle, and cloud characteristics. The results are discussed in the context of high resolution satellite (such as Landsat) retrieval applications. The current work extends the investigation on the inverse NIPA (Non-local Independent Pixel Approximation) as a tool for removing smoothing and improving retrievals of cloud optical depth. This is accomplished by: (1) Delineating the limits of NIPA applicability; (2) Exploring NIPA parameter dependences on cloud macrostructural features, such as mean cloud optical depth and geometrical thickness, degree of extinction and cloud top height variability. We also compare parameter values from empirical and theoretical considerations; (3) Examining the differences between applying NIPA on radiation quantities vs direct application on optical properties; (4) Studying the radiation budget importance of the NIPA corrections as a function of scale. Finally, we discuss fundamental adjustments that need to be considered for successful radiance inversion at non-conservative wavelengths and oblique Sun angles. These adjustments are necessary to remove roughening signatures which become more prominent with increasing absorption and solar zenith angle.

Oreopoulos, Lazaros↗
DOE OSTI2016

DMS role in ENSO cycle in the tropics

We examined the multiyear mean and variability of dimethyl sulfide (DMS) and its relationship to sulfate aerosols, as well as cloud microphysical and radiative properties. We conducted a 150 year simulation using preindustrial conditions produced by the Community Earth System Model embedded with a dynamic DMS module. The model simulated the mean spatial distribution of DMS emissions and burden, as well as sulfur budgets associated with DMS, SO 2 , H 2 SO 4 , and sulfate that were generally similar to available observations and inventories for a variety of regions. Changes in simulated sea-to-air DMS emissions and associated atmospheric abundance, along with associated aerosols and cloud and radiative properties, were consistently dominated by El Niño–Southern Oscillation (ENSO) cycle in the tropical Pacific region. Simulated DMS, aerosols, and clouds showed a weak positive feedback on sea surface temperature. This feedback suggests a link among DMS, aerosols, clouds, and climate on interannual timescales. The variability of DMS emissions associated with ENSO was primarily caused by a higher variation in wind speed during La Niña events. As a result, the simulation results also suggest that variations in DMS emissions increase the frequency of La Niña events but do not alter ENSO variability in terms of the standard deviation of the Niño 3 sea surface temperature anomalies.

58 GEOSCIENCES↗
NASA NTRS2020

Response of Surface Shortwave Cloud Radiative Effect to Greenhouse Gases and Aerosols and Its Impact on Summer Maximum Temperature

Shortwave cloud radiative effects (SWCREs), defined as the difference of the shortwave radiative flux between all-sky and clear-sky conditions at the surface, have been reported to play an important role in influencing the Earth's energy budget and temperature extremes. In this study, we employed a set of global climate models to examine the SWCRE responses to CO2, black carbon (BC) aerosols, and sulfate aerosols in boreal summer over the Northern Hemisphere. We found that CO2 causes positive SWCRE changes over most of the NH, and BC causes similar positive responses over North America, Europe, and eastern China but negative SWCRE over India and tropical Africa. When normalized by effective radiative forcing, the SWCRE from BC is roughly 3–5 times larger than that from CO2. SWCRE change is mainly due to cloud cover changes resulting from changes in relative humidity (RH) and, to a lesser extent, changes in cloud liquid water, circulation, dynamics, and stability. The SWCRE response to sulfate aerosols, however, is negligible compared to that for CO2 and BC because part of the radiation scattered by clouds under all-sky conditions will also be scattered by aerosols under clear-sky conditions. Using a multilinear regression model, it is found that mean daily maximum temperature (Tmax) increases by 0.15 and 0.13 K per watt per square meter (W m−2) increase in local SWCRE under the CO2 and BC experiment, respectively. When domain-averaged, the contribution of SWCRE change to summer mean Tmax changes was 10 %–30 % under CO2 forcing and 30 %–50 % under BC forcing, varying by region, which can have important implications for extreme climatic events and socioeconomic activities.

surface shortwave cloud radiative effect↗
NASA NTRS2012

Sensitivity of Marine Warm Cloud Retrieval Statistics to Algorithm Choices: Examples from MODIS Collection 6

The optical and microphysical structure of warm boundary layer marine clouds is of fundamental importance for understanding a variety of cloud radiation and precipitation processes. With the advent of MODIS (Moderate Resolution Imaging Spectroradiometer) on the NASA EOS Terra and Aqua platforms, simultaneous global/daily 1km retrievals of cloud optical thickness and effective particle size are provided, as well as the derived water path. In addition, the cloud product (MOD06/MYD06 for MODIS Terra and Aqua, respectively) provides separate effective radii results using the l.6, 2.1, and 3.7 ~m spectral channels. Cloud retrieval statistics are highly sensitive to how a pixel identified as being "notclear" by a cloud mask (e.g., the MOD35/MYD35 product) is determined to be useful for an optical retrieval based on a 1-D cloud model. The Collection 5 MODIS retrieval algorithm removed pixels associated with cloud'edges as well as ocean pixels with partly cloudy elements in the 250m MODIS cloud mask - part of the so-called Clear Sky Restoral (CSR) algorithm. Collection 6 attempts retrievals for those two pixel populations, but allows a user to isolate or filter out the populations via CSR pixel-level Quality Assessment (QA) assignments. In this paper, using the preliminary Collection 6 MOD06 product, we present global and regional statistical results of marine warm cloud retrieval sensitivities to the cloud edge and 250m partly cloudy pixel populations. As expected, retrievals for these pixels are generally consistent with a breakdown of the ID cloud model. While optical thickness for these suspect pixel populations may have some utility for radiative studies, the retrievals should be used with extreme caution for process and microphysical studies.

Platnick, Steven↗
DOE OSTI2016

Moist Process Biases in Simulations of the Madden–Julian Oscillation Episodes Observed during the AMIE/DYNAMO Field Campaign

Two Madden–Julian oscillation (MJO) episodes observed during the 2011 Atmospheric Radiation Measurement Program MJO Investigation Experiment (AMIE)/DYNAMO field campaign are simulated using a regional model with various cumulus parameterizations, a regional cloud-permitting model, and a global variable-resolution model with a high-resolution region centered over the tropical Indian Ocean. Model biases in relationships relevant to existing instability theories of MJO are examined and their relative contributions to the overall model errors are quantified using a linear statistical model. The model simulations capture the observed approximately log-linear relationship between moisture saturation fraction and precipitation, but precipitation associated with the given saturation fraction is overestimated especially at low saturation fraction values. This bias is a major contributor to the excessive precipitation during the suppressed phase of MJO. After accounting for this bias using a linear statistical model, the spatial and temporal structures of the model-simulated MJO episodes are much improved, and what remains of the biases is strongly correlated with biases in saturation fraction. The excess precipitation bias during the suppressed phase of the MJO episodes is accompanied by excessive column-integrated radiative forcing and surface evaporation. A large portion of the bias in evaporation is related to biases in wind speed, which are correlated with those of precipitation. Furthermore, these findings suggest that the precipitation bias sustains itself at least partly by cloud radiative feedbacks and convection–surface wind interactions.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2022

Impacts of Suppressing Excessive Light Rain on Aerosol Radiative Effects and Health Risks

Global climate models (GCMs) have been used widely to study radiative forcing and health risks of aerosols. A recent study using two GCMs found that light rain plays a dominant role in controlling aerosol loading. However, “too much light rain and too little heavy rain” is a longstanding bias in GCMs. It is unclear how much light rain affects aerosol-cloud-radiation interactions and health risks from air pollution. Here, in this work, we show that, with the correction of the rainfall intensity spectrum in the National Center for Atmospheric Research Community Atmosphere Model version 5.3 by introducing a stochastic deep convection scheme, the reduced frequency of light rain (1–20 mm d -1 ) results in changes of aerosol direct radiative effects (DRE) of up to -0.5 ± 0.03 W/m 2 and aerosol cloud radiative effects (CRE) of up to -0.9 ± 0.03 W/m 2 . The total (CRE + DRE) radiative effects of light rain-mediated aerosol changes exceed the present-day anthropogenic forcing of aerosols relative to preindustrial levels from the Coupled Model Intercomparison Project (CMIP5&6) models. However, the correction of the rainfall intensity spectrum has little effect on anthropogenic aerosol forcing (defined as the radiative perturbation due to changes in aerosol concentrations between the industrial era and preindustrial levels). Due to increased exposure to fine particulates (PM 2.5 ), the estimated global total premature mortality is much higher than previously estimated, by 300,000 ± 60,000 deaths per year, and is more severe in populous regions such as India and China. The findings in this study highlight the need to understand uncertainties in radiative effects and health risks of aerosols due to simulation biases of precipitation in GCMs.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Glaciation of mixed-phase clouds: insights from bulk model and bin-microphysics large-eddy simulation informed by laboratory experiment

Abstract. Mixed-phase clouds affect precipitation and radiation differently from liquid and ice clouds, posing greater challenges to their representation in numerical simulations. Recent laboratory experiments using the Pi Cloud Chamber explored cloud glaciation conditions based on increased injection of ice-nucleating particles. In this study, we use two approaches to reproduce the results of the laboratory experiments: a bulk scalar mixing model and large-eddy simulation (LES) with bin microphysics. The first approach assumes a well-mixed domain to provide an efficient assessment of the mean cloud properties for a wide range of conditions. The second approach resolves the energy-carrying turbulence, the particle size distribution, and their spatial distribution to provide more details. These modeling approaches enable a separate and detailed examination of liquid and ice properties, which is challenging in the laboratory. Both approaches demonstrate that, with an increased ice number concentration, the flow and microphysical properties exhibit the same changes in trends. Additionally, both approaches show that the ice integral radius reaches the theoretical glaciation threshold when the cloud is subsaturated with respect to liquid water. The main difference between the results of the two approaches is that the bulk model allows for the complete glaciation of the cloud. However, LES reveals that, in a dynamic system, the cloud is not completely glaciated as liquid water droplets are continuously produced near the warm lower boundary and subsequently mixed into the chamber interior. These results highlight the importance of the ice mass fraction in distinguishing the mixed-phase clouds and ice clouds.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

A new method for operating a continuous flow diffusion chamber to investigate immersion freezing: assessment and performance study

Glaciation in mixed-phase clouds predominately occurs through the immersion freezing mode where ice nucleating particles (INPs) immersed within supercooled droplets induce nucleation of ice. Currently, model representations of this process are a large source of uncertainty in simulating cloud radiative properties, and to constrain these estimates, continuous flow diffusion chamber (CFDC)-style INP devices are commonly used to assess the immersion freezing efficiencies of INPs. In this study, a new approach was explored to operating such an ice chamber that provides maximum activation of particles without droplet breakthrough and correction factor ambiguity to obtain high-quality INP measurements in a manner that has not been demonstrated as possible previously. The conditioning section of the chamber was maintained at ~ –20 °C and water relative humidity (RH w ) ~ 113 % conditions to maximize the droplet activation, and the droplets were supercooled with an independently temperature-controlled nucleation section at a steady cooling rate (0.5 °C min –1 ) to induce the freezing of droplets and evaporation of unfrozen droplets. The performance of the modified ice chamber was evaluated using four INP species: K-feldspar, illite-NX, Argentinian soil dust, and airborne arable dust that had shown ice nucleation over a wide span of supercooled temperatures. Dry dispersed and size-selected K-feldspar particles were generated in the laboratory. Illite-NX and soil dust particles were sampled during the second phase of the Fifth International Ice Nucleation Workshop (FIN-02) campaign, and airborne arable dust particles were sampled from the aerosol inlet located on the rooftop of the laboratory. The measured ice nucleation efficiencies of model aerosols with a surface active site density (n s ) metric were higher, but mostly agreed within one order of magnitude compared to literature results.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2018

Evaluation of a High-Resolution Numerical Weather Prediction Model’s Simulated Clouds Using Observations from CloudSat, GOES-13 and in Situ Aircraft

This study aimed to assess tropical cloud properties predicted by Environment and Climate Change Canada’s Global Environmental Multiscale (GEM)modelwhen run with the Milbrandt–Yau double-moment cloud microphysical scheme and one-way nesting that culminated at a (∼300 km)2 inner domain with 0.25 km horizontal grid spacing. The assessment utilized satellite and in situ data collected during the High Ice Water Content (HIWC) and High Altitude Ice Crystals (HAIC) projects for a mesoscale convective system on 16May 2015 over French Guiana.Data fromCloud- Sat’s cloud-profiling radar and GOES-13’s imager were compared to data either simulated directly by GEM or produced by operating on GEM’s cloud data with both the CFMIP (Cloud Feedback Model Intercomparison Project) Observation Simulator Package (COSP) instrument simulator and a three-dimensional Monte Carlo solar radiative transfer model. In situ observations were made from research aircraft – Canada’s National Research Council Convair-580 and the French SAFIRE Falcon-20 – whose flight paths were aligned with CloudSat’s ground-track. Spatial and temporal shifts of clouds simulated by GEM compared well to GOES-13 imagery. There are, however, differences between simulated and observed amounts of high and low cloud. While GEM did well at predicting ranges of ice-water content (IWC) near 11 km altitude (Falcon-20), it produces too much graupel and snow near 7 km (Convair-580). This produced large differences between CloudSat’s and COSP-generated radar reflectivities and two-way attenuations. On the other hand, CloudSat’s inferred values of IWC agree well with in situ samples at both altitudes. Generally, GEM’s visible reflectances exceeded GOES-13’s on account of having produced too much low-level liquid cloud. It is expected that GEM’s disproportioning of cloud hydrometeors will improve once it includes a better representation of secondary ice production.

Qu, Zhipeng↗
DOE OSTI2017

Retrieval of atmospheric properties of cloudy L dwarfs

Here, we present the first results from applying the spectral inversion technique in the cloudy L dwarf regime. This new framework provides a flexible approach to modelling cloud opacity which can be built incrementally as the data require and improves upon previous retrieval experiments in the brown dwarf regime by allowing for scattering in two-stream radiative transfer. Our first application of the tool to two mid-L dwarfs is able to reproduce their near-infrared spectra far more closely than grid models. Our retrieved thermal, chemical and cloud profiles allow us to estimate Teff = 1796 $+23\atop{-25}$ K and logg = 5.21$+0.05\atop{-0.08}$ for 2MASS J05002100+0330501, and for 2MASSW J2224438-015852 we find Teff = 1723 $+18\atop{-19}$ K and log g = 5.31 $+0.04\atop{-0.08}$, in close agreement with previous empirical estimates. Our best model for both objects includes an optically thick cloud deck which passes τcloud ≥ 1 (looking down) at a pressure of around 5 bar. The temperature at this pressure is too high for silicate species to condense, and we argue that corundum and/or iron clouds are responsible for this cloud opacity. Our retrieved profiles are cooler at depth and warmer at altitude than the forward grid models that we compare, and we argue that some form of heating mechanism may be at work in the upper atmospheres of these L dwarfs. We also identify anomalously high CO abundance in both targets, which does not correlate with the warmth of our upper atmospheres or our choice of cloud model, and find similarly anomalous alkali abundance for one of our targets. For these anomalies they may reflect unrecognized shortcomings in our retrieval model or inaccuracies in our gas phase opacities.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2022

Impact of Meteorological Factors on the Mesoscale Morphology of Cloud Streets during a Cold-Air Outbreak over the Western North Atlantic

We report postfrontal clouds (PFC) are ubiquitous in the marine boundary layer, and their morphology is essential to estimating the radiation budget in weather and climate models. Here we examine the roles of sea surface temperature (SST) and meteorological factors in controlling the mesoscale morphology and evolution of shallow clouds associated with a cold-air outbreak that occurred on 1 March 2020 during phase I of the Aerosol Cloud Meteorology Interactions over the Western Atlantic Experiment (ACTIVATE). Our results show that the simulated PFC structure and ambient conditions by the Weather Research and Forecasting (WRF) Model are generally consistent with observations from GOES-16 and dropsonde measurements. We also examine the thermodynamical and dynamical influences in the cloud mesoscale morphology using WRF sensitivity experiments driven by two meteorological forcing datasets with different domain-mean SST and spatial gradients, which lead to dissimilar values of hydrometeor water path and cloud core fraction. The SST from ERA5 leads to weaker stability and higher inversion height than the SST from FNL does. In addition, the use of large-scale meteorological forcings from ERA5 yields a distinctive time evolution of wind direction shear in the inner domain, which favors the formation and persistence of longer cloud rolls. Both factors contribute to a change in the time evolution of domain-mean water path and cloud core fraction of cloud streets. Our study takes advantage of the simulation driven by the differences between two large-scale forcing datasets to illustrate the importance of SST and wind direction shear in the cloud street morphology in a realistic scenario.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS2022

Impact of Meteorological Factors on the Mesoscale Morphology of Cloud Streets during a Cold-Air Outbreak over the Western North Atlantic

Postfrontal clouds (PFC) are ubiquitous in the marine boundary layer, and their morphology is essential to estimating the radiation budget in weather and climate models. Here we examine the roles of sea surface temperature (SST) and meteorological factors in controlling the mesoscale morphology and evolution of shallow clouds associated with a cold-air outbreak that occurred on 1 March 2020 during phase I of the Aerosol Cloud Meteorology Interactions over the Western Atlantic Experiment (ACTIVATE). Our results show that the simulated PFC structure and ambient conditions by the Weather Research and Forecasting (WRF) Model are generally consistent with observations from GOES-16 and dropsonde measurements. We also examine the thermodynamical and dynamical influences in the cloud mesoscale morphology using WRF sensitivity experiments driven by two meteorological forcing datasets with different domain-mean SST and spatial gradients, which lead to dissimilar values of hydrometeor water path and cloud core fraction. The SST from ERA5 leads to weaker stability and higher inversion height than the SST from FNL does. In addition, the use of large-scale meteorological forcings from ERA5 yields a distinctive time evolution of wind direction shear in the inner domain, which favors the formation and persistence of longer cloud rolls. Both factors contribute to a change in the time evolution of domain-mean water path and cloud core fraction of cloud streets. Our study takes advantage of the simulation driven by the differences between two large-scale forcing datasets to illustrate the importance of SST and wind direction shear in the cloud street morphology in a realistic scenario

Jingyi Chen↗
DOE OSTI2020

The ARM Data-oriented Metrics and Diagnostics Package for Climate Models - A New Tool for Evaluating Climate Models with Field Data

The U.S. Department of Energy (DOE) Atmospheric Radiation Measurement (ARM) program User Facility produces ground-based long-term continuous unique measurements for atmospheric state, precipitation, turbulent fluxes, radiation, aerosol, cloud and the land surface, which are collected at multiple sites. These comprehensive datasets have been widely used to calibrate climate models and are proven to be invaluable for climate model development and improvement. This article introduces an evaluation package to facilitate the use of ground-based ARM measurements in climate model evaluation. The ARM data-oriented metrics and diagnostics package (ARM-DIAGS) includes both ARM observational datasets and a Python-based analysis toolkit for computation and visualization. The observational datasets are compiled from multiple ARM data products and specifically tailored for use in climate model evaluation. In addition, ARM-DIAGS also includes simulation data from models participating the Coupled Model Inter-comparison Project (CMIP), which will allow climate-modeling groups to compare a new, candidate version of their model to existing CMIP models. The analysis toolkit is designed to make the metrics and diagnostics quickly available to the model developers.

54 ENVIRONMENTAL SCIENCES↗