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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 145 records · Page 8
All sourcesNASA NTRSDOE OSTI
DOE OSTI2020

An analysis of carrier dynamics in methylammonium lead triiodide perovskite solar cells using cross correlation noise spectroscopy

Using cross correlation current noise spectroscopy, we have investigated carrier dynamics in methylammonium lead triiodide solar cells. This method provides space selectivity for devices with a planar multi-layered structure, effectively amplifying current noise contributions coming from the most resistive element of the stack. In the studied solar cells, we observe near full-scale shot noise, indicating the dominance of noise generation by a single source, likely the interface between the perovskite and the spiro-organic 2,2',7,7'-tetrakis(N,N-di-p-methoxyphenyl-amine)9,9'-spirobifluorene hole-transport layer. In this paper, we argue that the strong 1/f noise term has contributions from both the perovskite layer and interfaces. It displays a non-ideal dependence on photocurrent, S $\propto$ I 1.4 (instead of usual S $\propto$ I 2 ), which is likely due to current-induced halide migration. Finally, we observe generation–recombination noise. We argue that this contribution is due to bimolecular recombination in the perovskite bulk absorption layer. Extrapolating our results, we estimate that at standard 1 sun illumination, the electron–hole recombination time is 5 microseconds.

14 SOLAR ENERGY↗
DOE OSTI2020

Ultrafast x-ray and electron scattering of free molecules: A comparative evaluation

Resolving gas phase molecular motions with simultaneous spatial and temporal resolution is rapidly coming within the reach of x-ray Free Electron Lasers (XFELs) and Mega-electron-Volt (MeV) electron beams. These two methods enable scattering experiments that have yielded fascinating new results, and while both are important methods for determining transient molecular structures in photochemical reactions, it is important to understand their relative merits. In the present study, we evaluate the respective scattering cross sections of the two methods and simulate their ability to determine excited state molecular structures in light of currently existing XFEL and MeV source parameters. Using the example of optically excited N-methyl morpholine and simulating the scattering patterns with shot noise, we find that the currently achievable signals are superior with x-ray scattering for equal samples and on a per-shot basis and that x-ray scattering requires fewer detected signal counts for an equal fidelity structure determination. Importantly, within the independent atom model, excellent structure determinations can be achieved for scattering vectors only to about 5 Å−1, leaving larger scattering vector ranges for investigating vibrational motions and wavepackets. Electron scattering has a comparatively higher sensitivity toward hydrogen atoms, which may point to applications where electron scattering is inherently the preferred choice, provided that excellent signals can be achieved at large scattering angles that are currently difficult to access.

74 ATOMIC AND MOLECULAR PHYSICS↗
NASA NTRS1991

Squeezed photon-number noise and sub-Poissonian electrical partition noise in a semiconductor laser

Amplitude noise on the light from a semiconductor laser produced a photocurrent fluctuation spectrum that was a maximum of 85 percent (-8.3 dB) below the shot-noise limit. Squeezing in semiconductor lasers is not limited by the overall quantum, or current transfer, efficiency from the laser injection current to the detector photocurrent. Current leakage away from the lasing junction does not introduce Poissonian partition noise.

Richardson, W. H.↗
DOE OSTI2025

Signatures of linearized gravity in atom interferometers: A simplified computational framework

We develop a general framework for calculating the leading-order, general relativistic contributions to the gravitational phase shift in single-photon atom interferometers within the context of linearized gravity. We show that the atom gradiometer observable, which only depends on the atom interferometer propagation phase, can be written in terms of three distinct contributions: the Doppler phase shift, which accounts for the tidal displacement of atoms along the baseline, the Shapiro phase shift, which accounts for the delay in the arrival time of photons at atom-light interaction points, and the Einstein phase shift, which accounts for the gravitational redshift measured by the atoms. For specific atom gradiometer configurations, we derive the signal and response functions for two physically motivated scenarios: (i) transient gravitational waves in the transverse-traceless gauge and, for the first time, in the proper detector frame, and (ii) transient massive objects sourcing weak and slow-varying Newtonian potentials. Here, we find that the Doppler contribution of realistic Newtonian noise sources (e.g., a freight truck or a piece of space debris) at proposed atom gradiometer experiments, such as AION, MAGIS, and AEDGE, can exceed the shot noise level and thus affect physics searches if not properly subtracted. Note: 44 pages including appendices, 4 figures; v2: different formatting, fixed typos, 28 pages including appendices, 5 figures, agrees with published version

Atom interferometry↗
DOE OSTI2024

Quantum limits of superconducting-photonic links and their extension to millimeter waves

Photonic addressing of superconducting circuits has been proposed to overcome wiring complexity and heat-load challenges. However, such superconducting-photonic links suffer from an efficiency-noise trade-off that limits scalability. This trade-off arises because increasing power conversion efficiency entails reducing optical power, which makes the converted signal susceptible to shot noise. We analyze this trade-off and find that the laser-driven qubit gate infidelity scales inversely with the number of photons used. While methods such as nonlinear detection or squeezed light could mitigate this effect, we consider generating higher-frequency electrical signals, such as millimeter waves (100 GHz), using laser light. At these higher frequencies, circuits have higher operating temperatures and cooling power budgets and alleviate constraints posed by the trade-off. Therefore, we demonstrate an optically driven cryogenic millimeter-wave source with a maximum power efficiency of 8 ×10 −5 that can generate a maximum of 0.7 μ⁢W of 80 GHz power, with a 1200-thermal-photon equivalent of added noise at 4K. Using this source, we perform frequency-domain spectroscopy of superconducting NbTiN resonators at 80–90 GHz. Our results show a promising approach to lessen the efficiency-noise constraints on superconducting-photonic links, while leveraging the benefits of photonic signal delivery. Further optimization of power efficiency and noise at high frequencies could make scalable photonic control of superconducting qubits viable at temperatures exceeding 1K.

Optoelectronics↗
NASA NTRS1975

Long-term X-ray studies of Sco X-1

No modulation of the 3-6 keV X-ray intensity of Sco X-1 at a level of excess of 1% was observed at the optical period of .787313d. Evidence is found for shot-noise character in a large fraction of the X-ray emission. Almost all of the Sco X-1 emission can be synthesized in terms of approximately 200 shots per day, each with a duration of approximately 1/3 day. A pinhole camera was used to obtain data and the data were statistically analyzed.

Holt, S. S.↗
NASA NTRS1976

Long term X-ray studies of Sco X-1

No modulation of the 3-6 keV X-ray intensity of Sco X-1 at a level of excess of 1% is observed at the optical period of .787313d. Evidence is found for shot-noise character in a large fraction or the X-ray emission. Almost all of the Sco X-1 emission can be synthesized in terms of approximately 200 shots per day, each with a duration of approximately 1/3 day.

Holt, S. S.↗
NASA NTRS2008

The (55)Fe X-ray Energy Response of Mercury Cadmium Telluride Near-Infrared Detector Arrays

The accurate determination of a detector's fundamental parameters, including read noise, dark current, and QE, relies on a proper measurement of a detector's conversion gain (e- ADU(exp -1)). Charge coupling effects, such as interpixel capacitance, attenuate photon shot noise and result in an overestimation of conversion gain when implementing the photon transfer technique. An approach involving (55)Fe X-rays provides a potentially straightforward measurement of conversion gain by comparing the observed instrumental counts (ADU) to the known charge (e-) liberated by the X-ray. This technique is already preferred within the CCD community, as the pair production energy for silicon is well established. In contrast, to date the pair production energy is unknown for HgCdTe, a material commonly used for near-infrared detectors. In this paper, we derive a preliminary calibration of the (55)Fe X-ray energy response of HgCdTe using 8 HST WFC3 1.7 micrometers flight grade detectors. Our conversion of the X-ray intensities from counts into electrons implements a technique that restores the 'true' gain via classical propagation of errors. For these detectors, our analysis yields preliminary results of good statistical precision: each Ka event generates 1849 +/- 46 electrons, which corresponds to a pair production energy of 3.21+/-f 0.08 eV. We are continuing to assess potential systematic effects to further refine the accuracy of this result.

Fox, Ori↗
NASA NTRS2015

Reconstructing Emission from Pre-Reionization Sources with Cosmic Infrared Background Fluctuation Measurements by the JWST

We present new methodology to use cosmic infrared background (CIB) fluctuations to probe sources at 10 less than or approx. equal to z less than or approx. equal to 30 from a James Webb Space Telescope (JWST) NIRCam configuration that will isolate known galaxies to 28 AB mag at 0.55 m. At present significant mutually consistent source-subtracted CIB fluctuations have been identified in the Spitzer and AKARI data at 25 m, but we demonstrate internal inconsistencies at shorter wavelengths in the recent CIBER data. We evaluate CIB contributions from remaining galaxies and show that the bulk of the high-z sources will be in the confusion noise of the NIRCam beam, requiring CIB studies. The accurate measurement of the angular spectrum of the fluctuations and probing the dependence of its clustering component on the remaining shot noise power would discriminate between the various currently proposed models for their origin and probe the flux distribution of its sources. We show that the contribution to CIB fluctuations from remaining galaxies is large at visible wavelengths for the current instruments precluding probing the putative Lyman-break of the CIB fluctuations. We demonstrate that with the proposed JWST configuration such measurements will enable probing the Lyman-break. We develop a Lyman-break tomography method to use the NIRCam wavelength coverage to identify or constrain, via the adjacent two-band subtraction, the history of emissions over 10 less than or approx. equal to z less than or approx. equal to 30 as the universe comes out of the Dark Ages. We apply the proposed tomography to the current SpitzerIRAC measurements at 3.6 and 4.5 m, to find that it already leads to interestingly low upper limit on emissions at z greater than or approx. equal to 30.

NIRCam beam↗
DOE OSTI2024

Measuring axion gradients with photon interferometry

We propose a novel search technique for axions with a C P -violating monopole coupling g ˜ Q to bulk Standard Model charges Q ∈ { B , L , B − L } . Gradients in the static axion field configurations sourced by matter induce achromatic circular photon birefringence via the axion-photon coupling g ϕ γ . Circularly polarized light fed into an optical or (open) radio-frequency (RF) Fabry-Pérot (FP) cavity develops a phase shift that accumulates up to the cavity finesse: the fixed axion spatial gradient prevents a cancellation known to occur for an axion dark-matter search. The relative phase shift between two FP cavities fed with opposite circular polarizations can be detected interferometrically. This time-independent signal can be modulated up to nonzero frequency by altering the cavity orientations with respect to the field gradient. Multiwavelength co-metrology techniques can be used to address chromatic measurement systematics and noise sources. With Earth as the axion source, we project reach beyond current constraints on the product of couplings g ˜ Q g ϕ γ for axion masses m ϕ ≲ 10 − 5 eV . If shot-noise-limited sensitivity can be achieved, an experiment using high-finesse RF FP cavities could reach a factor of ∼ 10 5 into new parameter space for g ˜ Q g ϕ γ for masses m ϕ ≲ 4 × 10 − 11 eV . Published by the American Physical Society 2024

72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS↗
NASA NTRS2003

Using Correlated Photons to Suppress Background Noise

A proposed method of suppressing the effect of background noise in an optical communication system would exploit the transmission and reception of correlated photons at the receiver. The method would not afford any advantage in a system in which performance is limited by shot noise. However, if the performance of the system is limited by background noise (e.g., sunlight in the case of a free-space optical communication system or incoherently scattered in-band photons in the case of a fiber-optic communication system), then the proposed method could offer an advantage: the proposed method would make it possible to achieve a signal-to-noise ratio (S/N) significantly greater than that of an otherwise equivalent background- noise-limited optical communication system based on the classical transmission and reception of uncorrelated photons. The figure schematically depicts a classical optical-communication system and a system according to the proposed method. In the classical system, a modulated laser beam is transmitted along an optical path to a receiver, the optics of which include a narrow-band-pass filter that suppresses some of the background noise. A photodetector in the receiver detects the laser-beam and background photons, most or all of which are uncorrelated. In the proposed system, correlated photons would be generated at the transmitter by making a modulated laser beam pass through a nonlinear parametric down-conversion crystal. The sum of frequencies of the correlated photons in each pair would equal the frequency of the incident photon from which they were generated. As in the classical system, the correlated photons would travel along an optical path to a receiver, where they would be band-pass filtered and detected. Unlike in the classical system, the photodetector in the receiver in this system would be one that intrinsically favors the detection of pairs of correlated photons over the detection of uncorrelated photons. Even though there would be no way of knowing the precise location and time of creation of a given pair of correlated signal photons in the nonlinear down-conversion crystal, the fact that the photons are necessarily created at the same time and place makes it possible to utilize conventional geometrical imaging optics to reunite the photons in coincidence in the receiving photodetector. Because most or all of the signal photons would be correlated while most or all of the noise photons would be uncorrelated, the S/N would be correspondingly enhanced in the photodetector output. An additional advantage to be gained by use of a correlated-photon detector is that it could be capable of recovering the signal even in the presence of background light so bright that a classical uncorrelated-photon detector would be saturated. A blocked-impurity-band (BIB) photodetector that preferentially detects pairs of correlated photons over uncorrelated ones and that operates at a quantum efficiency of 88 percent is commercially available. This detector must be cooled to the temperature of liquid helium to obtain the desired low-noise performance. It is planned to use this detector in a proof-of-principle demonstration. In addition, it may be possible to develop GaN-based photodetectors that could offer the desired low-noise performance at room temperature.

Jackson, Deborah↗
NASA NTRS1987

Coherence effects on quasi-periodic oscillations from Galactic X-ray sources

Shot noise models provide a useful mathematical representation for some physical models for the quasi-periodic oscillations recently observed from several Galactic bulge and burst X-ray sources. For such models, correlations between the shot onset times and oscillation phases can have important effects on the expected autocorrelation function and power spectrum, with important consequences for the interpretation of observed power spectra. Making use of analytic and Monte Carlo techniques, two physically plausible correlations of this kind, one corresponding to drift and jitter in the oscillation phase and the other to a random walk in the oscillation phase, are examined.

Elsner, R. F.↗
DOE OSTI2022

Realistic model of entanglement-enhanced sensing in optical fibers

Experimental limitations such as optical loss and noise have prevented entanglement-enhanced measurements from demonstrating a significant quantum advantage in sensitivity. Holland-Burnett entangled states can mitigate these limitations and still present a quantum advantage in sensitivity. Here we model a fiber-based Mach-Zehnder interferometer with internal loss, detector efficiency, and external phase noise and without pure entanglement. This model features a practical fiber source that transforms the two-mode squeezed vacuum (TMSV) into Holland-Burnett entangled states. We predict that a phase sensitivity 28% beyond the shot noise limit is feasible with current technology. Simultaneously, a TMSV source can provide about 25 times more photon flux than other entangled sources. This system will make fiber-based quantum-enhanced sensing accessible and practical for remote sensing and probing photosensitive materials.

Krueper, Gregory↗
DOE OSTI2024

Bayesian optimization of Fisher Information in nonlinear multiresonant quantum photonics gyroscopes

Abstract We propose an on-chip gyroscope based on nonlinear multiresonant optics in a thin film χ (2) resonator that combines high sensitivity, compact form factor, and low power consumption simultaneously. We theoretically analyze a novel holistic metric – Fisher Information capacity of a multiresonant nonlinear photonic cavity – to fully characterize the sensitivity of our gyroscope under fundamental quantum noise conditions. Leveraging Bayesian optimization techniques, we directly maximize the nonlinear multiresonant Fisher Information. Our holistic optimization approach orchestrates a harmonious convergence of multiple physical phenomena – including noise squeezing, nonlinear wave mixing, nonlinear critical coupling, and noninertial signals – all encapsulated within a single sensor-resonator, thereby significantly augmenting sensitivity. We show that ∼ 470 × $\sim 470{\times}$ improvement is possible over the shot-noise limited linear gyroscope with the same footprint, intrinsic quality factors, and power budget.

42 ENGINEERING↗
NASA NTRS1981

Calculation and observation of thermal electrostatic noise in solar wind plasma

Calculations, both approximate algebraic and numerical, have been carried out for the noise due to electrostatic waves incident on a dipole antenna. The noise is calculated both for a thermal equilibrium plasma, and one having several components at different temperatures. The results are compared with measurements from the IMP-6 satellite. In various frequency ranges, the noise power is dominated by Langmuir oscillations, by electron acoustic waves and by ion acoustic waves. The measurements are consistent with all of these, although the ion waves are not definitely observed, due to interference from shot noise.

Kellogg, P. J.↗
DOE OSTI2024

Enhanced imaging of electronic hot spots using quantum squeezed light

Detecting electronic hot spots is important for understanding the heat dissipation and thermal management of electronic and semiconductor devices. Optical thermoreflective imaging is being used to perform precise temporal and spatial imaging of heat on wires and semiconductor materials. We apply quantum squeezed light to perform thermoreflective imaging on micro-wires, surpassing the shot-noise limit of classical approaches. We obtain a far-field temperature sensing accuracy of 42 mK after 50 ms of averaging and show that a 256×256 pixel image can be constructed with such sensitivity in 10 min. We can further obtain single-shot temperature sensing of 1.6 K after only 10 μs of averaging, enabling a dynamical study of heat dissipation. Not only do the quantum images provide accurate spatiotemporal information about heat distribution but also the measure of quantum correlation provides additional information, inaccessible by classical techniques, which can lead to a better understanding of the dynamics. We apply the technique to both aluminum and niobium microwires and discuss the applications of the technique in studying electron dynamics at low temperatures.

75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND↗
NASA NTRS1982

Photon bunching and the photon-noise-limited performance of infrared detectors

The photon-noise-limited performance of a radiation detector exposed to a thermal background of temperature T is analyzed by calculating the resulting specific detectivity. Both ideal photon detectors of arbitrary quantum efficiency eta and ideal thermal detectors of arbitrary emissivity eta are considered; and the effects of both shot noise and excess noise are taken into account. The relative contributions of these two sources depend on the quantum efficiency or emissivity of the system. For frequencies nu such that hnu/kT is much less than eta, excess noise can make an appreciable contribution to the total system noise. For the case of the detection of the narrow-band radiation, the specific detectivity is independent of eta in the limit hnu/kT is much less than eta.

Boyd, R. W.↗
NASA NTRS1976

Long-term X-ray studies of Scorpius X-1. II - Evidence for flare-dominated intensity variations

Data on Sco X-1 obtained with the Ariel-5 All-Sky Monitor are analyzed for variability, and it is found that a large fraction of the X-ray emission at 3 to 6 keV can be represented by shot noise. The results indicate that almost all the emission in this range can be sensibly associated with a multiplicity of shotlike flares (about 200 a day), each having a duration of about 0.33 day. It is concluded that the overall consistency with a multiplicity of long-duration shots (rather than single flares superposed on a baseline continuum) may be generally characteristic of sources with an accretion disk.

Holt, S. S.↗