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At least 145 records · Page 8

Estimating List-Mode Data Sensitivities to Nuclear Data with MCNP6

Nuclear data are a vital component of predictive simulations used in applications like experiment design, stockpile stewardship, nuclear nonproliferation/safeguards, health physics, and criticality safety. A singular simulation requires the coalescence of different areas of nuclear data such as cross sections, angular distributions, and energy distributions of emitted neutrons for different materials and energy ranges. Improving nuclear data and thus reducing the uncertainty in simulated parameters could enable smaller, better-informed safety factors and ultimately reduce operational and procedural costs. There is a constant effort to garner a better understanding of the physical quantities represented by nuclear data through experiments. Integral experiment benchmarks use simulated and measured results to validate current nuclear data values. In the past, benchmarks primarily focused on the effective multiplication factor (k eff ); however, this limited scope has caused compensating errors and areas of nuclear data that lack validation. Compensating errors are inaccuracies in nuclear data that are obfuscated by cancellation when observing integrated values such as k eff . Diverse integral benchmark experiments that look for quantities of interest other than k eff and include multiple responses minimize the possibility of compensating errors and provides validation to areas of nuclear data previously lacking experimental validation. Benchmark experiments can be optimized during the design process to be highly dependent on specific areas of nuclear data. The dependence of a response in an experiment to a specific area/type of nuclear data is defined as sensitivity. A larger sensitivity means that nuclear data uncertainties will play a larger role in the response(s) resulting in larger bias. Currently, the sensitivity capabilities of the Monte Carlo N-Particle (MCNP ®1 ) transport code are limited to responses of k eff and tallied values (e.g., flux, surface current). As a part of the EUCLID project, this work explores estimating list-mode nuclear data sensitivities that can be used to design experiments aimed to constrain and reduce compensating errors in nuclear data by focusing on responses other than k eff . Tallied values are ideal quantities that are estimated with detectors during experiments. List-mode data (a list of neutron collection times) are the direct output of detector systems in subcritical neutron noise experiments. Expanding MCNP sensitivity capabilities to include the sensitivity of responses estimated from list-mode data, such as the prompt neutron decay constant (α) and multiplicity estimates (S and D), enables more direct comparison of simulated and measured experimental quantities. Additionally, deterministic tools such as SENSMG are capable of obtaining sensitivities to a wide variety of responses; however, these tools cannot handle complex geometries due to the assumptions made in discretizing the phase-space variables of the Boltzman transport equation.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

The effect of areal density asymmetries on scattered neutron spectra in ICF implosions

Scattered neutron spectroscopy is a diagnostic technique commonly used to measure areal density in inertial confinement fusion experiments. Deleterious areal density asymmetries modify the shape of the scattered neutron spectrum. In this work, a novel analysis is developed, which can be used to fit the shape change. This will allow experimental scattered neutron spectroscopy to directly infer the amplitude and mode of the areal density asymmetries, with little sensitivity to confounding factors that affect other diagnostics for areal density. The model is tested on spectra produced by a neutron transport calculation with both isotropic and anisotropic primary fusion neutron sources. Multiple lines of sight are required to infer the areal density distribution over the whole sphere—we investigate the error propagation and optimal detector arrangement associated with the inference of mode 1 asymmetries.

Crilly, A. J. (ORCID:0000000204299332)↗

Anisotropy in Thermal Conductivity of Ga2O3 under Irradiation: Ab-initio Investigations

Ga2O3 is a wide-bandgap semiconducting material known for its high breakdown electric field and thermal stability. Its various crystalline forms have shown great potential in power electronics, optoelectronics, and high-temperature applications. Specifically, ß-Ga2O3 has been recognized for its suitability in neutron and gamma radiation detection, making it ideal for sensor and detector applications [1]. Notably, ß-Ga2O3 exhibits anisotropic thermal conductivity, meaning that the magnitude of thermal conductivity varies with the crystallographic direction [2]. Under neutron irradiation, Ga2O3 undergoes a significant phenomenon, resulting in the formation of Helium bubbles within its crystalline matrix. The presence of Helium in Ga2O3 has been found to influence the material's anisotropic thermal conductivity. In this study, the objectives were twofold: firstly, to employ Density Functional Theory (DFT) to determine the most probable sites of Helium occupation in ß-Ga2O3, and secondly, to investigate the anisotropic variation in thermal conductivity when Helium is present in the crystalline matrix of ß-Ga2O3. These ab-initio DFT studies provide crucial insights into understanding the behavior of Helium in Ga2O3 and its impact on thermal conductivity, which can contribute to further advancements in sensor and detector applications based on this wide-bandgap semiconductor.

36 MATERIALS SCIENCE↗

Deployment of ADTimePix3 areaDetector Driver at Neutron and X-ray User Facilities

TimePix3 is a 65k hybrid pixel readout chip with simultaneous Time-of-Arrival (ToA) and Time-over-Threshold (ToT) recording in each pixel*. The chip operates without a trigger signal with a sparse readout where only pixels containing events are read out. The flexible architecture allows 40 MHits/s/cm² readout throughput, using simultaneous readout and acquisition by sharing readout logic with transport logic of superpixel matrix formed using 2x4 structure. The chip ToA records 1.5625 ns time resolution. The X-ray and charged particle events are counted directly. However, indirect neutron counts use 6Li fission in a scintillator matrix, such as ZnS(Ag). The fission space-charge region is limited to 5-9 um. A photon from scintillator material excites a photocathode electron, which is further multiplied in dual-stack MCP. The neutron count event is a cluster of electron events at the chip. We report on the EPICS areaDetector** ADTimePix3 driver that controls Serval*** using json commands. The driver directs data to storage and to a real-time processing pipeline and configures the chip. The time-stamped data are stored in raw .tpx3 file format and passed through a socket where the clustering software identifies individual neutron events. The conventional 2D images are available as images for each exposure frame, and a preview is useful for sample alignment. The areaDetector driver allows integration of time-enhanced capabilities of this detector into SNS beamlines controls and unprecedented time resolution.

Gofron, Kaz↗

Time extended production of neutrons during a solar flare

The most energetic neutral emissions expected from solar flares are gamma rays (10 MeV) from relativistic primary and secondary electron bremsstrahlung,from approx 0 meson decay, and from neutrons ( 50 MeV). Bremsstrahlung photon energies extend to that of the highest energy electron present, but the shape of the pi sup 0 gamma ray spectrum, peaking at 69 MeV, does not depend strongly on the proton spectrum above threshold, which is approx. 292 MeV for meson production on protons. The highest energy neutrons observed indicate directly the highest energy ions which interact at the Sun, and the presence or absence of anergy cutoff in the acceleration process. The high-energy proton spectrum shape can be determined from the neutron spectrum.

Chupp, E. L.↗

First direct observation of isomeric decay in neutron-rich odd-odd Ta186

Deexcitation γ rays associated with an isomeric state of 186 Ta were investigated. The isomers were produced in multinucleon transfer reactions between a 136 Xe beam and a natural W target and were collected and separated by the KEK Isotope Separation System. Two γ transitions with energies of 161.1(2) and 186.8(1) keV associated with an isomeric decay were observed for the first time. The half-life of the isomeric state of the neutral atom 186m Ta was deduced as 17(2) s. Based on the comparison with the previous measurements of the isomeric state using the Experimental Storage Ring at GSI Darmstadt and the coupling of angular momenta of individual particle orbitals in odd-odd nuclei, a decay scheme of 186m Ta was proposed.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Neutron Imaging Camera

The Neutron Imaging Camera (NIC) is based on the Three-dimensional Track Imager (3DTI) technology developed at GSFC for gamma-ray astrophysics applications. The 3-DTI, a large volume time-projection chamber, provides accurate, approximately 0.4 mm resolution, 3-D tracking of charged particles. The incident direction of fast neutrons, En > 0.5 MeV, are reconstructed from the momenta and energies of the proton and triton fragments resulting from (sup 3)He(n,p) (sup 3)H interactions in the 3-DTI volume. The performance of the NIC from laboratory and accelerator tests is presented.

Hunter, Stanley↗

Directional dependence of the event-by-event neutron-γ multiplicity correlations in 252 Cf(sf)

We differentiate the event-by-event n-γ multiplicity data from 252 Cf(sf) with respect to the energies of the emitted particles as well as their relative angles of emission. We determine that neutron emission enhances γ-ray emission around 0:7 and 1:2 MeV, but the only directional alignment was observed for E γ ≤ 0:7 MeV and tended to be parallel and antiparallel to neutrons emitted in the same event. The emission of γ rays at other energies was determined to be nearly isotropic. The presence of the emission and alignment enhancements is explained by positive correlations between neutron emission and quadrupole γ-ray emission along rotational bands in the de-exciting fragments. This observation corroborates the hypothesis of positive correlations between the angular momentum of a fragment and its intrinsic excitation energy. The results of this work are especially relevant in view of the recent theoretical and experimental interest in the generation of angular momentum in fission. Specifically, we have determined an alignment of the fragments angular momenta in a direction perpendicular to the direction of motion. We interpret the lack of n-γ angular correlations for fission fragments near closed shells as a weakening of the alignment process for spherical nuclei. Lastly, we have observed that statistical γ rays are emitted isotropically, indicating that the average angular momentum removed by this radiation is small. These results, and the analysis tools presented in this work, represent a stepping stone for future analysis of n-γ emission correlations and their connection to angular momentum properties.

73 NUCLEAR PHYSICS AND RADIATION PHYSICS↗

Reflectometry with Polarized Neutrons on In Situ Grown Thin Films

Originating from the demand for obtaining depth-resolved magnetization profiles from thin films and heterostructures, polarized neutron reflectometry (PNR) has developed into a unique research tool, which also finds application in the analysis of superconducting or soft matter thin films. While certain in situ sample environments such as gas-loading or humidity cells were quickly realized after PNR first emerged, preparing and growing thin magnetic films directly in the neutron beam could only be realized in recent years. Herein, a dedicated insight is given on the history and development of in situ thin film growth capabilities for PNR, from early pioneering experiments to the present day. The scientific and technological challenges as well as the advances of neutron sources, neutronics, and data treatment that have led to its realization are highlighted together with the unique research opportunities that it provides and recently obtained experimental results.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

Evolution of the two-neutron configuration from 11 Li to 13 Li

In this work we investigate the two-neutron decay of 13 Li and of the excited states of 11 Li populated via one-proton removal from 14 Be and 12 Be, respectively. A phenomenological model is used to describe the decay of 11 Li and 13 Li. While the first one displays important sequential components, the second one appears dominated by the direct two-neutron decay. A microscopic three-body model is used to extract information on the spatial configuration of the emitted neutrons before the decay and shows that the average distance between the neutrons increases going from 11 Li to 13 Li.

Dineutron decay↗

Neutron Imaging Camera

We describe the Neutron Imaging Camera (NIC) being developed for DTRA applications by NASA/GSFC and NSWC/Carderock. The NIC is based on the Three-dimensional Track Imager (3-DTI) technology developed at GSFC for gamma-ray astrophysics applications. The 3-DTI, a large volume time-projection chamber, provides accurate, approximately 0.4 mm resolution. 3-D tracking of charged particles. The incident direction of fast neutrons, E(sub N) > 0.5 MeV. arc reconstructed from the momenta and energies of the proton and triton fragments resulting from 3He(n,p)3H interactions in the 3-DTI volume. We present angular and energy resolution performance of the NIC derived from accelerator tests.

Hunter, Stanley D.↗

Uncertainty quantification and sensitivity analysis of a nuclear thermal propulsion reactor startup sequence

The research presented in this article describes progress in applying stochastic methods, uncertainty quantification, parametric studies, and variance-based sensitivity analysis (also known as Sobol sensitivity analysis) to a full-core model of a nuclear thermal propulsion (NTP) system simulated via the radiation transport code Griffin to simulate neutronics. Our goal is to develop a reduced-order (surrogate) model that can be rapidly sampled with perturbations to multiple input parameters. In this NTP system, reactivity and power feedback affect the rotation of control drums (CDs), which is itself controlled by a hybrid proportional-integral-derivative (PID) controller actuated by the power demand and reactivity feedback from the numerical model. This model uses reactor kinetic feedback (mean generation time [Λ] and effective delayed neutron fraction [ β eff ] from a transient Griffin simulation executed via Griffin’s improved quasi-static solver to provide the kinetic parameters) as inputs to functions that control the CD rotation angle. By investigating numerous stochastic approaches, we developed a dual-purpose surrogate model of the NTP system, using polynomial regression in the Multiphysics Object-Oriented Simulation Environment (MOOSE) Stochastic Tools Module (STM). The trained model can be rapidly sampled while simultaneously perturbing various input parameters, such as coefficients on the PID control or temperature (directly affecting the neutron cross section). The surrogate model delivers accurate (within 5%) results at speeds orders of magnitude faster (minutes, not days of computational time) than the base model. Once the surrogate model has been trained, distributions of the uncertain parameters can be changed at will to investigate the effects of perturbing multiple inputs as well as the effects of these inputs on the model output. For example, coefficients used in the PID control system may vary due to some type of physical interference, or uncertainty may exist in the temperature of the neutron cross sections in various regions of the reactor. A distribution can be placed on these parameters, and operational boundaries can be determined. The goal of this work is to support development of an advanced control system for operating CDs in a functioning NTP system. This work is a scoping study of the MOOSE STM.

21 - SPECIFIC NUCLEAR REACTORS AND ASSOCIATED PLAN↗

Measurements of low-mode asymmetries in the areal density of laser-direct-drive deuterium–tritium cryogenic implosions on OMEGA using neutron spectroscopy

Areal density is one of the key parameters that determines the confinement time in inertial confinement fusion experiments, and low-mode asymmetries in the compressed fuel are detrimental to the implosion performance. The energy spectra from the scattering of the primary deuterium–tritium (DT) neutrons off the compressed cold fuel assembly are used to investigate low-mode nonuniformities in direct-drive cryogenic DT implosions at the Omega Laser Facility. For spherically symmetric implosions, the shape of the energy spectrum is primarily determined by the elastic and inelastic scattering cross sections for both neutron-deuterium and neutron-tritium kinematic interactions. Two highly collimated lines of sight, which are positioned at nearly orthogonal locations around the OMEGA target chamber, record the neutron time-of-flight signal in the current mode. An evolutionary algorithm is being used to extract a model-independent energy spectrum of the scattered neutrons from the experimental neutron time-of-flight data and is used to infer the modal spatial variations (l = 1) in the areal density. Experimental observations of the low-mode variations of the cold-fuel assembly (ρL 0 + ρL 1 ) show good agreement with a recently developed model, indicating a departure from the spherical symmetry of the compressed DT fuel assembly. As a result, another key signature that has been observed in the presence of a low-mode variation is the broadening of the kinematic end-point due to the anisotropy of the dense fuel conditions.

47 OTHER INSTRUMENTATION↗

Ab initio nucleon-nucleus elastic scattering with chiral effective field theory uncertainties

Effective interactions for nucleon-nucleus elastic scattering from first principles require the use of the same nucleon-nucleon interaction in the structure and reaction calculations and a consistent treatment of the relevant operators at each order. Systematic investigations of the effect of truncation uncertainties of chiral nucleon-nucleon ( N N ) forces have been carried out for scattering observables in the two- and three-nucleons system as well as for bound-state properties of light nuclei. Here we extend this type of study to proton and neutron elastic scattering for 16 O and 12 C. Using the frameworks of the spectator expansion of multiple scattering theory as well as the no-core shell model, we employ one specific chiral interaction from the LENPIC collaboration and consistently calculate the leading-order effective nucleon-nucleus interaction up to the third chiral order, from which we extract elastic scattering observables. Then we apply pointwise as well as correlated uncertainty quantification for the estimation of the chiral truncation error. We calculate and analyze proton elastic scattering observables for 16 O and 12 C as well as neutron elastic scattering observables for 12 C between 65 and 185 MeV projectile kinetic energy. We find in all cases qualitatively similar results for the chiral truncation uncertainties as in few-body systems and assess them using similar diagnostic tools. The order-by-order convergence of the scattering observables for 16 O and 12 C is very reasonable around 100 MeV, while for higher energies the chiral expansion parameter becomes too large for convergence. Comparing proton and neutron differential cross sections reveals that their description is comparable up to around 100 MeV. Here, we also find a nearly perfect correlation between the differential cross section for neutron scattering and the N N Wolfenstein amplitudes for small momentum transfers. The diagnostic tools for studying order-by-order convergence in observables in few-body systems can be employed for observables in nucleon-nucleus scattering with only minor modifications provided the momentum scale in the problems is not too large. We also find that the chiral N N interaction on which our study is based gives a very good description of differential cross sections for 16 O and 12 C as low as 65-MeV projectile energy, particularly in the forward direction. In addition, the very forward direction of the neutron differential cross section mirrors the behavior of the N N interaction amazingly well.

6 ≤ A ≤ 19↗

Particle-in-cell simulations of burning inertial confinement fusion capsule implosions

Anomalies observed in the neutron spectral shift of high-yield shots at the National Ignition Facility (NIF) suggest the presence of suprathermal ions [E. P. Hartouni et al., Nat. Phys. 19, 72 (2023)], implying that kinetic effects play a significant role in burning inertial confinement fusion (ICF) plasmas. Furthermore, recent measurements of reaction-in-flight (RIF) neutrons offer a direct probe of the stopping power in the burning fuel region of high-energy alpha particles and up-scattered fuel ions. We have developed the particle-in-cell code PICNIC, an exactly energy-conserving particle-in-cell Monte-Carlo collision (PIC-MCC) code to simulate the burn stage in ICF. We present results from 1D spherical simulations of NIF shot N210808, which was the first to exceed the Lawson criterion for laser fusion. We find that the suprathermal ions generated by large-angle Rutherford and nuclear elastic scattering (NES) with fusion alphas produce an alpha knock-on neutron (AKN) signal consistent with the extent and relative yield of the AKN spectrum identified in ignition experiments at the NIF. Furthermore, we also find that the inclusion of large-angle scattering physics does not explain the anomalously large spectral shift observed in the experiment.

High-energy-density plasmas↗

Neutron diffraction reveals protonation states in pyridoxal‐5′‐phosphate‐free and glycine external aldimine‐bound serine hydroxymethyltransferase

Serine hydroxymethyltransferase (SHMT) is a critical enzyme in the one-carbon (1C) metabolism pathway catalyzing the reversible conversion of L-Ser into Gly and concurrent transfer of 1C unit to tetrahydrofolate (THF) to give 5,10-methylene-THF (5,10-MTHF), which is used in the downstream syntheses of biomolecules critical for cell proliferation. The cellular 1C metabolism is hijacked by many cancer types to support cancer cell proliferation, making SHMT a promising target for the design and development of novel small-molecule antimetabolite chemotherapies. To advance structure-assisted drug design, knowledge of SHMT catalysis is crucial, but can only be fully realized when the atomic details of each reaction step governed by the acid–base catalysis are elucidated by visualizing active site hydrogen atoms. Here, we used room-temperature neutron crystallography to directly determine protonation states in Thermus thermophilus SHMT (TthSHMT), capturing protomer A in the apo form lacking the coenzyme pyridoxal 5′-phosphate (PLP), and protomer B as a ternary complex with PLP–Gly-external aldimine and (6S)-5-methyltetrahydrofolate (5MTHF). We observed protonation of the Schiff base nitrogen in PLP–Gly and neutrality of the catalytic Lys226 side chain in the ternary complex, whereas Lys226 is protonated and positively charged in the apo-active site. Furthermore, we obtained an X-ray structure of TthSHMT in complex with the substrate THF, which binds identically as 5MTHF at the peripheral binding site. In conclusion, the unique structural and functional information provided by neutron crystallography, in combination with X-ray structures, can be employed in the rational design of SHMT inhibitors.

X-ray crystallography↗

Structure of 30 Mg explored via in-beam γ-ray spectroscopy

In the island of inversion, ground states of neutron-rich sd-shell nuclei exhibit strong admixtures of intruder configurations from the fp shell. The nucleus 30 Mg, located at the boundary of the island of inversion, serves as a cornerstone to track the structural evolution as one approaches this region. Spin-parity assignments for excited states in 30 Mg, especially negative-parity levels, have yet to be established. In the present work, the nuclear structure of 30Mg was investigated by in-beam gamma-ray spectroscopy mainly focusing on firm spin-parity determinations. High-intensity rare-isotope beams of 31 Mg, 32 Mg, 34 Si, and 35 P bombarded a Be target to induce nucleon removal reactions populating states in 30 Mg. Gamma rays were detected by the state-of-the-art gamma-ray tracking array GRETINA. For the direct one-neutron removal reaction, final-state exclusive cross sections and parallel momentum distributions were deduced. Multi-nucleon removal reactions from different projectiles were exploited to gain complementary information. With the aid of the parallel momentum distributions, an updated level scheme with revised spin-parity assignments was constructed. Spectroscopic factors associated with each state were also deduced. Results were confronted with large-scale shell-model calculations using two different effective interactions, showing excellent agreement with the present level scheme. Furthermore, a marked difference in the spectroscopic factors indicates that the full delineation of the transition into the island of inversion remains a challenge for theoretical models.

20 ≤ A ≤ 38↗

Multiphase magnetism in Yb 2 Ti 2 O 7

We use neutron scattering to show that ferromagnetism and antiferromagnetism coexist in the low T state of the pyrochlore quantum magnet Yb 2 Ti 2 O 7 . While magnetic Bragg peaks evidence long-range static ferromagnetic order, inelastic scattering shows that short-range correlated antiferromagnetism is also present. Small-angle neutron scattering provides direct evidence for mesoscale magnetic structure that we associate with metastable antiferromagnetism. Classical Monte Carlo simulations based on exchange interactions inferred from ⟨ 111 ⟩ -oriented high-field spin wave measurements confirm that antiferromagnetism is metastable within the otherwise ferromagnetic ground state. The apparent lack of coherent spin wave excitations and strong sensitivity to quenched disorder characterizing Yb 2 Ti 2 O 7 is a consequence of this multiphase magnetism.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗