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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 145 records · Page 8

Wigner time delay in photodetachment

Using Cl - as a test case,Wigner time delay in the photodetachment process has been investigated theoretically, along with the photoionization of the isoelectronic Ar atom, for the outer 3p shell using the relativistic-random-phase approximation (RRPA). Time delay was probed in these systems from threshold to 80 eV, to investigate threshold effects, the centrifugal barrier shape resonance, and the Cooper minimum region. This study focuses on Cl - because, for negative ions, the phase of the photoemission process is not dominated by the Coulomb phase as it is in photoionization. The results show significant differences, both qualitative and quantitative, between the time delays for Cl - and Ar photoemission at low photoelectron energy, but they are rather similar in the Cooper minimum region, where the Coulomb phase is small. In particular, the Wigner time delay in Cl - exhibits a dramatic energy dependence just above threshold, and a rapidly increasing time delay in the vicinity of the shape resonance. A strong angular dependence of time delay has also been found near the threshold region for the Cl - case, and is absent in the case of the photoionization of Ar. The origin of these phenomenologies is explained and a prospectus for future work is presented.

74 ATOMIC AND MOLECULAR PHYSICS↗

X-ray spectra of Hercules X-1. 3: Pulse phase dependence in high energy continuum

Pulse phase-dependent spectral changes in the high energy (less than 20 keV) continuum of Hercules X-1 were observed. Cyclotron absorption of underlying continua can reproduce the observed angular dependence in the high energy cutoff. Implications of this model, which include the possibility of determining the angular separation between the line of sight and the neutron star magnetic field if the absorbing electron spectrum is known are discussed.

Pravdo, S. H.↗

Axisymmetric Radiative Transfer Models of Kilonovae

The detailed observations of GW170817 proved for the first time directly that neutron star mergers are a major production site of heavy elements. The observations could be fit by a number of simulations that qualitatively agree, but can quantitatively differ (e.g., in total r-process mass) by an order of magnitude. We categorize kilonova ejecta into several typical morphologies motivated by numerical simulations, and apply a radiative transfer Monte Carlo code to study how the geometric distribution of the ejecta shapes the emitted radiation. We find major impacts on both spectra and light curves. The peak bolometric luminosity can vary by two orders of magnitude and the timing of its peak by a factor of five. These findings provide the crucial implication that the ejecta masses inferred from observations around the peak brightness are uncertain by at least an order of magnitude. Mixed two-component models with lanthanide-rich ejecta are particularly sensitive to geometric distribution. A subset of mixed models shows very strong viewing angle dependence due to lanthanide "curtaining," which persists even if the relative mass of lanthanide-rich component is small. The angular dependence is weak in the rest of our models, but different geometric combinations of the two components lead to a highly diverse set of light curves. We identify geometry-dependent P Cygni features in late spectra that directly map out strong lines in the simulated opacity of neodymium, which can help to constrain the ejecta geometry and to directly probe the r-process abundances.

79 ASTRONOMY AND ASTROPHYSICS↗

cos ( 4 φ ) azimuthal anisotropy in small- x DIS dijet production beyond the leading power TMD limit

Here we determine the first correction to the quadrupole operator in high-energy QCD beyond the transverse momentum dependent (TMD) limit of Weizsäcker-Williams and linearly polarized gluon distributions. These functions give rise to isotropic, respectively, ~cos2$\phi$ angular distributions in deep inelastic scattering (DIS) dijet production. On the other hand, the correction produces a ~cos4$\phi$ angular dependence which is suppressed by one additional power of the dijet transverse momentum scale (squared) P 2 .

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

Quantum Interference in Two-Atom Resonant X-ray Scattering of an Intense Attosecond Pulse

We theoretically investigate resonant x-ray scattering from two noninteracting Ne+ ions driven by an intense attosecond pulse using a nonrelativistic, QED-based time-dependent framework. Our model includes Rabi oscillations, photoionization, Auger decay, and quantum interference among elastic scattering and resonance fluorescence pathways. We analyze how the total scattering signal depends on pulse intensity, atomic configuration, and initial electronic state. We find that the total resonant scattering yield exceeds its nonresonant counterpart; the angular dependence of the signal qualitatively resembles a two-atom structure factor; and the visibility of interference fringes is sensitive to pulse area and the initial electronic state. Only a subset of final states reached via resonance fluorescence exhibits interference, determined by the indistinguishability of photon emission pathways. Fringe visibility is maximized in the linear scattering regime, where ionization is minimal and resonance fluorescence pathways can be largely indistinguishable. These results highlight optimal conditions for applying ultrafast resonant x-ray scattering to single-particle imaging.

Venkatesh, Akilesh↗

Retroreflection of Optical Radiation from Ellipsoidal-Porous Surfaces

The retroreflection of optical radiation from surfaces with roughness in the form of ellipsoidal pores and two-level roughness in the form of convex ellipsoids with elliptical-porous surfaces is studied using the ROKS-RG Monte-Carlo method software in the geometrical-optics approximation. The dependence of the retroreflection phase function on the parameters of bodies that simulates the rough surface is analyzed. It is shown that the angular dependence of the retroreflection from porous rough surfaces with arbitrarily oriented pores and the aspect ratio higher than unity is a pronounced peak with concave sides at all incidence angles.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

A spectral filter for ESMR's sidelobe errors

Fourier analysis was used to remove periodic errors from a series of NIMBUS-5 electronically scanned microwave radiometer brightness temperatures. The observations were all taken from the midnight orbits over fixed sites in the Australian grasslands. The angular dependence of the data indicates calibration errors consisted of broad sidelobes and some miscalibration as a function of beam position. Even though an angular recalibration curve cannot be derived from the available data, the systematic errors can be removed with a spectral filter. The 7 day cycle in the drift of the orbit of NIMBUS-5, coupled to the look-angle biases, produces an error pattern with peaks in its power spectrum at the weekly harmonics. About plus or minus 4 K of error is removed by simply blocking the variations near two- and three-cycles-per-week.

Chesters, D.↗

Expectations for high energy diffuse galactic neutrinos for different cosmic ray distributions

The interaction of cosmic rays with the gas contained in our Galaxy is a guaranteed source of diffuse high energy neutrinos. We provide expectations for this component by considering different assumptions for the cosmic ray distribution in the Galaxy which are intended to cover the large uncertainty in cosmic ray propagation models. We calculate the angular dependence of the diffuse galactic neutrino flux and the corresponding rate of High Energy Starting Events in IceCube by including the effect of detector angular resolution. Moreover we discuss the possibility to discriminate the galactic component from an isotropic astrophysical flux. We show that a statistically significant excess of events from the galactic plane in present IceCube data would disfavour models in which the cosmic ray density is uniform , thus bringing relevant information on the cosmic ray radial distribution.

79 ASTRONOMY AND ASTROPHYSICS↗

Focused ion beam milling of polycrystalline diamond

Focused ion beam (FIB) technology has a large potential for precise milling of ultrahard materials such as diamond. However, studies of the sputtering of diamond with ion species and energies relevant to the FIB technology are scarce. Here, we report a systematic study of the sputtering of polycrystalline diamond surfaces with ion beams in a wide range of ion energies (2 - 30 keV), incident beam angles (0 - 80°), and ion masses (N, O, Ar, and Xe). Results show that the sputter yield is relatively insensitive to ion energy but strongly depends on the ion species and incident beam angles. Bombardment with O ions results in sputter yields that are significantly larger than ballistic predictions due to chemical etching effects. Characteristic surface ripples develop for oblique beam incidence angle irradiation. The critical beam tilt angle for the onset of ripple formation and the wavelength of the ripples depend on ion species and energies. Ripples appear to suppress ion reflection at high beam tilt angles and, hence, a peak in the sputter yield angular dependence. In conclusion, these results have direct implications for the development of process parameter maps for high-precision ion-beam milling of diamond.

36 MATERIALS SCIENCE↗

Uniformity simulation of multiple-beam irradiation of a spherical laser target with the inclusion of radiation absorption and refraction

We consider the physicomathematical model for the simulation of the angular laser flux distribution in a spherical target with the inclusion of radiation refraction in the corona. The irradiation uniformity is simulated using the target irradiation scheme on a megajoule multiple-beam laser facility. Calculations are made of the time-dependent angular distribution of absorbed flux and of the angular distribution of the time-integrated characteristic – the absorbed energy with allowance for the temporal shape of laser pulses – as well as of the time dependence of absorption efficiency. Different versions of target irradiation are considered. Under conventional irradiation it is assumed that the axes of all laser beams of equal energy pass through the target centre and the irradiation nonuniformity is due to its geometry only. Also examined are three unconventional irradiation versions: when there is a small spread of beam energies, when the target is displaced from the common beam pointing centre, and when the beam axes have small random deviations from the target centre. It is shown that the nonuniformity of the angular distribution of absorbed flux is greatest when the target is displaced from the beam pointing centre. (interaction of laser radiation with matter. laser plasma)

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Determining Orientations of Optical Transition Dipole Moments Using Ultrafast X-ray Scattering

Here, identification of the initially prepared, optically active state remains a challenging problem in many studies of ultrafast photoinduced processes. We show that the initially excited electronic state can be determined using the anisotropic component of ultrafast time-resolved X-ray scattering signals. The concept is demonstrated using the time-dependent X-ray scattering of N -methyl morpholine in the gas phase upon excitation by a 200 nm linearly polarized optical pulse. Analysis of the angular dependence of the scattering signal near time zero renders the orientation of the transition dipole moment in the molecular frame and identifies the initially excited state as the 3pz Rydberg state, thus bypassing the need for further experimental studies to determine the starting point of the photoinduced dynamics and clarifying inconsistent computational results.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

Emissivity Measurements of Additively Manufactured Materials

The emissivity of common 3D printing materials such as ABS and PLA were measured using a reflectivity meter and have the measured value of approximately 0.92. Adding a conductive material to the filament appears to cause a decrease in the emissivity of the surface. The angular dependence of the emissivity and the apparent temperature was measured using a FLIR infrared camera showing that the emissivity does not change much for shallow angles less than 40 angular degrees, and drops off dramatically after 70 angular degrees.

36 MATERIALS SCIENCE↗

Cross Section Measurements Using the Zero Degree Detector

The Zero Degree Detector (ZDD) is an instrument that has been used in accelerator exposures to measure the angular dependence of particles produced in heavy ion fragmentation experiments. The ZDD uses two identical layers of pixelated silicon detectors that make coincident measurements over the active area of the instrument. The angular distribution of secondary particle produced in nuclear interactions for several heavy ions: and target materials will be presented along with performance characteristic of the instrument.

Christl, M. J.↗

Ionization of HCCI Neutral and Cations by Strong Laser Fields Simulated With Time Dependent Configuration Interaction

Strong field ionization of neutral iodoacetylene (HCCI) can produce a coherent superposition of the X and A cations. This superposition results in charge migration between the CC π orbital and the iodine π-type lone pair which can be monitored by strong field ionization with short, intense probe pulses. Strong field ionization of the X and A states of HCCI cation was simulated with time-dependent configuration interaction using singly ionized configurations and singly excited, singly ionized configurations (TD-CISD-IP) and an absorbing boundary. Studies with static fields were used to obtain the 3-dimensional angular dependence of instantaneous ionization rates by strong fields and the orbitals involved in producing the cations and dications. The frequency of charge oscillation is determined by the energy separation of the X and A states; this separation can change depending on the direction and strength of the field. Furthermore, fields along the molecular axis can cause extensive mixing between the field-free X and A configurations. For coherent superpositions of the X and A states, the charge oscillations are characterized by two frequencies–the driving frequency of the laser field of the probe pulse and the intrinsic frequency due to the energy separation between the X and A states. For linear and circularly polarized pulses, the ionization rates show marked differences that depend on the polarization direction of the pulse, the carrier envelope phase and initial phase of the superposition. Varying the initial phase of the superposition at the beginning of the probe pulse is analogous to changing the delay between the pump and probe pulses. The charge oscillation in the coherent superposition of the X and A states results in maxima and minima in the ionization yield as a function of the superposition phase

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

TROPOMI Geometry-dependent Lambertian-Equivalent surface Reflectivity (GLER) Product for Improved Trace-Gas Retrieval

Accurate information about the reflectivity of the Earth's surface is required for most satellite retrievals of atmospheric composition, and this information is generally taken from monthly surface reflectivity climatology that neglects angular dependence. Previously we introduced Geometry-dependent Lambertian-equivalent surface reflectivity (GLER) which captures solar and satellite viewing angle dependence as well as daily and seasonal changes. GLER is calculated from simulations of Rayleigh-only top-of-atmosphere (TOA) radiances over non-Lambertian surfaces. We use NASA's Moderate Resolution Imaging Spectroradiometer (MODIS) bidirectional reflectance distribution function (BRDF) product over land and the wind-dependent Cox–Munk wave-facet slope distribution including water-leaving radiance over water to accounts for surface BRDF. We have developed global GLER product, previously for the Ozone Monitoring Instrument (OMI) and recently for Sentinel-5 Precursor (S5P) TROPOspheric Monitoring Instrument (TROPOMI) with several new improvements and updates. We have implemented the near real time daily V006 MODIS MCD43C1 BRDF data and gap-filled with a daily BRDF coefficient climatology created from 2002-2017 V006 MCD43GF data. The NASA’s Global Modelling Initiative hourly 0.25 x 0.25 deg Replay simulations are used for more accurate determination of pixel specific terrain pressure. To improve detection of seasonal snow/ice scenes, we use the 4-km snow cover product from the Interactive Multi-sensor Snow and Ice Mapping System (IMS). Finally, we use an improved version of the vector linearized discrete ordinate radiative transfer (VLIDORT) for update of the top-of-atmosphere (TOA) radiance look-up-tables (LUTs). We demonstrate how the use of GLER is beneficial to TROPOMI’s high spatial resolution (up to 3.5 km x 3.5 km) measurements to monitor atmospheric trace gas pollutants down to the sub-city scale.

TROPOMI↗

Resistivity near a nematic quantum critical point: Impact of acoustic phonons

We revisit the issue of the resistivity of a two-dimensional electronic system tuned to a nematic quantum critical point (QCP), focusing on the nontrivial impact of the coupling to the acoustic phonons. Due to the unavoidable linear coupling between the electronic nematic order parameter and the lattice strain fields, long-range nematic interactions mediated by the phonons emerge in the problem. By solving the semiclassical Boltzmann equation in the presence of scattering by impurities and nematic fluctuations, we determine the temperature dependence of the resistivity as the nematic QCP is approached. One of the main effects of the nematoelastic coupling is to smooth the electronic nonequilibrium distribution function, making it approach the simple cosine angular dependence even when the impurity scattering is not too strong. We find that at temperatures lower than a temperature scale set by the nematoelastic coupling, the resistivity shows the T 2 behavior characteristic of a Fermi liquid. This is in contrast to the T 4/3 low-temperature behavior expected for a lattice-free nematic quantum critical point. More importantly, we show that the effective resistivity exponent α eff (T) in ρ(T) – ρ 0 ~ T α eff (T) displays a pronounced temperature dependence, implying that a nematic QCP cannot generally be characterized by a simple resistivity exponent. Furthermore, we discuss the implications of our results to the interpretation of experimental data, particularly in the nematic superconductor FeSe 1–x S x .

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗

Quasi-Floquet Prethermalization in a Disordered Dipolar Spin Ensemble in Diamond

Floquet (periodic) driving has recently emerged as a powerful technique for engineering quantum systems and realizing nonequilibrium phases of matter. A central challenge to stabilizing quantum phenomena in such systems is the need to prevent energy absorption from the driving field. Fortunately, when the frequency of the drive is significantly larger than the local energy scales of the many-body system, energy absorption is suppressed. The existence of this so-called prethermal regime depends sensitively on the range of interactions and the presence of multiple driving frequencies. Here, we report the observation of Floquet prethermalization in a strongly interacting dipolar spin ensemble in diamond, where the angular dependence of the dipolar coupling helps to mitigate the long-ranged nature of the interaction. Moreover, we extend our experimental observation to quasi-Floquet drives with multiple incommensurate frequencies. In contrast to a single-frequency drive, we find that the existence of prethermalization is extremely sensitive to the smoothness of the applied field. In conclusion, our results open the door to stabilizing and characterizing nonequilibrium phenomena in quasiperiodically driven systems.

36 MATERIALS SCIENCE↗

Anomalous and planar Hall effects in Co 1−x Ho x thin films across the magnetic sublattice compensation temperature

Metallic amorphous ferrimagnets derived from alloying 3d transition metals with 4f-electron rare earths host fascinating effects of compensation between the 3d and 4f magnetic sublattices. Here, a detailed study of the anisotropic magnetoresistance (Δρ xx ), planar Hall effect (ρ xy PHE ), and anomalous Hall effect (ρ xy AHE ) is reported on a series of Co 1−x Ho x thin films over a wide field–temperature (H–T) phase space. Close to the magnetic compensation temperature, the ρ xy AHE –H loops show a double sign reversal and signatures of spin-flop transition at higher fields. The Δρ xx and ρ xy PHE also display strong deviations from the classical angular dependence seen in soft ferromagnets like permalloy as the angle ϕ between in-plane current and magnetic field is scanned from 0 to 2π. It is argued that the non-zero orbital angular momentum of Ho ions in the lattice and stabilization of bubble domains below magnetic saturation may be responsible for such features. Direct imaging of magnetic textures with x-ray photoelectron microscopy shows the formation of stripe domain patterns in the regime of sublattice compensation. Such stripes are likely to transform into magnetic bubbles before full saturation is reached in a large magnetic field.

36 MATERIALS SCIENCE↗