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At least 145 records · Page 8

Photophysics of Laser Dye-Doped Polymer Membranes for Laser-Induced Fluorescence Photogrammetry

Laser-induced fluorescence target generation in dye-doped polymer films has recently been introduced as a promising alternative to more traditional photogrammetric targeting techniques for surface profiling of highly transparent or reflective membrane structures. We investigate the photophysics of these dye-doped polymers to help determine their long-term durability and suitability for laser-induced fluorescence photogrammetric targeting. These investigations included experimental analysis of the fluorescence emission pattern, spectral content, temporal lifetime, linearity, and half-life. Results are presented that reveal an emission pattern wider than normal Lambertian diffuse surface scatter, a fluorescence time constant of 6.6 ns, a pump saturation level of approximately 20 micro J/mm(exp 2), and a useful lifetime of more than 300,000 measurements. Furthermore, two demonstrations of photogrammetric measurements by laser-induced fluorescence targeting are presented, showing agreement between photogrammetric and physically measured dimensions within the measurement scatter of 100 micron.

Dorrington, Adrian A.↗

The Calipso Version 4.5 Stratospheric Aerosol Subtyping Algorithm

The accurate classification of aerosol types injected into the stratosphere is important to properly characterize their chemical and radiative impacts within the Earth climate system. The updated stratospheric aerosol subtyping algorithm used in the version 4.5 (V4.5) release of the Cloud Aerosol Lidar with Orthogonal Polarization (CALIOP) level 2 data products now delivers more comprehensive and accurate classifications than its predecessor. The original algorithm identified four aerosol subtypes for layers detected above the tropopause: volcanic ash, smoke, sulfate/other, and polar stratospheric aerosol (PSA). In the revised algorithm, sulfates are separately identified as a distinct, homogeneous subtype, and the diffuse, weakly scattering layers previously assigned to the sulfate/other class are recategorized as a fifth “unclassified” subtype. By making two structural changes to the algorithm and revising two thresholds, the V4.5 algorithm improves the ability to discriminate between volcanic ash and smoke from pyrocumulonimbus injections, improves the fidelity of the sulfate subtype, and more accurately reflects the uncertainties inherent in the classification process. The 532 nm lidar ratio for volcanic ash was also revised to a value more consistent with the current state of knowledge. This paper briefly reviews the previous version of the algorithm (V4.1 and V4.2) then fully details the rationale and impact of the V4.5 changes on subtype classification frequency for specific events where the dominant aerosol type is known based on the literature. Classification accuracy is best for volcanic ash due to its characteristically high depolarization ratio. Smoke layers in the stratosphere are also classified with reasonable accuracy, though during the daytime a substantial fraction are misclassified as ash. It is also possible for mixtures of ash and sulfate to be misclassified as smoke. The V4.5 sulfate subtype accuracy is less than that for ash or smoke, with sulfates being misclassified as smoke about one-third of the time. However, because exceptionally tenuous layers are now assigned to the unclassified subtype and the revised algorithm levies more stringent criteria for identifying an aerosol as sulfate, it is more likely that layers labeled as this subtype are in fact sulfate compared to those assigned the sulfate/other classification in the previous data release.

Jason L Tackett↗

Effect of EMIC Wave Normal Angle Distribution on Relativistic Electron Scattering in Outer RB

We present the equatorial and bounce average pitch angle diffusion coefficients for scattering of relativistic electrons by the H+ mode of EMIC waves. Both the model (prescribed) and self consistent distributions over the wave normal angle are considered. The main results of our calculation can be summarized as follows: First, in comparison with field aligned waves, the intermediate and highly oblique waves reduce the pitch angle range subject to diffusion, and strongly suppress the scattering rate for low energy electrons (E less than 2 MeV). Second, for electron energies greater than 5 MeV, the |n| = 1 resonances operate only in a narrow region at large pitch-angles, and despite their greatest contribution in case of field aligned waves, cannot cause electron diffusion into the loss cone. For those energies, oblique waves at |n| greater than 1 resonances are more effective, extending the range of pitch angle diffusion down to the loss cone boundary, and increasing diffusion at small pitch angles by orders of magnitude.

Khazanov, G. V.↗

Comparative accuracy of diffuse radiative properties computed using selected multiple scattering approximations

Computational results have been obtained for the spherical albedo, global transmission, and global absorption of plane-parallel layers composed of cloud droplets. These computations, obtained using the doubling method for the entire range of single scattering albedos and for optical depths between 0.1 and 100, are compared with corresponding results obtained using selected multiple scattering approximations. The spherical albedo and global absorption computed using asymptotic theory are found to be accurate to better than 5 percent for all values of the single scattering albedo, provided the optical thickness exceeds about 2. The diffuse two-stream approximations have relative accuracies that are much worse than 5 percent for the spherical albedo over most of the parameter space, yet are accurate to within 5 percent in the global absorption when the absorption is significant. The integrated delta-Eddington scheme appears to be the most suitable model over the entire range of variables, generally producing relative errors of less than 5 percent in both the spherical albedo and global absorption.

HARSHVARDHAN↗

Laser scattering in a hanging drop vapor diffusion apparatus for protein crystal growth in a microgravity environment

One type of hardware used to grow protein crystals in the microgravity environment aboard the U.S. Space Shuttle is a hanging drop vapor diffusion apparatus (HDVDA). In order to optimize crystal growth conditions, dynamic control of the HDVDA is desirable. A critical component in the dynamically controlled system is a detector for protein nucleation. We have constructed a laser scattering detector for the HDVDA capable of detecting the nucleation stage. The detector was successfully tested for several scatterers differing in size using dynamic light scattering techniques. In addition, the ability to detect protein nucleation using the HDVDA was demonstrated for lysozyme.

Casay, G. A.↗

Radiative Smoothing in Clouds at Transparent and Absorbing Wavelengths

For absorbing and transparent wavelengths, we discuss the effect of horizontal solar radiative fluxes in clouds on the accuracy of a conventional plane-parallel radiative transfer calculations for a single pixel, known as the Independent Pixel Approximation (IPA). We address the question of correlations between horizontal fluxes, IPA accuracies and radiative smoothing. By smoothing we understand a radiative transfer process whereby radiation does not follow the small-scale fluctuations of cloud structure, producing much smoother radiation fields. The scale eta that characterizes this process is called "radiative smoothing scale." We relate radiative smoothing to the photon's horizontal displacement that characterizes a "spot" of reflected light associated with a point source. We generalize the "spot-size" estimate derived for conservative scattering using the diffusion theory to the case of non-conservative scattering. For reflected light, theoretical results are confirmed with numerical simulations. The radiative smoothing scale eta is a critical value where IPA effectively breaks down; for scales smaller than TI, real radiation field are much smoother than their IPA counterparts for the same cloud structure. In addition to the estimate of il for absorbing wavelengths, we show that: (1) with more absorption, the scale break determined by eta in a log-log plot of wavenumber spectra moves towards smaller scales and (2) the smaller eta the flatter the small-scale slope which means less radiative smoothing, thus more accuracy in the IPA reflection.

Marshak, A.↗

Acceleration of cometary H2O group pickup ions by obliquely propagating nonlinear magnetosonic waves

The observations made during the encounter with comet Giacobini Zinner show that the character of MHD turbulence is governed by the magnetosonic (MS) waves generated by the pickup ions via a resonant cyclotron instability. The interaction of cometary ions in the mass loaded solar wind with MS waves propagating away from the comet and oblique to the interplanetary magnetic field (IMF) is investigated using the test particle approach. Ion trajectories, distribution functions, widths of pitch angle scattering and energy diffusion are obtained. We have also investigated the relationship between pitch angle scattering and the three parameters, namely, alpha, the angle between the solar wind flow direction and the ambient magnetic field, theta(sub BK), the angle between the ambient magnetic field and the wave propagation vector, and the ion injection velocity.

Srivastava, Krishna M.↗

The interplanetary transport of solar cosmic rays

Numerical solutions are presented for the propagation of solar cosmic rays in interplanetary space, including the effects of pitch-angle scattering and adiabatic focusing. The intensity-time profiles can be well fitted by a simple radial spatial diffusion equation with scattering mean-free path lambda(fit). The radial mean-free path so obtained is significantly larger than the true scattering mean-free path for low-rigidity particles due to both adiabatic focusing and the inapplicability of the diffusive approximation early in the event. The well-known discrepancy between lambda(fit) and the theoretical predictions may be resolved by these calculations.

Gombosi, T. I.↗

Diffusion NMR methods applied to xenon gas for materials study

We report initial NMR studies of (i) xenon gas diffusion in model heterogeneous porous media and (ii) continuous flow laser-polarized xenon gas. Both areas utilize the pulsed gradient spin-echo (PGSE) techniques in the gas phase, with the aim of obtaining more sophisticated information than just translational self-diffusion coefficients--a brief overview of this area is provided in the Introduction. The heterogeneous or multiple-length scale model porous media consisted of random packs of mixed glass beads of two different sizes. We focus on observing the approach of the time-dependent gas diffusion coefficient, D(t) (an indicator of mean squared displacement), to the long-time asymptote, with the aim of understanding the long-length scale structural information that may be derived from a heterogeneous porous system. We find that D(t) of imbibed xenon gas at short diffusion times is similar for the mixed bead pack and a pack of the smaller sized beads alone, hence reflecting the pore surface area to volume ratio of the smaller bead sample. The approach of D(t) to the long-time limit follows that of a pack of the larger sized beads alone, although the limiting D(t) for the mixed bead pack is lower, reflecting the lower porosity of the sample compared to that of a pack of mono-sized glass beads. The Pade approximation is used to interpolate D(t) data between the short- and long-time limits. Initial studies of continuous flow laser-polarized xenon gas demonstrate velocity-sensitive imaging of much higher flows than can generally be obtained with liquids (20-200 mm s-1). Gas velocity imaging is, however, found to be limited to a resolution of about 1 mm s-1 owing to the high diffusivity of gases compared with liquids. We also present the first gas-phase NMR scattering, or diffusive-diffraction, data, namely flow-enhanced structural features in the echo attenuation data from laser-polarized xenon flowing through a 2 mm glass bead pack. c2002 John Wiley & Sons, Ltd.

NASA Discipline Life Sciences Technologies↗

Comparison of Jovian and Terrestrial Lightning as Observed from Space

We compare the images of Jovian lightning taken by Galileo spacecraft with the images of terrestrial lightning observed by Lightning Imaging Spectrometer (LIS) onboard the TERRA spacecraft. Both data sets have good spatial resolution: Galileo's pixel is 25 km, or about half the atmospheric scale height, LIS pixel is 3-6 km, also about half of the scale height. This good resolution allows us to see that both Jovian and terrestrial lightning spots look diffuse because of the scattering in the clouds above. Previously we used the appearance of the diffuse spots on Jupiter to model lightning depths and the opacity and shape of the overlying clouds (Dyudina and Ingersoll, 2000). The comparison with LIS data allowed us to verify that the model is valid for terrestrial lightning. The irregular shapes of large terrestrial lightning suggests 30-km scale horizontal bolts. On Jupiter the spots, projected onto the horizontal plane, are nearly circular suggesting that the large size of the spots is mostly due to the horizontal diffusion of the photons scattered in the clouds. Unlike the Galileo observations, LIS has fine temporal resolution of 2 ms, or about 250 frames per single lightning flash. We will discuss the temporal evolution of terrestrial flashes and its implications for Jupiter.

Dyudina, Ulyana A.↗

A photometric function for diffuse reflection by particulate materials

A photometric function is proposed to describe the diffuse reflection of radiation by particulate materials. Both multiple scattering and the dominant effects of particle shadowing are included and the function is verified by comparisons with the photometries of laboratory surfaces. Brightness measurements of planetary and other diffusely scattering surfaces can be used to calculate the brightness for geometries other than those used in the measurements and for which the Minnaert function does not apply. The measurements also can be directly related to such surface characteristics as particle size, single-particle albedo, and compactness.

Meador, W. E.↗

Application of Kubelka-Munk theory of diffuse reflectance to geologic problems - The role of scattering

An understanding of the reflectance spectra of scattering media is vital for the appropriate interpretation of the reflectance spectra of planetary surfaces. When the absorption coefficient (k) and the mean size of the scattering centers are small, the Kubelka-Munk (K-M) theory of diffuse reflectance is valid. Since small values of k are characteristic of a wide variety of geologically important materials over a significant range of wavelength, the K-M theory should be applicable to appropriate portions of the reflectance spectra of these media if the dimensions of the scattering centers are sufficiently small. To test the utility of the K-M theory, a comparison is conducted of a set of theoretically generated spectra with a set of independently measured experimental spectra. The similarities found in the behavior of the two sets of spectra demonstrate the applicability of the K-M theory to the understanding of physical phenomena. Aspects of wavelength-dependent scattering are investigated.

Morris, R. V.↗

Laboratory simulation of diffuse reflectivity from a cloudy planetary atmosphere.

For the first time measurements in the multiple scattering regime of the diffuse reflectivity as a function of single scattering albedo have been made in a geometry that may be simulated by a plane parallel atmosphere of large optical depth. A comparison between the measurements and a theoretical computation of the diffuse reflectivity is presented. The measurements are within 1% agreement with the theoretical calculations for two different sizes of scattering particles which are larger than and smaller than the wavelength of the incident light, corresponding to the Mie and Rayleigh regimes, respectively.

Margolis, J. S.↗

Fundamental Concepts of Wave-Particle Interactions

Wave-particle interactions are fundamental to all collisionless plasmas, from the instabilitites generating the waves to the resonant interactions which cause pitch-angle scattering, particle energy diffusion and cross-field diffusion of particles.

wave particles plasmas collisionless plasmas scatt↗

Saturn's rings and Pioneer 11

Quantitative predictions of the diffuse reflection and transmission properties of Saturn's rings, relevant to the September 1979 Pioneer 11 flyby, are presented. Predictions are based on an elementary anisotropic scattering model. Interparticle separations are considered to be sufficiently large that mutual shadowing is negligible. Likely ranges in both the single scattering albedo and perpendicular optical thickness of the ring are considered. Situations of pronounced back-scattering and of isotropic scattering are treated individually. Spacecraft measurement of the radiation suffering diffuse scattering by the ring can provide a useful test of the basic ring model.

Price, M. J.↗

A Traceable Ground to On-Orbit Radiometric Calibration System for the Solar Reflective Wavelength Region

This paper describes the combination of a Mie scattering spectral BSDF and BTDF albedo standard whose calibration is traceable to the NIST SIRCUS Facility or the NIST STARR II Facility. The Space-based Calibration Transfer Spectroradiometer (SCATS) sensor uses a simple, invariant optical configuration and dedicated narrow band spectral channel modules to provide very accurate, polarization-insensitive, stable measurements of earth albedo and lunar disk albedo. Optical degradation effects on calibration stability are eliminated through use of a common optical system for observations of the Sun, Earth, and Moon. The measurements from space would be traceable to SI units through preflight calibrations of radiance and irradiance at NIST's SIRCUS facility and the invariant optical system used in the sensor. Simultaneous measurements are made in multiple spectral channels covering the solar reflective wavelength range of 300 nm to 2.4 microns. The large dynamic range of signals is handled by use of single-element, highly-linear detectors, stable discrete electronic components, and a non imaging optical configuration. Up to 19 spectral modules can be mounted on a single-axis drive to give direct pointing at the Earth and at least once per orbit view of the Sun and Moon. By observing the Sun on every orbit, the most stringent stability requirements of the system are limited to short time periods. The invariant optical system for both radiance and irradiance measurements also give excellent transfer to-orbit SI traceability. Emerging instrumental requirements for remotely sensing tropospheric trace species have led to a rethinking by some of the paradigm for Systeme International d'Unites (SI) traceability of the spectral irradiance and radiance radiometric calibrations to spectral albedo (sr(exp -1)) which is not a SI unit. In the solar reflective wavelength region the spectral albedo calibrations are tied often to either the spectral albedo of a solar diffuser or the Moon. This new type of Mie scattering diffuser (MSD) is capable of withstanding high temperatures, and is more Lambertian than Spectralon(tm). It has the potential of covering the entire solar reflective wavelength region. Laboratory measurements have shown that the specular reflectance component is negligible, and indicate that internal absorption by multiple scattering is small. This MSD, a true volume diffuser, exhibits a high degree of radiometric stability which suggests that measurements at the National Institute of Standards and Technology (NIST) could provide a spectral albedo standard. Measurements have been made of its radiometric stability under a simulated space environment of high energy gamma rays, high energy protons, and UV radiation from ambient down to the vacuum ultraviolet H Lyman alpha at 121.6 nm for its eventual use in space as a solar diffuser.

Heath, Donald F.↗

Detection of Objects Hidden in Highly Scattering Media Using Time-Gated Imaging Methods

Non-intrusive and non-invasive optical imaging techniques has generated great interest among researchers for their potential applications to biological study, device characterization, surface defect detection, and jet fuel dynamics. Non-linear optical parametric amplification gate (NLOPG) has been used to detect back-scattered images of objects hidden in diluted Intralipid solutions. To directly detect objects hidden in highly scattering media, the diffusive component of light needs to be sorted out from early arrived ballistic and snake photons. In an optical imaging system, images are collected in transmission or back-scattered geometry. The early arrival photons in the transmission approach, always carry the direct information of the hidden object embedded in the turbid medium. In the back-scattered approach, the result is not so forth coming. In the presence of a scattering host, the first arrival photons in back-scattered approach will be directly photons from the host material. In the presentation, NLOPG was applied to acquire time resolved back-scattered images under the phase matching condition. A time-gated amplified signal was obtained through this NLOPG process. The system's gain was approximately 100 times. The time-gate was achieved through phase matching condition where only coherent photons retain their phase. As a result, the diffusive photons, which were the primary contributor to the background, were removed. With a large dynamic range and high resolution, time-gated early light imaging has the potential for improving rocket/aircraft design by determining jets shape and particle sizes. Refinements to these techniques may enable drop size measurements in the highly scattering, optically dense region of multi-element rocket injectors. These types of measurements should greatly enhance the design of stable, and higher performing rocket engines.

Galland, Pierre A.↗