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Lidar Ratios for Dust Aerosols Derived From Retrievals of CALIPSO Visible Extinction Profiles Constrained by Optical Depths from MODIS-Aqua and CALIPSO/CloudSat Ocean Surface Reflectance Measurements

CALIPSO's (Cloud Aerosol Lidar Infrared Pathfinder Satellite Observations) analysis algorithms generally require the use of tabulated values of the lidar ratio in order to retrieve aerosol extinction and optical depth from measured profiles of attenuated backscatter. However, for any given time or location, the lidar ratio for a given aerosol type can differ from the tabulated value. To gain some insight as to the extent of the variability, we here calculate the lidar ratio for dust aerosols using aerosol optical depth constraints from two sources. Daytime measurements are constrained using Level 2, Collection 5, 550-nm aerosol optical depth measurements made over the ocean by the MODIS (Moderate Resolution Imaging Spectroradiometer) on board the Aqua satellite, which flies in formation with CALIPSO. We also retrieve lidar ratios from night-time profiles constrained by aerosol column optical depths obtained by analysis of CALIPSO and CloudSat backscatter signals from the ocean surface.

Young, Stuart A.↗

Mixing of Dust and NH3 Observed Globally over Anthropogenic Dust Sources

The global distribution of dust column burden derived from MODIS Deep Blue aerosol products is compared to NH3 column burden retrieved from IASI infrared spectra. We found similarities in their spatial distributions, in particular their hot spots are often collocated over croplands and to a lesser extent pastures. Globally, we found 22% of dust burden collocated with NH3, with only 1% difference between land-use databases. This confirms the importance of anthropogenic dust from agriculture. Regionally, the Indian subcontinent has the highest amount of dust mixed with NH3 (26 %), mostly over cropland and during the pre-monsoon season. North Africa represents 50% of total dust burden but accounts for only 4% of mixed dust, which is found over croplands and pastures in Sahel and the coastal region of the Mediterranean. In order to evaluate the radiative effect of this mixing on dust optical properties, we derive the mass extinction efficiency for various mixtures of dust and NH3, using AERONET sunphotometers data. We found that for dusty days the coarse mode mass extinction efficiency decreases from 0.62 to 0.48 square meters per gram as NH3 burden increases from 0 to 40 milligrams per square meter. The fine mode extinction efficiency, ranging from 4 to 16 square mters per gram, does not appear to depend on NH3 concentration or relative humidity but rather on mineralogical composition and mixing with other aerosols. Our results imply that a significant amount of dust is already mixed with ammonium salt before its long range transport. This in turn will affect dust lifetime, and its interactions with radiation and cloud properties

dust sources↗

The Origin and Evolution of Interstellar Dust

In this lecture I will discuss the many different manifestation of interstellar dust, and current dust models that satisfy interstellar extinction, diffuse infrared emission, and interstellar abundances constraints. Dust is made predominantly in AGB stars and Type I1 supernovae, and I will present observational evidence for the presence of dust in these sources. I will then present chemical evolution models that follow the abundance of dust which is determined by the combined processes of formation, destruction by interstellar shock waves, and accretion in molecular clouds. The model will be applied to the evolution of PAHs and the evolution of dust in the high-redshift galaxy (z=6.42) JD11.

Dwek, Eli↗

Peculiar ultraviolet interstellar extinction

In connection with investigations of the physical characteristics of interstellar dust, a study of objects with peculiar extinction might provide new insights about the composition, size distribution, formation, and destruction of the particulate matter. Meyer and Savage (1981) have found that the dust toward many stars exhibits peculiar UV extinction. The present investigation is concerned with International Ultraviolet Explorer (IUE) spectrophotometric measurements for a sample of stars judged by Meyer and Savage to have highly anomalous UV extinction as inferred from the broad-band Astronomical Netherlands Satellite (ANS) data. The reported IUE measurements provide the opportunity to determine if the ANS photometry measurements of Meyer and Savage are anomalous because of peculiar extinction.

Massa, D.↗

Environmental effects of an impact-generated dust cloud - Implications for the Cretaceous-Tertiary extinctions

A model of the evolution and radiative effects of a debris cloud from a hypothesized impact event at the Cretaceous-Tertiary boundary suggests that the cloud could have reduced the amount of light at the earth's surface below that required for photosynthesis for several months and, for a somewhat shorter interval, even below that needed for many animals to see. For 6 months to 1 year, the surface would cool; the oceans could cool only a few degrees Celsius at most, but the continents might cool a maximum of 40 Kelvin. Extinctions in the ocean may have been caused primarily by the temporary cessation of photosynthesis, but those on land may have been primarily induced by a combination of lowered temperatures and reduced light.

Pollack, J. B.↗

Interstellar dust and the IUE

Understanding of the physical nature of interstellar dust, as modified by observations of extinction obtained with IUE, is considered. Properties of extinction laws along various lines of sight, with emphasis on the bump, are reviewed. Correlations of the UV and optical/near infrared extinction are discussed. Other diagnostics of interstellar dust, such as the near infrared emission bands, polarization, far infrared thermal emission, and depletions are mentioned, and theories are summarized.

Mathis, John S.↗

The ultraviolet interstellar extinction curve in the Pleiades

The wavelength dependence of ultraviolet extinction in the Pleiades dust clouds has been determined from IUE observations of HD 23512, the brightest heavily reddened member of the Pleiades cluster. There is evidence for an anomalously weak absorption bump at 2200 A, followed by an extinction rise in the far ultraviolet with an essentially normal slope. A relatively weak absorption band at 2200 A and a weak diffuse absorption band at 4430 A seem to be common characteristics of dust present in dense clouds. Evidence is presented which suggests that the extinction characteristics found for HD 23512 are typical for a class of extinction curves observed in several cases in the Galaxy and in the LMC.

Witt, A. N.↗

Single-Scattering Properties of Ellipsoidal Dust Aerosols Constrained By Measured Dust Shape Distributions

Most global aerosol models approximate dust as spherical particles, whereas most remote sensing retrieval algorithms approximate dust as spheroidal particles with a shape distribution that conflicts with measurements. These inconsistent and inaccurate shape assumptions generate biases in dust single-scattering properties. Here, we obtain dust single-scattering properties by approximating dust as triaxial ellipsoidal particles with observationally constrained shape distributions. We find that, relative to the ellipsoidal dust optics obtained here, the spherical dust optics used in most aerosol models underestimate dust single-scattering albedo, mass extinction efficiency, and asymmetry parameter for almost all dust sizes in both the shortwave and longwave spectra. We further find that the ellipsoidal dust optics are in substantially better agreement with observations of the scattering matrix and linear depolarization ratio than the spheroidal dust optics used in most retrieval algorithms. However, relative to observations, the ellipsoidal dust optics overestimate the lidar ratio by underestimating the backscattering intensity by a factor of ∼2. This occurs largely because the computational method used to simulate ellipsoidal dust optics (i.e., the improved geometric optics method) underestimates the backscattering intensity by a factor of ∼2 relative to other computational methods (e.g., the physical geometric optics method). We conclude that the ellipsoidal dust optics with observationally constrained shape distributions can help improve global aerosol models and possibly remote sensing retrieval algorithms that do not use the backscattering signal.

Dust↗

Dust in the Small Magellanic Cloud

We discuss simultaneous dust model fits to our extinction and polarization data for the Small Magellanic Cloud (SMC) using existing dust models. Dust model fits to the wavelength dependent polarization are possible for stars with small lambda(sub max). They generally imply size distributions which are narrower and have smaller average sizes compared to those in the Galaxy. The best fits for the extinction curves are obtained with a power law size distribution. The typical, monotonic SMC extinction curve can be well fit with graphite and silicate grains if a small fraction of the SMC carbon is locked up in the grains. Amorphous carbon and silicate grains also fit the data well.

Rodrigues, C. V.↗

Gamma-ray Burst Afterglows as Probes of Environment and Blastwave Physics: Absorption by Host Galaxy Gas and Dust, Circumburst Media and the Distribution of P

We use a new approach to obtain limits on the absorbing columns towards a sample of 10 Gamma-ray Bursts observed by BeppoSAX from simultaneous fits to X-ray, optical and IR data, in counts space and including the effects of metallicity. For half the afterglows the best-fitting model to the SED includes SMC-like extinction (as opposed to LMC or MW) and in one LMC-like extinction, and in no cases is there a preference for MW-like extinction. Gas-to-dust ratios generally do not match those of the 3 standard and most well-known extinction models of SMC, LMC and MW, but tend to be higher. We compare the results from this method to those of previous works using other methods. We constrain the jet models for a subsample of the bursts by constraining the cooling break position and power law spectral slopes, allowing the injected electron energy index to be measured. We derive secure values of p from our spectral fits and comparison with the temporal optical and X-ray slopes for 4 afterglows. The mean of these single value, suggesting that either external factors such as circumburst medium play a strong role or that the microphysics is not identical for each GRB. For GRB 971214 we find that the circumburst medium has a wind-like density profile and the cooling frequency appears to be moving to higher frequencies.

Starling, R. L. C.↗

Ground-Based Lidar Measurements of Aerosols During ACE-2: Instrument Description, Results, and Comparisons with Other Ground-Based and Airborne Measurements

A micro-pulse lidar system (MPL) was used to measure the vertical and horizontal distribution of aerosols during the Aerosol Characterization Experiment 2 (ACE-2) in June and July of 1997. The MPL measurements were made at the Izana observatory (IZO), a weather station located on a mountain ridge (28 deg 18 min N, 16 deg 30 min W, 2367 m asl) near the center of the island of Tenerife, Canary Islands. The MPL was used to acquire aerosol backscatter, extinction, and optical depth profiles for normal background periods and periods influenced by Saharan dust from North Africa. System tests and calibration procedures are discussed, and an analysis of aerosol optical profiles acquired during ACE-2 is presented. MPL data taken during normal IZO conditions (no dust) showed that upslope aerosols appeared during the day and dissipated at night and that the layers were mostly confined to altitudes a few hundred meters above IZO. MPL data taken during a Saharan dust episode on 17 July showed that peak aerosol extinction values were an order of magnitude greater than molecular scattering over IZO, and that the dust layers extended to 5 km asl. The value of the dust backscatter-extinction ratio was determined to be 0.027 +/- 0.007 sr(exp -1). Comparisons of the MPL data with data from other collocated instruments showed good agreement during the dust episode.

Welton, Ellsworth J.↗

Ground-Based Lidar Measurements of Aerosols During ACE-2 Instrument Description, Results, and Comparisons with Other Ground-Based and Airborne Measurements

A micro-pulse lidar system (MPL) was used to measure the vertical and horizontal distribution or aerosols during the Aerosol Characterization Experiment 2 (ACE-2) in June and July of 1997. The MPL measurements were made at the Izana observatory (IZO), a weather station located on a mountain ridge (28 deg 18'N, 16 deg 30'W, 2367 m asl) near the center of the island of Tenerife, Canary Islands. The MPL was used to acquire aerosol backscatter, extinction, and optical depth profiles for normal background periods and periods influenced by Saharan dust from North Africa. System tests and calibration procedures are discussed, and in analysis of aerosol optical profiles acquired during ACE-2 is presented. MPL data taken during normal IZO conditions (no dust) showed that upslope aerosols appeared during the day and dissipated at night and that the layers were mostly confined to altitudes a few hundred meters above IZO. MPL data taken during a Saharan dust episode on 17 July showed that peak aerosol extinction values were an order of magnitude greater than molecular scattering over IZO. and that the dust layers extended to 5 km asl. The value of the dust backscatter-extinction ratio was determined to be 0.027 + 0.007 per sr. Comparisons of the MPL data with data from other co-located instruments showed good agreement during the dust episode.

Welton, Ellsworth J.↗

Mineral Dust Cycle in the Multiscale Online Nonhydrostatic AtmospheRe CHemistry Model (Monarch) Version 2.0

We present the dust module in the Multiscale Online Non-hydrostatic AtmospheRe CHemistry model (MONARCH) version 2.0, a chemical weather prediction system that can be used for regional and global modeling at a range of resolutions. The representations of dust processes in MONARCH were upgraded with a focus on dust emission (emission parameterizations, entrainment thresholds, considerations of soil moisture and surface cover), lower boundary conditions (roughness, potential dust sources), and dust–radiation interactions. MONARCH now allows modeling of global and regional mineral dust cycles using fundamentally different paradigms, ranging from strongly simplified to physics-based parameterizations. We present a detailed description of these updates along with four global benchmark simulations, which use conceptually different dust emission parameterizations, and we evaluate the simulations against observations of dust optical depth. We determine key dust parameters, such as global annual emission/deposition flux, dust loading, dust optical depth, mass-extinction efficiency, single-scattering albedo, and direct radiative effects. For dust-particle diameters up to 20 µm, the total annual dust emission and deposition fluxes obtained with our four experiments range between about 3500 and 6000 Tg, which largely depend upon differences in the emitted size distribution. Considering ellipsoidal particle shapes and dust refractive indices that account for size-resolved mineralogy, we estimate the global total (longwave and shortwave) dust direct radiative effect (DRE) at the surface to range between about −0.90 and −0.63 W m−2 and at the top of the atmosphere between −0.20 and −0.28 W m−2. Our evaluation demonstrates that MONARCH is able to reproduce key features of the spatiotemporal variability of the global dust cycle with important and insightful differences between the different configurations.

Dust cycle↗

Near-infrared absorption spectroscopy of interstellar hydrocarbon grains

We present new 3600 - 2700/cm (2.8 - 3.7 micrometer) spectra of objects whose extinction is dominated by dust in the diffuse interstellar medium. The observations presented here augment an ongoing study of the organic component of the diffuse interstellar medium. These spectra contain a broad feature centered near 3300/cm (3.0 micrometers) and/or a feature with a more complex profile near 2950/cm (3.4 micrometers), the latter of which is attributed to saturated aliphatic hydrocarbons in interstellar grains and is the primary interest of this paper. As in our earlier work, the similarity of the absorption bands near 2950/cm (3.4 micrometers) along different lines of sight and the correlation of these features with interstellar extinction reveal that the carrier of this band lies in the dust in the diffuse interstellar medium (DISM). At least 2.5% of the cosmic carbon in the local interstellar medium and 4% toward the Galactic center is tied up in the carrier of the 2950/cm (3.4 micrometer) band. The spectral structure of the diffuse dust hydrocarbon C-H stretch absorption features is reasonably similar to UV photolyzed laboratory ice residues and is quite similar to the carbonaceous component of the Murchison meteorite. The similarity between the DISM and the meteoritic spectrum suggests that some of the interstellar material originally incorporated into the solar nebula may have survived relatively untouched in primitive solar system bodies. Comparisons of the DISM spectrum to hydrogenated amorphous carbon and quenched carbonaceous composite are also presented. The A(sub V)/tau ratio for the 2950/cm (3.4 micrometer) feature is lower toward the Galactic center than toward sources in the local solar neighborhood (approximately 150 for the Galactic center sources vs. approximately 250 for the local ISM sources). A similar trend has been observed previously for silicates in the diffuse medium by Roche & Aitken, suggesting that (1) the silicate and carbonaceous materials in the DISM may be physically correlated and (2) there is either dust compositional variation in the galaxy or galactic variation in the grain population density distribution. We also note a possible absorption feature near 3050/cm (3.28 micrometers), a wavelength position that is characteristic of polycyclic aromatic hydrocarbons (PAHs).

Pendleton, Y. J.↗

GRB 090417B and its Host Galaxy: A Step Towards an Understanding of Optically-Dark Gamma-Ray Bursts

GRB 090417B was an unusually long burst with a T(sub 90) duration of at least 2130 s and a multi-peaked light curve at energies of 15-150 keV. It was optically dark and has been convincingly associated with a bright star-forming galaxy at a redshift of 0.345 that is broadly similar to the Milky Way. This is one of the few cases where a host galaxy has been clearly identified for a dark gamma-ray burst and thus an ideal candidate for studying the origin of dark bursts. We find that the dark nature of GRB 090417B can not be explained by high redshift, incomplete observations, or unusual physics in the production of the afterglow. The Swift/XRT X-ray data are consistent with the afterglow being obscured by a dense, localized sheet of dust approximately 30-80 pc from the burst along the line of sight. Assuming the standard relativistic fireball model for the afterglow we find that the optical flux is at least 2.5 mag fainter than predicted by the X -ray flux. We are able to explain the lack of an optical afterglow, and the evolution of the X -ray spectrum, by assuming that there is a sheet of dust along the line of sight approximately 30-80 pc from the progenitor. Our results suggest that this dust sheet imparts an extinction of A(sub v)> or = 12 mag, which is sufficient to explain the missing optical flux. GRB 090417B is an example of a gamma-ray burst that is dark due to the localized dust structure in its host galaxy.

Holland, Stephen T.↗

Infrared emission from dust in the Coma cluster of galaxies

Detailed calculations of the infrared emission from collisionally heated dust in the Coma cluster are presented. The proposed model includes continuous dust injection from galaxies, grain destruction by sputtering, and transient grain heating by the hot plasma. The computed infrared fluxes are in agreement with the upper limits obtained from the IRAS. The calculations, and constraints implied by the IRAS observations, suggest that the intracluster dust in the central region of the cluster must be significantly depleted compared to interstellar abundances. The observed visual extinction can therefore not be attributed to the presence of dust in that region. Extinction due to cluster galaxies or their haloes is ruled out as well. The only alternative explanation is that the extinction is caused by dust at great distances from the cluster center.

Dwek, Eli↗

Measurements of DSD Second Moment Based on Laser Extinction

Using a technique recently developed for estimating the density of surface dust dispersed during a rocket landing, measuring the extinction of a laser passing through rain (or dust in the rocket case) yields an estimate of the 2nd moment of the particle cloud, and rainfall drop size distribution (DSD) in the terrestrial meteorological case. With the exception of disdrometers, instruments that measure rainfall make in direct measurements of the DSD. Most common of these instruments are the rainfall rate gauge measuring the 1 1/3 th moment, (when using a D(exp 2/3) dependency on terminal velocity). Instruments that scatter microwaves off of hydrometeors, such as the WSR-880, vertical wind profilers, and microwave disdrometers, measure the 6th moment of the DSD. By projecting a laser onto a target, changes in brightness of the laser spot against the target background during rain, yield a measurement of the DSD 2nd moment, using the Beer-Lambert law. In order to detect the laser attenuation within the 8-bit resolution of most camera image arrays, a minimum path length is required, depending on the intensity of the rainfall rate. For moderate to heavy rainfall, a laser path length of 100 m is sufficient to measure variations in optical extinction using a digital camera. A photo-detector could replace the camera, for automated installations. In order to spatially correlate the 2nd moment measurements to a collocated disdrometer or tipping bucket, the laser's beam path can be reflected multiple times using mirrors to restrict the spatial extent of the measurement. In cases where a disdrometer is not available, complete DSD estimates can be produced by parametric fitting of DSD model to the 2nd moment data in conjunction with tipping bucket data. In cases where a disdrometer is collocated, the laser extinction technique may yield a significant improvement to insitu disdrometer validation and calibration strategies

Lane, John E.↗

A Wavelength Optimization Study on Visible and Infrared Propagation Systems in Coastal Environments

Electro-optical (EO) systems employed for communications, surveillance and weapons systems are commonly assessed in the North American and European continents. However, the atmospheric propagation environment in these regions is often dissimilar to most other parts of the world. In particular, atmospheric dust, industrial pollution, and smoke frequently reduce visibility to less than 5 km in Asia and South America significantly hampering EO system performance. Because atmospheric aerosol species vary considerably in size and chemistry, optimal wavelengths for EO systems vary from region to region. In this paper we examine the extinction effects from aerosol particles and water vapor on a regional basis. Theoretical studies are coupled with visibility and satellite climatologies to make an assessment for the coastal regions of the world. While longer wavelengths permit higher transmission by particles in regions significantly hampered by fine mode particles (such as industrial pollution and smoke), this advantage is commonly offset by high extinction values from water vapor. This offsetting effect is particularly strong in industrial and developing countries in the tropics and sub-tropics such as Southeast Asia and South America. Conversely, the advantage of low water vapor concentrations in longer wavelengths is offset by high mass-extinction efficiencies of atmospheric dust in this portion of the spectrum.

Reid, J. S.↗