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Results for “Collisional Radiative Modeling”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 145 records · Page 8
All sourcesNASA NTRSDOE OSTI
DOE OSTI2025

Coupling to rotational manifolds to improve gas-phase pump–probe spectroscopic models

The physical picture of gas-phase optical transitions is normally presented as an isolated two-level system balanced by upward and downward processes. Isolated models assume a phenomenological treatment of collisional dephasing but do not strictly account for collisional population exchange with the rotational baths. While this assumption is valid under low-intensity conditions, where excitation is rate-limiting, isolated models can deviate from Beer’s Law at sufficient pressures and monochromatic intensities when both collisional broadening and power broadening are comparable to (or greater than) lifetime broadening, which are not uncommon conditions for cavity enhanced spectroscopies in the mid-IR spectral range. Although this problem has been addressed by rate-equation models for linear absorption measurements, a general treatment for multi-level quantum mechanical models suitable for non-linear absorption measurements (two-photon/two-color/pump–probe) is lacking. Isolated models require physical parameter inputs that disagree with expected values by at least an order of magnitude. These non-physical models undermine the ability to predict non-linear signal strengths under untested conditions and thereby limit the potential to optimize the sensitivity of non-linear spectroscopies and to expand their analytical applications (e.g., new analytes and/or buffer gases, changes in cavity free-spectral-range, changes in intracavity powers or wavelengths, and accurate investigation of physical phenomena). In this study, we derive bath-coupled models for gaseous pump–probe spectroscopy by application of the quantum Lindblad equation and detailed balance. Bath-coupled models are shown to fit data consistently across variations in intensity and agree with all physically expected values.

Cavity ring-down spectroscopy↗
NASA NTRS1980

Dynamics of micrometeoroids

The spatial and orbital distributions of meteoroids of mass less than 10 to the -8 g are discussed. Pioneer 8 and 9, HEOS-2 and Helios 1 observations of the smallest meteoroids leaving the solar system in hyperbolic orbits due to radiation pressure (beta particles), intermediate mass particles arriving from the heliocentric spacecraft apex direction (alpha meteoroids) and the largest micrometeoroids observed with no preferred directionality (sporadic meteoroids) are reviewed, and evidence for the three groups of dynamically different micrometeoroids in lunar microcrater statistics is indicated. The collisional model of the origin of dust particles from the dispersion of sporadic meteoroids of cometary origin due to the Poynting-Robertson effect and collisions is then applied to account for the dynamics of the beta and alpha micrometeoroids.

Gruen, G.↗
NASA NTRS1987

X-ray and ultraviolet radiation from accreting white dwarfs. IV - Two-temperature treatment with electron thermal conduction

Results are reported from two-temperature calculations of the structures and X-ray spectra of radiation shocks generated by accretion onto nonmagnetic white dwarfs. The approach was necessitated by the domination of bremsstrahlung in the emission region by Compton cooling. Features of the shock model, which includes steady, spherical infall of fully ionized plasma and dominance of the stand-off shock by collisional processes, are summarized. A maximum hard X-ray temperature of about 50 keV and a maximum hard X-ray luminosity of 2 x 10 to the 36th ergs/sec were obtained. The results prove that the bulk of accretion energy cannot be transported to the star by electron thermal conduction, provided that bremsstrahlung cooling is dominant over cyclotron cooling.

Imamura, J. N.↗
NASA NTRS1992

Analysis of the upper atmosphere CO2(nu-2) vibrational temperatures retrieved from ATMOS/Spacelab 3 observations

An analysis of the upper atmospheric (80-116 km) CO2(nu-2) vibrational temperatures retrieved from atmospheric trace molecule spectroscopy (ATMOS) experiment Spacelab 3 spectra by using a nonlocal thermodynamic equilibrium (non-LTE) radiative transfer model is presented. Thermal collisions with atmospheric atomic oxygen keep this vibrational state very close to LTE up to around 100 km. Above this height, the different deviations from LTE retrieved from ATMOS/Spacelab 3 spectra for the Northern and the Southern Hemispheres are explained in terms of this collisional process and in terms of the different kinetic temperature profiles measured at those locations. From these simultaneous observations of the kinetic and CO2(nu-2) vibrational temperatures, a deactivation rate of CO2(nu-2) by O(3P) has been derived which leads to a rate coefficient value between 3 and 6 x 10 exp -12 cu cm/s and favors an independent or negative temperature dependence rate constant for the atmospheric temperature range. Cooling rates induced by the CO2 15-micron fundamental band in the upper mesosphere and lower thermosphere were derived from the simultaneous kinetic temperature, CO2(nu-2) vibrational temperature, and CO2 concentration, as measured by ATMOS/Spacelab 3, and found to be a factor of between 5 and 10 times larger than those generally accepted until very recently.

Lopez-Puertas, M.↗
NASA NTRS2011

Modelling the Huge, Herschel-Resolved Debris Ring around HD 207129

Debris disks, which are inferred from the observed infrared excess to be ensembles of dust, rocks. and probably planetesimals, arc common features of stellar systems. As the mechanisms of their fonnation and evolution are linked to those of planetary bodies, they provide valuable infonnation. The few well-resolved debris disks are even more valuable because they can serve as modelling benchmarks and help resolve degeneracies in modelling aspects such as typical grain sizes and distances. Here, we present an analysis of the HD 207129 debris disk, based on its well-covered spectral energy distribution and Herschel/PACS images obtained in the framework of the DUNES (DUst around NEarby Stars) programme. We use an empirical power-law approach to the distribution of dust and we then model the production and removal of dust by means of collisions, direct radiation pressure, and drag forces. The resulting best-fit model contains a total of nearly 10(sup -2) Earth masses in dust, with typical grain sizes in the planetesimal beh ranging from 4 to 7 micrometers. We constrain the dynamical excitation to be low, which results in very long collisional lifetimes and a drag that notably fills the inner gap, especially at 70 micrometers. The radial distribution stretches from well within 100 AU in an unusual, outward-riSing slope towards a rather sharp outer edge at about 170-190 AU. The inner edge is therefore smoother than that reported for Fomalhaut, but the contribution from the extended halo of barely bound grains is similarly small. Both slowly self-stirring and planetary perturbations could potentially have formed and shaped this disk.

Lohne, T.↗
NASA NTRS1966

Pion production in high-energy cosmic-ray collisions.

High energy cosmic ray collisional pion production spectrum and pion energy and angle distributions in CMS and laboratory frames from Landau- Milekhin hydrodynamic model of very high energy nucleon

NUCLEON-NUCLEON SCATTERING↗
NASA NTRS1998

Analysis of IUE Observations of Hydrogen in Comets

The 15-years worth of hydrogen Lyman-alpha observations of cometary comae obtained with the International Ultraviolet Explorer (IUE) satellite had gone generally unanalyzed because of two main modeling complications. First, the inner comae of many bright (gas productive) comets are often optically thick to solar Lyman-alpha radiation. Second, even in the case of a small comet (low gas production) the large IUE aperture is quite small as compared with the immense size of the hydrogen coma, so an accurate model which properly accounts for the spatial distribution of the coma is required to invert the infrared brightnesses to column densities and finally to H atom production rates. Our Monte Carlo particle trajectory model (MCPTM), which for the first time provides the realistic full phase space distribution of H atoms throughout the coma has been used as the basis for the analysis of IUE observations of the inner coma. The MCPTM includes the effects of the vectorial ejection of the H atoms upon dissociation of their parent species (H2O and OH) and of their partial collisional thermalization. Both of these effects are crucial to characterize the velocity distribution of the H atoms. This combination of the MCPTM and spherical radiative transfer code had already been shown to be successful in understanding the moderately optically thick coma of comet P/Giacobini-Zinner and the coma of comet Halley that varied from being slightly to very optically thick. Both of these comets were observed during solar minimum conditions. Solar activity affects both the photochemistry of water and the solar Lyman-alpha radiation flux. The overall plan of this program here was to concentrate on comets observed by IUE at other time during the solar cycle, most importantly during the two solar maxima of 1980 and 1990. Described herein are the work performed and the results obtained.

Combi, Michael R.↗
NASA NTRS1976

Mass ejection from the O4f star Zeta Puppis

Profiles of P Cygni lines and displaced absorption lines observed in high-resolution Copernicus UV scans of Zeta Pup from 907 to 1738 A are compared with profile calculations to derive an optical-depth scale of the lines as a function of height or velocity in the expanding envelope. The degrees of ionization of the elements C, N, O, Si, and S under equilibrium conditions at electron temperatures of 20,000 to 1 million K, radiation temperatures of 20,000 to 50,000 K, and electron number densities of 100 million to 1 trillion per cu cm are computed with a dilution factor of 0.1, taking into account collisional ionization by electrons, radiative ionization from the ground state, radiative recombination, and dielectric recombination. Observed and predicted relative ionization fractions are then compared to determine the electron and radiation temperatures. Crude and refined estimates of the mass-loss rate and velocity law are made, and radiative acceleration in the expanding envelope is analyzed. The derived model for Zeta Pup is found to have a mass-loss rate of about 7.2 millionths of a solar mass per year, a wind velocity that increases slowly outward and reaches 700 km/s about 28 solar masses, and a nearly isothermal envelope with an electron temperature of approximately 200,000 K.

Lamers, H. J. G. L. M.↗
NASA NTRS1979

The Balmer 9 and Balmer 11 lines of He II in the sun

The Balmer 9 and 11 lines of He II at 959 A and 942 A in solar spectra are identified. These lines are produced mainly by recombination following photoionization of He II by coronal XUV radiation. From analysis of the line intensities, the theoretical model of Avrett et al. (1976), is confirmed where it was found that an appreciable amount of He (2+) is present at temperatures of 1 - 2 x 10 to the 4th K and that the anomalously strong He II 304 line is produced primarily by collisional excitation. The suggestion of Kohl (1977) that the photoionization-recombination process is more important in active regions than in the quiet sun is confirmed, and we find that the 304-A line is produced largely by recombination in solar flares.

Raymond, J. C.↗
DOE OSTI2024

Electron tail suppression and effective collisionality due to synchrotron emission and absorption in mildly relativistic plasmas

Synchrotron radiation losses are a significant cause of concern for high-temperature aneutronic fusion reactions such as proton–Boron 11. The fact that radiation losses occur primarily in the high-energy tail, where the radiation itself has a substantial impact on the electron distribution, necessitates a self-consistent approach to modeling the diffusion and drag induced by synchrotron absorption and emission. Furthermore, an accurate model must account for the fact that the radiation emission spectrum is momentum-dependent, and the plasma opacity is frequency-dependent. Here, we present a simple Fokker–Planck operator, built on a newly solved-for blackbody synchrotron diffusion operator, which captures all relevant features of the synchrotron radiation. Focusing on magnetic mirror fusion plasmas, we show that significant suppression of the electron distribution occurs for relativistic values of the perpendicular electron momentum, which therefore emit much less radiation than predicted under the assumption of a Maxwell–Jüttner distribution.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2025

An Exceptionally Powerful, Radiatively Driven Ultrafast Outflow in the Rapidly Accreting AGN RE J1034+396

We report the analysis of ∼1 Ms of XMM-Newton observations of the rapidly accreting active galactic nucleus RE J1034+396. The 0.3–9 keV EPIC-pn spectra are well described by a model consisting of steep continuum emission from the corona accompanied by relativistically blurred reflection from a highly ionized accretion disk. The source is known to exhibit strong excess soft X-ray emission, which we show is well represented by thermal disk photons Comptonized by a warm plasma spanning the inner accretion flow. Additionally, the EPIC-pn data provide compelling evidence (ΔC ∼ 60 for four additional parameters) for the presence of an ultrafast outflow (UFO) with a line-of-sight velocity v/c = 0.307$^{+0.001}_{-0.005}$, and an emission signature consistent with reflection of the corona from modestly ionized, outflowing gas. The simultaneous 0.5–2.5 keV RGS spectra show clear absorption lines. Modelling of these data confirms the presence of the UFO and constrains its equivalent hydrogen column density, log N H /(atom cm −2 ) = 21.7$^{+0.1}_{-0.2}$. The RGS data also reveal at least two warm absorber components with a modest outflow velocity (1680$^{+40}_{-50}$ km s -1 ). The measured properties and time evolution of the UFO in RE J1034+396 suggest that it is formed from collisionally ionized plasma, launched from the disk surface and accelerated by radiation pressure. The high terminal velocity and substantial absorbing column density imply that the outflow carries sufficient momentum and energy to transform its environment, being capable of driving out essentially all dust and gas it interacts with along the line of sight, even if the AGN were initially surrounded by a Compton-thick absorber.

79 ASTRONOMY AND ASTROPHYSICS↗
NASA NTRS1980

Some implications of ultraviolet observations of quasars and active galaxies

The problem of the order of magnitude discrepancy in the expected and observed ratios of the Lyman and Balmer lines in quasars and active galaxies is reviewed. Whereas early photoionization models for the emission line regions predicted F(L-alpha)/F(H-beta) not less than 40, the observations give values for this ratio in the range 3-8. Attempts at explaining the observations have involved dust, both external and internal to the emission line regions, and improved treatments of the collisional processes and radiative transfer effects in dense (Ne about 10 to the 10th/cu cm), optically thick clouds. None of the effects considered is, by itself, able to explain all the observations, and a combination of several of them is probably required.

Davidsen, A. F.↗
NASA NTRS1993

Molecular line emission models of Herbig-Haro objects. II - HCO(+) emission

We present time-dependent models of the chemistry and temperature of interstellar molecular gas clumps that are exposed to the radiation from propagating stellar-jet shocks. The X-ray, EUV, and FUV radiation from the shock initiates ion chemistry and also heats the gas in the clumps. Using representative parameters, we show that, on the shock transit time between the clumps, the abundances of the ionized molecular species that are produced in the clumps can exceed the values determined from steady state models by several orders of magnitude. Collisional excitation by the heated gas can lead to measurable line emission from several ionized species; as in previous investigations of X-ray-irradiated molecular gas, we find that electron impacts contribute significantly to this process. We apply these results to the interpretation of the HCO(+) line emission that has already been detected in several Herbig-Haro objects. We demonstrate that this picture provides a natural explanation of the fact that the line intensity typically peaks ahead of the associated shock, as well as of the reported low line-center velocities and narrow line widths. We tabulate several diagnostic line intensities of HCO(+) and other molecular species that may be used to infer the physical conditions in the emitting gas.

Wolfire, Mark G.↗
NASA NTRS1977

Shock models of high-velocity interstellar Si III

Recent Copernicus observations of high-velocity interstellar Si III have been interpreted as evidence for collisionally ionized gas at 30,000 to 80,000 K. In this paper, these observations are summarized, and conductive-interface and shock-heating mechanisms are investigated as sources for the temperatures, column densities, and velocity fields. The conductive mechanism evidently cannot reproduce the observations, but radiatively cooling shocks of 50 to 100 km/s, produced by supernova remnants or stellar winds, may provide a viable explanation. Time-dependent calculations of the cooling and ionization behind such shocks show the importance of initial ionization conditions at 100,000 K and produce results substantially different from those of calculations which start at 1 million K.

Shull, J. M.↗
NASA NTRS1992

Qualitative spectroscopic study of magnetic nozzle flow

The physics of the magnetic nozzle flow for a 100-kW-level quasi-steady MPD thruster was studied by photographic spectroscopy focusing on the plasma model in the flow and the acceleration mechanism. Spectroscopic visualization for the flow-species analysis indicates that the plasma-exhaust flow dominated by NII species were confined by the magnetic nozzle effect to collimate the flow for the better thruster performance. Inside the nozzle, the plasma flow was found to be in nonhomogeneous collisional-radiative condition. There appears to be a substantial flow acceleration from the magnetic nozzle inlet to the outlet with slight expansion. This suggests that the flow resembles that of constant area supersonic duct flow with cooling.

Umeki, T.↗
DOE OSTI2024

Drag exerted by drift-acoustic radiation on a magnetic island

The Island Equilibrium and Transport (IslET) model is extended to allow for the effects of ion compressibility albeit for a constant electron temperature. The model describes fully relaxed, saturated, steady-state magnetic islands arising from the evolution of a tearing mode caused either by an instability or an externally imposed resonant perturbation. It assumes that the collision frequency lies in the semi-collisional regime. A salient new feature of the extended model is an equation describing the transport of parallel momentum. The model is applied to evaluate the drag exerted on a thin island by the emission of drift-acoustic waves.

Physics↗
NASA NTRS1972

Excitation of Na D-line radiation in collisions of sodium atoms with internally excited H2, D2, and N2

Excitation of D-line radiation in collisions of Na atoms with vibrationally excited N2, H2 and D2 was studied in two modulated crossed beam experiments. In both experiments, the vibrational excitation of the molecules was provided by heating the molecular beam source to temperatures in the range of 2000 to 3000 K, which was assumed to give populations according to the Boltzmann expression. In the first experiment, a total rate coefficient was measured as a function of molecular beam temperature, with absolute calibration of the photon detector being made using the black body radiation from the heated molecular beam source. Since heating affects both the internal energy and the collisional kinetic energy, the first experiment could not determine the relative contributions of internal energy transfer versus collisional excitation. The second experiment achieved partial separation of internal versus kinetic energy transfer effects by using a velocity-selected molecular beam. Using two simple models for the kinetic energy dependence of the transfer cross section for a given change in vibrational quantum number, the data from both experiments were used to determine parameters in the models.

Krause, H. F.↗
NASA NTRS1975

The atmosphere and ionosphere of Io

Models for Jupiter's innermost Galilean satellite's atmosphere, ionosphere, and sodium airglow are developed on the basis of recent observational data. The sodium emission detected by Brown (1973) is seen to require a collisional excitation process in Io's atmosphere, while the extended sodium emission measured by Trafton et al. (1974) may require scattering of the planetary radiation by an extended sodium cloud. The sodium is presumably present in bound form on Io's surface, and may be released by a sputtering mechanism proposed by Matson et al. (1974). The ionosphere detected by a radio occultation experiment on Pioneer 10 could be attributed to photoionization of atmospheric sodium, provided Io's atmosphere could sustain significant upward motions during daytime and downward motions during nighttime. The incomplete hydrogen torus observed by Judge and Carlson (1974) in the vicinity of Io appears to require a large supply of hydrogen from the satellite's atmosphere. Implications of the hydrogen torus for the energy and mass balance of Jupiter's magnetosphere are discussed.

Mcelroy, M. B.↗