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Results for “Gas/Surface Reflections or Scattering”

Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 145 records · Page 8
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DOE OSTI2026

Nonequilibrium magnons studied by inelastic neutron scattering

In this work, we explore time-resolved dynamics of non-equilibrium magnons in Rb2MnF4, a model two-dimensional square lattice Heisenberg antiferromagnet using a novel laser-neutron pump-probe technique. This technique uses a nanosecond pulsed laser to periodically excite magnons to out-of-equilibrium states and then probe the resulting dynamics using INS.

36 MATERIALS SCIENCE↗
NASA NTRS2019

Cloud Scattering Impact on Thermal Radiative Transfer and Global Longwave Radiation

The potential importance of longwave (LW) cloud scattering has been recognized but the actual estimate of this effect on thermal radiation varies greatly among different studies. General circulation models (GCMs) generally neglect or simplify the multiple scattering in the LW. In this study, we use a rigorous radiative transfer algorithm to explicitly consider LW multiple-scattering and apply the GCM to quantify the impact of cloud LW scattering on thermal radiation fluxes. Our study shows that the cloud scattering effect on downward thermal radiation at the surface is concentrated in the infrared atmospheric window spectrum (800–1250 cm9exp −1)). The scattering effect on the outgoing longwave radiation (OLR) is also present in the window region over low clouds but it is mainly in the far-infrared spectrum (300–600 cm(exp −1)) over high clouds. For clouds with small to moderate optical depth (τ < 10), the scattering effect on thermal fluxes shows large variation with the cloud τ and has a maximum at an optical depth of ∼3. For opaque clouds, the scattering effect approaches an asymptote and is smaller and less important. The 2-stream radiative transfer scheme could have an error over 10% with an RMS error around 3.5%–4.0% in the calculated LW flux. This algorithm error of the 2-stream approximation could readily exceed the no-scattering error in the LW, and thus it is worthless to include the time-consuming computation of multiple scattering in a 2-stream radiative transfer scheme. However, the calculation error rapidly decreases as stream number increases and the RMS error in LW flux using the 4-stream scheme is under 0.3%, an accuracy sufficient for most climate studies. We implement the 4-stream discrete-ordinate algorithm in the GISS GCM and run the GCM for 20 years with and without the LW scattering effect, respectively. When cloud LW scattering is included, we find that the global annual mean OLR is reduced by 2.7 W/m(exp 2), and the downward surface flux and the net atmospheric absorption are increased by 1.6 W/m2 and 1.8 W/m(exp 2), respectively. Using one year of ISCCP clouds and running the standalone radiative transfer offline, the global annual mean non-scattering errors in OLR, surface LW downward flux and net atmospheric absorption are 3.6 W/m(exp 2), −1.1 W/m(exp 2), and −2.5 W/m(exp 2), respectively. The global scattering impact of 2.7 W/m(exp 2) on the OLR is small when compared to the typical global OLR value of 240 W/m2, but it is significant when compared to cloud LW radiative forcing (30 W/m2) and net cloud forcing (−14 W/m(exp 2)). Overall, the effect of neglecting scattering on the thermal fluxes is comparable to the reported clear sky radiative effect of doubling CO2.

longwave cloud scattering↗
DOE OSTI2020

Higher-order phonon scattering: advancing the quantum theory of phonon linewidth, thermal conductivity and thermal radiative properties

Phonon scattering plays a central role in the quantum theory of phonon linewidth, which in turn governs important properties including infrared spectra, Raman spectra, lattice thermal conductivity, thermal radiative properties, and also signifi- cantly affects other important processes such as hot electron relaxation. Since Maradudin and Fein’s classic work in 1962, three-phonon scattering had been considered as the dominant intrinsic phonon scattering mechanism and has seen tremendous advances. However, the role of the higher-order four-phonon scattering had been persistently unclear and so was ignored. The tremendous complexity of the formalism and computational challenges stood in the way, prohibiting the direct and quantitative treatment of four-phonon scattering. In 2016, a rigorous four-phonon scattering formalism was developed, and the prediction was realized using empirical potentials. In 2017, the method was extended using first-principles calculated force constants, and the thermal conductivities of boron arsenides (BAs), Si and diamond were predicted. The predictions for BAs were later confirmed by several independent experiments. Four-phonon scattering has since been investigated in a range of materials and established as an important intrinsic scattering mechanism for thermal transport and radiative properties. Specifically, four-phonon scattering is important when the fourth-order scattering potential or phase space becomes relatively large. The former scenario includes: (i) nearly all materials when the temperature is high; (ii) strongly anharmonic (low thermal conductivity) materials, including most rocksalt compounds, halides, hydrides, chalcogenides and oxides. The latter scenario includes: (iii) materials with large acoustic–optical phonon band gaps, such as XY compounds with a large atomic mass ratio between X and Y; (iv) two- dimensional materials with reflection symmetry, such as single-layer graphene, single-layer boron nitride and carbon nanotubes; and (v) phonons with a large density of states, such as optical phonons, which are important for Raman, infrared and thermal radiative properties. Four-phonon scattering is expected to gain broad interest in various technologically important materials for thermoelectrics, thermal barrier coatings, thermal energy storage, phase change, nuclear power, ultra-high temperature ceramics, infrared spectra, Raman spectra, radiative transport, hot electron relaxation and radiative cooling. Four-phonon scattering has been, and will continue to be, established as an important intrinsic phonon scattering mechanism beyond three-phonon scattering. The prediction of four-phonon scattering will transition from a breakthrough to a new routine in the next decade.

Feng, Tianli↗
NASA NTRS2007

Fitting a Two-Component Scattering Model to Polarimetric SAR Data from Forests

Two simple scattering mechanisms are fitted to polarimetric synthetic aperture radar (SAR) observations of forests. The mechanisms are canopy scatter from a reciprocal medium with azimuthal symmetry and a ground scatter term that can represent double-bounce scatter from a pair of orthogonal surfaces with different dielectric constants or Bragg scatter from a moderately rough surface, which is seen through a layer of vertically oriented scatterers. The model is shown to represent the behavior of polarimetric backscatter from a tropical forest and two temperate forest sites by applying it to data from the National Aeronautic and Space Agency/Jet Propulsion Laboratory's Airborne SAR (AIRSAR) system. Scattering contributions from the two basic scattering mechanisms are estimated for clusters of pixels in polarimetric SAR images. The solution involves the estimation of four parameters from four separate equations. This model fit approach is justified as a simplification of more complicated scattering models, which require many inputs to solve the forward scattering problem. The model is used to develop an understanding of the ground-trunk double-bounce scattering that is present in the data, which is seen to vary considerably as a function of incidence angle. Two parameters in the model fit appear to exhibit sensitivity to vegetation canopy structure, which is worth further exploration. Results from the model fit for the ground scattering term are compared with estimates from a forward model and shown to be in good agreement. The behavior of the scattering from the ground-trunk interaction is consistent with the presence of a pseudo-Brewster angle effect for the air-trunk scattering interface. If the Brewster angle is known, it is possible to directly estimate the real part of the dielectric constant of the trunks, a key variable in forward modeling of backscatter from forests. It is also shown how, with a priori knowledge of the forest height, an estimate for the attenuation coefficient of the canopy can be obtained directly from the multi-incidence-angle polarimetric observations. This attenuation coefficient is another key variable in forward models and is generally related to the canopy density.

temperate forests↗