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Search indexed NASA NTRS and DOE OSTI research on propulsion, heat transfer, battery materials and energy systems. Follow report and document links to the original sources.

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All sourcesNASA NTRSDOE OSTI
DOE OSTI2021

Aerosol characteristics at the Southern Great Plains site during the HI-SCALE campaign

Abstract. Large uncertainties exist in global climate model predictions of radiative forcing due to insufficient understanding and simplified numerical representation of cloud formation and cloud–aerosol interactions. The Holistic Interactions of Shallow Clouds, Aerosols and Land Ecosystems (HI-SCALE) campaign was conducted near the DOE's Atmospheric Radiation Measurement (ARM) Southern Great Plains (SGP) site in north-central Oklahoma to provide a better understanding of land–atmosphere interactions, aerosol and cloud properties, and the influence of aerosol and land–atmosphere interactions on cloud formation. The HI-SCALE campaign consisted of two intensive observational periods (IOPs) (April–May and August–September, 2016), during which coincident measurements were conducted both on the G-1 aircraft platform and at the SGP ground site. In this study we focus on the observations at the SGP ground site. An Aerodyne high-resolution time-of-flight aerosol mass spectrometer (HR-ToF-AMS) and an Ionicon proton-transfer-reaction mass spectrometer (PTR-MS) were deployed, characterizing chemistry of non-refractory aerosol and trace gases, respectively. Contributions from various aerosol sources, including biogenic and biomass burning emissions, were retrieved using factor analysis of the AMS data. In general, the organic aerosols at the SGP site was highly oxidized, with oxygenated organic aerosol (OOA) identified as the dominant factor for both the spring and summer IOP though more aged in spring. Cases of isoprene-epoxydiol-derived secondary organic aerosol (IEPOX SOA) and biomass burning events were further investigated to understand additional sources of organic aerosol. Unlike other regions largely impacted by IEPOX chemistry, the IEPOX SOA at SGP was more highly oxygenated, likely due to the relatively weak local emissions of isoprene. Biogenic emissions appear to largely control the formation of organic aerosol (OA) during the HI-SCALE campaign. Potential HOM (highly oxygenated molecule) chemistry likely contributes to the highly oxygenated feature of aerosols at the SGP site, with impacts on new particle formation and global climate.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2024

Large spatiotemporal variability in aerosol properties over central Argentina during the CACTI field campaign

Abstract. Few field campaigns with extensive aerosol measurements have been conducted over continental areas in the Southern Hemisphere. To address this data gap and better understand the interactions of convective clouds and the surrounding environment, extensive in situ and remote sensing measurements were collected during the Cloud, Aerosol, and Complex Terrain Interactions (CACTI) field campaign conducted between October 2018 and April 2019 over the Sierras de Córdoba range of central Argentina. This study describes measurements of aerosol number, size, composition, mixing state, and cloud condensation nuclei (CCN) collected on the ground and from a research aircraft during 7 weeks of the campaign. Large spatial and multiday variations in aerosol number, size, composition, and CCN were observed due to transport from upwind sources controlled by mesoscale to synoptic-scale meteorological conditions. Large vertical wind shears, back trajectories, single-particle measurements, and chemical transport model predictions indicate that different types of emissions and source regions, including biogenic emissions and biomass burning from the Amazon and anthropogenic emissions from Chile and eastern Argentina, contribute to aerosols observed during CACTI. Repeated aircraft measurements near the boundary layer top reveal strong spatial and temporal variations in CCN and demonstrate that understanding the complex co-variability of aerosol properties and clouds is critical to quantify the impact of aerosol–cloud interactions. In addition to quantifying aerosol properties in this data-sparse region, these measurements will be valuable to evaluate predictions over the midlatitudes of South America and improve parameterized aerosol processes in local, regional, and global models.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Remote-sensing and radiosonde datasets collected in the San Luis Valley during the LAPSE-RATE campaign

Abstract. In July 2018, the International Society for Atmospheric Research using Remotely piloted Aircraft (ISARRA) hosted a flight week to showcase the role remotely piloted aircraft systems (RPASs) can have in filling the atmospheric data gap. This campaign was called Lower Atmospheric Process Studies at Elevation – a Remotely-piloted Aircraft Team Experiment (LAPSE-RATE). In support of this campaign, ground-based remote and in situ systems were also deployed for the campaign. The University of Oklahoma deployed the Collaborative Lower Atmospheric Mobile Profiling System (CLAMPS), the University of Colorado deployed two Doppler wind lidars, and the National Severe Storms Laboratory deployed a mobile mesonet with the ability to launch radiosondes. This paper focuses on the data products from these instruments that result in profiles of the atmospheric state. The data are publicly available in the Zenodo LAPSE-RATE community portal (https://zenodo.org/communities/lapse-rate/, 19 January 2021). The profile data discussed are available at https://doi.org/10.5281/zenodo.3780623 (Bell and Klein, 2020), https://doi.org/10.5281/zenodo.3780593 (Bell et al., 2020b), https://doi.org/10.5281/zenodo.3727224 (Bell et al., 2020a), https://doi.org/10.5281/zenodo.3738175 (Waugh, 2020b), https://doi.org/10.5281/zenodo.3720444 (Waugh, 2020a), and https://doi.org/10.5281/zenodo.3698228 (Lundquist et al., 2020).

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2023

CPC data from TAMU TRACER campaign in the Houston, TX region from July to September 2022

During TRACER, the Texas A&M Rapid Onsite Atmospheric Measurements Van (ROAM-V) was deployed to capture airmasses behind (maritime) and ahead (continental) of the passage of the sea-breeze front through Houston. On select sampling days, ROAM-V sampled in the morning/mid-day on the coast and then transited to a second inland site for the afternoon/evening. The suite of instruments deployed on ROAM-V included a Condensation Particle Counter (CPC; GRIMM Model 5.403 CPC), Scanning Mobility Particle Sizer (SMPS; TSI 3750 detector, TSI 3082 classifier, TSI 3088 neutralizer, TSI 3081A Differential Mobility Analyzer), Cloud Condensation Nuclei counter (Droplet Measurement Technologies CCN Counter), micro pulse lidar (Droplet Measurement Technologies Micro Pulse LiDAR (miniMPL)), and a Davis Rotating Uniform size-cut Monitor (DRUM; DRUMAir 4-DRUM). Before sampling at each location, the latitude and longitude were recorded using the GPS on the phone application “My Altitude”. Onboard the ROAM-V, aerosol samples are drawn through a shared isokinetic inlet at a flow rate ranging from 3.5 to 7.0 LPM. A portion of this flow is directed through a cyclone impactor (Brechtel, Inc. Model SCC 0.732) and 0.3 LPM is directed to the CPC. To correct the data for particle losses, we used a two-step method. First, the measured SMPS size distributions were used to calculate total particle loss through the inlet for every SMPS scan at a single deployment location. Second, the CPC data was corrected for particle losses using the average of the total losses per scan. This calculation was done separately for each deployment location due to changes in the measured size distributions between locations. Particle loss from diffusion (based on Kesten, 1991 and Gormley, 1949), inertial impaction in 90-degree bends (based on Aerosol Measurement, 2011 and Crane, 1977), and cyclone impactor efficiency (based on Dirgo, 1985) were included in the loss calculation. When the SMPS was not sampling at a location (in the case of an instrument malfunction or operator error), the reported CPC data was corrected with an average of the total losses for the entire campaign at the specified deployment location (e.g., if we needed to correct Galveston data, then the average of all calculated losses at Galveston was taken). These flatline corrections were used for all data on 22/07/13, 22/07/20, 22/07/22, and the data from Galveston on 22/08/09. An additional flatline correction of 14% was applied to all CPC data based on laboratory calibration prior to and after the campaign. In laboratory calibrations, we identified that for the same sample of air the field CPC (GRIMM Model 5.403 CPC) undercounted the total concentration of particles by 14% compared to the ground truth laboratory CPC (TSI Model 3750). This data was collected for ARM Field Campaign AFC07055 and supported by DOE ASR grant DE-SC0021047. For any further questions, please feel free to contact the instrument PI, Sarah D. Brooks, sbrooks@tamu.edu. Kesten et. al. Calibration of a TSI Model 3025 Ultrafine Condensation Particle Counter. Aerosol Science and Technology, 15:2, 107-111, 1991. Gormley et. al. Diffusion from a Stream Flowing through a Cylindrical Tube. Proceedings of the Royal Irish Academy, Vol 52, 163-169, 1948. Aerosol Measurement: Principles, Techniques, and Applications, Third Edition. John Wiley & Sons, Inc, 2011. Crane et. al. Inertial Deposition of Particles in a Bent Pipe. Journal of Aerosol Science, Vol 8, 161-170, 1977. Dirgo et. al. Cyclone Collection Efficiency: Comparison of Experimental Results with Theoretical Predictions. Aerosol Science and Technology, 4:4, 401-415, 1985.

54 ENVIRONMENTAL SCIENCES↗
DOE OSTI2021

Results from the Alfven Eigenmode Active Diagnostic during the 2019-2020 JET deuterium campaign

This paper presents results of extensive analysis of mode excitation observed during the operation of the Alfven Eigenmode Active Diagnostic (AEAD) in the JET tokamak during the 2019-2020 deuterium campaign. Six of eight toroidally spaced antennas, each with independent power and phasing, were successful in actively exciting stable MHD modes in 479 plasmas. In total, 4768 magnetic resonances were detected with up to fourteen fast magnetic probes. In this work, we present the calculations of resonant frequencies f0, damping rates \gamma < 0, and toroidal mode numbers n, spanning the parameter range f0 = 30 - 250 kHz, -\gamma = 0 - 13 kHz, and |n| < 30. In general, good agreement is seen between the resonant and the calculated toroidal Alfven Eigenmode frequencies, and between the toroidal mode numbers applied by the AEAD and estimated of the excited resonances. We note several trends in the database: the probability of resonance detection decreases with plasma current and external heating power; the normalized damping rate increases with edge safety factor but decreases with external heating. These results provide key information to prepare future experimental campaigns and to better understand the physics of excitation and damping of Alfven Eigenmodes in the presence of alpha particles during the upcoming DT campaign, thereby extrapolating with confidence to future tokamaks.

70 PLASMA PHYSICS AND FUSION TECHNOLOGY↗
NASA NTRS1989

Stratospheric ozone measurements from the 1985 MAP/GLOBUS NO(x) campaign

Nine experiments obtained stratospheric ozone measurements during the fall 1985 Middle Atmosphere Program (MAP) Global Budget of Stratospheric Trace Constituents (GLOBUS) NO(x) campaign. Measurements are grouped into four sets from four air masses and compared. Agreement between individual experiments and weighted mean profiles is generally within 10 percent and within absolute accuracies. Dobson Umkehr values in layer 5 differ by more than absolute accuracies from weighted mean profiles. Brewer sonde values for one data set are outside absolute accuracies near the ozone peak. Solar UV occultation measurements are 30-35 percent less than the weighted mean profile and outside absolute accuracies. Measurements from the Exospheric Satellite backscattered ultraviolet experiment, not previously compared with other techniques, agree within 10-15 percent of weighted mean profiles. Results of the campaign are generally consistent with those of four previous intercomparison campaigns.

Robbins, D.↗
NASA NTRS1992

The Olympus and ACTS propagation measurement campaigns in the U.S

The Jet Propulsion Laboratory under the auspices of NASA carries out radiowave propagation studies for satellite communications. As a prelude to the ACTS experiments, it was considered prudent to gather experience in 20/30 GHz propagation using the Olympus satellite beacons at 12, 20, and 30 GHz. Therefore, NASA funded an experiment program with Virginia Tech under JPL management to develop hardware and to collect data for the Olympus campaign. The paper reviews the results of the Olympus campaign. The experience gathered from this campaign is beneficial to the forthcoming ACTS propagation program which is also discussed in this paper.

Stutzman, Warren L.↗
NASA NTRS1992

Botswana water and surface energy balance research program. Part 1: Integrated approach and field campaign results

The Botswana water and surface energy balance research program was developed to study and evaluate the integrated use of multispectral satellite remote sensing for monitoring the hydrological status of the Earth's surface. Results of the first part of the program (Botswana 1) which ran from 1 Jan. 1988 - 31 Dec. 1990 are summarized. Botswana 1 consisted of two major, mutually related components: a surface energy balance modeling component, built around an extensive field campaign; and a passive microwave research component which consisted of a retrospective study of large scale moisture conditions and Nimbus scanning multichannel microwave radiometer microwave signatures. The integrated approach of both components in general are described and activities performed during the surface energy modeling component including the extensive field campaign are summarized. The results of the passive microwave component are summarized. The key of the field campaign was a multilevel approach, whereby measurements by various similar sensors were made at several altitudes and resolution. Data collection was performed at two adjacent sites of contrasting surface character. The following measurements were made: micrometeorological measurements, surface temperatures, soil temperatures, soil moisture, vegetation (leaf area index and biomass), satellite data, aircraft data, atmospheric soundings, stomatal resistance, and surface emissivity.

Vandegriend, A. A.↗
NASA NTRS1990

Preliminary results from the MAESTRO 1 Campaign over the Black Forest

The Joint Research Center (JRC) Ispra and the European Space Agency (ESA) have co-sponsored the deployment of the National Aeronautics and Space Agency (NASA) and Jet Propulsion Laboratory (JPL), C-, L-, and P-band polarimetric synthetic aperture radar (SAR) in Europe in mid-August 1989. This deployment represents the first opportunity for European agencies and institutes to evaluate the current state of the art of multifrequency polarimetric imaging technology over European Test Sites. Of particular interest to the Joint Research Center (JRC) Ispra is the Black Forest Test Site at Freiburg in the Federal Republic of Germany. This Test Site incorporates the Villingen region of the Black Forest to the south-west of Germany. This paper reports upon the activities undertaken in preparation for the MAESTRO 1 Campaign in the Black Forest Test Site. In particular this paper reports upon the ground data collection campaign for the Freiburg Test Site where extensive and intensive ground data measurements were undertaken. These measurements were based upon standard ground data collection protocols developed for forestry by the JRC and utilized throughout Europe for the MAESTRO 1 Campaign. The paper then goes on to present preliminary results derived from the SAR data using the JRC-developed software for polarimetric data interpretation, POLTOOL.

Churchill, P. N.↗
NASA NTRS1995

Preliminary results from the Sprites94 aircraft campaign: 1. Red sprites

The dual jet aircraft Sprites94 campaign yielded the first color imagery and unambiguously triangulated physical dimensions and heights of upper atmospheric optical emissions associated with thunderstorm systems. Low light level television images, in both color and in black and white (B/W), obtained during the campaign show that there are at least two distinctively different types of optical emissions spanning part or all of the distance between the anvil tops and the ionosphere. The first of these emissions, dubbed 'sprites' after their elusive nature, are luminous structures of brief (less than 16 ms) duration with a red main body that typically spans the latitude range 50-90 km, and possessing lateral dimensions of 5-30 km. Faint bluish tendrils often extend downward from the main body of sprites, occasionally appearing to reach cloud tops near 20 km. In this paper the principal characteristics of red sprites as observed during the Sprites94 campaign are described. The second distinctive type of emissions, 'blue jets,' are described in a companion paper (Wescott et al., this issue).

Sentman, D. D.↗
NASA NTRS1998

First results from the aerosol lidar and backscatter sonde intercomparison campaign STRAIT'1997 at table mountain facility during February-March 1997

First results of an intercomparison measurement campaign between three aerosol lidar instruments and in-situ backscatter sondes performed at Table Mountain Facility (34.4 deg N, 117.7 deg E, 2280 m asl) in February-March 1997 are presented. During the campaign a total of 414 hours of lidar data were acquired by the Aerosol-Temperature-Lidar (ATL, Goddard Space Flight Center) the Mobile-aerosol-Raman-Lidar (MARL, Alfred Wegener Institute), and the TMF-Aerosol-Lidar (TAL, Jet Propulsion Laboratory), and four backscatter sondes were launched. From the data set altitude profiles of backscatter ratio and volume depolarization of stratospheric background aerosols at altitudes between 15 and 25 km and optically thin high-altitude cirrus clouds at altitudes below 13 km are derived. On the basis of a sulfuric acid aerosol model color ratio profiles obtained from two wavelength lidar data are compared to the corresponding profiles derived from the sonde observations. We find an excellent agreement between the in-situ and ATL lidar data with respect to backscatter and color ratio. Cirrus clouds were present on 16 of 26 nights during the campaign. Lidar observations with 17 minute temporal and 120-300 m spatial resolution indicate high spatial and temporal variability of the cirrus layers. Qualitative agreement is found between concurrent lidar measurements of backscatter ratio and volume depolarization.

Beyerle, G.↗
NASA NTRS1999

Rocket/Radar Sporadic-E Experiment Conducted during the El Coqui 2 Campaign

In order to investigate the complex electrodynamics and neutral-plasma coupling inherent to sporadic-E layers in the earth's mid-latitude ionosphere, a series of rocket/radar experiments were planned as part of the NASA El Coqui H Campaign from Tortuguero Launch Range, Puerto Rico, in March-April, 1998. The rocket experiments consisted of two pairs of "mother-daughter" payloads with limited apogees so that the payloads "hovered" in the sporadic-E region (95-125 km). Each payload pair included vector DC and AC electric field detectors, a highly accurate flux-gate DC magnetometer, an ion mass spectrometer, an ionization gauge, and spaced-electric field receivers to measure the wavelength and phase velocity of the unstable plasma waves. Separate rockets were included to simultaneously carry aloft TMA trails to measure the neutral wind and its velocity shear, believed responsible for the sporadic-E layer formation. In addition to the rocket experiments, incoherent scatter radar measurements of plasma density and drift velocity were gathered almost every night during the 3 week campaign. Continuous VHF backscatter radar operations were carried out from a site near Salinas, Puerto Rico, where 3-m backscatter echoes were observed associated with sporadic-E and other types of low altitude ionospheric layers. Other radars that operated during the campaign included an HF backscatter system near Ponce, Puerto Rico, and a second VHF backscatter radar set up near Aguadila Puerto Rico. On 24 March 1998, one of the instrumented rockets was launched, attaining an apogee of 129 km. The payloads successfully pierced an intense sporadic-E layer observed by both the Arecibo radar and the in-situ density and ion mass spectrometer probes. In-situ DC electric fields revealed very low (about 1-2 mV/m) ambient fields with small amplitude structures of the same order. No high frequency (short scale) waves were observed, consistent with the VHF backscatter observations at the time of the launch. An overview of the observations will be presented.

Pfaff, R.F.↗
NASA NTRS1999

The Guara Campaign: Rocket-Radar Investigations of the Earth's Upper Atmosphere at the Magnetic and Geographic Equators

The Guara Campaign consisted of a series of sounding rockets that were launched from August to October, 1994 at a new launch facility at Alcantara, Brazil, which is within one degree of the Earth's magnetic equator. The campaign was based on focused scientific experiments designed to investigate the electrodynamics and irregularities in the ionosphere and mesosphere at the Earth's magnetic equator and to study their relationship with neutral upper atmosphere motions. In all, 13 large sounding rockets and 20 small meteorological rockets were launched as part of four different experiment groups designed to investigate: (1) the daytime equatorial electrojet, (2) very high altitude Spread-F processes, (3) sunset electrodynamics, and (4) middle atmosphere-thermosphere coupling at the equator. The instrumentation on the sounding rockets varied with each investigation, but primarily included experiments to measure electric fields, currents, plasma densities,- neutral winds, neutral densities and temperatures, and ionospheric instabilities. All of the experiments utilized ground-based scientific instruments including a VHF backscatter radar interferometer, magnetometers, ionosondes, and scintillation receivers. An overview of each investigation is provided, along with a description of the launch site and the ground-based experiments. Scientific highlights of the campaign are provided.

Pfaff, Robert F., Jr.↗
NASA NTRS2000

Sea WiFS Postlaunch Technical Report Series: The SeaBOARR-99 Field Campaign - Volume 8

This report documents the scientific activities during the second Sea-viewing Wide Field-of-view Sensor (Sea- WIFS) Bio-Optical Algorithm Round-Robin (SeaBOARR-99) field campaign, which took place from 2 May to 7 June 1999 on board the Royal Research Ship James Clark Ross during the eighth Atlantic Meridional Transect cruise (AMT-8). The ultimate objective of the SeaBOARR activity is to evaluate the effect of different measurement protocols on bio-optical algorithms using data from a variety of field campaigns. The SeaBOARR-99 field campaign was concerned with collecting a high quality data set of simultaneous in-water and above-water radiometric measurements. The deployment goals documented in this report were to: a) use four different surface glint correction methods to compute water-leaving radiances, Lw(lambda), from above-water data; b) use two different in-water profiling systems and three different methods to compute Lw(lambda) from in-water data; c) use instruments with a common calibration history to minimize intercalibration uncertainties; d) monitor the calibration stability of the instruments in the field with the original SeaWiFS Quality Monitor (SQM) and a commercial, second-generation device called the SQM-II, thereby allowing a distinction between differences in methods from changes in instrument performance; and e) compare the Lw(lambda) values estimated from the above- water and in- water measurements. In addition to describing the instruments deployed and the data collected, a preliminary analysis of part of the SeaBOARR-99 data set is presented (using only the data collected during clear sky, calm sea, and Case-I waters).

Hooker, Stanford B.↗
NASA NTRS1997

Equatorial Dynamics Observed by Rocket, Radar, and Satellite During the CADRE/MALTED Campaign: Programmatics and small-scale fluctuations - 1

In August 1994, the Mesospheric and Lower Thermospheric Equatorial Dynamics (MALTED) Program was conducted from the Alcantara rocket site in northeastern Brazil as part of the International Guard Rocket Campaign to study equatorial dynamics, irregularities, and instabilities in the ionosphere. This site was selected because of its proximity to the geographic (2.3 deg S) and magnetic (approx. 0.5 deg S) equators. MALTED was concerned with planetary wave modulation of the diurnal tidal amplitude, which exhibits considerable amplitude variability at equatorial and subtropical latitudes. Our goals were to study this global modulation of the tidal motions where tidal influences on the thermal structure are maximum, to study the interaction of these tidal structures with gravity waves and turbulence at mesopause altitudes, and to gain a better understanding of dynamic influences and variability on the equatorial middle atmosphere. Four (two daytime and two nighttime) identical Nike-Orion payloads designed to investigate small-scale turbulence and irregularities were coordinated with 20 meteorological falling-sphere rockets designed to measure temperature and wind fields during a 10-day period. These in situ measurements were coordinated with observations of global-scale mesospheric motions that were provided by various ground based radars and the Upper Atmosphere Research Satellite (UARS) through the Coupling and Dynamics of Regions Equatorial (CADRE) campaign. The ground-based observatories included the Jicamarca radar observatory near Lima, Peru, and medium frequency (MF) radars in Hawaii, Christmas Island, and Adelaide. Since all four Nike-Orion flights penetrated and overflew the electrojet with apogees near 125 km, these flights provided additional information about the electrodynamics and irregularities in the equatorial ionospheric E region and may provide information on wave coupling between the mesosphere and the electrojet. Simultaneous with these flights, the CUPRI 50-MHz radar (Cornell University) provided local sounding of the electrojet region. A description of the campaign logistics and the measurements performed with the Nike-Orion instrumentation and their implications for turbulence due to gravity waves and tidal instability in the mesosphere and lower thermosphere (MLT) are presented here. From a study of electron density fluctuations measured by rocket probes, we have found evidence for equatorial mesospheric neutral-atmospheric turbulence between 85 and 90 km. Furthermore, falling-sphere data imply that gravity wave breaking was a source for this turbulence. Mean motions and the various planetary, tidal, and gravity wave structures and their coherence and variability are the subjects of a companion paper.

Goldberg, Richard A.↗
NASA NTRS2001

An Assessment of the Ozone Loss During the 1999-2000 SOLVE Arctic Campaign

Ozone observations from ozonesondes, the lidars aboard the DC-8, in situ ozone measurements from the ER-2, and satellite ozone measurements from Polar Ozone and Aerosol Measurement III (POAM) were used to assess ozone loss during the Sage III Ozone Loss and Validation Experiment (SOLVE) 1999-2000 Arctic campaign. Two methods of analysis were used. In the first method a simple regression analysis is performed on the ozonesonde and POAM measurements within the vortex. In the second method, the ozone measurements from all available ozone data were injected into a free running diabatic trajectory model and carried forward in time from December 1 to March 15. Vortex ozone loss was then estimated by comparing the ozone values of those parcels initiated early in the campaign with those parcels injected later in the campaign. Despite the variety of observational techniques used during SOLVE, the measurements provide a fairly consistent picture. Over the whole vortex, the largest ozone loss occurs between 550 and 400 K potential temperatures (approximately 23-16 km) with over 1.5 ppmv lost by March 15, the end of the SOLVE mission period. An ozone loss rate of 0.04-0.05 ppmv/day was computed for March 15. Ozonesondes launched after March 15 suggest that an additional 0.5 ppmv or more ozone was lost between March 15 and April 1. The small disagreement between ozonesonde and POAM analysis of January ozone loss is found to be due to biases in vortex sampling. POAM makes most of its solar occultation measurements at the vortex edge during January 2000 which bias samples toward air parcels that have been exposed to sunlight and likely do experience ozone loss. Ozonesonde measurements and the trajectory technique use observations that are more distributed within the interior of the vortex. Thus the regression analysis of the POAM measurements tends to overestimate mid-winter vortex ozone loss. Finally, our loss calculations are broadly consistent with other loss computations using ER-2 tracer data and MLS satellite data, but we find no evidence for the 1992 high mid-January loss reported using the Match technique.

Schoeberl, Mark R.↗
NASA NTRS2000

An Assessment of the Ozone Loss During the 1999-2000 SOLVE Campaign

Ozone observations from ozonesondes, the DIAL and AROTEL lidars aboard the DC-8, in situ ozone measurements from the ER-2 and satellite ozone measurements from POAM were used to assess ozone loss during the SOLVE 1999-2000 campaign. We compare three different methods of computing the ozone loss. The first method simply compares the time sequence of ozonesondes taken at the same station inside the vortex from December through the end of March. In the second method, ozonesondes from a variety of stations are compared using a variant on the Match technique. This method uses short (approx. 5-10 day) forward diabatic trajectories to connect various sonde launches. In the third method, the measurements are simply injected into a diabatic trajectory model and carried forward in time from December 1 to March 16. Over 60,000 individual measurements were used in the last calculation. Again, ozone loss is estimated by comparing vortex interior measurements made early in the campaign with those made later in the campaign. The diabatic nature of the second and third methods calculation presumably corrects for the normal increase in ozone within the vortex due to downward advection. The three methods agree that the largest ozone loss occurs between 400 and 460 K potential temperatures (approx. 16-20 km) with slightly over 1.5 ppmv lost over the winter period. Between 460 K and 500 K (approx. 22 km) net ozone loss is less than 0.8 ppmv. From 500K to 600K (26 km) net loss is less than 0.5 ppmv.

Schoeberl, M. R.↗
NASA NTRS2001

Airborne Sun photometry and Closure Studies in SAFARI-2000 Dry Season Campaign

From August 13 to September 25, the Southern African Regional Science Initiative's (SAFARI 2000) dry-season airborne campaign studied the complex interactions between the region's ecosystems, air pollution, atmospheric circulation, land-atmosphere interactions, and land use change. The field campaign was timed to coincide with the annual winter fire season in Southern Africa. This challenging campaign. which coordinated ground-based measurement teams, multiple research aircraft, and satellite overpasses across nine African nations, was head quartered at the Petersburg International Airport in South Africa's Northern Province. Among many others, unique coordinated observations were made of the evolution of massive, thick haze layers produced by industrial emissions, biomass burning, marine and biogenic sources. The NASA Ames Airborne Tracking 14-channel Sunphotometer (AATS-14) was operated successfully aboard the University of Washington CV-580 during 24 data flights. The AATS-14 instrument measures the transmission of the direct solar beam at 14 discrete wavelengths (3501558 nm) from which we derive spectral aerosol optical depths (AOD), columnar water vapor (CWV) and columnar ozone. Flying at different altitudes over a fixed location allows derivation of layer AOD and CWV. Data taken during feasible vertical profiles allows derivation of aerosol extinction and water vapor density. In the talk, we show comparisons with ground-based AERONET sun/sky photometer results, with ground based MPL-Net lidar data, and with measurements from a lidar aboard the high flying ER-2 aircraft. We will use measurements from the Ames Solar Spectral Flux Radiometer to derive estimates of solar spectral forcing as a function of aerosol thickness. Validations of TOMS and Terra satellite aerosol and water-vapor retrievals will also be discussed.

Schmid, B.↗