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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,351 records · Page 75
All sourcesNASA NTRSDOE OSTI
DOE OSTI2014

Biodegradation test of SPS-LS blends as polymer electrolyte membrane fuel cells

Sulfonated polystyrene (SPS) can be applied as a proton exchange membrane fuel cell due to its fairly good chemical stability. In order to be applied as polymer electrolyte membrane fuel cells (PEMFCs), membrane polymer should have a good ionic conductivity, high proton conductivity, and high mechanical strength. Lignosulfonate (LS) is a complex biopolymer which has crosslinks and sulfonate groups. SPS-LS blends with addition of SiO{sub 2} are used to increase the proton conductivity and to improve the mechanical properties and thermal stability. However, the biodegradation test of SPS-LS blends is required to determine whether the application of these membranes to be applied as an environmentally friendly membrane. In this study, had been done the synthesis of SPS, biodegradability test of SPS-LS blends with variations of LS and SiO{sub 2} compositions. The biodegradation test was carried out in solid medium of Luria Bertani (LB) with an activated sludge used as a source of microorganism at incubation temperature of 37°C. Based on the results obtained indicated that SPS-LS-SiO{sub 2} blends are more decomposed by microorganism than SPS-LS blends. This result is supported by analysis of weight reduction percentage, functional groups with Fourier Transform Infrared (FTIR) Spectroscopy, and morphological surface with Scanning Electron Microscopy (SEM)

36 MATERIALS SCIENCE↗
DOE OSTI2014

Excluded volume and ion-ion correlation effects on the ionic atmosphere around B-DNA: Theory, simulations, and experiments

The ionic atmosphere around a nucleic acid regulates its stability in aqueous salt solutions. One major source of complexity in biological activities involving nucleic acids arises from the strong influence of the surrounding ions and water molecules on their structural and thermodynamic properties. Here, we implement a classical density functional theory for cylindrical polyelectrolytes embedded in aqueous electrolytes containing explicit (neutral hard sphere) water molecules at experimental solvent concentrations. Our approach allows us to include ion correlations as well as solvent and ion excluded volume effects for studying the structural and thermodynamic properties of highly charged cylindrical polyelectrolytes. Several models of size and charge asymmetric mixtures of aqueous electrolytes at physiological concentrations are studied. Our results are in good agreement with Monte Carlo simulations. Our numerical calculations display significant differences in the ion density profiles for the different aqueous electrolyte models studied. However, similar results regarding the excess number of ions adsorbed to the B-DNA molecule are predicted by our theoretical approach for different aqueous electrolyte models. These findings suggest that ion counting experimental data should not be used alone to validate the performance of aqueous DNA-electrolyte models.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2016

Inductively driven surface-plasma negative ion source for N-NBI use (invited)

The long-pulse surface-plasma source prototype is developed at Budker Institute of Nuclear Physics for negative-ion based neutral beam injector use. The essential source features are (1) an active temperature control of the ion-optical system electrodes by circulation of hot thermal fluid through the channels, drilled in the electrode bodies, (2) the concaved transverse magnetic field in the extraction and acceleration gaps, preventing the electrons trapping and avalanching, and (3) the directed cesium deposition via distribution tubes adjacent to the plasma grid periphery. The long term effect of cesium was obtained just with the single cesium deposition. The high voltage strength of ion-optical system electrodes was improved with actively heated electrodes. A stable H{sup −} beam with a current ∼1 A and energy 90 keV was routinely extracted and accelerated.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2017

Statistical mechanics of transport processes in active fluids: Equations of hydrodynamics

We present the equations of hydrodynamics including mass, linear momentum, angular momentum, and energy are derived by coarse-graining the microscopic equations of motion for systems consisting of rotary dumbbells driven by internal torques. In deriving the balance of linear momentum, we find that the symmetry of the stress tensor is broken due to the presence of non-zero torques on individual particles. The broken symmetry of the stress tensor induces internal spin in the fluid and leads us to consider the balance of internal angular momentum in addition to the usual moment of momentum. In the absence of spin, the moment of momentum is the same as the total angular momentum. In deriving the form of the balance of total angular momentum, we find the microscopic expressions for the couple stress tensor that drives the spin field. We show that the couple stress contains contributions from both intermolecular interactions and the active forces. The presence of spin leads to the idea of balance of moment of inertia due to the constant exchange of particles in a small neighborhood around a macroscopic point. We derive the associated balance of moment of inertia at the macroscale and identify the moment of inertia flux that induces its transport. Lastly, we obtain the balances of total and internal energy of the active fluid and identify the sources of heat and heat fluxes in the system.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2021

Design and evaluation of an open-source, conformable skin-cooling system for body magnetic resonance guided focused ultrasound treatments

Magnetic resonance guided focused ultrasound (MRgFUS) treatment of tumors uses inter-sonication delays to allow heat to dissipate from the skin and other near-field tissues. Despite inter-sonication delays, treatment of tumors close to the skin risks skin burns. This work has designed and evaluated an open-source, conformable, skin-cooling system for body MRgFUS treatments to reduce skin burns and enable ablation closer to the skin. A MR-compatible skin cooling system is described that features a conformable skin-cooling pad assembly with feedback control allowing continuous flow and pressure maintenance during the procedure. System performance was evaluated with hydrophone, phantom and in vivo porcine studies. Sonications were performed 10 and 5 mm from the skin surface under both control and forced convective skin-cooling conditions. 3D MR temperature imaging was acquired in real time and the accumulated thermal dose volume was measured. Gross analysis of the skin post-sonication was further performed. Device conformability was demonstrated at several body locations. Hydrophone studies demonstrated no beam aberration, but a 5–12% reduction of the peak pressure due to the presence of the skin-cooling pad assembly in the acoustic near field. Phantom evaluation demonstrated there is no MR temperature imaging precision reduction or any other artifacts present due to the coolant flow during MRgFUS sonication. The porcine studies demonstrated skin burns were reduced in size or eliminated when compared to the control condition. An open-source design of an MRgFUS active skin cooling system demonstrates device conformability with a reduction of skin burns while ablating superficial tissues.

60 APPLIED LIFE SCIENCES↗
DOE OSTI2012

ARE OUTFLOWS BIASING SINGLE-EPOCH C IV BLACK HOLE MASS ESTIMATES?

We use a combination of reverberation mapping data and single-epoch (SE) spectra of the C IV emission line in a sample of both low- and high-redshift active galactic nuclei to investigate sources of the discrepancies between C IV- and H{beta}-based SE black hole (BH) mass estimates. We find that for all reverberation mapped sources, there is a component of the line profile that does not reverberate, and the velocity characteristics of this component vary from object to object. The differing strength and properties of this non-variable component are responsible for much of the scatter in C IV-based BH masses compared to H{beta} masses. The C IV mass bias introduced by this non-variable component is correlated with the shape of the C IV line, allowing us to make an empirical correction to the BH mass estimates. Using this correction and accounting for other sources of scatter, such as poor data quality and data inhomogeneity, reduces the scatter between the C IV and H{beta} masses in our sample by a factor of {approx}2, to only {approx}0.2 dex. We discuss the possibility that this non-variable C IV component originates in an orientation-dependent outflow from either the proposed broad-line region disk wind or the intermediate-line region, a high-velocity inner extension of the narrow-line region.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Active galactic nucleus X-ray variability in the XMM-COSMOS survey

We used the observations carried out by XMM in the COSMOS field over 3.5 yr to study the long term variability of a large sample of active galactic nuclei (AGNs) (638 sources) in a wide range of redshifts (0.1 < z < 3.5) and X-ray luminosities (10{sup 41} < L {sub 0.5-10} <10{sup 45.5}). Both a simple statistical method to assess the significance of variability and the Normalized Excess Variance (σ{sub rms}{sup 2}) parameter were used to obtain a quantitative measurement of the variability. Variability is found to be prevalent in most AGNs, whenever we have good statistics to measure it, and no significant differences between type 1 and type 2 AGNs were found. A flat (slope –0.23 ± 0.03) anti-correlation between σ{sub rms}{sup 2} and X-ray luminosity is found when all significantly variable sources are considered together. When divided into three redshift bins, the anti-correlation becomes stronger and evolving with z, with higher redshift AGNs being more variable. We prove, however, that this effect is due to the pre-selection of variable sources: when considering all of the sources with an available σ{sub rms}{sup 2} measurement, the evolution in redshift disappears. For the first time, we were also able to study long term X-ray variability as a function of M {sub BH} and Eddington ratio for a large sample of AGNs spanning a wide range of redshifts. An anti-correlation between σ{sub rms}{sup 2} and M {sub BH} is found, with the same slope of anti-correlation between σ{sub rms}{sup 2} and X-ray luminosity, suggesting that the latter may be a by-product of the former. No clear correlation is found between σ{sub rms}{sup 2} and the Eddington ratio in our sample. Finally, no correlation is found between the X-ray σ{sub rms}{sup 2} and optical variability.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2014

Merger signatures in the galaxy cluster A98

We present results from Chandra and XMM-Newton observations of Abell 98 (A98), a galaxy cluster with three major components: a relatively bright subcluster to the north (A98N), a disturbed subcluster to the south (A98S), and a fainter subcluster to the far south (A98SS). We find evidence for surface brightness and temperature asymmetries in A98N consistent with a shock-heated region to the south, which could be created by an early stage merger between A98N and A98S. Deeper observations are required to confirm this result. We also find that A98S has an asymmetric core temperature structure, likely due to a separate ongoing merger. Evidence for this is also seen in optical data. A98S hosts a wide-angle tail radio source powered by a central active galactic nucleus (AGN). We find evidence for a cavity in the intracluster medium that has been evacuated by one of the radio lobes, suggesting that AGN feedback is operating in this system. Examples of cavities in non-cool core clusters are relatively rare. The three subclusters lie along a line in projection, suggesting the presence of a large-scale filament. We observe emission along the filament between A98N and A98S, and a surface brightness profile shows emission consistent with the overlap of the subcluster extended gas halos. We find the temperature of this region is consistent with the temperature of the gas at similar radii outside this bridge region. Lastly, we examine the cluster dynamics using optical data. We conclude A98N and A98S are likely bound to one another with a 67% probability, while A98S and A98SS are not bound at a high level of significance.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

The magnetic field and polarization properties of radio galaxies in different accretion states

We use the integrated polarized radio emission at 1.4 GHz (Π{sub 1.4 GHz}) from a large sample of active galactic nuclei (AGN; 796 sources at redshifts z<0.7) to study the large-scale magnetic field properties of radio galaxies in relation to the host galaxy accretion state. We find a fundamental difference in Π{sub 1.4 GHz} between radiative-mode AGN (i.e., high-excitation radio galaxies (HERGs) and radio-loud QSOs) and jet-mode AGN (i.e., low-excitation radio galaxies (LERGs)). While LERGs can achieve a wide range of Π{sub 1.4 GHz} (up to ∼30%), the HERGs and radio-loud QSOs are limited to Π{sub 1.4 GHz}≲15%. A difference in Π{sub 1.4 GHz} is also seen when the sample is divided at 0.5% of the total Eddington-scaled accretion rate, where the weakly accreting sources can attain higher values of Π{sub 1.4 GHz}. We do not find any clear evidence that this is driven by intrinsic magnetic field differences of the different radio morphological classes. Instead, we attribute the differences in Π{sub 1.4 GHz} to the local environments of the radio sources, in terms of both the ambient gas density and the magnetoionic properties of this gas. Thus, not only are different large-scale gaseous environments potentially responsible for the different accretion states of HERGs and LERGs, we argue that the large-scale magnetized environments may also be important for the formation of powerful AGN jets. Upcoming high angular resolution and broadband radio polarization surveys will provide the high-precision Faraday rotation measure and depolarization data required to robustly test this claim.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2015

The dense filamentary giant molecular cloud G23.0–0.4: Birthplace of ongoing massive star formation

We present observations of 1.5 square degree maps of the {sup 12}CO, {sup 13}CO, and C{sup 18}O (J = 1 − 0) emission toward the complex region of the supernova remnant (SNR) W41 and SNR G22.7–0.2. A massive (∼5×10{sup 5} M{sub ⊙}), large (∼84 × 15 pc), and dense (∼10{sup 3} cm{sup −3}) giant molecular cloud (GMC), G23.0–0.4 with V{sub LSR} ∼ 77 km s{sup −1}, is found to be adjacent to the two SNRs. The GMC displays a filamentary structure approximately along the Galactic plane. The filamentary structure of the dense molecular gas, traced by C{sup 18}O (J = 1 − 0) emission, is also coincident well with the distribution of the dust-continuum emission in the direction. Two dense massive MC clumps, two 6.7 GHz methanol masers, and one H ii/SNR complex, associated with the 77 km s{sup −1} GMC G23.0–0.4, are aligned along the filamentary structure, indicating the star-forming activity within the GMC. These sources have periodic projected spacing of 0.°18–0.°26 along the giant filament, which is consistent with the theoretical predictions of 0.°22. This indicates that the turbulence seems to dominate the fragmentation process of the dense gaseous filament on a large scale. The established 4.4 kpc distance of the GMC and the long dense filament traced by C{sup 18}O emission, together with the rich massive star-formation groups in the nearby region, suggest that G23.0–0.4 is probably located at the near side of the Scutum–Centaurus arm in the first quadrant. Considering the large scale and the elongation structure along the Galactic plane, we speculate that the dense filamentary GMC is related to the spiral density wave of the Milky Way.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2013

DENSE OPTICAL AND NEAR-INFRARED MONITORING OF CTA 102 DURING HIGH STATE IN 2012 WITH OISTER: DETECTION OF INTRA-NIGHT ''ORPHAN POLARIZED FLUX FLARE''

CTA 102, classified as a flat spectrum radio quasar at z = 1.037, produced an exceptionally bright optical flare in 2012 September. Following the Fermi Large Area Telescope detection of enhanced {gamma}-ray activity, we closely monitored this source in the optical and near-infrared bands for the 10 subsequent nights using 12 telescopes in Japan and South Africa. On MJD 56197 (2012 September 27, four to five days after the peak of bright {gamma}-ray flare), polarized flux showed a transient increase, while total flux and polarization angle (PA) remained almost constant during the ''orphan polarized-flux flare.'' We also detected an intra-night and prominent flare on MJD 56202. The total and polarized fluxes showed quite similar temporal variations, but the PA again remained constant during the flare. Interestingly, the PAs during the two flares were significantly different from the jet direction. The emergence of a new emission component with a high polarization degree (PD) up to 40% would be responsible for the observed two flares, and such a high PD indicates the presence of a highly ordered magnetic field at the emission site. We argue that the well-ordered magnetic field and even the observed directions of the PA, which is grossly perpendicular to the jet, are reasonably accounted for by transverse shock(s) propagating down the jet.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2023

$κ$monty: a Monte Carlo Compton scattering code including non-thermal electrons

Low-luminosity active galactic nuclei are strong sources of X-ray emission produced by Compton scattering originating from the accretion flows surrounding their supermassive black holes. The shape and energy of the resulting spectrum depend on the shape of the underlying electron distribution function (DF). In this work, we present an extended version of the GRMONTY code, called ΚMONTY. The GRMONTY code previously only included a thermal Maxwell–Jütner electron DF. We extend the GRMONTY code with non-thermal electron DFs, namely the κ and power-law DFs, implement Cartesian Kerr–Schild coordinates, accelerate the code with MPI, and couple the code to the non-uniform adaptive mesh refinement grid data from the general relativistic magnetohydrodynamics code BHAC. For the Compton scattering process, we derive two sampling kernels for both DFs. Finally, we present a series of code tests to verify the accuracy of our schemes. The implementation of non-thermal DFs opens the possibility of studying the effect of non-thermal emission on previously developed black hole accretion models.

79 ASTRONOMY AND ASTROPHYSICS↗
DOE OSTI2019

Quantum secret sharing with polarization-entangled photon pairs

Here, we describe and experimentally demonstrate a more practical three-party quantum secret sharing (QSS) protocol using polarization-entangled photon pairs. The source itself serves as an active participant and can switch between the required photon states by modulating the pump beam only, thereby making the protocol less susceptible to loss and amenable to fast switching. We derive a security proof based on quantum key distribution, demonstrating our QSS protocol to be secure against both eavesdropping and dishonest participants. Compared to three-photon protocols, the practical efficiency is dramatically improved as there is no need to generate, transmit, or detect a third photon.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2025

Bacteria export alarmone synthetases that produce (p)ppApp and (p)ppGpp

Guanosine penta- and tetraphosphate [(p)ppGpp] and their adenosine analogs [(p)ppApp] are bacterial second messengers known as alarmones. Members of the RelA-SpoT homolog (RSH) family synthesize (p)ppGpp to mediate the stringent response during nutrient starvation, whereas (p)ppApp synthetases have been identified as bactericidal toxins in diverse contexts including type VI secretion systems, toxin-antitoxin modules, and phages. Although alarmone synthesis has traditionally been viewed as a cytoplasmic process, early studies in Streptomyces suggested the existence of secreted alarmone synthetases. Here, we identify SaEAS, an exported alarmone synthetase (EAS) from Streptomyces albidoflavus, as the long-mysterious source of extracellular alarmone synthetase activity in Streptomyces. SaEAS produces both (p)ppGpp and (p)ppApp at rates exceeding 100,000 molecules per minute and has kinetic properties adapted to low substrate environments. A broader bioinformatic survey reveals ~600 EASs linked to a range of specialized bacterial secretion systems. Characterization of two additional EASs, VpEAS from Vibrio parahaemolyticus and AaEAS from Amycolatopsis azurea, shows that both produce (p)ppGpp exclusively and inhibit bacterial growth when localized to the cytoplasm. These findings challenge the longstanding view of (p)ppGpp as strictly pro-survival and unveil a diverse family of secreted RSH enzymes with potential roles in interbacterial antagonism and environmental signaling.

Ahmad, Shehryar↗
DOE OSTI2024

Control And Optimization Modular Modeling Application For Nuclear Deployment

The purpose of the COMMAND code is to provide a flexible, scalable tool for use in developing, integrating, and testing the technologies necessary for achieving autonomous operations of advanced nuclear reactors. The code enables users to efficiently implement custom simulations and experiments by combining key methods from different software modules. These modules are focused on: modeling and simulation tools, such as nuclear simulation tools used for high-fidelity modeling (e.g., Reactor Excursion and Leak Analysis Program [RELAP5-3D] and Monte Carlo N-Particle [MCNP]); machine learning and optimization tools (e.g., anomaly detection and data-driven modeling techniques); advanced control in its digital, high-performance, and supervisory control forms (e.g., proportional integral derivative (PID) control and model predictive control (MPC); and integration with hardware through industrial communication protocols. To ensure flexibility and scalability, COMMAND was designed to be both modular—the software “pieces” all inherit from generic building blocks and can be combined and connected to create complicated simulations—and high performing—designed for parallel processing, enabling simulations and experiments to take advantage of multi-core computers, servers, and nodes. The code is written in the Python programming language due to the language's popularity, active community, and open-source and cross-platform nature. Maintaining consistency with other simulation tools used within the nuclear energy community, users implement simulations and experiments through text input files, which define components, parameters, connections, etc., through lines of text. Given that COMMAND is written in Python, these input files are native Python scripts, and so use the standard Python structure and formatting. This also enables users to take advantage of Python's extensive package library to develop custom capabilities for their specific use cases.

Faber, Jacob [Idaho National Laboratory (INL), Ida↗
DOE OSTI2018

Nanoindentation of high-purity vapor deposited lithium films: A mechanistic rationalization of the transition from diffusion to dislocation-mediated flow

Nanoindentation experiments performed in high-purity vapor deposited lithium films at 31 °C reveal a strain rate and length scale dependence in the stress at which pop-in type events signal an abrupt transition from diffusion to dislocation-mediated flow. The stress level at which the transition to dislocation-mediated flow occurs varies with the strain rate and ranges from 88 to 208 times larger than the nominal yield strength of bulk, polycrystalline lithium. Variation in the indentation strain rate reveals the relationship between the stress required to initiate the transition and the length scale at which the transition occurs follows the power-law relation, hardness × depth 1.17 = 1.545 N/m 0.83 , where the magnitude of the exponent and constant reflect the defect structure of the film. In conclusion, a rationalization of the transition is provided through direct comparisons between the measured cumulative distribution function (CDF) and the CDF hypothesized for the activation of a Frank–Read source.

36 MATERIALS SCIENCE↗
DOE OSTI2012

Improved capture gamma-ray libraries for nuclear applications

The neutron-capture reaction is of fundamental use in identifying and analyzing the γ-ray spectrum from an unknown object as it gives unambiguous information on exactly what isotopes are absorbing the neutrons. There are many applications where this can be used passively (nonproliferation), or actively where an external neutron source is used to probe an unknown assembly (planetary studies).

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗
DOE OSTI2016

SNL API-653 In-Service Tank Inspection and Evaluation Tank ID: 981-A2-T0 (West)

An API Standard 653 In-Service inspection was completed on Tank 981-A2-T0 (West) located at the Sandia National Laboratories TAIV tank farm in Albuquerque, NM on September 22, 2015. The inspection was completed to collect data to evaluate the mechanical integrity and fitness for continued service of the tank. No indication or records of any previous inspection were identified for this tank. The inspection and engineering evaluation were completed using API-653, 5 th Edition and conservative engineering practices. The tank was not removed from service, so an internal inspection could not be completed. The tank was also fully insulated. The insulation was removed in specified areas of the tank shell and tank chime to accommodate an acoustic emission scan of the tank and an ultrasonic thickness evaluation of portions of the tank. The acoustic emission scan resulted in a grade of B / I - II indicating an overall TANKPAC grade B and composite grade II indicating minor active damage with highly concentrated sources related to corrosion found in the southeast and west side section of the tank. Eight Potential Localized Damage sources were found mainly in the west side (re-test in 2 years). The tank chime could not be inspected due to the configuration of the insulation welded angle support. An ultrasonic guided bulk wave inspection was completed on the tank shell to assess the lower shell section. At the time of the inspection the limited data collected showed minimal material loss from the shell at the thickness monitoring locations, however, visual inspection and pit depth gauge measurements showed > 3/16” inch pitting and significant general external surface corrosion on the shell at the shell to floor joint. This corrosion is caused by the insulation sheeting support welded angle iron trapping moisture and dirt against the tank shell. This tank should be removed from service, internally inspected, and repaired. Ultrasonic thickness measurement locations were established on this tank and the data is included in this report. The limited data collected indicated minimal material loss at these locations, with the only noted corrosion occurring on the tank shell to floor joint as noted above. An API-653 Annex B Evaluation of Tank Bottom Settlement was completed and the results are included in this report. No significant settlement issues were identified.

42 ENGINEERING↗