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At least 1,369 records · Page 76

Status Report for NEET In-Pile Sensor Irradiation Capabilities at TREAT

The recently-established in-pile sensor development project under the Nuclear Energy Enabling Technology (NEET) program is focused on the development of measurement technologies to enable acquisition of data focused on the performance, properties, and boundary conditions of nuclear fuels/materials under irradiation in nuclear reactors. These sensors can be used in steady state irradiation tests to measure parameters of interest under conditions representing normal nuclear plant operation, or in transient irradiation tests to determine specimen performance under postulated unplanned conditions. In either case, development of suitable sensor technologies must include instrument irradiations to help guide sensor material/design selection, verify instrument performance, and demonstrate deployment viability. The Transient Reactor Test facility (TREAT) while just a part of the overall capabilities portfolio needed to enable this sensor development mission, has unique capabilities and characteristics that make it well poised for a number of instrument irradiation data objectives including sensor survivability screening, response characterization, qualification tests, and in-situ properties measurements. TREAT’s brilliantly-basic design, when married with appropriate irradiation hardware and analytic capabilities, fills a crucial capability gap between out-of-pile testing and irradiation in steady state high power research reactors. Leveraging a recently developed approach to irradiation testing in TREAT, the present work demonstrates that cost-effective and scientifically-impactful instrument irradiation capabilities for TREAT are a well-placed capability in the NEET in-pile sensor development project.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Iodobutane Deep Bed Adsorption Test Report

The Department of Energy (DOE) Nuclear Technology Research and Development (NTRD) Program Material Recovery and Waste Form Development (MRWFD) Campaign Off-gas Sigma Team has supported research and development on iodine control and iodine waste forms for the past several years. As a part of this on-going research, two deep-bed iodobutane adsorption tests have been performed with higher NO x levels. High (>1,000) iodine decontamination factors (DFs, the ratios of the inlet iodine concentrations divided by the outlet iodine concentrations, when the gas flowrate is constant) were achieved with both the silver aerogel and silver zeolite sorbents. The iodine adsorption mass transfer zone (the depth of the sorbent bed in which adsorption is occurring at any specific time) for these tests was estimated at 4 inches for both sorbents under the test conditions. Silver utilization for silver aerogel sorbent reached 41% (up to 12 g adsorbed iodine per 100 g silver aerogel sorbent), while silver utilization reached 43% (up to 6.8 g adsorbed iodine per 100 g silver zeolite sorbent). These values are generally consistent with results for prior methyl iodide adsorption tests. The results also indicate that, during iodine adsorption process, the organic iodide molecule decomposes so that the iodine can be adsorbed. Even when sorbent breakthrough is reached, the organic iodide molecule continues to decompose; and the unadsorbed iodine that passes through bed is no longer in the form of the original organic iodide; but in the form of iodine compounds that are soluble in NaOH solutions, such as HI or I 2 . This research and development has included iodine adsorption tests using a laboratory-scale test system containing segmented fixed beds of iodine adsorbents in series. Non-radioactive synthetic gas mixtures were blended from air, nitrogen, NO, NO 2 , water, and the target iodine compounds to represent dissolver off-gas (DOG) streams from used nuclear fuel aqueous reprocessing.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Radiation hardness of the low gain avalanche diodes developed by NDL and IHEP in China

This paper presents a study on the radiation hardness of low gain avalanche detector (LGAD) developed by the Novel Device Laboratory (NDL) in Beijing and the Institute of High Energy Physics (IHEP) of Chinese Academy of Sciences, in the context of an upgrade project of the ATLAS detector for the high luminosity phase of LHC. NDL LGAD sensors with different layouts, epitaxial resistivity and doping profile were irradiated up to 1.02 × 10 15 n eq /cm 2 by 70 MeV protons at Cyclotron and Radioisotope Center (CYRIC). The timing resolution of NDL LGAD sensors reached 50 ps and the collected charge reached 3 - 4 fC after irradiation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Multiple Critical Unresolved Region Integral Experiment (MCURIE): A Proposed Integral Critical Experimental Framework for Unresolved Region and Intermediate Energies

The Critical Unresolved Region Integral Experiment (CURIE) critical experiment was performed at the National Criticality Experiments Research Center (NCERC) at the Device Assembly Facility (DAF) at the Nevada Nuclear Security Sites (NNSS) in 2020. The objective of CURIE was to improve the quality of integral nuclear data in the uranium-235 ( 235 U) unresolved resonance region (URR) by performing benchmark integral experiments that were sensitive to the URR energy ranges. The CURIE experiment was evaluated for the International Criticality Safety Benchmark Evaluation Project (ICSBEP) handbook and the benchmark evaluation was accepted in 2022. The URR is a region within the intermediate neutron energy range (the intermediate energy ranges from 0.7 eV to 100 keV). The observed resonance structure in neutron cross sections is due to discrete energy levels in the nucleus and are characterized by resonance parameters. In the URR region, the resonance parameters are only partially resolved as the resolution of the experiment techniques becomes comparable to the average width of the resonances themselves, and the resonances are so close to one another that the structure cannot be determined empirically. The ENDF/B-VIII.0 and JEFF-3.3 nuclear data libraries define the URR as beginning at 2.25 keV and continuing until 25 keV. There are minimal intermediate neutron energy benchmarks available in the ICSBEP benchmark handbook, and aside from CURIE there are none that are highly sensitive in the URR energy region. There is a current need for additional experiments sensitive to the URR energy region. There is a new proposed subgroup for the Organization for Economic Co-operation and Development and Nuclear Energy Agency (OECD NEA) Working Party on International Nuclear Data Evaluation Cooperation (WPEC), so any new models or information will need experimental validation and testing. The NEA Working Party on Nuclear Criticality Safety (WPNCS) recent experimental needs and priority list includes intermediate energy 235 U and 238 U experiments, as does the recent Integral Experiments to Address Nuclear Criticality Safety Needs Meeting (May 2023). A variant on the original CURIE experiment called the Multiple Critical Unresolved Region Integral Experiment (MCURIE) is proposed to provide further investigation of the intermediate and URR energy region for uranium. MCURIE will utilize existing fuels at NCERC but use alternative moderators and reflectors to modify the neutron absorption, scattering, and fission spectra of the experiments, allowing for precise targeting of nuclear data sensitivities. The overall goal of MCURIE is to develop a framework for designing and performing integral benchmark experiments with high sensitivities in the intermediate and URR energy regions for nuclear data validation.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Design Report on the MiniFuel Instrumented Test Apparatus for Understanding Radiation Effects

Most nuclear fuels irradiations at Oak Ridge National Laboratory (ORNL) over the past decade have been conducted using MiniFuel—a static capsule design employing subscale fuel specimens to collect separate-effects irradiated fuel performance data. Irradiation conditions for MiniFuel experiments are predicted pre-test using reactor physics, and thermal models are verified post-irradiation via SiC dilatometry and various spectrometry methods. Relevant fuel performance parameters are also observed post-irradiation in a hot cell, thereby providing a single data point for each parameter representing the cumulative effects of the irradiation conditions. Substantially more data can be harvested from a single test and within a shorter duration by instrumenting irradiation vehicles and measuring desired quantities in situ. This report presents the design and analysis of the MiniFuel INstrumented Irradiation Test Apparatus for Understanding Radiation Effects (MINITAURE)—an instrumented test rig based on the separate-effects MiniFuel concept that aims to capture fission gas release (FGR) and thermal conductivity degradation of fuel specimens during irradiation in the High Flux Isotope Reactor (HFIR). MINITAURE will be integrated with the Materials Irradiation Facility (MIF) located in the HFIR building outside the reactor containment. The MIF will act as the instrumentation and control center for the experiment, enabling real-time feedback from in situ sensors and control of irradiation temperatures via a gas delivery system. Two unique capsule designs were developed to capture each phenomenon: the thermal conductivity capsule, which uses a thermopile method to estimate fuel specimen thermal conductivity, and the fission gas release capsule, which will have continuous flowing gas communication to high-purity germanium detectors that are housed in the MIF for monitoring FGR. This report details the reactor physics and heat transfer modeling activities that were used to inform the experiment design and predict capsule performance. It also describes out-of-pile activities conducted to stand up this new capability and verify the measurement techniques. Modeling efforts to date have demonstrated the feasibility of the in situ measurement techniques and supported the development of the MINITAURE assembly configuration. Out-of-pile testing of the thermal conductivity measurement shows promise in capturing relative changes in thermal conductivity. However, significant errors exist in the measured absolute value, posing a need for further refinement.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Aluminum-clad Spent Nuclear Fuel Engineering Scale Drying Experiment Design

The purpose of this document is to provide the technical specifications for the Engineering Scale Design for the drying tests of aluminum-clad spent nuclear fuel (ASNF). The engineering scale design is to accommodate both forced helium drying (FHD) as well as vacuum drying. The experiments will employ mock ASNF assemblies with a limited number of chemically treated aluminum plates to simulate the aluminum hydroxides found on ASNF. The goal here is to understand the transformation that may occur in plates including the loss of chemisorbed water and changes in morphology. Physiosorbed and bulk water found in experiments will be dried in the process and the effect on drying operations noted. Decay heat will be simulated in one assembly using a custom designed resistance heating element. A typical radial arrangement of assemblies will be employed using a modified Type 1A Basket design. For the chamber/canister, a single assembly layer with full radial dimension will be employed. Modifications to the standard canister design and configuration include the addition of a siphon tube to enable recirculation of hot gas for forced helium drying. A ring of ports/flanges are added near the top of the chamber to accommodate the feedthroughs for instrumentation and power needed for the experiment and data collection. Four viewports are added to the main section of the chamber with two in line with one of the fuel assembly and siphon tube. The other two viewports are on the opposite side of the chamber. The purpose here is to provide the option of thermal imaging in addition to the nearly four dozen thermocouples available inside the chamber. Modeling of the chamber, basket, and mock ASNF assemblies was conducted to estimate temperature distributions throughout the chamber during forced helium drying and over the anticipated drying period. This modeling was used as input to decisions on the Engineering Scale Design. Work on modeling continues in the period during setup and testing to develop preliminary drying models. Analysis of experimental results will later be used to validate these and subsequent models.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Payload Production for the Fire Testing of Primary Containment Vessels

One safety concern for the storage of nuclear or hazardous materials within the Department of Energy (DOE) complex is the pressure response behaviors of Primary Containment Vessels (PCVs) of a 9975 shipping package. Although there are many conservative estimates for the pressure response behavior of PCV in high temperature environments, these estimations remain unchecked by experiment. Conservative estimates frequently build in large safety margins which result in a reduced operating range and potentially unnecessary operation restrictions. In an attempt to alleviate some of these barriers, Nuclear & Criticality Safety Engineering (N&CSE) has requested the fire testing of primary containment vessels.

12 MANAGEMENT OF RADIOACTIVE AND NON-RADIOACTIVE W↗

Results of a 2000 hour wear test of the NEXIS ion engine

The Nuclear Electric Xenon Ion System (NEXIS) ion thruster was developed for potential outer planet robotic missions under NASA's Prometheus program. This engine was designed to operate at power levels ranging from 16 to over 20 kWe at specific impulses of 6000 to 7500 s for burn times of up to 10 years, satisfying the requirements of nuclear electric propulsion systems such as that on the proposed Prometheus 1 mission to explore the icy moons of Jupiter. State-of-the-art performance and life assessment tools were used to design the thruster. Following the successful performance validation of a Laboratory Model thruster, Development Model hardware was fabricated and subjected to vibration and wear testing. The results of a 2000-hour wear test are reported herein. Thruster performance achieved the target requirements and was steady for the duration of the test. Ion optics performance was similarly stable. Discharge loss increases of 6 eV/ion were observed in the first 500 hours of the test and were attributed to primary electron energy decreases due to cathode insert conditioning. Relatively high recycle rates were observed and were identified to be high-voltage-to-ground arcs in the back of the thruster caused by wire insulation outgassing and electron penetration through the plasma screen. Field emission of electrons between the accelerator and screen grids was observed and attributed to evolution of field emitter sites at accelerator grid aperture edges caused by ion bombardment. Preliminary modeling and analysis indicates that the NEXIS engine can meet mission performance requirements over the required lifetime. Finally, successful validation of the NEXIS design methodology, design tools, and technologies with the results of the wear test and companion performance and vibration tests presents significant applicability of the NEXIS development effort to missions of near-term as well as long-term interest for NASA.

Nuclear Electric Xenon Ion System (NEXIS)Thruster ↗

MULTI-MISSION THERMOELECTRIC GENERATOR ASSEMBLY TESTING AND LAUNCH OPERATIONS FOR MARS 2020

The Space Nuclear Power and Isotope Technologies (SNPIT) division at Idaho National Laboratory (INL) fuels, performs acceptance testing, and provides spacecraft integration support of Radioisotope Power Systems (RPS) in support of National Aeronautics and Space Administration (NASA) missions. Recently the SNPIT team completed assembly, testing and launch support of the Multi-Mission Radioisotope Thermoelectric Generator (MMRTG) for the Mars 2020 Perseverance Rover mission.

07 ISOTOPE AND RADIATION SOURCES↗

MULTI-MISSION THERMOELECTRIC GENERATOR ASSEMBLY TESTING AND LAUNCH OPERATIONS FOR MARS 2020

The Space Nuclear Power and Isotope Technologies (SNPIT) division at Idaho National Laboratory (INL) fuels, performs acceptance testing, and provides spacecraft integration support of Radioisotope Power Systems (RPS) in support of National Aeronautics and Space Administration (NASA) missions. Recently the SNPIT team completed assembly, testing and launch support of the Multi-Mission Radioisotope Thermoelectric Generator (MMRTG) for the Mars 2020 Perseverance Rover mission.

07 ISOTOPE AND RADIATION SOURCES↗

Performance Analysis and Simulaion of the Hydraulic Scram System in TREAT Reactor

The Transient Reactor Test Facility (TREAT) at Idaho National Laboratory (INL) serves a vital role in nuclear fuel safety research, enabling transient experiments that simulate reactivity excursions and accident scenarios. Central to these operations is the transient control rod drive system (TCRDS), which drives rapid motion of the transient control rods such that TREAT can simulate rapid power changes typical of reactor accidents. The reliability and performance of this system are critical for protecting both fuel specimens and reactor infrastructure. This study presents the initial phase of a two-year investigation into the dynamics and reliability of the TREAT hydraulic TCRDS. Conducted in collaboration with INL, the research employs a combined computational and experimental approach to analyze the system's response time, pressure transients, and potential failure modes. Emphasis is placed on understanding how fluid characteristics influence the TCRDS’s ability to achieve both rapid power changes and mechanical stability. The TRDS and the skid that powers it will be analyzed throughout this investigation. Computational modeling using computational fluid dynamics (CFD) will simulate the hydraulic response under varying conditions. In parallel, experimental testing planned at INL will validate these models and capture key performance metrics. This paper outlines the system design, analytical framework, and modeling strategies that form the foundation for later testing. Ultimately, this work aims to support improvements to the TCRDS’s design and reliability, contributing to the broader goal of enhancing nuclear fuel safety and sustaining TREAT’s mission as a premier nuclear fuel test facility.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Los Alamos National Laboratory Floodplain Assessment for Fire Risk Mitigations at the Lower Slobbovia Testing Site in (TA-36)

The National Nuclear Security Administration (NNSA), a semi-autonomous agency within the U.S. Department of Energy (DOE), is proposing to take fire pre-suppression actions at Los Alamos National Laboratory (LANL) Technical Area (TA) 36. Constructing a fire break and a fuel break surrounding the Lower Slobbovia explosives testing site in addition to the current vegetation mowing practices would establish a safety perimeter to help prevent fires from spreading away from the firing point. NNSA has prepared this floodplain assessment in accordance with 10 Code of Federal Regulations (CFR) Part 1022 Compliance with Floodplain and Wetland Environmental Review Requirements (10 CFR 1022), which was promulgated to implement DOE requirements under Executive Order 11988 Floodplain Management (EO 1977). A floodplain is defined in 10 CFR 1022 as “the lowlands adjoining inland and coastal waters and relatively flat areas and flood prone areas of offshore islands,” and a base floodplain as “the 100-year floodplain, that is, a floodplain with a 1.0 percent chance of flooding in any given year (CFR 2003).” This floodplain assessment evaluates potential impacts to floodplain values and functions from implementation of the proposed action, identifies alternatives to the Proposed Action, and allows for meaningful public comment.

54 ENVIRONMENTAL SCIENCES↗

MCNP Analysis fo the Aqua-SETH Experiment in TREAT

The versatile Transient Reactor Test (TREAT) Facility’s capability to deliver customized transient nuclear power excursions gives researchers and developers a multitude of specialized testing options. In conjunction with reactorprescribed delivery of neutron flux, experiment design requires specimen packaging to meet TREAT safety containment requirements and experimenter test objectives. These objectives may range from the very simple separate effects tests (generally dry capsule) to the more complex integral scale testing wherein prototypic boundary or specimen reactor environment conditions are created. The historic MARK-III sodium flow loop that achieved thermalhydraulic prototypic test conditions serves as an example of the more complex experiment design package.

11 NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Expansion of the Fuel Motion Monitoring System

The Idaho National Laboratory (INL) Transient Reactor Test Facility (TREAT) Fuel Motion Monitoring System (FMMS) is a diagnostic tool used to visualize the movement and location of fuel within the nuclear reactor during transient experiments. TREAT is designed to test the behavior of nuclear fuel under accident conditions, such as a rapid power increase. The TREAT FMMS, also referred to as the “hodoscope” because of the system’s massive steel collimator component, is located on the North beam port of the reactor. While the FMMS system is capable of incorporating a total of 360 sensors, initial refurbishment efforts resulted in a array of 96 fast neutron detectors. This initial array was configured to provide a narrow (2 channels) full-length view of experiment vessels with an extended 4-channel–wide region in the center of the array capable of providing a full view of all initially planned experiments. Planning and efforts to expand the FMMS array began immediately following the restart of TREAT. An additional 96 detectors were evaluated, characterized, and prepared for installation at TREAT during the summer of 2018. Unfortunately, funding reductions forced the project towards a 5-year hiatus. In October of 2023 funding from the Department of Energy’s Nuclear Science User Facilities enabled the expansion to recommence. This report serves to document the activities performed to expand the FMMS detector array to 192 channels in order to provide a broader view of the larger and more sophisticated test capsules currently planned for future irradiation in the TREAT reactor. This expansion also included doubling the data acquisition capability, addressing the new heat load on the system, and synchronizing the time for all digital components.

11 - NUCLEAR FUEL CYCLE AND FUEL MATERIALS↗

Flowing gas, non-nuclear experiments on the gas core reactor

Variations in cavity wall and injection configurations of the gas core reactor were aimed at establishing flow patterns that give a maximum of the nuclear criticality eigenvalue. Correlation with the nuclear effect was made using multigroup diffusion theory normalized by previous benchmark critical experiments. Air was used to simulate the hydrogen propellant in the flow tests, and smoked air, argon, or Freon to simulate the central nuclear fuel gas. Tests were run both in the down-firing and upfiring directions. Results showed that acceptable flow patterns with volume fraction for the simulated nuclear fuel gas and high flow rate ratios of propellant to fuel can be obtained. Using a point injector for the fuel, good flow patterns are obtained by directing the outer gas at high velocity long the cavity wall, using louvered injection schemes. Recirculation patterns were needed to stabilize the heavy central gas when different gases are used.

Kunze, J. F.↗