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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 1,369 records · Page 76
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

Electron Spin-Polarization Dependent Damage to Chiral Amino Acid l-Histidine

The damage of approximately monolayer films of L-histidine by low-energy spin-polarized electrons (SPE) ejected from a magnetized cobalt substrate has been probed using X-ray photoelectron spectroscopy (XPS). Average damage cross sections for N-containing motifs of L-histidine are 25-30 and 2-5 Mb for zwitterions and neutral molecules, respectively. Here, the magnetization direction of the substrate, which controls the ejected SPE helicity, was reversed in situ, and statistically significant differences in the damage cross sections of 10-30% were measured between positive and negative electron helicities. This is the first measurement of spin dichroism (SD) in an amino acid. The differential cross sections suggest that inelastic scattering of SPE with chiral molecules could contribute to the persistence of one enantiomer vs the other under certain irradiation conditions, particularly for the zwitterionic species.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2015

Constraining Data Mining with Physical Models: Voltage- and Oxygen Pressure-Dependent Transport in Multiferroic Nanostructures

Development of new generation electronic devices requires understanding and controlling the electronic transport in ferroic, magnetic, and optical materials, which is hampered by two factors. First, the complications of working at the nanoscale, where interfaces, grain boundaries, defects, and so forth, dictate the macroscopic characteristics. Second, the convolution of the response signals stemming from the fact that several physical processes may be activated simultaneously. Here, we present a method of solving these challenges via a combination of atomic force microscopy and data mining analysis techniques. Rational selection of the latter allows application of physical constraints and enables direct interpretation of the statistically significant behaviors in the framework of the chosen physical model, thus distilling physical meaning out of raw data. We demonstrate our approach with an example of deconvolution of complex transport behavior in a bismuth ferrite–cobalt ferrite nanocomposite in ambient and ultrahigh vacuum environments. Measured signal is apportioned into four electronic transport patterns, showing different dependence on partial oxygen and water vapor pressure. These patterns are described in terms of Ohmic conductance and Schottky emission models in the light of surface electrochemistry. Finally and furthermore, deep data analysis allows extraction of local dopant concentrations and barrier heights empowering our understanding of the underlying dynamic mechanisms of resistive switching.

36 MATERIALS SCIENCE↗
DOE OSTI2016

Spin–orbit torque-assisted switching in magnetic insulator thin films with perpendicular magnetic anisotropy

As an in-plane charge current flows in a heavy metal film with spin-orbit coupling, it produces a torque on and thereby switches the magnetization in a neighbouring ferromagnetic metal film. Such spin-orbit torque (SOT)-induced switching has been studied extensively in recent years and has shown higher efficiency than switching using conventional spin-transfer torque. Here we report the SOT-assisted switching in heavy metal/magnetic insulator systems. The experiments used a Pt/BaFe 12 O 19 bilayer where the BaFe 12 O 19 layer exhibits perpendicular magnetic anisotropy. As a charge current is passed through the Pt film, it produces a SOT that can control the up and down states of the remnant magnetization in the BaFe 12 O 19 film when the film is magnetized by an in-plane magnetic field. Furthermore, it can reduce or increase the switching field of the BaFe 12 O 19 film by as much as about 500 Oe when the film is switched with an out-of-plane field.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2018

Biexcitons in monolayer transition metal dichalcogenides tuned by magnetic fields

Abstract We present time-integrated four-wave mixing measurements on monolayer MoSe 2 in magnetic fields up to 25 T. The experimental data together with time-dependent density function theory calculations provide interesting insights into the biexciton formation and dynamics. In the presence of magnetic fields the coherence at negative and positive time delays is dominated by intervalley biexcitons. We demonstrate that magnetic fields can serve as a control to enhance the biexciton formation and help search for more exotic states of matter, including the creation of multiple exciton complexes and excitonic condensates.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2019

Elastic colloidal monopoles and reconfigurable self-assembly in liquid crystals

Monopole-like electrostatic interactions are ubiquitous in condensed matter, but they are often screened by counter-ions and cannot be switched from attractive to repulsive. In colloidal science, where the main goal is to develop colloidal particles that mimic and exceed the diversity and length scales of atomic and molecular assembly, electrostatically charged particles cannot change the sign of their surface charge or transform from monopoles to higher-order multipoles. In liquid-crystal colloids, elastic interactions between particles arise to minimize the free energy associated with elastic distortions in the long-range alignment of rod-like molecules around the particles. In dipolar quadrupolar and hexadecapolar nematic colloids, the symmetries of such elastic distortions mimic both electrostatic multipoles and the outermost occupied electron shells of atoms. Electric and magnetic switching, spontaneous transformations and optical control of elastic multipoles, as well as their interactions with topological defects and surface boundary conditions, have been demonstrated in such colloids. However, it has long been understood that elastic monopoles should relax to uniform or higher-order multipole states because of the elastic torques that they induce. We develop nematic colloids with strong elastic monopole moments and with elastic torques balanced by the optical torques induced by ambient light. We demonstrate the monopole-to-quadrupole reconfiguration of these colloidal particles by unstructured light, which resembles the driving of atoms between the ground state and various excited states. We show that the sign of the elastic monopoles can be switched, and that like-charged monopoles attract whereas oppositely charged ones repel, unlike in electrostatics. We also demonstrate the out-of-equilibrium dynamic assembly of these colloidal particles. This diverse and surprising behaviour is explained using a model that considers the balance of the optical and elastic torques that are responsible for the excited-state elastic monopoles and may lead to light-powered active-matter systems and self-assembled nanomachines.

36 MATERIALS SCIENCE↗
DOE OSTI2018

Reversible Fe(II) uptake/release by magnetite nanoparticles

Magnetite commonly coexists with aqueous Fe2+ (Fe2+(aq)) in anoxic subsurface environments. Complex interactions between magnetite and Fe2+(aq) profoundly impact redox potential fluctuations in surrounding environment and biogeochemical cycles of important elements and contaminants. However, the ability of magnetite to act as a source/sink of electron equivalents through fluctuations in solution pH or the activity of Fe2+(aq) remains poorly quantified. We systematically studied the interrelationships between equilibrium Fe2+(aq) concentrations and structural versus surface-localized Fe?II)/Fe?III) ratios in magnetite using micro X-ray diffraction and synchrotron-based X-ray magnetic circular dichroism, respectively, under different controlled experimental conditions. Relative to pH 7, at pH 6 proton-promoted dissolution yields Fe2+(aq) release from magnetite nanoparticles, coupled to a decrease in the structural Fe?II)/Fe?III) ratio by electron hopping along the octahedral sublattice from the particle interior to the surface. At pH 8, magnetite sorbs Fe2+(aq), increasing both the structural and surface-localized Fe?II)/Fe?III) ratio. Amendments of Fe2+(aq) inhibit acidic Fe2+(aq) release and promote Fe2+(aq) uptake at more basic conditions, whereas increasing magnetite loading facilitates Fe2+(aq)–magnetite interaction at the same respective pH extremes. The reversible flow of Fe?II) across the magnetite–solution interface under different conditions implies that the redox reactivity of magnetite nanoparticles is quickly responsive to changes in environmental conditions, such as an increase in pH due to groundwater passing through carbonate-rich rocks, via a dynamic redistribution of electron equivalents between particle interiors and the solid/water interface.

Peng, Huan↗
DOE OSTI2015

Exchange bias in zinc ferrite-FeNiMoB based metallic glass composite thin films

The Exchange bias phenomenon and methods to manipulate the bias field in a controlled manner are thrust areas in magnetism due to its sophisticated theoretical concepts as well as advanced technological utility in the field of spintronics. The Exchange bias effect is observed as a result of ferromagnetic-antiferromagnetic (FM-AFM) exchange interaction, usually observed as a loop shift on field cooling below the Neel temperature of AFM. In the present study, we have chosen zinc ferrite which is a well known antiferromagnet, and FeNiMoB based metallic glass as the ferromagnet. The films were prepared by RF sputtering technique. The thickness and composition was obtained by RBS. The magnetic studies using SQUID VSM indicate exchange bias effect in the system. The effect of thermal annealing on exchange bias effect was studied. The observed exchange bias in the zinc ferrite-FeNiMoB system is not due to FM-AFM coupling but due to spin glass-ferromagnetic interaction.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
DOE OSTI2015

Unusual spin correlations in a nanomagnet

We show how atomic-scale exchange phenomena can be controlled and exploited in nanoscale itinerant magnets to substantially improve magnetic properties. Cluster-deposition experiments, first-principle simulations, and analytical calculations are used to demonstrate the effect in Co{sub 2}Si nanoclusters, which have average sizes varying from about 0.6 to 29.5 nm. The cluster-deposited nanoparticles exhibit average magnetic moments of up to 0.70 μ{sub B}/Co at 10 K and 0.49 μ{sub B}/Co at 300 K with appreciable magnetocrystalline anisotropies, in sharp contrast to the nearly vanishing bulk magnetization. The underlying spin correlations and associated cluster-size dependence of the magnetization are explained by a surface induced ferromagnetic spin polarization with a decay length of the order of 1 nm, much larger than the nearest-neighbor interatomic distance in the alloy.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2020

Modification of terahertz emission spectrum using microfabricated spintronic emitters

Terahertz (THz) radiation with sub-millimeter wavelength falls in the gap between optical and radio frequencies. Conventional THz emitters do not intertwine with spin degrees of freedom. However, it was recently shown that broadband THz radiation can be efficiently created also by exploiting spin-based effects on ultrafast time scales. Here, we demonstrate the generation and control of THz radiation from microstructured spintronic THz emitters based on the inverse spin-Hall effect. Using time-domain THz spectroscopy, we compare the THz spectra of different stripe patterns made of Fe/Pt bilayers with a spectrum obtained from an extended Fe/Pt bilayer film. It is found that the THz spectrum can be altered by a proper choice of the microstructure dimensions. The experimentally observed spectra are interpreted in terms of a simplified multi-slit interference model, which captures the main experimental features. Our results pave the way for an efficient control of THz light emitted from magnetic heterostructures. This is a crucial step forward for the design and realization of directional THz sources.

Wu, Weipeng↗
DOE OSTI2022

In-situ tunable giant electrical anisotropy in a grating gated AlGaN/GaN two-dimensional electron gas.

Materials with in-plane electrical anisotropy have great potential for designing artificial synaptic devices. However, natural materials with strong intrinsic in-plane electrical anisotropy are rare. We introduce a simple strategy to produce extremely large electrical anisotropy via grating gating of a semiconductor two-dimensional electron gas (2DEG) of AlGaN/GaN. We show that periodically modulated electric potential in the 2DEG induces in-plane electrical anisotropy, which is significantly enhanced in a magnetic field, leading to an ultra large electrical anisotropy. This is induced by a giant positive magnetoresistance and a giant negative magnetoresistance under two orthogonally oriented in-plane current flows, respectively. This giant electrical anisotropy is in situ tunable by tailoring both the grating gate voltage and the magnetic field. Our semiconductor device with controllable giant electrical anisotropy will stimulate new device applications, such as multi-terminal memtransistors and bionic synapses.

36 MATERIALS SCIENCE↗
DOE OSTI2023

Effect of aspect ratio on plasma response to resonant magnetic perturbations in tokamak devices

A systematic numerical study is carried out, computing and comparing the plasma response to the resonant magnetic perturbation (RMP) field, applied for controlling edge localized modes (ELMs), in a series of tokamak plasmas with varying aspect ratio and utilizing the MARS-F code. The aspect ratio is scanned either by varying the plasma major radius at a fixed minor radius or by varying the latter while fixing the former. Both approaches yield similar results when compared in terms of quantities with proper normalizations. In general, a non-monotonic dependence of the resonant response field (normalized by the vacuum counterpart) near the plasma edge is found with varying aspect ratio, indicating that a given ELM control coil current configuration strongly favors plasmas with a certain aspect ratio. This optimal aspect ratio, on the other hand, depends on the toroidal as well as poloidal (i.e., coil phasing) spectra of the applied RMP field. The equilibrium (edge) safety factor, the plasma shape, and the plasma toroidal flow are all fixed to ensure that the effects identified here are predominantly due to the plasma aspect ratio.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗
DOE OSTI2018

HIGH FUSION PERFORMANCE IN SUPER H-MODE EXPERIMENTS ON ALCATOR C-MOD AND DIII-D

We report that the “Super H-Mode” regime is predicted to enable pedestal height and fusion performance substantially higher than standard H-Mode operation. This regime exists due to a bifurcation of the pedestal pressure, as a function of density, that is predicted by the EPED model to occur in strongly shaped plasmas above a critical pedestal density. Experiments on Alcator C-Mod and DIII-D have achieved access to the Super H-Mode (and Near Super H) regime, and obtained very high pedestal pressure, including the highest pedestal pressure ever achieved on a tokamak (p ped ~80kPa) in C-Mod experiments operating near the ITER magnetic field. DIII-D Super H experiments have demonstrated high performance, including the highest stored energy in the present configuration of DIII-D (W~2.2-3.2MJ), while utilizing only about half of the available heating power (P heat ~7-12 MW). These DIII-D experiments have obtained the highest value of peak fusion gain, Q DT,equiv ~0.5, ever achieved on a medium scale (R<2m) tokamak. Sustained high performance operation (β N ~2.9, H 98 ~1.6) has been achieved utilizing n=3 magnetic perturbations for density and impurity control. High pedestal and global performance has been maintained in the presence of deuterium and nitrogen gas puffing, which enables a more radiative divertor condition. Lastly, Super H-Mode access is predicted for ITER and expected, based on both theoretical prediction and observed normalized performance, to allow ITER to achieve its performance goals (Q=10) at I p < 15MA, and to enable more compact, cost effective pilot plant and reactor designs.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2021

Landau Damping with Electron Lenses in Space-Charge Dominated Beams

Further progress of fundamental physics requires accelerated beams of high intensity. The intensities, however, are limited by many factors, including coherent beam instabilities. Usual methods to control the instabilities, such as octupole magnets, beam feedback dampers and employment of chromatic effects, may be ineffective or insufficient. In this study, electron lenses were proposed as a means to provide stabilizing spread in the beam betatron frequencies. It was shown that electron lenses are uniquely effective for Landau damping of transverse beam instabilities in high energy particle accelerators, and that their employment does not compromise incoherent (single particle) stability, dynamic aperture and the beam lifetime. Here we consider effectiveness of the Landau damping with electron lenses when the space charge tune shift cannot be neglected. We demonstrate that the desired stability can be assured with proper choice of the electron beam parameters and current distributions.

43 PARTICLE ACCELERATORS↗
DOE OSTI2015

Isotropic in-plane quenched disorder and dilution induce a robust nematic state in electron-doped pnictides

The phase diagram of electron-doped pnictides is studied varying the temperature, electronic density, and isotropic in-plane quenched disorder strength and dilution by means of computational techniques applied to a three-orbital (xz,yz,xy) spin-fermion model with lattice degrees of freedom. In experiments, chemical doping introduces disorder but in theoretical studies the relationship between electronic doping and the randomly located dopants, with their associated quenched disorder, is difficult to address. Moreover, in this publication, the use of computational techniques allows us to study independently the effects of electronic doping, regulated by a global chemical potential, and impurity disorder at randomly selected sites. Surprisingly, our Monte Carlo simulations reveal that the fast reduction with doping of the N eel T N and the structural T S transition temperatures, and the concomitant stabilization of a robust nematic state, is primarily controlled in our model by the magnetic dilution associated with the in-plane isotropic disorder introduced by Fe substitution. In the doping range studied, changes in the Fermi surface produced by electron doping affect only slightly both critical temperatures. Our results also suggest that the specific material-dependent phase diagrams experimentally observed could be explained as a consequence of the variation in disorder profiles introduced by the different dopants. Finally, our findings are also compatible with neutron scattering and scanning tunneling microscopy, unveiling a patchy network of locally magnetically ordered clusters with anisotropic shapes, even though the quenched disorder is locally isotropic. Our study reveals a remarkable and unexpected degree of complexity in pnictides: the fragile tendency to nematicity intrinsic of translational invariant electronic systems needs to be supplemented by quenched disorder and dilution to stabilize the robust nematic phase experimentally found in electron-doped 122 compounds.

97 MATHEMATICS AND COMPUTING↗
DOE OSTI2017

Landau Damping of Beam Instabilities by Electron Lenses

Modern and future particle accelerators employ increasingly higher intensity and brighter beams of charged particles and become operationally limited by coherent beam instabilities. Usual methods to control the instabilities, such as octupole magnets, beam feedback dampers, and use of chromatic effects, become less effective and insufficient. Here, we show that, in contrast, Lorentz forces of a low-energy, magnetically stabilized electron beam, or “electron lens,” easily introduce transverse nonlinear focusing sufficient for Landau damping of transverse beam instabilities in accelerators. It is also important to note that, unlike other nonlinear elements, the electron lens provides the frequency spread mainly at the beam core, thus allowing much higher frequency spread without lifetime degradation. For the parameters of the Future Circular Collider, a single conventional electron lens a few meters long would provide stabilization superior to tens of thousands of superconducting octupole magnets.

43 PARTICLE ACCELERATORS↗
DOE OSTI2017

Localized Control of Curie Temperature in Perovskite Oxide Film by Capping-Layer-Induced Octahedral Distortion

With reduced dimensionality, it is often easier to modify the properties of ultrathin films than their bulk counterparts. Strain engineering, usually achieved by choosing appropriate substrates, has been proven effective in controlling the properties of perovskite oxide films. An emerging alternative route for developing new multifunctional perovskite is by modification of the oxygen octahedral structure. Here we report the control of structural oxygen octahedral rotation in ultrathin perovskite SrRuO 3 films by the deposition of a SrTiO 3 capping layer, which can be lithographically patterned to achieve local control. Here, using a scanning Sagnac magnetic microscope, we show an increase in the Curie temperature of SrRuO 3 due to the suppression octahedral rotations revealed by the synchrotron x-ray diffraction. Lastly, this capping-layer-based technique may open new possibilities for developing functional oxide materials.

36 MATERIALS SCIENCE↗
DOE OSTI2024

Quantum Spin Dynamics Due to Strong Kitaev Interactions in the Triangular-Lattice Antiferromagnet CsCeSe 2

The extraordinary properties of the Kitaev model have motivated an intense search for new physics in materials that combine geometrical and bond frustration. In this Letter, we employ inelastic neutron scattering, spin wave theory, and exact diagonalization to study the spin dynamics in the perfect triangular-lattice antiferromagnet (TLAF) CsCeSe 2 . This material orders into a stripe phase, which is demonstrated to arise as a consequence of the off-diagonal bond-dependent terms in the spin Hamiltonian. By studying the spin dynamics at intermediate fields, we identify an interaction between the single-magnon state and the two-magnon continuum that causes decay of coherent magnon excitations, level repulsion, and transfer of spectral weight to the continuum that are controlled by the strength of the magnetic field. Our results provide a microscopic mechanism for the stabilization of the stripe phase in TLAF and show how complex many-body physics can be present in the spin dynamics in a magnet with strong Kitaev coupling even in an ordered ground state. Published by the American Physical Society 2024

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗