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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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DOE OSTI2018

It’s all right(-handed neutrinos): a new W ' model for the R D ( ∗ ) anomaly

The measured B-meson semi-leptonic branching ratios R D and R D ∗ have long-standing deviations between theory and experiment. We introduce a model which explains both anomalies through a single interaction by introducing a right-handed neutrino as the missing energy particle. This interaction is mediated by a heavy charged vector boson (W ') which couples only to right-handed quarks and leptons of the Standard Model through the mixing of these particles with new vector-like fermions. Previous W ' models for the R D ( ∗ ) anomaly were strongly constrained from flavor changing neutral currents and direct collider searches for Z' → τ τ resonances. We show that relying on right-handed fermion mixing enables us to avoid these constraints, as well as other severe bounds from electroweak precision tests and neutrino mixing.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2018

Will X-ray Safety Glasses Become Mandatory for Radiological Vascular Interventions?

PurposeThe annual permissible radiation ocular lens dose has been reduced to 20 millisieverts (mSv) in the current European directive 2013/59/Euratom. The aim of this study was to evaluate the personal radiation dose for vascular interventions with special focus on ocular lens dose.Materials and MethodsFrom May 2016 to October 2016, the personal radiation doses of two interventionists and four technicians were prospectively recorded during 206 vascular interventions. The position of personnel, intervention type and fluoroscopy time were recorded. Parameters evaluated were total body dose measured by film dosimeter, hand dose measured by ring thermoluminescent dosimeter (TLD) and ocular lens dose measured by TLD placed in front of the safety glasses. Linear regression analysis was used to estimate the dose at 2 and 5 years.ResultsThe ocular lens dose, hand and total body dose of the two interventionists were 11/5, 56/47 and 0.6 mSv each, respectively. The estimated 5-year ocular dose was 113.08 mSv (95% CI 38.2–187.97)/40.95 (95% CI 16.9–64.7). Similarly, hand dose was 608.4 mSv (95% CI 442.78–774.38)/514.47 (95% CI 329.83–699.10) and body dose 6.07 mSv (95% CI 4.70–8.22)/5.12 (95% CI 3.65–6.59), respectively. Amongst four technicians, only the first assistant showed recordings of 0.3 mSv body dose, 2 mSv ocular lens dose and 5 mSv hand dose.ConclusionThe yearly ocular lens dose, particularly for interventionists dealing with complex interventions, could cross the permitted yearly limit set by the new Euratom directive. Therefore, X-ray safety glasses would become mandatory for complex radiological vascular interventions.Level of EvidenceLevel III, non-randomized controlled cohort/follow-up study.

62 RADIOLOGY AND NUCLEAR MEDICINE↗

DOE OSTI2021

Bayesian optimization for chemical products and functional materials

The design of chemical-based products and functional materials is vital to modern technologies, yet remains expensive and slow. Artificial intelligence and machine learning offer new approaches to leverage data to overcome these challenges. Herein this review focuses on recent applications of Bayesian optimization (BO) to chemical products and materials including molecular design, drug discovery, molecular modeling, electrolyte design, and additive manufacturing. Numerous examples show how BO often requires an order of magnitude fewer experiments than Edisonian search. The essential equations for BO are introduced in a self-contained primer specifically written for chemical engineers and others new to the area. Finally, the review discusses four current research directions for BO and their relevance to product and materials design.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2024

Towards understanding stress corrosion cracking of austenitic stainless steels exposed to realistic sea salt brines

Not Available

36 MATERIALS SCIENCE↗

DOE OSTI2023

Sintered nanostructured alloys for advanced fusion energy applications

Not Available

36 MATERIALS SCIENCE↗

DOE OSTI2025

High-temperature nanoindentation creep studies on castable and sintered nanostructured low-activation ferritic-martensitic alloys

In this article, we present the creep characteristics of two reduced activation ferritic-martensitic steels of identical starting compositions formed by different fabrication routes: a nanostructured ferritic alloy commonly referred to as a castable nanostructured alloy (CNA) and a sintered nanostructured alloy (SNA) variant. Through a series of nanoindentation experiments spanning a temperature range of 25 °C to 650 °C, with a maximum load of 100 mN, we find creep behaviors in the cast and sintered materials to be remarkably similar. The creep stress exponent (n) for CNA and SNA were found to be in the range of 8–35 and the activation volume was ∼14–42b 3 , underscoring a dominance of dislocation-mediated mechanisms in both alloys. Notably, we observed a decline in the creep stress exponent with increasing temperature, attributable to the heightened influence of thermally activated dislocations. This phenomenon suggests a potential transition in the deformation mechanism towards a thermally activated dislocation climb process, significantly impacting the observed creep behavior.

36 MATERIALS SCIENCE↗

DOE OSTI2018

Remote visual analysis of large turbulence databases at multiple scales

The remote analysis and visualization of raw large turbulence datasets is challenging. Current accurate direct numerical simulations (DNS) of turbulent flows generate datasets with billions of points per time-step and several thousand time-steps per simulation. Until recently, the analysis and visualization of such datasets was restricted to scientists with access to large supercomputers. The public Johns Hopkins Turbulence database simplifies access to multi-terabyte turbulence datasets and facilitates the computation of statistics and extraction of features through the use of commodity hardware. In this paper, we present a framework designed around wavelet-based compression for high-speed visualization of large datasets and methods supporting multi-resolution analysis of turbulence. By integrating common technologies, this framework enables remote access to tools available on supercomputers and over 230 terabytes of DNS data over the Web. Finally, the database toolset is expanded by providing access to exploratory data analysis tools, such as wavelet decomposition capabilities and coherent feature extraction.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2019

Energy transfer for storage or recovery in capacitive deionization using a DC-DC converter

Energy recovery from capacitive deionization (CDI) has the potential to increase overall desalination efficiency. We here define the storage (one-way) and utilization (round-trip) efficiencies between a CDI cell and an energy storage device using a generic direct current/direct current (DC/DC) converter circuit. Presented is a closed-form analytical model for the case of a supercapacitor (SC) as the energy storage device and a buck-boost converter as the DC/DC converter. The model is benchmarked with a numerical model, showing good agreement. Also presented is a comparison among energy transfer methods wherein desalination productivity is fixed. For constant current operation, this condition requires higher currents to compensate for the inactive time introduced by the converter. For fixed productivity, the mean current of the converter circuit approaches the constant current value for higher initial voltages and lower capacitances in the supercapacitor. Finally, we show the effect of relevant parameters of the SC in the storage and utilization efficiency. The model predicts storage and utilization efficiencies of at least 90% for an initial voltage of 1 V or higher and reasonable CDI and SC parameters. Finally, we provide engineering operational parameters to maximize the efficiency of energy transfer and guidance in the selection of electronic components.

25 ENERGY STORAGE↗

DOE OSTI2023

High-Sensitivity Low-Energy Ion Spectroscopy with Sub-Nanometer Depth Resolution Reveals Oxidation Resistance of MoS 2 Increases with Film Density and Shear-Induced Nanostructural Modifications of the Surface

For decades, density has been attributed as a critical aspect of the structure of sputter-deposited nanocrystalline molybdenum disulfide (MoS 2 ) coatings impacting oxidation resistance and wear resistance. Despite its importance, there are few examples in the literature that explicitly investigate the relationship between the density and oxidation behaviors of MoS 2 coatings. Aging and oxidation are primary considerations for the use of MoS 2 coatings in aerospace applications as they inevitably experience prolonged storage in water and oxygen-rich environments prior to use. Oxidation that is either limited to the first few nanometers or through the bulk of the coating can result in seizure due to high initial coefficients of friction or component failure from excessive wear. High-sensitivity low-energy ion spectroscopy (HS-LEIS) and Rutherford backscattering spectrometry (RBS) are both used to understand the extent of oxidation throughout the first ~10 nanometers of the surface of pure sputtered nanocrystalline MoS 2 coatings after high-temperature aging and how it is impacted by the density of coatings as measured by RBS. Results show that low-density coatings (ρ = 3.55 g/cm 3 ) exhibit a more columnar microstructure and voiding, which act as pathways for oxidative species to penetrate and interact with edge sites, causing severe surface and subsurface oxidation. Furthermore, HS-LEIS of surfaces sheared prior to oxidation reveals that the oxidation resistance of low-density MoS 2 coatings can be significantly improved by shear-induced reorientation of the surface microstructure to a basal orientation and elimination of pathways for oxygen into the bulk through compaction of surface and subsurface voids.

36 MATERIALS SCIENCE↗

DOE OSTI2022

Evolving Interior Mixing Regimes in a Tidal River Plume

Microstructure profiling was utilized to estimate vertical mixing (via vertical turbulent buoyancy flux) during a tidal pulse in the interior Merrimack River plume in calm winds. Multiple stratified shear mixing regimes appear and evolve with time. Initially the plume acts as a nearfield jet, with mixing in the plume (plume layer mixing) and over the plume-ambient interface (nearfield interfacial mixing). As the plume grows, interfacial mixing is suppressed offshore of the nearfield as currents slow, diminishing turbulent exchange between plume and shelf. At the end of ebb, ambient tidal currents reverse direction below plume, initiating another mode of internal, interfacial mixing (coined here as tidal interfacial mixing), allowing exchange between plume and ambient waters offshore. This work highlights previously unreported tidally modulated mixing within the near and midfield of a river plume.

54 ENVIRONMENTAL SCIENCES↗

DOE OSTI2021

Measuring the capabilities of quantum computers

Quantum computers can now run interesting programs, but each processor’s capability—the set of programs that it can run successfully—is limited by hardware errors. These errors can be complicated, making it difficult to accurately predict a processor’s capability. Benchmarks can be used to measure capability directly, but current benchmarks have limited flexibility and scale poorly to many-qubit processors. We show how to construct scalable, efficiently verifiable benchmarks based on any program by using a technique that we call circuit mirroring. With it, we construct two flexible, scalable volumetric benchmarks based on randomized and periodically ordered programs. We use these benchmarks to map out the capabilities of twelve publicly available processors, and to measure the impact of program structure on each one. We find that standard error metrics are poor predictors of whether a program will run successfully on today’s hardware, and that current processors vary widely in their sensitivity to program structure.

97 MATHEMATICS AND COMPUTING↗

DOE OSTI2023

Contactless measurement of the photovoltage in BiVO 4 photoelectrodes

The power output of photoelectrochemical devices for solar energy-to-fuel conversion is determined by the photovoltage of the junction under illumination. In the presence of fast redox couples, the photovoltage can be obtained directly from current–voltage measurements of the device. However, for slow redox couples (H + /H 2 , O 2 /H 2 O) used in solar fuel photoelectrodes, photovoltage measurements are not straightforward, due to the kinetic overpotentials during charge transfer. Here we show that the photovoltage of BiVO 4 electrodes in contact with fast electron donors KI, Na 2 SO 3 or H 2 O 2 or K 4 Fe(CN) 6 can be measured in a contactless way with vibrating Kelvin probe surface photovoltage (SPV) spectroscopy. The photovoltage varies with illumination wavelength and intensity and matches the open circuit potential of the electrodes, obtained separately from electrochemical measurements. Plots of the photovoltage versus irradiance can be used to predict the oxidizing power of each electrode under zero applied bias. Except for K 4 Fe(CN) 6 , which causes shunting in the BiVO 4 electrode, photovoltage values correlate well with the built-in potential of each junction. Furthermore, the ability to obtain photovoltage information through contactless SPV measurements will be useful in the search for solid–liquid junctions with superior energy conversion properties.

14 SOLAR ENERGY↗

DOE OSTI2014

Negative magnetoresistance in a low-k dielectric

We observed negative magnetoresistance in amorphous SiCOH, a low-k dielectric, applying modest magnetic fields (<150 Gauss) at room temperature. The conductivity increases with increasing magnetic field. The change in conductivity due to the applied magnetic field increases with electric field and has little or no temperature dependence over the range studied. The magnitude of the effect is independent of the orientation of magnetic field relative to the direction of current flow. The effect is attributed to spin constraints associated with double occupancy of a trap site under the assumption that trap sites which have double occupancy have lower hopping frequencies than traps that have single occupancy.