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At least 145 records · Page 8
All sourcesNASA NTRSDOE OSTI
DOE OSTI2026

Meteoric 10Be Flux Calibration Data for the East River Watershed, Colorado, USA

This data package contains tabular and geospatial data used to quantify and model meteoric beryllium-10 fluxes in the East River watershed, Colorado, USA. The tabular component includes calibration-site data from five glacial moraine sites and includes environmental variables used to evaluate spatial controls on meteoric 10Be delivery, including elevation, mean annual precipitation (MAP), mean snow depth, and mean snow water equivalent (SWE). These site-level data were used to compare observed fluxes with environmental gradients across the watershed and to evaluate the effects of erosion correction on flux estimates. The package also includes supporting slope and curvature values used to assess topographic inputs to the erosion analysis. A second component of the data package contains updated manuscript tables and regression outputs used to summarize the relationships between meteoric 10Be flux and environmental predictors. These tables include meteoric 10Be sample information and AMS results, site-level environmental values, site-level meteoric 10Be inventory and flux values, watershed-averaged predicted fluxes, soil bulk density measurements, fine-fraction values, soil pH measurements, and regression statistics including slope, intercept, coefficient of determination, and p-value. The regression products include both standard linear regressions and regressions in which the intercept is constrained to pass through zero, and they support the analyses presented in the companion manuscript. Together, these tabular files provide the numerical basis for the manuscript tables and the regression-based interpretation of meteoric 10Be flux variability in a snow-dominated mountain watershed. The geospatial component of the package consists of GeoTIFF raster files used to generate the map products presented in Figures 2 and 6 of the companion manuscript. These rasters represent watershed-scale spatial layers for environmental variables and regression-based predictions of meteoric 10Be flux. This dataset contains comma-separated values files (.csv), Microsoft Excel files (.xlsx), GeoTIFF raster files (.tif), and upporting metadata files, including CSV data dictionaries and readme text files (.csv, .txt). The tabular files can be opened with standard spreadsheet software, and the raster files can be viewed and analyzed in GIS software such as ArcGIS Pro or QGIS. Together, these files document the numerical and spatial datasets used to calibrate and predict meteoric 10Be delivery in the East River watershed.

East River↗
DOE OSTI2020

Control of the Plasma-Material Interface for Long Pulse Optimization in EAST and KSTAR

This is the Final Technical Report for the Grant DE-SC0016322. The major goals of the project are to use HIDRA to evaluate and optimize the FLiLi and LiMIT concepts, in preparation for the final designs of liquid Li PFCs for testing in EAST long pulse discharges. In the first year the goal is to fully commission HIDRA and begin liquid Li tests. In the second year it is to test the FLiLi and LiMIT designs in HIDRA and start the production of the first LiMIT test plate for EAST.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2023

Assessing the link between aerosol mixing state, structure and composition and their optical properties: Ascension Island as a testbed for the South‐East Atlantic aerosol regimes

Forest and savanna fires are a major source of pollution over the globe. Such fire events emit to the atmosphere a considerable amount of “fluffy” fractal black looking particles that are often referred to as black carbon (BC) or soot aerosols. In fact, BC particles (aerosols) emitted from savanna and agricultural fires over the African continent play an important role in the region’s and the global climate. These fires occur each year between July and October, which is referred to as the biomass burning (BB) season and are considered among the globe's largest man-made emission sources of BC particles. However, during these fire events, not only BC particles are emitted, but also other types of particles and gases that can interact with each other to create new particles, generating a slew of particles often generally referred to as BB aerosols. Although the majority of the fire emissions occur inland in the sub-Saharan part of Africa, their effect reaches far beyond the continent due to the prevailing easterly winds, which transport those aerosols over the South-East Atlantic (SEA) ocean, off the west-coast of Africa. The reason why these particles are so important to the regional and global climate is that they absorb sunlight radiation, which overall warms the climate. However, the magnitude of this warming effect is highly uncertain and depends upon a multitude of aspects. Our overarching goal for this project was to better understand the changes in the aerosol properties as they transport from fire sources downstream toward the ocean and how this can eventually affect the earth's radiative budget in terms of warming or cooling. Following the above, our work here was focused on the investigation of the African BB aerosol plumes mixing state (mixing of BB aerosols and other aerosol types), composition and size distribution as they transport from the African continent towards the SEA ocean, and their link with some of the commonly measurable bulk optical properties such as mass absorption coefficient (MAC) and single scattering albedo (SSA). We utilized three field missions that were conducted over the SEA ocean between 2016 and 2018. Specifically, we used (1) ground-based measurements from the DOE ARM Mobile Facility (AMF1), which was deployed at Ascension Island (ASI) for the LASIC (Layered Atlantic Smoke Interactions with Clouds) campaign between June 2016 and October 2017, (2) airborne measurements from the UK CLARIFY (Clouds and Aerosol Radiative impacts and Forcing) campaign during Aug-Sep-2017, and (3) airborne measurements from the ORACLES (Observations of Aerosols above Clouds and their interactions) campaign during Aug-2017, and Sep-Oct-2018. The three campaigns cover a relatively large region, from the western African coast on the east towards Ascension Island in the middle of the SEA to the west. We used the data gathered by these campaigns to find how BB properties and composition change from near emission sources (the ORACLES campaign flights) downstream (the CLARIFY flights and the ground based LASIC measurements). We used particle trajectory following methodologies to connect the measurements from the different campaigns, which allowed us to follow a certain aerosol plume (airmass) from near-source towards Ascension Island. We found out that atmospheric aging processes governed by the UV light from the sun (photochemistry) and cloud processes (aqueous chemistry) govern the changes seen in the particle composition during the transport were more dominant in dictating aerosol composition than specific emission composition or source types. We assessed how aerosol optical properties change during the BB season and what are the main drivers of this change. We found that the enhanced ratio of BC to CO is well correlated with single scattering albedo (SSA) and mass absorption coefficient (MACBC), providing a simple way to estimate the aerosol optical characteristics in the south-eastern Atlantic Ocean. From the analysis of the location of BB, the primary source fuel, the water content in the fuel, combined with the mean cloud cover and precipitation in the transport areas of the BB plume, we conclude that the increase in BC/CO from June to August is likely to be caused by burning becoming more flaming (hot fires), and the decrease in BC/CO in September and October may be caused by smoldering (colder) fires. We found that aerosol hygroscopicity increases with decreasing altitude below 2km, and that enhanced BB hygroscopicity at lower altitudes is mainly due to a lower organic aerosol (OA) fraction, increased sulfate fraction, and greater hygroscopicity parameter of OA at lower altitudes.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2025

Ecohydrological controls on root and microbial respiration in the East River watershed of Colorado

The main objective of this project was to conduct exploratory work to quantify how snow and rain water inputs influence the CO2 coming from the soil surface (soil CO2 flux), and its plant and microbial sources, in the East River watershed, near Crested Butte, Colorado. Knowledge gained from this effort laid the groundwork for a more comprehensive (ongoing) follow-on grant that is using a combination of experiments, field observations, machine learning and simulation modeling to fully disentangle these relationships. New field measurements were made at four locations along an elevational transect on Snodgrass Mountain at Rocky Mountain Biological Laboratory. These sites were chosen to differ in total snowpack and water table depth, and included both deciduous (aspen) and evergreen (spruce/fir) forest types. We used automated measurements of soil CO2 concentrations to quantify the total soil CO2 flux, and the vertical CO2 production within the soil profile at each site. Isotope (radiocarbon, 14C) measurements determined how much of the CO2 emitted from the soil surface came from plant respiration (root metabolism) versus microbial respiration (decomposition of soil organic matter) sources. Supporting data on plant phenology and microbial dynamics provided context for the observed variation in respiration sources. This work was motivated by our overarching hypothesis that quantifying belowground plant and microbial processes separately, and how they are influenced by snow and rain inputs, is necessary for understanding and predicting how the East River watershed ecosystems will respond to future environmental change.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Power production from the U.S. east coast offshore wind lease areas

The accompanying file include information regarding the set up of WRF simulations of power production and wake extents from offshore wind lease areas along the U.S. east coast, and also data presented in figures in the "Wind power production from the U.S. east coast offshore lease areas" paper and the associated MATLAB data processing code.

17 WIND ENERGY↗
NASA NTRS2013

Groundwater Depletion in the Middle East from GRACE with Implications for Transboundary Water Management in the Tigris-Euphrates-Western Iran Region

In this study, we use observations from the Gravity Recovery and Climate Experiment (GRACE) satellite mission to evaluate freshwater storage trends in the north-central Middle East, including portions of the Tigris and Euphrates River Basins and western Iran, from January 2003 to December 2009. GRACE data show an alarming rate of decrease in total water storage of approximately -27.2 plus or minus 0.6 millimeters per year equivalent water height, equal to a volume of 143.6 cubic kimometers during the course of the study period. Additional remote-sensing information and output from land surface models were used to identify that groundwater losses are the major source of this trend. The approach used in this study provides an example of ''best current capabilities'' in regions like the Middle East, where data access can be severely limited. Results indicate that the region lost 17.3 plus or minus 2.1 millimeters per year equivalent water height of groundwater during the study period, or 91.3 plus or minus 10.9 cubic kilometers in volume. Furthermore, results raise important issues regarding water use in transboundary river basins and aquifers, including the necessity of international water use treaties and resolving discrepancies in international water law, while amplifying the need for increased monitoring for core components of the water budget.

GRACE↗
NASA NTRS2021

Vegetation Monitoring Optimization with Normalized Difference Vegetation Index and Evapotranspiration Using Remote Sensing Measurements and Land Surface Models Over East Africa

The majority of people in East Africa rely on the agro-pastoral system for their livelihood, which is highly vulnerable to droughts and flooding. Agro-pastoral droughts are endemic to the region and are considered the main natural hazard that contributes to food insecurity. Drought begins with rainfall deficit, gradually leading to soil moisture deficit, higher land surface temperature, and finally impacts to vegetation growth. Therefore, monitoring vegetation conditions is essential in understanding the progression of drought, potential effects on food security, and providing early warning information needed for drought mitigation decisions. Because vegetation processes couple the land and atmosphere, monitoring of vegetation conditions requires consideration of both water provision and demand. While there is consensus in using either the Normalized Difference Vegetation Index (NDVI) or evapotranspiration(ET) for vegetation monitoring, a comprehensive assessment optimizing the use of both has not yet been done. Moreover, the evaluation methods for understanding the relationships between NDVI and ET for vegetation monitoring are also limited. Taking these gaps into account we have developed a framework to optimize vegetation monitoring using both NDVI and ET by identifying where they perform the best by using triple collocation and cross-correlation methods. We estimated the random error structure in Moderate Resolution Imaging Spectroradiometer (MODIS) NDVI; ET from the Operational Simplified Surface Energy Balance (SSEBop) model; and ET from land surface models (LSMs). LSM ET and SSEBop ET have been found to be better indicators for vegetation monitoring during extreme drought events, while NDVI could provide better information on vegetation condition during wetter than normal conditions. The random error structures of these variables suggest that LSM ET is most likely to provide important information for vegetation monitoring over low and high ends of the vegetation fraction areas. Over moderate vegetative areas, any of these variables could provide important vegetation information for drought characterization and food security assessments. While this study provides a framework for optimizing vegetation monitoring for drought and food security assessments over East Africa, the framework can be adopted to optimize vegetation monitoring over any other drought and food insecure region of the world.

triple collocation↗
NASA NTRS2021

A Dusty Atmospheric River Brings Floods to the Middle East

Torrential rainfall and rapid snowmelt in April 2017 caused deadly floods in northwestern Iran. An atmospheric river (AR), propagating across the Middle East and North Africa, was found responsible for this extreme event. The snowmelt was triggered by precipitation and warm advection associated with the AR. Total satellite-based rainfall for April 2017 was moderately below normal, suggesting that a heavy flood can happen during dry years. The AR was fed by moisture from the Mediterranean and Red Seas. Despite its adverse societal consequences, this event was beneficial to the recovery of the desiccating Lake Urmia. The impacts of this AR were not limited to flooding; it also facilitated dust transport to the region. This distinct characteristic of the ARs in the Middle East is attributed to major mineral dust sources located along their pathways. This event was reasonably predicted at 7-day lead time, crucially important for successful early warning systems.

Atmospheric river↗
NASA NTRSDate not supplied

Potential Impacts of Climate Change on Future Transboundary Water Conflicts in the Middle East

We analyzed the latest climate model projections (CMIP6) of precipitation and temperature for the very high emissions scenario, SSP5-8.5, to detect potential future changes in the Middle East. A baseline period (1981-2010) was compared with the middle (2040-2069) and end (2070-2099) of the 21st century. The Tigris-Euphrates headwaters was identified as the hotspot of future compound effects of climate change in the region. In particular, the Southeastern Anatolia Project (in Turkish, GAP) region is likely to see the most dramatic compound changes of any area in the Middle East. That assessment was based on the model projections that showed rapid warming, increased interannual precipitation variability, and decreased precipitation all coinciding in an area of massive irrigation development and known transboundary water tension. It is likely that GAP would exacerbate environmental, agricultural, water conflict, and public health issues in the region, therefore its adverse impacts might outnumber its benefits in coming decades. This study attempts to warn decision-makers of the urgent need to integrate these trends to water resource planning and international negotiations.

Middle East↗
NASA NTRS2023

Fine particulate concentrations over East Asia derived from aerosols measured by the Advanced Himawari Imager using machine learning

Fine particulate matter with a diameter below 2.5 μm (PM 2.5 ) is deleterious to the cardiovascular and respiratory systems. It is often difficult to assess the effects of PM 2.5 on human health over regions with limited ground monitoring sites, especially in East Asia. As an alternative, we estimated near-surface PM 2.5 concentrations by analyzing Advanced Himawari Imager (AHI) Yonsei Aerosol Retrieval (YAER) products. This study incorporates daytime data for East Asia covering the Korean Peninsula, China, Japan, Southeast Asia, and southern Mongolia. We collocated AHI YAER product pixels with meteorological, land-cover, and other ancillary data for the period from March 2018 to February 2019. To estimate PM 2.5 concentrations over wide areas spanning many countries displaying various relationships between aerosol optical depth and PM 2.5 , monthly models were developed by considering both the spatial and temporal characteristics of ground-based PM 2.5 measurements. Random forest machine learning model estimated ground-level mass concentrations of PM 2.5 ; subsequent 10-fold cross validation (CV) yielded a CV R 2 value of 0.81 and a CV root mean squared error (RMSE) of 12.3 μg m -3 . We investigated the spatial pattern of PM 2.5 concentrations over multiple countries and seasonal variation in PM 2.5 concentrations. Diurnal variation of a severe PM 2.5 event in the Korean Peninsula was investigated as a case study. The model captured the extremely heterogeneous spatial distribution of PM 2.5 concentrations peaked around local noon. To measure the capability of the developed model to estimate PM 2.5 concentrations in areas with few in-situ data, its predictive performance was evaluated using a dataset independent of the training process with an R 2 of 0.60 and RMSE of 8.18 μg m −3 . This study demonstrates the potential for satellite-based PM 2.5 estimation for areas with insufficient measuring stations.

Pm2.5↗
DOE OSTI2021

Stream discharge and water quality data for East Fork Poplar Creek beginning 2012

This data note describes 15-min discharge and in situ water quality data at two locations along East Fork Poplar Creek in east Tennessee, USA. Data records include temperature, gauge height, water surface elevation above mean sea level, and volumetric discharge. Water quality measurements include temperature, specific conductance, pH, dissolved oxygen (percent saturation and concentration), turbidity, and less extensive fDOM data at one site. The data records begin in 2012 at one site and 2015 at the second site; monitoring at both sites is ongoing (as of 2021). The goal of this data collection is to improve understanding of watershed functions, hydrologic dynamics, and material flux. The data will contribute to site conceptual and numerical models, exposure and risk evaluation, remediation selection and design, and performance monitoring. The data are publicly available and can be accessed via unique url or DOI.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Long-term hydrological, biogeochemical, and climatological data from Walker Branch Watershed, East Tennessee, USA

In 1967, the original Walker Branch Watershed (WBW) project was established to study elemental cycling and mass balances in a relatively unimpacted watershed. Over the next 50+ years, findings from additional experimental studies and long-term observations on WBW advanced understanding of catchment hydrology, biogeochemistry, and ecology and established WBW as a seminal site for catchment science. The 97.5-ha WBW is located in East Tennessee, USA, on the U.S. Department of Energy's Oak Ridge Reservation. Vegetation on the watershed is characteristic of an eastern deciduous, second-growth forest. The watershed is divided into two subcatchments: the West Fork (38.4 ha) and the East Fork (59.1 ha). Headwater streams draining these subcatchments are fed by multiple springs, and thus flow is perennial. Stream water is high in base cations due to weathering of dolomite bedrock and nutrient concentrations are low. Long-term observations of climate, hydrology, and biogeochemistry include daily (1969–2014) and 15-min (1994–2014) stream discharge and annual runoff (1969–2014); hourly, daily, and annual rainfall (1969–2012); daily climate and soil temperature (1993–2010); and weekly stream water chemistry (1989–2013). These long-term datasets are publicly available on the WBW website (https://walkerbranch.ornl.gov/long-term-data/). While collection of these data has ceased, related long-term measurements continue through the National Ecological Observatory Network (NEON), where WBW is the core terrestrial and aquatic site in the Appalachian and Cumberland Plateau region (NEON's Domain 7) of the United States. These long-term datasets have been and will continue to be important in evaluating the influence of climatic and environmental drivers on catchment processes.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Increasing temperature and flow management alter mercury dynamics in East Fork Poplar Creek

East Fork Poplar Creek (EFPC) is a mercury (Hg) contaminated creek in east Tennessee, USA. Stream restoration activities included the initiation of a flow management programme in 1996 in which water from a nearby lake was pumped to the head of the creek. We conducted regular water sampling for 2 years along the length of EFPC during active flow management and for 5 years after flow management stopped. Total Hg and total monomethylmercury (MMHg) concentration and flux decreased in the uppermost reaches of EFPC that were closest to the point of water addition. Most water quality parameters, including DOC concentration, remained unchanged after flow management termination. Nevertheless, SUVA 254 , a measure of dissolved organic matter (DOM) composition, increased and coincided with increased dissolved Hg (Hg D ) concentration and flux and decreased Hg solid-water partitioning coefficients throughout EFPC. Higher SUVA 254 and Hg D concentration have potential implications for bioavailability and MMHg production. Total and dissolved MMHg concentrations increased in lower reaches of EFPC after the end of flow management and these increases were most pronounced during spring and early summer when biota are more susceptible to exposure and uptake. A general warming trend in the creek after active flow management ended likely acted in concert with higher Hg D concentration to promote higher MMHg concentration. Total and dissolved MMHg concentrations were positively correlated with water temperature above a threshold value of 10°C. Concentration changes for Hg and MMHg could not be accounted for by changes in creek discharge that accompanied the cessation of flow management. In addition to the changing DOM composition in-stream, other watershed-scale factors likely contributed to the observed patterns, as these changes occurred over months rather than instantaneously after flow management stopped. Nevertheless, similar changes in MMHg have not been observed in a tributary to EFPC.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Seasonal delay of Sahelian rainfall driven by an east–west contrast in radiative forcing in idealized CESM experiments

Recent studies suggest the observed seasonal delay of rainfall over the Sahel is mainly driven by anthropogenic aerosol forcing, which features a robust east–west contrasting changes in recent decades, with negative and positive top-of-the-atmosphere shortwave radiative forcing in South and East Asia (SA&EA) and in North America and Europe (NA&EU), respectively. Their individual effects on the Sahel rainfall annual cycle remain unclear. Here, by designing idealized sensitivity experiments based on Community Earth System Model (CESM1.2), we show that both negative radiative forcing over SA&EA and positive radiative forcing over NA&EU contribute to the delayed phase and enhanced amplitude of Sahel rainfall annual cycle. To understand the underlying physical processes, both the convective quasi-equilibrium (CQE) and atmospheric energetic frameworks are utilized. Both frameworks can well explain the seasonal delay in the rainfall annual cycle over the Sahel under the regional radiative forcings, with the CQE framework showing stronger explanatory power. Based on the insights from both frameworks, we conducted a moisture budget analysis and found that the negative radiative forcing over SA&EA causes an anomalous low-level anticyclonic circulation, which transports more moisture to the Sahel. As the anomalous anticyclone is stronger in summer and fall compared to spring, rainfall is delayed in the Sahel. Further, under the influence of the positive radiative forcing over NA&EU, more warming in the northern hemisphere causes northward transport of moisture to the northern tropics associated with the cross-equatorial transport of energy. The moisture transport increases relativehumidity over the Sahel and enhances the effective atmospheric heat capacity that delays the seasonal rainfall.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

An analysis of controlled detachment by seeding various impurity species in high performance scenarios on DIII-D and EAST

Experiments at DIII-D and EAST have demonstrated simultaneous high confinement, divertor detachment, and active control of detachment level, all of which are required for ITER. Comparing detachment control via T e and J sat , it appears that is the most straightforward sensor to use for accessing detachment onset, while J sat offers more precise control of degree of detachment. Based on these results, control using nitrogen seeding has so far shown the best ability to follow a target value with the low disruptivity and little to no degradation of performance when an Internal Transport Barrier (ITB) is present, but not all facilities allow its use. Neon seeding also can be paired with feedback control with low impact on core performance as long as there is no disruption, however shots with neon seeding commonly disrupted during these experiments. Argon is effective in EAST, but tends to degrade performance (by ≈ 10%β p ) when detachment is achieved. With ideal conditions and strike point position control, data from a single Langmuir probe are an acceptable input to the control algorithm, but this simple system is easily defeated by strike point displacement comparable to the T e or J sat scale lengths. The presence of an ITB seems to be critical to retaining core performance in detachment in these parameter ranges, as the pedestal pressure tends to decrease as a result of impurity seeding.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
DOE OSTI2020

Contrasting Regional Carbon Cycle Responses to Seasonal Climate Anomalies Across the East-West Divide of Temperate North America

Across temperate North America, interannual variability (IAV) in gross primary production (GPP) and net ecosystem exchange (NEE) and their relationship with environmental drivers are poorly understood. Here, we examine IAV in GPP and NEE and their relationship to environmental drivers using two state-of-the-science flux products: NEE constrained by surface and space-based atmospheric CO 2 measurements over 2010-2015 and satellite up-scaled GPP from FluxSat over 2001-2017. We show that the arid western half of temperate North America provides a larger contribution to IAV in GPP (104% of east) and NEE (127% of east) than the eastern half, in spite of smaller magnitude of annual mean GPP and NEE. This occurs because anomalies in western ecosystems are temporally coherent across the growing season leading to an amplification of GPP and NEE. In contrast, IAV in GPP and NEE in eastern ecosystems is dominated by seasonal compensation effects, associated with opposite responses to temperature anomalies in spring and summer. Terrestrial biosphere models in the MsTMIP ensemble generally capture these differences between eastern and western temperate North America, although there is considerable spread between models.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2020

Contrasting aerosol effects on longwave cloud forcing in South East Asia and Amazon simulated with Community Atmosphere Model version 5.3

Aerosols modify cloud microphysical and radiative properties and thus impact the shortwave (SW) and longwave cloud forcing (LWCF). This study first reports the finding of contrasting aerosol effects on LWCF in South East Asia and Amazon in the Community Atmosphere Model version 5.3 (CAM5.3), which corresponds to the sum of LW indirect and semi-direct effects investigated in Ghan et al., (2012). A series of numerical experiments is conducted to decompose the complex aerosol effects on LWCF. Our analysis indicates that the cooling (negative aerosol effects on LWCF) in Amazon is due mainly to the aerosol effects on warm clouds and the inhibition of vertical motion by the aerosol-induced radiative cooling. In contrast, the warming (positive aerosol effects on LWCF) in South East Asia is due mainly to the aerosol effect on homogeneous freezing, thus reducing the ice particle size and prolonging the existence of ice cloud. Our results emphasize that a comprehensive analysis of integrated aerosol effects on both warm and ice clouds is necessary for better understanding the aerosol effects on LWCF.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

An Overview of Atmospheric Features Over the Western North Atlantic Ocean and North American East Coast - Part 1: Analysis of Aerosols, Gases, and Wet Deposition Chemistry

The Western North Atlantic Ocean (WNAO) and adjoining East Coast of North America are of great importance for atmospheric research and have been extensively studied for several decades. This broad region exhibits complex meteorological features, diverse cloud types, and a wide range of conditions associated with gas and particulate species that originate from many sources regionally and from other continents. As Part 1 of a 2-part paper series, this work provides a characterization of quantities associated with atmospheric chemistry, including gases, aerosols, and wet deposition, based on satellite observations, ground-based data, model simulations, and reanalysis products. Key results include spatial and seasonal differences in composition along the North American East Coast and over the WNAO associated with varying sources of smoke and dust and meteorological drivers such as temperature, moisture, and precipitation. Spatial and seasonal variations of tropospheric carbon monoxide and ozone highlight different pathways towards accumulation of these species in the troposphere. Spatial distributions of speciated aerosol optical depth and vertical profiles of aerosol mass mixing ratios show a clear seasonal cycle highlighting the influence of both natural and anthropogenic sources in addition to the impact of intercontinental transport on their vertical profiles. Analysis of long-term climate model simulations of aerosol species and satellite observations of carbon monoxide confirm that there has been a significant decline in recent decades among anthropogenic constituents owing to regulatory activities. The results can inform current and future lines of research for the region.

Corral, Andrea↗