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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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At least 145 records · Page 8
All sourcesNASA NTRSDOE OSTI
NASA NTRS2018

Polarization-Controlled Directional Multiphoton Photoemission from Hot Spots on Single Au Nanoshells

Directional photoemission from single Au nanoshells is demonstrated in the low-intensity, multiphoton regime. Thisdirectionality is shown to be due to the plasmonic excitation of highly photoemissive, nanometer scale surface regions, which are characterized by correlated momentum mapping, scanning electron microscopy (SEM), and laser polarization-dependence studies. Furthermore, the photoelectron flux from a single nanoshell can be systematically rotated by over 90° in momentum space simply by polarization-controlled coupling to different hot spots. Photoelectrondistributions are directly characterized in momentum space via velocity map imaging (VMI) of the two-dimensional transverse (px, py) momentum components for single nanoshells. For the majority of nanoshells studied, the photoemission is directionally orthogonal to the laser polarization, which implicates nanoscale crevice-shaped "hotspots" clearly observed in the correlated SEM/VMI studies, with the near-field plasmonic nature of these crevices clarified further via finite-element simulations. These results rationalize the large photoemission enhancements observed in previous Au nanoshell studies, but more importantly provide a novel experimental access to directionally tunable electron emission from nanoscale sources. The ability to control photoemission/photocurrent angular distributions at the nanoscale with only modest optical fields indicates a new parameter for optimizing nanoplasmonic system performance and suggests new plasmonic applications such as ultrafast, polarization-controlled photoelectric/photovoltaic switches.

Pettine, Jacob↗
NASA NTRS1987

Integrated optics implementation of a fiber optic rotation sensor - Analysis and development

The Jet Propulsion Laboratory is developing a fiber optic rotation sensor (FORS) for use on the Mariner Mark II series of planetary explorer craft and in other space applications. FORS is a closed-loop phase-nulling device and embodies a number of interesting innovations. Chief among these are the incorporation of the device's couplers, phase modulators, and polarizer on a single lithium niobate (LinbO3) integrate optics chip and a novel means of reading out angular position and rotation rate based on optical beat detection. Various aspects of the FORS design and operation are described and discussed. Particular attention is paid to analyzing errors attributable to polarizer imperfection and the so-called residual Michelson effect.

Bartman, R. K.↗
NASA NTRS2002

Nonlinear Drift-Kinetic Equation in the Presence of a Circularly Polarized Wave

Equations of the single particle motion and nonlinear kinetic equation for plasma in the presence of a circularly polarized wave of arbitrary frequency in the drift approximation are presented. The nonstationarity and inhomogeneity of the plasma-wave system are taken into account. The time dependent part of the ponderomotive force is discussed.

Khazanov, G. V.↗
NASA NTRS2003

Measurement of Characteristics of Micron Size Individual Dust Particles of Astrophysical Interest

A laboratory facility for levitating single isolated dust particles in an electrodynamic balance has been developed at NASA's Marshall Space Flight Center for conducting studies of the physical and optical properties of the analogs of interstellar and interplanetary dust grains of 0.2-20 micron size under controlled pressures/temperatures simulating astrophysical environments. We plan three classes of experiments using this facility: (1) Charge characteristics of micron size single dust grains: The photoelectric efficiencies, yields, and equilibrium potentials when exposed to UV radiation found from these measurements will provide much-needed photoelectric emission data for individual dust particles; (2) Infrared optical properties of dust particles: Specifically, we will determines the complex refractive indices, the extinction coefficients, the scattering phase functions, and the polarization properties of single dust grains of interest in interstellar environments, in the 1- 25 micron spectral region; (3) Condensation experiments to investigate the deposition of volatile gases on colder nucleated particles in dense interstellar clouds and lower planetary atmospheres: The measured data will permit determination of the sticking efficiencies of volatile gases of astrophysical interest. Brief descriptions of the experimental setup for the last two classes of experiments will be given. We will present results of measurements of photoelectric emission using 0.2-6.6 micron size silica particles exposed to UV radiation at 120-200 nm and also results of radiation pressure measurements using the same size silica particles and laser light at 5320 Angstrom.

Craven, P. D.↗
NASA NTRS1973

Polarization phenomena in multiphoton ionization of atoms

The theory of multiphoton ionization for an atomic system of arbitrary complexity is developed using a density matrix formalism. An expression is obtained which determines the differential N-photon ionization cross section as a function of the polarization states of the target atom and the incident radiation. The parameters which characterize the photoelectron angular distribution are related to the general reduced matrix elements for the N-photon transition. Two-photon ionization of unpolarized atoms is treated as an illustration of the use of the theory. The dependence of the multiphoton ionization cross section on the polarization state of the incident radiation, which has been observed in two- and three-photon ionization of Cs, is accounted for by the theory. Finally, the photoelectron spin polarization produced by the multiphoton ionization of unpolarized atoms, like the analogous polarization resulting from single-photon ionization, is found to depend on the circular polarization of the incident radiation.

Jacobs, V. L.↗
NASA NTRS1973

Polarization phenomena in multiphoton ionization of atoms.

The theory of multiphoton ionization for an atomic system of arbitrary complexity is developed using a density matrix formalism. An expression is obtained which determines the differential N-photon ionization cross section as a function of the polarization states of the target atom and the incident radiation. The parameters which characterize the photo-electron angular distribution are related to the general reduced matrix elements for the N-photon transition. Two-photon ionization of unpolarized atoms is treated as an illustration of the use of the theory. The dependence of the multiphoton ionization cross section on the polarization state of the incident radiation, which has been observed in two- and three-photon ionization of Cs, is accounted for by the theory. Finally, the photoelectron spin polarization produced by the multiphoton ionization of unpolarized atoms, like the analogous polarization resulting from single-photon ionization, is found to depend on the circular polarization of the incident radiation.

Jacobs, V. L.↗
NASA NTRS2019

Dependence of DOLP on Coronal Electron Temperature, Speed, and Structure

The degree of linear polarization (DOLP) is an important measure of the fraction of the total K-coronal brightness due to Thomson scattering of photospheric brightness off the coronal electrons that is linearly polarized. However, the corona is also brightened by the F-coronal brightness due to scattering of photospheric brightness off everything else in the corona except the electrons, which remains totally unpolarized at least up to a coronal height of 5 R. As a result, to measure the DOLP, the F- and K-coronal brightness need to be separated by taking three consecutive images by turning a linear polarizer through three well-defined angles or with a single image using a polarization camera. In this regard, the theoretically computed DOLP would be a helpful tool to compare with the experimentally measured DOLP on the real corona in order to estimate how well the F-coronal brightness is removed from the total coronal brightness to isolate the K-coronal brightness. This is important because the K-coronal brightness ratios at (410.3 nm/390.0 nm) and (423.3 nm/398.7 nm) can be used to generate maps of electron temperature and speed, respectively, and the individual K-coronal brightness at all four wavelengths can be used independently to generate maps of the electron density in the corona. In this article, for a spherically symmetric model (SSM) corona with assumed temperatures of 1.0 MK and 2.0 MK and radial flow speeds of 0.0 km/s and 250.0 km/ s for the coronal electrons, we have computed the wavelength-dependent DOLP from 370.0 nm to 470.0 nm in intervals of 1.0 nm, and for a spherically asymmetric model (SAM) corona containing a simulation of the Bastille Day coronal mass ejection, streamers, and quiet areas, we have generated maps of DOLP at the four wavelengths 390.0, 398.7, 410.3, and 423.3 nm. Finally, we have used these theoretically computed models of DOLP to compare with the experimentally measured DOLP.

Reginald, Nelson↗
NASA NTRS1993

LRAT: Lightning Radiative Transfer

In this report, we extend to cloud physics the work done for single and multiple scattering of electromagnetic waves. We consider the scattering of light, visible or infrared, by a spherical cloud represented by a statistically homogeneous ensemble of configurations of N identical spherical water droplets whose centers are uniformly distributed in its volume V. The ensemble is specified by the average number rho of scatterers in unit volume and by rho f(R) with f(R) as the distribution function for separations R of pairs. The incident light, vector-phi(sub 0) a plane electromagnetic wave with harmonic time dependence, is from outside the cloud. The propagation parameter kappa(sub 0) and the index of refraction eta(sub 0) determine physically the medium outside the distribution of scatterers. We solve the interior problem separately to obtain the bulk parameters for the scatterer equivalent to the ensemble of spherical droplets. With the interior solution or the equivalent medium approach, the multiple scattering problem is reduced to that of an equivalent single scatterer excited from outside illumination. A dispersion relation which determines the bulk propagation parameter K and the bulk index of refraction eta of the cloud is given in terms of the vector equivalent scattering amplitude vector-G and the dyadic scattering amplitude tilde-g of the single object in isolation. Based on this transfer model we will have the ability to consider clouds composed of inhomogeneous distribution of water and/or ice particles and we will be able to take into account particle size distributions within the cloud. We will also be able to study the effects of cloud composition (i.e., particle shape, size, composition, orientation, location) on the polarization of the single or the multiple scattered waves. Finally, this study will provide a new starting point for studying the problem of lightning radiative transfer.

Phanord, Dieudonne D.↗
NASA NTRS2015

Coming of Age: Polarization as a Probe of Plant Canopy Water Status

We tested the hypothesis that the relative water content (RWC) of the sunlit leaves in a plant canopy may be estimated from polarized canopy imagery. Recently (IGARSS, July 27-31, 2015, Milan, Italy), we reported the results of laboratory polarization measurements of single detached leaves during dry down. We found that RWC was linearly related to the ratio of the reflectance of the interior of the leaf and the leaf transmittance. Here we report application of the laboratory results to estimate RWC for sunlit leaves in a plant canopy. Using a commercial-off-the-shelf (COTS) Nikon 810 camera with Nikkor 300 mm lens and Polaroid type HN-22 linear polarizer, we photographed in the principle plane a plant canopy displaying a gradient of water stress and collected, at each of multiple points along the gradient, two images, one with the polarization filter oriented for maximum scene response and a second with the filter oriented for minimum scene response. We converted the digital values in the two images to reflectance factor with reference to images of a white, flat, horizontal Spectralon surface. We classified the polarization imagery, identifying reflecting leaves, transmitting leaves, other sunlit vegetation and shadows. For each image pair we normalized the leaf internal reflectance by dividing by the cosine of the angle of incidence of the sunlight on the leaf, selected the leaf maximum transmittance in the scene and divided to obtain the ratio reflectance/transmittance, which we compared with leaf RWC. We determined the leaf relative water content by harvesting a section of leaf and immediately placing it in a sealed container in an ice chest. Later in the laboratory the leaf sample was weighed, rehydrated, weighed, dried and again weighed. RWC was determined using the standard formula. Our experimental results support our hypothesis, suggesting that the RWC of sunlit leaves in a plant canopy may be estimated from analysis of polarization imagery collected by a COTS camera system. Unlike remotely sensed estimates of canopy equivalent water thickness, our estimates of the RWC of sunlit canopy leaves provide leaf physiological information. We propose RWC estimates based upon sunlit leaves are more relevant to assessing the water status of a plant canopy than would be RWC estimates based upon large FOV canopy measurements.

estimates↗
NASA NTRS2002

Laboratory Studies of the Optical Properties and Condensation Processes of Cosmic Dust Particles

A laboratory facility for levitating single isolated dust particles in an electrodynamics balance has been developing at NASA/Marshall Space Flight Center for conducting a variety of experimental, of astrophysical interest. The objective of this research is to employ this innovative experimental technique for studies of the physical and optical properties of the analogs of cosmic grains of 0.2-10 micron size in a chamber with controlled pressure/temperatures simulating astrophysical environments. In particular, we will carry out three classes of experiments to investigate the microphysics of the analogs of interstellar and interplanetary dust grains. (1) Charge characteristics of micron size single dust grains to determine the photoelectric efficiencies, yields, and equilibrium potentials when exposed to UV radiation. These measurements will provide the much-needed photoelectric emission data relating to individual particles as opposed to that for the bulk materials available so far. (2) Infrared optical properties of dust particles obtained by irradiating the particles with radiation from tunable infrared diode lasers and measuring the scattered radiation. Specifically, the complex refractive indices, the extinction coefficients, the scattering phase functions, and the polarization properties of single dust grains of interest in interstellar environments, in the 1-25 micron spectral region will be determined. (3) Condensation experiments to investigate the deposition of volatile gases on colder nucleated particles in dense interstellar clouds and lower planetary atmospheres. The increase in the mass or m/q ratio due to condensation on the particle will be monitored as a function of the dust particle temperature and the partial pressure of the injected volatile gas. The measured data wild permit determination of the sticking efficiencies of volatile gases of astrophysical interest. Preliminary results based on photoelectric emission experiments on 0.2-6.6 micron size silica particles exposed to UV radiation in the 120-200 nm spectral region will be presented.

Abbas, Mian M.↗
DOE OSTI2024

Self‐Potential Tomography Preconditioned by Particle Swarm Optimization—Application to Monitoring Hyporheic Exchange in a Bedrock River

Abstract A self‐potential (SP) data‐inversion algorithm was developed and tested on an analytical model of electrical‐potential profile data attributed to single and multiple polarized electrical sources. The developed algorithm was then validated by an application to SP‐monitoring field data measured on the floodplain of East Fork Poplar Creek, Oak Ridge, Tennessee, to image electrical sources in areas conducive to preferential flow into the flood plain from the bedrock‐lined riverbed. The algorithm combined stochastic source‐localization by particle‐swarm‐optimization (PSO) of electrical sources characterized by simplified geometries with source tomography by regularized weighted least‐squares minimization of a quadratic objective function. Prior information was incorporated by preconditioning the tomography algorithm by PSO results. Variable percentages of random noise were added to analytical‐model data to evaluate the algorithm performance. Results indicated that true parameters of single‐source models were inverted and approximated with small residual error, whereas inversion of analytical‐model data representing multiple electrical sources accurately approximated the locations of the sources but miscalculated some parameters because of the non‐uniqueness of the inverse‐model solution. Source tomography applied to analytical model data during testing produced a spatially continuous parameter field that identified the locations of point‐scale synthetic dipole sources of electrical current flow with varying degrees of accuracy depending on the prior information incorporated into the tomography. When applied to SP‐monitoring field data, the algorithm imaged electrical sources within a known fault that intersects the bedrock riverbed and flood plain of East Fork Poplar Creek and depicted dynamic electrical conditions attributed to hyporheic exchange.

54 ENVIRONMENTAL SCIENCES↗
NASA NTRS1992

Backscattering from a randomly rough dielectric surface

A backscattering model for scattering from a randomly rough dielectric surface is developed based on an approximate solution of a pair of integral equations for the tangential surface fields. Both like and cross-polarized scattering coefficients are obtained. It is found that the like polarized scattering coefficients contain two types of terms: single scattering terms and multiple scattering terms. The single scattering terms in like polarized scattering are shown to reduce the first-order solutions derived from the small perturbation method when the roughness parameters satisfy the slightly rough conditions. When surface roughnesses are large but the surface slope is small, only a single scattering term corresponding to the standard Kirchhoff model is significant. If the surface slope is large, the multiple scattering term will also be significant. The cross-polarized backscattering coefficients satisfy reciprocity and contain only multiple scattering terms. The difference between vertical and horizontal scattering coefficients is found to increase with the dielectric constant and is generally smaller than that predicted by the first-order small perturbation model. Good agreements are obtained between this model and measurements from statistically known surfaces.

Fung, Adrian K.↗
DOE OSTI2026

Single-Molecule Tracking Measurements Reveal the Detailed Mechanisms of Molecular Diffusion in Solvent Mixtures under Nanoconfinement

Understanding mass transport mechanisms in nanopores is important for developing advanced materials for chemical separations, chemical sensing, and energy storage. This paper reports a novel imaging platform that is employed for the first time to investigate the detailed diffusion dynamics of single rhodamine B (RhB) dye molecules confined within solution-filled cylindrical anodic aluminum oxide (AAO) nanopores. The imaging platform relies on illumination of horizontally-oriented AAO nanopores in a highly inclined and laminated optical (HILO) light sheet microscopy geometry. The method was used to investigate the translational and orientational dynamics of single rhodamine B (RhB) molecules within horizontally-oriented 5- and 10-nm diameter AAO nanopores filled with water–ethanol mixtures. The established platform enabled the observation of one-dimensional motion along the pore axis involving occasional short- or long-term immobilization at the single-molecule level. Analysis of cumulative squared-displacement distributions revealed fast (5 – 30 µm²/s), intermediate (1 – 5 µm²/s), and slow (< 1 µm²/s) diffusion components. From the effects of mixture composition and pore size on the contributions of these three components, we inferred that the fast, intermediate, and slow components could be assigned to desorption-mediated hopping, crawling, and wiggling motions, respectively. The platform based on the horizontally-oriented AAO nanopores also permitted single-molecule emission polarization measurements that revealed the negligible steric confinement of individual diffusing RhB molecules within the AAO nanopores. The imaging platform based on AAO membranes and HILO microscopy provided a unique means to investigate how solvation-mediated surface interactions and nanoconfinement govern molecular transport in nanoporous environments.

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CH↗
NASA NTRS1992

Non-mechanical optical path switching and its application to dual beam spectroscopy including gas filter correlation radiometry

A non-mechanical optical switch is developed for alternately switching a monochromatic or quasi-monochromatic light beam along two optical paths. A polarizer polarizes light into a single, e.g., vertical component which is then rapidly modulated into vertical and horizontal components by a polarization modulator. A polarization beam splitter then reflects one of these components along one path and transmits the other along the second path. In the specific application of gas filter correlation radiometry, one path is directed through a vacuum cell and one path is directed through a gas correlation cell containing a desired gas. Reflecting mirrors cause these two paths to intersect at a second polarization beam splitter which reflects one component and transmits the other to recombine them into a polarization modulated beam which can be detected by an appropriate single sensor.

Sachse, Glen W.↗
NASA NTRS1976

High resolution Fourier interferometer-spectrophotopolarimeter

A high-resolution Fourier interferometer-spectrophotopolarimeter is provided using a single linear polarizer-analyzer the transmission axis azimuth of which is positioned successively in the three orientations of 0 deg, 45 deg, and 90 deg, in front of a detector; four flat mirrors, three of which are switchable to either of two positions to direct an incoming beam from an interferometer to the polarizer-analyzer around a sample cell transmitted through a medium in a cell and reflected by medium in the cell; and four fixed focussing lenses, all located in a sample chamber attached at the exit side of the interferometer. This arrangement can provide the distribution of energy and complete polarization state across the spectrum of the reference light entering from the interferometer; the same light after a fixed-angle reflection from the sample cell containing a medium to be analyzed; and the same light after direct transmission through the same sample cell, with the spectral resolution provided by the interferometer.

Fymat, A. L.↗
NASA NTRS1979

On the design of a postprocessor for a search for extraterrestrial intelligence /SETI/ system

The design of an on-line postprocessor for a search for extraterrestrial intelligence (SETI) system is described. Signal processing tasks of the postprocessor include: (1) analysis of power level, phase coherence, and state of polarization of single-channel signals in a search for significant signals; (2) grouping or aggregation of adjacent channel data, time averaging of data; and (3) the detection of drifting and modulated signals. Control functions include multichannel spectrum analyzer frequency and clock control, system calibration and selfdiagnostic, control of data flow to and from short-term and long-term (archival) memories, and operation of detection subsystems, such as a visual display and a tunable receiver.

Healy, T. J.↗
NASA NTRS1980

On the low lying singlet states of BeO

Calculations of the ground and low-lying singlet states of BeO are performed in order to gain an understanding of the techniques needed to treat the excited states of other, more complex, ionic molecules. The MCSCF and CI calculations are based on a Gaussian basis set of slightly better than double zeta plus polarization quality for single configuration descriptions of the states. The calculated X-A and X-B state separations are found to be in agreement with experimental measurements. The 1 Sigma - and 1 Delta states are predicted to lie approximately 40,000 kaysers above the ground state and are identified as the C and D states.The 2 1 Pi state is found to be approximately 15,000 kaysers and the 3 1 Sigma + state is found to be approximately 65,000 kaysers above the ground state.

Bauschlicher, C. W., Jr.↗