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At least 145 records · Page 8

Relating Satellite-Based Contrail Detection to NWA Output

Contrail-induced cloud cover has been shown to be a significant factor in regional climate change over the United States of America. As air traffic increases, the potential for globally significant impacts also rises. To better understand and predict these potential climatic effects, it is necessary to develop models that can accurately represent contrail properties based on ambient atmospheric variables including temperature, relative humidity and winds. Several high-resolution numerical weather analyses (NWA) including the 20-km Rapid Update Cycle (RUC) and the University of Oklahoma Center for Analysis and Prediction of Storms Advanced Regional Prediction System (ARPS) can provide the temperature, humidity and wind information necessary to diagnose contrail formation. One outstanding problem that must be addressed to achieve a realistic simulation of contrails is the large uncertainties in upper tropospheric relative humidity (UTH) in numerical weather analyses. Current numerical weather analyses tend to underestimate UTH due to large dry biases in the balloon soundings used to construct the analyses. To evaluate each of the models, we match several months of contrail properties derived from satellite and surface observations to the NWA-derived humidity, vertical velocity, wind shear and atmospheric stability. The relationships between several contrail properties (including optical depth and areal contrail coverage) and the NWA-derived statistics will be analyzed to determine under which atmospheric conditions widespread contrail outbreaks are favored.

Duda, David P.↗

Patterns in the sky: Natural visualization of aircraft flow fields

The objective of the current publication is to present the collection of flight photographs to illustrate the types of flow patterns that were visualized and to present qualitative correlations with computational and wind tunnel results. Initially in section 2, the condensation process is discussed, including a review of relative humidity, vapor pressure, and factors which determine the presence of visible condensate. Next, outputs from computer code calculations are postprocessed by using water-vapor relationships to determine if computed values of relative humidity in the local flow field correlate with the qualitative features of the in-flight condensation patterns. The photographs are then presented in section 3 by flow type and subsequently in section 4 by aircraft type to demonstrate the variety of condensed flow fields that was visualized for a wide range of aircraft and flight maneuvers.

Campbell, James F.↗

Dependence of tropospheric temperature on the parameterization of cumulus convection in the GLAS model of the general circulation

Analysis of the simulation of seasonal change by the GLAS model of the general circulation reveals deficiencies in the simulation of tropospheric temperature and of convective cloud cover. These interrelated deficiencies are due to a spurious doubling from January to July in the convective cloud cover of the Northern Hemisphere. The spurious doubling, in turn, is due to the oversensitivity of cumulus convection, in the GLAS model, to the specific humidity of the lower atmosphere. The oversensitivity is enhanced by a feedback mechanism which perpetuates the existence of deep, penetrative convective clouds at certain preferred locations. The cumulus parameterization scheme has been modified to more realistically relate the onset of cumulus convection to the relative humidity of the lower atmosphere. The modified parameterization has improved the simulation of tropospheric temperature, planetary albedo and convective cloud cover as well as their seasonal variations. Comparison of this experiment with its control has shown a high degree of interrelation among these fields in the GLAS model and has demonstrated the sensitivity of the atmospheric heat budget to the design of the cumulus parameterization scheme. Also, the modification to the cumulus scheme has demonstrated a plausible mechanism to explain the correlation between convective cloud cover and relative humidity in the real atmosphere.

Helfand, H. M.↗

Operational Assimilation of GOES Data into a Mesoscale Model

A technique has been developed for assimilating GOES-derived skin temperature tendencies and insolation into the surface energy budget equation of a mesoscale model so that the simulated rate of temperature change closely agrees with the satellite observations. A critical assumption of the technique is that the availability of moisture (either from the soil or vegetation) is the least known term in the model's surface energy budget. Therefore, the simulated latent heat flux, which is a function of surface moisture availability, is adjusted based upon differences between the modeled and satellite- observed skin temperature tendencies. An advantage of this technique is that satellite temperature tendencies are assimilated in an energetically consistent manner that avoids energy imbalances and surface stability problems that arise from direct assimilation of surface shelter temperatures. The fact that the rate of change of the satellite skin temperature is used rather than the absolute temperature means that sensor calibration is not as critical. The technique has been employed on a semi-operational basis at the Global Hydrology and Climate Center (GHCC) within the Penn State/National Center for Atmospheric Research (PSU/NCAR) Mesoscale Model (MM5) since 1 November 1998. We performed the assimilation on a model grid centered over the Southeastern US. In addition, a control run without assimilation was performed to provide insight into the performance of the assimilation technique. Bulk verification statistics (BIAS and RMSE) of surface air temperature and relative humidity of more than 250 case days has been performed to date. Results show that assimilation of the satellite data results reduces both the bias and RMSE for simulations of surface air temperature and relative humidity. We are working with forecasters at the National Weather Service Forecast Office located in Birmingham, AL to evaluate the impact of the assimilation on precipitation forecasts. In addition, work is currently underway to determine the ability of both the assimilation technique and Early Eta to sense the significant changes that occur in both leaf expansion and soil moisture conditions during the Spring-Summer of 1999. This will be accomplished via examination of the simulated surface energy budgets from both modeling systems.

Lapenta, William↗

Nighttime Cirrus Detection using Atmospheric Infrared Sounder Window Channels and Total Column Water Vapor

A method of cirrus detection at nighttime is presented that utilizes 3.8 and 10.4 (micro)m infrared (IR) window brightness temperature differences (dBT) and total column precipitable water (PW) measurements. This technique is applied to the Atmospheric Infrared Sounder (AIRS) and Advanced Microwave Sounding Unit A (AMSU-A) instrument suite on board EOS-Aqua, where dBT is determined from sets of carefully selected AIRS window channels, while PW is derived from the synergistic AIRS and AMSU-A water vapor retrievals. Simulated and observed dBT for a particular value of PW are not constant; several physical factors impact dBT, including the variability in temperature and relative humidity profiles, surface emissivity, instrument noise, and skin/ near-surface air temperature differences. We simulate clear-sky dBT over a realistic range of PWs using 8350 radiosondes that have varying temperature and relative humidity profiles. Thresholds between cloudy and uncertain sky conditions are derived once the scatter in the clear-sky dBT is determined. Simulations of optically thin cirrus indicate that this technique is most sensitive to cirrus optical depth in the 10 (micro)m window of 0.1-0.15 or greater over the tropical and subtropical oceans, where surface emissivity and skin/near-surface air temperature impacts on the IR radiances are minimal. The method at present is generally valid over oceanic regions only, specifically, the tropics and subtropics. The detection of thin cirrus, and other cloud types, is validated using observations at the Atmospheric Radiation Measurement (ARM) program site located at Manus Island in the tropical western Pacific for 89 coincident EOS-Aqua overpasses. Even though the emphasis of this work is on the detection of thin cirrus at nighttime, this technique is sensitive to a broad cloud morphology. The cloud detection technique agrees with ARM-detected clouds 82-84% of the time, which include thin cirrus, as well as other cloud types. Most of the disagreements are well explained by AIRS footprint-scale heterogeneity compared to ARM point measurements, cirrus overlying lower-layer water clouds, possible mixed phase microphysics in midlevel clouds, and significant IR channel noise for cold BT scenes over deep convective towers.

Atmospheric Radiation Measurement (RAM)↗

Evaluation of cloudiness parameterizations using a cumulus ensemble model

Diagnostic cloudiness parameterizations in large-scale models are evaluated by using a two-dimensional numerical cumulus ensemble model. The model covers a large horizontal domain (512 km) but resolves individual clouds. This study explores the dependence of diagnostic relations (between cloud amount and a large-scale variable) on cloud regime, horizontal averaging distance, and cloud type for tropical convective cloud regimes. Large-scale variables, including relative humidity, cumulus mass flux, large-scale vertical velocity and surface precipitation rate, are examined. It is shown that the total cloud amount can be better estimated as the sum of separate estimates of stratiform and convective cloud amounts using different large-scale variables than by an estimate of the total cloud amount using any single large-scale variable. The stratiform cloud amount can best be estimated by using relative humidity. The convective cloud amount can be diagnosed by using cumulus mass flux. Neither set of diagnostic relations depends significantly on the stimulated cloud regime or horizontal averaging distance, but other diagnostic relations do show some such dependence. These results are interpreted and their implications for cloudiness parameterization are discussed.

Xu, Kuan-Man↗

Absorption of sound in air - High-frequency measurements

The absorption of sound in air at frequencies from 4 to 100 kHz in 1/12 octave intervals, for temperatures from 255.4 K (0 F) to 310.9 K (100 F) in 5.5 K (10 F) intervals, and at 10% relative-humidity increments between 0% and saturation has been measured. The values of free-field absorption have been analyzed to determine the relaxation frequency of oxygen for each of the 92 combinations of temperature and relative humidity studied and the results are compared to an empirical expression. The relaxation frequencies of oxygen have been analyzed to determine the microscopic energy-transfer rates.

Bass, H. E.↗

Airborne High Spectral Resolution Lidar-2 Measurements of Enhanced Depolarization in Marine Aerosols

Airborne NASA Langley Research Center (LaRC) High Spectral Resolution Lidar-2 (HSRL-2) measurements acquired during the recent NASA EVS-3 Aerosol Cloud Meteorology Interactions over the Western Atlantic Experiment (ACTIVATE) revealed enhanced particulate linear depolarization associated with aerosols within the marine boundary layer. These HSRL-2 observations were acquired off the east coast of the United States in February and March 2020 when this lidar was deployed on the NASA LaRC UC-12 aircraft. HSRL-2 measured profiles of aerosol backscattering, extinction,and depolarization at 355 and 532nm and aerosol backscattering and depolarization at 1064nm. Typically HSRL-2 measures low (<5%) linear particulate depolarization associated with marine sea salt aerosols. However, during several ACTIVATE flights, particularly those that occurred with outbreaks of cold, dry air, linear particulate depolarization exceeded 15-20% (532nm) for aerosols within a few hundred meters above the surface. These high values indicated that these particles were nonspherical. Elevated depolarization values were also observed at 355 and 1064 nm. HSRL-2 measured aerosol extinction/backscatter ratio (“lidar ratio”) values around 20-25 sr (355 and 532 nm) that are typically associated with sea salt particles. Coincident measurements of relative humidity from dropsondes released from the UC-12and in situ Diode Laser Hygrometer (DLH) measurements flown on the NASA HU-25 aircraft showed that highest depolarization values of these nonspherical particles were found when the relative humidity (RH)was below 50-60%.These lidar observations of elevated depolarization associated with sea salt aerosol are consistent with previous lidar measurements of sea salt aerosols in dry conditions. We discuss these HSRL-2 measurements also in the context of coincident airborne in situ measurements of particle size and composition acquired on the HU-25 aircraft. We also found that CALIOP satellite measurements observed elevated depolarization during some similar cold air outbreaks. In such cases, the operational CALIOP algorithms attributed the elevated depolarization to nonspherical dust particles rather than the more likely scenario of nonspherical sea salt particles associated with low RH.

aerosols↗

The washout of combustion-generated hydrogen chloride

The coefficient for the washout from a rocket exhaust cloud of HCl generated by the combustion of an ammonium perchlorate-based solid rocket propellant such as that to be used for the Space Shuttle Booster is determined. A mathematical model of HCl scavenging by rain is developed taking into account rain droplet size, fall velocity and concentration under various rain conditions, partitioning of exhaust HCl between liquid and gaseous phases, the tendency of HCl to promote water vapor condensation and the concentration and size of droplets within the exhaust cloud. The washout coefficient is calculated as a function of total cloud water content, total HCl content at 100% relative humidity, condensation nuclei concentration and rain intensity. The model predictions are compared with experimental results obtained in scavenging tests with solid rocket exhaust and raindrops of different sizes, and the large reduction in washout coefficient at high relative humidities predicted by the model is not observed. A washout coefficient equal to 0.0000512 times the -0.176 power of the mass concentration of HCl times the 0.773 power of the rainfall intensity is obtained from the experimental data.

Fenton, D. L.↗

Observation of hydration of single, modified carbon aerosols

We have compared the hydration behavior of single carbon particles that have been treated by exposure to gaseous H2SO4 with that of untreated particles. Untreated carbon particles did not hydrate as the relative humidity varied from 0 to 80% at 23 C. In contrast, treated particles hydrated under subsaturation conditions; mass increases of up to 30% were observed. The mass increase is consistent with sulfuric acid equilibration with the ambient relative humidity in the presence of inert carbon. For the samples studied, the average amount of absorbed acid was 14% +/- 6% by weight, which corresponds to a surface coverage of approximately 0.1 monolayer. The mass fraction of surface-absorbed acid is comparable to the soluble mass fraction observed by Whitefield et al. (1993) in jet aircraft engine aerosols. Estimates indicate this mass fraction corresponds to 0.1% of the available SO2 exiting an aircraft engine ending up as H2SO4 on the carbon aerosol. If this heterogeneous process occurs early enough in the exhaust plume, it may compete with homogeneous nucleation as a mechanism for producing sulfuric acid rich aerosols.

Wyslouzil, B. E.↗

Utilization of Airborne Observations to Assess Model Parametrizations of Critical RH Profiles in the Arctic Ocean

Observational paucity is a reality in the Arctic Ocean. This is especially true for near-surface variables such as temperature, moisture, heat fluxes and BL clouds. As a result, modeling has become one of the major avenues for understanding current and future Arctic trends. Reanalyses are frequently used to force global ocean circulation and sea-ice models. But in northern high latitudes, model integrations and reanalyses are known to have large uncertainties in temperature and humidity profiles, and in boundary layer cloudiness. These are common sources of error in the surface radiative budget terms.An important way to diagnose these biases spatially and temporally is by using satellite remote sensing data. However, remotely-sensed observations also have large uncertainties, especially in near-surface temperature and relative humidity profiles.In situ observational studies are important in bridging our knowledge gap in regions such as the Arctic Ocean. Here, we utilize airborne and ship observations from the ARISE, ACME-IV, and ASCOS campaigns to construct critical relative humidity (RH) profiles over the Beaufort Sea. Such profiles are used as parameterization inputs in the NASA GOES global model to derive the total water condensate in a model grid-box, which determines the cloud fraction. Currently, the critical RH profiles are derived by global AIRS data, relaying mostly on mid-latitude regions, which are not necessarily relevant to the Arctic.We derive campaign-wide mean, standard deviation, and critical RH values, for grid size of 50x50 km and altitude bins between 50 to 400 m, covering both open-ocean and sea-ice covered regions. We compare profiles over open ocean and sea-ice, and look at correlations between the observed critical RH values and water condensate (by cloud number concentration) from observations versus the modeled ones. We then input our calculated values of minimal critical RH values into a set of GEOS single column model (SCM) simulations over the ARISE and ASCOS regions and compare the differences between the predicted values of cloud liquid water path (LWP), ice water path (IWP) and surface fluxes with the observed ones under the range of input parameterizations. Finally, we discuss the implications on surface radiative budget predictions in this region.

Segal-Rozenhaimer, Michal↗

Observation of airplane flow fields by natural condensation effects

In-flight condensation patterns can illustrate a variety of airplane flow fields, such as attached and separated flows, vortex flows, and expansion and shock waves. These patterns are a unique source of flow visualization that has not been utilized previously. Condensation patterns at full-scale Reynolds number can provide useful information for researchers experimenting in subscale tunnels. It is also shown that computed values of relative humidity in the local flow field provide an inexpensive way to analyze the qualitative features of the condensation pattern, although a more complete theoretical modeling is necessary to obtain details of the condensation process. Furthermore, the analysis revealed that relative humidity is more sensitive to changes in local static temperature than to changes in pressure.

Campbell, James F.↗

Evaluation of Global Fire Weather Database Reanalysis and Short-Term Forecast Products

Daily Fire Weather Index (FWI) System components calculated from the NASA Modern-Era Retrospective analysis for Research and Applications, Version 2 (MERRA-2), are compared to FWI calculations from a global network of weather stations over 2004–2018, and short-term, experimental (8 d) daily FWI forecasts are evaluated for their skill across the Terrestrial Ecoregions of the World for 2018. FWI components from MERRA-2 were, in general, biased low compared to station data, but this reflects a mix of coherent low and high biases of different magnitudes. Biases in different MERRA-2 FWI components were related to different biases in weather input variables for different regions, but temperature and relative humidity biases were the most important overall. FWI forecasts had high skill for 1–2 d lead times for most of the world. For longer lead times, forecast skill decreased most quickly at high latitudes and was most closely related to decreasing skill of relative humidity forecasts. These results provide a baseline for the evaluation and use of fire weather products calculated from global analysis and forecast fields.

Global Fire Weather Database↗

Evaluation of Different MODIS AOD Retrieval Algorithms for PM (sub 2.5) Estimation in the Western, Midwestern and Southeastern United States with Implications for Public Health

This study was part of the research activities of the Center for Applied Atmospheric Research and Education (CAARE) funded by the NASA MUREP (Minority University Research and Education Project) Institutional Research Opportunity (MIRO) Program. Satellite measurements of Aerosol Optical Depth (AOD) have been shown to be correlated with ground measurements of fine particulate matter less than 2.5 microns PM (sub 2.5), which in turn has been linked to respiratory and heart diseases. The strength of the correlation between AOD and PM (sub 2.5) varies for different AOD retrieval algorithms and geographic regions. We evaluated several Moderate Resolution Imaging Spectrometer (MODIS) AOD products from different satellites (Aqua vs. Terra), retrieval algorithms (Dark Target versus Deep Blue), Collections (5.1 versus 6) and spatial resolutions (10-kilometers versus 3-kilometers) for cities in the Western, Midwestern and Southeastern U.S. We developed and validated PM (sub 2.5) prediction models using remotely-sensed AOD data, which were improved by incorporating meteorological variables (temperature, relative humidity, precipitation, wind speed, and wind direction) from the North American Land Data Assimilation System Phase 2 (NLDAS-2). Adding these meteorological data significantly improved the predictive power of all the PM (sub 2.5) models, especially in the Western U.S. Temperature, relative humidity and wind speed were the most significant meteorological variables throughout the year in the Western U.S. Wind speed was the most significant meteorological variable for the cold season while temperature was the most significant variable for the warm season in the Midwestern and Southeastern U.S. Our study re-establishes the connection between PM (sub 2.5) and public health concerns including respiratory and cardiovascular diseases (asthma, high blood pressure, coronary heart disease, heart attack, and stroke). Using PM (sub 2.5) data and health data from the Centers for Disease Control and Prevention (CDC)'s Behavioral Risk Factor Surveillance System (BRFSS), our statistical analysis showed that heart attack and stroke occurrences had the strongest correlations with PM (sub 2.5).

Environmental Public Health↗

Vermont Wildland Fires: Investigating the Role of Antecedent Conditions and Recent Environmental Trends in Exacerbating Fire Risk and Potential in Vermont

Under a changing climate, increases in dry conditions and extreme heat events are projected to exacerbate wildfire risk in the northeastern U.S. In recent years, Vermont has observed higher annual temperatures, more frequent heatwaves, increased annual precipitation, extreme flood events, and decreased snowfall. The mechanisms through which environmental factors contribute to increased fire risk in humid environments, such as Vermont, are poorly understood. The team partnered with the National Weather Service, the Vermont Division of Forests, and the University of Vermont to investigate phenological trends and antecedent conditions influencing wildland fire risk. For the phenological analysis, from 2001 to 2023, vegetation data, phenological dates, and snow water equivalent (SWE) values were accessed from Landsat 5Thematic Mapper (TM), Landsat 7Enhanced Thematic Mapper Plus (ETM+), Landsat 8Operational Land Imager (OLI), Landsat 9OLI-2, the Moderate Resolution Imaging Spectroradiometer (MODIS), and the Snow Data Assimilation System (SNODAS), respectively. For the antecedent condition analysis, from 2008 to 2023, soil moisture, Environmental Stress Index, wind speed, minimum relative humidity, and daily precipitation data were obtained from the Global Land Data Assimilation System (GLDAS), SERVIR, gridMET Wind, gridMET Humidity, and NClimGrid, respectively. The study found that green-up dates over the study period remain relatively stable, while snowmelt dates appear increasingly variable. Minimum relative humidity was the most significant environmental variable correlated with wildfire risk in Vermont. Results from this study will inform the National Weather Service's preparation of fire forecasts before prescribed burns and support community outreach by the Vermont Agency of Natural Resources.

Wildland Fire↗

Small Particle Glovebox Experiments - Preliminary Results

A substantial portion of the asteroid samples returned by the HAYABUSA2 and OSIRIS-REx missions will consist of small (submm) components (due to the collection of those particles on the asteroid surface and due to the fragmenting of larger, friable material post-collection). In order to minimize the alteration/oxidation of asteroid regolith, the bulk collections will be stored and curated in nitrogen purged gloveboxes. The processing of small particles in an N2 glovebox will present challenges that are different from those experienced during lunar and meteorite sample processing. Particles in this size range are susceptible to unpredictable electrostatic charging that can result in sample loss during processing operations. Methods for the handling of sub-mm particles have been well developed for environments with ambient atmospheric conditions and relative humidity (RH) ranges between 40-70%. In such conditions, a number of factors can be successfully employed to minimize the effects of triboelectric charging, including the use of Po-210 sources that neutralize excess charge and the utilization of conductive manipulation tools and sample substrates. However, relative humidity levels above 40% also contribute significantly to dissipation of triboelectric effects. We had not previously investigated our charge mitigation methods in a completely dry, nitrogen-purged environment, or whether they would be sufficient in enabling the successful processing of sub-mm samples. Current glovebox configurations in use in our lunar and meteorite curation laboratories are optimized for the processing of macroscopic samples and tools; these glovebox designs are likely unsuitable for the processing of collections for which the bulk collection is comprised of sub-mm components. Small particle sample preparation requires the use of an optical magnification instrument – typically a stereo binocular microscope with at least 20x magnification. Current glovebox designs are not optimized for the utilization or integration of stereo microscopes; while many current cabinets include microscope viewports that enable the use of small, externally mounted stereo microscopes, the focusing methods (usually involving the use of a lab jack) lack the fidelity and precision required for small particle manipulation and imaging. Working distances of higher (>50x magnification) objective lenses may preclude the external use of a stereo microscope through a viewport; in order to successfully manipulate and image very small (< 20m) particles, stereo and digital microscope systems that are integrated within the glovebox should be investigated. Finally, ergonomic considerations for small particle work within a glovebox must be considered to minimize risk of injury to sample processors. In order to investigate some of the unknown parameters relating to small particle processing within an N2 glovebox, we conducted preliminary, qualitative experiments utilizing a small lunar cabinet that was originally used for film development.

C. J. Snead↗

Certification of Upper Air Sounding System to Support NASA Launch Operations

A new upper air sounding system (Vaisala MW51) has been installed at the United States Space Force’s Eastern Range (ER). The NASA Marshall Space Flight Center’s Natural Environments Branch has assessed MW51 test data from the ER to certify the new system for use in Artemis Program launch operations. Certification criteria are based on legacy system capabilities and vehicle design environments, and include criteria for wind, temperature, and relative humidity, as well as effective vertical resolution (EVR) of wind data. The test data consists of near simultaneous (within 15 seconds) releases of two MW51 sondes and one legacy system sonde. Difference statistics (root mean square) between MW51 and legacy system wind, temperature, and relative humidity data are assessed against the certification criteria. Wind data from dual MW51 releases are used in spectral/coherence analyses to assess the EVR criteria. The MW51 system must demonstrate it meets these criteria to be used in NASA Artemis launch operations.

Frank Leahy↗

Cirrus cloud model parameterizations: Incorporating realistic ice particle generation

Recent cirrus cloud modeling studies have involved the application of a time-dependent, two dimensional Eulerian model, with generalized cloud microphysical parameterizations drawn from experimental findings. For computing the ice versus vapor phase changes, the ice mass content is linked to the maintenance of a relative humidity with respect to ice (RHI) of 105 percent; ice growth occurs both with regard to the introduction of new particles and the growth of existing particles. In a simplified cloud model designed to investigate the basic role of various physical processes in the growth and maintenance of cirrus clouds, these parametric relations are justifiable. In comparison, the one dimensional cloud microphysical model recently applied to evaluating the nucleation and growth of ice crystals in cirrus clouds explicitly treated populations of haze and cloud droplets, and ice crystals. Although these two modeling approaches are clearly incompatible, the goal of the present numerical study is to develop a parametric treatment of new ice particle generation, on the basis of detailed microphysical model findings, for incorporation into improved cirrus growth models. For example, the relation between temperature and the relative humidity required to generate ice crystals from ammonium sulfate haze droplets, whose probability of freezing through the homogeneous nucleation mode are a combined function of time and droplet molality, volume, and temperature. As an example of this approach, the results of cloud microphysical simulations are presented showing the rather narrow domain in the temperature/humidity field where new ice crystals can be generated. The microphysical simulations point out the need for detailed CCN studies at cirrus altitudes and haze droplet measurements within cirrus clouds, but also suggest that a relatively simple treatment of ice particle generation, which includes cloud chemistry, can be incorporated into cirrus cloud growth.

Sassen, Kenneth↗