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NASA NTRS2018

Propynal, an Interstellar Molecule with an Exceptionally Strong C≡C Infrared Band - Laboratory Infrared Data and Applications

Isomers with the formulaC3H2Ohave intrigued and puzzled astronomers and astrochemists for many years, with propynal and cyclopropenone, but not propadienone, known to be interstellar. However, there is a severe lack of laboratory spectra of the solid phases of these compounds with which to investigate their interstellar chemistry. Here we present the first infrared spectra of amorphous and crystalline forms of propynal, HCC C(O)H, at multiple temperatures. Band positions are tabulated and band strengths are derived in terms of absorption coefficients and integrated intensities. Optical constants are calculated for amorphous propynal, refractive indices aremeasured, and densities are estimated. Three laboratory astrochemistry applications are described, including a new spectral identification in an earlier paper. It is shown that propynal’s C C infrared absorbance is about 30 000 per cent stronger than the corresponding feature in acetylene. This band’s intensity and spectral position make it an attractive candidate for astronomical searches involving interstellar ices.

astrochemistry – ISM: molecules↗
NASA NTRS1990

Studies of dust grain properties in infrared reflection nebulae

A model has been developed for reflection nebulae around luminous IR sources embedded in dense dust clouds. The shape of the IR spectrum is shown to be the result of a combination of the scattering properties of the dust, the spectrum of the illuminating source, and foreground extinction, while geometry plays a minor role. Comparison of the model results with IR observations of the reflection nebula surrounding OMC-2/IRS 1 shows that either a grain size distribution like that found in the diffuse ISM, or consisting of larger grains, can explain the observed shape of the spectrum. However, the absolute intensity level of the scattered light, as well as the observed polarization, requires large grains. By adding water-ice mantles to the silicate and graphite cores, the 3.08 micron ice-band feature observed in the spectra of several IR reflection nebulae has been modeled. It is shown that this ice band arises naturally in optically thick reflection nebulae containing ice-coated grains.

Pendleton, Y. J.↗
NASA NTRS2003

OMEGA Observations of Mars Analogue Rocks

In the last 20 years, imaging spectrometry in the visible and near infrared onboard spacecraft has become an essential technique to study surfaces and atmospheres of planetary objects, prior and in addition to in-situ analyses. Remote sensing experiments analyzing the sunlight reflected by planetary surfaces can be used to derive the mineralogical composition and physical properties of the natural surfaces and atmospheres observed. This technique was successfully used on Mars with ISM instrument. As an improvement of ISM, OMEGA onboard MARS-EXPRESS will play a key role in the mineralogical mapping of the Martian surface. We present the reflectance measurements made with OMEGA during on ground calibration sessions on natural slabs of rocks and minerals part of a database which will be used on similar future American instruments (as CRISM onboard MRO). We discuss the implication on the scientific capabilities of OMEGA instrument.

Bonello, G.↗
NASA NTRS2018

Propynal, an Interstellar Molecule with an Exceptionally Strong C ≡ C Infrared Band – Laboratory Infrared Data and Applications

Isomers with the formula C3H2O have intrigued and puzzled astronomers and astrochemists for many years, with propynal and cyclopropenone, but not propadienone, known to be interstellar. However, there is a severe lack of laboratory spectra of the solid phases of these compounds with which to investigate their interstellar chemistry. Here we present the first infrared spectra of amorphous and crystalline forms of propynal, HCC—C(O)H, at multiple temperatures. Band positions are tabulated and band strengths are derived in terms of absorption coefficients and integrated intensities. Optical constants are calculated for amorphous propynal, refractive indices are measured, and densities are estimated. Three laboratory astrochemistry applications are described, including a new spectral identification in an earlier paper. It is shown that propynal's C≡C infrared absorbance is about 30 000 per cent stronger than the corresponding feature in acetylene. This band's intensity and spectral position make it an attractive candidate for astronomical searches involving interstellar ices.

astrochemistry – ISM: molecules↗
NASA NTRS1995

Toward the detection of pure carbon clusters in the Interstellar Medium (ISM)

Determination of the form and distribution of carbon in the universe is critical to understanding the origin of life on Earth and elsewhere. Two potentially large reservoirs of carbon in the interstellar medium (ISM) remain unexplored. These are polycyclic aromatic hydrocarbons (PAH) and pure carbon clusters. Little information exists on the structures, properties, and transition frequencies of pure carbon clusters. The work described is designed to provide a specific inventory of laboratory frequencies and physical properties of this carbon clusters so that efforts can be made to detect them in cold interstellar sources by far-infrared astronomy. Data is given from infrared laser spectroscopy determination of the structure of C3, C4, C5, C6, C7, and C9.

Heath, J. R.↗
NASA NTRS2021

Extragalactic Magnetism with SOFIA (Legacy Program). I. The Magnetic Field in the Multiphase Interstellar Medium of M51*

The recent availability of high-resolution far-infrared (FIR) polarization observations of galaxies using HAWC+/SOFIA has facilitated studies of extragalactic magnetic fields in the cold and dense molecular disks. We investigate whether any significant structural differences are detectable in the kiloparsec-scale magnetic field of the grand design face-on spiral galaxy M51 when traced within the diffuse (radio) and the dense and cold (FIR) interstellar medium (ISM). Our analysis reveals a complex scenario where radio and FIR polarization observations do not necessarily trace the same magnetic field structure. We find that the magnetic field in the arms is wrapped tighter at 154 μm than at 3 and 6 cm; statistically significant lower values for the magnetic pitch angle are measured at FIR in the outskirts (R ≥ 7 kpc) of the galaxy. This difference is not detected in the interarm region. We find strong correlations of the polarization fraction and total intensity at FIR and radio with the gas column density and 12CO(1–0) velocity dispersion. We conclude that the arms show a relative increase of small-scale turbulent B-fields at regions with increasing column density and dispersion velocities of the molecular gas. No correlations are found with H i neutral gas. The star formation rate shows a clear correlation with the radio polarized intensity, which is not found in FIR, pointing to a small-scale dynamo-driven B-field amplification scenario. This work shows that multiwavelength polarization observations are key to disentangling the interlocked relation between star formation, magnetic fields, and gas kinematics in the multiphase ISM.

Spiral galaxies↗
NASA NTRS1991

Measurement of the spectral signature of small carbon clusters at near and far infrared wavelengths

A significant percentage of the carbon inventory of the circumstellar and interstellar media may be in the form of large refractory molecules (or small grains) referred to as carbon clusters. At the small end, uneven numbers of carbon atoms seem to be preferred, whereas above 12 atoms, clusters containing an even number of carbon atoms appear to be preferred in laboratory chemistry. In the lab, the cluster C-60 appears to be a particularly stable form and has been nicknamed Bucky Balls because of its resemblance to a soccer ball and to geodesic domes designed by Buckminster Fuller. In order to investigate the prevalence of these clusters, and their relationship to the polycyclic aromatic hydrocarbons (PAHs) that have become the newest focus of IR astronomy, it is necessary to determine the spectroscopic characteristics of these clusters at near and far infrared wavelengths. Described here is the construction of a near to far IR laser magnetic resonance spectrometer that has been built at the University of California Berkeley in order to detect and characterize these spectra. The equipment produces carbon clusters by laser evaporation of a graphitic target. The clusters are then cooled in a supersonic expansion beam in order to simulate conditions in the interstellar medium (ISM). The expansion beam feeds into the spectrometer chamber and permits concentrations of clusters sufficiently high as to permit ultra-high resolution spectroscopy at near and far IR wavelengths. The first successful demonstration of this apparatus occurred last year when the laboratory studies permitted the observational detection of C-5 in the stellar outflow surrounding IRC+10216 in the near-IR. Current efforts focus on reducing the temperature of the supersonic expansion beam that transport the C clusters evaporated from a graphite target into the spectrometer down to temperatures as low as 1 K.

Tarter, J.↗
NASA NTRS1990

Contribution of cool dust to the FIR brightness distribution of NGC 6946 Sc(s)2

A few galaxies have been observed at submillimeter wavelengths (Stark et al., 1988; Eales, Wynn-Williams, and Duncan, 1988). These observations do not support the hypothesis that there exist substantial amounts of cool dust generating submillimeter radiation in excess of predictions from modified blackbody curves of the form (1/lambda)exp 1.5 B sub v (v, T) fit to total 100 and 160 micron fluxes. However, researchers find relatively cold dust (approx. 17 to 23 degrees K) at several interarm locations in the central 5 minute by 5 minute region of NGC 6946 Sc(s)II. Since molecular gas is the predominate constituent of the interstellar medium (ISM) in this region, such low dust temperatures are indicative of quiescent molecular clouds and low star formation rates. Based on the contribution of cool grains to the 160 micron surface brightness distribution, regions of low star formation activity can be identified. A 1/lambda exp 1.5 emissivity law is assumed for this analysis. Researchers assumed a two temperature grain model in an effort to decompose the far infrared surface brightness distribution of NGC 6946 into contributions from cool, quiescent and active, star forming regions. This model has some validity; although an oversimplification of the dust energetics, researchers find from it that, where giant HII regions are sparse, a significant fraction of the 160 micron emission is emitted by a cool grain component which the Infrared Astronomy Satellite (IRAS) could barely detect.

Engargiola, Greg↗
NASA NTRS1990

The infrared structure of M33

IRAS spatial observations of M33 are presented and compared to UV optical, and radio wavelength data. At 12, 25, 60, and 100 microns the emission appears as two bright spiral arms superposed on a diffuse disk, with localized sources at the position of the nucleus and the brightest H II region complexes. The global IR properties of M33 are characteristic of quiescent spirals. The 8-30 micron mid-IR global emission is about 20 percent of the far-IR emission, similar to the ratio of these fluxes found for the local ISM. The local IR excess of M33 is about 2-3 times larger than the excess derived for H II regions in the Galaxy. The radial distributions of the IR colors are flat or nearly flat, implying near-constant dust temperatures across the diffuse disk. The integrated F(IR)-to-radio continuum emission of M33 follows the relation seen in other galaxies, but the radial distribution of the two emission components differ. A striking correlation is seen between the IR emission structure and the distribution of H II regions.

Rice, W.↗
NASA NTRS1987

The large scale gas and dust distribution in the galaxy: Implications for star formation

Infrared Astronomy Observations are presented for the diffuse infrared (IR) emissions from the galactic plane at wavelengths of 60 and 100 microns and the total far infrared intensity and its longitudinal variations in the disk were derived. Using available CO, 5 GHz radio-continuum, and HI data, the IR luminosity per hydrogen mass and the ingrared excess (IRE) ratio in the Galaxy were derived. The longitudinal profiles of the 60 and 100 micron emission were linearly decomposed into three components that are associated with molecular (H2), neutral (HI), and ionized (HII) phases in the interstellar medium (ISM), and the relevant dust properties were derived in each phase. Implications of the findings for various models of the diffuse IR emisison and for star formation in the galactic disk are discussed.

Sodroski, T. J.↗
NASA NTRS2005

From Astrochemistry to Astrobiology

Tremendous strides have been made in our understanding of interstellar material over the past twenty five years thanks to significant developments in observational astronomy and laboratory astrophysics. Twenty years ago the composition of interstellar dust was largely guessed at, the concept of ices in dense molecular clouds ignored, and the notion of large, abundant, gas phase, carbon-rich molecules widespread throughout the interstellar medium (ISM) considered impossible. Today the composition of interstellar dust is reasonably well understood. In molecular clouds, the birthplace of stars and planets, these cold dust particles are coated with mixed molecular ices whose composition is very well constrained. Lastly, the signature of carbon-rich polycyclic aromatic hydrocarbons (PAHs), shockingly large molecules by early interstellar chemistry standards, is widespread throughout the Universe. The first part of this talk will describe how infrared spectroscopic studies of interstellar space, combined with laboratory simulations of interstellar ice chemistry, have revealed the widespread presence of interstellar PAHs and the composition of interstellar ices, the building blocks of comets. The remainder of the presentation will focus on the photochemical evolution of these materials and astrobiology. Within a molecular cloud, and especially the presolar nebula, materials frozen into the ices are photoprocessed by ultraviolet light and produce more complex molecules. As these materials are the building blocks of comets and related to carbonaceous micrometeorites, they are likely to have been important sources of complex materials delivered to the early Earth and their composition may be related to the origin of life.

Allamandola, L. J.↗
NASA NTRS1987

A radiative bow shock wave (?) driven by nuclear ejecta in a Seyfert galaxy

New VLA maps at 2 cm of the 13-arcsec-scale linear radio source in the center of NGC 1068 are described. The northeast lobe shows a limb-brightened conical morphology, very sharp 'leading' edges, and a magnetic field running parallel to these edges. The spectral index between 2 and 6 cm in these line-brightened regions is near 1.0. The northeast subpeak has a very steep radio spectrum between 18 and 2 cm which is attributed to inverse Compton losses of the relativistic electrons on the infrared photons. The spectral indices in the southwest lobe lie in the range 0.9-1.5 except in its northern parts, where a much larger index is found. The northeast lobe radio emission could arise in either the cocoon of old jet material which has passed through the internal shock in the ejecta and blown out to either side, or in interstellar material compressed by a bow shock wave driven into the galactic ISM.

Wilson, Andrew S.↗
NASA NTRS1989

Intermittent behavior of galactic dynamo activities

Recent observations by Beck and Golla of far-infrared and radio continuum emission from nearby spiral galaxies suggest that the galactic magnetic field strength is connected to the current star formation rate. The role of star formation on the generation of large-scale galactic magnetic field is studied in this paper. Using a simple galactic model, it is shown how the galactic dynamo depends strongly on the turbulent velocity of the interstellar medium. When the star formation efficiency is high, the ISM is churned which in turn amplifies the galactic magnetic field. Between active star formation epochs, the magnetic field is in dormant state and decays at a negligible rate. If density waves trigger star formation, then they also turn on the otherwise dormant dynamo.

Ko, C. M.↗
NASA NTRS2017

High-Resolution IR Absorption Spectroscopy of Polycyclic Aromatic Hydrocarbons in the 3-micrometers Region: Role of Periphery

In this work we report on high-resolution IR absorption studies that provide a detailed view on how the peripheral structure of irregular polycyclic aromatic hydrocarbons (PAHs) affects the shape and position of their 3-micrometers absorption band. To this purpose we present mass-selected, high-resolution absorption spectra of cold and isolated phenanthrene, pyrene, benz[a]antracene, chrysene, triphenylene, and perylene molecules in the 2950-3150 per cm range. The experimental spectra are compared with standard harmonic calculations, and anharmonic calculations using a modified version of the SPECTRO program that incorporates a Fermi resonance treatment utilizing intensity redistribution. We show that the 3-micrometers region is dominated by the effects of anharmonicity, resulting in many more bands than would have been expected in a purely harmonic approximation. Importantly, we find that anharmonic spectra as calculated by SPECTRO are in good agreement with the experimental spectra. Together with previously reported high-resolution spectra of linear acenes, the present spectra provide us with an extensive dataset of spectra of PAHs with a varying number of aromatic rings, with geometries that range from open to highly-condensed structures, and featuring CH groups in all possible edge configurations. We discuss the astrophysical implications of the comparison of these spectra on the interpretation of the appearance of the aromatic infrared 3-micrometers band, and on features such as the two-component emission character of this band and the 3-micrometers emission plateau.

techniques: spectroscopic↗
NASA NTRS2005

Cooked GEMS - Insights into the Hot Origins of Crystalline Silicates in Circumstellar Disks and the Cold Origins of GEMS

The comparison of interstellar, circumstellar and primitive solar nebula silicates has led to a significant conundrum in the understanding of the nature of solid materials that begin the planet forming processes. Crystalline silicates are found in circumstellar regions around young stars and also evolved stars ejecting particles into the interstellar medium (ISM) but they are not seen in the interstellar medium itself, the source material for star and planet formation. Crystalline silicates are minor to major components of all known early solar system materials that have been examined as meteorites or interplanetary dust samples. The strong presence of Mg-rich crystalline silicates in Oort cloud comets and their minor presence in some Kuiper belt comets is also indicated by 11.2 m peak in approx. 10 microns "silicate" infrared feature. This evidence strongly indicates that Mg-rich crystalline silicates were abundant components of the solar nebula disk out to at least 10 AU, and present out to 30 AU.

Brownlee, D. E.↗
NASA NTRS1984

A far-infrared survey of the galactic center

The region within + or - 1.5 deg of the galactic center has been surveyed at a resolution of 1 arcmin between 40 and 250 microns. Forty-seven FIR sources were detected in the field, 38 of them spatially coincident with prominent radio-emitting regions. The 27 sources associated with H II regions have luminosities ranging from 500,000 to ten million solar luminosities, average infrared excesses of 16, and average dust-to-gas ratios of 0.002. They are located in a narrow band centered on Sgr A. Each FIR source appears to be powered by small numbers of early type O stars. The initial luminosity functions for these sources is best fitted by an exponential form with an e-folding luminosity of 2.3 million solar luminosities. The extended thermal emission of the region is consistent with a population of 30,000-50,000 ZAMS stars embedded in an ISM with a Lyman-continuum optical depth of 1-1.5.

Odenwald, S. F.↗
NASA NTRS2001

New Interstellar Dust Models Consistent with Interstellar Extinction, Emission and Abundances Constraints

We present new interstellar dust models that are consistent with both, the FUV to near-IR extinction and infrared (IR) emission measurements from the diffuse interstellar medium. The models are characterized by different dust compositions and abundances. The problem we solve consists of determining the size distribution of the various dust components of the model. This problem is a typical ill-posed inversion problem which we solve using the regularization approach. We reproduce the Li Draine (2001, ApJ, 554, 778) results, however their model requires an excessive amount of interstellar silicon (48 ppM of hydrogen compared to the 36 ppM available for an ISM of solar composition) to be locked up in dust. We found that dust models consisting of PAHs, amorphous silicate, graphite, and composite grains made up from silicates, organic refractory, and water ice, provide an improved fit to the extinction and IR emission measurements, while still requiring a subsolar amount of silicon to be in the dust. This research was supported by NASA Astrophysical Theory Program NRA 99-OSS-01.

Zubko, V.↗
DOE OSTI2022

Optical properties of Peaked Spectrum radio sources

ABSTRACT In this work, we study the optical properties of compact radio sources selected from the literature in order to determine the impact of the radio-jet in their circumnuclear environment. Our sample includes 58 Compact Steep Spectrum (CSS) and GigaHertz Peaked Spectrum (GPS) and 14 Megahertz-Peaked spectrum (MPS) radio sources located at z ≤ 1. The radio luminosity (LR) of the sample varies between Log LR ∼ 23.2 and 27.7 W Hz−1. We obtained optical spectra for all sources from SDSS-DR12 and performed a stellar population synthesis using the starlight code. We derived stellar masses (M⋆), ages 〈t⋆〉, star formation rates (SFR), metallicities 〈Z⋆〉 and internal reddening AV for all young AGNs of our sample. A visual inspection of the SDSS images was made to assign a morphological class for each source. Our results indicate that the sample is dominated by intermediate to old stellar populations and there is no strong correlation between optical and radio properties of these sources. Also, we found that young AGNs can be hosted by elliptical, spiral and interacting galaxies, confirming recent findings. When comparing the optical properties of CSS/GPS and MPS sources, we do not find any significant difference. Finally, the Mid-Infrared WISE colours analysis suggests that the compact radio sources defined as powerful AGNs are, in general, gas-rich systems.

79 ASTRONOMY AND ASTROPHYSICS↗