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All sourcesNASA NTRSDOE OSTI
NASA NTRS2012

The Cloud-Aerosol Transport System (CATS): A New Lidar for Aerosol and Cloud Profiling from the International Space Station

Spaceborne lidar profiling of aerosol and cloud layers has been successfully implemented during a number of prior missions, including LITE, ICESat, and CALIPSO. Each successive mission has added increased capability and further expanded the role of these unique measurements in wide variety of applications ranging from climate, to air quality, to special event monitoring (ie, volcanic plumes). Many researchers have come to rely on the availability of profile data from CALIPSO, especially data coincident with measurements from other A-Train sensors. The CALIOP lidar on CALIPSO continues to operate well as it enters its fifth year of operations. However, active instruments have more limited lifetimes than their passive counterparts, and we are faced with a potential gap in lidar profiling from space if the CALIOP lidar fails before a new mission is operational. The ATLID lidar on EarthCARE is not expected to launch until 2015 or later, and the lidar component of NASA's proposed Aerosols, Clouds, and Ecosystems (ACE) mission would not be until after 2020. Here we present a new aerosol and cloud lidar that was recently selected to provide profiling data from the International Space Station (ISS) starting in 2013. The Cloud-Aerosol Transport System (CATS) is a three wavelength (1064,532,355 nm) elastic backscatter lidar with HSRL capability at 532 nm. Depolarization measurements will be made at all wavelengths. The primary objective of CATS is to continue the CALIPSO aerosol and cloud profile data record, ideally with overlap between both missions and EarthCARE. In addition, the near real time (NRT) data capability ofthe ISS will enable CATS to support operational applications such as aerosol and air quality forecasting and special event monitoring. The HSRL channel will provide a demonstration of technology and a data testbed for direct extinction retrievals in support of ACE mission development. An overview of the instrument and mission will be provided, along with a summary of the science objectives and simulated data. Input from the ICAP community is desired to help plan our NRT mission goals and interactions with ICAP forecasters.

Welton, Ellsworth J.↗
NASA NTRSDate not supplied

The Relationship Of Size Distributions To Spectral (300 - 700 Nm) Extinction Parameterization Of Ambient In Situ Aerosols Measured During FIREX-AQ And The Influence Of Aerosol Composition

Hyperspectral (300 - 700 nm, 0.7 nm resolution) aerosol extinction spectra were measured at seven fires in six states in the western United States during the Fire Influence on Regional to Global Environments and Air Quality (FIREX-AQ) field campaign in July and August 2019. Obtained using an in situ aerosol sampling method, these spectra are directly comparable to other in situ aerosol measurements such as size distribution and composition. A previous deployment of the in situ Spectral Aerosol Extinction (SpEx) instrument that measured fine mode aerosols (50% size cut of 1.3 µm particle diameter) around the Korean peninsula showed that over this spectral range 2nd order polynomials provided a better fit to the logarithmically transformed spectra than linear fits (representative of Ångström exponents). The two fit parameters (a1, a2) of the polynomials are related to the classic Ångström exponent but provide additional information via their two-dimensional parameter space. The previous work was limited by the lack of commensurate size distribution information. Here, using the FIREX-AQ spectra set it is possible to expand on the previous analysis in three specific ways: 1) size distribution information is available to further elucidate how size distribution maps into (a1, a2) space, 2) the sampled size distributions include larger particles than the Korean study, and 3) the FIREX-AQ data set exhibits smoke-related spectral features in the UV part of the spectrum that are not present in background air nor were they observed previously in the Korean study. The UV spectral features are particularly intriguing as they likely arise from the absorption component of the extinction measurement and therefore may be related to composition. The relationships between the ambient in situ aerosol size distributions, the extinction spectra, and composition will be presented.

Carolyn Jordan↗
NASA NTRS2023

The Coupling Between Tropical Meteorology, Aerosol Lifecycle, Convection, and Radiation, During the Clouds, Aerosol and Monsoon Processes Philippines Experiment (CAMP2Ex)

The NASA Cloud, Aerosol, and Monsoon Processes Philippines Experiment (CAMP2Ex) employed the NASA P-3, Stratton Park Engineering Company (SPEC) Learjet 35, and a host of satellites and surface sensors to characterize the coupling of aerosol processes, cloud physics, and atmospheric radiation within the Maritime Continent’s complex southwest monsoonal environment. Conducted in the late summer of 2019 from Luzon Philippines in conjunction with the Office of Naval Research Propagation of Intraseasonal Tropical OscillatioNs (PISTON) experiment with its R/VSally Ride stationed in the North Western Tropical Pacific, CAMP2Ex documented diverse biomass burning, industrial and natural aerosol populations and their interactions with small to congestus convection. The 2019 season exhibited El Nino and associated drought, high biomass burning emissions, and an early monsoon transition allowing for observation of pristine to massively polluted environments as they advected through intricate diurnal mesoscale and radiative environments into the monsoonal trough. CAMP2Ex’s preliminary results indicate 1) increasing aerosol loadings tend to invigorate congestus convection in height and increase liquid water paths; 2) lidar, polarimetry, and geostationary Advanced Himawari Imager remote sensing sensors have skill in quantifying diverse aerosol and cloud properties and their interaction; and 3) high resolution remote sensing technologies are able to greatly improve our ability to evaluate the radiation budget in complex cloud systems. Through the development of innovative informatics technologies, CAMP2Ex provides a benchmark dataset of an environment of extremes for the study of aerosol, cloud and radiation processes as well as a crucible for the design of future observing systems.

CAMP2Ex↗
NASA NTRS2013

Assessment of Error in Aerosol Optical Depth Measured by AERONET Due to Aerosol Forward Scattering

We present an analysis of the effect of aerosol forward scattering on the accuracy of aerosol optical depth (AOD) measured by CIMEL Sun photometers. The effect is quantified in terms of AOD and solar zenith angle using radiative transfer modeling. The analysis is based on aerosol size distributions derived from multi-year climatologies of AERONET aerosol retrievals. The study shows that the modeled error is lower than AOD calibration uncertainty (0.01) for the vast majority of AERONET level 2 observations, ~99.53%. Only ~0.47% of the AERONET database corresponding mostly to dust aerosol with high AOD and low solar elevations has larger biases. We also show that observations with extreme reductions in direct solar irradiance do not contribute to level 2 AOD due to low Sun photometer digital counts below a quality control cutoff threshold.

AERONET↗
NASA NTRS2013

Influence of Observed Diurnal Cycles of Aerosol Optical Depth on Aerosol Direct Radiative Effect

The diurnal variability of aerosol optical depth (AOD) can be significant, depending on location and dominant aerosol type. However, these diurnal cycles have rarely been taken into account in measurement-based estimates of aerosol direct radiative forcing (ADRF) or aerosol direct radiative effect (ADRE). The objective of our study was to estimate the influence of diurnal aerosol variability at the top of the atmosphere ADRE estimates. By including all the possible AERONET sites, we wanted to assess the influence on global ADRE estimates. While focusing also in more detail on some selected sites of strongest impact, our goal was to also see the possible impact regionally.We calculated ADRE with different assumptions about the daily AOD variability: taking the observed daily AOD cycle into account and assuming diurnally constant AOD. Moreover, we estimated the corresponding differences in ADREs, if the single AOD value for the daily mean was taken from the the Moderate Resolution Imaging Spectroradiometer (MODIS) Terra or Aqua overpass times, instead of accounting for the true observed daily variability. The mean impact of diurnal AOD variability on 24 h ADRE estimates, averaged over all AERONET sites, was rather small and it was relatively small even for the cases when AOD was chosen to correspond to the Terra or Aqua overpass time. This was true on average over all AERONET sites, while clearly there can be much stronger impact in individual sites. Examples of some selected sites demonstrated that the strongest observed AOD variability (the strongest morning afternoon contrast) does not typically result in a significant impact on 24 h ADRE. In those cases, the morning and afternoon AOD patterns are opposite and thus the impact on 24 h ADRE, when integrated over all solar zenith angles, is reduced. The most significant effect on daily ADRE was induced by AOD cycles with either maximum or minimum AOD close to local noon. In these cases, the impact on 24 h ADRE was typically around 0.1-0.2W/sq m (both positive and negative) in absolute values, 5-10% in relative ones.

optical depth↗
NASA NTRS2016

Interpreting the Ultraviolet Aerosol Index Observed with the OMI Satellite Instrument to Understand Absorption by Organic Aerosols: Implications for Atmospheric Oxidation and Direct Radiative Effects

Satellite observations of the ultraviolet aerosol index (UVAI) are sensitive to absorption of solar radiation by aerosols; this absorption affects photolysis frequencies and radiative forcing. We develop a global simulation of the UVAI using the 3-D chemical transport model GEOSChem coupled with the Vector Linearized Discrete Ordinate Radiative Transfer model (VLIDORT). The simulation is applied to interpret UVAI observations from the Ozone Monitoring Instrument (OMI) for the year 2007. Simulated and observed values are highly consistent in regions where mineral dust dominates the UVAI, but a large negative bias (-0.32 to -0.97) exists between simulated and observed values in biomass burning regions. We determine effective optical properties for absorbing organic aerosol, known as brown carbon (BrC), and implement them into GEOS-Chem to better represent observed UVAI values over biomass burning regions. The inclusion of absorbing BrC decreases the mean bias between simulated and OMI UVAI values from -0.57 to -0.09 over West Africa in January, from -0.32 to +0.0002 over South Asia in April, from -0.97 to -0.22 over southern Africa in July, and from -0.50 to +0.33 over South America in September. The spectral dependence of absorption after including BrC in the model is broadly consistent with reported observations for biomass burning aerosol, with absorbing Angstrom exponent (AAE) values ranging from 2.9 in the ultraviolet (UV) to 1.3 across the UV-Near IR spectrum. We assess the effect of the additional UV absorption by BrC on atmospheric photochemistry by examining tropospheric hydroxyl radical (OH) concentrations in GEOS-Chem. The inclusion of BrC decreases OH by up to 30% over South America in September, up to 20% over southern Africa in July, and up to 15% over other biomass burning regions. Global annual mean OH concentrations in GEOS-Chem decrease due to the presence of absorbing BrC, increasing the methyl chloroform lifetime from 5.62 to 5.68 years, thus reducing the bias against observed values. We calculate the direct radiative effect (DRE) of BrC using GEOS-Chem coupled with the radiative transfer model RRTMG (GC-RT). Treating organic aerosol as containing more strongly absorbing BrC changes the global annual mean all-sky top of atmosphere (TOA) DRE by +0.03Wm(exp -2) and all-sky surface DRE by -0.08Wm(exp -2). Regional changes of up to +0.3Wm(exp -2) at TOA and down to -1.5Wm(exp -2) at the surface are found over major biomass burning regions.

Air Pollution↗
NASA NTRS2019

Updated MISR Over-Water Research Aerosol Retrieval Algorithm - Part 2: A Multi-Angle Aerosol Retrieval Algorithm for Shallow, Turbid, Oligotrophic, and Eutrophic Waters

Coastal waters serve as transport pathways to the ocean for all agricultural and other runoff from terrestrial sources, and many are the sites for upwelling of nutrient rich, deep water; they are also some of the most biologically productive on Earth. Estimating the impact coastal waters have on the global carbon budget requires relating satellite-based remote-sensing retrievals of biological productivity (e.g., chlorophyll alpha concentration) to in situ measurements taken in near-surface waters. The Multi-angle Imaging SpectroRadiometer (MISR) can uniquely constrain the "atmospheric correction" needed to derive ocean color from remote-sensing imagers. Here, we retrieve aerosol amount and type from MISR over all types of water. The primary limitation is an upper bound on aerosol optical depth (AOD), as the algorithm must be able to distinguish the surface. This updated MISR research aerosol retrieval algorithm (RA) also assumes that light reflection by the underlying ocean surface is Lambertian. The RA computes the ocean surface reflectance (R (sub rs)) analytically for a given AOD, aerosol optical model, and wind speed. We provide retrieval examples over shallow, turbid, and eutrophic waters and introduce a productivity and turbidity index (PTI), calculated from retrieved spectral R (sub rs), that distinguished water types (similar to the the normalized difference vegetation index, NDVI, over land). We also validate the new algorithm by comparing spectral AOD and Angstrom exponent (ANG) results with 2419 collocated AErosol RObotic NETwork (AERONET) observations. For AERONET 558 nanometer-interpolated AOD less than 1.0, the root-mean square error (RMSE) is 0.04 and linear correlation coefficient is 0.95. For the 502 cloud-free MISR and AERONET collocations with an AERONET AOD greater than 0.20, the ANG RMSE is 0.25 and r is 0.89. Although MISR RA AOD retrieval quality does not appear to be substantially impacted by the presence of turbid water, the MISR-RA-retrieved Angstrom exponent seems to suffer from increased uncertainty under such conditions. MISR supplements current ocean color sources in regions where sunglint precludes retrievals from single-view-angle instruments. MISR atmospheric correction should also be more robust than that derived from single-view instruments such as the Moderate Resolution Imaging Spectroradiometer (MODIS). This is especially true in regions of shallow, turbid, and eutrophic waters, locations where biological productivity can be high, and single-view-angle retrieval algorithms struggle to separate atmospheric from oceanic features.

Satellite Remote Sensing↗
NASA NTRSDate not supplied

AERACEPT (Aerosol Rapid Analysis Combined Entry Probe/sonde Technology): Design for Venus Aerosol Sampling

Aerosols (clouds, hazes, dusts) are drivers of key planetary processes, including mass and energy transfer; planetary climate evolution, as in the divergence of Venus and Earth; and are even of habitability interest, as Earth’s fog and cloud water have a substantial microbial presence. However, aerosols are highly dynamic, and once-in-a-lifetime flagship missions are not enough to fully characterize them. AERACEPT (AErosol Rapid Analysis Combined Entry Probe/sonde Technology) is an early-stage (TRL 2-3) technology combining the functions of an entry vehicle and aerosol-sampling passive descent sonde into a single aeroshell body. It is designed to reduce the mass, volume, and complexity of planetary aerosol science to within a small spacecraft footprint, allowing more frequent or concurrent missions. It is particularly well suited for a Venus mission, where the particles of greatest interest are within the subsonic descent regime, and is included in the Nephele mission concept study for a small spacecraft targeting Venus cloud and haze particles between 60 and 47 km.

Venus↗
DOE OSTI2025

Aerosol Microphysics and Chemical Measurements at Mt. Soledad and Scripps Pier during the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) from February 2023 to February 2024 UCSD Library Collection

This dataset includes guest instrument measurements and other PI products for aerosol microphysics and chemical measurements collected at Mt. Soledad and Scripps Pier during the Eastern Pacific Cloud Aerosol Precipitation Experiment (EPCAPE) from February 2023 to February 2024. The measurements include the following instruments at Mt. Soledad: High-Resolution Time-of-Flight Aerosol Mass Spectrometer (HR-ToF-AMS, Aerodyne), Scanning Electrical Mobility Spectrometer (SEMS, Brechtel Manufacturing Inc.), Aerodynamic Particle Sizer (APS, Droplet Measurements Technologies), Single Particle Soot Photometer (SP2, Drople Measurements Technologies), Meteorological Station (WXT520, Vaisala), Ozone (Teco), and trace gas proxies (Teledyne). In addition, the analyses of particle filters collected at Mt. Soledad for three dry-diameter size cuts (<1 micron, <0.5 micron, <0.18 micron) and at Scripps Pier for one dry-diameter size cut (<1 micron) by Fourier Transform Infrared (FTIR) and X-ray Fluorescence (XRF) are reported. A differential mobility analyzer operated as a scanning mobility particle sizer (SMPS, TSI Inc.), a printed particle optical spectrometer (POPS, Grimm), and a continuous flow diffusion cloud condensation nuclei (CCN, DMT) counter provide the mobility aerosol size distribution (30-360 nm), optical size distribution (150 - 6000 nm), size-resolved CCN distribution (30-360 nm) at 0.2, 0.4, 0.6, 0.8, and 1.0% supersaturation. Measurements are reported for both sampling from an isokinetic aerosol inlet and from a Counterflow Virtual Impactor (CVI, Brechtel Manufacturing Inc.). The data are available at the following link: https://library.ucsd.edu/dc/collection/bb0898306q

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1979

Application of a coupled aerosol formation: Radiative transfer model to climatic studies of aerosols

A sophisticated one dimensional physical-chemical model of the formation and evolution of stratospheric aerosols was used to predict the size and number concentration of the stratospheric aerosols as functions of time and altitude following: a large volcanic eruption; increased addition of carbonyl sulfide (OCS) or sulfur dioxide (SO2) to the troposphere; increased supersonic aircraft (SST) flights in the stratosphere; and, large numbers of space shuttle (SS) flights through the stratosphere. A radiative-convective one dimensional climate sensitivity study, using the results of the aerosol formation model, was performed to assess the ground level climatic significance of these perturbations to the stratospheric aerosol layer. Volcanic eruptions and large OCS or SO2 increases could cause significant climatic changes. Currently projected SS launches and moderate fleets of SST's are unlikely to upset the stratospheric aerosol layer enough to significantly impact climate.

Toon, O. B.↗
NASA NTRS1984

Aerosol distributions and an arctic aerosol front during AGASP - Norwegian Arctic

Vertical profiles of aerosol characteristics obtained near Svalbard, Norway, during the Arctic Gas and Aerosol Sampling Program indicate that high aerosol concentrations and strong visible haze were distributed throughout the troposphere. Layers of Arctic haze were observed in both dry air and moist air. A research flight on March 31, 1983, crossed a previously undocumented Arctic aerosol front structure. Condensation nucleus concentrations of 450/cu cm within the polluted continental air mass south of the front decreased to 80/cu cm within the clean Arctic air north of the front. Aerosols above the Aitken size range decreased one order of magnitude in both number and mass across this same air mass boundary.

Ratz, W. E.↗
NASA NTRS1994

Validation of stratospheric aerosol and gas experiments 1 and 2 satellite aerosol optical depth measurements using surface radiometer data

The stratospheric aerosol measurement 2, stratospheric aerosol and gas experiment (SAGE) 1, and SAGE 2 series of solar occultation satellite instruments were designed for the study of stratospheric aerosols and gases and have been extensively validated in the stratosphere. They are also capable, under cloud-free conditions, of measuring the extinction due to aerosols in the troposphere. Such tropospheric extinction measurements have yet to be validated by appropriate lidar and in situ techniques. In this paper published atmospheric aerosol optical depth measurements, made from high-altitude observatories during volcanically quiet periods, have been compared with optical depths calculated from local SAGE 1 and SAGE 2 extinction profiles. Surface measurements from three such observatories have been used, one located in Hawaii and two within the continental United States. Data have been intercompared on a seasonal basis at wave-lenths between 0.5 and 1.0 micron and found to agree within the range of measurement errors and expected atmospheric variation. The mean rms difference between the optical depths for corresponding satellite and surface measured data sets is 29%, and the mean ratio of the optical depths is 1.09.

Kent, G. S.↗
NASA NTRS1995

Nonsphericity of dust-like tropospheric aerosols: Implications for aerosol remote sensing and climate modeling

T-matrix computations of light scattering by polydispersions of randomly oriented nonspherical aerosols and Mie computations for equivalent spheres are compared. Findings show that even moderate nonsphericity results in suubstantial errors in the retrieved aerosol optical thickness if satellite reflectance measurements are analyzed using Mie theory. On the other hand, the use of Mie theory for nonspherical aerosols produces negligible errors in the computation of albedo and flux related quantities, provided that the aerosol size distribution and optical thickness are known beforehand. The first result can be explained by large nonspherical-spherical differences in scattering phase function, while the second result follows from small nonspherical-spherical differences in single-scattering albedo and asymmetry parameter. No cancellation of errors occurs if one consistently uses Mie theory in the retrieval algorithm and then in computing the albedo for the retrieved aerosol optical thickness.

Mishchenko, M. I.↗
NASA NTRS2002

Towards Improved MODIS Aerosol Retrieval over the US East Coast Region: Re-examining the Aerosol Model and Surface Assumptions

The MODerate resolution Imaging Spectrometer (MODIS) aboard the Terra and recently the Aqua platform, produces a set of aerosol products over both ocean and land regions. Previous validation efforts have shown that from a global perspective, aerosol optical depth (AOD) is successfully retrieved from MODIS. Even over coastal regions, the over- land and over-ocean retrievals are consistent with each other, and well matched with ground-based sunphotometer measurements (such as AERONET). However, the East Coast of the United States is one region where there is consistently a discrepancy between land and ocean retrievals. Over the ocean, MODIS AODs are consistent with coastal sunphotometer measurements, but over land, AODs are consistently over- estimated. In this study we use field data from the Chesapeake Lighthouse and Aircraft Measurements for Satellites experiment (CLAMS), (held during summer 2001) to determine the aerosol properties at a number of sites. Using the 6-S radiative transfer package, we compute simulated satellite radiances and compare them with observed MODIS radiances. We believe that the AOD over-estimation is not likely due to an incorrect choice of the urban/industrial aerosol models. Using 6-S to do an atmospheric correction for a very low AOD case, we show rather, that the discrepancies are likely a result of incorrect assumptions about the surface reflectance properties. Understanding and improving MODIS retrievals over the East Coast will not only improve the global quality of MODIS, but also would enable the use of MODIS as a tool for monitoring regional aerosol events.

Levy, R. C.↗
NASA NTRS2004

Cavity Ring-Down Measurement of Aerosol Optical Properties During the Asian Dust Above Monterey Experiment and DOE Aerosol Intensive Operating Period

Large uncertainties in the effects of aerosols on climate require improved in-situ measurements of extinction coefficient and single-scattering albedo. This paper describes preliminary results from Cadenza, a new continuous wave cavity ring-down (CW-CRD) instrument designed to address these uncertainties. Cadenza measures the aerosol extinction coefficient for 675 nm and 1550 nm light, and simultaneously measures the scattering coefficient at 675 nm. In the past year Cadenza was deployed in the Asian Dust Above Monterey (ADAM) and DOE Aerosol Intensive Operating Period (IOP) field projects. During these flights Cadenza produced measurements of aerosol extinction in the range from 0.2 to 300/Mm with an estimated precision of 0.1/Mm for 1550 nm light and 0.2/Mm for 675 nm light. Cadenza data from the ADAM and Aerosol IOP missions compared favorably with data from the other instruments aboard the CIRPAS Twin Otter aircraft and participating in those projects. We present comparisons between the Cadenza measurements and those from a TSI nephelometer, Particle Soot Absorption Photometer (PSAP), and the AATS 14 sun-photometer. Measurements of the optical properties of smoke and dust plumes sampled during these campaigns are presented and estimates of heating rates due to these plumes are made.

Ricci, K.↗
NASA NTRS2003

Airborne Cavity Ring-Down Measurement of Aerosol Extinction and Scattering During the Aerosol IOP

Large uncertainties in the effects of aerosols on climate require improved in-situ measurements of extinction coefficient and single-scattering albedo. This paper describes preliminary results from Cadenza, a new continuous wave cavity ring-down (CW-CRD) instrument designed to address these uncertainties. Cadenza measures the aerosol extinction coefficient for 675 nm and 1550 nm light, and simultaneously measures the scattering coefficient at 675 nm. In the past year Cadenza was deployed in the Asian Dust Above Monterey (ADAM) and DOE Aerosol Intensive Operating Period (IOP) field projects. During these flights Cadenza produced measurements of aerosol extinction in the range from 0.2 to 300 Mm-1 with an estimated precision of 0.1 Min-1 for 1550 nm light and 0.2 Mm-1 for 675 nm light. Cadenza data from the ADAM and Aerosol IOP missions compared favorably with data from the other instruments aboard the CIRPAS Twin Otter aircraft and participating in those projects.= We present comparisons between the Cadenza measurements and those friom a TSI nephelometer, Particle Soot Absorption Photometer (PSAP), and the AATS 14 sun-photometer. Measurements of the optical properties of smoke and dust plumes sampled during these campaigns are presented and estimates of heating rates due to these plumes are made.

Strawa, A. W.↗
NASA NTRS2004

Measurements of HNO3, SO2 High Resolution Aerosol SO4 (sup 2-), and Selected Aerosol Species Aboard the NASA DC-8 Aircraft: During the Transport and Chemical Evolution Over the Pacific Airborne Mission (TRACE-P)

The UNH investigation during TRACE-P provided measurements of selected acidic gases and aerosol species aboard the NASA DC-8 research aircraft. Our investigation focused on measuring HNO3, SO2, and fine (less than 2 microns) aerosol SO4(sup 2-) with two minute time resolution in near-real-time. We also quantified mixing ratios of aerosol ionic species, and aerosol (210)Pb and (7)Be collected onto bulk filters at better than 10 minute resolution. This suite of measurements contributed extensively to achieving the principal objectives of TRACE-P. In the context of the full data set collected by experimental teams on the DC-8, our observations provide a solid basis for assessing decadal changes in the chemical composition and source strength of Asian continental outflow. This region of the Pacific should be impacted profoundly by Asian emissions at this time with significant degradation of air quality over the next few decades. Atmospheric measurements in the western Pacific region will provide a valuable time series to help quantify the impact of Asian anthropogenic activities. Our data also provide important insight into the chemical and physical processes transforming Asian outflow during transport over the Pacific, particularly uptake and reactions of soluble gases on aerosol particles. In addition, the TRACE-P data set provide strong constraints for assessing and improving the chemical fields simulated by chemical transport models.

Talbot, Robert W.↗
NASA NTRS2005

In Situ Aerosol Profile Measurements and Comparisons with SAGE 3 Aerosol Extinction and Surface Area Profiles at 68 deg North

Under funding from this proposal three in situ profile measurements of stratospheric sulfate aerosol and ozone were completed from balloon-borne platforms. The measured quantities are aerosol size resolved number concentration and ozone. The one derived product is aerosol size distribution, from which aerosol moments, such as surface area, volume, and extinction can be calculated for comparison with SAGE III measurements and SAGE III derived products, such as surface area. The analysis of these profiles and comparison with SAGE III extinction measurements and SAGE III derived surface areas are provided in Yongxiao (2005), which comprised the research thesis component of Mr. Jian Yongxiao's M.S. degree in Atmospheric Science at the University of Wyoming. In addition analysis continues on using principal component analysis (PCA) to derive aerosol surface area from the 9 wavelength extinction measurements available from SAGE III. Ths paper will present PCA components to calculate surface area from SAGE III measurements and compare these derived surface areas with those available directly from in situ size distribution measurements, as well as surface areas which would be derived from PCA and Thomason's algorithm applied to the four wavelength SAGE II extinction measurements.

Source record↗