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At least 145 records · Page 8

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DOE OSTI2014

Theoretical predictions of properties and volatility of chlorides and oxychlorides of group-4 elements. II. Adsorption of tetrachlorides and oxydichlorides of Zr, Hf, and Rf on neutral and modified surfaces

With the aim to interpret results of gas-phase chromatography experiments on volatility of group-4 tetrachlorides and oxychlorides including those of Rf, adsorption enthalpies of these species on neutral, and modified quartz surfaces were estimated on the basis of relativistic, two-component Density Functional Theory calculations of MCl{sub 4}, MOCl{sub 2}, MCl{sub 6}{sup −}, and MOCl{sub 4}{sup 2} with the use of adsorption models. Several mechanisms of adsorption were considered. In the case of physisorption of MCl{sub 4}, the trend in the adsorption energy in the group should be Zr > Hf > Rf, so that the volatility should change in the opposite direction. The latter trend complies with the one in the sublimation enthalpies, ΔH{sub sub}, of the Zr and Hf tetrachlorides, i.e., Zr < Hf. On the basis of a correlation between these quantities, ΔH{sub sub}(RfCl{sub 4}) was predicted as 104.2 kJ/mol. The energy of physisorption of MOCl{sub 2} on quartz should increase in the group, Zr < Hf < Rf, as defined by increasing dipole moments of these molecules along the series. In the case of adsorption of MCl{sub 4} on quartz by chemical forces, formation of the MOCl{sub 2} or MOCl{sub 4}{sup 2−} complexes on the surface can take place, so that the sequence in the adsorption energy should be Zr > Hf > Rf, as defined by the complex formation energies. In the case of adsorption of MCl{sub 4} on a chlorinated quartz surface, formation of the MCl{sub 6}{sup 2−} surface complexes can occur, so that the trend in the adsorption strength should be Zr ≤ Hf < Rf. All the predicted sequences, showing a smooth change of the adsorption energy in the group, are in disagreement with the reversed trend Zr ≈ Rf < Hf, observed in the “one-atom-at-a-time” gas-phase chromatography experiments. Thus, currently no theoretical explanation can be found for the experimental observations.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗

DOE OSTI2016

Characterization of the CW starter plasma RF matching network for operating the SNS H{sup −} ion source with lower H{sub 2} flows

The Spallation Neutron Source H{sup −} ion source is operated with a pulsed 2-MHz RF (50-60 kW) to produce the 1-ms long, ∼50 mA H{sup −} beams at 60 Hz. A continuous low power (∼300 W) 13.56-MHz RF plasma, which is initially ignited with a H{sub 2} pressure bump, serves as starter plasma for the pulsed high power 2-MHz RF discharges. To reduce the risk of plasma outages at lower H{sub 2} flow rates which is desired for improved performance of the following radio frequency quadrupole, the 13.56-MHz RF matching network was characterized over a broad range of its two tuning capacitors. The H-α line intensity of the 13.56-MHz RF plasma and the reflected power of the 13.56-MHz RF were mapped against the capacitor settings. Optimal tunes for the maximum H-α intensity are consistent with the optimal tunes for minimum reflected power. Low limits of the H{sub 2} flow rate not causing plasma outages were explored within the range of the map. A tune region that allows lower H{sub 2} flow rate has been identified, which differs from the optimal tune for global minimum reflected power that was mostly used in the past.

46 INSTRUMENTATION RELATED TO NUCLEAR SCIENCE AND ↗

DOE OSTI2018

A single electron transistor charge sensor in strong rf fields

We measure the charge sensitivity, S e , of a single electron transistor (SET) in the presence of strong (V rf ~ e/C g ) spurious radio frequency (rf) signals at frequencies up to 50 MHz, where C g is the gate capacitance. Although S e appears to degrade when exposed to V rf , we find that broadening of conduction peaks is largely due to the measurement technique and show that S e is maintained even with strong V rf present. We show cancellation of a known V rf signal at 1 MHz, demonstrating that a stable bias point in the presence of rf signals is possible.

47 OTHER INSTRUMENTATION↗

DOE OSTI2018

Observation of multipath effects in the detection of RF-modulated x-rays

As part of the Air Force Research Laboratory’s ongoing research in particle accelerators and beams, we recently began investigating the interaction of RF-modulated x-ray beams with RF structures. Additionally, these bremsstrahlung x-rays, produced using an S-band RF electron linac and tungsten foil, were able to drive RF signals at the linac frequency and its integer harmonics in an S-band waveguide. This was interpreted as a result of secondary electron production inside the waveguide by the modulated x-ray beam and implied that the primary electron beam RF modulation was preserved, to at least some degree, through both the processes of x-ray and secondary electron production. The strength of these signals induced on the waveguide varied as the distance of the waveguide from the tungsten foil changed, with the nature of these changes suggesting the existence of an interference process resulting from multipath propagation of the modulated x-rays. Here, we report on our initial attempt to verify this multipath propagation by altering the configuration of shielding and reflective masses in the environment of the waveguide. Finally, these measurements support the existence of a multipath propagation effect and further indicate that the RF modulation of the x-rays is preserved as they undergo scattering events inside the accelerator vault.

43 PARTICLE ACCELERATORS↗

DOE OSTI2022

In situ detection of RF breakdown on microfabricated surface ion traps

We report microfabricated surface ion traps are a principal component of many ion-based quantum information science platforms. The operational parameters of these devices are pushed to the edge of their physical capabilities as the experiments strive for increasing performance. When the applied radio-frequency (RF) voltage is increased excessively, the devices can experience damaging electric discharge events known as RF breakdown. We introduce two novel techniques for in situ detection of RF breakdown, which we implemented while characterizing the breakdown threshold of surface ion traps produced at Sandia National Laboratories. In these traps, breakdown did not always occur immediately after increasing the RF voltage, but often minutes or even hours later. This result is surprising in the context of the suggested mechanisms for RF breakdown in vacuum. Additionally, the extent of visible damage caused by breakdown events increased with the applied voltage. To minimize the probability for damage when RF power is first applied to a device, our results strongly suggest that the voltage should be ramped up over the course of several hours and monitored for breakdown.

71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSIC↗

DOE OSTI2025

Integrated modeling of RF-induced tungsten erosion at ICRH antenna structures in the WEST tokamak *

This paper introduces STRIPE (Simulated Transport of RF Impurity Production and Emission), an advanced modeling framework developed to analyze material erosion and the global transport of eroded impurities originating from radio-frequency (RF) antenna structures in magnetic confinement fusion devices. STRIPE integrates multiple physics modules: SolEdge3x for scrape-off-layer plasma profiles, COMSOL for 3D RF rectified sheath potentials, RustBCA for erosion yields and surface interactions, and global impurity transport for 3D ion energy-angle distributions and impurity transport. The framework is applied to an ion cyclotron RF-heated L-mode discharge (#57877) in the WEST tokamak, where it predicts a thirty-fold increase in gross tungsten erosion at antenna limiters during the transition from ohmic to ICRH operation. Additionally, under ICRH conditions, a tenfold enhancement in erosion is observed when comparing RF sheath effects to purely thermal sheath conditions. High-charge-state oxygen ions ($\mathrm{O}$ 6+ and above) are identified as the dominant contributors to tungsten sputtering. To validate the model, a synthetic diagnostic tool based on inverse photon efficiency (S/XB coefficients) from the ColRadPy collisional-radiative model enables direct comparison with spectroscopic measurements. Model predictions using a plasma composition of 1% oxygen and 99% deuterium show good agreement with observed W − I (400.9 nm) emission for discharge #57877, supporting the accuracy of the STRIPE framework. This study focuses specifically on gross erosion calculations to demonstrate STRIPE’s capabilities. Future extensions of this work will incorporate net erosion, re-deposition, self-sputtering effects, and whole-device modeling of sputtered tungsten impurity transport. STRIPE is also being applied to other RF-heated linear and toroidal devices, offering valuable insights for antenna design, impurity control, and performance optimization in next-generation fusion reactors.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2024

H - Ion Source RF Plasma Testing with 13 MHz and 27 MHz at the Spallation Neutron Source (SNS)

The baseline RF-driven H⁻ ion source configuration at the Spallation Neutron Source (SNS) facility uses a continuous wave (CW) 600 W 13 MHz RF system to ignite and maintain a low-density plasma inside the ion source vacuum chamber. After the continuous low-density 13 MHz plasma has been established, a pulsed (typical 1 ms pulse width and 60 Hz pulse repetition rate) 80 kW 2 MHz RF system is used to increase the plasma density to produce the pulsed H⁻ ion beam. Incremental upgrades and improvements to the SNS ion source systems have resulted in the ability to reliably operate an H⁻ ion source for SNS neutron production run cycles that can last up to four months. Conditions inside the SNS H⁻ ion source evolve throughout a four-month run cycle due to changes in impurity levels, sputtering, and erosion. As the internal ion source conditions change during the run cycle, there can also be changes in plasma stability and the 13 MHz RF power level required to ignite the plasma. This paper presents the preliminary results of testing performed on the SNS Ion Source Test Stand (ISTS) system where we looked at plasma ignition and plasma stability using 27 MHz RF in place of the baseline 13 MHz RF system.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗

DOE OSTI2025

Coincident learning for beam-based rf station fault identification using phase information at the SLAC linac coherent light source

Anomalies in radio-frequency (rf) stations can result in unplanned downtime and performance degradation in linear accelerators such as SLAC’s Linac Coherent Light Source (LCLS). Detecting these anomalies is challenging due to the complexity of accelerator systems, high data volume, and scarcity of labeled fault data. Prior work identified faults using beam-based detection, combining rf amplitude and beam position monitor data. Due to the simplicity of the rf amplitude data, classical methods are sufficient to identify faults, but the recall is constrained by the low-frequency and asynchronous characteristics of the data. In this work, we leverage high-frequency, time-synchronous rf phase data to enhance anomaly detection in the LCLS accelerator. Due to the complexity of phase data, classical methods fail, and we instead train deep neural networks within the Coincident Anomaly Detection (CoAD) framework. We find that applying CoAD to phase data detects nearly 3 times as many anomalies as when applied to amplitude data, while achieving broader coverage across rf stations. Furthermore, the rich structure of phase data enables us to cluster anomalies into distinct physical categories. Through the integration of auxiliary system status bits, we link clusters to specific fault signatures, providing additional granularity for uncovering the root cause of faults. We also investigate interpretability via Shapley values, confirming that the learned models focus on the most informative regions of the data and providing insight for cases where the model makes mistakes. This work demonstrates that phase-based anomaly detection for rf stations improves both diagnostic coverage and root cause analysis in accelerator systems and that deep neural networks are essential for effective analysis.

Accelerator Physics (physics.acc-ph)↗

DOE OSTI2017

Peel-and-Stick Sensors Powered by Directed RF Energy

PARC, a Xerox Company, is developing a low-cost system of peel-and-stick wireless sensors that will enable widespread building environment sensor deployment with the potential to deliver up to 30% energy savings. The system is embodied by a set of RF hubs that provide power to automatically located sensor nodes, and relay data wirelessly to the building management system (BMS). The sensor nodes are flexible electronic labels powered by rectified RF energy transmitted by an RF hub and can contain multiple printed and conventional sensors. The system design overcomes limitations in wireless sensors related to power delivery, lifetime, and cost by eliminating batteries and photovoltaic devices. Sensor localization is performed automatically by the inclusion of a programmable multidirectional antenna array in the RF hub. Comparison of signal strengths while the RF beam is swept allows for sensor localization, reducing installation effort and enabling automatic recommissioning of sensors that have been relocated, overcoming a significant challenge in building operations. PARC has already demonstrated wireless power and temperature data transmission up to a distance of 20m with less than one minute between measurements, using power levels well within the FCC regulation limits in the 902-928 MHz ISM band. The sensor’s RF energy harvesting antenna achieves high performance with dimensions below 5cm x 9cm

Lalau-Keraly, Christopher↗

DOE OSTI2017

Miniaturized magnet-less RF electron trap. II. Experimental verification

Atomic microsystems have the potential of providing extremely accurate measurements of timing and acceleration. But, atomic microsystems require active maintenance of ultrahigh vacuum in order to have reasonable operating lifetimes and are particularly sensitive to magnetic fields that are used to trap electrons in traditional sputter ion pumps. Our paper presents an approach to trapping electrons without the use of magnetic fields, using radio frequency (RF) fields established between two perforated electrodes. The challenges associated with this magnet-less approach, as well as the miniaturization of the structure, are addressed. These include, for example, the transfer of large voltage (100–200 V) RF power to capacitive loads presented by the structure. The electron trapping module (ETM) described here uses eight electrode elements to confine and measure electrons injected by an electron beam, within an active trap volume of 0.7 cm 3 . The operating RF frequency is 143.6 MHz, which is the measured series resonant frequency between the two RF electrodes. It was found experimentally that the steady state electrode potentials on electrodes near the trap became more negative after applying a range of RF power levels (up to 0.15 W through the ETM), indicating electron densities of ≈3 × 10 5 cm -3 near the walls of the trap. The observed results align well with predicted electron densities from analytical and numerical models. The peak electron density within the trap is estimated as ~1000 times the electron density in the electron beam as it exits the electron gun. Finally, this successful demonstration of the RF electron trapping concept addresses critical challenges in the development of miniaturized magnet-less ion pumps.

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗

DOE OSTI2026

Python-EPICS RF Conditioning Automatic Control System at the Spallation Neutron Source

The RF Test Facility (RFTF) at the Spallation Neutron Source (SNS) is used for the conditioning of RF compo-nents such as ceramic vacuum windows and power cou-plers prior to their installation in the H- ion linear accel-erator. This process exposes components to high-power RF fields and thermal cycling to improve performance and remove surface impurities. To automate and optimize this process, a Python-based EPICS control system was developed alongside targeted hardware upgrades. The system enables real-time monitoring and control of RF power levels, temperature, and vacuum pressure. A user-friendly graphical interface was implemented using CS-Studio (Phoebus), allowing operators to adjust parameters and collect data efficiently. The system integrates a High-Power Protection Module (HPM) for interlocks based on vacuum and arc detection, ensuring safe operation. These upgrades have significantly improved the efficiency, accuracy, and safety of RF conditioning at the SNS RFTF. This paper describes the updated RF conditioning sys-tem, highlighting the software and hardware develop-ments and their application in support of the Proton Pow-er Upgrade (PPU) project.

Lee, Sung-Woo [ORNL] (ORCID:000000030915835X)↗

DOE OSTI2024

On Forced RF Generation of CW Magnetrons for SRF Accelerators

CW magnetrons, initially developed for industrial RF heaters, were suggested to power RF cavities of superconducting accelerators due to their higher efficiency and lower cost than traditionally used klystrons, IOTs or solid-state amplifiers. RF amplifiers driven by a master oscillator serve as coherent RF sources. CW magnetrons are regenerative RF generators with a huge regenerative gain. This causes regenerative instability with a large noise when a magnetron operates with the anode voltage above the threshold of self-excitation. Traditionally for stabilization of magnetrons is used injection locking by a quite small signal. Then the magnetron except the injection locked oscillations may generate noise. This may preclude use of standard CW magnetrons in some SRF accelerators. Recently we developed briefly described below a mode for forced RF generation of CW magnetrons when the magnetron startup is provided by the injected forcing signal and the regenerative noise is suppressed. The mode is most suitable for powering high Q-factor SRF cavities.

43 PARTICLE ACCELERATORS↗

DOE OSTI2012

EM modeling of RF drive in DTL tank 4: preliminary results

A 3-D MicroWave Studio model for the RF drive in the LANSCE DTL tank 4 has been built. Both eigensolver and time-domain modeling are used to evaluate maximal fields in the drive module and RF coupling. The LANSCE DTL tank 4 has recently been experiencing RF problems, which may or may not be related to its replaced RF coupler. This situation stimulated a request by Dan Rees to provide EM modeling of the RF drive in the DTL tank 4 (T4). Jim O'Hara provided a CAD model that was imported into the CST Microwave Studio (MWS) and after some modifications became a part of a simplified MWS model of the T4 RF drive. This technical note describes the model and presents simulation results.

43 PARTICLE ACCELERATORS↗

DOE OSTI2012

Novel Crab Cavity RF Design – Phase 1

The design and construction of electron-ion colliders, EIC, will be facilitated by the development of an SRF “crab crossing” cavity with 0.5 to 1.5 GHz frequency and 20 to 50 MV of total integrated voltage. The development of RF cavities that provide a transverse kick to the particle beam will include RF design, computer modeling, and hardware development. Current state of the art crab cavities provide 2- 5 MV of integrated voltage, and most of the existing designs require complex schemes to damp unwanted RF modes. We propose a novel design for TEM-like, room-temperature, two-bar structures, or hybrid structures with one resonant bar and one input coax per module, which can also be implemented for SRF conditions. Unwanted modes are coupled out of the cavity by the coax input line, and this provides a uniquely simple method to reduce the strength of higher-order modes. Critical phase stability for the crabbing voltage is provided by the low-level RF system, which controls the RF to the input ports of the novel crab cavity design. Designs for a series of cavities, or for multiple-module cavities, will provide the 20-50 MV of integrated voltage in an electron-ion collider, while meeting the critical thermal and mechanical requirements for heat loads, alignment, and phase stability. RF designs for various module alternatives were evaluated in Phase I. A single module of a hybrid design with one resonant bar and one coax input was built for room-temperature, low-power testing with a bead-pull measurement. Several additional designs were explored that made use of a high RT/Q, voltage-efficient, S-mode structure.

Neubauer, Michael↗

DOE OSTI2018

Summary of RF Technology Program Activities, October 2013 - September 2017

The goals of the National RF Research and Development Program (NRRDP) are to advance the basic understanding of high-power radio frequency (RF) in a plasma environment, and to maintain the high-power transmitters and cooling water systems required to support the ITER Ion Cylcotron Range of Frequencies (ICRF) transmission line high power component testing and operation of the Proto-Material Plasma Exposure eXperiment (MPEX) device. The work includes the study of the RF sheath, and development of RF-related diagnostics. These include active and passive spectroscopic diagnostics that can provide local and line integrated measurements of RF and Direct Current (DC) electric fields in the edge plasma of fusion devices, as well as measurements of other parameters. One of these, the Doppler Free Saturation Spectroscopy (DFSS) diagnostic, utilizes a laser beam split into two intersecting, counter-propagating pump and probe beams, whose intersection defines the measurement region. DFSS has demonstrated measurements of atomic spectra with 500 times greater resolution than passive Optical Emission Spectroscopy (OES). This allows Stark effect based electric field measurements to be made with two orders of magnitude high sensitivity than with OES. Measurements have been made using an ORNL electron-cyclotron resonant (ECR) plasma source producing densities up to 10 19 m -3 , in the vicinity of an RF-biased planar electrode.

47 OTHER INSTRUMENTATION↗

DOE OSTI2024

Low RF Loss DC Conductive Ceramic for High Power Input Coupler Windows for SRF Cavities

Euclid Techlabs, LLC is developing a low RF loss/DC conductive MgTi ceramics for high power input coupler windows for SRF cavities, under DOE SBIR phase II grant DE-SC0017150. JLab was subcontracted to: fabricate two 500 kW capable pre-stressed coaxial windows; provide an RF testing fixture, and test the window with low power and high power RF. This collaboration helped to develop a better material for high power RF windows, with low RF loss and less prone to arcing, with the potential to improve the state of the art high power RF window performance.

36 MATERIALS SCIENCE↗

DOE OSTI2026

Correlating Surface Processing of Nb Superconducting RF Cavities with the Evolution of Surface Electronic States

Superconducting-radio frequency (RF) cavities provide an efficient way to accelerate particle beams with extremely high acceleration gradients while generating very small power dissipation. The few nanometers of the surface play a critical role in defining the RF performance of superconducting Nb based cavities. Over the past two decades, several pioneering surface treatment and processing methods have emerged, enabling remarkable improvements in superconducting cavity performance by simultaneously achieving high quality factors with increasing maximum acceleration gradients. These processing approaches include chemical polishing, distinct multi-step thermal treatments under ultra-high vacuum (UHV) conditions over low to high temperature regimes, as well as high-temperature treatments under controlled nitrogen atmospheres. Beyond their macroscopic impact on RF performance, these methods produce distinct surface oxide configurations characterized by different valence states, oxide thicknesses, chemical uniformity, and oxygen concentration profiles extending into the near-surface bulk of niobium. In this work, we are trying to understand how the surface-processing methods and the resulting oxide/oxygen profiles affect the electronic structure of surface and the mechanism of superconductivity. Using a combination of X-ray photoemission and X-ray absorption spectroscopies, we investigate how the valence-band structure and the electronic density of states (DoS) near the Fermi level evolve under different surface treatments. By employing tunable photon energies across multiple elemental absorption edges, we use resonant photoemission to disentangle and identify the elemental contributions to specific valence-band features. Our observations show that different surface-processing methods lead to distinct temperature evolutions of the DoS and valence-band states near the Fermi level. Our results suggest variations in different Nb-O orbital hybridizations in distinct processes and point towards the possibility of different underlying mechanisms of superconductivity governed by surface chemistry and oxide configuration. We also correlate these distinct superconducting mechanisms with RF cavity performance, specifically focusing on measured surface resistance, the nature of the Q-slope, and quench fields observed in superconducting RF measurements. These results will enable us to identify the potential limiting factors and relevant controllable parameters that can be further optimized to improve the performance of superconducting RF cavities.

Tripathi, Malvika [Fermilab] (ORCID:00000001989251↗

DOE OSTI2019

RF beam scattering by cylindrical filaments and interfacial density fluctuations

Radio Frequency (RF) waves are routinely used in tokamaks for heating, current drive, NTM control, as well as for diagnostics purposes. Frequently, RF waves, aiming towards the plasma core, propagate through a turbulent environment. The latter can exhibit strong coherent density fluctuations as well as filamentary structures mainly (though, not perfectly) aligned along the local magnetic field lines. The scattering process of RF waves by these structures is studied both analytically and numerically. RF waves can be either single plane waves or spatially confined beams. For that purpose, the filaments are considered to have cylindrical shape with infinite length with the cylinder axis not aligned with the local magnetic field and the results are compared to the ones from the study of the aligned case. On the other hand, the interfacial density fluctuations are considered periodic with spatial periods larger, smaller or of the same order of the wavelength of the incident RF waves. The frequency range of the RF waves studied is mainly in the Electron Cyclotron (EC) range of frequencies for ITER-like and Medium Size Tokamak applications. Furthermore, the study covers a variety of density contrasts, filament sizes and fluctuation strengths.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗