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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 145 records · Page 8

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NASA NTRS1974

The saturation spectrum of parametric instabilities

Recent calculations on the nonlinear saturation spectrum of the parametric decay instability are described. The initial calculations did not use the correct expression for the spontaneous emission term and were aimed at obtaining the distribution of spectral energy in the unstable part of wave vector space. Results of those initial calculations are combined here with the correct expression for the spontaneous emission term to obtain the distribution of spectral energy in the stable part of wave vector space. These latter calculations are believed to be relevant to the interpretation of the so called plasma line spectra obtained in ionospheric heating experiments at Arecibo, Puerto Rico.

Fejer, J. A.↗

NASA NTRS1983

Thermal and suprathermal protons and alpha particles in the earth's plasma sheet

Detailed proton energy spectra in the quasi-stable distant plasma sheet over the energy range from approximately 13 keV to approximately 130 keV are presented. These spectra are compared with spectra of simultaneously measured alpha particles in the energy range from approximately 30 keV/Q to approximately 130 keV/Q. The proton spectra are then extended into the higher energy range up to approximately 1 MeV, thereby supplementing the study of Sarris et al. (1981). The temporal behavior of the spectra in the higher energy range is discussed. It is found that below about 16 keV the proton spectra can be represented by a Maxwellian distribution; above this level, a suprathermal tail is found that cannot be represented by a single power law.

Ipavich, F. M.↗

NASA NTRS1984

Applications of space tethers

The dynamics of orbiting tethered bodies are reviewed and several practical aplications are examined. Two tethered masses in orbit will seek a local vertical orientation and a stable equilibrium, with energy transferred to the 'upper' object. The tether tensions are provided by accelerations as low a 0.0004 g., permitting long tethers an relatively large masses at the ends. The Shuttle can send a payload into a transfer orbit by placing it at the upper end of the tether, unreeling the tether, then releasing the tether and thereby imparting the excess energy to the satellite while the Orbiter falls to a lower perigee. A 10 ton payload could be unreeled on a 148 km tether, released to a 12 n. mi. apogee, and the Orbiter would be in full deorbit. Similarly, the Orbiter can tether down to deorbit form the Space Station, boosting the Station to a higher orbit. The station can then unreel a large satellite, release it to a higher orbit, thereby returning to the stations original orbit. Unreeling a wire 10 km from the Space station and having the wire cut the earth's magnetic field lines, then closing the contact between the upward and lower ends of the wire, can, with modifications, either provide power or thrust without propellants for the Station.

Bekey, I.↗

NASA NTRS1994

A model of galactic cosmic rays for use in calculating linear energy transfer spectra

The Galactic Cosmic Rays (GCR) contain fully stripped nuclei, from Hydrogen to beyond the Iron group, accelerated to high energies and are a major component of the background radiation encountered by satellites and interplanetary spacecraft. This paper presents a GCR model which is based upon our current understanding of the astrophysics of GCR transport through interstellar and interplanetary space. The model can be used to predict the energy spectra for all stable and long-lived radioactive species from H to Ni over an energy range from 50 to 50,000 MeV/nucleon as a function of a single parameter, the solar modulation level phi. The details of this model are summarized, phi is derived for the period 1974 to present, and results from this model during the 1990/1991 Combined Release and Radiation Effects Satellite (CRRES) mission are presented.

Chen, J.↗

DOE OSTI2019

Renewable electricity storage using electrolysis

Electrolysis converts electrical energy into chemical energy by storing electrons in the form of stable chemical bonds. The chemical energy can be used as a fuel or converted back to electricity when needed. Water electrolysis to hydrogen and oxygen is a well-established technology, whereas fundamental advances in CO 2 electrolysis are still needed to enable short-term and seasonal energy storage in the form of liquid fuels. This paper discusses the electrolytic reactions that can potentially enable renewable energy storage, including water, CO 2 and N 2 electrolysis. Recent progress and major obstacles associated with electrocatalysis and mass transfer management at a system level are reviewed. We conclude that knowledge and strategies are transferable between these different electrochemical technologies, although there are also unique complications that arise from the specifics of the reactions involved.

25 ENERGY STORAGE↗

DOE OSTI2023

Status of CEBAF Upgrades

Extending CEBAF energy reach by increasing the number of recirculations, while using the existing SRF system is being explored. Proposed energy upgrade is based on a new approach to multi-pass acceleration of electrons in a single Fixed Field Alternating Gradient (FFA) beam line, configured with Halbach-style permanent magnets. Encouraged by recent success of CBETA, a proposal was formulated to nearly ?double? CEBAF energy by replacing the highest energy arcs with a pair of FFA arcs. The new non-scaling FFA arcs would support simultaneous transport of additional 6 passes with energies spanning a factor of two. One of the challenges of the multi-pass (11) linac optics is to assure uniform focusing in a vast range of energies, in a fixed field lattice. Here, we propose a triplet lattice that would provide a stable periodic solution covering energy ratio of 1:33. The current CEBAF injection at 123 MeV, makes optical matching in the first linac virtually impossible due to extremely high energy span ratio (1:175). Replacement of the current injector with a 650 MeV recirculating injector will alleviate that problem. Orbital and optical matching from the FFA arcs to the linacs is implemented as a compact non-adiabatic insert. Presented scheme would promise to deliver a 22 GeV beam with normalized emittance of 76 mm·mrad and with a relative energy spread of 1×10-3. Further recirculation beyond 22 GeV is limited by large, 974 MeV per electron, energy loss due to synchrotron radiation

Bogacz, Alex↗

DOE OSTI2021

Electrodes with silicon oxide active materials for lithium ion cells achieving high capacity, high energy density and long cycle life performance

Improved negative electrodes can comprise a silicon based active material blended with graphite to provide more stable cycling at high energy densities. In some embodiments, the negative electrodes comprise a blend of polyimide binder mixed with a more elastic polymer binder with a nanoscale carbon conductive additive. The silicon-based blended graphite negative electrodes can be matched with positive electrodes comprising nickel rich lithium nickel manganese cobalt oxides to form high energy density cells with good cycling properties.

Venkatachalam, Subramanian↗

DOE OSTI2023

Electrodes with silicon oxide active materials for lithium ion cells achieving high capacity, high energy density and long cycle life performance

Venkatachalam, Subramanian↗

DOE OSTI2020

Optimization of laser-target parameters for the production of stable lithium beam

A laser ion source coupled with a radio frequency quadrupole linac accelerator is being proposed as a suitable system for the production of a low energy, high-current stable lithium beam. In order to maximize the lithium yield, plasmas generated by laser ablation of different materials based on lithium (Li, LiOH, and LiNbO3) have been characterized by using a Faraday cup and an electrostatic ion analyzer in the time of flight configuration. A wide range of laser power density has been investigated (109–1012 W/cm2) using two Nd:YAG lasers operating at different wavelengths (1064 nm and 532 nm), pulse durations (6 ns and 17 ns), and maximum energies (1400 mJ and 210 mJ). This paper outlines the pros and cons of the investigated materials by studying how the ion energy, yields, and charge state distributions are modified when the laser power density is changed. Considerable attention has been paid to the higher charge states of oxygen, which may occur with the same mass-to-charge ratio of Li3+. The analysis has evidenced that LiNbO3 represents a valid target since it allows minimizing the O6+/7Li3+ ratio down to 2.5% by using a laser power density of 1.8 × 1010 W/cm2. For such a condition, a Li3+ current of 1.4 mA/cm2 has been measured.

Cannavò, A. (ORCID:0000000309759630)↗

DOE OSTI2022

Perspective—Is Sustainable Electrowinning of Neodymium Metal Achievable?

Rare–earth metals such as neodymium are central to numerous technologically important applications such as electrified transportation, renewable energy harvesting, and magnetic data storage. Presently, neodymium metal is produced via electrolysis of Nd 2 O 3 –containing NdF 3 –LiF molten salts at high temperatures. However, this conventional electrolytic route has several drawbacks including emissions of greenhouse gases such as CO 2 and perfluorocarbons, which are harmful to the environment. In this perspective, an alternate concept based on electrolysis of NdCl 3 –containing chloride–based molten salts is explored and its potential advantages are discussed. Notably, NdCl 3 can be obtained via direct non–carbothermic chlorination of Nd 2 O 3 , supported by thermodynamic calculations and experimental evidence from literature. The chloride–based molten salt electrolysis route also offers the possibility of incorporating a non–consumable or dimensionally stable anode leading to reduced electrical energy consumption, stable cell operation and ease of process scalability.

36 MATERIALS SCIENCE↗

DOE OSTI2023

CEBAF 22 GeV FFA energy upgrade

Extending the energy reach of CEBAF by increasing the number of recirculations, while using the existing linacs is explored. This energy upgrade is based on the multi-pass acceleration of electrons in a single non-scaling Fixed Field Alternating Gradient (FFA) beam line, using Halbach-style permanent magnets. Encouraged by the recent successful demonstration of CBETA, a proposal was formulated to nearly double the energy of CEBAF from 12 to 22~GeV by replacing the highest energy arcs with FFA transport. The new FFA arcs would support simultaneous transport of an additional 6 passes spanning roughly a factor of two in energy. One of the challenges of the multi-pass (11) linac optics is to assure uniform focusing over a wide range of energies. Here, we propose a triplet lattice that provides a stable periodic solution covering an energy ratio of 1:33. The current CEBAF injection at 123 MeV, makes optical matching in the first linac impossible due to the extremely high energy ratio (1:175). Replacement of the current injector with a 650 MeV recirculating injector will alleviate this issue. Orbital and optical matching from the FFA arcs to the linacs is implemented as a compact non-adiabatic insert. The design presented here is anticipated to deliver a 22 GeV beam with normalized emittance of 76 mm·mrad and a relative energy spread of 1×10\textsuperscript{-3}. Further recirculation beyond 22 GeV is limited by the large (974 MeV per electron) energy loss due to synchrotron radiation.

Benesch, J.↗

DOE OSTI2023

CEBAF 22 GeV FFA energy upgrade

Benesch, J.↗

NASA NTRS2001

High Coverages of Hydrogen on a (10,0) Carbon Nanotube

The binding energy of H to a (10,0) carbon nanotube is calculated at 24, 50, and 100% coverage. Several different bonding configurations are considered for the 50% coverage case. Using the ONIOM (our own n-layered integrated molecular orbital and molecular mechanics) approach, the average C-H bond energy for the most stable 50% coverage and for the 100% coverage are 57.3 and 38.6 kcal/mol, respectively. Considering the size of the bond energy of H2, these values suggest that it will be difficult to achieve 100% atomic H coverage on a (10,0) nanotube.

Bauschlicher, Charles W., Jr.↗

DOE OSTI2023

Revisiting the SGTE lattice stability of bcc aluminum

The CALPHAD framework rests on the ability to assign well-defined free energies to all phases, including mechanically unstable ones. Given the experimental difficulties associated with the latter, researchers have turned to computational methods to obtain a theoretically justified definition of the free energy of mechanically unstable phases. Recently, a method called “inflection detection” has been shown to yield free energies that are broadly consistent with the current SGTE (Scientific Group Thermodata Europe) standard for pure elements, which were obtained through an extrapolation of stable solid solutions free energies towards unstable end members. Despite this general agreement, apparent failures for a few elements stand out, notably for the bcc–fcc enthalpy difference for the common element Al. Furthermore we revisit the definition of the bcc Al enthalpy and show that a careful CALPHAD-based analysis of enthalpy trends in five different mechanically stable binary solid solutions in fact does agree very well with the inflection-detection approach.

36 MATERIALS SCIENCE↗

DOE OSTI2023

22 GeV CEBAF with Novel Fixed Field Alternating Gradient Design

Extending the energy reach of CEBAF up to 22 GeV within the existing tunnel is being explored. Proposed energy upgrade can be achieved by increasing the number of recirculations, while using the existing CEBAF SRF cavity system. Presented scheme is based on an exciting new approach to acceleratie electrons efficiently with multiple passes in a single FFA beam line. Encouraged by recent success of the CBETA Test Accelerator, a proposal was formulated raise CEBAF energy by replacing the highest-energy arcs with Fixed Field Alternating Gradient (FFA) arcs. The new pair of arcs configured with FFA lattice would support simultaneous transport of additional 6 passes with energies spanning a factor of two, using the non-scaling FFA principle implemented with Halbach-derived permanent magnets - a novel magnet technology that significantly saves energy and lowers operating costs. One of the challenges of the multi-pass (11) linac optics is to provide uniform focusing in a vast range of energies, using fixed field lattice. Here, we propose a triplet lattice scaled up with increasing momentum along the linac. This would provide a stable periodic solution covering energy ratio of 1:33. The current CEBAF configured with a 123 MeV injector, makes optical matching in the first linac virtually impossible due to extremely high energy span ratio (1:175). Therefore, we envision replacement of the current injector with a 650 MeV 3-pass recirculating injector based on the existing LERF facility. Finally, the 22 GeV CEBAF would promise to deliver in 10-passes a beam with normalized emittance of 80 mm·mrad and with a relative energy spread of 1.5 × 10-3. Further recirculation beyond 22 GeV is limited by large, 974 MeV per electron, energy loss due to synchrotron radiation.

Bogacz, Slawomir↗

DOE OSTI2025

Migratory Strategy is a Key Factor Driving Interactions at Wind Energy Facilities in At-Risk North American Bats

Animal migration remains poorly understood for many organisms, impeding understanding of movement dynamics and limiting conservation actions. We develop a framework that scales from movements of individuals to the dynamics of continental migration using data synthesis of endogenous markers, which we apply to three North American bat species with unexplained high rates of fatalities at wind energy facilities. The two species experiencing the highest fatality rates exhibit a "pell-mell" migration strategy in which individuals move from summer habitats in multiple directions, both to higher and lower latitudes, during autumn. We link movements to higher latitudes to encounters with wind energy facilities and report that the timing of pell-mell migration strongly overlaps with that of fatalities at the continental level. These findings support the hypothesis that migration distance and strategy are drivers of increased interactions with wind energy facilities, highlighting the significance of understanding migratory strategy to achieve conservation goals.

08 HYDROGEN↗

DOE OSTI2022

Studies of the weak interaction in atomic systems: towards measurements of atomic parity non-conservation in francium

Abstract Tests of the standard model of particle physics should be carried out over the widest possible range of energies. Here we present our plans and progress for an atomic parity non-conservation experiment using the heaviest alkali, francium ( Z = 87), which has no stable isotope. Low-energy tests of this kind have sensitivity complementary to higher energy searches, e.g. at the large hadron collider.

74 ATOMIC AND MOLECULAR PHYSICS↗

DOE OSTI2020

Active Learning Accelerated Discovery of Stable Iridium Oxide Polymorphs for the Oxygen Evolution Reaction

The discovery of high-performing and stable materials for sustainable energy applications is a pressing goal in catalysis and materials science. Understanding the relationship between a material’s structure and functionality is an important step in the process, such that viable polymorphs for a given chemical composition need to be identified. Machine-learning-based surrogate models have the potential to accelerate the search for polymorphs that target specific applications. Herein, we report a readily generalizable active-learning (AL) accelerated algorithm for identification of electrochemically stable iridium oxide polymorphs of IrO 2 and IrO 3 . The search is coupled to a subsequent analysis of the electrochemical stability of the discovered structures for the acidic oxygen evolution reaction (OER). Structural candidates are generated by identifying all 956 structurally unique AB2 and AB3 prototypes in existing materials databases (more than 38000). Next, using an active learning approach, we find 196 IrO 2 polymorphs within the thermodynamic amorphous synthesizability limit and reaffirm the global stability of the rutile structure. We find 75 synthesizable IrO 3 polymorphs and report a previously unknown FeF 3 -type structure as the most stable, termed α-IrO 3 . To test the algorithms performance, we compare to a random search of the candidate space and report at least a 2-fold increase in the rate of discovery. Additionally, the AL approach can acquire the most stable polymorphs of IrO 2 and IrO 3 with fewer than 30 density functional theory optimizations. Analysis of the structural properties of the discovered polymorphs reveals that octahedral local coordination environments are preferred for nearly all low-energy structures. Subsequent Pourbaix Ir–H 2 O analysis shows that α-IrO3 is the globally stable solid phase under acidic OER conditions and supersedes the stability of rutile IrO 2 . Calculation of theoretical OER surface activities reveal ideal weaker binding of the OER intermediates on α-IrO 3 than on any other considered iridium oxide. We emphasize that the proposed AL algorithm can be easily generalized to search for any binary metal oxide structure with a defined stoichiometry.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗