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At least 1,297 records · Page 72
All sourcesNASA NTRSDOE OSTI
DOE OSTI2024

Frustrated Ising charge correlations in the kagome metal ScV 6 Sn 6

Here we resolve the real-space nature of the high-temperature, short-range charge correlations in the kagome metal ScV 6 Sn 6 . Diffuse scattering appears along a frustrated wave vector q H = ($\frac{1}{3}, \frac{1}{3}, \frac{1}{2}$) at temperatures far exceeding the charge order T CO = 92 K, preempting long-range charge order with wave vectors along q$_{\bar{K}}$ = ($\frac{1}{3}, \frac{1}{3}, \frac{1}{3}$). Using a combination of real space and reciprocal space analysis, we resolve the nature of the interactions between the primary out-of-plane Sc-Sn chain instability and the secondary strain-mediated distortion of the in-plane V kagome network. Finally, a minimal model of the diffuse scattering data reveals a high-temperature, short-ranged "zig-zag" phase of in-plane correlations that maps to a frustrated triangular lattice Ising model with antiferromagnetic interactions and provides a real-space understanding of the origin frustrated charge order in this material.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2025

Finite-temperature kinetic ferromagnetism in the square-lattice Hubbard model

While the exact phase diagram of the Fermi-Hubbard model remains poorly understood despite decades of progress, nearly 60 years ago Nagaoka proved that a single dopant in an otherwise halffilled Hubbard system can bring about ferromagnetism through kinetic means. The phenomenon was recently observed with ultracold atoms in triangular optical lattices. Here, we explore the kinetic ferromagnetism within the square lattice Hubbard model and its strong-coupling counterpart, the t − J model, at finite temperatures in the thermodynamic limit via numerical linked-cluster expansions. We find evidence of ferromagnetic Nagaoka polarons at dopings up to ∼ 30% away from half filling for a variety of interaction strengths and at temperatures as low as 0.2 of the hopping energy. We map out the boundaries of this phase through analyzing various correlation functions.

Newby, Robin C. [San José State University] (ORCID↗
DOE OSTI2017

Quantum spin liquid with seven elementary particles

We present an exactly solvable model of a quantum spin liquid with Abelian anyons in d = 2 spatial dimensions. With spins 1/2 on a triangular lattice and six-body interactions, our model has zero spin correlation length and localized elementary excitations like the toric codes of Kitaev and Wen. In contrast to those earlier models, it has more elementary particles—four bosons and three fermions—and higher topological degeneracy of 64 on a torus. Elementary excitations are boson-fermion pairs that come in 12 distinct flavors. We use string operators to expose the topological nature of the model.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

Magnetic ground states and magnetodielectric effect in R Cr ( BO 3 ) 2 ( R = Y and Ho)

Here, the layered perovskites RCr(BO 3 ) 2 (R = Y and Ho) with magnetic triangular lattices were studied by performing ac/dc susceptibility, specific heat, elastic and inelastic neutron scattering, and dielectric constant measurements. The results show (i) both samples' Cr 3+ spins order in a canted antiferromagnetic structure with T N around 8–9 K, while the Ho 3+ ions do not order down to T =1.5 K in HoCr(BO 3 ) 2 ; (ii) when a critical magnetic field HC around 2-3 T is applied below T N , the Cr 3+ spins in the Y compound and both the Cr 3+ and Ho 3+ spins in the Ho compound order in a ferromagnetic state; (iii) both samples exhibit dielectric constant anomalies around the transition temperature and critical field, but the Ho compound displays a much stronger magnetodielectric response. We speculate that this is due to the magnetostriction, which depends on both the Cr 3+ and the Ho 3+ ions' ordering in the Ho compound. Moreover, by using linear spin-wave theory to simulate the inelastic neutron scattering data, we estimated the Y compound's intralayer and interlayer exchange strengths as ferromagnetic J 1 = –0.12 meV and antiferromagnetic J 2 = 0.014 meV, respectively. The competition between different kinds of superexchange interactions results in the ferromagnetic intralayer interaction.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

Emergence of chiral spin liquids via quantum melting of noncoplanar magnetic orders

Quantum spin liquids (QSLs) are highly entangled states of quantum magnets which lie beyond the Landau paradigm of classifying phases of matter via broken symmetries. A physical route to arriving at QSLs is via frustration-induced quantum melting of ordered states such as valence bond crystals or magnetic orders. Using extensive exact diagonalization (ED) and density-matrix renormalization group (DMRG)we show studies of concrete S U ( 2 ) invariant spin models on honeycomb, triangular, and square lattices, that chiral spin liquids (CSLs) emerge as descendants of triple- Q spin crystals with tetrahedral magnetic order and a large scalar spin chirality. Such ordered-to-CSL melting transitions may yield lattice realizations of effective Chern-Simons-Higgs field theories. We provides a distinct unifying perspective on the emergence of CSLs and suggests that materials with certain noncoplanar magnetic orders might provide a good starting point to search for CSLs.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

Anisotropy and multiband superconductivity in Sr 2 RuO 4 determined by small-angle neutron scattering studies of the vortex lattice [Anisotropy and multiband superconductivity in Sr 2 RuO 4 ]

Despite numerous studies the exact nature of the order parameter in superconducting Sr 2 RuO 4 remains unresolved. We have extended previous small-angle neutron scattering studies of the vortex lattice in this material to a wider field range, higher temperatures, and with the field applied close to both the <100> and <110> basal plane directions. Measurements at high field were made possible by the use of both spin polarization and analysis to improve the signal-to-noise ratio. Rotating the field towards the basal plane causes a distortion of the square vortex lattice observed for H // <001> and also a symmetry change to a distorted triangular symmetry for fields close to <100>.The vortex lattice distortion allows us to determine the intrinsic superconducting anisotropy between the c axis and the Ru-O basal plane, yielding a value of ~60 at low temperature and low to intermediate fields. This greatly exceeds the upper critical field anisotropy of ~20 at low temperature, reminiscent of Pauli limiting. Indirect evidence for Pauli paramagnetic effects on the unpaired quasiparticles in the vortex cores are observed, but a direct detection lies below the measurement sensitivity. The superconducting anisotropy is found to be independent of temperature but increases for fields > 1 T, indicating multiband superconductvity in Sr 2 RuO 4 . Lastly, the temperature dependence of the scattered intensity provides further support for gap nodes or deep minima in the superconducting gap.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2017

Chiral liquid phase of simple quantum magnets

We study a T=0 quantum phase transition between a quantum paramagnetic state and a magnetically ordered state for a spin S=1 XXZ Heisenberg antiferromagnet on a two-dimensional triangular lattice. The transition is induced by an easy-plane single-ion anisotropy D. At the mean-field level, the system undergoes a direct transition at a critical D=D c between a paramagnetic state at D>D c and an ordered state with broken U(1) symmetry at D c . We show that beyond mean field the phase diagram is very different and includes an intermediate, partially ordered chiral liquid phase. Specifically, we find that inside the paramagnetic phase the Ising (J z ) component of the Heisenberg exchange binds magnons into a two-particle bound state with zero total momentum and spin. This bound state condenses at D>D c , before single-particle excitations become unstable, and gives rise to a chiral liquid phase, which spontaneously breaks spatial inversion symmetry, but leaves the spin-rotational U(1) and time-reversal symmetries intact. This chiral liquid phase is characterized by a finite vector chirality without long-range dipolar magnetic order. In our analytical treatment, the chiral phase appears for arbitrarily small J z because the magnon-magnon attraction becomes singular near the single-magnon condensation transition. This phase exists in a finite range of D and transforms into the magnetically ordered state at some D c . In conclusion, we corroborate our analytic treatment with numerical density matrix renormalization group calculations.

36 MATERIALS SCIENCE↗
DOE OSTI2017

Tuning the antiferromagnetic helical pitch length and nanoscale domain size in Fe 3 PO 4 O 3 by magnetic dilution

The insulating magnetic material Fe 3 PO 4 O 3 features a noncentrosymmetric lattice composed of Fe 3 + triangular units. Frustration, due to competing near-neighbor (J 1 ) and next-nearest-neighbor (J 2 ) antiferromagnetic interactions, was recently suggested to be the origin of an antiferromagnetic helical ground state with unusual needlelike nanoscale magnetic domains in Fe 3 PO 4 O 3 . Magnetic dilution is shown here to tune the ratio of these magnetic interactions, thus providing deeper insight into this unconventional antiferromagnet. Dilution of the Fe 3+ lattice in Fe 3 PO 4 O 3 was accomplished by substituting nonmagnetic Ga 3+ to form the solid solution series Fe 3-x Ga x PO 4 O 3 with x=0.012, 0.06, 0.25, 0.5, 1.0, 1.5. Magnetic susceptibility and neutron powder diffraction data from this series are presented. A continuous decrease of both the helical pitch length and the domain size is observed with increasing dilution up to at least x=0.25, while for x≥0.5, the compounds lack long-range magnetic order entirely. The decrease in the helical pitch length with increasing x can be qualitatively understood by reduction of the ratio of J 2 /J 1 in the Heisenberg model, consistent with mean-field considerations. Intriguingly, the magnetic correlation length in the ab plane remains nearly equal to the pitch length for each value of x≤0.25, showing that the two quantities are intrinsically connected in this unusual antiferromagnet.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Muon spin relaxation study of spin dynamics in the extended kagome systems YBaCo 4 O 7 + δ ( δ = 0 , 0.1 )

Here, we present muon spin relaxation (μSR) measurements of the extended kagome systems YBaCo 4 O 7+δ (δ = 0,0.1), comprising two interpenetrating kagome sublattice of Co(I) 3+ (S = 3/2) and a triangle sublattice of Co(II) 2+ (S = 2). The zero- and longitudinal-field μ SR spectra of the stoichiometric compound YBaCo 4 O 7 unveil that the triangular subsystem orders at TN = 101 K. In contrast, the muon spin relaxation rate pertaining to the kagome subsystem shows persistent spin dynamics down to T = 20 K and then a sublinear decrease λ(T ) ~ T 0.66(5) on cooling towards T = 4 K. In addition, the introduction of interstitial oxygen (δ = 0.1) is found to drastically affect the magnetism. For the fast-cooling experiment (>10 K/min), YBaCo 4 O 7.1 enters a regime characterized by persistent spin dynamics below 90 K. For the slow-cooling experiment (1 K/min), evidence is obtained for the phase separation into interstitial oxygen-poor and oxygen-rich regions with distinct correlation times. The observed temperature, cooling rate, and oxygen content dependencies of spin dynamics are discussed in terms of a broad range of spin-spin correlation times, relying on a different degree of frustration between the kagome and triangle sublattices as well as of oxygen migration.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Magnetic interactions in PdCrO 2 and their effects on its magnetic structure

We report a neutron scattering study of the metallic triangular lattice antiferromagnet PdCrO 2 . Powder neutron diffraction measurements confirm that the crystalline space group symmetry remains R$\bar{3}$m below T N . This implies that magnetic interactions consistent with the crystal symmetry do not stabilize the noncoplanar magnetic structure, which was one of two structures previously proposed on the basis of single crystal neutron diffraction measurements. Inelastic neutron scattering measurements find two gaps at low energies, which can be explained as arising from a dipolar-type exchange interaction. This symmetric anisotropic interaction also stabilizes a magnetic structure very similar to the coplanar magnetic structure, which was also suggested by the single crystal diffraction study. In conclusion, the higher-energy magnon dispersion can be modelled by linear spin-wave theory with exchange interactions up to sixth nearest neighbors, but discrepancies remain which hint at additional effects unexplained by the linear theory.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Full commuting projector Hamiltonians of interacting symmetry-protected topological phases of fermions

In this work, using the decorated domain wall procedure, we construct finite-depth local unitaries that realize fermionic symmetry-protected topological (SPT) phases. This results in explicit full commuting projector Hamiltonians, where "full" implies the fact that the ground state as well as all excited states of these Hamiltonians realize the nontrivial SPT phase. We begin by constructing explicit examples of 1+1D phases protected by the symmetry group G =$\mathbb{Z}_2^T$×$\mathbb{Z}_2^F$, which also has a free fermion realization in class BDI, and by the symmetry group G =$\mathbb{Z}_4$×$\mathbb{Z}_4^F$, which does not. We then turn to 2+1D, and construct the square roots of the Levin-Gu bosonic SPT phase, protected by $\mathbb{Z}_2$×$\mathbb{Z}_2^F$ symmetry, in a concrete model of fermions and spins on the triangular lattice. Edge states and the anomalous symmetry action on them are explicitly derived. Although this phase has a free fermion representation as two copies of p + ip superconductors combined with their p - ip counterparts with a different symmetry charge, the full set of commuting projectors is only realized in the strongly interacting version, which also implies that it admits a many-body localized realization.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Weak ferromagnetism and glassy state in κ - ( BEDT - TTF ) 2 Hg ( SCN ) 2 Br

SInce the first observation of weak ferromagnetism in the charge-transfer salt kappa-(BEDT-TTF)(2)Cu[N(CN)(2)]Cl [U. Welp et al., Phys. Rev. Lett. 69, 840 (1992)], no further evidence of a ferromagnetic state in this class of organic materials has been reported. Here, static and dynamic spin susceptibility measurements on kappa-(BEDT-TTF)(2)Hg(SCN)(2)Br exhibit weak ferromagnetism below 20 K on the geometrically frustrated background. Our experimental results suggest that frustrated spins in the molecular dimers suppress long-range antiferromagnetic order, forming a spin-glass-type ground state of the triangular lattice in the insulating phase which locally contains ferromagnetic polarons. Moreover, specific-heat data reveal an excess peak located around 5 K, indicating the glassy nature of the electrons as well.

Hemmida, M.↗
DOE OSTI2018

Correlations and electronic order in a two-orbital honeycomb lattice model for twisted bilayer graphene

The recent observation of superconductivity in proximity to an insulating phase in twisted bilayer graphene (TBG) at small “magic” twist angles has been linked to the existence of nearly flat bands, which make TBG a fresh playground to investigate the interplay between correlations and superconductivity. The low-energy narrow bands were shown to be well described by an effective tight-binding model on the honeycomb lattice (the dual of the triangular Moiré superlattice) with a local orbital degree of freedom. In this paper, we perform a strong-coupling analysis of the proposed (p x ,p y ) two-orbital extended Hubbard model on the honeycomb lattice. By decomposing the interacting terms in the particle-particle and particle-hole channels, we classify the different possible superconducting, magnetic, and charge instabilities of the system. In the pairing case, we pay particular attention to the two-component (d–wave) pairing channels, which admit vestigial phases with nematic or chiral orders, and study their phenomenology. Furthermore, we explore the strong-coupling regime by obtaining a simplified spin-orbital exchange model which may describe a putative Mott-type insulating state at quarter-filling. Our mean-field solution reveals a rich intertwinement between ferromagnetic and antiferromagnetic orders with different types of nematic and magnetic orbital orders. Altogether, our work provides a solid framework for further investigations of the phase diagram of the two-orbital extended Hubbard model in both strong- and weak-coupling regimes.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Intertwined superfluidity and density wave order in a p -orbital Bose condensate

We study a continuum model of the weakly interacting Bose gas in the presence of an external field with minima forming a triangular lattice. The second lowest band of the single-particle spectrum ( p band) has three minima at nonzero momenta. We consider a metastable Bose condensate at these momenta and find that, in the presence of interactions that vary slowly over the lattice spacing, the order parameter space is isomorphic to S 5 . We show that the enlarged symmetry leads to the loss of topologically stable vortices, as well as two extra gapless modes with quadratic dispersion. Here, the former feature implies that this non-Abelian condensate is a “failed superfluid” that does not undergo a Berezinskii-Kosterlitz-Thouless (BKT) transition. Order-by-disorder splitting appears suppressed, implying that signatures of the S 5 manifold ought to be observable at low temperatures.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2019

Chemical disorder and spin-liquid-like magnetism in the van der Waals layered 5 d transition metal halide Os 0.55 Cl 2

Here, single crystals of the van der Waals layered 5d transition-metal compound Os 0.55 Cl 2 were grown and characterized by x-ray diffraction, magnetization and heat-capacity measurements, and atomic resolution electron microscopy. The crystals are stable in air and easily cleaved. The structure is derived from the CdCl 2 structure type, with triangular layers of transition metal sites coordinated by edge-sharing octahedra of Cl and separated by a van der Waals gap. On average, only 55% of the metal sites are occupied by Os, and evidence for short- and long-ranged vacancy orders is observed by diffraction and real-space imaging. Magnetization data indicate magnetocrystalline anisotropy due to spin-orbit coupling, antiferromagnetic correlations, and no sign of magnetic order or spin freezing down to 0.4 K. Heat-capacity measurements in applied magnetic fields show only a broad, field-dependent anomaly. The magnetic susceptibility and heat capacity obey power laws at low temperature and low field with exponents close to 0.5. The power law behaviors of the low-temperature heat capacity and magnetic susceptibility suggest gapless magnetic fluctuations prevent spin freezing or ordering in Os 0.55 Cl 2 . Divergence of the magnetic Gruneisen parameter indicates nearness to a magnetic quantum critical point. Similarities to behaviors of spin-liquid materials are noted, and in total the findings suggest Os 0.55 Cl 2 may be an example of a quantum spin liquid in the limit of strong chemical disorder.

36 MATERIALS SCIENCE↗
DOE OSTI2019

Examination of flow and nonflow factorization methods in small collision systems

Two-particle correlations have been used extensively to study hydrodynamic flow patterns in heavy-ion collisions. In small collision systems, such as $p + p$ and $p + A$, where particle multiplicities are much smaller than in $A + A$ collisions, nonflow effects from jet correlations, momentum conservation, particle decays, etc. can be significant, even when imposing a large pseudorapidity gap between the particles. A number of techniques to subtract the nonflow contribution in two-particle correlations have been developed by experiments at the CERN Large Hadron Collider (LHC) and then used to measure particle flow in $p + p$ and $p + Pb$ collisions. Recently, experiments at the BNL Relativistic Heavy Ion Collider (RHIC) have explored the possibility of adopting these techniques for small collision systems at lower energies. In this paper, we test these techniques using Monte Carlo generators pythia and hijing, which do not include any collective flow, and ampt, which does. We find that it is crucial to examine the results of such tests both for correlations integrated over particle transverse momentum $p_T$ and differentially as a function of $p_T$. Our results indicate reasonable nonflow subtraction for $p + p$ collisions at the highest LHC energies, while failing if applied to $p + p$ collisions at RHIC. In the case of $p + Au$ collisions at RHIC, both hijing and ampt results indicate a substantial over-estimate of nonflow for $p_T ≳ GeV/c$ and hence an underestimate of elliptic flow and overestimate of triangular flow.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2020

Disentangling contributions to small-system collectivity via scans of light nucleus-nucleus collisions

The observation of multiparticle azimuthal correlations in high-energy small-system collisions has led to intense debate on its origin and the possible coexistence from two competing theoretical scenarios: one based on initial-state intrinsic momentum anisotropy, and the other based on final-state interaction model (FSM) collective response to the collision geometry. To complement the previous scan of asymmetric collision systems ( p +Au, d +Au, and He+Au), we propose a scan of small symmetric collision systems at the Brookhaven National Laboratory Relativistic Heavy Ion Collider, such as C+C, O+O, Al+Al, and Ar+Ar$\sqrt{s_\text{NN}}$ = 0.2 TeV , to provide further insights in disentangling contributions from these two scenarios. These symmetric small systems have the advantage of providing a better controlled initial geometry dominated by the average shape of the overlap region as opposed to fluctuation-driven geometries in asymmetric systems. In this work, a transport model is employed to investigate the expected geometry response in the FSM scenario. Different trends of elliptic flow with increasing charge particle multiplicity are observed between symmetric and asymmetric systems, whereas triangular flow appears to show a similar behavior. Furthermore, a comparison of O+O collisions at $\sqrt{s_\text{NN}}$ = 0.2 TeV and at $\sqrt{s_\text{NN}}$ = 2.76 ₋ 7 TeV as proposed at the CERN Large Hadron Collider, provides a unique opportunity to disentangle the collision geometry effects at the nucleon level from those arising from subnucleon fluctuations.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2021

Gluonic hot spot initial conditions in heavy-ion collisions

The initial conditions in heavy-ion collisions are calculated in many different frameworks. The importance of nucleon position fluctuations within the nucleus and subnucleon structure has been established when modeling initial conditions for input to hydrodynamic calculations. However, there remain outstanding puzzles regarding these initial conditions, including the measurement of the near equivalence of the elliptical v 2 and triangular v 3 flow coefficients in ultracentral 0–1% Pb + Pb collisions at the CERN Large Hadron Collider. Recently a calculation termed magma incorporating gluonic hot spots via two-point correlators in the color glass condensate framework, and no nucleons, provided a simultaneous match to these flow coefficients measured by the ATLAS experiment, including in ultracentral 0–1% collisions. Our calculations reveal that the magma initial conditions do not describe the experimental data when run through full hydrodynamic sonic simulations or when the hot spots from one nucleus resolve hot spots from the other nucleus, as predicted in the color glass condensate framework. Finally, we also explore alternative initial condition calculations and discuss their implications.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗