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Results for “CIRCULAR POLARIZATION”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 145 records · Page 8
All sourcesNASA NTRSDOE OSTI
NASA NTRS2017

A Ka-Band (26 GHz) Circularly Polarized 2x2 Microstrip Patch Sub-Array with Compact Feed

A Ka-Band (26 gigahertz) 2 by 2 sub-array with square-shaped microstrip patch antenna elements having two truncated corners for circular polarization (CP) is presented. In addition, the layout for a new compact microstrip feed network for the sub-array is also presented. The compact feed network offers a footprint size reduction of near 60 percent over traditional sub-array at 26 gigahertz. Experimental data indicates that a truncation amount a equals 0.741 millimeters for an isolated patch element results in a return loss (S (sub II)) of minus 35 decibels at 26.3 gigahertz. Furthermore, the measured S (sub II) for the proof-of-concept sub-array with the above elements is better than minus 10.0 decibels at 27.7 gigahertz. However, the impedance match and the operating frequency can be fine-tuned to 26 gigahertz by adjusting the feed network dimensions. Lastly, good agreement is observed between the measured and simulated S (sub II) for the subarray for both right hand and left hand CP. The goal of this effort is utilize the above sub-array as a building block for a larger N by N element array, which would serve as a feed for a reflector antenna for satellite communications.

Microstrip↗
DOE OSTI2023

Nonlocal metasurface for circularly polarized light detection

Modern-day sensing and imaging applications increasingly rely on accurate measurements of the primary physical quantities associated with light waves: intensity, wavelength, directionality, and polarization. These are conventionally performed with a series of bulky optical elements, but recently, it has been recognized that optical resonances in nanostructures can be engineered to achieve selective photodetection of light waves with a specific set of predetermined properties. Here, we theoretically illustrate how a thin silicon layer can be patterned into a dislocated nanowire-array that affords detection of circularly polarized light with an efficiency that reaches the theoretical limit for circular dichroism of a planar detector in a symmetric external environment. The presence of a periodic arrangement of dislocations is essential in achieving such unparalleled performance as they enable selective excitation of nonlocal, guided-mode resonances for one handedness of light. We also experimentally demonstrate compact, high-performance chiral photodetectors created from these dislocated nanowire-arrays. This work highlights the critical role defects can play in enabling new nanophotonic functions and devices.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗
DOE OSTI2023

Chiral Perovskite Nanoplatelets with Tunable Circularly Polarized Luminescence in the Strong Confinement Regime

Chiral perovskite nanocrystals have emerged as an interesting chiral excitonic platform that combines both structural flexibility and superior optoelectronic properties. Despite several recent demonstrations of optical activity in various chiral perovskite nanocrystals, efficient circularly polarized luminescence (CPL) with tunable energies remains a challenge. The chirality imprinting mechanism as a function of perovskite nanocrystal dimensionality remains elusive. Here, in this study, atomically thin inorganic perovskite nanoplatelets (NPLs) are synthesized with precise control of layer thickness and are functionalized by chiral surface ligands, serving as a unique platform to probe the chirality transfer mechanism at the organic/perovskite interface. It is found that chirality is successfully imprinted into mono-, bi-, and tri-layer inorganic perovskite NPLs, exhibiting tunable circular dichroism (CD) and CPL responses. However, chirality transfer decreases in thicker NPLs, resulting in decreased CD and CPL dissymmetry factors for thicker NPLs. Aided by large-scale first-principles calculations, it is proposed that chirality transfer is mainly mediated through a surface distortion rather than a hybridization of electronic states, giving rise to symmetry breaking in the perovskite lattice and spin-split conduction bands. The findings described here provide an in-depth understanding of chirality transfer and design principles for distorted-surface perovskites for chiral photonic applications.

36 MATERIALS SCIENCE↗
DOE OSTI2021

Transitions between Rydberg states in two-color corotating circularly polarized laser pulses

We present a study of higher-order Raman (Λ, V, and S) transitions between Rydberg states involving the absorption and emission of at least three photons in the interaction of two-color corotating circularly polarized laser pulses with the hydrogen atom. Our analysis is based on results of numerical solutions of the corresponding time-dependent Schrödinger equation. Here, the results for the interaction with (ω,2ω) fields show that the simultaneous interaction with both fields results in an excited state distribution over a broad range of magnetic quantum numbers. Indications of the impact of the Λ, V, and S transitions are found via the analysis of final distributions resulting from the preparation of the atom in specific Rydberg states. Furthermore, we show that similar mechanisms for the redistribution of population between Rydberg states are present in two-color fields with larger differences in the central frequencies, i.e., (ω,3ω) and (ω,4ω) fields.

74 ATOMIC AND MOLECULAR PHYSICS↗
NASA NTRS1972

NGC 1068, 3C 273, and Scorpius X-1 - Circular polarization disputed.

Discussion of data for the Seyfert galaxy NGC 1068, the quasar 3C 273, and the X-ray source Sco X-1, for all of which it has been claimed or strongly suggested that they have large circular polarization of the order of 1% (Severny et al., 1971). In contrast the present authors obtained unambiguously null results with upper limits about 0.05% for NGC 1068 and 3C 273. For Sco X-1 no statistically significant polarization was found on three nights, and only some marginal evidence for a fluctuation or transient polarization on one night.

Kemp, J. C.↗
DOE OSTI2019

Dissociative photoionization of NO across a shape resonance in the XUV range using circularly polarized synchrotron radiation

We report benchmark results for dissociative photoionization (DPI) spectroscopy and dynamics of the NO molecule in the region of the σ* shape resonance in the ionization leading to the NO + (c 3 Π) ionic state. The experimental study combines well characterized extreme ultraviolet (XUV) circularly polarized synchrotron radiation, delivered at the DESIRS beamline (SOLEIL), with ion-electron coincidence 3D momentum spectroscopy. The measured (N + , e) kinetic energy correlation diagrams reported at four discrete photon energies in the extended 23-33 eV energy range allow for resolving the different active DPI reactions and underline the importance of spectrally resolved studies using synchrotron radiation in the context of time-resolved studies where photoionization is induced by broadband XUV attosecond pulses. In the dominant DPI reaction which leads to the NO + (c 3 Π) ionic state, photoionization dynamics across the σ* shape resonance are probed by molecular frame photoelectron angular distributions where the parallel and perpendicular transitions are highlighted, as well as the circular dichroism CDAD(θ e ) in the molecular frame. The latter also constitute benchmark references for molecular polarimetry. The measured dynamical parameters are well described by multichannel Schwinger configuration interaction calculations. Finally, similar results are obtained for the DPI spectroscopy of highly excited NO + electronic states populated in the explored XUV photon energy range.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2023

Wavelength-Dependent Spin Excitation with Circularly Polarized Light in CdSe Nanoplatelets

Zinc-blende (ZB) cadmium selenide (CdSe) nanoplatelets (NPLs) have drawn increasing attention as an ideal condensed-phase material for facilitating photon-to-spin transduction in quantum networks. Yet, a systematic investigation of their fidelity in converting circularly polarized light (CPL) to exciton spin polarization as a function of excitation wavelength is lacking. Here, this work demonstrates using time-resolved transient absorption (TA) spectroscopy combined with density functional theory calculations that ZB CdSe NPLs exhibit wavelength-dependent CPL-induced spin polarization. The capacity of CPL to inject spin polarization is maximized for resonant excitation of band-edge valence-to-conduction band (VB/CB) transitions, and the degree to which CPL induces spin polarization can be modified for non-resonant excitation wavelengths as excitation occurs at k-points away from the Γ point from VB states with varying degrees of mixed heavy-hole (HH) and light-hole (LH) characters. Furthermore, it is highlighted that spin polarization within the LH exciton (LX) population created from resonant LH/CB excitation is retained upon LX → HH exciton (HX) relaxation due to the slow electron spin-flip rate (~1.1 ps) compared to the LH → HH inter-band relaxation rate (~200 fs).

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
DOE OSTI2025

Differential absorption of circularly polarized light by a centrosymmetric crystal

Crystalline solids are governed by universal structure-property relationships derived from their crystal symmetry, leading to paradigmatic rules on what properties they can and cannot exhibit. A long-held structure-property relationship is that centrosymmetric crystals cannot differentially absorb circularly polarized light. In this study, we demonstrate the design, synthesis, and characterization of the centrosymmetric material Li 2 Co 3 (SeO 3 ) 4 , which violates this relationship not by defying symmetry-imposed selection rules but by invoking a photophysical process not previously characterized for crystalline solids. This process originates from an interference between linear dichroism and linear birefringence, referred to as LD-LB, and involves strong chiroptical signals that invert upon sample flipping. Here, in addition to enabling a chiroptical response under centrosymmetry, this process opens up photonic engineering opportunities based on crystalline solids.

36 MATERIALS SCIENCE↗
NASA NTRS1999

Efficient IR Transmission Diffraction Grating for Circularly Polarized Light

Numerical methods, using rigorous coupled wave theory, are used to design rectangular relief diffraction gratings for an infrared application which requires comparable first order efficiencies in the TE and TM polarization states. The depth, period, and fill factor of the grating are varied to identify optimal two level binary lamellar grating profiles which predict efficiencies for individual TM and TE polarizations above 75 percent, while keeping the difference between the two efficiencies within 10 percent. The application at hand is a rotating, transmissive diffractive scanner for space-based coherent lidar. The operating wavelength is 2.0 microns. A collimated, circularly polarized beam is incident on the diffractive scanner at the Bragg angle; 30 and 45 degree beam deflection angles being studied. Fused silica is the substrate material of choice. Selected designs are fabricated on 3 inch fused silica substrates using lithographic methods. The performance of the test pieces is measured and compared to theoretical predictions.

Cole, Helen↗
DOE OSTI2023

Turn‐on Circularly Polarized Luminescence in Chiral Indium Chlorides by 5s 2 Metal Centers

Abstract Introducing chirality into the metal‐halide hybrids has enabled many emerging properties including chiroptical activity, spin‐dependent transport, and ferroelectricity. However, most of the chiral metal‐halide hybrids to date are non‐emissive, and the underlying mechanism remains elusive. Here, we show a new strategy to turn on the circularly polarized luminescence (CPL) in chiral metal‐halide hybrids. We demonstrate that alloying Sb 3+ into chiral indium‐chloride hybrids dramatically increases the photoluminescence quantum yield in two new series of chiral indium‐antimony chlorides. These materials exhibit strong CPL signals with tunable energy and a high dissymmetry factor up to 1.5×10 −2 . Mechanistic studies reveal that the emission originates from the self‐trapped excitons centered in 5s 2 Sb 3+ . Moreover, near‐ultraviolet pumped white light is demonstrated with a polarization up to 6.0 %. Our work demonstrates new strategies towards highly luminescent chiral metal‐halide hybrids.

Wang, Zhiyu↗
NASA NTRS1985

Omnidirectional, circularly polarized, cylindrical microstrip antenna

A microstrip cylindrical antenna comprised of two concentric subelements on a ground cylinder, a vertically polarized (E-field parallel to the axis of the antenna cylinder) subelement on the inside and a horizontally polarized (E-field perpendicular to the axis) subelement on the outside. The vertical subelement is a wraparound microstrip radiator. A Y-shaped microstrip patch configuration is used for the horizontally polarized radiator that is wrapped 1.5 times to provide radiating edges on opposite sides of the cylindrical antenna for improved azimuthal pattern uniformity. When these subelements are so fed that their far fields are equal in amplitude and phased 90.degree. from each other, a circularly polarized EM wave results. By stacking a plurality of like antenna elements on the ground cylinder, a linear phased array antenna is provided that can be beam steered to the desired elevation angle.

Stanton, Philip H.↗
DOE OSTI2022

Turn-on Circularly Polarized Luminescence in Chiral Indium Chlorides by 5s 2 Metal Centers

Introducing chirality into the metal-halide hybrids has enabled many emerging properties including chiroptical activity, spin-dependent transport, and ferroelectricity. However, most of the chiral metal-halide hybrids to date are non-emissive, and the underlying mechanism remains elusive. Here, in this study, we show a new strategy to turn on the circularly polarized luminescence (CPL) in chiral metal-halide hybrids. We demonstrate that alloying Sb 3+ into chiral indium-chloride hybrids dramatically increases the photoluminescence quantum yield in two new series of chiral indium-antimony chlorides. These materials exhibit strong CPL signals with tunable energy and a high dissymmetry factor up to 1.5×10 -2 . Mechanistic studies reveal that the emission originates from the self-trapped excitons centered in 5s 2 Sb 3+ . Moreover, near-ultraviolet pumped white light is demonstrated with a polarization up to 6.0 %. Our work demonstrates new strategies towards highly luminescent chiral metal-halide hybrids.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS2017

Evolution of Circular Polarization Ratio (CPR) Profiles of Kilometer-scale Craters on the Lunar Maria

When sufficiently large impact craters form on the Moon, rocks and unweathered materials are excavated from beneath the regolith and deposited into their blocky ejecta. This enhances the rockiness and roughness of the proximal ejecta surrounding fresh impact craters. The interior of fresh craters are typically also rough, due to blocks, breccia, and impact melt. Thus, both the interior and proximal ejecta of fresh craters are usually radar bright and have high circular polarization ratios (CPR). Beyond the proximal ejecta, radar-dark halos are observed around some fresh craters, suggesting that distal ejecta is finer-grained than background regolith. The radar signatures of craters fade with time as the regolith grows.

moon↗
DOE OSTI2022

Aggregation-Induced Emission and Circularly Polarized Luminescence Duality in Tetracationic Binaphthyl-Based Cyclophanes

Here, we report an approach to the synthesis of highly charged enantiopure cyclophanes by the insertion of axially chiral enantiomeric binaphthyl fluorophores into the constitutions of pyridinium-based macrocycles. Remarkably, these fluorescent tetracationic cyclophanes exhibit a significant AIE compared to their neutral optically active binaphthyl precursors. A combination of theoretical calculations and time-resolved spectroscopy reveal that the AIE originates from limited torsional vibrations associated with the axes of chirality present in the chiral enantiomeric binaphthyl units and the fine-tuning of their electronic landscape when incorporated within the cyclophane structure. Furthermore, these highly charged enantiopure cyclophanes display CPL responses both in solution and in the aggregated state. This unique duality of AIE and CPL in these tetracationic cyclophanes is destined to be of major importance in future development of photonic devices and bio-applications.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1971

Wide-angle, circularly polarized, omnidirectional-array antenna

Modified conventional turnstile antenna features bifoliate pattern with relatively high gain and good circularity over solid area enclosed by the 0.26 and 1.31 radian angles of elevation. These antennas are intended for high altitude balloon use, their permissible weight is restricted to one pound.

Boyer, R. B.↗